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Resonances are essential for understanding the interactions between light and matter in photonic systems. The real frequency response of the non-Hermitian systems depends on the complex-valued resonance frequencies, which are the poles of electromagnetic response functions. The zeros of the response functions are often used for designing devices, since the zeros can be located close to the real axis, where they have significant impact on scattering properties. While methods are available to determine the locations of the poles, there is a lack of appropriate approaches to find the zeros in photonic systems. We present an approach to compute poles and zeros based on contour integration of electromagnetic quantities. This also allows to extract sensitivities with respect to geometrical or other parameters enabling efficient device design. The approach is applied to a topical example in nanophotonics, an illuminated metasurface, where the emergence of reflection zeros due to the underlying resonance poles is explored using residue-based modal expansions. The generality and simplicity of the theory allows straightforward transfer to other areas of physics. We expect that easy access to zeros will enable new computer-aided design methods in photonics and other fields.

Physical systems and signals are often characterized by complex functions of frequency in the harmonic-domain. The extension of such functions to the complex frequency plane has been a topic of growing interest as it was shown that specific complex frequencies could be used to describe both ordinary and exceptional physical properties. In particular, expansions and factorized forms of the harmonic-domain functions in terms of their poles and zeros under multiple physical considerations have been used. In this work, we start from a general property of continuity and differentiability of the complex functions to derive the multiple-order singularity expansion method. We rigorously derive the common singularity and zero expansion and factorization expressions, and generalize them to the case of singularities of arbitrary order, whilst deducing the behaviour of these complex frequencies from the simple hypothesis that we are dealing with physically realistic signals., Comment: Main manuscript: 13 pages, 5 figures. Supporting information: 6 pages, 3 figures

Full wavefront control by photonic components requires that the spatial phase modulation on an incoming optical beam ranges from 0 to 2{\pi}. Because of their radiative coupling to the environment, all optical components are intrinsically non-Hermitian systems, often described by reflection and transmission matrices with complex eigenfrequencies. Here, we show that Parity-Time symmetry breaking -- either explicit or spontaneous -- moves the position of Zero singularities of the reflection or transmission matrices from the real axis to the upper part of the complex frequency plane. A universal 0 to 2{\pi}-phase gradient of an output channel as a function of the real frequency excitation is thus realized whenever the discontinuity branch bridging a Zero and a Pole, i.e a pair of singularities, is crossing the real axis. This basic understanding is applied to engineer electromagnetic fields at interfaces, including, but not limited to, metasurfaces. Non-Hermitian topological features associated with exceptional degeneracies or branch cut crossing are shown to play a surprisingly pivotal role in the design of resonant photonic systems.

We study the effect of coupled resonances and quasi-bound states in the continuum (quasi-BICs) on the Purcell factor in dielectric resonant nanoantennas. We analyze numerically interfering resonances in a nanodisk with and without a substrate when the modes are coupled to an emitter localized inside the nanodisk, and we quantify the modal contributions to the Purcell factor also reconstructing the radiation patterns of the resonant system. It is revealed that the Purcell effect can be boosted substantially for a strong coupling of resonances in the quasi-BIC regime.

Light interaction with optical cavities is of fundamental interest to enhance the light-matter interaction and to shape the spectral features of the electromagnetic fields. Important efforts have been carried out to develop modal theories of open optical cavities relying on an expansion of the fields on the eigen-fields of the cavity. Here, we show how such an expansion predicts the temporal dynamics of optical resonators. We consider a Fabry-Perot cavity to derive the full analytical expressions of the internal and scattered field on the quasi-normal modes basis together with the complex eigen-frequencies. We evince the convergence and accuracy of this expansion before deriving the impulse response function (IRF) of the open cavity. We benefit from this modal expansion and IRF to demonstrate that the eigen-modes of the open cavity impact the signals only during the transient regimes and not in the permanent regime.

Quasinormal mode (QNM) expansion is a popular tool to analyze light-matter interaction in nanoresonators. However, expanding far-field quantities such as the energy flux is an open problem because QNMs diverge with an increasing distance to the resonant systems. We introduce a theory to compute modal expansions of far-field quantities rigorously. The presented approach is based on the complex eigenfrequencies of QNMs. The divergence problem is circumvented by using contour integration with an analytical continuation of the far-field quantity into the complex frequency plane. We demonstrate the approach by computing the angular resolved modal energy flux in the far field of a nanophotonic device.

Resonant States (RS), also known as Quasi-Normal Modes (QNMs), are eigenstates that arise in spectral expansions of linear response functions of open systems. Manipulation of these spatially `divergent' oscillating functions requires a departure from the usual definitions of inner product, normalization and orthogonality typically encountered in the studies of closed systems. We show that once RS fields are expanded on a multipole basis, Gaussian regularization methods provide \emph{analytical} results for crucial RS inner product integrals \added{in the problematic region exterior to the scattering system}. Our demonstrations are carried out in the context of light scattering by spatially bounded objects composed of both electrically and magnetically dispersive media, with demonstrative analytic calculations being shown to \emph{completely} retrieve the results of exact Mie theory., Comment: 39 pages, 12 figures

Modal analysis based on the quasi-normal modes (QNM), also called resonant states, has emerged as a promising way for modeling the resonant interaction of light with open optical cavities. However, the fields associated with QNM in open photonic cavities diverge far away from the scatterer and the possibility of expanding the scattered field with resonant contributions only has not been established. Here, we address these two issues while restricting our study to the case of a dispersionless spherical scatterer. First, we derive the rigorous pole expansion of the $T$-matrix coefficients that link the scattered to the incident fields associated with an optical resonator. This expansion evinces the existence of a non-resonant term. Second, in the time domain, the causality principle allows us to solve the problem of divergence and to derive a modal expansion of the scattered field that does not diverge far from the scatterer.

Polarizability expressions are commonly used in optics and photonics to model the light scattering by small particles. Models based on Taylor series of the scattering coefficients of the particles fail to predict the morphologic resonances hosted by dielectric particles. Here, we propose to use the factorization of the special functions appearing in the expression of the Mie scattering coefficients to derive point-like models. These models can be applied to reproduce both Mie resonances of dielectric particles and plasmonic resonances of metallic particles. They provide simple but robust tools to predict accurately the electric and magnetic Mie resonances in dielectric particles., Comment: 11 pages, 7 figures

This work studies the limits of far and near-field electromagnetic response of sub-wavelength scatterers, like the unitary limit and of lossless scatterers, and the ideal absorption limit of lossy particles. These limit behaviors are described in terms of analytic formulas that approximate finite size effects while rigorously including radiative corrections. This analysis predicts the electric and/or magnetic limit responses of both metallic and dielectric nanoparticles while quantitatively describing near-field enhancements., Comment: 9 pages, 8 figures, 2 tables