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2. Evidence of a surprising channeling of ring-opening energy to the H2 product in the H + c-C3H6 [right arrow] H2 + C3H5 abstraction reaction

Author

Shuman, Nicholas S., Srivastava, Abneesh, Picconatto, Carl A., Danese, David S., Ray, Paresh C., and Valentini, James J.

Subjects
Chemical reactions -- Research, Isomerism -- Research, Cyclopropane compounds -- Research, Cyclopropane compounds -- Chemical properties, Chemistry, Physical and theoretical -- Research, Chemicals, plastics and rubber industries
Abstract

The product energy disposal in the abstraction reaction H + c-C3H6 [right arrow] H2(v', j') + C3H5 at 1.6 eV collision energy is characterized by quantum-state-selective, doppler-resolved REMPI detection of the H2(v', j') product. The H2(v', j') product is observed with total energy, translational plus rotational plus vibrational, in excess of the total energy available if the C3H5 product is a cyclopropyl radical.

Published
2003

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