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In this perspective, we discuss thermal imbalance and the associated electron-mediated thermal transport in quantum electronic devices at very low temperatures. We first present the theoretical approaches describing heat transport in nanoscale conductors at low temperatures, in which quantum confinement and interactions play an important role. We then discuss the experimental techniques for generating and measuring heat currents and temperature gradients on the nanoscale. Eventually we review the most important quantum effects on heat transport, and discuss implications for quantum technologies and future directions in the field., Comment: To appear in Appl. Phys. Lett. as a Perspective

We report a theoretical study of multiterminal Josephson junctions under the influence of a magnetic field $B$. We consider a ballistic rectangular two-dimensional metal $N_0$ connected by the edges to the left, right, top and bottom superconductors $S_L$, $S_R$, $S_T$ and $S_B$, respectively. We numerically calculate in the large-gap approximation the critical current $I_c$ versus $B$ between the left and right $S_L$ and $S_R$ for various aspect ratios, with the top and bottom $S_T$ and $S_B$ playing the role of superconducting mirrors. We find the critical current $I_c$ to be enhanced by orders of magnitude, especially at long distance, due to the phase rigidity provided by the mirrors. We obtain superconducting quantum interference device-like magnetic oscillations. With symmetric couplings, the self-consistent superconducting phase variables of the top and bottom mirrors take the values $0$ or $\pi$, as for emerging Ising degrees of freedom. We propose a simple effective Josephson junction circuit model that is compatible with these microscopic numerical calculations. From the $I_c(B)$ patterns we infer where the supercurrent flows in various device geometries. In particular in the elongated geometry, we show that the supercurrent flows between all pairs of contacts, which allows exploring the full phase space of the relevant phase differences., Comment: 15 pages, 6 figures, minor modifications

In this article we classify all $L_9$-free finite groups.

We study the interplay between Coulomb blockade and superconductivity in a tunable superconductor-superconductor-normal metal single-electron transistor. The device is realized by connecting the superconducting island via an oxide barrier to the normal metal lead and with a break junction to the superconducting lead. The latter enables Cooper pair transport and (multiple) Andreev reflection. We show that those processes are relevant also far above the superconducting gap and that signatures of Coulomb blockade may reoccur at high bias while they are absent for small bias in the strong-coupling regime. Our experimental findings agree with simulations using a master equation approach in combination with the full counting statistics of multiple Andreev reflection., Comment: Manuscript only, supplement available upon request

The multiterminal Josephson effect aroused considerable interest recently, in connection with theoretical and experimental evidence for correlations among Cooper pairs, that is, the so-called Cooper quartets. It was further predicted that the spectrum of Andreev bound states in such devices could host Weyl-point singularities. However, the relative phase between the Cooper pair and quartet supercurrents has not yet been addressed experimentally. Here, we propose an experiment involving four-terminal Josephson junctions with two independent orthogonal supercurrents, and calculate the critical current contours (CCCs) from a multiterminal Josephson junction circuit theory. We predict a generically $\pi$-shifted contribution of both the local or nonlocal second-order Josephson harmonics. Furthermore, we show that these lead to marked nonconvex shapes for the CCCs in zero magnetic field, where the dissipative state reenters into the superconducting one. Eventually, we discuss distinctive features of the non-local Josephson processes in the CCCs. The experimental observation of the latter could allow providing firm evidence of the $\pi$-shifted Cooper quartet current-phase relation., Comment: Third revision: manuscript in final form

Current flow in electronic devices can be asymmetric with bias direction, a phenomenon underlying the utility of diodes and known as non-reciprocal charge transport. The promise of dissipationless electronics has recently stimulated the quest for superconducting diodes, and non-reciprocal superconducting devices have been realized in various non-centrosymmetric systems. Probing the ultimate limits of miniaturization, we have created atomic-scale Pb--Pb Josephson junctions in a scanning tunneling microscope. Pristine junctions stabilized by a single Pb atom exhibit hysteretic behavior, confirming the high quality of the junctions, but no asymmetry between the bias directions. Non-reciprocal supercurrents emerge when inserting a single magnetic atom into the junction, with the preferred direction depending on the atomic species. Aided by theoretical modelling, we trace the non-reciprocity to quasiparticle currents flowing via Yu-Shiba-Rusinov (YSR) states inside the superconducting energy gap. Our results open new avenues for creating atomic-scale Josephson diodes and tuning their properties through single-atom manipulation.

Depinning of nanoscale magnetic textures, such as domain walls, vortices and skyrmions, is of paramount importance for magnetic storage and information processing. We measure time-resolved magnetic switching statistics of an individual, non-single-domain Fe$_3$O$_4$ nanoparticle using a micrometer-scale superconducting quantum interference device. Surprisingly, a strong narrowing of the waiting-time distributions before reaching the final state is observed as compared to the exponential distribution expected for a single barrier. The magnetization reversal across the nanostructure is thus shown to result from multiple serial barriers in the minimum energy pathway., Comment: 5 pages and suppl information available on request

When electrons populate a flat band their kinetic energy becomes negligible, forcing them to organize in exotic many-body states to minimize their Coulomb energy. The zeroth Landau level of graphene under magnetic field is a particularly interesting strongly interacting flat band because inter-electron interactions are predicted to induce a rich variety of broken-symmetry states with distinct topological and lattice-scale orders. Evidence for these stems mostly from indirect transport experiments that suggest that broken-symmetry states are tunable by boosting the Zeeman energy or by dielectric screening of the Coulomb interaction. However, confirming the existence of these ground states requires a direct visualization of their lattice-scale orders. Here, we image three distinct broken-symmetry phases in graphene using scanning tunneling spectroscopy. We explore the phase diagram by tuning the screening of the Coulomb interaction by a low or high dielectric constant environment, and with a magnetic field. In the unscreened case, we unveil a Kekul\'e bond order, consistent with observations of an insulating state undergoing a magnetic-field driven Kosterlitz-Thouless transition. Under dielectric screening, a sublattice-unpolarized ground state emerges at low magnetic fields, and transits to a charge-density-wave order with partial sublattice polarization at higher magnetic fields. The Kekul\'e and charge-density-wave orders furthermore coexist with additional, secondary lattice-scale orders that enrich the phase diagram beyond current theory predictions. This screening-induced tunability of broken-symmetry orders may prove valuable to uncover correlated phases of matter in other quantum materials., Comment: Main text + SI

Constriction-based Josephson weak-links display a thermal bi-stability between two states exhibiting zero and finite voltages. This manifests in experiments either as hysteresis in weak-links current voltage characteristics or as random telegraphic signal in voltage. In the latter case, a noise-driven amplification of a sinusoidal excitation of the device is observed, at frequencies matching the characteristic switching frequency in telegraphic signal, a phenomenon known as stochastic resonance. The observed behavior is understood using a two-state model of stochastic resonance and is exploited to illustrate an enhanced signal-to-noise-ratio in a micro-SQUID as a magnetic field sensor., Comment: 23 pages, 7 figures, suppl. info. available on request

Tunneling across superconducting junctions proceeds by a rich variety of processes, which transfer single electrons, Cooper pairs, or even larger numbers of electrons by multiple Andreev reflections. Photon-assisted tunneling combined with the venerable Tien-Gordon model has long been a powerful tool to identify tunneling processes between superconductors. Here, we probe superconducting tunnel junctions including an impurity-induced Yu-Shiba-Rusinov (YSR) state by exposing a scanning tunneling microscope with a superconducting tip to microwave radiation. We find that a simple Tien-Gordon description describes tunneling of single electrons and Cooper pairs into the bare substrate, but breaks down for tunneling via YSR states by resonant Andreev reflections. We develop an improved theoretical description which is in excellent agreement with the data. Our results establish photon-assisted tunneling as a powerful tool to analyze tunneling processes at the atomic scale which should be particularly informative for unconventional and topological superconductors.

Graphene's original promise to succeed silicon faltered due to pervasive edge disorder in lithographically patterned deposited graphene and the lack of a new electronics paradigm. Here we demonstrate that the annealed edges in conventionally patterned graphene epitaxially grown on a silicon carbide substrate (epigraphene) are stabilized by the substrate and support a protected edge state. The edge state has a mean free path that is greater than 50 microns, 5000 times greater that the bulk states and involves a theoretically unexpected Majorana-like zero-energy non-degenerate quasiparticle that does not produce a Hall voltage. In seamless integrated structures, the edge state forms a zero-energy one-dimensional ballistic network with essentially dissipationless nodes at ribbon-ribbon junctions. Seamless device structures offer a variety of switching possibilities including quantum coherent devices at low temperatures. This makes epigraphene a technologically viable graphene nanoelectronics platform that has the potential to succeed silicon nanoelectronics., Comment: File contains article and supplementary. Nature Communications (in print)

The quantum phase-coherent behavior of superconducting weak links (WL) is often quenched in the finite voltage state, due to the heat dissipation and related thermal hysteresis. The latter can be reduced by improving heat evacuation and/or by lowering the critical current, so that a phase-dynamic regime is obtained, albeit over a narrow bias-current and temperature range. Here we demonstrate that an inductive shunt with well-chosen parameters introduces unexpected nonlinear dynamics that destabilize an otherwise stable fixed point in the dissipative branch. This leads to a nonhysteretic behavior with large voltage oscillations in intrinsically hysteretic WL-based micron-size superconducting quantum interference devices. A dynamic thermal model quantitatively describes our observations and further allows us to elaborate on the optimal shunting conditions., Comment: The model section has been revised in the latest version, 9 pages, 11 figures

Micron-sized superconducting interference devices ($\mu$-SQUIDs) based on constrictions optimized for minimizing thermal runaway are shown to exhibit voltage oscillations with applied magnetic flux despite their hysteretic behavior. We explain this remarkable feature by a significant supercurrent contribution surviving deep into the resistive state, due to efficient heat evacuation. A resistively shunted junction model, complemented by a thermal balance determining the amplitude of the critical current, describes well all experimental observations, including the flux modulation of the (dynamic) retrapping current and voltage by introducing a single dimensionless parameter. Thus hysteretic $\mu$-SQUIDs can be operated in the voltage read-out mode with a faster response. The quantitative modeling of this regime incorporating both heating and phase dynamics paves the way for further optimization of $\mu$-SQUIDs for nano-magnetism., Comment: 10 pages, 11 figures, Revised

Future generations of photoelectrodes for solar fuel generation must employ inexpensive, earth-abundant absorber materials in order to provide a large-scale source of clean energy. These materials tend to have poor electrical transport properties and exhibit carrier diffusion lengths which are significantly shorter than the absorption depth of light. As a result, many photo-excited carriers are generated too far from a reactive surface, and recombine instead of participating in solar-to-fuel-conversion. We demonstrate that plasmonic resonances in metallic nanostructures and multi-layer interference effects can be engineered to strongly concentrate sunlight close to the electrode/liquid interface, precisely where the relevant reactions take place. By comparing spectral features in the enhanced photocurrent spectra to full-field electromagnetic simulations, the contribution of surface plasmon excitations is verified. These results open the door to the optimization of a wide variety of photochemical processes by leveraging the rapid advances in the field of plasmonics.