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Any given prescription of quantum time travel necessarily endows a Hilbert space to the chronology-violating (CV) system on the closed timelike curve (CTC). However, under the two foremost models, Deutsch's prescription (D-CTCs) and postselected teleportation (P-CTCs), the CV system is treated very differently: D-CTCs assign a definite form to the state on this system, while P-CTCs do not. To further explore this distinction, we present a methodology by which an operational notion of state may be assigned to their respective CV systems. This is accomplished via a conjunction of state tomography and weak measurements, with the latter being essential in leaving any notions of self-consistency intact. With this technique, we are able to verify the predictions of D-CTCs and, perhaps more significantly, operationally assign a state to the system on the P-CTC. We show that, for any given combination of chronology-respecting input and unitary interaction, it is always possible to recover the unique state on the P-CTC, and we provide a few specific examples in the context of select archetypal temporal paradoxes. We also demonstrate how this state may be derived from analysis of the P-CTC prescription itself, and we explore how it compares to its counterpart in the CV state predicted by D-CTCs., Comment: 17 pages, 9 figures

We consider the question: Is it possible to measure two temperatures simultaneously using a single thermometer? Under common circumstances, where the thermometer can interact with only one bath at a time and the interaction leads to complete thermalization, this is clearly impossible because the final state of the thermometer would be independent of the temperature of the first bath. In this work, we show that this task can indeed be accomplished with the assistance of quantum control. In particular, we consider a composite particle with multiple quantum degrees of freedom (DoF) as a temperature sensor, where one of the DoF -- termed as internal DoF -- is susceptible to the local temperature, thereby functioning as a thermometer, whereas another DoF -- termed external DoF -- is quantum-controlled. We leverage the entanglement between the aforementioned DoF in a composite particle for two-temperature thermometry by preparing the external DoF in a quantum superposition, exposing the internal DoF to two local temperatures. We show that such a particle used in a Mach-Zehnder type interferometer, or a quantum switch -- which allows quantum control over the order of application of quantum channels -- can be used to estimate two temperatures simultaneously, thus affirming our main proposition. For each of these setups, we obtain the variance in the estimated temperatures through the multi-parameter Cram\'er-Rao bound, and compare their performances based on the range of total variance of the two temperatures estimated. On benchmarking all the setups based on the total variance of the estimated temperatures, we find that a quantum switch with a qudit probe outperforms other setups. On restricting our probe to be a qubit, we find that quantum switch performs equally well as a Mach-Zehnder type interferometer., Comment: 14 pages, 10 figures

What does it mean for a causal structure to be `unknown'? Can we even talk about `repetitions' of an experiment without prior knowledge of causal relations? And under what conditions can we say that a set of processes with arbitrary, possibly indefinite, causal structure are independent and identically distributed? Similar questions for classical probabilities, quantum states, and quantum channels are beautifully answered by so-called "de Finetti theorems", which connect a simple and easy-to-justify condition -- symmetry under exchange -- with a very particular multipartite structure: a mixture of identical states/channels. Here we extend the result to processes with arbitrary causal structure, including indefinite causal order and multi-time, non-Markovian processes applicable to noisy quantum devices. The result also implies a new class of de Finetti theorems for quantum states subject to a large class of linear constraints, which can be of independent interest., Comment: Reference added and minor revision. 11 main + 4 references + 5 appendix = 20 pages, 3 figures

Current quantum technologies are at the cusp of becoming useful, but still face formidable obstacles such as noise. Noise severely limits the ability to scale quantum devices to the point that they would offer an advantage over classical devices. To understand the sources of noise it is necessary to fully characterise the quantum processes occurring across many time steps; only this would reveal any time-correlated noise called non-Markovian. Previous efforts have attempted such a characterisation but obtained only a limited reconstruction of such multi-time processes. In this work, we fully characterise a multi-time quantum process on superconducting hardware using in-house and cloud-based quantum processors. We achieve this by employing sequential measure-and-prepare operations combined with post-processing. Employing a recently developed formalism for multi-time processes, we detect general multi-time correlated noise. We also detect quantum correlated noise which demonstrates that part of the noise originates from quantum sources, such as physically nearby qubits on the chip. Our findings and techniques are expected to advance error-mitigation techniques in current quantum hardware, a necessary component to scale up the technology and achieve its true potential., Comment: 9 pages, 5 figures, 4 tables

Single layers of transition metal dichalcogenides, such as WSe$_2$ have gathered increasing attention due to their intense electron-hole interactions, being considered promising candidates for developing novel optical applications. Within the few-layer regime, these systems become highly sensitive to the surrounding environment, enabling the possibility of using a proper substrate to tune desired aspects of these atomically-thin semiconductors. In this scenario, the dielectric environment provided by the substrates exerts significant influence on electronic and optical properties of these layered materials, affecting the electronic band-gap and the exciton binding energy. However, the corresponding effect on the luminescence of transition metal dichalcogenides is still under discussion. To elucidate these impacts, we used a broad set of materials as substrates for single-layers of WSe$_2$, enabling the observation of these effects over a wide range of electrical permittivities. Our results demonstrate that an increasing permittivity induces a systematic red-shift of the optical band-gap of WSe$_2$, intrinsically related to a considerable reduction of the luminescence intensity. Moreover, we annealed the samples to ensure a tight coupling between WSe$_2$and its substrates, reducing the effect of undesired adsorbates trapped in the interface. Ultimately, our findings reveal how critical the annealing temperature can be, indicating that above a certain threshold, the heating treatment can induce adverse impacts on the luminescence. Furthermore, our conclusions highlight the influence the dielectric properties of the substrate have on the luminescence of WSe$_2$, showing that a low electrical permittivity favours preserving the native properties of the adjacent monolayer, Comment: 16 pages, 8 figures

Indefinite causal order is a key feature involved in the study of quantum higher order transformations. Recently, intense research has been focused on possible advantages related to the lack of definite causal order of quantum processes. Quite often the quantum switch is claimed to provide advantages in information-theoretic and thermodynamic tasks. We address here the question whether indefinite causal order is a resource for quantum thermodynamics. Inspired by previous results in the literature, we show that indefinite causal order is not necessary for the reported increase in free energy and ergotropy. More specifically, we show that a simple causally ordered process, which replaces the system's state with a new one before the final measurement, outperforms the quantum switch in all thermodynamic tasks considered so far. We further show that a similar advantage can be also achieved without completely discarding system, if we allow for non-Markovian interactions between the system and an environment. We extend the analysis to more extreme examples of indefinite causal order, showing that they do not provide an advantage either. Finally, we discuss a possible way to study the advantages that may arise from indefinite causal order in a general scenario.

Gravitationally bound neutrons have become an important tool in the experimental searches for new physics, such as modifications to Newton's force or candidates for dark matter particles. Here we include the relativistic effects of mass-energy equivalence into the model of gravitationally bound neutrons. Specifically, we investigate a correction in a gravitationally bound neutron's Hamiltonian due to the presence of an external magnetic field. We show that the neutron's additional weight due to mass-energy equivalence will cause a small shift in the neutron's eigenenergies and eigenstates, and examine how this relativistic correction would affect experiments with trapped neutrons. We further consider the ultimate precision in estimating the relativistic correction to the precession frequency and find that, at short times, a joint measurement of both the spin and motional degrees of freedom provides a metrological enhancement as compared to a measurement of the spin alone.

Past studies of the billiard-ball paradox, a problem involving an object that travels back in time along a closed timelike curve (CTC), typically concern themselves with entirely classical histories, whereby any trajectorial effects associated with quantum mechanics cannot manifest. Here we develop a quantum version of the paradox, wherein a (semiclassical) wave packet evolves through a region containing a wormhole time machine. This is accomplished by mapping all relevant paths on to a quantum circuit, in which the distinction of the various paths is facilitated by representing the billiard particle with a clock state. For this model, we find that Deutsch's prescription (D-CTCs) provides self-consistent solutions in the form of a mixed state composed of terms which represent every possible configuration of the particle's evolution through the circuit. In the equivalent circuit picture (ECP), this reduces to a binomial distribution in the number of loops of time machine. The postselected teleportation prescription (P-CTCs) on the other hand predicts a pure-state solution in which the loop counts have binomial coefficient weights. We then discuss the model in the continuum limit, with a particular focus on the various methods one may employ in order to guarantee convergence in the average number of clock evolutions. Specifically, for D-CTCs, we find that it is necessary to regularise the theory's parameters, while P-CTCs alternatively require more contrived modification., Comment: 18 pages, 9 figures

According to the general theory of relativity, time can flow at different rates depending on the configuration of massive objects, affecting the temporal order of events. Recent research has shown that, combined with quantum theory, this gravitational effect can result in events with an indefinite temporal order, which can be tested through the violation of Bell-type inequalities. According to Einstein, we shall assume physical equivalence of a uniform gravitational field and a corresponding acceleration of a reference system. Here we construct a non-gravitational scenario where accelerating particles interacting with optical cavities result in a violation of the temporal Bell inequalities analogous to the gravitational case. However, we find that the inequalities can also be violated by time-like events, exposing an ambiguity in their use as a theory-independent test of indefinite temporal order.

A quantum system and a thermal bath can reach thermal equilibrium through an interaction, whereupon the system acquires the same temperature as the bath. But how does a delocalised quantum system thermalise with a bath whose local temperature varies, as, for example, in the Tolman effect? Here we formulate two scenarios in which the notion of a ``superposition of temperatures'' may arise. First: a probe interacting with two different baths dependent on the state of another quantum system (control). Second: a probe interacting with a single bath whose purified state is a superposition of states corresponding to different temperatures. We show that the two scenarios are fundamentally different and can be operationally distinguished. Moreover, we show that the probe does not in general thermalise even when the involved temperatures are equal, and that the final probe state is sensitive to the specific realisation of the thermalising channels. Our models may be applied to scenarios involving joint quantum, gravitational, and thermodynamic phenomena, and explain some recent results found in quantum intereference of relativistic probes thermalising with Unruh or Hawking radiation. Finally, we show that our results are reproduced in partial and pre-thermalisation processes, and thus our approach and conclusions hold beyond the idealised scenarios, where thermalisation is incomplete., Comment: 13 pages, including references and appendix, 5 figures. Significant rewording of arguments in several sections, updated references

Being a flexible wide band gap semiconductor, hexagonal boron nitride (h-BN) has great potential for technological applications like efficient deep ultraviolet light sources, building block for two-dimensional heterostructures and room temperature single photon emitters in the ultraviolet and visible spectral range. To enable such applications, it is mandatory to reach a better understanding of the electronic and optical properties of h-BN and the impact of various structural defects. Despite the large efforts in the last years, aspects such as the electronic band gap value, the exciton binding energy and the effect of point defects remained elusive, particularly when considering a single monolayer. Here, we directly measured the density of states of a single monolayer of h-BN epitaxially grown on highly oriented pyrolytic graphite, by performing low temperature scanning tunneling microscopy (STM) and spectroscopy (STS). The observed h-BN electronic band gap on defect-free regions is $(6.8\pm0.2)$ eV. Using optical spectroscopy to obtain the h-BN optical band gap, the exciton binding energy is determined as being of $(0.7\pm0.2)$ eV. In addition, the locally excited cathodoluminescence and photoluminescence show complex spectra that are typically associated to intragap states related to carbon defects. Moreover, in some regions of the monolayer h-BN we identify, using STM, point defects which have intragap electronic levels around 2.0 eV below the Fermi level., Comment: 50 Pages, 8 Figures, 100+ references

We consider the effect of gravity on extended quantum systems (EQS) in the low energy regime. We model the gravitational effect due to a nearby source mass as a redshift in the internal Hamiltonian of the EQS. Due to the dependence of the energy spectrum of the EQS on the position of the massive particle (via the redshift) at zero temperature, our model predicts gravitational decoherence of the massive particle in the position basis. We show that the decoherence effect is multiplicative, in the sense that the increase in number of EQS gravitationally interacting with a single massive particle leads to an increase in its decoherence. If the considered model of gravitational redshift holds alongside the linearity of quantum mechanics (as an appropriate limit of an accepted theory for coupling quantum matter with gravity) to allow for a spatial superposition of the source mass, we propose that the same methodology can be applied to continuous fields, which are essentially EQS. This could provide an upper limit on the number of undiscovered fields by observing coherent superpositions of masses, e.g., in a matter wave interferometer. Besides, by taking a spin chain as a toy model of an EQS, we analyse the dependence of the new effect on relevant system parameters and identify the number of independent spin chains that can cause a detectable effect., Comment: 11 pages, 6 figures

One of the key ways in which quantum mechanics differs from relativity is that it requires a fixed background reference frame for spacetime. In fact, this appears to be one of the main conceptual obstacles to uniting the two theories. Additionally, a combination of the two theories is expected to yield non-classical, or "indefinite", causal structures. In this paper, we present a background-independent formulation of the process matrix formalism - a form of quantum mechanics that allows for indefinite causal structure - while retaining operationally well-defined measurement statistics. We do this by postulating an arbitrary probability distribution of measurement outcomes across discrete "chunks" of spacetime, which we think of as physical laboratories, and then requiring that this distribution be invariant under any permutation of laboratories. We find (a) that one still obtains nontrivial, indefinite causal structures with background independence, (b) that we lose the idea of local operations in distinct laboratories, but can recover it by encoding a reference frame into the physical states of our system, and (c) that permutation invariance imposes surprising symmetry constraints that, although formally similar to a superselection rule, cannot be interpreted as such., Comment: 8 pages + 3 page appendix

The task of compression of data -- as stated by the source coding theorem -- is one of the cornerstones of information theory. Data compression usually exploits statistical redundancies in the data according to its prior distribution. Motivated by situations where one does not have access to the statistics of data, but has some information about a transformation that is going to be applied to it, we propose a novel method for data compression called reverse compression. It is defined in such a way that works for both classical and quantum information processes, and furthermore relies exclusively on the channel to be used: all input data leading to indistinguishable outputs is compressed to the same state, regardless of their prior distribution. Moreover, this process can be characterized as a higher order operation within the type of preprocessing. We also consider as an example the application of the method to the classical and quantum erasure channel. The examples suggest that noiseless reverse compression can take place only in trivial cases, although meaningful instances of noisy reverse compression can exist.

The causal order of events need not be fixed: whether a bus arrives before or after another at a certain stop can depend on other variables -- like traffic. Coherent quantum control of causal order is possible too and is a useful resource for several tasks. However, quantum control implies that a controlling system carries the which-order information -- if the control is traced out, the order of events remains in a probabilistic mixture. Can the order of two events be in a pure superposition, uncorrelated with any other system? Here we show that this is not possible for a broad class of processes: a pure superposition of any pair of Markovian, unitary processes with equal local dimensions and different causal orders is not a valid process, namely it results in non-normalised probabilities when probed with certain operations. The result imposes constraints on novel resources for quantum information processing and on possible processes in a theory of quantum gravity., Comment: 6+4 pages, two pictures, final version

General relativity predicts the existence of closed timelike curves (CTCs), along which an object could travel to its own past. A consequence of CTCs is the failure of determinism, even for classical systems: one initial condition can result in multiple evolutions. Here we introduce a new quantum formulation of a classic example, where a billiard ball can travel along two possible trajectories: one unperturbed and one, along a CTC, where it collides with its past self. Our model includes a vacuum state, allowing the ball to be present or absent on each trajectory, and a clock, which provides an operational way to distinguish the trajectories. We apply the two foremost quantum theories of CTCs to our model: Deutsch's model (D-CTCs) and postselected teleportation (P-CTCs). We find that D-CTCs reproduce the classical solution multiplicity in the form of a mixed state, while P-CTCs predict an equal superposition of the two trajectories, supporting a conjecture by Friedman et al. [Phys. Rev. D 42, 1915 (1990)]., Comment: 15 pages, 8 figures

Quantum mechanics allows operations to be in indefinite causal order. Recently there have been active discussions on enhanced communication strategies through exotic causal structures. In light of this, through the process matrix formalism, we formulate different classical capacities for a bi-partite quantum process. We find that a one-way communication protocol through an arbitrary process cannot outperform a causally separable process, i.e., we can send at most one bit per qubit. Next, we study bi-directional communication through a causally separable process. Our result shows, a bi-directional protocol cannot exceed the limit of one way communication protocol. Finally, we generalise this result to multi-party broadcast communication protocol through a definite ordered process.

Quantum interference of "clocks", namely of particles with time-evolving internal degrees of freedom (DOFs), is a promising avenue to test genuine general relativistic effects in quantum systems. The clock acquires which path information while experiencing different proper times on traversing the arms of the interferometer, leading to a drop in its path visibility. We consider scenarios where the clock is subject to environmental noise as it transits through the interferometer. In particular, we develop a generalized formulation of interferometric visibility affected by noise on the clock. We find that, for small noise and small proper time difference between the arms, the noise further reduces the visibility, while in more general situations it can either increase or reduce the visibility. As an example, we investigate the effect of a thermal environment constituted by a single field mode and show that the visibility drops further as the temperature is increased. Additionally, by considering noise models based on standard quantum channels, we show that interferometric visibility can increase or decrease depending on the type of noise and also the time scale and transition probabilities. The quantification of the effect of noise on the visibility -- particularly in the case of a thermal environment paves the way for a better estimate on the expected outcome in an actual experiment., Comment: 21 pages, 11 figures, Accepted in Quantum

The theory of general relativity predicts the existence of closed time-like curves (CTCs), which theoretically would allow an observer to travel back in time and interact with their past self. This raises the question of whether this could create a grandfather paradox, in which the observer interacts in such a way to prevent their own time travel. Previous research has proposed a framework for deterministic, reversible, dynamics compatible with non-trivial time travel, where observers in distinct regions of spacetime can perform arbitrary local operations with no contradiction arising. However, only scenarios with up to three regions have been fully characterised, revealing only one type of process where the observers can verify to both be in the past and future of each other. Here we extend this characterisation to an arbitrary number of regions and find that there exist several inequivalent processes that can only arise due to non-trivial time travel. This supports the view that complex dynamics is possible in the presence of CTCs, compatible with free choice of local operations and free of inconsistencies.

In theories of communication, it is usually presumed that the involved parties perform actions in a fixed causal order. However, practical and fundamental reasons can induce uncertainties in the causal order. Here we show that a maximal uncertainty in the causal order forbids asymptotic quantum communication, while still enabling the noisy transfer of classical information. Therefore causal order, like shared entanglement, is an additional resource for communication. The result is formulated within an asymptotic setting for processes with no fixed causal order, which sets a basis for a quantum information theory in general quantum causal structures., Comment: 5 pages, 1 figure

Supervised learning algorithms take as input a set of labelled examples and return as output a predictive model. Such models are used to estimate labels for future, previously unseen examples drawn from the same generating distribution. In this paper we investigate the possibility of using supervised learning to estimate the dimension of a non-Markovian quantum environment. Our approach uses an ensemble learning method, the Random Forest Regressor, applied to classically simulated data sets. Our results indicate this is a promising line of research.

We present a method to detect quantum memory in a non-Markovian process. We call a process Markovian when the environment does not provide a memory that retains correlations across different system-environment interactions. We define two types of non-Markovian processes, depending on the required memory being classical or quantum. We formalise this distinction using the process matrix formalism, through which a process is represented as a multipartite state. Within this formalism, a test for entanglement in a state can be mapped to a test for quantum memory in the corresponding process. This allows us to apply separability criteria and entanglement witnesses to the detection of quantum memory. We demonstrate the method in a simple model where both system and environment are single interacting qubits and map the parameters that lead to quantum memory. As with entanglement witnesses, our method of witnessing quantum memory provides a versatile experimental tool for open quantum systems., Comment: Main text: 5 pages, 2 figures. Appendix: 6 pages, 4 figures