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The intrinsic anomalous Nernst effect in a magnetic material is governed by the Berry curvature at the Fermi energy and can be realized in non-collinear antiferromagnets with vanishing magnetization. Thin films of (001)-oriented Mn$_{3}$NiN have their chiral antiferromagnetic structure located in the (111) plane facilitating the anomalous Nernst effect unusually in two orthogonal in-plane directions. The sign of each component of the anomalous Nernst effect is determined by the local antiferromagnetic domain state. In this work, a temperature gradient is induced in a 50 nm thick Mn$_{3}$NiN two micron-size Hall cross by a focused scanning laser beam, and the spatial distribution of the anomalous Nernst voltage is used to image and identify the octupole macrodomain arrangement. Although the focused laser beam width may span many individual domains, cooling from room temperature through the antiferromagnetic transition temperature in an in-plane magnetic field prepares the domain state producing a checkerboard pattern resulting from the convolution of contributions from each domain. These images together with atomistic and micromagnetic simulations suggest an average macrodomain of the order of $1 {\mu}m^{2}$., Comment: 25 pages 4 figures, 6 supplementary figures F.J. and J.K. both contributed equally to this manuscript. The following article has been accepted by Applied Physics Letters. After it is published, it will be found at https://aip.scitation.org/journal/apl

The NaZn13 type itinerant magnet LaFe13-xSix has seen considerable interest due to its unique combination of large magnetocaloric effect and low hysteresis. Here we demonstrate, with a combination of magnetometry, bespoke microcalorimetry and inelastic neutron scattering that this is due to the presence of paramagnetic spin fluctuations, which build up as the critical point is approached. While thermal measurements show significant latent heat independent changes in the heat capacity, inelastic neutron scattering reveals the presence of broad quasielastic scattering that persists above Tc, in addition to a finite Q quasielastic peak at Q=0.52 A$^{-1}$ (close to a 100 Bragg reflection in this system at Q = 0.54 A$^{-1}$). This finite Q quasielastic peak appears only in the paramagnetic state and when in proximity to the itinerant metamagnetic transition. We associate these observations with a hidden competing phase and spin fluctuations close to the transition temperature and magnetic field, that persist across the magnetic transition.

Here we present a magnetic thin film with a weak ferrimagnetic (FIM) phase above the N\'eel temperature ($T_{N}$ = 240 K) and a non-collinear antiferromagnetic (AFM) phase below, exhibiting a small net magnetisation due to strain-associated canting of the magnetic moments. A long-range ordered FIM phase has been predicted in related materials, but without symmetry analysis. We now perform this analysis and use it to calculate the MOKE spectra in AFM and FIM phases. From the good agreement between the form of the measured and predicted MOKE spectra, we propose the AFM and FIM phases share the magnetic space group C2'/m' and that the symmetry driven magneto-optic and magneto-transport properties are maximised at room temperature in the FIM phase due to the non-zero intrinsic Berry phase contribution present in these materials. A room temperature FIM phase with large optical and transport signatures, as well as sensitivity to lattice strain and magnetic field, has useful prospects for high-speed spintronic applications., Comment: 21 pages 4 figures 1 table 4 supplementary figures 1 supplementary table Co-first author: F. Johnson and J. Z\'azvorka Corresponding authors: L. F. Cohen and M. Veis; Typos corrected and discussion of symmetry added; title changed to be concise; text on figures made larger

We present measurements of ferromagnetic-resonance - driven spin pumping and inverse spin-Hall effect in NbN/Y3Fe5O12 (YIG) bilayers. A clear enhancement of the (effective) Gilbert damping constant of the thin-film YIG was observed due to the presence of the NbN spin sink. By varying the NbN thickness and employing spin-diffusion theory, we have estimated the room temperature values of the spin diffusion length and the spin Hall angle in NbN to be 14 nm and -1.1 10-2, respectively. Furthermore, we have determined the spin-mixing conductance of the NbN/YIG interface to be 10 nm-2. The experimental quantification of these spin transport parameters is an important step towards the development of superconducting spintronic devices involving NbN thin films.

We examine the evidence for multiband superconductivity and non s-wave pairing in the non-centrosymmetric superconductor Nb$_{0.18}$Re$_{0.82}$, using electrical transport, magnetization and specific heat measurements. In the normal state, both the evolution of resistivity with temperature and with magnetic field support a multiband picture. In the superconducting state, the Werthamer, Helfand and Hohenberg (WHH) model cannot adequately describe the temperature dependence of the upper critical field, $H_{c2}(T)$, over the whole temperature range measured. In addition, the observed $H_{c2}(0)$ exceeds the Pauli limit, suggesting non-s-wave pairing. Interestingly, the Kadowaki-Woods ratio and Uemura plot reveal a behavior in Nb$_{0.18}$Re$_{0.82}$ which is similar to that found in unconventional superconductors. The temperature dependence of the lower critical field, $H_{c1}(T)$, follows an anomalous $T^3$ behavior and the derived normalized superfluid density ($\rho_s$) is well explained using a nodeless two-gap description. Phase-fluctuation analysis conducted on the reversible magnetization data, reveals a significant deviation from the mean-field conventional s-wave behavior. This trend is interpreted in terms of a non s-wave spin-triplet component in the pairing symmetry as might be anticipated in a non-centrosymmetric superconductor where anti-symmetric spin-orbit coupling plays a dominant role., Comment: 24 pages, 7 figures

We quantify the spin Hall angle {\theta}SH and spin diffusion length lsd of Nb from inverse spin-Hall effect (iSHE) measurements in Nb/Ni80Fe20 bilayers under ferromagnetic resonance. By varying the Nb thickness tNb and comparing to a Ni80Fe20/Pt reference sample, room temperature values of {\theta}SH and lsd for Nb are estimated to be approximately -0.001 and 30 nm, respectively. We also investigate the iSHE as a function of temperature T for different tNb. Above the superconducting transition temperature Tc of Nb, a clear tNb-dependent T evolution of the iSHE is observed whereas below Tc, the iSHE voltage drops rapidly and is below the sensitivity of our measurement setup at a lower T. This suggests the strong decay of the quasiparticle (QP) charge-imbalance relaxation length across Tc, as supported by an additional investigation of the iSHE in a different sample geometry along with model calculation. Our finding suggests careful consideration should be made when developing superconductor spin-Hall devices that intend to utilize QP-mediated spin-to-charge interconversion., Comment: 25 pages, 7 figures, SM; note that the title of the manuscript has been changed to "Spin-pumping-induced inverse spin-Hall effect in Nb/Ni80Fe20 bilayers and its strong decay across the superconducting transition temperature."

We report a detailed study of isofield magnetic relaxation and isothermal magnetization measurements with $H$$\parallel$c on an underdoped Ba$_{0.75}$K$_{0.25}$Fe$_2$As$_2$ pnictide single crystal, with superconducting transition temperature $T_c$ = 28 K. The second magnetization peak (SMP) has been observed at temperatures below $T_c$/2 and vanished at higher temperatures. The observed behaviour of the SMP has been studied by measuring the magnetic field dependence of relaxation rate, $R(H)$ and by performing the Maley's analysis. The results suggest that the crossover from collective to plastic pinning observed in the SMP disappears above 12 K with plastic pinning replacing collective pinning. An interesting $H$-$T$ phase diagram is obtained. The critical current density ($J_c$) was estimated using Bean's model and found to be $\sim$ $3.4 \times 10^9$ A/m$^2$ at 10 K in the SMP region, which is comparable to an optimally doped Ba-KFe$_2$As$_2$ superconductor and may be exploited for potential technological applications. The pinning mechanism is found to be unconventional and does not follow the usual $\delta l$ and $\delta T_c$ pinning models, which suggest the intrinsic nature of pinning in the compound., Comment: 8 pages, 9 figures

Spin pumping is becoming an established method to generate voltages from magnetic dynamics. The standard detection method of spin pumping is based on open circuit voltage measurement across ferromagnetic (FM) and non-magnetic (NM) bi-layers, where the inverse spin-Hall effect (ISHE) can convert spin currents into electrical charge accumulation. In this paper, we present that it is also possible to measure the associated electric charge current generated in FM/NM bi-layers, by using a macroscopic closed circuitry detection method. Using variable load resistors connected in series to the sample, we quantified charge currents and associated electric power dissipation as a function of the load resistance. By using basic circuit analysis, we are able to describe spin pumping cells as a non-ideal voltage source or equivalent current source with an internal resistor.

Nanomagnetic arrays are widespread in data storage and processing. As current technologies approach fundamental limits on size and thermal stability, extracting additional functionality from arrays is crucial to advancing technological progress. One design exploiting the enhanced magnetic interactions in dense arrays is the geometrically-frustrated metamaterial 'artificial spin ice' (ASI). Frustrated systems offer vast untapped potential arising from their unique microstate landscapes, presenting intriguing opportunities from reconfigurable logic to magnonic devices or hardware neural networks. However, progress in such systems is impeded by the inability to access more than a fraction of the total microstate space. Here, we present a powerful surface-probe lithography technique, magnetic topological lithography, providing access to all possible microstates in ASI and related nanomagnetic arrays. We demonstrate the creation of two previously elusive states; the spin-crystal ground state of dipolar kagome ASI and high-energy, low-entropy 'monopole-chain' states exhibiting negative effective temperatures.

We study the effect of proton irradiation on Ba(Fe$_{0.96}$Co$_{0.04}$)$_2$As$_2$ superconducting single crystals from combined magnetisation and magnetoresistivity measurements. The study allows the extraction of the values of the apparent pinning energy $U_0$ of the samples prior to and after irradiation, as well as comparison of the values of $U_0$ obtained from the flux-flow reversible region with those from the flux-creep irreversible region. Irradiation reduces $T_c$ modestly, but significantly reduces $U_0$ in both regimes: the critical current density $J_c$ is modified, most strikingly by the disappearance of the second magnetisation peak after irradiation. Analysis of the functional form of the pinning force and of the temperature dependence of $J_c$ for zero field, indicates that proton irradiation in this case has not changed the pinning regime, but has introduced a high density of shallow point-like defects. By consideration of a model that takes into account the effect of disorder on the irreversibility line, the data suggests that irradiation produced a considerable reduction in the average effective disorder overall, consistent with the changes observed in $U_0$ and $J_c$., Comment: 5 pages 7 figures

As charge carriers traverse a single superconductor ferromagnet interface they experience an additional spin-dependent phase angle which results in spin mixing and the formation of a bound state called the Andreev Bound State. This state is an essential component in the generation of long range spin triplet proximity induced superconductivity and yet the factors controlling the degree of spin mixing and the formation of the bound state remain elusive. Here we demonstrate that point contact Andreev reflection can be used to detect the bound state and extract the resulting spin mixing angle. By examining spectra taken from La1.15Sr1.85Mn2O7 single crystal - Pb junctions, together with a compilation of literature data on highly spin polarised systems, we show that the existence of the Andreev Bound State both resolves a number of long standing controversies in the Andreev literature as well as defining a route to quantify the strength of spin mixing at superconductor-ferromagnet interfaces. Intriguingly we find that for these high transparency junctions, the spin mixing angle appears to take a relatively narrow range of values across all the samples studied. The ferromagnets we have chosen to study share a common property in terms of their spin arrangement, and our observations may point to the importance of this property in determining the spin mixing angle under these circumstances., Comment: 17 pages, 1 table, 3 figures. arXiv admin note: substantial text overlap with arXiv:1503.00533

Realising the promise of next-generation magnetic nanotechnologies is contingent on the development of novel methods for controlling magnetic states at the nanoscale. There is currently demand for simple and flexible techniques to access exotic magnetisation states without convoluted fabrication and application processes. 360 degree domain walls (metastable twists in magnetisation separating two domains with parallel magnetisation) are one such state, which is currently of great interest in data storage and magnonics. Here, we demonstrate a straightforward and powerful process whereby a moving magnetic charge, provided experimentally by a magnetic force microscope tip, can write and manipulate magnetic charge states in ferromagnetic nanowires. The method is applicable to a wide range of nanowire architectures with considerable benefits over existing techniques. We confirm the method's efficacy via the injection and spatial manipulation of 360 degree domain walls in Py and Co nanowires. Experimental results are supported by micromagnetic simulations of the tip-nanowire interaction., Comment: in Scientific Reports (2016)

We investigate a series of manganese oxides, the La0.225Pr0.4(Ca1-xSrx)0.375MnO3 system. The x = 0 sample is a prototype compound for the study of phase separation in manganites, where ferromagnetic and charge ordered antiferromagnetic phases coexist. Replacing Ca2+ by Sr2+ gradually turns the system into a homogeneous ferromagnet. Our results show that the material structure plays a major role in the observed magnetic properties. On cooling, at temperatures below 100 K, a strong contraction of the lattice is followed by an increase in the magnetization. This is observed both through thermal expansion and magnetostriction measurements, providing distinct evidence of magneto-elastic coupling in these phase separated compounds.

The effect of the short milling times on R5(Si,Ge)4 R =Gd, Tb magnetocaloric material properties was investigated. In particular, the effect of milling on atomic structure, particles size and morphology, magnetic, and magnetocaloric effect was studied. With short milling times (< 2.5h), a reduction of the Gd5Si1.3Ge2.7 and Tb5Si2Ge2 particles size was achieved down to approximately 3.5 DSm. For both compositions the main differences are a consequence of the milling effect on the coupling of the structural and magnetic transitions. In the Gd5Si1.3Ge2.7 case, a second-order phase transition emerges at high temperatures as a result of ball milling. Consequently, there is a decrease in the magnetocaloric effect of 35% after 150 minutes of milling. Interestingly, an opposite effect is observed in Tb5Si2Ge2 where a 23% increase of the magnetocaloric effect was achieved, driven by the enhancement of the coupling between magnetic and structural transitions arising from internal strain promoted by the milling process., Comment: 15 pages, 6 figures, Submitted to Materials & Design

Vortex dynamics in a multiband anisotropic superconducting such as the Fe based superconductors, is interesting and potentially important for applications. In this study we examine flux-creep data for fields along the second magnetization peak observed in M(H) curves of BaFe$_{1.9}$Ni$_{0.1}$As$_2$ for H//c-axis, H//ab$-planes and H forming a 45$^o$ angle with ab-planes. We find that the M-H loops taken from the different field directions can be collapsed onto a single universal curve at all temperatures with a simple scaling factor equivalent to the superconducting anisotropy, showing not only that the vortex pinning is isotropic, three dimensional and most likely related to point like defects. The resulting critical currents however, taken from the Bean model appears to show enhanced low field pinning for H//c. The features in the vortex- dynamics also differ in different field orientations and show no direct correlation with the second magnetization peak Hp as is the case with a direct crossover in pinning regimes. Isofield plots of the scaled activation energy obtained from flux-creep data is found to be a smooth function of temperature as the Hp(T) line is crossed consistent with a single type of pinning regime operating at this field, independent of field orientation. The functional form of the Hp(T) lines in the resulting phase diagrams also support this view., Comment: 6 pages, 6 figures. arXiv admin note: substantial text overlap with arXiv:1209.1594

Manganites are one of only a small number of material families currently being trialled as room temperature magnetic refrigerants. Here we examine the dependence of the thermal conductivity, K, of La0.67Ca0.33MnO3+/-{\delta} as a function of density, grain size and silver impregnation around room temperature. We use a simple effective medium model to extract relevant trends in the data and demonstrate a threefold increase in thermal conductivity by silver impregnation., Comment: 4 pages, 4 figures

Flux-creep data was obtained for fields along the second magnetization peak observed in M(H) curves of BaFe{1.9}Ni{0.1}As2 for H||c-axis. H||ab-planes and H forming a 45 degrees angle with ab-planes. The M-H loops from the different field directions can be collapsed onto a universal curve with a scaling factor equivalent to the superconducting anisotropy, showing that the pinning is three dimensional, although with remarkable differences in the vortex-dynamics as a function of field orientation. The resulting relaxation rate, R, when plotted as a function of field and temperature does not show any specific feature in the vicinity of the second magnetization peak field Hp, the relaxation shows a maximum at a field H_2 well above Hp for H||c and a minimum at H^* for fields well below Hp for H||ab$ and H$-45-ab. Isofield plots of the scaled activation energy obtained from flux-creep data at several different temperatures also do not show any evidence of a change in the pinning mechanism as the peak field is crossed. The Hp lines in the resulting phase diagrams do not appear to be consistent with a description-terms of a collective-plastic pinning crossover., Comment: 4 pages, 5 figures

We report the room temperature observation of significant ballistic electron transport in shallow etched four-terminal mesoscopic devices fabricated on an InSb/AlInSb quantum well (QW) heterostructure with a crucial partitioned growth-buffer scheme. Ballistic electron transport is evidenced by a negative bend resistance signature which is quite clearly observed at 295 K and at current densities in excess of 10$^{6}$ A/cm$^{2}$. This demonstrates unequivocally that by using effective growth and processing strategies, room temperature ballistic effects can be exploited in InSb/AlInSb QWs at practical device dimensions.

We study the vortex-dynamics of a BaFe{1.82}Ni_{0.18}As_2 crystal with Tc = 8 K, by measuring flux-creep over the second magnetisation (or fish-tail) peak for both H//c-axis and H//ab planes. Magnetic relaxation data show an anomalously long initial stage of relaxation, lasting approximately10 minutes for H//c-axis and 2-3 min for H//ab, resembling a transient effect with a lower relaxation rate, which is followed by the usual log(time) relaxation. Interestingly, study of the relaxation rate R vs H for both stages of relaxation and for both field directions, are featureless over the field range associated with the fish-tail. The same trend was confirmed by plotting R vs T obtained from flux-creep data measured as a function of temperature for a fixed field (H//$c-axis). A plot of the activation energy U(M,T) calculated from the time relaxation of the magnetisation at a fixed field also shows a smooth behavior further supporting the view that the fish-tail peak is not associated with a crossover in vortex pinning regime within the collective pinning scenario., Comment: 4 pages, 4 figures

We describe the influence of hard wall confinement and lateral dimension on the low temperature transport properties of long diffusive channels and ballistic crosses fabricated in an InSb/InxAl1-xSb heterostructure. Partially diffuse boundary scattering is found to play a crucial role in the electron dynamics of ballistic crosses and substantially enhance the negative bend resistance. Experimental observations are supported by simulations using a classical billiard ball model for which good agreement is found when diffuse boundary scattering is included., Comment: 10 pages, 7 figures

We report on isofield magnetic relaxation data on a single crystal of $Ba_{1-x}K_xFe_2As_2$ with superconducting transition temperature $T_c$= 32.7 K which exhibit the so called fish-tail effect. A surface map of the superconducting transition temperature shows that the superconducting properties are close to homogeneous across the sample. Magnetic relaxation data, M(t), was used to obtain the activation energy U(M) in order to study different vortex dynamics regimes. Results of this analysis along with time dependent measurements as a function of field and temperature extended to the reversible region of some M(H) curves demonstrate that the irreversibility as well the second magnetization peak position, $H_p(T)$, are time dependent and controlled by plastic motion of the vortex state. In the region delimited by a characteristic field Hon (well below $H_p$), and $H_p$, the vortex dynamics is controlled by collective pinning. For fields below Hon the activation energy, $U_0$, increases with field as expected for collective pinning, but the pinning mechanism is likely to be in the single vortex limit., Comment: 8 pages, 8 figures, one table

Point contact Andreev reflection spectra have been taken as a function of temperature and magnetic field on the polycrystalline form of the newly discovered iron-based superconductor Sr2ScFePO3. A zero bias conductance peak which disappears at the superconducting transition temperature, dominates all of the spectra. Data taken in high magnetic fields show that this feature survives until 7T at 2K and a flattening of the feature is observed in some contacts. Here we inspect whether these observations can be interpreted within a d-wave, or nodal order parameter framework which would be consistent with the recent theoretical model where the height of the P in the Fe-P-Fe plane is key to the symmetry of the superconductivity. However, in polycrystalline samples care must be taken when examining Andreev spectra to eliminate or take into account artefacts associated with the possible effects of Josephson junctions and random alignment of grains., Comment: Published version

Oxypnictide superconductor NdFeAsO0.85 sample was irradiated with 2 GeV Ta ions at a fluence of 5x10^10 ions/cm2. High resolution transmission electron microscopy study revealed that the irradiation produced columnar-like defects. The effect of these defects on the irreversible magnetisation in polycrystalline randomly oriented fragments was studied as a function of field angle and field sweep rate. We find that the critical current density is enhanced at fields below the matching field (~1 Tesla) but only marginally. The pinning enhancement is anisotropic and maximum along the defect direction at high temperatures but the pinning then becomes more isotropic at low temperatures. The creep rate is suppressed at high temperatures and at fields below the matching field, indicating the columnar defects are efficient pinning sites at these H and T conditions., Comment: 10 pages, 4 figures

We present high field magneto-transport data from a range of 30nm wide InSb/InAlSb quantum wells. The low temperature carrier mobility of the samples studied ranged from 18.4 to 39.5 m2V-1s-1 with carrier densities between 1.5x1015 and 3.28x1015 m-2. Room temperature mobilities are reported in excess of 6 m2V-1s-1. It is found that the Landau level broadening decreases with carrier density and beating patterns are observed in the magnetoresistance with non-zero node amplitudes in samples with the narrowest broadening despite the presence of a large g-factor. The beating is attributed to Rashba splitting phenomenon and Rashba coupling parameters are extracted from the difference in spin populations for a range of samples and gate biases. The influence of Landau level broadening and spin-dependent scattering rates on the observation of beating in the Shubnikov-de Haas oscillations is investigated by simulations of the magnetoconductance. Data with non-zero beat node amplitudes are accompanied by asymmetric peaks in the Fourier transform, which are successfully reproduced by introducing a spin-dependent broadening in the simulations. It is found that the low-energy (majority) spin up state suffers more scattering than the high-energy (minority) spin down state and that the absence of beating patterns in the majority of (lower density) samples can be attributed to the same effect when the magnitude of the level broadening is large.

Bulk samples of TbFeAsO$_{0.9}$F$_{0.1}$ (T$_{c}$(on) = 50K) were measured by point contact Andreev reflection spectroscopy. The spectra show unambiguous evidence for multiple gap-like features plus the presence of high bias shoulders. By measuring the spectra as a function of temperature with both gold and superconducting niobium tips, we establish that the gap-like features are associated with superconducting order parameter in this material. We discuss whether the well defined zero bias conductance peak that we observe infrequently is associated with a nodal superconducting order parameter., Comment: 11 pages, 5 figures, published version

Here we use global and local magnetometry and Hall probe imaging to investigate the electromagnetic connectivity of the superconducting current path in the oxygen-deficient fluorine-free Nd-based oxypnictides. High resolution transmission electron microscopy and scanning electron microscopy show strongly-layered crystallites, evidence for a ~ 5nm amorphous oxide around individual particles, and second phase neodymium oxide which may be responsible for the large paramagnetic background at high field and at high temperatures. From global magnetometry and electrical transport measurements it is clear that there is a small supercurrent flowing on macroscopic sample dimensions (mm), with a lower bound for the average (over this length scale) critical current density of the order of 103 A/cm2. From magnetometry of powder samples and local Hall probe imaging of a single large conglomerate particle ~120 microns it is clear that on smaller scales, there is better current connectivity with a critical current density of the order of 5 x 104 A/cm2. We find enhanced flux creep around the second peak anomaly in the magnetisation curve and an irreversibility line significantly below Hc2(T) as determined by ac calorimetry., Comment: 11 pages, 4 figures

The newly discovered oxypnictide family of superconductors show very high critical temperatures of up to 55K. Whilst there is growing evidence that suggests a nodal order parameter, point contact Andreev reflection spectroscopy can provide crucial information such as the gap value and possibly the number of energy gaps involved. For the oxygen deficient NdFeAsO0.85 with a Tc of 45.5K, we show that there is clearly a gap value at 4.2K that is of the order of 7meV, consistent with previous studies on oxypnictides with lower Tc. Additionally, taking the spectra as a function of gold tip contact pressure reveals important changes in the spectra which may be indicative of more complex physics underlying this structure., Comment: 11 pages, 3 figures. New references included, extra discussion. This version is accepted in Superconductor Science and Technology

Here we use highly sensitive magnetisation measurements performed using a Hall probe sensor on single crystals of highly anisotropic high temperature superconductors $Bi_{2}Sr_{2}CaCu_{2}O_{8}$ to study the dynamic interactions between the two species of vortices that exist in such superconductors. We observe a remarkable and clearly delineated high temperature regime that mirrors the underlying vortex phase diagram. Our results map out the parameter space over which these dynamic interaction processes can be used to create vortex ratchets, pumps and other fluxonic devices., Comment: 7 pages, 3 figures, to be published in Supercond. Sci. Technol

The spin-orbit (SO) coupling parameters for lowest conduction subband due to structural (SIA) and bulk (BIA) inversion asymmetry are calculated for a range of carrier densities in [001]-grown delta-doped n-type InSb/In1-xAlxSb asymmetric quantum wells using the established 8 band k.p formalism [PRB 59,8 R5312 (1999)]. We present calculations for conditions of zero bias at 10 K. It is shown that both the SIA and BIA parameters scale approximately linearly with carrier density, and exhibit a marked dependence on well width when alloy composition is adjusted to allow maximum upper barrier height for a given well width. In contrast to other material systems the BIA contribution to spin splitting is found to be of significant and comparable value to the SIA mechanism in these structures. We calculate the spin lifetime for spins oriented along [11-0] based on D'yakonov-Perel mechanism using both the theory of Averkiev et al. [J. Phys.:Condens. Matter 14 (2002)] and also the rate of precession of spins about the effective magnetic field, taking into account all three SO couplings, showing good agreement.Spin lifeime for this direction is largest in the narrow wells over the range of moderate carrier densities considered, which is attributed to the reduced magnitude of the k-cubic BIA parameter in narrow wells. The inherently large BIA induced SO coupling in these systems is shown to have considerable effect on the spin lifetime, which exhibits significant reduction in the maximum spin lifetime compared to previous studies which consider systems with relatively weak BIA induced SO coupling. The relaxation rate of spins oriented in the [001] direction is dominated by the k-linear SIA and BIA coupling parameters and at least an order of magnitude greater than in the [11-0] direction., Comment: 18 pages 12 figures

Electromagnetic metamaterials are a class of materials which have been artificially structured on a subwavelength scale. They are currently the focus of a great deal of interest because they allow access to previously unrealisable properties like a negative refractive index. Most metamaterial designs have so far been based on resonant elements, like split rings, and research has concentrated on microwave frequencies and above. In this work, we present the first experimental realisation of a non-resonant metamaterial designed to operate at zero frequency. Our samples are based on a recently-proposed template for an anisotropic magnetic metamaterial consisting of an array of superconducting plates. Magnetometry experiments show a strong, adjustable diamagnetic response when a field is applied perpendicular to the plates. We have calculated the corresponding effective permeability, which agrees well with theoretical predictions. Applications for this metamaterial may include non-intrusive screening of weak DC magnetic fields., Comment: 6 pages, 3 figures

We report on the synthesis of highly oriented a-axis CrO2 films onto (0001) sapphire by atmospheric pressure CVD from CrO3 precursor, at growth temperatures down to 330 degree Celsius, i.e. close to 70 degrees lower than in published data for the same chemical system. The films keep the high quality magnetic behaviour as those deposited at higher temperature, which can be looked as a promising result in view of their use with thermally sensitive materials, e.g. narrow band gap semiconductors., Comment: 13 pages, 4 figures

We present an in-depth analysis of the experimental estimation of cross sections in Surface Enhanced Raman Scattering (SERS) by vibrational pumping. The paper highlights the advantages and disadvantages of the technique, pinpoints the main aspects and limitations, and provides the underlying physical concepts to interpret the experimental results. Examples for several commonly used SERS probes are given, and a discussion on future possible developments is also presented., Comment: To be submitted to J. Phys. Chem. B

We provide conclusive demonstration of vibrational pumping under Surface Enhanced Raman Scattering (SERS) conditions by performing anti-Stokes/Stokes ratio measurements down to 10 K using dried silver colloids, the dye rhodamine 6G and 676 nm laser excitation. The method we propose allows the measurement of the SERS cross sections for different modes and the determination of the asymmetry between the anti-Stokes and Stokes SERS cross sections., Comment: 3 figures 4 pages submitted to Phys. Rev. Lett

We make systematic measurements of Raman anti-Stokes/Stokes (aS/S) ratios using two different laser excitations (514 and 633 nm) of rhodamine 6G (RH6G) on dried Ag colloids over a wide range of temperatures (100 to 350 K). We show that a temperature scan allows the separation of the contributions to the aS/S ratios from {\it resonance effects} and {\it heating/pumping}, thus decoupling the two main aspects of the problem. The temperature rise is found to be larger when employing the 633 nm laser. In addition, we find evidence for mode specific vibrational pumping at higher laser power densities. We analyze our results in the framework of ongoing discussion on laser heating/pumping under SERS conditions., Comment: 4 figures

We present a detailed study of the dynamic interactions between Josephson vortices and stacks of pancake vortices in a Bi2Sr2CaCu2O8 single crystal, obtained by measuring the effect of applied inplane magnetic field pulses on the c-axis magnetisation. The predominant interaction is to relax the system towards equilibrium. However, using a highly sensitive AC technique we are able to measure also the forces acting to drive the system away from equilibrium, consistent with the existence of dragging interactions between the Josephson and pancake systems. Such forces were discussed recently as the basis of possible flux ratchet devices., Comment: 4 pages, 4 figures

We demonstrate that the variation of the Andreev reflection with applied magnetic field provides a direct means of comparing the properties of MgB2 with the theory for a dirty two-band superconductor, and we find good agreement between the two. The ratio of electron diffusivities in the s and p bands can be inferred from this experiment. We find that the field dependence of the density of states at the Fermi level in the p band is independent of the field direction, and that the anisotropic upper critical field is determined by the anisotropic diffusivity in the s band.

Highly (001) oriented thin films of Co2MnSi have been grown on lattice matched GaAs(001) without a buffer layer. Stoichiometric films exhibited a saturation magnetization slightly reduced from the bulk value and films grown at the highest substrate temperature of 689 K showed the lowest resistivity (33 micro.ohm.cm at 4.2 K) and the lowest coercivity (14 Oe). The spin polarization of the transport current was found to be of the order of 55% as determined by point contact Andreev reflection spectroscopy. The reduced magnetization obtained was attributed to the antiferromagnetic Mn2As phase. Twofold in-plane magnetic anisotropy was observed due to the inequivalence of the <110> directions, and this was attributed to the nature of the bonding at the reconstructed GaAs surface., Comment: 15 pages, 4 figures

The Blonder-Tinkham-Klapwijk model of the Point-Contact Andreev Reflection spectroscopy does not provide an adequate description of experiment in the presence of magnetic field. We demonstrate this using a junction between a niobium tip and a copper film. We modify the the-ory to explicitly take into account the contribution to conductance that stems from the normal vortex cores in the superconductor. These results have important implications for interpretation of transport spin polarisation measurements using PCAR technique. We demonstrate that stray magnetic fields can be responsible for the experimentally observed dependence of the spin po-larisation on the strength of the interface barrier, and potential misassignment of the inferred spin polarisation., Comment: 4 pages PDF only

Two sets of MgB2 samples doped with up to 5 at. % of Al were prepared in different laboratories using different procedures. Decreases in the a and c lattice parameters were observed with Al doping confirming Al substitution onto the Mg site. The critical temperature (Tc) remained largely unchanged with Al doping. For 1 - 2.5 at.% doping, at 20K the in-field critical current densities (Jc's) were enhanced, particularly at lower fields. At 5K, in-field Jc was markedly improved, e.g. at 5T Jc was enhanced by a factor of 20 for a doping level of 1 at.% Al. The improved Jcs correlate with increased sample resistivity indicative of an increase in the upper critical field, Hc2, through alloying., Comment: 17 pages, 4 figures, to be published in Superconductor Science and Technology

First order ferromagnetic (FM) to antiferromagnetic (AFM) phase transition in doped-CeFe$_2$ alloys is studied with micro-Hall probe technique. Clear visual evidence of magnetic phase-coexistence on micrometer scales and the evolution of this phase-coexistence as a function of temperature, magnetic field and time across the first order FM-AFM transition is presented. Such phase-coexistence and metastability arise as natural consequence of an intrinsic disorder-influenced first order transition. Generality of this phenomena involving other classes of materials is discussed., Comment: 11 pages of text and 3 figures

Thin films of Co2MnSi have been grown on a-plane sapphire substrates from three elemental targets by dc magnetron co-sputtering. These films are single phase, have a strong (110) texture and a saturation magnetization of 4.95 uB/formula unit at 10 K. Films grown at the highest substrate temperature of 715 K showed the lowest resistivity (47 uOhm cm at 4.2 K) and the lowest coercivity (18 Oe). The spin polarization of the transport current was found to be of the order of 54% as determined by point contact Andreev reflection spectroscopy. A decrease in saturation magnetization with decreasing film thickness and different transport behaviour in thinner films indicate a graded disorder in these films grown on non-lattice matched substrates., Comment: 15 pages, 4 figures

We have performed a comparative study of two thin films of magnesium diboride (MgB2) grown by different techniques. The critical current density at different temperatures and magnetic fields was evaluated from magnetisation curves, the structure of superconducting order parameter was obtained from point-contact spectroscopy, and the scattering rates were evaluated by fitting the temperature dependent normal-state resistivity to the two-band model. The films have similar critical temperatures close to 39 K, but the upper critical fields were different by a factor of 2 (5.2T and 2.5 T at 20 K). We have found that the film with higher Hc2 also had stronger scattering in the sigma band and smaller value of the superconducting gap in this band. As the scattering in sigma band is primarily due to the defects in boron plane, our results are consistent with the assumption that disordering the boron planes leads to enhanced Hc2 and better pinning properties in magnetic field., Comment: Paper presented at EUCAS'03

Double-gap superconductivity in an epitaxial MgB2 film has been studied by means of point-contact spectroscopy in magnetic field up to 8 Tesla. The relatively fast disappearance of the feature associated with the pi-band gap at a field around 1 T is caused by the line broadening due to strong pair breaking rather than to a collapse of the double-gap state. This pair breaking was found to increase linearly with field. Field dependences of the order parameters Delta_pi and Delta_sigma in the pi and sigma bands were measured in field applied parallel and perpendicular to the film, at T = 4.2 K. In perpendicular field, both order parameters survive to a common Hc2, which is about 6.5 T for this direction. In parallel field, the decrease of Delta_sigma is much more gradual, consistent with the Hc2 being about 4 times greater in this ori-entation. The difference in Delta_pi measured in the two field orientations is however smaller than the difference of Delta_sigma. We compare these results with the data on tunnelling spectroscopy and specific heat measurements of MgB2 single crystals and find consistency between the different experimental approaches., Comment: 4 pages, 5 figures Revised: discussion of the distribution of gap values

With the aim of probing the effect of magnetic disorder in the low-temperature excitations of manganites, specific-heat measurements were performed in zero field, and in magnetic fields up to 9 T in polycrystalline samples of La_{0.7-x}Y_{x}Ca_{0.3}MnO_{3}, with Y concentrations x=0, 0.10, and 0.15. Yttrium doping yielded the appearance of a cluster-glass state, giving rise to unusual low-temperature behavior of the specific-heat. The main feature observed in the results is a strong enhancement of the specific-heat linear term, which is interpreted as a direct consequence of magnetic disorder. The analysis was further corroborated by resistivity measurements in the same compounds., Comment: 9 pages, 2 figures

We present magnetisation data on crystalline and polycrystalline MgB2 before and after irradiation with ~1MeV protons. In the virgin crystal the critical current density is below our noise floor of 103A/cm2 over most of the field range. However, after irradiation a peak occurs in the current density as a function of applied magnetic field as the upper critical field Hc2 is approached. After subsequent ageing over a time period of three months, the peak effect is greatly enhanced, exhibiting much stronger pinning over a wide field range, and the upper critical field is approximately doubled, accompanied by a 2K reduction in transition temperature. Similar studies were made on polycrystalline fragments, where irradiation leads to an increased irreversibility field (Jc is enhanced at high fields but decreased at low fields) and a suppression in transition temperature. However, after two years of ageing both parameters returned towards those of the virgin sample., Comment: 18 pages 4 figs

The two tone intermodulation arising in MgB2 thin films deposited in-situ by planar magnetron sputtering on sapphire substrates is studied. Samples are characterised using an open-ended dielectric puck resonator operating at 8.8 GHz. The experimental results show that the third order products increase with the two-tone input power with a slope ranging between 1.5 and 2.3. The behaviour can be understood introducing a mechanism of vortex penetration in grain boundaries as the most plausible source of non linearities in these films. This assumption is confirmed by the analysis of the field dependence of the surface resistance, that show a linear behaviour at all temperatures under test., Comment: 13 pages, 3 figures; to be published in Appl. Phys. Lett

We review recent measurements of upper (Hc2) and lower (Hc1) critical fields in clean single crystals of MgB2, and their anisotropies between the two principal crystallographic directions. Such crystals are far into the "clean limit" of Type II superconductivity, and indeed for fields applied in the c-direction, the Ginzburg-Landau parameter k is only about 3, just large enough for Type II behaviour. Because m0Hc2 is so low, about 3 T for fields in the c-direction, MgB2 has to be modified for it to become useful for high-current applications. It should be possible to increase Hc2 by the introduction of strong electron scattering (but because of the electronic structure and the double gap that results, the scatterers will have to be chosen carefully). In addition, pinning defects on a scale of a few nm will have to be engineered in order to enhance the critical current density at high fields., Comment: BOROMAG Conference Invited paper. To appear in Supercond. Sci. Tech

We discuss pinning properties of MgB2 thin films grown by pulsed-laser deposition (PLD) and by electron-beam (EB) evaporation. Two mechanisms are identified that contribute most effectively to the pinning of vortices in randomly oriented films. The EB process produces low defected crystallites with small grain size providing enhanced pinning at grain boundaries without degradation of Tc. The PLD process produces films with structural disorder on a scale less that the coherence length that further improves pinning, but also depresses Tc.

Despite the intense activity in the year since the discovery of superconductivity in MgB2, key parameters, in particular the upper and lower critical fields Hc2 and Hc1 and their anisotropies, are not well-established, largely because of the difficulty of growing MgB2 crystals. Attempts have been made to deduce these parameters from experiments on polycrystalline material, but they have substantial uncertainties. Hc2 is particularly important for applications, as it is the field which quenches bulk super-conductivity. In terms of understanding MgB2, it is now clear that the conventional electron-phonon interaction is strong enough to account for the high transition temperature Tc, but the consequences of the double super-conducting gap for the anisotropy and its dependence on temperature, are uncertain. Here we describe detailed direct measurements of Hc1(T) and Hc2(T) for the two principal crystallographic directions in a clean single crystal of MgB2. For fields in the c-direction, $\mu_0 H^c_{c1}(0)$ = $0.28 +- 0.01T$ and $\mu_0 H^c_{c2}(0)$ is $3 +- 0.5T$; this ratio of critical fields is rather low and implies that MgB2 is only just a Type II super-conductor. The anisotropies of both critical fields are close to 2., Comment: 3 pages 3 figures