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To harness the intriguing properties of two-dimensional van der Waals (vdW) ferromagnets (FMs) for versatile applications, the key challenge lies in the reliable material synthesis for scalable device production. Here, we demonstrate the epitaxial growth of single-crystalline 1T-CrTe2 thin films on 2-inch sapphire substrates. Benefiting from the uniform surface energy of the dangling bond-free Al2O3(0001) surface, the layer-by-layer vdW growth mode is observed right from the initial growth stage, which warrants precise control of the sample thickness and atomically smooth surface morphology across the entire wafer. Moreover, the presence of the Coulomb interaction at the CrTe2/Al2O3 interface serves as an effective tuning parameter to tailor the anomalous Hall response, and the structural optimization of the CrTe2-based spin-orbit torque device leads to a substantial switching power reduction by 54%. Our results may lay out a general framework for the design of energy-efficient spintronics based on configurable vdW FMs., Comment: 20 pages, 4 figures

The intrinsic magnetic topological insulator MnBi2Te4 (MBT) has provided a platform for the successful realization of exotic quantum phenomena. To broaden the horizons of MBT-based material systems, we intercalate ferromagnetic MnTe layers to construct the [(MBT)(MnTe)m]N superlattices by molecular beam epitaxy. The effective incorporation of ferromagnetic spacers mediates the anti-ferromagnetic interlayer coupling among the MBT layers through the exchange spring effect at the MBT/MnTe hetero-interfaces. Moreover, the precise control of the MnTe thickness enables the modulation of relative strengths among the constituent magnetic orders, leading to tunable magnetoelectric responses, while the superlattice periodicity serves as an additional tuning parameter to tailor the spin configurations of the synthesized multi-layers. Our results demonstrate the advantages of superlattice engineering for optimizing the magnetic interactions in MBT-family systems, and the ferromagnet-intercalated strategy opens up new avenues in magnetic topological insulator structural design and spintronic applications., Comment: 20 pages, 5 figures

By means of local ion implantation, we investigated the influence of lateral interface on current-induced magnetic switching by spin-orbit torque in a perpendicularly magnetized Pt/Co/Ta multilayer. The experimental results show that, in this system, the domain wall motion under electrical current can be affected by two mechanisms: symmetry breaking and current-driven N\'eel wall motion at the lateral interface. The dominant mechanism is symmetry breaking (current-driven N\'eel wall motion) at the large (small) current. Due to the competitive relationship of these two mechanisms, the non-hysteresis effect magnetic switching without an external magnetic field is obtained. Based on the non-hysteresis effect magnetic switching, we can realize AND and OR logic gates without resetting.

Symmetry breaking is a characteristic to determine which branch of a bifurcation system follows upon crossing a critical point. Specifically, in spin-orbit torque (SOT) devices, a fundamental question arises: how to break the symmetry of the perpendicular magnetic moment by the in-plane spin polarization? Here, we show that the chiral symmetry breaking by the DMI can induce the deterministic SOT switching of the perpendicular magnetization. By introducing a gradient of saturation magnetization or magnetic anisotropy, non-collinear spin textures are formed by the gradient of effective SOT strength, and thus the chiral symmetry of the SOT-induced spin textures is broken by the DMI, resulting in the deterministic magnetization switching. We introduce a strategy to induce an out-of-plane (z) gradient of magnetic properties, as a practical solution for the wafer-scale manufacture of SOT devices., Comment: 16 pages, 4 figures

Heavy metal/ferromagnetic layers with perpendicular magnetic anisotropy (PMA) have potential applications for high-density information storage in racetrack memories and nonvolatile magnetic random access memories. Writing and erasing of information in these devices are carried out by domain wall (DW) motion and deterministic magnetization switching via electric current generated spin orbital torques (SOTs) with an assistance of in-plane bias field to break the symmetry. Improvements in energy efficiency could be obtained when the switching of perpendicular magnetization is controlled by an electric current generated SOTs without the in-plane bias fields. Here, we report on reversible electric-current-driven magnetization switching through DW motion in Pt/Co/Cr trilayers with PMA at room temperature due to the formation of homochiral Neel-type domain, in which an in-plane effective Dzyaloshinskii-Moriya interaction field exists. Fully deterministic magnetic magnetization switching in this trilayers is based on the enhancement of SOTs from a dedicated design of Pt/Co/Cr structures with two heavy metals Pt and Cr which show the opposite sign of spin Hall angles. We also demonstrated that the simultaneously accompanying Joule heating effect also plays a key role for field-free magnetization switching through the decrease of the propagation field., Comment: 6 figures, 16 pages

Magnetic trilayers having large perpendicular magnetic anisotropy (PMA) and high spin-orbit torques (SOTs) efficiency are the key to fabricate nonvolatile magnetic memory and logic devices. In this work, PMA and SOTs are systematically studied in Pt/Co/Cr stacks as a function of Cr thickness. An enhanced perpendicular anisotropy field around 10189 Oe is obtained and is related to the interface between Co and Cr layers. In addition, an effective spin Hall angle up to 0.19 is observed due to the improved antidamping-like torque by employing dissimilar metals Pt and Cr with opposite signs of spin Hall angles on opposite sides of Co layer. Finally, we observed a nearly linear dependence between spin Hall angle and longitudinal resistivity from their temperature dependent properties, suggesting that the spin Hall effect may arise from extrinsic skew scattering mechanism. Our results indicate that 3d transition metal Cr with a large negative spin Hall angle could be used to engineer the interfaces of trilayers to enhance PMA and SOTs., Comment: 14 pages, 6 figures