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Detailed γ-ray spectroscopy of the exotic neon isotope $^{28}$Ne has been performed for the first time using the one-neutron removal reaction from $^{29}$Ne on a liquid hydrogen target at 240 MeV/nucleon. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for $^{28}$Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder p-wave strength providing evidence of the breakdown of the N=20 and N=28 shell gaps. Only a weak, possible f-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large p-wave and small f-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.

The collective structure of $^{106}$Cd is elucidated by multi-step Coulomb excitation of a 3.849 MeV/A beam of $^{106}$Cd on a 1.1 mg/cm$^{2}$ $^{208}$Pb target using GRETINA-CHICO2 at ATLAS. Fourteen E2 matrix elements were obtained. The nucleus $^{106}$Cd is a prime example of emergent collectivity that possesses a simple structure: it is free of complexity caused by shape coexistence and has a small, but collectively active number of valence nucleons. This work follows in a long and currently active quest to answer the fundamental question of the origin of nuclear collectivity and deformation, notably in the cadmium isotopes. The results are discussed in terms of phenomenological models, the shell model, and Kumar-Cline sums of E2 matrix elements. The 〈02+||E2||21+〉 matrix element is determined for the first time, providing a total, converged measure of the electric quadrupole strength, 〈Q2〉, of the first-excited 21+ level relative to the 01+ ground state, which does not show an increase as expected of harmonic and anharmonic vibrations. Strong evidence for triaxial shapes in weakly collective nuclei is indicated; collective vibrations are excluded. This is contrary to the only other cadmium result of this kind in $^{114}$Cd by C. Fahlander et al. (1988) [38], which is complicated by low-lying shape coexistence near midshell.

International audience; The collective structure of 106Cd is elucidated by multi-step Coulomb excitation of a 3.849 MeV/A beam of 106Cd on a 1.1 mg/cm2208Pb target using GRETINA-CHICO2 at ATLAS. Fourteen E2 matrix elements were obtained. The nucleus 106Cd is a prime example of emergent collectivity that possesses a simple structure: it is free of complexity caused by shape coexistence and has a small, but collectively active number of valence nucleons. This work follows in a long and currently active quest to answer the fundamental question of the origin of nuclear collectivity and deformation, notably in the cadmium isotopes. The results are discussed in terms of phenomenological models, the shell model, and Kumar-Cline sums of E2 matrix elements. The 〈02+||E2||21+〉 matrix element is determined for the first time, providing a total, converged measure of the electric quadrupole strength, 〈Q2〉, of the first-excited 21+ level relative to the 01+ ground state, which does not show an increase as expected of harmonic and anharmonic vibrations. Strong evidence for triaxial shapes in weakly collective nuclei is indicated; collective vibrations are excluded. This is contrary to the only other cadmium result of this kind in 114Cd by C. Fahlander et al. (1988) [38], which is complicated by low-lying shape coexistence near midshell.

The excitation energy of deformed intruder states (specifically the 2p2h bandhead) as a function of proton number Z along N=20 is of interest both in terms of better understanding the evolution of nuclear structure between spherical Ca40 and the Island of Inversion nuclei, and for benchmarking theoretical descriptions in this region. At the center of the N=20 Island of Inversion, the npnh (where n=2,4,6) neutron excitations across a diminished N=20 gap result in deformed and collective ground states, as observed in Mg32. In heavier isotones, npnh excitations do not dominate in the ground states but are present in the relatively low-lying level schemes. With the aim of identifying the expected 2p2h - s1/2+ state in P35, the only N=20 isotone for which the neutron 2p2h excitation bandhead has not yet been identified, the S36(d,He3)P35 reaction has been revisited in inverse kinematics with the HELical Orbit Spectrometer (HELIOS) at the Argonne Tandem Linac Accelerator System (ATLAS). While a candidate state has not been located, an upper limit for the transfer reaction cross section to populate such a configuration within a 2.5 to 3.6 MeV energy range provides a stringent constraint on the wave function compositions in both S36 and P35.

International audience; The low-spin structure of the semimagic Ni64 nucleus has been considerably expanded: combining four experiments, several 0+ and 2+ excited states were identified below 4.5 MeV, and their properties established. The Monte Carlo shell model accounts for the results and unveils an unexpectedly complex landscape of coexisting shapes: a prolate 0+ excitation is located at a surprisingly high energy (3463 keV), with a collective 2+ state 286 keV above it, the first such observation in Ni isotopes. The evolution in excitation energy of the prolate minimum across the neutron N=40 subshell gap highlights the impact of the monopole interaction and its variation in strength with N.

Detailed spectroscopy of the neutron-unbound nucleus $^{28}$F has been performed for the first time following proton/neutron removal from $^{29}$Ne/$^{29}$F beams at energies around 230 MeV/nucleon. The invariant-mass spectra were reconstructed for both the $^{27}$F$^{(*)}+n$ and $^{26}$F$^{(*)}+2n$ coincidences and revealed a series of well-defined resonances. A near-threshold state was observed in both reactions and is identified as the $^{28}$F ground state, with $S_n(^{28}$F$)=-199(6)$ keV, while analysis of the $2n$ decay channel allowed a considerably improved $S_n(^{27}$F$)=1620(60)$ keV to be deduced. Comparison with shell-model predictions and eikonal-model reaction calculations have allowed spin-parity assignments to be proposed for some of the lower-lying levels of $^{28}$F. Importantly, in the case of the ground state, the reconstructed $^{27}$F$+n$ momentum distribution following neutron removal from $^{29}$F indicates that it arises mainly from the $1p_{3/2}$ neutron intruder configuration. This demonstrates that the island of inversion around $N=20$ includes $^{28}$F, and most probably $^{29}$F, and suggests that $^{28}$O is not doubly magic., 6 pages, 3 figures, Supplemental Material, accepted for publication in Physical Review Letters

An extensive, model-independent analysis of the nature of triaxial deformation in Ge76, a candidate for neutrinoless double-beta (0νββ) decay, was carried out following multistep Coulomb excitation. Shape parameters deduced on the basis of a rotational-invariant sum-rule analysis provided considerable insight into the underlying collectivity of the ground-state and γ bands. Both sequences were determined to be characterized by the same β and γ deformation parameter values. In addition, compelling evidence for low-spin, rigid triaxial deformation in Ge76 was obtained for the first time from the analysis of the statistical fluctuations of the quadrupole asymmetry deduced from the measured E2 matrix elements. These newly determined shape parameters are important input and constraints for calculations aimed at providing, with suitable accuracy, the nuclear matrix elements relevant to 0νββ.

International audience; One of the most exotic light neutron-rich nuclei currently accessible for experimental study is Mg40, which lies at the intersection of the nucleon magic number N=28 and the neutron drip line. Low-lying excited states of Mg40 have been studied for the first time following a one-proton removal reaction from Al41, performed at the Radioactive Isotope Beam Factory of RIKEN Nishina Center with the DALI2 γ-ray array and the ZeroDegree spectrometer. Two γ-ray transitions were observed, suggesting an excitation spectrum that shows unexpected properties as compared to both the systematics along the Z=12, N≥20 Mg isotopes and available state-of-the-art theoretical model predictions. A possible explanation for the observed structure involves weak-binding effects in the low-lying excitation spectrum.

The neutron-rich $^{122-131}$Sb isotopes were produced as fission fragments in the reaction $^{9}$Be($^{238}$U,~f) with 6.2 MeV/u beam energy. An unique setup, consisting of AGATA, VAMOS++ and EXOGAM detectors, was used which enabled the prompt-delayed gamma-ray ($\gamma$) spectroscopy of fission fragments in the time range of 100 ns - 200 $\mu$s. New isomers, prompt and delayed transitions were established in the even-A $^{122-130}$Sb isotopes. In the odd-A $^{123-131}$Sb isotopes, new prompt and delayed $\gamma$-ray transitions were identified, in addition to the confirmation of the previously known isomers. The half-lives of the isomeric states and the $B(E2)$ transition probabilities of the observed transitions depopulating these isomers were extracted. The experimental data was compared with the theoretical results obtained in the framework of Large-Scale Shell-Model (LSSM) calculations in a restricted model space. Modifications of several components of the shell model interaction were introduced to obtain a consistent agreement with the excitation energies and the $B(E2)$ transition probabilities in neutron-rich Sn and Sb isotopes. The isomeric configurations in Sn and Sb were found to be relatively pure. Further, the calculations revealed that the presence of a single valence proton, mainly in the $g_{7/2}$ orbital in Sb isotopes, leads to significant mixing (due to the $\nu\pi$ interaction) of: (i) the neutron seniorities ($\upsilon_{\nu}$) and (ii) the neutron angular momentum ($I_{\nu}$). The above features have a weak impact on the excitation energies, but have an important impact on the $B(E2)$ transition probabilities. In addition, a constancy of the relative excitation energies irrespective of neutron seniority and neutron number in Sn and Sb was observed., Comment: 23 pages, 18 figures, 10 tables

International audience; The structure of 71 Zn was investigated by one-neutron transfer and heavy-ion induced complex (deep-inelastic) reactions using the GRETINA-CHICO2 and the Gammasphere setups, respectively. The observed inversion between the 9/2 + and 1/2 − states is explained in terms of the role of neutron pairing correlations. Non-collective sequences of levels were delineated above the 9/2 + isomeric state. These are interpreted as being associated with a modest oblate deformation in the framework of Monte-Carlo shell-model calculations carried out with the A3DA-m Hamiltonian in the pfg9/2d5/2 valence space. Similarities with the structure of Ni402868 were observed and the shape-coexistence mechanism in the N=40 region of neutron-rich nuclei is discussed in terms of the so-called Type-II shell evolution, with an emphasis on proton–neutron correlations between valence nucleons, especially those involving the shape-driving g9/2 neutron orbital.

International audience; A new experimental setup to measure prompt-delayed $\gamma$ -ray coincidences from isotopically identified fission fragments, over a wide time range of 100ns-200μ s, is presented. The fission fragments were isotopically identified, on an event-by-event basis, using the VAMOS++ large acceptance spectrometer. The prompt $\gamma$ rays emitted at the target position and corresponding delayed $ \gamma$ rays emitted at the focal plane of the spectrometer were detected using, respectively, thirty two crystals of the AGATA $\gamma$ -ray tracking array and seven EXOGAM HPGe Clover detectors. Fission fragments produced in fusion and transfer-induced fission reactions, using a$^{238}$U beam at an energy of 6.2 MeV/u impinging on a$^{9}$Be target, were used to characterize and qualify the performance of the detection system.

Background: Levels fulfilling the seniority scheme and relevant isomers are commonly observed features in semimagic nuclei; for example, in Sn isotopes (Z=50). Seniority isomers in Sn, with dominantly pure neutron configurations, directly probe the underlying neutron-neutron (νν) interaction. Furthermore, an addition of a valence proton particle or hole, through neutron-proton (νπ) interaction, affects the neutron seniority as well as the angular momentum. Purpose: Benchmark the reproducibility of the experimental observables, like the excitation energies (EX) and the reduced electric-quadrupole transition probabilities [B(E2)], with the results obtained from shell-model interactions for neutron-rich Sn and Sb isotopes with N

The octupole strength present in the neutron-rich, radiocative nucleus 146Ba has been experimentally determined for the first time using Coulomb excitation. To achieve this, A=146 fission fragments from CARIBU were post-accelerated by the Argonne Tandem Linac Accelerator System (ATLAS) and impinged on a thin 208Pb target. Using the GRETINA γ-ray spectrometer and the CHICO2 heavy-ion counter, the reduced transition probability B(E3; 3-→0+) was determined as 48(+21-29) W.u. The new result provides further experimental evidence for the presence of a region of octupole deformation surrounding the neutron-rich barium isotopes.

International audience; The distribution of single-particle strength in $^{67,69}$Ni was characterized with one-neutron knockout reactions from intermediate-energy $^{68,70}$Ni secondary beams, selectively populating neutron-hole configurations at N=39 and 41, respectively. The spectroscopic strengths deduced from the measured partial cross sections to the individual final states, as tagged by their γ-ray decays, are used to identify and quantify neutron configurations in the wave functions. While $^{69}$Ni compares well with shell-model predictions, the results for $^{67}$Ni challenge the validity of current effective shell-model Hamiltonians by revealing discrepancies that cannot be explained so far. These results suggest that our understanding of the low-lying states in the neutron-rich, semimagic Ni isotopes may be incomplete and requires further investigation on both the experimental and theoretical sides.

Near shell closures, the presence of unexpected states at low energies provides a critical test of our understanding of the atomic nucleus. New measurements for the N=42 isotones Co2769 and Cu2971, along with recent data and calculations in the Ni isotopes, establish a full set of complementary, deformed, intruder states astride the closed-shell Ni28 isotopes. Nuclei with a one-proton hole or one-proton particle adjacent to Z=28 were populated in β-decay experiments and in multinucleon transfer reactions. A β-decaying isomer, with a 750(250)-ms half-life, has been identified in Co422769. It likely has low spin and accompanies the previously established 7/2- state. Complementary data for the levels of isotonic Cu422971 support the presence of a deformed, ΔJ=1 band built on the proton intruder 7/2- level at 981 keV. These data, together with recent studies of lower-mass Co and Cu isotopes and extensive work near Ni68, support the view that intruder states based on particle-hole excitations accompany all closed proton shells with Z≥28.

Expérience réalisée au NSCL

The isomeric and β-decay properties of neutron-rich Sc53-57 and Ca53,54 nuclei near neutron number N=32 are reported, and the low-energy level schemes of Sc53,54,56 and Ti53-57 are presented. The low-energy level structures of the 21Sc isotopes are discussed in terms of the coupling of the valence 1f7/2 proton to states in the corresponding 20Ca cores. Implications with respect to the robustness of the N=32 subshell closure are discussed, as well as the repercussions for a possible N=34 subshell closure.

β decay of the Cr6137 ground state has been studied. A new half-life of 233±11 ms has been deduced, and seven delayed γ rays have been assigned to the daughter Mn6136. The low-energy level structure of Mn6136 is similar to that of the less neutron-rich Mn57,59 nuclei. The odd-A25Mn isotopes follow the systematic trend in the yrast states of the even-even, Z+1 26Fe isotopes, and not that of the Z-1 24Cr isotopes, where a possible onset of collectivity has been suggested to occur already at N=36.

β-decay properties of neutron-rich Ca isotopes have been obtained. Half-life values were determined for the first time for Ca54 (86±7 ms), Ca55 (22±2 ms), and Ca56 (11±2 ms). The half-life of 230±60 ms deduced for Ca53 is significantly longer than reported previously, where the decay chain K53 → Ca53 → Sc53 was considered. A delayed γ ray with an energy of 247 keV was identified following β decay of Ca54 and is proposed to depopulate the 11+ level in Sc54. The β-decay properties compare favorably with the results of shell-model calculations completed in the full pf space with the GXPF1 interaction. The half-lives of the neutron-rich Ca isotopes are also compared with gross β-decay theory. The systematic trend of the neutron-rich Ca half-lives is consistent with the presence of a subshell gap at N=32.