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On the context of the Cern n_TOF collaboration the 232Th(n,2n)231Th reaction cross section has been measured relative to the 56Fe(n,p)56Mn and 27Al(n,a)24Na reaction cross sections by the activation method for neutron energies up to 11 MeV. The neutrons were produced via the 2H(d,n) reaction using a deuterium filled gas-cell, at the 5.5MV TANDEM Accelerator of NCSR "Demokritos". In addition to the experimental work, theoretical Statistical model calculations have been performed using the computer code STAPRE/F. The code STAPRE is designed to calculate energy averaged cross sections for particle induced nuclear reactions with several emitted particles and gamma rays under the assumption of sequential evaporation. For the first evaporation step preequilibrium emission is taken into account while population of states resulting from the first equilibrium evaporation step is calculated using the Hauser-Feschbach theory. Fission process competition is also taken into account in the evaporation steps. Sensitive parameters for the calculation, like level density parameters, have been adopted after fitting experimental data for the competing (n,f) reaction. The results are being compared to the experimental data.

The 232 Th(n,2n) 231 Th reaction cross-section was measured relative to the 56 Fe(n,p) 56 Mn and 27 Al(n,a) 24 Na reaction cross-sections with the activation method for neutron energies up to 11 MeV. Neutrons were produced by the 2 H(d,n) reaction in the 5.5 MV Tandem accelerator of the NCSR ‘‘Demokritos’’. The characteristic g lines of the product nuclei 231 Th (25.646 keV) and 56 Mn (846.771 keV) or 24 Na (1368 keV) were measured with an 80 mm 2 Si(Li) and a 20% reverseelectrode coaxial germanium detector, respectively. The results indicate that our values are in agreement with the JEF2 and BROND2 database values up to 9 MeV and slightly higher than those from all the libraries for higher energies. r 2003 Elsevier Science B.V. All rights reserved.