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Efficient optical classical and quantum information processing imposes on light novel requirements: chirality with low threshold non-linearities. In this work we demonstrate a chiral lasing from an optical modes due to emerging photonic Rashba-Dresselhaus spin-orbit coupling (SOC). For this purpose we developed a new electrically tunable device based on an optical cavity filled with birefringent liquid crystal (LC) and perovskite crystals. Our novel method for the growth of single crystals of CsPbBr$_3$ inorganic perovskite in polymer templates allows us to reach a strong light-matter coupling regime between perovskite excitons and cavity modes, and induce polariton condensation. The sensitivity of the LC to external electric fields lets us to tune the condensate energy in situ and induce synthetic SOC. This shapes the condensate between a single linearly polarized or two circularly polarized separated in momentum, emitting coherent light. The difference in the condensation thresholds between the two SOC regimes can be used to switch on and off the chiral condensate emission with a voltage., Comment: 8 pages, 5 figures

Rhenium disulfide (ReS2) belongs to group-VII transition metal dichalcogenide (TMDs) with attractive properties such as exceptionally high refractive index and significant oscillator strength, large in-plane birefringence, and good chemical stability. Unlike most other TMDs, the peculiar optical properties of ReS2 persist from bulk to the monolayer, making this material potentially suitable for applications in optical devices. In this work, we demonstrate with unprecedented clarity the strong coupling between cavity modes and excited states, which results in a strong polariton interaction, showing the interest of such materials as a solid-state counterpart of Rydberg atomic systems. Moreover, we definitively clarify the nature of important spectral features, shedding light on some controversial aspects or incomplete interpretations and demonstrating that their origin is due to the interesting combination of the very high refractive index and the large oscillator strength expressed by these TMDs.

The field of spinoptronics is underpinned by good control over photonic spin-orbit coupling in devices that possess strong optical nonlinearities. Such devices might hold the key to a new era of optoelectronics where momentum and polarization degrees-of-freedom of light are interwoven and interfaced with electronics. However, manipulating photons through electrical means is a daunting task given their charge neutrality and requires complex electro-optic modulation of their medium. In this work, we present electrically tunable microcavity exciton-polariton resonances in a Rashba-Dresselhaus spin-orbit coupling field at room temperature. We show that a combination of different spin orbit coupling fields and the reduced cavity symmetry leads to tunable formation of Berry curvature, the hallmark of quantum geometrical effects. For this, we have implemented a novel architecture of a hybrid photonic structure with a two-dimensional perovskite layer incorporated into a microcavity filled with nematic liquid crystal. Our work interfaces spinoptronic devices with electronics by combining electrical control over both the strong light-matter coupling conditions and artificial gauge fields.

Artificial gauge fields, simulating real phenomenologies that unfold in a vast variety of systems, offer extraordinary possibilities to study extreme physical effects in many different environments, from high energy physics to quantum mechanics and cosmology. They are also at the heart of topological physics. Here, exploiting a strongly anisotropic material under strong coupling regime, we experimentally synthesize a Yang-Mills non-Abelian gauge field acting on an exciton-polariton quantum flow like a magnetic field. We observe experimentally the corresponding curved trajectories and spin precession. This motion follows chromodynamics equations which normally describe the quarks strong interactions and their color. Our work therefore opens exciting perspectives of simulating quark-gluon dynamics using highly flexible photonic simulators. It makes of sub-atomic physics a potential new playground to apply topological physics concepts.

Polaritonic devices exploit the coherent coupling between excitonic and photonic degrees of freedom to perform highly nonlinear operations with low input powers. Most of the current results exploit excitons in epitaxially grown quantum wells and require low temperature operation, while viable alternatives have yet to be found at room temperature. Here we show that large single-crystal flakes of two-dimensional layered perovskite are able to sustain strong polariton nonlinearities at room temperature with no need to be embedded in an optical cavity. In particular, exciton-exciton interaction energies are measured to be remarkably similar to the ones known for inorganic quantum wells at cryogenic temperatures, and more than one order of magnitude larger than alternative room temperature polariton devices reported so far. Thanks to their easy fabrication, large dipolar oscillator strengths and strong nonlinearities, these materials hold great promises to realize actual polariton devices at room temperature., Comment: 16 pages, 4 figures, plus Supporting file

Hybrid organic-inorganic perovskites have emerged as very promising materials for photonic applications, thanks to the great synthetic versatility that allows to tune their optical properties. In the two-dimensional (2D) crystalline form, these materials behave as multiple quantum-well heterostructures with stable excitonic resonances up to room temperature. In this work strong light-matter coupling in 2D perovskite single-crystal flakes is observed, and the polarization-dependent exciton-polariton response is used to disclose new excitonic features. For the first time, an out-of-plane component of the excitons is observed, unexpected for such 2D systems and completely absent in other layered materials, such as transition-metal dichalcogenides. By comparing different hybrid perovskites with the same inorganic layer but different organic interlayers, it is shown how the nature of the organic ligands controllably affects the out-of-plane exciton-photon coupling. Such vertical dipole coupling is particularly sought in those systems, e.g. plasmonic nanocavities, in which the direction of the field is usually orthogonal to the material sheet. Organic interlayers are shown to affect also the strong birefringence associated to the layered structure, which is exploited in this work to completely rotate the linear polarization degree in only few microns of propagation, akin to what happens in metamaterials., Comment: 11 pages, 14 figures (included supporting info)