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1. First production of X-rays at the ThomX high-intensity Compton source

Author

Jacquet, M, Alexandre, P, Alkadi, M, Alves, M, Amer, M, Amoudry, L, Auguste, D, Babigeon, J, Balcou, P, Baltazar, M, Benabderrahmane, C, el Fekih, R, Benoit, A, Berteaud, P, Biagini, M, Blin, A, Bobault, S, Bonanzingamarco, M, Bonenfant, J, Bonis, J, Bouanani, Y, Bouaziz, S, Bouvet, F, Bravin, A, Bruni, C, Bruyere, C, Bzyl, H, Cassinari, L, Cassou, K, Cayla, J, Chabaud, T, Chaikovska, I, Chance, S, Chapelle, C, Chaumat, V, Chiche, R, Cobessi, A, Cormier, E, Cornebise, P, Couprie, M, Cuoq, R, Dalifard, O, Degallaix, J, Delerue, N, Del Net, W, Diaz, A, Dietrich, Y, Diop, M, Dorkel, R, Douillet, D, Drebot, I, Dugal, J, Dupraz, K, Dupuy, E, El Ajjouri, M, El Kamchi, N, El Khaldi, M, Elleaume, H, Ergenlik, E, Estève, F, Favier, P, Fernandez, M, Gamelin, A, Garaut, J, Garolfi, L, Gauron, P, Gauthier, F, Girault, P, Gonnin, A, Grasset, D, Guerard, E, Guler, H, Haissinski, J, Hazemann, J, Helder, D, Herbeaux, C, Herry, E, Hodeau, J, Horodynski, J, Hubert, N, Iaquaniello, G, Jacquet, P, Jeantet, P, Jehanno, D, Jules, E, Kapoujyan, G, Kubytskyi, V, Labat, M, Labaye, F, Lacipière, J, Lacroix, M, Lahéra, E, Langlet, M, Lebarillec, T, Ledu, J, Le Duc, G, Le Guidec, D, Leluan, B, Lepercq, P, Lestrade, A, Jacquet M., Alexandre P., Alkadi M., Alves M., Amer M., Amoudry L., Auguste D., Babigeon J. L., Balcou P., Baltazar M., Benabderrahmane C., el Fekih R. B., Benoit A., Berteaud P., Biagini M., Blin A., Bobault S., Bonanzingamarco M., Bonenfant J., Bonis J., Bouanani Y., Bouaziz S., Bouvet F., Bravin A., Bruni C., Bruyere C., Bzyl H., Cassinari L., Cassou K., Cayla J. N., Chabaud T., Chaikovska I., Chance S., Chapelle C., Chaumat V., Chiche R., Cobessi A., Cormier E., Cornebise P., Couprie M. E., Cuoq R., Dalifard O., Degallaix J., Delerue N., Del Net W., Diaz A., Dietrich Y., Diop M., Dorkel R., Douillet D., Drebot I., Dugal J. P., Dupraz K., Dupuy E., El Ajjouri M., El Kamchi N., El Khaldi M., Elleaume H., Ergenlik E., Estève F., Favier P., Fernandez M., Gamelin A., Garaut J. F., Garolfi L., Gauron P., Gauthier F., Girault P., Gonnin A., Grasset D., Guerard E., Guler H., Haissinski J., Hazemann J. L., Helder D., Herbeaux C., Herry E., Hodeau J. L., Horodynski J. M., Hubert N., Iaquaniello G., Jacquet P., Jeantet P., Jehanno D., Jules E., Kapoujyan G., Kubytskyi V., Labat M., Labaye F., Lacipière J., Lacroix M., Lahéra E., Langlet M., Lebarillec T., Ledu J. F., Le Duc G., Le Guidec D., Leluan B., Lepercq P., Lestrade A., Jacquet, M, Alexandre, P, Alkadi, M, Alves, M, Amer, M, Amoudry, L, Auguste, D, Babigeon, J, Balcou, P, Baltazar, M, Benabderrahmane, C, el Fekih, R, Benoit, A, Berteaud, P, Biagini, M, Blin, A, Bobault, S, Bonanzingamarco, M, Bonenfant, J, Bonis, J, Bouanani, Y, Bouaziz, S, Bouvet, F, Bravin, A, Bruni, C, Bruyere, C, Bzyl, H, Cassinari, L, Cassou, K, Cayla, J, Chabaud, T, Chaikovska, I, Chance, S, Chapelle, C, Chaumat, V, Chiche, R, Cobessi, A, Cormier, E, Cornebise, P, Couprie, M, Cuoq, R, Dalifard, O, Degallaix, J, Delerue, N, Del Net, W, Diaz, A, Dietrich, Y, Diop, M, Dorkel, R, Douillet, D, Drebot, I, Dugal, J, Dupraz, K, Dupuy, E, El Ajjouri, M, El Kamchi, N, El Khaldi, M, Elleaume, H, Ergenlik, E, Estève, F, Favier, P, Fernandez, M, Gamelin, A, Garaut, J, Garolfi, L, Gauron, P, Gauthier, F, Girault, P, Gonnin, A, Grasset, D, Guerard, E, Guler, H, Haissinski, J, Hazemann, J, Helder, D, Herbeaux, C, Herry, E, Hodeau, J, Horodynski, J, Hubert, N, Iaquaniello, G, Jacquet, P, Jeantet, P, Jehanno, D, Jules, E, Kapoujyan, G, Kubytskyi, V, Labat, M, Labaye, F, Lacipière, J, Lacroix, M, Lahéra, E, Langlet, M, Lebarillec, T, Ledu, J, Le Duc, G, Le Guidec, D, Leluan, B, Lepercq, P, Lestrade, A, Jacquet M., Alexandre P., Alkadi M., Alves M., Amer M., Amoudry L., Auguste D., Babigeon J. L., Balcou P., Baltazar M., Benabderrahmane C., el Fekih R. B., Benoit A., Berteaud P., Biagini M., Blin A., Bobault S., Bonanzingamarco M., Bonenfant J., Bonis J., Bouanani Y., Bouaziz S., Bouvet F., Bravin A., Bruni C., Bruyere C., Bzyl H., Cassinari L., Cassou K., Cayla J. N., Chabaud T., Chaikovska I., Chance S., Chapelle C., Chaumat V., Chiche R., Cobessi A., Cormier E., Cornebise P., Couprie M. E., Cuoq R., Dalifard O., Degallaix J., Delerue N., Del Net W., Diaz A., Dietrich Y., Diop M., Dorkel R., Douillet D., Drebot I., Dugal J. P., Dupraz K., Dupuy E., El Ajjouri M., El Kamchi N., El Khaldi M., Elleaume H., Ergenlik E., Estève F., Favier P., Fernandez M., Gamelin A., Garaut J. F., Garolfi L., Gauron P., Gauthier F., Girault P., Gonnin A., Grasset D., Guerard E., Guler H., Haissinski J., Hazemann J. L., Helder D., Herbeaux C., Herry E., Hodeau J. L., Horodynski J. M., Hubert N., Iaquaniello G., Jacquet P., Jeantet P., Jehanno D., Jules E., Kapoujyan G., Kubytskyi V., Labat M., Labaye F., Lacipière J., Lacroix M., Lahéra E., Langlet M., Lebarillec T., Ledu J. F., Le Duc G., Le Guidec D., Leluan B., Lepercq P., and Lestrade A.

Abstract

With the increase in laser power and finesse of optical cavities over the last decade, laboratory-size Compton sources are very promising. These sources produce X-rays through interactions between relativistic electrons and laser photons and, in term of brightness, fall between large synchrotron facilities and classical laboratory X-ray sources. The ThomX source is the French project in this field. This article first presents a state of the art of high-intensity Compton sources, then the ThomX source is briefly described, and the first results are detailed, in particular the production of the first X-rays, the acquisition of the first spectrum and the first image of the beam. Finally, the next objectives are discussed.

Published
2024

2. The ThomX ICS source

Author

Dupraz, K, Alkadi, M, Alves, M, Amoudry, L, Auguste, D, Babigeon, J, Baltazar, M, Benoit, A, Bonis, J, Bonenfant, J, Bruni, C, Cassou, K, Cayla, J, Chabaud, T, Chaikovska, I, Chance, S, Chaumat, V, Chiche, R, Cobessi, A, Cornebise, P, Dalifard, O, Delerue, N, Dorkel, R, Douillet, D, Dugal, J, El Kamchi, N, El Khaldi, M, Ergenlik, E, Favier, P, Fernandez, M, Gamelin, A, Garaut, J, Garolfi, L, Gauron, P, Gauthier, F, Gonnin, A, Grasset, D, Guerard, E, Guler, H, Haissinski, J, Herry, E, Iaquaniello, G, Jacquet, M, Jules, E, Kubytskyi, V, Langlet, M, Le Barillec, T, Ledu, J, Leguidec, D, Leluan, B, Lepercq, P, Letellier-Cohen, F, Marie, R, Marrucho, J, Martens, A, Mageur, C, Mercadier, G, Mercier, B, Mistretta, E, Monard, H, Moutardier, A, Neveu, O, Nutarelli, D, Omeich, M, Peinaud, Y, Petrilli, Y, Pichet, M, Plaige, E, Prevost, C, Rudnicky, P, Soskov, V, Taurigna-Quere, M, Trochet, S, Vallerand, C, Vitez, O, Wicek, F, Wurth, S, Zomer, F, Alexandre, P, Ben El Fekih, R, Berteaud, P, Bouvet, F, Cuoq, R, Diaz, A, Dietrich, Y, Diop, M, Pedeau, D, Dupuy, E, Marteau, F, Helder, D, Hubert, N, Veteran, J, Labat, M, Lestrade, A, Letresor, A, Lopes, R, Loulergue, A, Louvet, M, Marchand, P, El Ajjouri, M, Muller, D, Nadji, A, Nadolski, L, Nagaoka, R, Petit, S, Pollina, J, Ribeiro, F, Ros, M, Salvia, J, Bobault, S, Sebdaoui, M, Sreedharan, R, Bouanai, Y, Hazemann, J, Hodeau, J, Roy, E, Jeantet, P, Lacipiere, J, Robert, P, Horodynski, J, Bzyl, H, Chapelle, C, Biagini, M, Walter, P, Bravin, A, Del Net, W, Lahera, E, Proux, O, Elleaume, H, Cormier, E, Dupraz K., Alkadi M., Alves M., Amoudry L., Auguste D., Babigeon J. -L., Baltazar M., Benoit A., Bonis J., Bonenfant J., Bruni C., Cassou K., Cayla J. -N., Chabaud T., Chaikovska I., Chance S., Chaumat V., Chiche R., Cobessi A., Cornebise P., Dalifard O., Delerue N., Dorkel R., Douillet D., Dugal J. -P., El Kamchi N., El Khaldi M., Ergenlik E., Favier P., Fernandez M., Gamelin A., Garaut J. -F., Garolfi L., Gauron P., Gauthier F., Gonnin A., Grasset D., Guerard E., Guler H., Haissinski J., Herry E., Iaquaniello G., Jacquet M., Jules E., Kubytskyi V., Langlet M., Le Barillec T., Ledu J. -F., Leguidec D., Leluan B., Lepercq P., Letellier-Cohen F., Marie R., Marrucho J. -C., Martens A., Mageur C., Mercadier G., Mercier B., Mistretta E., Monard H., Moutardier A., Neveu O., Nutarelli D., Omeich M., Peinaud Y., Petrilli Y., Pichet M., Plaige E., Prevost C., Rudnicky P., Soskov V., Taurigna-Quere M., Trochet S., Vallerand C., Vitez O., Wicek F., Wurth S., Zomer F., Alexandre P., Ben El Fekih R., Berteaud P., Bouvet F., Cuoq R., Diaz A., Dietrich Y., Diop M., Pedeau D., Dupuy E., Marteau F., Helder D., Hubert N., Veteran J., Labat M., Lestrade A., Letresor A., Lopes R., Loulergue A., Louvet M., Marchand P., El Ajjouri M., Muller D., Nadji A., Nadolski L., Nagaoka R., Petit S., Pollina J. -P., Ribeiro F., Ros M., Salvia J., Bobault S., Sebdaoui M., Sreedharan R., Bouanai Y., Hazemann J. -L., Hodeau J. -L., Roy E., Jeantet P., Lacipiere J., Robert P., Horodynski J. -M., Bzyl H., Chapelle C., Biagini M., Walter P., Bravin A., Del Net W., Lahera E., Proux O., Elleaume H., Cormier E., Dupraz, K, Alkadi, M, Alves, M, Amoudry, L, Auguste, D, Babigeon, J, Baltazar, M, Benoit, A, Bonis, J, Bonenfant, J, Bruni, C, Cassou, K, Cayla, J, Chabaud, T, Chaikovska, I, Chance, S, Chaumat, V, Chiche, R, Cobessi, A, Cornebise, P, Dalifard, O, Delerue, N, Dorkel, R, Douillet, D, Dugal, J, El Kamchi, N, El Khaldi, M, Ergenlik, E, Favier, P, Fernandez, M, Gamelin, A, Garaut, J, Garolfi, L, Gauron, P, Gauthier, F, Gonnin, A, Grasset, D, Guerard, E, Guler, H, Haissinski, J, Herry, E, Iaquaniello, G, Jacquet, M, Jules, E, Kubytskyi, V, Langlet, M, Le Barillec, T, Ledu, J, Leguidec, D, Leluan, B, Lepercq, P, Letellier-Cohen, F, Marie, R, Marrucho, J, Martens, A, Mageur, C, Mercadier, G, Mercier, B, Mistretta, E, Monard, H, Moutardier, A, Neveu, O, Nutarelli, D, Omeich, M, Peinaud, Y, Petrilli, Y, Pichet, M, Plaige, E, Prevost, C, Rudnicky, P, Soskov, V, Taurigna-Quere, M, Trochet, S, Vallerand, C, Vitez, O, Wicek, F, Wurth, S, Zomer, F, Alexandre, P, Ben El Fekih, R, Berteaud, P, Bouvet, F, Cuoq, R, Diaz, A, Dietrich, Y, Diop, M, Pedeau, D, Dupuy, E, Marteau, F, Helder, D, Hubert, N, Veteran, J, Labat, M, Lestrade, A, Letresor, A, Lopes, R, Loulergue, A, Louvet, M, Marchand, P, El Ajjouri, M, Muller, D, Nadji, A, Nadolski, L, Nagaoka, R, Petit, S, Pollina, J, Ribeiro, F, Ros, M, Salvia, J, Bobault, S, Sebdaoui, M, Sreedharan, R, Bouanai, Y, Hazemann, J, Hodeau, J, Roy, E, Jeantet, P, Lacipiere, J, Robert, P, Horodynski, J, Bzyl, H, Chapelle, C, Biagini, M, Walter, P, Bravin, A, Del Net, W, Lahera, E, Proux, O, Elleaume, H, Cormier, E, Dupraz K., Alkadi M., Alves M., Amoudry L., Auguste D., Babigeon J. -L., Baltazar M., Benoit A., Bonis J., Bonenfant J., Bruni C., Cassou K., Cayla J. -N., Chabaud T., Chaikovska I., Chance S., Chaumat V., Chiche R., Cobessi A., Cornebise P., Dalifard O., Delerue N., Dorkel R., Douillet D., Dugal J. -P., El Kamchi N., El Khaldi M., Ergenlik E., Favier P., Fernandez M., Gamelin A., Garaut J. -F., Garolfi L., Gauron P., Gauthier F., Gonnin A., Grasset D., Guerard E., Guler H., Haissinski J., Herry E., Iaquaniello G., Jacquet M., Jules E., Kubytskyi V., Langlet M., Le Barillec T., Ledu J. -F., Leguidec D., Leluan B., Lepercq P., Letellier-Cohen F., Marie R., Marrucho J. -C., Martens A., Mageur C., Mercadier G., Mercier B., Mistretta E., Monard H., Moutardier A., Neveu O., Nutarelli D., Omeich M., Peinaud Y., Petrilli Y., Pichet M., Plaige E., Prevost C., Rudnicky P., Soskov V., Taurigna-Quere M., Trochet S., Vallerand C., Vitez O., Wicek F., Wurth S., Zomer F., Alexandre P., Ben El Fekih R., Berteaud P., Bouvet F., Cuoq R., Diaz A., Dietrich Y., Diop M., Pedeau D., Dupuy E., Marteau F., Helder D., Hubert N., Veteran J., Labat M., Lestrade A., Letresor A., Lopes R., Loulergue A., Louvet M., Marchand P., El Ajjouri M., Muller D., Nadji A., Nadolski L., Nagaoka R., Petit S., Pollina J. -P., Ribeiro F., Ros M., Salvia J., Bobault S., Sebdaoui M., Sreedharan R., Bouanai Y., Hazemann J. -L., Hodeau J. -L., Roy E., Jeantet P., Lacipiere J., Robert P., Horodynski J. -M., Bzyl H., Chapelle C., Biagini M., Walter P., Bravin A., Del Net W., Lahera E., Proux O., Elleaume H., and Cormier E.

Abstract

ThomX is a new generation Compact Compton Source. It is currently commissioned by and at the IJCLab (Laboratoire de physique des 2 infinis - Irène Joliot-Curie (UMR9012)) at Orsay. The first beam is expected at the begining of 2021. The aim of ThomX is to demonstrate the characteristics of an intense and Compact (lab-size) X-ray source based on Compton Scattering. The performances are mostly driven by the laser optical system which is above the state of the art of stored laser power. Proof of principle of various X-ray techniques will be performed thanks to the versatile ThomX beamline. Firstly, this article presents the machine description. Secondly, the issues and limits of the laser system are discussed. Then, the ThomX beamline is described and the machine status conclude the ThomX presentation. Finally, the expected performances for the next years and the possible experiments that can be made with this new machine are detailed.

Published
2020

3. The ThomX project status

Author

Alessandro Variola, Auguste, D., Blin, A., Bonis, J., Bouaziz, S., Bruni, C., Cassou, K., Chaikovska, I., Chancé, S., Chaumat, V., Chiche, R., Cornebise, P., Dalifard, O., Delerue, N., Demma, T., Drebot, I., Dupraz, K., El Khaldi, M., El Khamci, N., Gauron, P., Gonnin, A., Guerard, E., Haissinski, J., Jacquet, M., Jehanno, D., Jouvin, M., Jules, E., Labaye, F., Lacroix, M., Langlet, M., Le Guidec, D., Letellier, F., Lepercq, P., Marie, R., Marrucho, J. C., Martens, A., Mistretta, E., Mercier, B., Monard, H., Peinaud, Y., Perus, A., Pieyre, B., Plaige, E., Prevost, C., Roulet, T., Roux, R., Soskov, V., Stocchi, A., Vallerand, C., Vermes, A., Wicek, F., Yan, Y., Zhang, J., Zomer, F., El Ajjouri, M., Alexandre, P., Benabderrahmane, C., Bouvet, F., Couprie, M. E., Cassinari, L., Dietrich, Y., Deblay, P., Diop, M., Gacoin, M. P., Herbeaux, C., Hubert, N., Labat, M., Lebasque, P., Lestrade, A., Lopes, R., Loulergue, A., Marchand, P., Marteau, F., Muller, D., Nadji, A., Nagaoka, R., Pollina, J. P., Ribeiro, F., Ros, M., Sreedharan, R., Bruyère, C., Cobessi, A., Del-Net, W., Hazemann, J. L., Hodeau, J. L., Jeantet, P., Lacipière, J., Proux, O., Cormier, E., Lhermite, J., Bravin, A., Le Duc, G., Susini, J., Viguerie, L., Rousselière, H., Walter, P., Elleaume, H., Esteve, F., Horodinsky, J. M., Pawels, N., Robert, P., Sierra, S., ThomX - Dept. Accelerateurs, Laboratoire de l'Accélérateur Linéaire (LAL), Centre National de la Recherche Scientifique (CNRS)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Sud - Paris 11 (UP11)-Centre National de la Recherche Scientifique (CNRS)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Sud - Paris 11 (UP11), Centre National de la Recherche Scientifique (CNRS)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Sud - Paris 11 (UP11), Synchrotron SOLEIL (SSOLEIL), Centre National de la Recherche Scientifique (CNRS), SERAS (SERAS), Institut Néel (NEEL), Université Joseph Fourier - Grenoble 1 (UJF)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Centre National de la Recherche Scientifique (CNRS)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Centre National de la Recherche Scientifique (CNRS), Matériaux, Rayonnements, Structure (MRS), Centre d'Etudes Lasers Intenses et Applications (CELIA), Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Bordeaux (UB), European Synchrotron Radiation Facility (ESRF), Grenoble Institut des Neurosciences (GIN), Université Joseph Fourier - Grenoble 1 (UJF)-Institut National de la Santé et de la Recherche Médicale (INSERM), Christine Petit-Jean-Genaz, Gianluigi Arduini, Peter Michel, Volker RW Schaa, Université Paris-Sud - Paris 11 (UP11)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS)-Université Paris-Sud - Paris 11 (UP11)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS), Université Paris-Sud - Paris 11 (UP11)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS), Service Etudes et Réalisation d'Appareillages Scientifiques (NEEL - SERAS), Matériaux, Rayonnements, Structure (NEEL - MRS), Université de Bordeaux (UB)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Centre National de la Recherche Scientifique (CNRS), [GIN] Grenoble Institut des Neurosciences (GIN), and Starita, Sabine

Subjects
ThomX, [PHYS.PHYS.PHYS-ACC-PH]Physics [physics]/Physics [physics]/Accelerator Physics [physics.acc-ph], [PHYS.PHYS.PHYS-ACC-PH] Physics [physics]/Physics [physics]/Accelerator Physics [physics.acc-ph]
Abstract

Work supported by the French Agence Nationale de la recherche as part of the program EQUIPEX under reference ANR-10-EQPX-51, the Ile de France region, CNRS-IN2P3 and Université Paris Sud XI - http://accelconf.web.cern.ch/AccelConf/IPAC2014/papers/wepro052.pdf; A collaboration of seven research institutes and an industry has been set up for the ThomX project, a compact Compton Backscattering Source (CBS) based in Orsay - France. After a period of study and definition of the machine performance, a full description of all the systems has been provided. The infrastructure work has been started and the main systems are in the call for tender phase. In this paper we will illustrate the definitive machine parameters and components characteristics. We will also update the results of the different technical and experimental activities on optical resonators, RF power supplies and on the electron gun.

4. The ThomX ICS source

Author

Kevin Dupraz, Muath Alkadi, Manuel Alves, Loic Amoudry, Didier Auguste, Jean-Luc Babigeon, Michel Baltazar, Alain Benoit, Julien Bonis, Jean Bonenfant, Christelle Bruni, Kevin Cassou, Jean-Noël Cayla, Thomas Chabaud, Iryna Chaikovska, Sophie Chance, Vincent Chaumat, Ronic Chiche, Alain Cobessi, Patrick Cornebise, Olivier Dalifard, Nicolas Delerue, Remy Dorkel, Denis Douillet, Jean-Phillipe Dugal, Noureddine El Kamchi, Mohamed El Khaldi, Ezgi Ergenlik, Pierre Favier, Marco Fernandez, Alexis Gamelin, Jean-Francois Garaut, Luca Garolfi, Philippe Gauron, Frédéric Gauthier, Alexandre Gonnin, Denis Grasset, Eric Guerard, Hayg Guler, Jacques Haissinski, Emmanuel Herry, Gregory Iaquaniello, Marie Jacquet, Eric Jules, Vlacheslav Kubytskyi, Marc Langlet, Titouan Le Barillec, Jean-François Ledu, Damien Leguidec, Bruno Leluan, Pierre Lepercq, Frédéric Letellier-Cohen, Rodolphe Marie, Jean-Claude Marrucho, Aurélien Martens, Christophe Mageur, Gabriel Mercadier, Bruno Mercier, Eric Mistretta, Hugues Monard, Alexandre Moutardier, Olivier Neveu, Daniele Nutarelli, Maher Omeich, Yann Peinaud, Yann Petrilli, Marc Pichet, Eric Plaige, Christophe Prévost, Philippe Rudnicky, Viktor Soskov, Monique Taurigna-Quéré, Stéphane Trochet, Cynthia Vallerand, Olivier Vitez, François Wicek, Sébastien Wurth, Fabian Zomer, Patrick Alexandre, Rachid Ben El Fekih, Philippe Berteaud, François Bouvet, Renaud Cuoq, Antonio Diaz, Yannick Dietrich, Massamba Diop, Dominique Pedeau, Eric Dupuy, Fabrice Marteau, Dias Helder, Nicolas Hubert, José Veteran, Marie Labat, Alain Lestrade, Antoine Letrésor, Robert Lopes, Alexandre Loulergue, Marc Louvet, Patrick Marchand, Moussa El Ajjouri, Didier Muller, Amor Nadji, Laurent Nadolski, Ryutaro Nagaoka, Sylvain Petit, Jean-Pierre Pollina, Fernand Ribeiro, Manuel Ros, Julien Salvia, Sébastien Bobault, Mourad Sebdaoui, Rajesh Sreedharan, Yazid Bouanai, Jean-Louis Hazemann, Jean-Louis Hodeau, Emmanuel Roy, Philippe Jeantet, Jérôme Lacipière, Pierre Robert, Jean-Michel Horodynski, Harold Bzyl, Christophe Chapelle, Marica Biagini, Philippe Walter, Alberto Bravin, William Del Net, Eric Lahéra, Olivier Proux, Hélène Elleaume, Eric Cormier, Laboratoire de Physique des 2 Infinis Irène Joliot-Curie (IJCLab), Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), Synchrotron SOLEIL (SSOLEIL), Centre National de la Recherche Scientifique (CNRS), Laboratoire de l'Accélérateur Linéaire (LAL), Centre National de la Recherche Scientifique (CNRS)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Sud - Paris 11 (UP11), Matériaux, Rayonnements, Structure (MRS), Institut Néel (NEEL), Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP ), Université Grenoble Alpes (UGA)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP ), Université Grenoble Alpes (UGA), SERAS (SERAS), Ingénierie Radioprotection Sûreté Démantèlement (IRSD), Laboratori Nazionali di Frascati (LNF), Istituto Nazionale di Fisica Nucleare (INFN), Laboratoire d'Archéologie Moléculaire et Structurale (LAMS), Institut de Chimie du CNRS (INC)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS), European Synchrotron Radiation Facility (ESRF), Observatoire des Sciences de l'Univers de Grenoble (OSUG ), Institut national des sciences de l'Univers (INSU - CNRS)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Institut National de Recherche pour l’Agriculture, l’Alimentation et l’Environnement (INRAE)-Université Grenoble Alpes (UGA), Rayonnement Synchrotron et Recherche Medicale (RSRM), European Synchrotron Radiation Facility (ESRF)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut National de la Santé et de la Recherche Médicale (INSERM), Institut Universitaire de France (IUF), Ministère de l'Education nationale, de l’Enseignement supérieur et de la Recherche (M.E.N.E.S.R.), LETELLIER, Frédéric, Université Paris-Sud - Paris 11 (UP11)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS), Matériaux, Rayonnements, Structure (NEEL - MRS), Service Etudes et Réalisation d'Appareillages Scientifiques (NEEL - SERAS), Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut de Chimie du CNRS (INC)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS), Institut national des sciences de l'Univers (INSU - CNRS)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Institut National de Recherche pour l’Agriculture, l’Alimentation et l’Environnement (INRAE)-Université Grenoble Alpes (UGA)-Météo-France, Dupraz, K, Alkadi, M, Alves, M, Amoudry, L, Auguste, D, Babigeon, J, Baltazar, M, Benoit, A, Bonis, J, Bonenfant, J, Bruni, C, Cassou, K, Cayla, J, Chabaud, T, Chaikovska, I, Chance, S, Chaumat, V, Chiche, R, Cobessi, A, Cornebise, P, Dalifard, O, Delerue, N, Dorkel, R, Douillet, D, Dugal, J, El Kamchi, N, El Khaldi, M, Ergenlik, E, Favier, P, Fernandez, M, Gamelin, A, Garaut, J, Garolfi, L, Gauron, P, Gauthier, F, Gonnin, A, Grasset, D, Guerard, E, Guler, H, Haissinski, J, Herry, E, Iaquaniello, G, Jacquet, M, Jules, E, Kubytskyi, V, Langlet, M, Le Barillec, T, Ledu, J, Leguidec, D, Leluan, B, Lepercq, P, Letellier-Cohen, F, Marie, R, Marrucho, J, Martens, A, Mageur, C, Mercadier, G, Mercier, B, Mistretta, E, Monard, H, Moutardier, A, Neveu, O, Nutarelli, D, Omeich, M, Peinaud, Y, Petrilli, Y, Pichet, M, Plaige, E, Prevost, C, Rudnicky, P, Soskov, V, Taurigna-Quere, M, Trochet, S, Vallerand, C, Vitez, O, Wicek, F, Wurth, S, Zomer, F, Alexandre, P, Ben El Fekih, R, Berteaud, P, Bouvet, F, Cuoq, R, Diaz, A, Dietrich, Y, Diop, M, Pedeau, D, Dupuy, E, Marteau, F, Helder, D, Hubert, N, Veteran, J, Labat, M, Lestrade, A, Letresor, A, Lopes, R, Loulergue, A, Louvet, M, Marchand, P, El Ajjouri, M, Muller, D, Nadji, A, Nadolski, L, Nagaoka, R, Petit, S, Pollina, J, Ribeiro, F, Ros, M, Salvia, J, Bobault, S, Sebdaoui, M, Sreedharan, R, Bouanai, Y, Hazemann, J, Hodeau, J, Roy, E, Jeantet, P, Lacipiere, J, Robert, P, Horodynski, J, Bzyl, H, Chapelle, C, Biagini, M, Walter, P, Bravin, A, Del Net, W, Lahera, E, Proux, O, Elleaume, H, and Cormier, E

Subjects
Beamline, ThomX, [PHYS.PHYS.PHYS-ACC-PH]Physics [physics]/Physics [physics]/Accelerator Physics [physics.acc-ph], General Physics and Astronomy, 01 natural sciences, law.invention, 010309 optics, X-ray, Optics, law, 0103 physical sciences, Laser power scaling, Physics, Machine description, 010308 nuclear & particles physics, business.industry, Compton scattering, [PHYS.PHYS.PHYS-ACC-PH] Physics [physics]/Physics [physics]/Accelerator Physics [physics.acc-ph], Laser, High power Fabry-Perot cavity, lcsh:QC1-999, Proof of concept, Compact compton source, business, Beam (structure), lcsh:Physics
Abstract

International audience; ThomX is a new generation Compact Compton Source. It is currently commissioned by and at the IJCLab (Laboratoire de physique des 2 infinis - Irène Joliot-Curie (UMR9012)) at Orsay. The first beam is expected at the begining of 2021. The aim of ThomX is to demonstrate the characteristics of an intense and Compact (lab-size) X-ray source based on Compton Scattering. The performances are mostly driven by the laser optical system which is above the state of the art of stored laser power. Proof of principle of various X-ray techniques will be performed thanks to the versatile ThomX beamline. Firstly, this article presents the machine description. Secondly, the issues and limits of the laser system are discussed. Then, the ThomX beamline is described and the machine status conclude the ThomX presentation. Finally, the expected performances for the next years and the possible experiments that can be made with this new machine are detailed.

Published
2020
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5. High-Energy Resolution Fluorescence Detected X-Ray Absorption Spectroscopy: A Powerful New Structural Tool in Environmental Biogeochemistry Sciences.

Author

Proux O, Lahera E, Del Net W, Kieffer I, Rovezzi M, Testemale D, Irar M, Thomas S, Aguilar-Tapia A, Bazarkina EF, Prat A, Tella M, Auffan M, Rose J, and Hazemann JL

Subjects
Ecology, Environmental Monitoring, X-Ray Absorption Spectroscopy
Abstract

The study of the speciation of highly diluted elements by X-ray absorption spectroscopy (XAS) is extremely challenging, especially in environmental biogeochemistry sciences. Here we present an innovative synchrotron spectroscopy technique: high-energy resolution fluorescence detected XAS (HERFD-XAS). With this approach, measurement of the XAS signal in fluorescence mode using a crystal analyzer spectrometer with a ∼1-eV energy resolution helps to overcome restrictions on sample concentrations that can be typically measured with a solid-state detector. We briefly describe the method, from both an instrumental and spectroscopic point of view, and emphasize the effects of energy resolution on the XAS measurements. We then illustrate the positive impact of this technique in terms of detection limit with two examples dealing with Ce in ecologically relevant organisms and with Hg species in natural environments. The sharp and well-marked features of the HERFD-X-ray absorption near-edge structure spectra obtained enable us to determine unambiguously and with greater precision the speciation of the probed elements. This is a major technological advance, with strong benefits for the study of highly diluted elements using XAS. It also opens new possibilities to explore the speciation of a target chemical element at natural concentration levels, which is critical in the fields of environmental and biogeochemistry sciences., (Copyright © by the American Society of Agronomy, Crop Science Society of America, and Soil Science Society of America, Inc.)

Published
2017
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6. Determination of the local structure of CsBi 4-x Pb x Te 6 (x = 0, 0.5) by X-ray absorption spectroscopy.

Author

Wakita T, Paris E, Mizokawa T, Hacisalihoglu MY, Terashima K, Okazaki H, Proux O, Kieffer I, Lahera E, Del Net W, Olivi L, Takano Y, Muraoka Y, Yokoya T, and Saini NL

Abstract

We have studied the local structure and valence electronic unoccupied states of thermoelectric CsBi 4 Te 6 and superconducting CsBi 3.5 Pb 0.5 Te 6 (T c ∼ 3 K) by extended X-ray absorption fine structure (EXAFS) and X-ray absorption near edge structure (XANES) measurements. The Bi-L 3 edge EXAFS reveals wide Bi-Te distance distribution for both compounds indicating complex atomic arrangements in the studied system. The mean square relative displacements (MSRDs) of the Bi-Te bond distances appear largely increased in Pb substituted system due to larger overall local disorder, however, one of the Bi-Te bonds shows a reduced disorder. On the other hand, the Bi-L 3 edge XANES is hardly affected by Pb substitution while the Te-L 1 edge XANES reveals increased density of unoccupied Te 5p states. This suggests that the carriers introduced by the Pb substitution in CsBi 4-x Pb x Te 6 preferentially goes on Te sites. Similarly, the Cs-L 3 edge XANES also shows small changes due to Pb-substitution and reduced local disorder indicated by the reduced width of the Cs-L 3 edge white line. We have also shown that the X-ray photoemission spectroscopy (XPS) measurements on various electronic core levels are in a qualitative agreement with the XANES results. These findings are consistent with carrier doping and a reduced disorder in one direction to be likely factors to drive the thermoelectric CsBi 4 Te 6 into a bulk superconductor by Pb-substitution in CsBi 4-x Pb x Te 6 .

Published
2016
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7. Sulfur radical species form gold deposits on Earth.

Author

Pokrovski GS, Kokh MA, Guillaume D, Borisova AY, Gisquet P, Hazemann JL, Lahera E, Del Net W, Proux O, Testemale D, Haigis V, Jonchière R, Seitsonen AP, Ferlat G, Vuilleumier R, Saitta AM, Boiron MC, and Dubessy J

Abstract

Current models of the formation and distribution of gold deposits on Earth are based on the long-standing paradigm that hydrogen sulfide and chloride are the ligands responsible for gold mobilization and precipitation by fluids across the lithosphere. Here we challenge this view by demonstrating, using in situ X-ray absorption spectroscopy and solubility measurements, coupled with molecular dynamics and thermodynamic simulations, that sulfur radical species, such as the trisulfur ion S3(-), form very stable and soluble complexes with Au(+) in aqueous solution at elevated temperatures (>250 °C) and pressures (>100 bar). These species enable extraction, transport, and focused precipitation of gold by sulfur-rich fluids 10-100 times more efficiently than sulfide and chloride only. As a result, S3(-) exerts an important control on the source, concentration, and distribution of gold in its major economic deposits from magmatic, hydrothermal, and metamorphic settings. The growth and decay of S3(-) during the fluid generation and evolution is one of the key factors that determine the fate of gold in the lithosphere.

Published
2015
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8. Monitoring morphology and hydrogen coverage of nanometric Pt/γ-Al2 O3 particles by in situ HERFD-XANES and quantum simulations.

Author

Gorczyca A, Moizan V, Chizallet C, Proux O, Del Net W, Lahera E, Hazemann JL, Raybaud P, and Joly Y

Abstract

Platinum nanoclusters highly dispersed on γ-alumina are widely used as heterogeneous catalysts. To understand the chemical interplay between the Pt nanoparticles, the support, and the reductive atmosphere, we performed X-ray absorption near edge structure (XANES) in situ experiments recorded in high energy resolution fluorescence detection (HERFD) mode. Spectra are assigned by comparison with simulated XANES spectra on models obtained by molecular dynamics (DFT-MD). We propose platinum cluster morphologies and quantify the hydrogen coverages compatible with XANES spectra recorded at variable hydrogen pressures and temperatures. Using cutting-edge methodologies to assign XANES spectra, this work gives unequalled atomic insights into the characterization of supported nanoclusters., (© 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.)

Published
2014
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9. High-resolution spectroscopy on an X-ray absorption beamline.

Author

Hazemann JL, Proux O, Nassif V, Palancher H, Lahera E, Da Silva C, Braillard A, Testemale D, Diot MA, Alliot I, Del Net W, Manceau A, Gélébart F, Morand M, Dermigny Q, and Shukla A

Subjects
Computer-Aided Design, Equipment Design, Equipment Failure Analysis, Reproducibility of Results, Sensitivity and Specificity, Spectrometry, X-Ray Emission instrumentation, Spectrometry, X-Ray Emission methods, Transducers
Abstract

A bent-crystal spectrometer based on the Rowland circle geometry has been installed and tested on the BM30b/FAME beamline at the European Synchrotron Radiation Facility to improve its performances. The energy resolution of the spectrometer allows different kinds of measurements to be performed, including X-ray absorption spectroscopy, resonant inelastic X-ray scattering and X-ray Raman scattering experiments. The simplicity of the experimental device makes it easily implemented on a classical X-ray absorption beamline. This improvement in the fluorescence detection is of particular importance when the probed element is embedded in a complex and/or heavy matrix, for example in environmental sciences.

Published
2009
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