1. Absence of 3a0 charge density wave order in the infinite-layer nickelate NdNiO2
- Author
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Parzyck, CT, Gupta, NK, Wu, Y, Anil, V, Bhatt, L, Bouliane, M, Gong, R, Gregory, BZ, Luo, A, Sutarto, R, He, F, Chuang, Y-D, Zhou, T, Herranz, G, Kourkoutis, LF, Singer, A, Schlom, DG, Hawthorn, DG, and Shen, KM
- Subjects
Physical Sciences ,Condensed Matter Physics ,Nanoscience & Nanotechnology - Abstract
A hallmark of many unconventional superconductors is the presence of many-body interactions that give rise to broken-symmetry states intertwined with superconductivity. Recent resonant soft X-ray scattering experiments report commensurate 3a0 charge density wave order in infinite-layer nickelates, which has important implications regarding the universal interplay between charge order and superconductivity in both cuprates and nickelates. Here we present X-ray scattering and spectroscopy measurements on a series of NdNiO2+x samples, which reveal that the signatures of charge density wave order are absent in fully reduced, single-phase NdNiO2. The 3a0 superlattice peak instead originates from a partially reduced impurity phase where excess apical oxygens form ordered rows with three-unit-cell periodicity. The absence of any observable charge density wave order in NdNiO2 highlights a crucial difference between the phase diagrams of cuprate and nickelate superconductors.
- Published
- 2024