Search

Metal photocathodes are an important source of high-brightness electron beams, ubiquitous in the operation of both large-scale accelerators and table-top microscopes. When the surface of a metal is nano-engineered with patterns on the order of the optical wavelength, it can lead to the excitation and confinement of surface plasmon polariton waves which drive nonlinear photoemission. In this work, we aim to evaluate gold plasmonic nanogrooves as a concept for producing bright electron beams for accelerators via nonlinear photoemission. We do this by first comparing their optical properties to numerical calculations from first principles to confirm our ability to fabricate these nanoscale structures. Their nonlinear photoemission yield is found by measuring emitted photocurrent as the intensity of their driving laser is varied. Finally, the mean transverse energy of this electron source is found using the solenoid scan technique. Our data demonstrate the ability of these cathodes to provide a tenfold enhancement in the efficiency of photoemission over flat metals driven with a linear process. We find that these cathodes are robust and capable of reaching sustained average currents over 100 nA at optical intensities larger than 2 GW/cm$^2$ with no degradation of performance. The emittance of the generated beam is found to be highly asymmetric, a fact we can explain with calculations involving the also asymmetric roughness of the patterned surface. These results demonstrate the use of nano-engineered surfaces as enhanced photocathodes, providing a robust, air-stable source of high average current electron beams with great potential for industrial and scientific applications., 9 pages, 9 figures

Machine learning (ML) tools are able to learn relationships between the inputs and outputs of large complex systems directly from data. However, for time-varying systems, the predictive capabilities of ML tools degrade if the systems are no longer accurately represented by the data with which the ML models were trained. For complex systems, re-training is only possible if the changes are slow relative to the rate at which large numbers of new input-output training data can be non-invasively recorded. In this work, we present an approach to deep learning for time-varying systems that does not require re-training, but uses instead an adaptive feedback in the architecture of deep convolutional neural networks (CNN). The feedback is based only on available system output measurements and is applied in the encoded low-dimensional dense layers of the encoder-decoder CNNs. First, we develop an inverse model of a complex accelerator system to map output beam measurements to input beam distributions, while both the accelerator components and the unknown input beam distribution vary rapidly with time. We then demonstrate our method on experimental measurements of the input and output beam distributions of the HiRES ultra-fast electron diffraction (UED) beam line at Lawrence Berkeley National Laboratory, and showcase its ability for automatic tracking of the time varying photocathode quantum efficiency map. Our method can be successfully used to aid both physics and ML-based surrogate online models to provide non-invasive beam diagnostics.

Pulsed electron beam sources are increasingly in demand, especially as probes for ultrafast science and as patterning tools in lithography applications. Plasmonic nanostructures have been shown to enhance multiphoton photocurrent from metal cathodes by orders of magnitude, but for many applications it is also important to characterize the transverse electron beam properties. Here, we present preliminary work demonstrating a DC photogun setup for characterizing plasmonic photoemitters at Lawrence Berkeley National Laboratory, including measurement of photocurrent and the asymmetric transverse phase space of photoemitted beams from plasmonic nanogroove resonator arrays. This lays the groundwork for future studies of emerging plasmon-enhanced photoemitter designs, such as plasmonic lens nanoemitters.

One of the frontiers in electron scattering is to couple ultrafast temporal resolution with highly localized probes to investigate the role of microstructure on material properties. Here, taking advantage of the high average brightness of our electron source, we demonstrate the generation of ultrafast relativistic electron beams with picometer-scale emittance and their ability to probe nanoscale features on materials with complex microstructures. The electron beam is tightly focused at the sample plane by a custom in-vacuum lens system, and its evolution around the waist is accurately reconstructed. We then use the focused beam to characterize a Ti-6 wt% Al polycrystalline sample by correlating the diffraction and imaging modality, showcasing the capability to locate grain boundaries and map adjacent crystallographic domains with sub-micron precision. This work provides a paradigm for ultrafast electron instrumentation, enabling characterization techniques such as relativistic ultrafast electron nano-diffraction and ultrafast scanning transmission electron microscopy. Electrons have been used to map the structural properties of materials since the discovery of the particle-wave duality, while recent advances in ultrafast electron sources enabled time-resolved electron scattering techniques to probe atomic-scale structural dynamics with femtosecond temporal accuracy. The authors demonstrate ultrafast nano-diffraction with relativistic beams as well as scanning transmission electron microscopy enabling them to probe the micro-texture in complex heterogeneous materials.

We discuss our experiments that apply ultrafast electron diffraction (UED) to study structural dynamics of the phase transition in single crystal tantalum ditelluride, TaTe2, a quasi-2D quantum material which exhibits a trimer superstructure at cryogenic temperatures. Intense near-infrared (NIR) pulses at 1030 nm are employed to quench the low temperature, atomically ordered state and the process is captured by ultrashort bunches of electrons as a function of pump-probe time delay. The diffraction signatures of the trimer superstructure recover on picosecond time scales. These measurements of TaTe2 underscore moreover the applicability of the HiRES UED beamline at Lawrence Berkeley National Laboratory (LBNL) to probe ultrafast structural dynamics of complex materials.

Machine learning (ML) tools are able to learn relationships between the inputs and outputs of large complex systems directly from data. However for time-varying systems, the predictive capabilities of ML tools degrade if the systems are no longer accurately represented by the data with which the ML models were trained. For complex systems, re-training is only possible if the changes are slow relative to the rate at which large numbers of new input-output training data can be non-invasively recorded. In this work, we present an approach to deep learning for time-varying systems which does not require re-training. Our approach is to include adaptive feedback in the architecture of deep generative convolutional neural networks (CNN). The feedback is based only on available system output measurements and is applied in the encoded low-dimensional dense layers of the encoder-decoder CNNs. Our approach is inspired by biological systems in which separate groups of neurons interact and are controlled and synchronized by external feedbacks. We demonstrate this approach by developing an inverse model of a complex charged particle accelerator system, mapping output beam measurements to input beam distributions, while both the accelerator components and the unknown input beam distribution vary rapidly with time. We demonstrate our methods on experimental measurements of the input and output beam distributions of the HiRES ultra-fast electron diffraction (UED) beam line at Lawrence Berkeley National Laboratory. Our method can be successfully used to aid both physics and ML-based surrogate online models to provide non-invasive beam diagnostics. We also demonstrate our method for automatically tracking the time varying quantum efficiency map of a particle accelerator’s photocathode.

We report the first ultrafast study of TaTe2, utilizing MeV-scale ultrafast electron diffraction to reveal rapid photo-induced melting of its low-temperature trimer superstructure. Density-functional calculations indicate intra-trimer charge transfer as a trigger of this transformation.

The technological developments that led to the miniaturization of satellites, bringing to the market mini ( Small platforms allow reducing costs of development and management of single missions but also ease the possibility of using distributed systems in space making use of more satellites flying in formation or as a constellation. Furthermore, mini, micro and nano satellites are optimal candidate as platforms for the test and validation in space of innovative technologies with a lower level of maturity and thus not directly usable onboard “standard” sized satellites. The new generation of mini, micro and nano satellites can be proficiently used for the exploration and commercial utilization of small bodies of the Solar System (NEA, NEO, MBC, Asteroids); the characterisation of those bodies, in terms of composition, dimensions and interior structure, is of fundamental importance for the study of the evolution of our Solar System but also for the exploitation of extraterrestrial natural resources. There is a considerable advantage in using deployable systems onboard small satellites as these have considerable limitations in some of the resources, mainly mass and volume. The identification of payloads capable of minimising resources usage at launch, still guaranteeing in flight performances analogues to those of more “expensive”, in terms of resources, instruments is an extremely valuable benefit. The capability of using deployable telescopes allows to access scientific objectives and applications otherwise difficult to reach. In fact, remote sensing payload in the VIS/IR is strongly handicapped by the limited resources available onboard a mini-satellite which limits the size of the primary mirror and/or the length of the telescope assembly, thus resulting in reduced performances in terms of spatial resolution and signal to noise ratio. Precision-deployable, stable, optical telescopes that fit inside smaller, lower cost launch vehicles and small platform are a prime example of a technology that will yield breakthrough benefits for future scientific as well as more commercially-oriented applications. The DORA (Deployable Optics for Remote sensing Applications) project has been funded by the Italian Ministry of Research in the framework of the Italian National Research Plan 2015-2020 with a 30 months contract in a partnership between private companies (led by SITAEL the largest Italian privately-owned Company operating in the Space Sector), INAF (IAPS-Rome and Astronomical Observatory of Padua) the Parthenope University in Naples and Politecnico of Milan. Objective of the project is the design, realisation and test of a prototype of deployable optical system for Remote Sensing applications in the VIS and IR spectral ranges; a deployable telescope and straylight shield will be interfaced to a focal plane instrument (e.g. camera, imaging spectrometer, Fourier spectrometer). The telescope shall be stored in a closed configuration during launch to minimize volume and will be fully deployed in operative configuration once in flight by means of actuators. Similar deployable systems can be used to extend antennas used in microwave instrumentations (e.g., radiometers). The range of applications of such optomechanical technologies, in a space environment and onboard small satellites, are potentially very wide extending from Earth Observation satellites, used for environmental monitoring and for risk management, to Solar System exploration missions. In the framework of the DORA study the deployable optical system will be interfaced to an infrared Fourier spectrometer. We are taking advantage of the availability of the prototype of a miniaturised Fourier Spectrometer named MIMA (Mars Infrared MApper) [1] originally designed and built for the ExoMars 2020 mission but finally not among the selected payload; MIMA will be interfaced as a focal plane instrument to the Deployable telescope. MIMA is a double pendulum interferometer providing spectra in the 2 – 25 μm wavelength domain with a resolving power of 1000 at 2 μm and 80 at 25 μm. The radiometric performances are SNR >40 in the near infrared and a NEDe = 0.002 in the thermal region. The instrument design is very compact, with a total mass of 1 kg and an average power consumption of 5 W. The prototype has been tested and reached a Technology Readiness Level (TRL) of 5 level of development. The original FOV of the MIMA instrument was 3.2° which, although adequate for the in-situ analysis of the Martian soil, it is not sufficient to guarantee challenging results for typical Remote Sensing applications; thus MIMA will be matched to a 30 cm diameter, f/#=16, Cassegrain deployable telescope to reduce the FOV to ≤0.3°. The large sized primary mirror will guarantee the increase in collecting area needed to compensate for the considerable reduction of the FOV of the instrument. Such a combined instrument can be used proficiently for the study of small bodies of the Solar System. These bodies are remnants of original planetesimals from which the planets were formed. Differently from planets, which have experienced alterations during their evolution, the majority of small-sized asteroids underwent much less internal heating, resulting in a better preservation of their pristine composition. Since small bodies were the impactors of the primordial Earth, they may have been the principal carriers of water and organic material, the building blocks necessary to create life. A MWIR spectrometer like MIMA onboard a small mission will improve our understanding of the primordial cosmochemistry from small bodies remote sensing observations, providing unique data related to surface properties, mineralogy and thermal inertia. The scientific objectives can be summarised as: Analyse the thermophysical properties of the surface by measuring the temperature changes occurring during the diurnal cycle; Provide information on surface mineralogical composition and physical properties (grain size distribution, roughness); Search for thermal anomalies associated to the presence of surface rocks; Measure the thermal inertia of the surface The presentation will describe the development status of the DORA project providing detailed information on its expected performances. Acknowledgments. This study is funded by Ministry of Research PNR 2015-2020, specialisation area “aerospace” project n.ARS01_00653 References: [1] G. Bellucci et al., (2007). Proc. SPIE 6744, Sensors, Systems, and Next-Generation Satellites XI, 67441R, doi: 10.1117/12.737912

Ultrafast electron diffraction (UED) has become a leading technique for investigation of structural dynamics in solids providing high spatial and temporal resolutions. Radio frequency (RF) based photoinjectors providing Mega-electron-volt (MeV) scale electron beams are improving the source brightness and instrument versatility and are largely responsible for advancement of the field of structural dynamics. At Lawrence Berkeley National Laboratory (LBNL), an RF photoinjector gun for ultrafast structural studies using UED has been in development and is now producing high-quality scientific results. Here we describe some factors that enable UED of materials at LBNL and present some exemplary results.

Physical review accelerators and beams 23(4), 043401 (2020). doi:10.1103/PhysRevAccelBeams.23.043401, In state of the art photoinjector electron sources, thermal emittance from photoemission dominates the final injector emittance. Therefore, low thermal emittance cathode developments and diagnostics are very important. Conventional thermal emittance measurements for the high gradient gun are time-consuming and thus thermal emittance is not measured as frequently as quantum efficiency during the lifetime of photocathodes, although both are important properties for the photoinjector optimizations. In this paper, a single shot measurement of photoemission transverse momentum, i.e., thermal emittance per rms laser spot size, is proposed for photocathode rf guns. By tuning the gun solenoid focusing, the electrons’ transverse momenta at the cathode are imaged to a downstream screen, which enables a single shot measurement of both the rms value and the detailed spectra of the photoelectrons’ transverse momenta. Both simulations and proof of principle experiments are reported., Published by American Physical Society, College Park, MD

Nanoscale electron pulses are increasingly in demand, including as probes of nanoscale ultrafast dynamics and for emerging light source and lithography applications. Using electromagnetic simulations, we show that gold plasmonic lenses as multiphoton photoemitters provide unique advantages, including emission from an atomically at surface, nanoscale pulse diameter regardless of laser spot size, and femtosecond-scale response time. We then present fabrication of prototypes with sub-nm roughness via e-beam lithography, as well as electro-optical characterization using cathodoluminescence spectromicroscopy. Finally, we introduce a DC photogun at LBNL built for testing ultrafast photoemitters. We discuss measurement considerations for ultrafast nanoemitters and predict that we can extract tens of pA photocurrent from a single plasmonic lens using a Ti:Sa oscillator. Altogether, this lays the groundwork to develop and test a broad class of plasmon-enhanced ultrafast nanoemitters.

We show the capability of plasmonic lenses for next-generation ultrafast electron sources. Using electromagnetic simulations, we design structures capable of femtosecond, nanoscale electron pulses. Plasmonic properties of template-stripped gold prototypes are characterized using cathodoluminescence spectromicroscopy.

Quasi-two-dimensional transition-metal dichalcogenides are a key platform for exploring emergent nanoscale phenomena arising from complex interactions. Access to the underlying degrees-of-freedom on their natural time scales motivates the use of advanced ultrafast probes sensitive to self-organised atomic-scale patterns. Here, we report the first ultrafast investigation of TaTe2, which exhibits unique charge and lattice trimer order characterised by a transition upon cooling from stripe-like chains into a $(3 \times 3)$ superstructure of trimer clusters. Utilising MeV-scale ultrafast electron diffraction, we capture the photo-induced TaTe2 structural dynamics -- exposing a rapid $\approx\!1.4$ ps melting of its low-temperature ordered state followed by recovery via thermalisation into a hot cluster superstructure. Density-functional calculations indicate that the initial quench is triggered by intra-trimer Ta charge transfer which destabilises the clusters, unlike melting of charge density waves in other TaX2 compounds. Our work paves the way for further exploration and ultimately rapid optical and electronic manipulation of trimer superstructures., Comment: Main text and supplementary information: 30 pages, 4 main figures, 24 supplementary figures

Precise manipulation of high brightness electron beams requires detailed knowledge of the particle phase space shape and evolution. As ultrafast electron pulses become brighter, new operational regimes become accessible with emittance values in the picometer range, with enormous impact on potential scientific applications. Here we present a new characterization method for such beams and demonstrate experimentally its ability to reconstruct the 4D transverse beam matrix of strongly correlated electron beams with subnanometer emittance and submicrometer spot size, produced with the HiRES beamline at Lawrence Berkeley National Laboratory. Our work extends the reach of ultrafast electron accelerator diagnostics into picometer-range emittance values, opening the way to complex nanometer-scale electron beam manipulation techniques.

Author(s): Durham, DB; Riminucci, F; Ciabattini, F; Mostacci, A; Minor, AM; Cabrini, S; Filippetto, D | Abstract: Simultaneous spatiotemporal confinement of energetic electron pulses to femtosecond and nanometer scales is a topic of great interest in the scientific community, given the potential impact of such developments across a wide spectrum of scientific and industrial applications. For example, in ultrafast electron scattering, nanoscale probes would enable accurate maps of structural dynamics in materials with nanoscale heterogeneity, thereby leading to an understanding of the role of boundaries and defects on macroscopic properties. On the other hand, advances in this field are mostly limited by the brightness and size of the electron source. We present the design, fabrication, and optical characterization of bullseye plasmonic lenses for next-generation ultrafast electron sources. Using electromagnetic simulations, we examine how the interplay between light-plasmon coupling, plasmon propagation, dispersion, and resonance governs the properties of the photoemitted electron pulse. We also illustrate how the pulse duration and strength can be tuned by geometric design and predict that sub-10-fs pulses with nanoscale diameter can be achieved. We then fabricate lenses in gold films and characterize their plasmonic properties using cathodoluminescence spectromicroscopy, demonstrating suitable plasmonic behavior for ultrafast nanoscale photoemission.

© 2019 Author(s). The very-high-frequency gun (VHF-Gun) is a new concept photo-injector developed and built at the Lawrence Berkeley National Laboratory (LBNL) for generating high-brightness electron beams capable of driving X-ray free electron lasers (FELs) at MHz-class repetition rates. The gun that purposely uses established and mature radiofrequency and mechanical technologies has demonstrated over the last many years the capability of reliably operating in continuous wave mode at the design accelerating fields and required vacuum and mechanical performance. The results of VHF-Gun technology demonstration were reported elsewhere [Sannibale et al., Phys. Rev. Spec. Top.-Accel. Beams 15, 103501 (2012)]; here in this paper, we provide and analyze examples of the experimental results of the first high-brightness beam tests performed at the Advanced Photo-injector EXperiment test facility at LBNL that demonstrated the gun capability of delivering the beam quality required for driving high repetition rate X-ray FELs.

High brightness, high repetition rate electron beams are key components for optimizing the performance of next generation scientific instruments, such as MHz-class X-ray Free Electron Laser (XFEL) and Ultra-fast Electron Diffraction/Microscopy (UED/UEM). In the Advanced Photo-injector EXperiment (APEX) at Berkeley Lab, a photoelectron gun based on a 185.7 MHz normal conducting re-entrant RF cavity, has been proven to be a feasible solution to provide high brightness, high repetition rate electron beam for both XFEL and UED/UEM. Based on the success of APEX, a new electron gun system, named APEX2, has been under development to further improve the electron beam brightness. For APEX2, we have designed a new 162.5 MHz two-cell photoelectron gun and achieved a significant increase on the cathode launching field and the beam exit energy. For a fixed charge per bunch, these improvements will allow for the emittance reduction and hence to an increased beam brightness. The design of APEX2 gun cavity is a complex problem with multiple design goals and restrictions, some even competing each other. For a systematic and comprehensive search for the optimized cavity geometry, we have developed and implemented a novel optimization method based on the Multi-Objective Genetic Algorithm (MOGA).

The paper provides recent updates about the ESA study: Sample Canister Capture Mechanism Design and Breadboard developed under the Mars Robotic Exploration Preparation (MREP) program. The study is part of a set of feasibility studies aimed at identifying, analysing and developing technology concepts enabling the future international Mars Sample Return (MSR) mission. The MSR is a challenging mission with the purpose of sending a Lander to Mars, acquire samples from its surface/subsurface and bring them back to Earth for further, more in depth, analyses. In particular, the technology object of the Study is relevant to the Capture Mechanism that, mounted on the Orbiter, is in charge of capturing and securing the Sample Canister, or Orbiting Sample, accommodating the Martian soil samples, previously delivered in Martian orbit by the Mars Ascent Vehicle. An elegant breadboard of such a device was implemented and qualified under an ESA contract primed by OHB-CGS S.p.A. and supported by Politecnico di Milano, Department of Aerospace Science and Technology: in particular, functional tests were conducted at PoliMi-DAST and thermal and mechanical test campaigns occurred at Serms s.r.l. facility. The effectiveness of the breadboard design was demonstrated and the obtained results, together with the design challenges, issues and adopted solutions are critically presented in the paper. The breadboard was also tested on a parabolic flight to raise its Technology Readiness Level to 6; the microgravity experiment design, adopted solutions and results are presented as well in the paper.

We report on experimental activities on HiRES, a novel ultrafast electron diffraction beamline under development at LBNL. The instrument provides high-flux of relativistic electron pulses with sub-picosecond duration, which are then shaped in transverse and longitudinal phase space producing small spot sizes with femtosecond resolution. Alternatively beam shaping can be used to achieve large lateral coherence lengths for chemical and biological applications.

© 2017 authors. Published by the American Physical Society. Published by the American Physical Society under the terms of the "https://creativecommons.org/licenses/by/4.0/" Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI. The past decade was characterized by an increasing scientific demand for extending towards higher repetition rates (MHz class and beyond) the performance of already operating lower repetition rate accelerator-based instruments such as x-ray free electron lasers (FELs) and ultrafast electron diffraction (UED) and microscopy (UEM) instruments. Such a need stimulated a worldwide spread of a vibrant R&D activity targeting the development of high-brightness electron sources capable of operating at these challenging rates. Among the different technologies pursued, rf guns based on room-temperature structures resonating in the very high frequency (VHF) range (30-300 MHz) and operating in continuous wave successfully demonstrated in the past few years the targeted brightness and reliability. Nevertheless, recently proposed upgrades for x-ray FELs and the always brightness-frontier applications such as UED and UEM are now requiring a further step forward in terms of beam brightness in electron sources. In this paper, we present a few possible upgrade paths that would allow one to extend, in a relatively simple and cost-effective way, the performance of the present VHF technology to the required new goals.

© 2017 authors. Published by the American Physical Society. Published by the American Physical Society under the terms of the "https://creativecommons.org/licenses/by/4.0/" Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI. K-Cs-Sb bialkali antimonide photocathodes grown by a triple-element codeposition method have been found to have excellent quantum efficiency (QE) and outstanding near-atomic surface smoothness and have been employed in the VHF gun in the Advanced Photoinjector Experiment (APEX), however, their robustness in terms of their lifetime at elevated photocathode temperature has not yet been investigated. In this paper, the relationship between the lifetime of the K-Cs-Sb photocathode and the photocathode temperature has been investigated. The origin of the significant QE degradation at photocathode temperatures over 70 °C has been identified as the loss of cesium atoms from the K-Cs-Sb photocathode, based on the in situ x-ray analysis on the photocathode film during the decay process. The findings from this work will not only further the understanding of the behavior of K-Cs-Sb photocathodes at elevated temperature and help develop more temperature-robust cathodes, but also will become an important guide to the design and operation of the future high-field rf guns employing the use of such photocathodes.

© 2016, American Physical Society. All rights reserved. The need to operate an rf-gun-based electron photoinjector with a beam emitted away from the cathode center can occur under various circumstances. First, in some cases the cathode can be affected by ion back-bombardment that progressively reduces the quantum efficiency (QE) in its center, making off-axis operation mandatory; second, in some cases the drive laser intensity can be sufficiently high to generate QE depletion in the cathode area illuminated by the laser, forcing off-axis operation; last, in cathodes with nonuniform QE distribution it could be convenient to operate off axis to exploit a better QE. However, operation in this mode may lead to growth of the projected transverse beam emittances due to correlations between the transverse and longitudinal degrees of freedom that are introduced within the gun and downstream rf cavities. A strategy is described to mitigate this emittance growth by allowing the beam to propagate along a carefully tuned off-axis trajectory in downstream rf cavities to remove the time-dependent rf kicks introduced in the gun. Along this trajectory, short range wakefields do not degrade the emittance, and long range wakefields degrade the emittance for very high repetition rate only.

The development of undulator technologies capable of generating sub-cm undulator periods is assuming an increasing importance in X-ray free electron laser (FEL) applications. Indeed, such devices jointly with the high brightness electron beams already demonstrated at operating facilities would allow for lower energy, more compact electron linacs with a beneficial impact on the size and cost of X-ray FEL facilities. A novel design super-conducting undulator is being developed at the Lawrence Berkeley National Laboratory (LBNL) with the potential of sub-cm periods with reasonably large undulator parameter and gap. The potential and capability of such undulator technology need to be experimentally demonstrated. In this paper, the possibility of constructing an infrared FEL by combining the new undulator with the high brightness beam from the APEX injector facility at LBNL is investigated. Calculations show that the resulting FEL, when operated in self-amplified-spontaneous-emission mode, is expected to deliver a saturated power of almost a MW within a ∼ 4 m undulator length, in a single-spike of coherent radiation at ∼ 2 μ m wavelength. It will be also shown that the small-period of the undulator associated with the relatively low energy of the APEX beam, forces the FEL to operate in a regime with unusual and interesting characteristics. The alternative option of laser seeding the FEL is also briefly examined, showing the potential to reduce the saturation length even further.

Requirements and challenges for high-brightness electron injectors operating in a high-repetition-rate X-ray FEL are described. Schemes presently under development or study are reviewed, and their advantages and limitations are compared. Beam dynamics and engineering/technological aspects are addressed, with a particular emphasis placed on how the high-repetition-rate requirement impacts the choice of cathodes and of gun/accelerator technologies, and on how those choices consequently impact beam dynamics.

A new technique, named “laser comb”, was tested during the last SPARC run. It is able to produce electron pulse trains with a charge of some hundreds pC, a repetition rate of some terahertz, and a sub-picosecond length. This technique is based on the velocity bunching configuration of the SPARC injector. It can be useful to drive pump and probe free-electron laser experiments, to generate coherent excitation of plasma waves in plasma accelerators, and to produce narrow band terahertz radiation. In this paper, we describe the experimental results achieved so far and provide a comparison with simulations.

A study of the status of biomass briquetting and its perspectives in Brazil was conducted including determination of the availability and characteristics of the agro-residues for briquetting. Wood residues, rice husk and coffee husk were characterized and identified as the more promising agro-residues for briquetting in the short-term in Brazil. A survey was carried out in order to determine the number of briquetting factories in Brazil, and also to determine: used briquetting technologies, briquettes production, briquettes sale prices, the status of biomass briquetting market and its future perspectives.

A 250-TW laser system (FLAME - Frascati laser for acceleration and multidisciplinary experiments) is now in its commissioning phase in a new laboratory at LNF-INFN in the framework of the PLASMONX (Plasma acceleration and monochromatic X-ray generation) project. The laser will deliver < 25 fs duration pulses with an energy up to 6J, at a 10Hz repetition rate. An ad hoc target area has also been designed and is currently being set up, allowing the first test experiments of electron laser wakefield acceleration to be carried out over the next few months in a safe, radiation-protected environment. An overview of the main features of the laser system and target area is given, along with a survey of the design and set-up of the self-injection test experiment, which is expected to reach the production of sub-GeV electron bunches. © 2010 Taylor and Francis.

Inverse Compton scattering is a promising method to implement a high-brightness, ultra-short, energy tuneable X-ray source at accelerator facilities and at laser facilities using laser wake-field acceleration. We have developed an inverse Compton X-ray source driven by the multi-10-TW laser installed at Daresbury Laboratory. Polarized X-ray pulses will be generated through the interaction of laser pulses with electron bunches delivered by the energy recovery linac commissioned at the ALICE facility with spectral peaks ranging from 0.4 to 12 A, depending on the electron bunch energy and the scattering geometry. X-ray pulses containing up to 107 photons per pulse will be created from head-on collisions, with a pulse duration comparable to the incoming electron bunch length. For transverse collisions the laser pulse transit time defines the X-ray pulse duration. The peak spectral brightness is predicted to be up to 1021 photon/(s mm2 mrad2 0.1% Δλ/λ). Called COBALD, this source will be initially used as a short-pulse diagnostic for the ALICE electron beam and will explore the extreme challenges of photon/electron beam synchronization, which is a fundamental requirement for all conventional accelerator and laser wake-field-acceleration-based sources.

The SPARC photo-injector is an RD the beam transverse and longitudinal parameters at the exit of the gun have been measured, and the photo-injector settings optimized to achieve best performance. Several beam dynamics topics have been experimentally studied in this first phase of operation, as, for example, the effect of photocathode driver laser beam shaping and the evolution of the beam transverse emittance. These studies have been made possible by the use of a novel diagnostic tool, the “emittance-meter” which enables the measurement of the transverse beam parameters at different positions along the propagation axis in the very interesting region at the exit of the RF gun. The new idea of extending the e-meter capabilities came out more recently. Information on the beam longitudinal phase space and correlations with the transverse planes can be retrieved by the slicing technique. In this paper, we illustrate the basic concept of the measurement together with simulations that theoretically validate the methodology. Some preliminary results are discussed and explained with the aid of code simulations.

After the formidable results of X-ray 4th generation light sources based on free electron lasers around the world, a new revolutionary step is undergoing to extend the FEL performance from the present few hundred Hz to MHz-class repetition rates. In such facilities, temporally equi-spaced pulses will allow for a wide range of previously non-accessible experiments. The Advanced Photo-injector EXperiment (APEX) at the Lawrence Berkeley National Laboratory (LBNL), is devoted to test the capability of a novel scheme electron source, the VHF-Gun, to generate the required electron beam brightness at MHz repetition rates. In linac-based FELs, the ultimate performance in terms of brightness is defined at the injector, and in particular, cathodes play a major role in the game. Part of the APEX program consists in testing high quantum efficiency photocathodes capable to operate at the conditions required by such challenging machines. Results and status of these tests at LBNL are presented.

The APEX electron source at LBNL combines the high-repetition-rate with the high beam brightness typical of photoguns, delivering low emittance electron pulses at MHz frequency. Proving the high beam quality of the beam is an essential step for the success of the experiment, opening the doors of the high average power to brightness-hungry applications as X-Ray FELs, MHz ultrafast electron diffraction etc.. As first step, a complete characterization of the beam parameters is foreseen at the Gun beam energy of 750 keV. Diagnostics for low and high current measurements have been installed and tested, and measurements of cathode lifetime and thermal emittance in a RF environment with mA current performed. The recent installation of a double slit system, a deflecting cavity and a high precision spectrometer, allow the exploration of the full 6D phase space. Here we discuss the present layout of the machine and future upgrades, showing the latest results at low and high repetition rate, together with the tools and techniques used.

We report on measurements and analysis of a field-emitted electron current in the very-high-frequency (VHF) gun, a room temperature rf gun operating at high field and continuous wave (CW) mode at the Lawrence Berkeley National Laboratory (LBNL). The VHF gun is the core of the Advanced Photo-injector Experiment (APEX) at LBNL, geared toward the development of an injector for driving the next generation of high average power x-ray free electron lasers. High accelerating fields at the cathode are necessary for the high-brightness performance of an electron gun. When coupled with CW operation, such fields can generate a significant amount of field-emitted electrons that can be transported downstream the accelerator forming the so-called ``dark current.'' Elevated levels of a dark current can cause radiation damage, increase the heat load in the downstream cryogenic systems, and ultimately limit the overall performance and reliability of the facility. We performed systematic measurements that allowed us to characterize the field emission from the VHF gun, determine the location of the main emitters, and define an effective strategy to reduce and control the level of dark current at APEX. Furthermore, the energy spectra of isolated sources have been measured. A simple model for energy data analysis was developed that allows one to extract information on the emitter from a single energy distribution measurement.

SPARC-X is a two branch project consisting in the SPARC test facility dedicated to the development and test of critical subsystems such as high brightness photoinjector and a modular expandable undulator for SASE-FEL experiments at 500 nm with seeding, and the SPARK facility aiming at generation of high brilliance coherent radiation in the 1.5-13 nm range, based on the achieved expertise. The projects are supported by MIUR (Research Department of Italian Government) and Regione Lazio. SPARC has completed the commissioning phase of the photoinjector in November 2006. The achieved experimental results are here summarized together with the status of the second phase commissioning plans. The SPARK project is based on the generation of ultra high peak brightness electron beams at the energy of 1 and 2 GeV generating radiation in the 1.5-13 nm range. The construction is at the moment planned in two steps starting with a 1 GeV Linac. The project layout including both RF-compression and magnetic chicane techniques has been studied.

This paper discusses the extension to different electron beam aspect ratio of the Child-Langmuir law for the maximum achievable current density in electron guns. Using a simple model, we derive quantitative formulas in good agreement with simulation codes. The new scaling laws for the peak current density of temporally long and transversely narrow initial beam distributions can be used to estimate the maximum beam brightness and suggest new paths for injector optimization.

This paper describes the scientific aims and potentials as well as the preliminary technical design of RUDE, an innovative tool for multi-disciplinary investigations in a wide field of scientific, technological and industrial applications. IRIDE will be a high intensity "particles factory", based on a combination of high duty cycle radio-frequency superconducting electron linacs and of high energy lasers. Conceived to provide unique research possibilities for particle physics, for condensed matter physics, chemistry and material science, for structural biology and industrial applications, IRIDE will open completely new research possibilities and advance our knowledge in many branches of science and technology. [RIDE is also supposed to be realized in subsequent stages of development depending on the assigned priorities. (C) 2013 Elsevier B.V. All rights reserved.

We present the design and optimization of a new instrument for ultrafast electron diffraction and imaging. The proposed instrument merges the high peak current and relativistic electron energies of radio-frequency guns, with the high average electron flux of static electron microscopes, extending the beam parameter space achievable with relativistic electrons by many orders of magnitude. An immediate consequence of this work is a broader range of accessible science by using electron probes, enabling techniques as femtosecond nano-diffraction and coherent diffraction imaging, and paving the way to direct observation of ultrafast dynamics in complex and isolated samples, from nanocrystals, to nano/micro droplets and organic molecules.

The Advanced Photoinjector Experiment (APEX) at the Lawrence Berkeley National Laboratory is dedicated to the development of a high-brightness high-repetition rate (MHz-class) electron injector for x-ray free-electron laser (FEL) and other applications where high repetition rates and high brightness are simultaneously required. The injector is based on a new concept rf gun utilizing a normal-conducting (NC) cavity resonating in the VHF band at 186 MHz, and operating in continuous wave (cw) mode in conjunction with high quantum efficiency photocathodes capable of delivering the required charge at MHz repetition rates with available laser technology. The APEX activities are staged in three phases. In phase 0, the NC cw gun is built and tested to demonstrate the major milestones to validate the gun design and performance. Also, starting in phase 0 and continuing in phase I, different photocathodes are tested at the gun energy and at full repetition rate for validating candidate materials to operate in a high-repetition rate FEL. In phase II, a room-temperature pulsed linac is added for accelerating the beam at several tens of MeV to reduce space charge effects and allow the measurement of the brightness of the beam from the gun when integrated in an injector scheme. The installation of the phase 0 beam line and the commissioning of the VHF gun are completed, phase I components are under fabrication, and initial design and specification of components and layout for phase II are under way. This paper presents the phase 0 commissioning results with emphasis on the experimental milestones that have successfully demonstrated the APEX gun capability of operating at the required performance.

Higher order harmonic generation in a free-electron laser amplifier operating in the superradiant regime [R. H. Dicke, Phys. Rev. 93, 99 (1954).] has been observed. Superradiance has been induced by seeding a single-pass amplifier with the second harmonic of a Ti:sapphire laser, generated in a beta-Barium borate crystal, at seed intensities comparable to the free-electron laser saturation intensity. Pulse energy and spectral distributions of the harmonics up to the 11th order have been measured and compared with simulations.

A reliable transverse emittance measurement for high-brightness electron beams is of utmost importance for the successful development of fourth generation light sources and for the beam transport in plasmabased accelerators. When the beam exhibits a significant energy spread, typical quadrupole scan emittance measurements may be affected depending on the beam properties and on the quadrupoles arrangement. The emittance degradation induced by chromatic effects in measurements involving magnetic lattices is evaluated analytically for different configurations. Analytical and numerical calculations compared with measurements have been used to evaluate the consequent error on the emittance value measured for single and double quadrupole schemes and for typical operating conditions at the SPARC facility