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1. Disentangling the evolution of electrons and holes in photoexcited ZnO nanoparticles

Author: Christopher J. Milne, Natalia Nagornova, Thomas Pope, Hui-Yuan Chen, Thomas Rossi, Jakub Szlachetko, Wojciech Gawelda, Alexander Britz, Tim B. van Driel, Leonardo Sala, Simon Ebner, Tetsuo Katayama, Stephen H. Southworth, Gilles Doumy, Anne Marie March, C. Stefan Lehmann, Melanie Mucke, Denys Iablonskyi, Yoshiaki Kumagai, Gregor Knopp, Koji Motomura, Tadashi Togashi, Shigeki Owada, Makina Yabashi, Martin M. Nielsen, Marek Pajek, Kiyoshi Ueda, Rafael Abela, Thomas J. Penfold, and Majed Chergui
Subjects: Crystallography, QD901-999
Abstract: The evolution of charge carriers in photoexcited room temperature ZnO nanoparticles in solution is investigated using ultrafast ultraviolet photoluminescence spectroscopy, ultrafast Zn K-edge absorption spectroscopy, and ab initio molecular dynamics (MD) simulations. The photoluminescence is excited at 4.66 eV, well above the band edge, and shows that electron cooling in the conduction band and exciton formation occur in
Published: 2023
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2. Pink-beam serial femtosecond crystallography for accurate structure-factor determination at an X-ray free-electron laser

Author: Karol Nass, Camila Bacellar, Claudio Cirelli, Florian Dworkowski, Yaroslav Gevorkov, Daniel James, Philip J. M. Johnson, Demet Kekilli, Gregor Knopp, Isabelle Martiel, Dmitry Ozerov, Alexandra Tolstikova, Laura Vera, Tobias Weinert, Oleksandr Yefanov, Jörg Standfuss, Sven Reiche, and Christopher J. Milne
Subjects: pink beams, serial femtosecond crystallography, de novo protein structure determination, single-wavelength anomalous diffraction, xfels, large bandwidths, data-quality indicators, Crystallography, QD901-999
Abstract: Serial femtosecond crystallography (SFX) at X-ray free-electron lasers (XFELs) enables essentially radiation-damage-free macromolecular structure determination using microcrystals that are too small for synchrotron studies. However, SFX experiments often require large amounts of sample in order to collect highly redundant data where some of the many stochastic errors can be averaged out to determine accurate structure-factor amplitudes. In this work, the capability of the Swiss X-ray free-electron laser (SwissFEL) was used to generate large-bandwidth X-ray pulses [Δλ/λ = 2.2% full width at half-maximum (FWHM)], which were applied in SFX with the aim of improving the partiality of Bragg spots and thus decreasing sample consumption while maintaining the data quality. Sensitive data-quality indicators such as anomalous signal from native thaumatin micro-crystals and de novo phasing results were used to quantify the benefits of using pink X-ray pulses to obtain accurate structure-factor amplitudes. Compared with data measured using the same setup but using X-ray pulses with typical quasi-monochromatic XFEL bandwidth (Δλ/λ = 0.17% FWHM), up to fourfold reduction in the number of indexed diffraction patterns required to obtain similar data quality was achieved. This novel approach, pink-beam SFX, facilitates the yet underutilized de novo structure determination of challenging proteins at XFELs, thereby opening the door to more scientific breakthroughs.
Published: 2021
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3. Advances in long-wavelength native phasing at X-ray free-electron lasers

Author: Karol Nass, Robert Cheng, Laura Vera, Aldo Mozzanica, Sophie Redford, Dmitry Ozerov, Shibom Basu, Daniel James, Gregor Knopp, Claudio Cirelli, Isabelle Martiel, Cecilia Casadei, Tobias Weinert, Przemyslaw Nogly, Petr Skopintsev, Ivan Usov, Filip Leonarski, Tian Geng, Mathieu Rappas, Andrew S. Doré, Robert Cooke, Shahrooz Nasrollahi Shirazi, Florian Dworkowski, May Sharpe, Natacha Olieric, Camila Bacellar, Rok Bohinc, Michel O. Steinmetz, Gebhard Schertler, Rafael Abela, Luc Patthey, Bernd Schmitt, Michael Hennig, Jörg Standfuss, Meitian Wang, and Christopher J. Milne
Subjects: serial femtosecond crystallography, x-ray free-electron lasers, single-wavelength anomalous diffraction, de novo protein structure determination, anomalous data-quality indicators, Crystallography, QD901-999
Abstract: Long-wavelength pulses from the Swiss X-ray free-electron laser (XFEL) have been used for de novo protein structure determination by native single-wavelength anomalous diffraction (native-SAD) phasing of serial femtosecond crystallography (SFX) data. In this work, sensitive anomalous data-quality indicators and model proteins were used to quantify improvements in native-SAD at XFELs such as utilization of longer wavelengths, careful experimental geometry optimization, and better post-refinement and partiality correction. Compared with studies using shorter wavelengths at other XFELs and older software versions, up to one order of magnitude reduction in the required number of indexed images for native-SAD was achieved, hence lowering sample consumption and beam-time requirements significantly. Improved data quality and higher anomalous signal facilitate so-far underutilized de novo structure determination of challenging proteins at XFELs. Improvements presented in this work can be used in other types of SFX experiments that require accurate measurements of weak signals, for example time-resolved studies.
Published: 2020
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4. Femtosecond X-ray emission study of the spin cross-over dynamics in haem proteins

Author: Dominik Kinschel, Camila Bacellar, Oliviero Cannelli, Boris Sorokin, Tetsuo Katayama, Giulia F. Mancini, Jérémy R. Rouxel, Yuki Obara, Junichi Nishitani, Hironori Ito, Terumasa Ito, Naoya Kurahashi, Chika Higashimura, Shotaro Kudo, Theo Keane, Frederico A. Lima, Wojciech Gawelda, Peter Zalden, Sebastian Schulz, James M. Budarz, Dmitry Khakhulin, Andreas Galler, Christian Bressler, Christopher J. Milne, Thomas Penfold, Makina Yabashi, Toshinori Suzuki, Kazuhiko Misawa, and Majed Chergui
Subjects: Science
Abstract: The change from low-spin hexacoordinated to high-spin pentacoordinated domed form in heam upon ligand detachment and the reverse process underlie the respiratory function. The authors, using femtosecond time-resolved X-ray emission spectroscopy, capture the transient states connecting the two forms in myoglobin-NO upon NO photoinduced detachment.
Published: 2020
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5. Taking a snapshot of the triplet excited state of an OLED organometallic luminophore using X-rays

Author: Grigory Smolentsev, Christopher J. Milne, Alexander Guda, Kristoffer Haldrup, Jakub Szlachetko, Nicolo Azzaroli, Claudio Cirelli, Gregor Knopp, Rok Bohinc, Samuel Menzi, Georgios Pamfilidis, Dardan Gashi, Martin Beck, Aldo Mozzanica, Daniel James, Camila Bacellar, Giulia F. Mancini, Andrei Tereshchenko, Victor Shapovalov, Wojciech M. Kwiatek, Joanna Czapla-Masztafiak, Andrea Cannizzo, Michela Gazzetto, Mathias Sander, Matteo Levantino, Victoria Kabanova, Elena Rychagova, Sergey Ketkov, Marian Olaru, Jens Beckmann, and Matthias Vogt
Subjects: Science
Abstract: OLED materials based on thermally activated delayed fluorescence have promising efficiency. Here, the authors investigate an organometallic multicore Cu complex as luminophore, by pump-probe X-ray techniques at three different facilities deriving a complete picture of the charge transfer in the triplet excited state.
Published: 2020
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6. Tracking multiple components of a nuclear wavepacket in photoexcited Cu(I)-phenanthroline complex using ultrafast X-ray spectroscopy

Author: Tetsuo Katayama, Thomas Northey, Wojciech Gawelda, Christopher J. Milne, György Vankó, Frederico A. Lima, Rok Bohinc, Zoltán Németh, Shunsuke Nozawa, Tokushi Sato, Dmitry Khakhulin, Jakub Szlachetko, Tadashi Togashi, Shigeki Owada, Shin-ichi Adachi, Christian Bressler, Makina Yabashi, and Thomas J. Penfold
Subjects: Science
Abstract: Nonadiabatic excited state processes involve mixing of electronic and nuclear wavefunctions, which are difficult to disentangle. Here the authors explore by time-resolved X-ray absorption near edge structure the wavepacket dynamics of a copper(I)-phenanthroline complex, resolving different vibrational modes.
Published: 2019
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7. Revealing hole trapping in zinc oxide nanoparticles by time-resolved X-ray spectroscopy

Author: Thomas J. Penfold, Jakub Szlachetko, Fabio G. Santomauro, Alexander Britz, Wojciech Gawelda, Gilles Doumy, Anne Marie March, Stephen H. Southworth, Jochen Rittmann, Rafael Abela, Majed Chergui, and Christopher J. Milne
Subjects: Science
Abstract: Metal-oxide nanostructures are used in a range of light-driven applications, yet the fundamentals behind their properties are poorly understood. Here the authors probe photoexcited zinc oxide nanoparticles using time-resolved X-ray spectroscopy, identifying photocatalytically-active hole traps as oxygen vacancies in the lattice.
Published: 2018
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8. Demonstration of femtosecond X-ray pump X-ray probe diffraction on protein crystals

Author: Nadia L. Opara, Istvan Mohacsi, Mikako Makita, Daniel Castano-Diez, Ana Diaz, Pavle Juranić, May Marsh, Alke Meents, Christopher J. Milne, Aldo Mozzanica, Celestino Padeste, Valérie Panneels, Marcin Sikorski, Sanghoon Song, Henning Stahlberg, Ismo Vartiainen, Laura Vera, Meitian Wang, Philip R. Willmott, and Christian David
Subjects: Crystallography, QD901-999
Abstract: The development of X-ray free-electron lasers (XFELs) has opened the possibility to investigate the ultrafast dynamics of biomacromolecules using X-ray diffraction. Whereas an increasing number of structures solved by means of serial femtosecond crystallography at XFELs is available, the effect of radiation damage on protein crystals during ultrafast exposures has remained an open question. We used a split-and-delay line based on diffractive X-ray optics at the Linac Coherent Light Source XFEL to investigate the time dependence of X-ray radiation damage to lysozyme crystals. For these tests, crystals were delivered to the X-ray beam using a fixed-target approach. The presented experiments provide probe signals at eight different delay times between 19 and 213 femtoseconds after a single pump event, thereby covering the time-scales relevant for femtosecond serial crystallography. Even though significant impact on the crystals was observed at long time scales after exposure with a single X-ray pulse, the collected diffraction data did not show significant signal reduction that could be assigned to beam damage on the crystals in the sampled time window and resolution range. This observation is in agreement with estimations of the applied radiation dose, which in our experiment was clearly below the values expected to cause damage on the femtosecond time scale. The experiments presented here demonstrate the feasibility of time-resolved pump-multiprobe X-ray diffraction experiments on protein crystals.
Published: 2018
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9. Opportunities for Chemistry at the SwissFEL X-ray Free Electron Laser

Author: Christopher J. Milne, Peter Radi, Bill Pedrini, Henrik Lemke, Gregor Knopp, Pavle Juranic, Gerhard Ingold, Christoph P. Hauri, Uwe Flechsig, Rolf Follath, Christian Erny, Yunpei Deng, Paul Beaud, and Luc Patthey
Subjects: Swissfel, X-ray free electron laser, Chemistry, QD1-999
Abstract: X-ray techniques have long been applied to chemical research, ranging from powder diffraction tools to analyse material structure to X-ray fluorescence measurements for sample composition. The development of high-brightness, accelerator-based X-ray sources has allowed chemists to use similar techniques but on more demanding samples and using more photon-hungry methods. X-ray Free Electron Lasers (XFELs) are the latest in the development of these large-scale user facilities, opening up new avenues of research and the possibility of more advanced applications for a range of research. The SwissFEL XFEL project at the Paul Scherrer Institute will begin user operation in the hard X-ray (2.1–12.4 keV) photon energy range in 2018 with soft X-ray (240–1930 eV) user operation to follow and here we will present the details of this project, it's operating capabilities, and some aspects of the experimental stations that will be particularly attractive for chemistry research. SwissFEL is a revolutionary new machine that will complement and extend the time-resolved chemistry efforts in the Swiss research community.
Published: 2017
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10. A Dispersive Inelastic X-ray Scattering Spectrometer for Use at X-ray Free Electron Lasers

Author: Jakub Szlachetko, Maarten Nachtegaal, Daniel Grolimund, Gregor Knopp, Sergey Peredkov, Joanna Czapla–Masztafiak, and Christopher J. Milne
Subjects: dispersive X-ray spectrometer, von Hamos geometry, inelastic X-ray scattering, X-ray free electron laser, SwissFEL, segmented crystal, Technology, Engineering (General). Civil engineering (General), TA1-2040, Biology (General), QH301-705.5, Physics, QC1-999, Chemistry, QD1-999
Abstract: We report on the application of a short working distance von Hamos geometry spectrometer to measure the inelastic X-ray scattering (IXS) signals from solids and liquids. In contrast to typical IXS instruments where the spectrometer geometry is fixed and the incoming beam energy is scanned, the von Hamos geometry allows measurements to be made using a fixed optical arrangement with no moving parts. Thanks to the shot-to-shot capability of the spectrometer setup, we anticipate its application for the IXS technique at X-ray free electron lasers (XFELs). We discuss the capability of the spectrometer setup for IXS studies in terms of efficiency and required total incident photon flux for a given signal-to-noise ratio. The ultimate energy resolution of the spectrometer, which is a key parameter for IXS studies, was measured to the level of 150 meV at short crystal radius thanks to the application of segmented crystals for X-ray diffraction. The short working distance is a key parameter for spectrometer efficiency that is necessary to measure weak IXS signals.
Published: 2017
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11. SwissFEL: The Swiss X-ray Free Electron Laser

Author: Christopher J. Milne, Thomas Schietinger, Masamitsu Aiba, Arturo Alarcon, Jürgen Alex, Alexander Anghel, Vladimir Arsov, Carl Beard, Paul Beaud, Simona Bettoni, Markus Bopp, Helge Brands, Manuel Brönnimann, Ingo Brunnenkant, Marco Calvi, Alessandro Citterio, Paolo Craievich, Marta Csatari Divall, Mark Dällenbach, Michael D’Amico, Andreas Dax, Yunpei Deng, Alexander Dietrich, Roberto Dinapoli, Edwin Divall, Sladana Dordevic, Simon Ebner, Christian Erny, Hansrudolf Fitze, Uwe Flechsig, Rolf Follath, Franziska Frei, Florian Gärtner, Romain Ganter, Terence Garvey, Zheqiao Geng, Ishkhan Gorgisyan, Christopher Gough, Andreas Hauff, Christoph P. Hauri, Nicole Hiller, Tadej Humar, Stephan Hunziker, Gerhard Ingold, Rasmus Ischebeck, Markus Janousch, Pavle Juranić, Mario Jurcevic, Maik Kaiser, Babak Kalantari, Roger Kalt, Boris Keil, Christoph Kittel, Gregor Knopp, Waldemar Koprek, Henrik T. Lemke, Thomas Lippuner, Daniel Llorente Sancho, Florian Löhl, Carlos Lopez-Cuenca, Fabian Märki, Fabio Marcellini, Goran Marinkovic, Isabelle Martiel, Ralf Menzel, Aldo Mozzanica, Karol Nass, Gian Luca Orlandi, Cigdem Ozkan Loch, Ezequiel Panepucci, Martin Paraliev, Bruce Patterson, Bill Pedrini, Marco Pedrozzi, Patrick Pollet, Claude Pradervand, Eduard Prat, Peter Radi, Jean-Yves Raguin, Sophie Redford, Jens Rehanek, Julien Réhault, Sven Reiche, Matthias Ringele, Jochen Rittmann, Leonid Rivkin, Albert Romann, Marie Ruat, Christian Ruder, Leonardo Sala, Lionel Schebacher, Thomas Schilcher, Volker Schlott, Thomas Schmidt, Bernd Schmitt, Xintian Shi, Markus Stadler, Lukas Stingelin, Werner Sturzenegger, Jakub Szlachetko, Dhanya Thattil, Daniel M. Treyer, Alexandre Trisorio, Wolfgang Tron, Seraphin Vetter, Carlo Vicario, Didier Voulot, Meitian Wang, Thierry Zamofing, Christof Zellweger, Riccardo Zennaro, Elke Zimoch, Rafael Abela, Luc Patthey, and Hans-Heinrich Braun
Subjects: X-ray free electron laser, linac, X-rays, undulator, SwissFEL, X-ray optics, X-ray photon diagnostics, ultrafast X-ray science, X-ray detector, JUNGFRAU, serial femtosecond crystallography, Technology, Engineering (General). Civil engineering (General), TA1-2040, Biology (General), QH301-705.5, Physics, QC1-999, Chemistry, QD1-999
Abstract: The SwissFEL X-ray Free Electron Laser (XFEL) facility started construction at the Paul Scherrer Institute (Villigen, Switzerland) in 2013 and will be ready to accept its first users in 2018 on the Aramis hard X-ray branch. In the following sections we will summarize the various aspects of the project, including the design of the soft and hard X-ray branches of the accelerator, the results of SwissFEL performance simulations, details of the photon beamlines and experimental stations, and our first commissioning results.
Published: 2017
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12. Ultrafast X-ray Absorption Studies of the Structural Dynamics of Molecular and Biological Systems in Solution

Author: Christopher J. Milne, Thomas J. Penfold, Susanne Karlsson, Frank van Mourik, Marco Reinhard, Hannelore Rittmann-Frank, Frederico A. Lima, Van-Thai Pham, Renske M. Van der Veen, and Majed Chergui
Subjects: X-ray absorption spectroscopy, Chemistry, QD1-999
Abstract: We review our recent studies of excited state structures and dynamics of chemical and biological systems with pico- and femtosecond X-ray absorption spectroscopy in the liquid phase.
Published: 2011
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13. Ultrafast Structural Dynamics in Condensed Matter

Author: Paul Beaud, Steven L. Johnson, Ekaterina Vorobev, Christopher J. Milne, Andrin Caviezel, Simon O. Mariager, Raquel A. De Souza, Urs Staub, and Gerhard Ingold
Subjects: Coherent phonons, Femtosecond x-rays, Phase transitions, Strongly correlated electron systems, Ultrafast structural dynamics, Chemistry, QD1-999
Abstract: We review our recent activity in the field of photo-induced structural dynamics in crystalline solids studied using femtosecond X-ray diffraction techniques.
Published: 2011
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14. EXAFS Structural Determination of the Pt2(P2O5H2)44– Anion in Solution

Author: Renske M. van der Veen, Christopher J. Milne, Van-Thai Pham, Amal El Nahhas, Julia A. Weinstein, Jonathan Best, Camelia N. Borca, Christian Bressler, and Majed Chergui
Subjects: Diplatinum complexes, Exafs, Molecular structures, Chemistry, QD1-999
Abstract: We present the first structural determination of the Pt2(P2O5H2)44– anion in solution by analyzing the extended X-ray absorption fine structure (EXAFS) spectrum of the Pt LIII edge. The data could be fit with a simple model involving single and multiple scattering paths to near and far P-atoms, bridging O-atoms, and the other Pt-atom in the binuclear complex. A Pt–Pt distance of 2.876(28) Å and a Pt–P bond length of 2.32(4) Å are obtained. These values are in line with distances found in previous X-ray diffraction studies. The assignment of the EXAFS spectrum of the Pt2(P2O5H2)44– anion in its ground state is required for future time-resolved X-ray absorption measurements with the goal of determining the structure and dynamics of the complex in the 1,3A2u excited states.
Published: 2008
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15. Light-Induced Spin Crossover Probed by Ultrafast Optical and X-ray Spectroscopies

Author: Wojciech Gawelda, Andrea Cannizzo, Van-Thai Pham, Amal El Nahhas, Christopher J. Milne, Renske van der Veen, Christian Bressler, and Majed Chergui
Subjects: Fluorescence, Iron (ii) complexes, Optical absorption, Spin crossover, Ultrafast, X-ray absorption, Chemistry, QD1-999
Abstract: The photoinduced energy and structural relaxation of aqueous iron(II)-tris-bipyridine ([FeII(bpy)3]2+), upon excitation into its singlet metal-to-ligand charge transfer (1MLCT) band, and the population of its short-lived (?0.6 ns) high-spin excited state have been characterized by combined ultrafast optical and X-ray spectroscopies. Polychromatic femtosecond fluorescence up-conversion reveals a very short lived 1MLCT emission band, which decays in ?20 fs by intersystem crossing to a 3MLCT, whose very weak emission is also observed. Transient absorption studies show that the latter decays in
Published: 2007
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16. Atomic-scale observation of solvent reorganization influencing photoinduced structural dynamics in a copper complex photosensitizer

Author: Tetsuo Katayama, Tae-Kyu Choi, Dmitry Khakhulin, Asmus O. Dohn, Christopher J. Milne, György Vankó, Zoltán Németh, Frederico A. Lima, Jakub Szlachetko, Tokushi Sato, Shunsuke Nozawa, Shin-ichi Adachi, Makina Yabashi, Thomas J. Penfold, Wojciech Gawelda, and Gianluca Levi
Subjects: General Chemistry
Abstract: Photochemical reactions in solution are governed by a complex interplay between transient intramolecular electronic and nuclear structural changes and accompanying solvent rearrangements. State-of-the-art time-resolved X-ray solution scattering has emerged in the last decade as a powerful technique to observe solute and solvent motions in real time. However, disentangling solute and solvent dynamics and how they mutually influence each other remains challenging. Here, we simultaneously measure femtosecond X-ray emission and scattering to track both the intramolecular and solvation structural dynamics following photoexcitation of a solvated copper photosensitizer. Quantitative analysis assisted by molecular dynamics simulations reveals a two-step ligand flattening strongly coupled to the solvent reorganization, which conventional optical methods could not discern. First, a ballistic flattening triggers coherent motions of surrounding acetonitrile molecules. In turn, the approach of acetonitrile molecules to the copper atom mediates the decay of intramolecular coherent vibrations and induces a further ligand flattening. These direct structural insights reveal that photoinduced solute and solvent motions can be intimately intertwined, explaining how the key initial steps of light harvesting are affected by the solvent on the atomic time and length scale. Ultimately, this work takes a step forward in understanding the microscopic mechanisms of the bidirectional influence between transient solvent reorganization and photoinduced solute structural dynamics.
Published: 2023

17. Ultrafast Energy Transfer from Photoexcited Tryptophan to the Haem in Cytochrome c

Author: Camila Bacellar, Jérémy R. Rouxel, Rebecca A. Ingle, Giulia F. Mancini, Dominik Kinschel, Oliviero Cannelli, Yang Zhao, Claudio Cirelli, Gregor Knopp, Jakub Szlachetko, Frederico A. Lima, Samuel Menzi, Dmitry Ozerov, Georgios Pamfilidis, Katharina Kubicek, Dmitry Khakhulin, Wojciech Gawelda, Angel Rodriguez-Fernandez, Mykola Biednov, Christian Bressler, Christopher A. Arrell, Philip J. M. Johnson, Christopher J. Milne, and Majed Chergui
Subjects: spectroscopy, picosecond, fluorescence decay kinetics, x-ray-absorption, myoglobin, long-range electron, General Materials Science, transfer rates, dynamics, Physical and Theoretical Chemistry, femtosecond, electron-transfer reactions
Abstract: We report femtosecond Fe K-edge absorption (XAS) and nonresonant X-ray emission (XES) spectra of ferric cytochrome C (Cyt c) upon excitation of the haem (>300 nm) or mixed excitation of the haem and tryptophan (
Published: 2023

18. Ultrafast structural changes direct the first molecular events of vision

Author: Thomas Gruhl, Tobias Weinert, Matthew Rodrigues, Christopher J Milne, Giorgia Ortolani, Karol Nass, Eriko Nango, Saumik Sen, Philip J M Johnson, Claudio Cirelli, Antonia Furrer, Sandra Mous, Petr Skopintsev, Daniel James, Florian Dworkowski, Petra Båth, Demet Kekilli, Dmitry Ozerov, Rie Tanaka, Hannah Glover, Camila Bacellar, Steffen Brünle, Cecilia M Casadei, Azeglio D Diethelm, Dardan Gashi, Guillaume Gotthard, Ramon Guixà-González, Yasumasa Joti, Victoria Kabanova, Gregor Knopp, Elena Lesca, Pikyee Ma, Isabelle Martiel, Jonas Mühle, Shigeki Owada, Filip Pamula, Daniel Sarabi, Oliver Tejero, Ching-Ju Tsai, Niranjan Varma, Anna Wach, Sébastien Boutet, Kensuke Tono, Przemyslaw Nogly, Xavier Deupi, So Iwata, Richard Neutze, Jörg Standfuss, Gebhard FX Schertler, and Valerie Panneels
Subjects: basis-sets, Multidisciplinary, software, energy-storage, dynamics, Photobiology, isomerization, rhodopsin, excited-state, retinal chromophore, counterion displacement, Visual system, crystallography, X-ray crystallography
Abstract: Vision is initiated by the rhodopsin family of light-sensitive G protein-coupled receptors (GPCRs). A photon is absorbed by the 11-cis retinal chromophore of rhodopsin, which isomerizes within 200 femtoseconds to the all-trans conformation, thereby initiating the cellular signal transduction processes that ultimately lead to vision. However, the intramolecular mechanism by which the photoactivated retinal induces the activation events inside rhodopsin remains experimentally unclear. Here we use ultrafast time-resolved crystallography at room temperature to determine how an isomerized twisted all-trans retinal stores the photon energy that is required to initiate the protein conformational changes associated with the formation of the G protein-binding signalling state. The distorted retinal at a 1-ps time delay after photoactivation has pulled away from half of its numerous interactions with its binding pocket, and the excess of the photon energy is released through an anisotropic protein breathing motion in the direction of the extracellular space. Notably, the very early structural motions in the protein side chains of rhodopsin appear in regions that are involved in later stages of the conserved class A GPCR activation mechanism. Our study sheds light on the earliest stages of vision in vertebrates and points to fundamental aspects of the molecular mechanisms of agonist-mediated GPCR activation., 視覚に関わるタンパク質の超高速分子動画 --薄暗いところで光を感じる仕組み--. 京都大学プレスリリース. 2023-03-23.
Published: 2023

19. Pink-beam serial femtosecond crystallography for accurate structure-factor determination at an X-ray free-electron laser

Author: Oleksandr Yefanov, A. Tolstikova, Demet Kekilli, Y. Gevorkov, Tobias Weinert, Claudio Cirelli, Camila Bacellar, Isabelle Martiel, Jörg Standfuss, Laura Vera, Dmitry Ozerov, Florian S. N. Dworkowski, Sven Reiche, Daniel James, Christopher J. Milne, Philip J. M. Johnson, Karol Nass, and Gregor Knopp
Subjects: Diffraction, serial femtosecond crystallography, Materials science, de novo protein structure determination, Physics::Optics, single-wavelength anomalous diffraction, Biochemistry, law.invention, law, ddc:530, General Materials Science, pink beams, large bandwidths, Crystallography, Free-electron laser, General Chemistry, Condensed Matter Physics, Laser, xfels, Research Papers, Phaser, Synchrotron, Full width at half maximum, data-quality indicators, QD901-999, Femtosecond, Structure factor
Abstract: IUCrJ 8(6), 905 - 920 (2021). doi:10.1107/S2052252521008046, Serial femtosecond crystallography (SFX) at X-ray free-electron lasers (XFELs) enables essentially radiation-damage-free macromolecular structure determination using microcrystals that are too small for synchrotron studies. However, SFX experiments often require large amounts of sample in order to collect highly redundant data where some of the many stochastic errors can be averaged out to determine accurate structure-factor amplitudes. In this work, the capability of the Swiss X-ray free-electron laser (SwissFEL) was used to generate large-bandwidth X-ray pulses [$��/��$ = 2.2% full width at half-maximum (FWHM)], which were applied in SFX with the aim of improving the partiality of Bragg spots and thus decreasing sample consumption while maintaining the data quality. Sensitive data-quality indicators such as anomalous signal from native thaumatin micro-crystals and de novo phasing results were used to quantify the benefits of using pink X-ray pulses to obtain accurate structure-factor amplitudes. Compared with data measured using the same setup but using X-ray pulses with typical quasi-monochromatic XFEL bandwidth (��/�� = 0.17% FWHM), up to fourfold reduction in the number of indexed diffraction patterns required to obtain similar data quality was achieved. This novel approach, pink-beam SFX, facilitates the yet underutilized de novo structure determination of challenging proteins at XFELs, thereby opening the door to more scientific breakthroughs., Published by Chester
Published: 2021

20. A compact and cost-effective hard X-ray free-electron laser driven by a high-brightness and low-energy electron beam

Author: Claudio Cirelli, Rafael Abela, Thomas J. Schmidt, Vladimir Arsov, Eduard Prat, Leonardo Sala, M. Aiba, B. Keil, Gian Luca Orlandi, Karol Nass, Luc Patthey, Marco Calvi, F. Marcellini, Rolf Follath, Terence Garvey, Daniela Kiselev, Martin Paraliev, Alexander Dietrich, Christian Erny, Steven L. Johnson, Albert Romann, Arturo Alarcon, Peter Radi, Henrik T. Lemke, Micha Dehler, Pavel Chevtsov, Bruce D. Patterson, Martin Huppert, Maik Kaiser, J. Alex, Jean-Yves Raguin, S. Redford, Christoph Kittel, Mathias Sander, Fabian Märki, Christopher Arrell, Jens Rehanek, Zheqiao Geng, Thomas Schietinger, A. Wrulich, Claude Pradervand, Simona Bettoni, Roger Biffiger, Simon Ebner, Elke Zimoch, Cigdem Ozkan Loch, Sladana Dordevic, Majed Chergui, C. Svetina, Gregor Knopp, Vincent Esposito, D. Treyer, Roger Kalt, C. Gough, A. Trisorio, A. Hauff, Paul Beaud, Hans-Heinrich Braun, Alexandre Gobbo, G. Marinkovic, Roberto Dinapoli, Rasmus Ischebeck, Marco Pedrozzi, Daniel Llorente Sancho, W. Koprek, Alexander Malyzhenkov, Eugenio Ferrari, Leonid Rivkin, Philip J. M. Johnson, Yunieski Arbelo, Romain Ganter, Mike Seidel, Carlo Vicario, A. Citterio, Roman Mankowsky, Gerhard Ingold, L. Stingelin, F. Frei, M. Bopp, Carl Beard, Stephan Hunziker, Florian Löhl, Ariana Cassar, Volker Schlott, Philipp Dijkstal, Paolo Craievich, Didier Voulot, Giulia F. Mancini, Sven Reiche, Daniel Engeler, Aldo Mozzanica, Pavle Juranić, Andreas Dax, Uwe Flechsig, Christopher J. Milne, Serhane Zerdane, Markus Janousch, Yunpei Deng, M. Jurcevic, Isabelle Martiel, Nicole Hiller, Tine Celcer, T. Schilcher, Christoph P. Hauri, Michael Laznovsky, M. Stadler, Bill Pedrini, Camila Bacellar, and Marta Csatari Divall
Subjects: Brightness, Population, 02 engineering and technology, Radiation, 01 natural sciences, law.invention, 010309 optics, Optics, law, 0103 physical sciences, Thermal emittance, education, single, Physics, education.field_of_study, business.industry, Free-electron laser, 021001 nanoscience & nanotechnology, Laser, Atomic and Molecular Physics, and Optics, Electronic, Optical and Magnetic Materials, radiation, Cathode ray, Physics::Accelerator Physics, statistical properties, 0210 nano-technology, business, Lasing threshold
Abstract: We present the first lasing results of SwissFEL, a hard X-ray free-electron laser (FEL) that recently came into operation at the Paul Scherrer Institute in Switzerland. SwissFEL is a very stable, compact and cost-effective X-ray FEL facility driven by a low-energy and ultra-low-emittance electron beam travelling through short-period undulators. It delivers stable hard X-ray FEL radiation at 1-A wavelength with pulse energies of more than 500 μJ, pulse durations of ~30 fs (root mean square) and spectral bandwidth below the per-mil level. Using special configurations, we have produced pulses shorter than 1 fs and, in a different set-up, broadband radiation with an unprecedented bandwidth of ~2%. The extremely small emittance demonstrated at SwissFEL paves the way for even more compact and affordable hard X-ray FELs, potentially boosting the number of facilities worldwide and thereby expanding the population of the scientific community that has access to X-ray FEL radiation. The first lasing results at SwissFEL, an X-ray free-electron laser, are presented, highlighting the facility’s unique capabilities. A general comparison to other major facilities is also provided.
Published: 2020

21. Advances in long-wavelength native phasing at X-ray free-electron lasers

Author: Camila Bacellar, Filip Leonarski, Ivan Usov, Shahrooz Nasrollahi Shirazi, Petr Skopintsev, Karol Nass, Dmitry Ozerov, Natacha Olieric, Michael Hennig, Tobias Weinert, Aldo Mozzanica, Christopher J. Milne, Florian S. N. Dworkowski, T. Geng, Gregor Knopp, M. Sharpe, S. Redford, Claudio Cirelli, Rafael Abela, R. Bohinc, Isabelle Martiel, Andrew S. Doré, Gebhard F. X. Schertler, Przemyslaw Nogly, Robert K. Y. Cheng, Daniel James, Luc Patthey, Michel O. Steinmetz, Shibom Basu, Laura Vera, Mathieu Rappas, C. Casadei, Robert M. Cooke, Jörg Standfuss, Meitian Wang, and Bernd Schmitt
Subjects: Free electron model, serial femtosecond crystallography, Materials science, de novo protein structure determination, 02 engineering and technology, single-wavelength anomalous diffraction, Biochemistry, Signal, law.invention, Reduction (complexity), 03 medical and health sciences, Optics, law, Serial femtosecond crystallography, X-ray free-electron lasers, Single-wavelength anomalous diffraction, De novo protein structure determination, Anomalous data-quality indicators, General Materials Science, lcsh:Science, 030304 developmental biology, 0303 health sciences, anomalous data-quality indicators, business.industry, General Chemistry, 021001 nanoscience & nanotechnology, Condensed Matter Physics, Laser, Phaser, Research Letters, Wavelength, x-ray free-electron lasers, Femtosecond, lcsh:Q, 0210 nano-technology, business, Order of magnitude
Abstract: Long-wavelength pulses from the Swiss X-ray free-electron laser (XFEL) have been used for de novo protein structure determination by native single-wavelength anomalous diffraction (native-SAD) phasing of serial femtosecond crystallography (SFX) data. In this work, sensitive anomalous data-quality indicators and model proteins were used to quantify improvements in native-SAD at XFELs such as utilization of longer wavelengths, careful experimental geometry optimization, and better post-refinement and partiality correction. Compared with studies using shorter wavelengths at other XFELs and older software versions, up to one order of magnitude reduction in the required number of indexed images for native-SAD was achieved, hence lowering sample consumption and beam-time requirements significantly. Improved data quality and higher anomalous signal facilitate so-far underutilized de novo structure determination of challenging proteins at XFELs. Improvements presented in this work can be used in other types of SFX experiments that require accurate measurements of weak signals, for example time-resolved studies., IUCrJ, 7 (6), ISSN:2052-2525
Published: 2020

22. From Femtosecond Excited-State and Dissociation Dynamics to Nanosecond Reaction Kinetics: Following C-H Bond Activation with X-rays

Author: Raphael M. Jay, Ambar Banerjee, Torsten Leitner, Robert Stefanuik, Ru-Pan Wang, Jessica Harich, Emma Beale, Victoria Kabanova, Abdullah Kahraman, Anna Wach, Dimitri Ozerov, Christopher A. Arrell, Philip J. M. Johnson, Grigory Smolentsev, Thomas Huthwelker, Camilia N. Borca, Claudio Cirelli, Camila Bacellar, Christopher J. Milne, Nils Huse, Michael Odelius, and Philippe Wernet
Abstract: Using ultrafast X-ray absorption spectroscopy, we observe how a rhodium carbonyl catalyst is formed on femtosecond timescales and reveal the decisive orbital interactions which facilitate the efficient cleavage of an alkane C-H bond from solution.
Published: 2022

23. XFELs: cutting edge X-ray light for chemical and material sciences

Author: Kelly J. Gaffney, Makina Yabashi, Kiyotaka Asakura, and Christopher J. Milne
Subjects: Materials science, business.industry, X-ray, General Physics and Astronomy, 02 engineering and technology, Edge (geometry), 021001 nanoscience & nanotechnology, 01 natural sciences, 010309 optics, Optics, 0103 physical sciences, Physical and Theoretical Chemistry, 0210 nano-technology, business
Abstract: Kiyotaka Asakura, Kelly J. Gaffney, Christopher Milne, and Makina Yabashi introduce the PCCP themed issue on X-ray free-electron lasers (XFELs).
Published: 2020

24. A von Hamos spectrometer for in situ sulfur speciation by non-resonant sulfur Kα emission spectroscopy

Author: Adam H. Clark, Jakub Szlachetko, Joanna Czapla-Masztafiak, Stephan Hitz, Christopher J. Milne, Urs Vogelsang, Dzulija Kuzmenko, David Müller, Maarten Nachtegaal, and Dominik Kinschel
Subjects: In situ, Materials science, Spectrometer, 010401 analytical chemistry, Resolution (electron density), Analytical chemistry, chemistry.chemical_element, 010501 environmental sciences, 01 natural sciences, Sulfur, Chemical reaction, 0104 chemical sciences, Analytical Chemistry, Crystal, chemistry, Methanation, Emission spectrum, Spectroscopy, 0105 earth and related environmental sciences
Abstract: A von Hamos geometry based wavelength dispersive spectrometer combined with an in situ reactor cell has been developed to measure non-resonant sulfur Kα emission for the in situ speciation of low concentrations of sulfur. The spectrometer operates at 15 cm focusing radius, is equipped with a curved Si(111) crystal and a position sensitive detector, and is capable of achieving an energy resolution of 0.56 eV at 2.3 keV. We present the details of the spectrometer and dedicated sample-cell design to study chemical reactions in situ. The spectrometer capabilities are exemplified by an in situ study of sulfur speciation during H2S poisoning of SiO2 supported Ru nanoparticles performing CO methanation.
Published: 2019

25. Online tender X-ray spectrometer for X-ray FELs (TXS): the first experience

Author: Rasmus Ischebeck, David Mueller, Camila Bacellar, Dmitry Ozerov, Aldo Mozzanica, Christopher J. Milne, Pavle Juranić, Yunieski Arbelo Pena, Claudio Cirelli, Karol Nass, and Jens Rehanek
Subjects: X-ray spectroscopy, Materials science, Optics, business.industry, X-ray, business
Published: 2021

26. Hard X-ray transient grating spectroscopy on bismuth germanate

Author: Christopher Arrell, Danny Fainozzi, Claudio Cirelli, Luc Patthey, Paul Beaud, Laura Foglia, Edwin Divall, Riccardo Mincigrucci, Christian David, Keith A. Nelson, Urs Staub, Elia Razzoli, Mathias Sander, Maria Grazia Izzo, Andre Al Haddad, Dmitry Ozerov, Yunpei Deng, Roman Mankowsky, Eugenio Ferrari, Sara Catalini, Serhane Zerdane, Henrik T. Lemke, Adam Kubec, Renato Torre, Frieder Koch, Jérémy R. Rouxel, Benedikt Rösner, Cristian Svetina, Cettina Bottari, Majed Chergui, Simon Gerber, Gediminas Seniutinas, Georgios Pamfilidis, Max Burian, Filippo Bencivenga, Hiroki Ueda, Giulia F. Mancini, Aldo Mozzanica, Christopher J. Milne, Alessandro Gessini, Claudio Masciovecchio, Bill Pedrini, Florian Döring, Riccardo Cucini, Philip J. M. Johnson, Alexei Maznev, Gregor Knopp, Laboratoire Hubert Curien [Saint Etienne] (LHC), and Université Jean Monnet [Saint-Étienne] (UJM)-Centre National de la Recherche Scientifique (CNRS)-Institut d'Optique Graduate School (IOGS)
Subjects: Diffraction, Materials science, Physics::Optics, FOS: Physical sciences, 02 engineering and technology, Grating, 01 natural sciences, Bismuth germanate, law.invention, 010309 optics, chemistry.chemical_compound, Optics, law, 0103 physical sciences, Talbot effect, ComputingMilieux_MISCELLANEOUS, Condensed Matter - Materials Science, [PHYS.PHYS.PHYS-OPTICS]Physics [physics]/Physics [physics]/Optics [physics.optics], business.industry, Free-electron laser, Materials Science (cond-mat.mtrl-sci), 021001 nanoscience & nanotechnology, Laser, non-linear spectroscopy, ultrafast laser, free electron laser, phonon dynamics, Atomic and Molecular Physics, and Optics, Electronic, Optical and Magnetic Materials, chemistry, 0210 nano-technology, business, Ultrashort pulse, Excitation, Physics - Optics, Optics (physics.optics)
Abstract: Optical-domain Transient Grating (TG) spectroscopy is a versatile background-free four-wave-mixing technique used to probe vibrational, magnetic and electronic degrees of freedom in the time domain. The newly developed coherent X-ray Free Electron Laser sources allow its extension to the X-ray regime. Xrays offer multiple advantages for TG: their large penetration depth allows probing the bulk properties of materials, their element-specificity can address core-excited states, and their short wavelengths create excitation gratings with unprecedented momentum transfer and spatial resolution. We demonstrate for the first time TG excitation in the hard X-ray range at 7.1 keV. In Bismuth Germanate (BGO), the nonresonant TG excitation generates coherent optical phonons detected as a function of time by diffraction of an optical probe pulse. This experiment demonstrates the ability to probe bulk properties of materials and paves the way for ultrafast coherent four-wave-mixing techniques using X-ray probes and involving nanoscale TG spatial periods., Comment: 11 pages, 4 figures
Published: 2021
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27. Supernova neutrino burst detection with the deep underground neutrino experiment: DUNE Collaboration

Author: M. A. Hernandez Morquecho, Jonas Rademacker, P. De Lurgio, C. A. Ternes, E. T. Worcester, H. Schellman, G. P. Zeller, C. J. Solano Salinas, Mingshui Chen, Andrew White, S. Berkman, André Rubbia, C. Barnes, Joshua Barrow, B. Bhuyan, O. V. Mineev, M. Bishai, Sandip Pakvasa, M. Chalifour, N. Poonthottathil, H. Berns, A. S. Hesam, S. H. Kettell, John Marshall, G. Sirri, Evgueni Goudzovski, M. A. Arroyave, J. Hugon, M. Kirby, D. Brailsford, Laura Paulucci, A. Hourlier, E. Hazen, L. Pasqualini, Christian Farnese, Armin Karcher, D. Smargianaki, Christopher L. Marshall, M. Karolak, H. Mendez, Y.-J. Jwa, Y. Karyotakis, Artur M. Ankowski, B. Morgan, L. Patrizii, Stefan Antusch, Paola Sala, N. Moggi, Claire Shepherd-Themistocleous, G. Mandrioli, M. R. While, A. M. Gago, R. Diurba, J. Berger, Alessandro Menegolli, B. Carlus, D. Boyden, T. Le, G. Christodoulou, L. Hertel, J. S. Díaz, B. Ramson, R. Gandrajula, Akitaka Ariga, Marvin L Marshak, R. Zaki, Ina Sarcevic, Eric W. Hoppe, Manuel Alejandro Segura Delgado, Kam-Biu Luk, M. Tzanov, K. Qi, J. A. B. Coelho, C. Vignoli, C. E. Lane, Giuseppe Benedetto Cerati, N. Bostan, David Delepine, Dave M Newbold, F. Krennrich, C. Mauger, J. Yu, D. Edmunds, P. Novella, K. Zeug, Z. Parsa, L. O. Arnold, Janice L. Thompson, F. Kamiya, K. Kothekar, S. Calvez, A. Chiriacescu, T. Rehak, M. V. Diwan, V. Savinov, P. Melas, T. Safford, E. Tatar, Hui Wang, V. Bellini, C. Alt, B. Abi, W. Flanagan, V. Papadimitriou, G. Zhu, S. Centro, J. J. Russell, W. C. Griffith, H. R. Gallagher, M. A. Uchida, N. Martinez, L. Greenler, Bo Yu, A. V. Waldron, D. J. Payne, C. Gotti, T. Miedema, S. Magill, Deywis Moreno, Utku Kose, Julián Félix, D. MacFarland, K. Gollwitzer, F. Varanini, S. Henry, K. Grzelak, B. Guo, Frank Filthaut, J. Reichenbacher, F. Muheim, Ralf Lehnert, T. A. Bolton, J. Greer, Y. T. Tsai, L. Camilleri, S. Nagu, J. A. Maloney, Z. Vallari, F. Bay, H.E. Rogers, Andrea Dell'Acqua, Y. Cui, P. A. Rodrigues, C. Wret, J. Zuklin, Paul Keener, D. A. Harris, Andrea Zani, Mario Campanelli, M. Newcomer, H. W. Sobel, C. Distefano, Ornella Palamara, M. A. Ramirez Delgado, J. D. Eisch, Riccardo Papaleo, D. Cherdack, Paolo Carniti, Leigh H. Whitehead, Karol Hennessy, S. Söldner-Rembold, P. Fernandez Menendez, J. Han, C. Y. Chi, M. Groh, Jeremy Wolcott, R. LaZur, Yu. Onishchuk, T. Hamernik, L. Pickering, John Evans, A. Weinstein, A. Sitraka, L. Bagby, S. J. Brice, Nicolas Lurkin, E. Raguzin, L. C. J. Rice, H. Carranza, Milos Lokajicek, K. Nishimura, H. S. Budd, C. S. Lin, A. A. Machado, Kevin J. Kelly, D. Sgalaberna, J. M. LoSecco, R. Petti, Y. Xiao, Ionel Lazanu, E. Zhivun, C. McGrew, Marzio Nessi, Chia-Chan Chang, M. Nebot-Guinot, C. Grant, Jaroslaw Pasternak, Z. Djurcic, W. Gu, D. Duchesneau, N. Kazaryan, Kendall Mahn, Jorge Molina, M. Oberling, H. O. Back, S. Sacerdoti, J. Sensenig, C. Montanari, E. Conley, B. Howard, D. M. DeMuth, A. Chatterjee, S. Kohn, F. Drielsma, J. L. Bazo Alba, Jane Nachtman, Y. A. Ramachers, D. A. Martinez Caicedo, R. M. de Almeida, Yasar Onel, V. Zutshi, Sandeep Miryala, Enrique Calvo, V. Radeka, C. Touramanis, S. Manly, P. Hamilton, R. G. Van de Water, J. Hoff, K. V. Tsang, J. Maneira, C. Rubbia, J. Calcutt, K. Warburton, M. Nalbandyan, T. Loew, P. Ding, F. Diaz, R. Hatcher, M. Zhao, A. Olivares Del Campo, F. Cavalier, Joshua R. Klein, Vasundhara Singh, Christopher Brew, Pavel Snopok, Y. Rigaut, Dave Sankey, J. Asaadi, E. Valencia, E. James, Roberto Gutiérrez, J. Pinzino, Rakesh Kumar, Ranjan Dharmapalan, Lynn Wood, S. Narita, R.A. Rameika, R. Illingworth, D. Vargas, Patrick Dunne, A. Bitadze, Yichen Li, A. G. Cocco, C. Andreopoulos, T. Kosc, R. J. Wilson, S. Fuess, E. Cristaldo, H. Razafinime, Alessandro Montanari, B. Zamorano, Warner A. Miller, M. C. Sanchez, Marc Weber, Wladyslaw Henryk Trzaska, A. Izmaylov, C. Morris, Dong Jo Kim, H. Muramatsu, K. Spurgeon, Z. Pavlovic, R. Gran, Claudia Brizzolari, D. Vanegas Forero, S. Biagi, M. Tenti, Alberto Cervelli, M. Roda, F. Terranova, C. Cuesta, J. Marteau, Irakli Lomidze, W. Metcalf, X. Luo, A. Booth, G. Petrillo, N.V. Mokhov, J. Barranco Monarca, Jianbei Liu, Zviad Tsamalaidze, H. da Motta, L. M. Cremaldi, Carl Grace, M. Bonesini, M. Muether, O. G. Miranda, A. N. Khotjantsev, N. Tsverava, R. B. Patterson, T. Young, A. Stuart, M. J. Wilking, D. Redondo, S. R. Mishra, F. Bento Neves, A. Gendotti, A. Himmel, M. Rajaoalisoa, P. Bour, C. Wilkinson, M. Greenwood, F. F. Wilson, Nektarios Benekos, Marco Adinolfi, D. Pugnere, T. Wongjirad, M. A. Vermeulen, Andrew Brandt, E. Bechetoille, S. Roy, A. Delbart, N. J. C. Spooner, J. M. Paley, C. Patrick, Antonio Ereditato, José W. F. Valle, N. Yershov, Renato Potenza, D. Lorca, M. Toups, R. Guenette, E. Pantic, L. Di Giulio, J. Martin-Albo, L. Molina Bueno, M. P. Decowski, Gustaaf Brooijmans, K. Moffat, V. Galymov, Dario Gnani, L. Mualem, S. Tufanli, J. Mills, Irina Mocioiu, D. Mladenov, A. L. Renshaw, C. N. Booth, L. Zambelli, Orlando L. G. Peres, S. Menary, P. C. de Holanda, D. A. Dwyer, S. Prince, J. Haiston, Marco Pallavicini, T. J. Langford, E. Niner, Nikolaos Simos, L. V. Gomez Bermeo, E. Gamberini, Haleh Khani Hadavand, E. Chardonnet, A. Mastbaum, G. Prior, Filippo Resnati, J. Stock, M. Kordosky, F. Andrianala, B. Tapia Oregui, N. Nayak, James Stewart, W. Ketchum, C. A. Moura, J. Spitz, L. Stanco, E. McCluskey, Ihn Sik Seong, L. W. Koerner, J. Franc, B. R. Littlejohn, R. M. Berner, K. Vaziri, A. Marchionni, K. Mason, A. Rafique, Randall P. Johnson, E. Motuk, J. A. Nowak, T. Patzak, M. D. Messier, G. Savage, A. M. Iliescu, Yasaman Farzan, David Cussans, J. Soto-Oton, Alex Reynolds, K. Biery, Yanchu Wang, Konstantinos Manolopoulos, S. Bordoni, James Mueller, William J. Marciano, V. Aushev, W. Fox, G. Pessina, C. M. Sutera, E. Smith, A. D. Marino, J. J. De Vries, S. Shafaq, Olga Mena, S. Ravat, W. Mu, D. Marfatia, C. Hohl, R. Haenni, R. K. Plunkett, P. Cotte, C. Jesús-Valls, J.V. Dawson, F. Azfar, T. Wachala, A. P. Furmanski, Barry King, P.T. Smith, Juraj Bracinik, Andrew Blake, L. Jiang, Kristian Harder, J. Hewes, D. Newhart, A. J. Roeth, R. Acciarri, A. Borkum, N. McConkey, R. Mazza, Keith Rielage, J. G. Boissevain, J. Smolik, A. McNab, Stephen P. Gent, C. Castromonte, G. Vasseur, G. Lehmann Miotto, N. Dokania, Paolo Calafiura, Q. David, C. S. Mishra, Vlastimil Kus, Seodong Shin, M. Santos-Maldonado, S. Li, Sukalyan Chattopadhyay, Laura Dominé, Silvia Pascoli, Kim Siyeon, J. Zalesak, Gabriella Carini, Thorsten Lux, M. Dabrowski, Pedro A. N. Machado, T. Alion, A. Scarff, L. Corwin, L. Simard, S. L. Mufson, L. Pagani, J. Rodriguez Rondon, Alec Habig, Sandro Palestini, P. N. Ratoff, Timothy M. Shaw, D. Braga, S. Di Domizio, G. Meng, C. Petta, T. Kutter, Matheus Hostert, S. Murphy, R. Bajou, R. Northrop, V. J. Guarino, A. Joglekar, Marco Verzocchi, L. S. Gomez Fajardo, K. S. McFarland, C. T. Macias, Jürgen Pozimski, R. Raboanary, F. Sergiampietri, P. Schlabach, Z. Ahmad, Rex Tayloe, F. Marinho, F. Barao, Jianming Bian, D. Autiero, Poonam Mehta, C. Backhouse, Stephen J. Parke, J. Perry, T. Schaffer, B. Russell, K. Herner, R. Van Berg, J. Chaves, Francesco Gonnella, B. Paulos, N. Solomey, Laura Manenti, R. Sipos, S. Matsuno, Z. Ghorbani-Moghaddam, J. K. Nelson, Hem Raj Sharma, Karol Lang, S. Bertolucci, Piera Sapienza, M. Shamma, A. Lambert, N. P. Samios, Andrew Smith, M. Manrique Plata, J. Bremer, C. K. Jung, G. Yang, I. Kreslo, Kyung-Suk Cho, A. Sousa, J. Urheim, D. Montanari, Giorgio Riccobene, A. Heavey, Grzegorz Deptuch, Stephen Hillier, M. Gold, Sergei Striganov, G. Brunetti, M. Vagins, T. Yang, A. Rappoldi, S. Ventura, S. Dennis, J. Ahmed, Narendra Sahu, Yi Chen, S. P. Kasetti, M. Betancourt, E. Pennacchio, Y. Penichot, K. Francis, F. Cavanna, Chao Zhang, A. Muir, A. Mazzacane, P. P. Koller, D. Whittington, N. Gallice, Wei Wu, G. Karagiorgi, F. W. Sippach, T. Li, F. Bonini, S. J. Patton, E. Church, M. Parvu, James A. Anderson, V. A. Kostelecký, S. Gao, D. Garcia-Gamez, V. Paolone, V. Pec, J. Pillow, S. Vergani, P. Vahle, G. A. Horton-Smith, C. Lastoria, E. Ewart, Claire David, D. Naples, I. Rakhno, Kazuhiro Terao, A. Paudel, V. Basque, G. S. Varner, M. H. Shaevitz, N. Barros, I. Caro Terrazas, R. Itay, Simon Lin, K. Wood, H. Duyang, H. Meyer, Katsuya Yonehara, S. Bolognesi, J. L. Raaf, J. Singh, V. A. Kudryavtsev, J. Wang, E. Kearns, A. C. Ezeribe, D. Belver, S. Zucchelli, S. Gollapinni, C. Sarasty, A. de Gouvea, Rukmani Mohanta, S. Martynenko, D. Shooltz, A. Schukraft, Andrew Norman, T. E. Coan, A. Lister, G. S. Davies, I. De Bonis, R. S. Fitzpatrick, B. Radics, Alan Watson, M. Spanu, Xiaolu Ji, L. Di Noto, A. M. Szelc, Alessandro Thea, K. Lande, E. D. Zimmerman, M. A. Leigui de Oliveira, Mafalda Dias, M. Wetstein, Ph. Lebrun, A. Christensen, S. Gwon, Matthew L Strait, L. Da Silva Peres, O. Goodwin, Jitendra Kumar, A. Gallego-Ros, M. Zito, G. Barenboim, N. Buchanan, S. Pordes, P. Weatherly, K. K. Guthikonda, James John Brooke, N. Mauri, A. Lawrence, Michael Mulhearn, I. K. Furic, M. M. Khabibullin, G. Testera, A. M. Teklu, John Matthews, A. Olivier, E. Blucher, L. Rakotondravohitra, B. Stillwell, M. Wallbank, S. B. Boyd, Matthew Mewes, Kai Loo, J. Trevor, W. E. Sondheim, Nikolina Ilic, T. Hill, M. O. Wascko, C. E. Tull, I. Kadenko, D. Waters, S. Prakash, D. Ruterbories, Antonino Sergi, S. Childress, T. Miao, A. Verdugo, D. Wenman, S. C. Timm, Y. Bezawada, R. Sharma, M. Biassoni, D. Pershey, V. P. Luzio, R. Saakyan, R. Nandakumar, E. Kemp, Aldo Penzo, R. J. Nichol, P. Guzowski, M. Eads, S. Rosauro-Alcaraz, M. Sorel, D. Totani, Sandhya Choubey, Burak Bilki, Christopher J. Milne, J. C. Freeman, Kaushik De, Jordan Ott, Niki Saoulidou, A. Aranda-Fernandez, A. Mefodiev, V. N. Solovov, A. Holin, Gareth J. Barker, C. Cattadori, Patrick Green, R. Howell, M. Soderberg, A. C. Weber, X. Pons, J. G. Learned, T. Stokes, M. J. Dolinski, L. Montaño Zetina, M. J. Rodriguez Alonso, M. A. Acero, Yu. Kudenko, L. Li, J. Fowler, J. A. Musser, M. Leyton, M. E. Convery, D. Gratieri, J. R. T. de Mello Neto, S. Balasubramanian, G. A. Valdiviesso, E. Brianne, C. Mossey, Kenneth Long, F. Pietropaolo, Raj Gandhi, T. Hasegawa, Giovanni Bellettini, M. Bhattacharjee, E. Granados, T. Lord, L. Zazueta, Alexander Deisting, B. Rebel, S. Green, Mathieu Bongrand, B. Behera, S. Emery, E. Mazzucato, H. Y. Liao, M. Masud, Amelia Maio, W. C. Louis, J. Freestone, D. Rivera, A. Surdo, S. Kasai, M. Worcester, H. S. Chen, George Adamov, A. Guglielmi, D. Franco, Joleen Pater, S. J. M. Peeters, K. Koehler, S. Alonso Monsalve, M. C. Goodman, G. Ge, Alexander Tapper, Thomas Strauss, D. C. Christian, Gregory Iles, A. Friedland, K. M. Heeger, K. Mavrokoridis, P. Lasorak, Srubabati Goswami, Z. Williams, S. Rescia, Andrés Castillo, David H. Adams, S. Santana, C. Mariani, D. A. Sanders, Carlos Escobar, R. A. Gomes, E. Gramellini, G. C. Blazey, J. Vasel, T. Durkin, H. Y. 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A., Karolak M., Karyotakis Y., Kasai S., Kasetti S.P., Kashur L., Kazaryan N., Kearns E., Keener P., Kelly K.J., Kemp E., Ketchum W., Kettell S.H., Khabibullin M., Khotjantsev A., Khvedelidze A., Kim D., King B., Kirby B., Kirby M., Klein J., Koehler K., Koerner L.W., Kohn S., Koller P.P., Kordosky M., Kosc T., Kose U., Kostelecky V.A., Kothekar K., Krennrich F., Kreslo I., Kudenko Y., Kudryavtsev V.A., Kulagin S., Kumar J., Kumar R., Kuruppu C., Kus V., Kutter T., Lambert A., Lande K., Lane C.E., Lang K., Langford T., Lasorak P., Last D., Lastoria C., Laundrie A., Lawrence A., Lazanu I., LaZur R., Le T., Learned J., LeBrun P., Lehmann Miotto G., Lehnert R., Leigui de Oliveira M.A., Leitner M., Leyton M., Li L., Li S., Li S.W., Li T., Li Y., Liao H., Lin C.S., Lin S., Lister A., Littlejohn B.R., Liu J., Lockwitz S., Loew T., Lokajicek M., Lomidze I., Long K., Loo K., Lorca D., Lord T., LoSecco J.M., Louis W.C., Luk K.B., Luo X., Lurkin N., Lux T., Luzio V.P., MacFarland D., Machado 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Subjects: Physics and Astronomy (miscellaneous), Physics::Instrumentation and Detectors, Astrophysics::High Energy Astrophysical Phenomena, Astrophysics, Computer Science::Digital Libraries, 01 natural sciences, Physics::Geophysics, Neutrino experiment, 0103 physical sciences, Deep Underground Neutrino Experiment, 010303 astronomy & astrophysics, Engineering (miscellaneous), Supernova, Neutrino, Physics, Time projection chamber, Neutrino, LAr TPC, Accretion (meteorology), 010308 nuclear & particles physics, High Energy Physics::Phenomenology, Galaxy, Supernova, Neutrino detector, Computer Science::Mathematical Software, Liquid argon, High Energy Physics::Experiment, Neutrino
Abstract: This document was prepared by the DUNE collaboration using the resources of the Fermi National Accelerator Laboratory (Fermilab), a U.S. Department of Energy, Office of Science, HEP User Facility. Fermilab is managed by Fermi Research Alliance, LLC (FRA), acting under Contract No. DE-AC02-07CH11359. This work was supported by CNPq, FAPERJ, FAPEG and FAPESP, Brazil; CFI, IPP and NSERC, Canada;CERN;MŠMT,Czech Republic; ERDF, H2020-EU and MSCA, European Union; CNRS/IN2P3 and CEA, France; INFN, Italy; FCT, Portugal; NRF, South Korea; CAM, Fundación “La Caixa” and MICINN, Spain; SERI and SNSF, Switzerland; TÜB˙ITAK, Turkey; The Royal Society and UKRI/STFC, United Kingdom; DOE and NSF, United States of America. This research used resources of the National Energy Research Scientific Computing Center (NERSC), a U.S. Department of Energy Office of Science User Facility operated under Contract No. DE-AC02-05CH11231., Data Availability Statement This manuscript has no associated data or the data will not be deposited. [Authors’ comment: This manuscript describes sensitivity studies for the DUNE experiment using simulation only, and as such there are no experimental data to report.], The deep underground neutrino experiment (DUNE), a 40-kton underground liquid argon time projection chamber experiment, will be sensitive to the electron-neutrino flavor component of the burst of neutrinos expected from the next Galactic core-collapse supernova. Such an observation will bring unique insight into the astrophysics of core collapse as well as into the properties of neutrinos. The general capabilities of DUNE for neutrino detection in the relevant few- to few-tens-of-MeV neutrino energy range will be described. As an example, DUNE’s ability to constrain the νe spectral parameters of the neutrino burst will be considered., Commissariat à l'Énergie Atomique et aux Énergies Alternatives CEA, Fundação de Amparo à Pesquisa do Estado de São Paulo FAPESP, U.S. Department of Energy DE-AC02-05CH11231 USDOE, Fundação Carlos Chagas Filho de Amparo à Pesquisa do Estado do Rio de Janeiro FAPERJ, Ministerstvo Školství, Mládeže a Tělovýchovy MŠMT, Fundação para a Ciência e a Tecnologia FCT, Royal Society, Ministerio de Ciencia e Innovación MICINN, Natural Sciences and Engineering Research Council of Canada NSERC, UK Research and Innovation UKRI, Instituto Nazionale di Fisica Nucleare INFN, Centre National de la Recherche Scientifique CNRS, Conselho Nacional de Desenvolvimento Científico e Tecnológico CNPq, National Research Foundation of Korea NRF, Institut National de Physique Nucléaire et de Physique des Particules IN2P3, H2020-EU, European Commission EC, European Regional Development Fund ERDF, TÜBİTAK, CERN, U.S. Department of Energy USDOE, Fundação de Amparo à Pesquisa do Estado de Goiás FAPEG, Multiple Sclerosis Center of Atlanta MSCA, Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung SNF, Singapore Eye Research Institute SERI, Fermi Research Alliance, LLC DE-AC02-07CH11359, National Science Foundation NSF, Science and Technology Facilities Council STFC
Published: 2021
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28. Neutrino interaction classification with a convolutional neural network in the DUNE far detector

Author: R.A. Rameika, J. Perry, M. Kirby, E. Zhivun, K. Zeug, R. LaZur, Marzio Nessi, D. Lorca, R. M. Berner, Sandip Pakvasa, J. J. De Vries, S. Shafaq, Jonas Rademacker, G. P. Zeller, R. Guenette, A. Hourlier, A. McNab, G. Vasseur, C. Petta, C. Grant, A. Olivares Del Campo, Joshua R. Klein, Vasundhara Singh, D. M. DeMuth, A. Chatterjee, P. Debbins, Paola Sala, G. Mandrioli, John G. Learned, S. Kohn, F. Drielsma, Joshua Barrow, John Marshall, Janice L. Thompson, F. Kamiya, E. Motuk, E. Gamberini, B. J. P. Jones, L. Di Giulio, J. Martin-Albo, E. Bechetoille, Gustaaf Brooijmans, K. Moffat, L.S. Rochester, T. L. Usher, R. Staley, Bo Yu, A. V. Waldron, Gabriella Carini, M. Dabrowski, Francesco Gonnella, C. Vilela, B. Zamorano, Warner A. Miller, Wladyslaw Henryk Trzaska, A. M. Gago, R. Diurba, N. Bostan, J. Spitz, M. Pozzato, Y. Cui, P. A. Rodrigues, J. D. Eisch, F. Cavanna, Sofia Vallecorsa, K. E. Duffy, Danny Marfatia, E. Segreto, Xin Qian, T. A. Mohayai, C. J. 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H., Whittington, D., Wilking, M. J., Wilkinson, C., Williams, Z., Wilson, F., Wilson, R. J., Wolcott, J., Wongjirad, T., Wood, K., Wood, L., Worcester, E., Worcester, M., Wret, C., Wu, W., Xiao, Y., Yang, G., Yang, T., Yershov, N., Yonehara, K., Young, T., Yu, B., Yu, J., Zaki, R., Zalesak, J., Zambelli, L., Zamorano, B., Zani, A., Zazueta, L., Zeller, G. P., Zennamo, J., Zeug, K., Zhang, C., Zhao, M., Zhivun, E., Zhu, G., Zimmerman, E. D., Zito, M., Zucchelli, S., Zuklin, J., Zutshi, V., Zwaska, R., Institut de Physique des 2 Infinis de Lyon (IP2I Lyon), Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Claude Bernard Lyon 1 (UCBL), Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS), AstroParticule et Cosmologie (APC (UMR_7164)), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Centre National de la Recherche Scientifique (CNRS)-Université de Paris (UP), Institut de Recherches sur les lois Fondamentales de l'Univers (IRFU), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay, Laboratoire de l'Accélérateur Linéaire (LAL), Centre National de la Recherche Scientifique (CNRS)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Sud - Paris 11 (UP11), Laboratoire d'Annecy de Physique des Particules (LAPP), Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS), Laboratoire de Physique Subatomique et de Cosmologie (LPSC), Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP ), Université Grenoble Alpes (UGA), DUNE, XENON (IHEF, IoP, FNWI), ATLAS (IHEF, IoP, FNWI), Abi, B, Acciarri, R, Acero, M, Adamov, G, Adams, D, Adinolfi, M, Ahmad, Z, Ahmed, J, Alion, T, Alonso Monsalve, S, Alt, C, Anderson, J, Andreopoulos, C, Andrews, M, Andrianala, F, Andringa, S, Ankowski, A, Antonova, M, Antusch, S, Aranda-Fernandez, A, Ariga, A, Arnold, L, Arroyave, M, Asaadi, J, Aurisano, A, Aushev, V, Autiero, D, Azfar, F, Back, H, Back, J, Backhouse, C, Baesso, P, Bagby, L, Bajou, R, Balasubramanian, S, Baldi, P, Bambah, B, Barao, F, Barenboim, G, Barker, G, Barkhouse, W, Barnes, C, Barr, G, Barranco Monarca, J, Barros, N, Barrow, J, Bashyal, A, Basque, V, Bay, F, Bazo Alba, J, Beacom, J, Bechetoille, E, Behera, B, Bellantoni, L, Bellettini, G, Bellini, V, Beltramello, O, Belver, D, Benekos, N, Bento Neves, F, Berger, J, Berkman, S, Bernardini, P, Berner, R, Berns, H, Bertolucci, S, Betancourt, M, Bezawada, Y, Bhattacharjee, M, Bhuyan, B, Biagi, S, Bian, J, Biassoni, M, Biery, K, Bilki, B, Bishai, M, Bitadze, A, Blake, A, Blanco Siffert, B, Blaszczyk, F, Blazey, G, Blucher, E, Boissevain, J, Bolognesi, S, Bolton, T, Bonesini, M, Bongrand, M, Bonini, F, Booth, A, Booth, C, Bordoni, S, Borkum, A, Boschi, T, Bostan, N, Bour, P, Boyd, S, Boyden, D, Bracinik, J, Braga, D, Brailsford, D, Brandt, A, Bremer, J, Brew, C, Brianne, E, Brice, S, Brizzolari, C, Bromberg, C, Brooijmans, G, Brooke, J, Bross, A, Brunetti, G, Buchanan, N, Budd, H, Caiulo, D, Calafiura, P, Calcutt, J, Calin, M, Calvez, S, Calvo, E, Camilleri, L, Caminata, A, Campanelli, M, Caratelli, D, Carini, G, Carlus, B, Carniti, P, Caro Terrazas, I, Carranza, H, Castillo, A, Castromonte, C, Cattadori, C, Cavalier, F, Cavanna, F, Centro, S, Cerati, G, Cervelli, A, Cervera Villanueva, A, Chalifour, M, Chang, C, Chardonnet, E, Chatterjee, A, Chattopadhyay, S, Chaves, J, Chen, H, Chen, M, Chen, Y, Cherdack, D, Chi, C, Childress, S, Chiriacescu, A, Cho, K, Choubey, S, Christensen, A, Christian, D, Christodoulou, G, Church, E, Clarke, P, Coan, T, Cocco, A, Coelho, J, Conley, E, Conrad, J, Convery, M, Corwin, L, Cotte, P, Cremaldi, L, Cremonesi, L, Crespo-Anadon, J, Cristaldo, E, Cross, R, Cuesta, C, Cui, Y, Cussans, D, Dabrowski, M, Da Motta, H, Da Silva Peres, L, David, C, David, Q, Davies, G, Davini, S, Dawson, J, De, K, De Almeida, R, Debbins, P, De Bonis, I, Decowski, M, De Gouvea, A, De Holanda, P, De Icaza Astiz, I, Deisting, A, De Jong, P, Delbart, A, Delepine, D, Delgado, M, Dell'Acqua, A, De Lurgio, P, De Mello Neto, J, Demuth, D, Dennis, S, Densham, C, Deptuch, G, De Roeck, A, De Romeri, V, De Vries, J, Dharmapalan, R, Dias, M, Diaz, F, Diaz, J, Di Domizio, S, Di Giulio, L, Ding, P, Di Noto, L, Distefano, C, Diurba, R, Diwan, M, Djurcic, Z, Dokania, N, Dolinski, M, Domine, L, Douglas, D, Drielsma, F, Duchesneau, D, Duffy, K, Dunne, P, Durkin, T, Duyang, H, Dvornikov, O, Dwyer, D, Dyshkant, A, Eads, M, Edmunds, D, Eisch, J, Emery, S, Ereditato, A, Escobar, C, Escudero Sanchez, L, Evans, J, Ewart, E, Ezeribe, A, Fahey, K, Falcone, A, Farnese, C, Farzan, Y, Felix, J, Fernandez-Martinez, E, Fernandez Menendez, P, Ferraro, F, Fields, L, Filkins, A, Filthaut, F, Fitzpatrick, R, Flanagan, W, Fleming, B, Flight, R, Fowler, J, Fox, W, Franc, J, Francis, K, Franco, D, Freeman, J, Freestone, J, Fried, J, Friedland, A, Fuess, S, Furic, I, Furmanski, A, Gago, A, Gallagher, H, Gallego-Ros, A, Gallice, N, Galymov, V, Gamberini, E, Gamble, T, Gandhi, R, Gandrajula, R, Gao, S, Garcia-Carballeira, F, Garcia-Gamez, D, Garcia-Peris, M, Gardiner, S, Gastler, D, Ge, G, Gelli, B, Gendotti, A, Gent, S, Ghorbani-Moghaddam, Z, Gibin, D, Gil-Botella, I, Girerd, C, Giri, A, Gnani, D, Gogota, O, Gold, M, Gollapinni, S, Gollwitzer, K, Gomes, R, Gomez Bermeo, L, Gomez Fajardo, L, Gonnella, F, Gonzalez-Cuevas, J, Goodman, M, Goodwin, O, Goswami, S, Gotti, C, Goudzovski, E, Grace, C, Graham, M, Gramellini, E, Gran, R, Granados, E, Grant, A, Grant, C, Gratieri, D, Green, P, Green, S, Greenler, L, Greenwood, M, Greer, J, Griffith, W, Groh, M, Grudzinski, J, Grzelak, K, Gu, W, Guarino, V, Guenette, R, Guglielmi, A, Guo, B, Guthikonda, K, Gutierrez, R, Guzowski, P, Guzzo, M, Gwon, S, Habig, A, Hackenburg, A, Hadavand, H, Haenni, R, Hahn, A, Haigh, J, Haiston, J, Hamernik, T, Hamilton, P, Han, J, Harder, K, Harris, D, Hartnell, J, Hasegawa, T, Hatcher, R, Hazen, E, Heavey, A, Heeger, K, Heise, J, Hennessy, K, Henry, S, Hernandez Morquecho, M, Herner, K, Hertel, L, Hesam, A, Hewes, J, Higuera, A, Hill, T, Hillier, S, Himmel, A, Hoff, J, Hohl, C, Holin, A, Hoppe, E, Horton-Smith, G, Hostert, M, Hourlier, A, Howard, B, Howell, R, Huang, J, Hugon, J, Iles, G, Ilic, N, Iliescu, A, Illingworth, R, Ioannisian, A, Itay, R, Izmaylov, A, James, E, Jargowsky, B, Jediny, F, Jesus-Valls, C, Ji, X, Jiang, L, Jimenez, S, Jipa, A, Joglekar, A, Johnson, C, Johnson, R, Jones, B, Jones, S, Jung, C, Junk, T, Jwa, Y, Kabirnezhad, M, Kaboth, A, Kadenko, I, Kamiya, F, Karagiorgi, G, Karcher, A, Karolak, M, Karyotakis, Y, Kasai, S, Kasetti, S, Kashur, L, Kazaryan, N, Kearns, E, Keener, P, Kelly, K, Kemp, E, Ketchum, W, Kettell, S, Khabibullin, M, Khotjantsev, A, Khvedelidze, A, Kim, D, King, B, Kirby, B, Kirby, M, Klein, J, Koehler, K, Koerner, L, Kohn, S, Koller, P, Kordosky, M, Kosc, T, Kose, U, Kostelecky, V, Kothekar, K, Krennrich, F, Kreslo, I, Kudenko, Y, Kudryavtsev, V, Kulagin, S, Kumar, J, Kumar, R, Kuruppu, C, Kus, V, Kutter, T, Lambert, A, Lande, K, Lane, C, Lang, K, Langford, T, Lasorak, P, Last, D, Lastoria, C, Laundrie, A, Lawrence, A, Lazanu, I, Lazur, R, Le, T, Learned, J, Lebrun, P, Lehmann Miotto, G, Lehnert, R, Leigui De Oliveira, M, Leitner, M, Leyton, M, Li, L, Li, S, Li, T, Li, Y, Liao, H, Lin, C, Lin, S, Lister, A, Littlejohn, B, Liu, J, Lockwitz, S, Loew, T, Lokajicek, M, Lomidze, I, Long, K, Loo, K, Lorca, D, Lord, T, Losecco, J, Louis, W, Luk, K, Luo, X, Lurkin, N, Lux, T, Luzio, V, Macfarland, D, Machado, A, Machado, P, Macias, C, Macier, J, Maddalena, A, Madigan, P, Magill, S, Mahn, K, Maio, A, Maloney, J, Mandrioli, G, Maneira, J, Manenti, L, Manly, S, Mann, A, Manolopoulos, K, Manrique Plata, M, Marchionni, A, Marciano, W, Marfatia, D, Mariani, C, Maricic, J, Marinho, F, Marino, A, Marshak, M, Marshall, C, Marshall, J, Marteau, J, Martin-Albo, J, Martinez, N, Martinez Caicedo, D, Martynenko, S, Mason, K, Mastbaum, A, Masud, M, Matsuno, S, Matthews, J, Mauger, C, Mauri, N, Mavrokoridis, K, Mazza, R, Mazzacane, A, Mazzucato, E, Mccluskey, E, Mcconkey, N, Mcfarland, K, Mcgrew, C, Mcnab, A, Mefodiev, A, Mehta, P, Melas, P, Mellinato, M, Mena, O, Menary, S, Mendez, H, Menegolli, A, Meng, G, Messier, M, Metcalf, W, Mewes, M, Meyer, H, Miao, T, Michna, G, Miedema, T, Migenda, J, Milincic, R, Miller, W, Mills, J, Milne, C, Mineev, O, Miranda, O, Miryala, S, Mishra, C, Mishra, S, Mislivec, A, Mladenov, D, Mocioiu, I, Moffat, K, Moggi, N, Mohanta, R, Mohayai, T, Mokhov, N, Molina, J, Molina Bueno, L, Montanari, A, Montanari, C, Montanari, D, Montano Zetina, L, Moon, J, Mooney, M, Moor, A, Moreno, D, Morgan, B, Morris, C, Mossey, C, Motuk, E, Moura, C, Mousseau, J, Mu, W, Mualem, L, Mueller, J, Muether, M, Mufson, S, Muheim, F, Muir, A, Mulhearn, M, Muramatsu, H, Murphy, S, Musser, J, Nachtman, J, Nagu, S, Nalbandyan, M, Nandakumar, R, Naples, D, Narita, S, Navas-Nicolas, D, Nayak, N, Nebot-Guinot, M, Necib, L, Negishi, K, Nelson, J, Nesbit, J, Nessi, M, Newbold, D, Newcomer, M, Newhart, D, Nichol, R, Niner, E, Nishimura, K, Norman, A, Norrick, A, Northrop, R, Novella, P, Nowak, J, Oberling, M, Olivares Del Campo, A, Olivier, A, Onel, Y, Onishchuk, Y, Ott, J, Pagani, L, Pakvasa, S, Palamara, O, Palestini, S, Paley, J, Pallavicini, M, Palomares, C, Pantic, E, Paolone, V, Papadimitriou, V, Papaleo, R, Papanestis, A, Paramesvaran, S, Parke, S, Parsa, Z, Parvu, M, Pascoli, S, Pasqualini, L, Pasternak, J, Pater, J, Patrick, C, Patrizii, L, Patterson, R, Patton, S, Patzak, T, Paudel, A, Paulos, B, Paulucci, L, Pavlovic, Z, Pawloski, G, Payne, D, Pec, V, Peeters, S, Penichot, Y, Pennacchio, E, Penzo, A, Peres, O, Perry, J, Pershey, D, Pessina, G, Petrillo, G, Petta, C, Petti, R, Piastra, F, Pickering, L, Pietropaolo, F, Pillow, J, Pinzino, J, Plunkett, R, Poling, R, Pons, X, Poonthottathil, N, Pordes, S, 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Sarasty, C, Sarcevic, I, Savage, G, Savinov, V, Scaramelli, A, Scarff, A, Scarpelli, A, Schaffer, T, Schellman, H, Schlabach, P, Schmitz, D, Scholberg, K, Schukraft, A, Segreto, E, Sensenig, J, Seong, I, Sergi, A, Sergiampietri, F, Sgalaberna, D, Shaevitz, M, Shafaq, S, Shamma, M, Sharma, H, Sharma, R, Shaw, T, Shepherd-Themistocleous, C, Shin, S, Shooltz, D, Shrock, R, Simard, L, Simos, N, Sinclair, J, Sinev, G, Singh, J, Singh, V, Sipos, R, Sippach, F, Sirri, G, Sitraka, A, Siyeon, K, Smargianaki, D, Smith, A, Smith, E, Smith, P, Smolik, J, Smy, M, Snopok, P, Soares Nunes, M, Sobel, H, Soderberg, M, Solano Salinas, C, Soldner-Rembold, S, Solomey, N, Solovov, V, Sondheim, W, Sorel, M, Soto-Oton, J, Sousa, A, Soustruznik, K, Spagliardi, F, Spanu, M, Spitz, J, Spooner, N, Spurgeon, K, Staley, R, Stancari, M, Stanco, L, Steiner, H, Stewart, J, Stillwell, B, Stock, J, Stocker, F, Stokes, T, Strait, M, Strauss, T, Striganov, S, Stuart, A, Summers, D, Surdo, A, Susic, V, Suter, L, Sutera, C, Svoboda, R, Szczerbinska, B, Szelc, A, Talaga, R, Tanaka, H, Tapia Oregui, B, Tapper, A, Tariq, S, Tatar, E, Tayloe, R, Teklu, A, Tenti, M, Terao, K, Ternes, C, Terranova, F, Testera, G, Thea, A, Thompson, J, Thorn, C, Timm, S, Tonazzo, A, Torti, M, Tortola, M, Tortorici, F, Totani, D, Toups, M, Touramanis, C, Trevor, J, Trzaska, W, Tsai, Y, Tsamalaidze, Z, Tsang, K, Tsverava, N, Tufanli, S, Tull, C, Tyley, E, Tzanov, M, Uchida, M, Urheim, J, Usher, T, Vagins, M, Vahle, P, Valdiviesso, G, Valencia, E, Vallari, Z, Valle, J, Vallecorsa, S, Van Berg, R, Van De Water, R, Vanegas Forero, D, Varanini, F, Vargas, D, Varner, G, Vasel, J, Vasseur, G, Vaziri, K, Ventura, S, Verdugo, A, Vergani, S, Vermeulen, M, Verzocchi, M, Vieira De Souza, H, Vignoli, C, Vilela, C, Viren, B, Vrba, T, Wachala, T, Waldron, A, Wallbank, M, Wang, H, Wang, J, Wang, Y, Warburton, K, Warner, D, Wascko, M, Waters, D, Watson, A, Weatherly, P, Weber, A, Weber, M, Wei, H, Weinstein, A, Wenman, D, Wetstein, M, While, M, White, A, Whitehead, L, Whittington, D, Wilking, M, Wilkinson, C, Williams, Z, Wilson, F, Wilson, R, Wolcott, J, Wongjirad, T, Wood, K, Wood, L, Worcester, E, Worcester, M, Wret, C, Wu, W, Xiao, Y, Yang, G, Yang, T, Yershov, N, Yonehara, K, Young, T, Yu, B, Yu, J, Zaki, R, Zalesak, J, Zambelli, L, Zamorano, B, Zani, A, Zazueta, L, Zeller, G, Zennamo, J, Zeug, K, Zhang, C, Zhao, M, Zhivun, E, Zhu, G, Zimmerman, E, Zito, M, Zucchelli, S, Zuklin, J, Zutshi, V, Zwaska, R, Abi B., Acciarri R., Acero M.A., Adamov G., Adams D., Adinolfi M., Ahmad Z., Ahmed J., Alion T., Alonso Monsalve S., Alt C., Anderson J., Andreopoulos C., Andrews M.P., Andrianala F., Andringa S., Ankowski A., Antonova M., Antusch S., Aranda-Fernandez A., Ariga A., Arnold L.O., Arroyave M.A., Asaadi J., Aurisano A., Aushev V., Autiero D., Azfar F., Back H., Back J.J., Backhouse C., Baesso P., Bagby L., Bajou R., Balasubramanian S., Baldi P., Bambah B., Barao F., Barenboim G., Barker G.J., Barkhouse W., Barnes C., Barr G., Barranco Monarca J., Barros N., Barrow J.L., Bashyal A., Basque V., Bay F., Bazo Alba J.L., Beacom J.F., Bechetoille E., Behera B., Bellantoni L., Bellettini G., Bellini V., Beltramello O., Belver D., Benekos N., Bento Neves F., Berger J., Berkman S., Bernardini P., Berner R.M., Berns H., Bertolucci S., Betancourt M., Bezawada Y., Bhattacharjee M., Bhuyan B., Biagi S., Bian J., Biassoni M., Biery K., Bilki B., Bishai M., Bitadze A., Blake A., Blanco Siffert B., Blaszczyk F.D.M., Blazey G.C., Blucher E., Boissevain J., Bolognesi S., Bolton T., Bonesini M., Bongrand M., Bonini F., Booth A., Booth C., Bordoni S., Borkum A., Boschi T., Bostan N., Bour P., Boyd S.B., Boyden D., Bracinik J., Braga D., Brailsford D., Brandt A., Bremer J., Brew C., Brianne E., Brice S.J., Brizzolari C., Bromberg C., Brooijmans G., Brooke J., Bross A., Brunetti G., Buchanan N., Budd H., Caiulo D., Calafiura P., Calcutt J., Calin M., Calvez S., Calvo E., Camilleri L., Caminata A., Campanelli M., Caratelli D., Carini G., Carlus B., Carniti P., Caro Terrazas I., Carranza H., Castillo A., Castromonte C., Cattadori C., Cavalier F., Cavanna F., Centro S., Cerati G., Cervelli A., Cervera Villanueva A., Chalifour M., Chang C., Chardonnet E., Chatterjee A., Chattopadhyay S., Chaves J., Chen H., Chen M., Chen Y., Cherdack D., Chi C., Childress S., Chiriacescu A., Cho K., Choubey S., Christensen A., Christian D., Christodoulou G., Church E., Clarke P., Coan T.E., Cocco A.G., Coelho J.A.B., Conley E., Conrad J.M., Convery M., Corwin L., Cotte P., Cremaldi L., Cremonesi L., Crespo-Anadon J.I., Cristaldo E., Cross R., Cuesta C., Cui Y., Cussans D., Dabrowski M., Da Motta H., Da Silva Peres L., David C., David Q., Davies G.S., Davini S., Dawson J., De K., De Almeida R.M., Debbins P., De Bonis I., Decowski M.P., De Gouvea A., De Holanda P.C., De Icaza Astiz I.L., Deisting A., De Jong P., Delbart A., Delepine D., Delgado M., Dell'acqua A., De Lurgio P., De Mello Neto J.R.T., Demuth D.M., Dennis S., Densham C., Deptuch G., De Roeck A., De Romeri V., De Vries J.J., Dharmapalan R., Dias M., Diaz F., Diaz J.S., Di Domizio S., Di Giulio L., Ding P., Di Noto L., Distefano C., Diurba R., Diwan M., Djurcic Z., Dokania N., Dolinski M.J., Domine L., Douglas D., Drielsma F., Duchesneau D., Duffy K., Dunne P., Durkin T., Duyang H., Dvornikov O., Dwyer D.A., Dyshkant A.S., Eads M., Edmunds D., Eisch J., Emery S., Ereditato A., Escobar C.O., Escudero Sanchez L., Evans J.J., Ewart E., Ezeribe A.C., Fahey K., Falcone A., Farnese C., Farzan Y., Felix J., Fernandez-Martinez E., Fernandez Menendez P., Ferraro F., Fields L., Filkins A., Filthaut F., Fitzpatrick R.S., Flanagan W., Fleming B., Flight R., Fowler J., Fox W., Franc J., Francis K., Franco D., Freeman J., Freestone J., Fried J., Friedland A., Fuess S., Furic I., Furmanski A.P., Gago A., Gallagher H., Gallego-Ros A., Gallice N., Galymov V., Gamberini E., Gamble T., Gandhi R., Gandrajula R., Gao S., Garcia-Carballeira F., Garcia-Gamez D., 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Higuera A., Hill T., Hillier S.J., Himmel A., Hoff J., Hohl C., Holin A., Hoppe E., Horton-Smith G.A., Hostert M., Hourlier A., Howard B., Howell R., Huang J., Hugon J., Iles G., Ilic N., Iliescu A.M., Illingworth R., Ioannisian A., Itay R., Izmaylov A., James E., Jargowsky B., Jediny F., Jesus-Valls C., Ji X., Jiang L., Jimenez S., Jipa A., Joglekar A., Johnson C., Johnson R., Jones B., Jones S., Jung C.K., Junk T., Jwa Y., Kabirnezhad M., Kaboth A., Kadenko I., Kamiya F., Karagiorgi G., Karcher A., Karolak M., Karyotakis Y., Kasai S., Kasetti S.P., Kashur L., Kazaryan N., Kearns E., Keener P., Kelly K.J., Kemp E., Ketchum W., Kettell S.H., Khabibullin M., Khotjantsev A., Khvedelidze A., Kim D., King B., Kirby B., Kirby M., Klein J., Koehler K., Koerner L.W., Kohn S., Koller P.P., Kordosky M., Kosc T., Kose U., Kostelecky V.A., Kothekar K., Krennrich F., Kreslo I., Kudenko Y., Kudryavtsev V.A., Kulagin S., Kumar J., Kumar R., Kuruppu C., Kus V., Kutter T., Lambert A., Lande K., Lane C.E., Lang K., Langford T., Lasorak P., Last D., Lastoria C., Laundrie A., Lawrence A., Lazanu I., Lazur R., Le T., Learned J., Lebrun P., Lehmann Miotto G., Lehnert R., Leigui De Oliveira M.A., Leitner M., Leyton M., Li L., Li S., Li S.W., Li T., Li Y., Liao H., Lin C.S., Lin S., Lister A., Littlejohn B.R., Liu J., Lockwitz S., Loew T., Lokajicek M., Lomidze I., Long K., Loo K., Lorca D., Lord T., Losecco J.M., Louis W.C., Luk K.B., Luo X., Lurkin N., Lux T., Luzio V.P., MacFarland D., MacHado A.A., MacHado P., MacIas C.T., MacIer J.R., Maddalena A., Madigan P., Magill S., Mahn K., Maio A., Maloney J.A., Mandrioli G., Maneira J., Manenti L., Manly S., Mann A., Manolopoulos K., Manrique Plata M., Marchionni A., Marciano W., Marfatia D., Mariani C., Maricic J., Marinho F., Marino A.D., Marshak M., Marshall C., Marshall J., Marteau J., Martin-Albo J., Martinez N., Martinez Caicedo D.A., Martynenko S., Mason K., Mastbaum A., Masud M., Matsuno S., Matthews J., Mauger C., Mauri N., Mavrokoridis K., Mazza R., Mazzacane A., Mazzucato E., McCluskey E., McConkey N., McFarland K.S., McGrew C., McNab A., Mefodiev A., Mehta P., Melas P., Mellinato M., Mena O., Menary S., Mendez H., Menegolli A., Meng G., Messier M.D., Metcalf W., Mewes M., Meyer H., Miao T., Michna G., Miedema T., Migenda J., Milincic R., Miller W., Mills J., Milne C., Mineev O., Miranda O.G., Miryala S., Mishra C.S., Mishra S.R., Mislivec A., Mladenov D., Mocioiu I., Moffat K., Moggi N., Mohanta R., Mohayai T.A., Mokhov N., Molina J., Molina Bueno L., Montanari A., Montanari C., Montanari D., Montano Zetina L.M., Moon J., Mooney M., Moor A., Moreno D., Morgan B., Morris C., Mossey C., Motuk E., Moura C.A., Mousseau J., Mu W., Mualem L., Mueller J., Muether M., Mufson S., Muheim F., Muir A., Mulhearn M., Muramatsu H., Murphy S., Musser J., Nachtman J., Nagu S., Nalbandyan M., Nandakumar R., Naples D., Narita S., Navas-Nicolas D., Nayak N., Nebot-Guinot M., Necib L., Negishi K., Nelson J.K., Nesbit J., Nessi M., Newbold D., Newcomer M., Newhart D., Nichol R., Niner E., Nishimura K., Norman A., Norrick A., Northrop R., Novella P., Nowak J.A., Oberling M., Olivares Del Campo A., Olivier A., Onel Y., Onishchuk Y., Ott J., Pagani L., Pakvasa S., Palamara O., Palestini S., Paley J.M., Pallavicini M., Palomares C., Pantic E., Paolone V., Papadimitriou V., Papaleo R., Papanestis A., Paramesvaran S., Parke S., Parsa Z., Parvu M., Pascoli S., Pasqualini L., Pasternak J., Pater J., Patrick C., Patrizii L., Patterson R.B., Patton S.J., Patzak T., Paudel A., Paulos B., Paulucci L., Pavlovic Z., Pawloski G., Payne D., Pec V., Peeters S.J.M., Penichot Y., Pennacchio E., Penzo A., Peres O.L.G., Perry J., Pershey D., Pessina G., Petrillo G., Petta C., Petti R., Piastra F., Pickering L., Pietropaolo F., Pillow J., Pinzino J., Plunkett R., Poling R., Pons X., Poonthottathil N., Pordes S., Potekhin M., Potenza R., Potukuchi B.V.K.S., Pozimski J., Pozzato M., Prakash S., Prakash T., Prince S., Prior G., Pugnere D., Qi K., Qian X., Raaf J.L., Raboanary R., Radeka V., Rademacker J., Radics B., Radovic A., Rafique A., Raguzin E., Rai M., Rajaoalisoa M., Rakhno I., Rakotondramanana H.T., Rakotondravohitra L., Ramachers Y.A., Rameika R., Ramirez Delgado M.A., Ramson B., Rappoldi A., Raselli G., Ratoff P., Ravat S., Razafinime H., Real J.S., Rebel B., Redondo D., Reggiani-Guzzo M., Rehak T., Reichenbacher J., Reitzner S.D., Renshaw A., Rescia S., Resnati F., Reynolds A., Riccobene G., Rice L.C.J., Rielage K., Rigaut Y., Rivera D., Rochester L., Roda M., Rodrigues P., Rodriguez Alonso M.J., Rodriguez Rondon J., Roeth A.J., Rogers H., Rosauro-Alcaraz S., Rossella M., Rout J., Roy S., Rubbia A., Rubbia C., Russell B., Russell J., Ruterbories D., Saakyan R., Sacerdoti S., Safford T., Sahu N., Sala P., Samios N., Sanchez M.C., Sanders D.A., Sankey D., Santana S., Santos-Maldonado M., Saoulidou N., Sapienza P., Sarasty C., Sarcevic I., Savage G., Savinov V., Scaramelli A., Scarff A., Scarpelli A., Schaffer T., Schellman H., Schlabach P., Schmitz D., Scholberg K., Schukraft A., Segreto E., Sensenig J., Seong I., Sergi A., Sergiampietri F., Sgalaberna D., Shaevitz M.H., Shafaq S., Shamma M., Sharma H.R., Sharma R., Shaw T., Shepherd-Themistocleous C., Shin S., Shooltz D., Shrock R., Simard L., Simos N., Sinclair J., Sinev G., Singh J., Singh V., Sipos R., Sippach F.W., Sirri G., Sitraka A., Siyeon K., Smargianaki D., Smith A., Smith E., Smith P., Smolik J., Smy M., Snopok P., Soares Nunes M., Sobel H., Soderberg M., Solano Salinas C.J., Soldner-Rembold S., Solomey N., Solovov V., Sondheim W.E., Sorel M., Soto-Oton J., Sousa A., Soustruznik K., Spagliardi F., Spanu M., Spitz J., Spooner N.J.C., Spurgeon K., Staley R., Stancari M., Stanco L., Steiner H.M., Stewart J., Stillwell B., Stock J., Stocker F., Stokes T., Strait M., Strauss T., Striganov S., Stuart A., Summers D., Surdo A., Susic V., Suter L., Sutera C.M., Svoboda R., Szczerbinska B., Szelc A.M., Talaga R., Tanaka H.A., Tapia Oregui B., Tapper A., Tariq S., Tatar E., Tayloe R., Teklu A.M., Tenti M., Terao K., Ternes C.A., Terranova F., Testera G., Thea A., Thompson J.L., Thorn C., Timm S.C., Tonazzo A., Torti M., Tortola M., Tortorici F., Totani D., Toups M., Touramanis C., Trevor J., Trzaska W.H., Tsai Y.T., Tsamalaidze Z., Tsang K.V., Tsverava N., Tufanli S., Tull C., Tyley E., Tzanov M., Uchida M.A., Urheim J., Usher T., Vagins M.R., Vahle P., Valdiviesso G.A., Valencia E., Vallari Z., Valle J.W.F., Vallecorsa S., Van Berg R., Van De Water R.G., Vanegas Forero D., Varanini F., Vargas D., Varner G., Vasel J., Vasseur G., Vaziri K., Ventura S., Verdugo A., Vergani S., Vermeulen M.A., Verzocchi M., Vieira De Souza H., Vignoli C., Vilela C., Viren B., Vrba T., Wachala T., Waldron A.V., Wallbank M., Wang H., Wang J., Wang Y., Warburton K., Warner D., Wascko M., Waters D., Watson A., Weatherly P., Weber A., Weber M., Wei H., Weinstein A., Wenman D., Wetstein M., While M.R., White A., Whitehead L.H., Whittington D., Wilking M.J., Wilkinson C., Williams Z., Wilson F., Wilson R.J., Wolcott J., Wongjirad T., Wood K., Wood L., Worcester E., Worcester M., Wret C., Wu W., Xiao Y., Yang G., Yang T., Yershov N., Yonehara K., Young T., Yu B., Yu J., Zaki R., Zalesak J., Zambelli L., Zamorano B., Zani A., Zazueta L., Zeller G.P., Zennamo J., Zeug K., Zhang C., Zhao M., Zhivun E., Zhu G., Zimmerman E.D., Zito M., Zucchelli S., Zuklin J., Zutshi V., Zwaska R., UAM. Departamento de Física Teórica, Université Claude Bernard Lyon 1 (UCBL), Université de Lyon-Université de Lyon-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Centre National de la Recherche Scientifique (CNRS)-Université Paris Cité (UPCité), Université Paris-Sud - Paris 11 (UP11)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS), and Ministerio de Ciencia, Innovación y Universidades (España)
Subjects: Neutrino Oscillations. Neutrino detectors, Physics - Instrumentation and Detectors, Physics::Instrumentation and Detectors, far detector, 01 natural sciences, Physics, Particles & Fields, High Energy Physics - Experiment, charged current, High Energy Physics - Experiment (hep-ex), [PHYS.HEXP]Physics [physics]/High Energy Physics - Experiment [hep-ex], Particle Physics Experiments, Muon neutrino, neutrino/e: particle identification, Neutrino detectors, Detectors and Experimental Techniques, physics.ins-det, Charged current, neutrino: interaction, Informática, Physics, Telecomunicaciones, Neutrino oscillations, Neutrino interactions, neural network, DUNE, Deep Underground Neutrino Experiment, Instrumentation and Detectors (physics.ins-det), Experiment (hep-ex), Neutrino detector, Physical Sciences, CP violation, Neutrino, Particle Physics - Experiment, Particle physics, data analysis method, 530 Physics, neural network, Astrophysics::High Energy Astrophysical Phenomena, CONSERVATION, FOS: Physical sciences, Astronomy & Astrophysics, Deep Learning, neutrino: deep underground detector, neutrino physics, 0103 physical sciences, Object Detection, CP: violation, Deep Underground Neutrino Experiment, High Energy Physics, [PHYS.PHYS.PHYS-INS-DET]Physics [physics]/Physics [physics]/Instrumentation and Detectors [physics.ins-det], Neutrinos, 010306 general physics, Neutrino oscillation, neutrino/mu: particle identification, IOU, Science & Technology, DUNE, Neutrino interactions, 010308 nuclear & particles physics, hep-ex, High Energy Physics::Phenomenology, Física, Neutrino Interaction, Detector, 530 Physik, sensitivity, efficiency, High Energy Physics::Experiment, Electron neutrino
Abstract: The Deep Underground Neutrino Experiment is a next-generation neutrino oscillation experiment that aims to measure CP-violation in the neutrino sector as part of a wider physics program. A deep learning approach based on a convolutional neural network has been developed to provide highly efficient and pure selections of electron neutrino and muon neutrino charged-current interactions. The electron neutrino (antineutrino) selection efficiency peaks at 90% (94%) and exceeds 85% (90%) for reconstructed neutrino energies between 2–5 GeV. The muon neutrino (antineutrino) event selection is found to have a maximum efficiency of 96% (97%) and exceeds 90% (95%) efficiency for reconstructed neutrino energies above 2 GeV. When considering all electron neutrino and antineutrino interactions as signal, a selection purity of 90% is achieved. These event selections are critical to maximize the sensitivity of the experiment to CP-violating effects., Fermi Research Alliance, LLC (FRA) DE-AC02-07CH11359, National Council for Scientific and Technological Development (CNPq), Carlos Chagas Filho Foundation for Research Support of the State of Rio de Janeiro (FAPERJ), FAPEG, Brazil, Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP), Canada Foundation for Innovation, Institute of Particle Physics, Canada, Natural Sciences and Engineering Research Council of Canada (NSERC), CERN, Ministry of Education, Youth & Sports - Czech Republic Czech Republic Government, ERDF, European Union, H2020-EU, European Union, MSCA, European Union, Centre National de la Recherche Scientifique (CNRS), French Atomic Energy Commission, Istituto Nazionale di Fisica Nucleare (INFN), Portuguese Foundation for Science and Technology European Commission, NRF, South Korea, Comunidad de Madrid, La Caixa Foundation, Spanish Government, State Secretariat for Education, Research and Innovation, Switzerland, Swiss National Science Foundation (SNSF), Turkiye Bilimsel ve Teknolojik Arastirma Kurumu (TUBITAK), Royal Society of London, UKRI/STFC, United Kingdom, United States Department of Energy (DOE), National Science Foundation (NSF)
Published: 2020

29. Spin cascade and doming in ferric hemes: Femtosecond X-ray absorption and X-ray emission studies

Author: Georgios Pamfilidis, Dmitry Khakhulin, Christian Bressler, Gregor Knopp, Claudio Cirelli, Jakub Szlachetko, Jérémy R. Rouxel, Mykola Biednov, Frederico A. Lima, Rebecca A. Ingle, Philip J. M. Johnson, Camila Bacellar, Christopher Arrell, Angel Rodriguez-Fernandez, Wojciech Gawelda, Oliviero Cannelli, Majed Chergui, Samuel Menzi, Dominik Kinschel, Katharina Kubicek, Giulia F. Mancini, and Christopher J. Milne
Subjects: inorganic chemicals, ferric hemoproteins, spectroscopy, Hemeprotein, ultrafast, Iron, Doming, x-ray spectroscopy, spin states, Photochemistry, nitric-oxide-binding, cytochrome-c, Ferrous, chemistry.chemical_compound, Protein Domains, medicine, Humans, Respiratory function, Heme, doming, Multidisciplinary, biology, vibrational-relaxation, Chemistry, Nitric oxide binding, Cytochrome c, carbon-monoxide, resolved resonance raman, low-temperature, Cytochromes c, Spectrometry, X-Ray Emission, dynamics, electron-transfer, Kinetics, X-Ray Absorption Spectroscopy, myoglobin recombination, biology.protein, Commentary, Ferric, medicine.drug
Abstract: The structure-function relationship is at the heart of biology, and major protein deformations are correlated to specific functions. For ferrous heme proteins, doming is associated with the respiratory function in hemoglobin and myoglobins. Cytochrome c (Cyt c) has evolved to become an important electron-transfer protein in humans. In its ferrous form, it undergoes ligand release and doming upon photoexcitation, but its ferric form does not release the distal ligand, while the return to the ground state has been attributed to thermal relaxation. Here, by combining femtosecond Fe K-alpha and K-beta X-ray emission spectroscopy (XES) with Fe K-edge X-ray absorption near-edge structure (XANES), we demonstrate that the photocycle of ferric Cyt c is entirely due to a cascade among excited spin states of the iron ion, causing the ferric heme to undergo doming, which we identify. We also argue that this pattern is common to a wide diversity of ferric heme proteins, raising the question of the biological relevance of doming in such proteins.
Published: 2020

30. Volume IV The DUNE far detector single-phase technology

Author: L. Di Giulio, J. Martin-Albo, S. Ravat, W. Mu, D. Marfatia, T. Kosc, D. Autiero, Poonam Mehta, A. Borkum, N. McConkey, G. Karagiorgi, Robert Wilson, L. M. Cremaldi, Stephen P. Gent, T. Young, Julián Félix, D. MacFarland, Andrew Smith, M. Manrique Plata, J. Freestone, D. Rivera, B. Stillwell, Marco Verzocchi, A. Lambert, Orlando L. G. Peres, K. Gollwitzer, E. Kemp, G. Yang, I. Kreslo, F. Varanini, M. Chalifour, A. Holin, S. J. Patton, R. J. Nichol, Giovanni Bellettini, V. A. Kudryavtsev, M. Sorel, E. Church, S. Kasai, H. O. Back, A. Lister, S. Santana, C. Mariani, Carlos Escobar, J. C. Freeman, Kaushik De, M. J. Rodriguez Alonso, M. A. Acero, A. Christensen, G. S. Varner, S. Sacerdoti, D. Shooltz, Seodong Shin, M. Santos-Maldonado, T. Schaffer, Jeremy Wolcott, J. Vasel, J. A. Gonzalez-Cuevas, J. Franc, C. Mossey, Jonas Rademacker, G. P. Zeller, Joshua Barrow, John Marshall, Alessandro Thea, H. A. Tanaka, W. C. Louis, E. Hazen, Armin Karcher, D. Smargianaki, Christopher L. Marshall, M. Soderberg, A. C. Weber, Christopher J. Milne, E. Brianne, A. Aranda-Fernandez, J. Calcutt, K. Warburton, M. Nalbandyan, Dave Sankey, J. Asaadi, F. Diaz, E. Valencia, B. Kirby, A. Bross, K. Koehler, M. A. Uchida, Y. Bezawada, D. Warner, C. E. Thorn, Srubabati Goswami, Z. Williams, Gregory Iles, A. Friedland, K. M. Heeger, V. P. Luzio, G. C. Blazey, J. Barranco Monarca, Carl Grace, A. M. Gago, E. James, M. Newcomer, H. W. Sobel, Roberto Gutiérrez, C. Vignoli, R. Hatcher, M. Zhao, F. Cavalier, M. A. Hernandez Morquecho, N. Poonthottathil, Ara Ioannisian, W. Metcalf, T. Wongjirad, H. T. Rakotondramanana, D. Cherdack, M. A. Ramirez Delgado, R. Diurba, G. Christodoulou, S. Calvez, T. Durkin, H. Y. Wei, M. Muether, S. Roy, A. Caminata, A. Scarpelli, Christopher Brew, Pavel Snopok, Y. Rigaut, L. Escudero Sanchez, K. Kothekar, W. Flanagan, V. Papadimitriou, S. J. Brice, Nicolas Lurkin, M. V. Diwan, Andrew White, S. Berkman, H. Muramatsu, Z. Pavlovic, A. A. Machado, Christian Farnese, A. Mastbaum, Alfredo G. Cocco, G. Zhu, S. Centro, S. Henry, J. Rout, P. de Jong, H. Carranza, Milos Lokajicek, K. Nishimura, A. Delbart, N. J. C. Spooner, C. McGrew, E. Pantic, Mario Campanelli, David Cussans, B. T. Fleming, K. Negishi, F. Spagliardi, J. Nesbit, André Rubbia, Akitaka Ariga, Marvin L Marshak, F. Pietropaolo, F. D. M. Blaszczyk, T. Hasegawa, Kate Scholberg, O. Gogota, R. Poling, Simon Jones, A. Tonazzo, M. P. Andrews, R. Petti, S. Bertolucci, M. Bonesini, A. F. Moor, C. Barnes, A. S. Hesam, S. H. Kettell, M. Bongrand, M. R. While, D. J. Payne, C. Gotti, A. Chiriacescu, Paul Keener, Leigh H. Whitehead, James Stewart, A. Mazzacane, L. W. Koerner, T. Rehak, C. Andreopoulos, F. Terranova, Jaroslaw Pasternak, E. Raguzin, L. C. J. Rice, J. L. Bazo Alba, S. Li, J. Hartnell, M. Potekhin, N. Moggi, D. J. Summers, J. Berger, L. Cremonesi, Katsuya Yonehara, T. E. Coan, Claire Shepherd-Themistocleous, B. Radics, Karol Hennessy, S. Söldner-Rembold, C. S. Lin, L. Greenler, B. Guo, Frank Filthaut, R. B. Patterson, E. Pennacchio, E. Zhivun, C. Cuesta, T. Loew, G. Prior, D. Duchesneau, Lina Necib, S. Rescia, W. Gu, Andrés Castillo, N. Kazaryan, O. G. Miranda, C. Patrick, Robert Shrock, José W. F. Valle, J. Reichenbacher, D. A. Sanders, John F. Beacom, S. Tufanli, S. Ventura, Riccardo Papaleo, J. Zennamo, A. De Roeck, M. Calin, P. Ding, Alessandro Menegolli, B. V. K. S. Potukuchi, T. Le, T. Wachala, L. O. Arnold, J. R. Macier, A. M. Teklu, E. Blucher, L. Hertel, F. W. Sippach, S. Childress, T. Miao, P. Fernandez Menendez, J. Han, R. Gandrajula, C. Y. Chi, Marzio Nessi, Aldo Penzo, Ina Sarcevic, Kendall Mahn, Jorge Molina, F. Bonini, Eric W. Hoppe, M. Groh, Barry King, R. Mazza, Keith Rielage, Patrick Dunne, M. Mellinato, D. Lorca, R. Guenette, F. Bento Neves, L. Pickering, Manuel Alejandro Segura Delgado, J. J. Russell, H. R. Gallagher, J. Zuklin, Steven Gardiner, P. Madigan, D. Douglas, Daniel Gastler, S. Manly, P. Hamilton, L. 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A., Terranova, F., Testera, G., Thea, A., Thompson, J. L., Thorn, C., Timm, S., Tonazzo, A., Torti, M., Tortola, M., Tortorici, F., Totani, D., Toups, M., Touramanis, C., Trevor, J., Trzaska, W. H., Tsai, Y. T., Tsamalaidze, Z., Tsang, K., Tsverava, N., Tufanli, S., Tull, C., Tyley, E., Tzanov, M., Uchida, M. A., Urheim, J., Usher, T., Vagins, M., Vahle, P., Valdiviesso, G., Valencia, E., Vallari, Z., Valle, J. W., Vallecorsa, S., Berg, R. Van, de Water, R. G. Van, Forero, D. Vanega, Varanini, F., Vargas, D., Varner, G., Vasel, J., Vasseur, G., Vaziri, K., Ventura, S., Verdugo, A., Vergani, S., Vermeulen, M. A., Verzocchi, M., de Souza, H. Vieira, Vignoli, C., Vilela, C., Viren, B., Vrba, T., Wachala, T., Waldron, A. V., Wallbank, M., Wang, H., Wang, J., Wang, Y., Warburton, K., Warner, D., Wascko, M., Waters, D., Watson, A., Weatherly, P., Weber, A., Weber, M., Wei, H., Weinstein, A., Wenman, D., Wetstein, M., While, M. R., White, A., Whitehead, L. H., Whittington, D., Wilking, M. J., Wilkinson, C., Williams, Z., Wilson, F., Wilson, R. J., Wolcott, J., Wongjirad, T., Wood, K., Wood, L., Worcester, E., Worcester, M., Wret, C., Wu, W., Xiao, Y., Yang, G., Yang, T., Yershov, N., Yonehara, K., Young, T., Yu, B., Yu, J., Zalesak, J., Zambelli, L., Zamorano, B., Zani, A., Zazueta, L., Zeller, G., Zennamo, J., Zeug, K., Zhang, C., Zhao, M., Zhivun, E., Zhu, G., Zimmerman, E. D., Zito, M., Zucchelli, S., Zuklin, J., Zutshi, V., Zwaska, R., Abi B., Acciarri R., Acero M.A., Adamov G., Adams D., Adinolfi M., Ahmad Z., Ahmed J., Alion T., Monsalve S.A., Alt C., Anderson J., Andreopoulos C., Andrews M., Andrianala F., Andringa S., Ankowski A., Antonova M., Antusch S., Aranda-Fernandez A., Ariga A., Arnold L.O., Arroyave M.A., Asaadi J., Aurisano A., Aushev V., Autiero D., Azfar F., Back H., Back J.J., Backhouse C., Baesso P., Bagby L., Bajou R., Balasubramanian S., Baldi P., Bambah B., Barao F., Barenboim G., Barker G., Barkhouse W., Barnes C., Barr G., Monarca J.B., Barros N., Barrow J.L., Bashyal A., Basque V., Bay F., Alba J.B., Beacom J.F., Bechetoille E., Behera B., Bellantoni L., Bellettini G., Bellini V., Beltramello O., Belver D., Benekos N., Neves F.B., Berger J., Berkman S., Bernardini P., Berner R.M., Berns H., Bertolucci S., Betancourt M., Bezawada Y., Bhattacharjee M., Bhuyan B., Biagi S., Bian J., Biassoni M., Biery K., Bilki B., Bishai M., Bitadze A., Blake A., Siffert B.B., Blaszczyk F., Blazey G., Blucher E., Boissevain J., Bolognesi S., Bolton T., Bonesini M., Bongrand M., Bonini F., Booth A., Booth C., Bordoni S., Borkum A., Boschi T., Bostan N., Bour P., Boyd S., Boyden D., Bracinik J., Braga D., Brailsford D., Brandt A., Bremer J., Brew C., Brianne E., Brice S.J., Brizzolari C., Bromberg C., Brooijmans G., Brooke J., Bross A., Brunetti G., Buchanan N., Budd H., Caiulo D., Calafiura P., Calcutt J., Calin M., Calvez S., Calvo E., Camilleri L., Caminata A., Campanelli M., Caratelli D., Carini G., Carlus B., Carniti P., Terrazas I.C., Carranza H., Castillo A., Castromonte C., Cattadori C., Cavalier F., Cavanna F., Centro S., Cerati G., Cervelli A., Villanueva A.C., Chalifour M., Chang C., Chardonnet E., Chatterjee A., Chattopadhyay S., Chaves J., Chen H., Chen M., Chen Y., Cherdack D., Chi C., Childress S., Chiriacescu A., Cho K., Choubey S., Christensen A., Christian D., Christodoulou G., Church E., Clarke P., Coan T.E., Cocco A.G., Coelho J., Conley E., Conrad J., Convery M., Corwin L., Cotte P., Cremaldi L., Cremonesi L., Crespo-Anadon J.I., Cristaldo E., Cross R., Cuesta C., Cui Y., Cussans D., Dabrowski M., Motta H.D., Peres L.D.S., David Q., Davies G.S., Davini S., Dawson J., De K., Almeida R.M.D., Debbins P., Bonis I.D., Decowski M., Gouvea A.D., Holanda P.C.D., Astiz I.L.D.I., Deisting A., Jong P.D., Delbart A., Delepine D., Delgado M., Dell'acqua A., Lurgio P.D., Neto J.R.D.M., Demuth D.M., Dennis S., Densham C., Deptuch G., Roeck A.D., Romeri V.D., Vries J.D., Dharmapalan R., Dias M., Diaz F., Diaz J., Domizio S.D., Giulio L.D., Ding P., Noto L.D., Distefano C., Diurba R., Diwan M., Djurcic Z., Dokania N., Dolinski M., Domine L., Douglas D., Drielsma F., Duchesneau D., Duffy K., Dunne P., Durkin T., Duyang H., Dvornikov O., Dwyer D., Dyshkant A., Eads M., Edmunds D., Eisch J., Emery S., Ereditato A., Escobar C., Sanchez L.E., Evans J.J., Ewart E., Ezeribe A.C., Fahey K., Falcone A., Farnese C., Farzan Y., Felix J., Fernandez-Martinez E., Menendez P.F., Ferraro F., Fields L., Filkins A., Filthaut F., Fitzpatrick R.S., Flanagan W., Fleming B., Flight R., Fowler J., Fox W., Franc J., Francis K., Franco D., Freeman J., Freestone J., Fried J., Friedland A., Fuess S., Furic I., Furmanski A.P., Gago A., Gallagher H., Gallego-Ros A., Gallice N., Galymov V., Gamberini E., Gamble T., Gandhi R., Gandrajula R., Gao S., Garcia-Gamez D., Garcia-Peris M.A., Gardiner S., Gastler D., Ge G., Gelli B., Gendotti A., Gent S., Ghorbani-Moghaddam Z., Gibin D., Gil-Botella I., Girerd C., Giri A., Gnani D., Gogota O., Gold M., Gollapinni S., Gollwitzer K., Gomes R.A., Bermeo L.G., Fajardo L.S.G., Gonnella F., Gonzalez-Cuevas J., Goodman M.C., Goodwin O., Goswami S., Gotti C., Goudzovski E., Grace C., Graham M., Gramellini E., Gran R., Granados E., Grant A., Grant C., Gratieri D., Green P., Green S., Greenler L., Greenwood M., Greer J., Griffith C., Groh M., Grudzinski J., Grzelak K., Gu W., Guarino V., Guenette R., Guglielmi A., Guo B., Guthikonda K., Gutierrez R., Guzowski P., Guzzo M.M., Gwon S., Habig A., Hackenburg A., Hadavand H., Haenni R., Hahn A., Haigh J., Haiston J., Hamernik T., Hamilton P., Han J., Harder K., Harris D.A., Hartnell J., Hasegawa T., Hatcher R., Hazen E., Heavey A., Heeger K.M., Hennessy K., Henry S., Morquecho M.H., Herner K., Hertel L., Hesam A.S., Hewes J., Pichardo A.H., Hill T., Hillier S.J., Himmel A., Hoff J., Hohl C., Holin A., Hoppe E., Horton-Smith G.A., Hostert M., Hourlier A., Howard B., Howell R., Huang J., Hugon J., Iles G., Iliescu A.M., Illingworth R., Ioannisian A., Itay R., Izmaylov A., James E., Jargowsky B., Jediny F., Jesus-Valls C., Ji X., Jiang L., Jimenez S., Jipa A., Joglekar A., Johnson C., Johnson R., Jones B., Jones S., Jung C., Junk T., Jwa Y., Kabirnezhad M., Kaboth A., Kadenko I., Kamiya F., Karagiorgi G., Karcher A., Karolak M., Karyotakis Y., Kasai S., Kasetti S.P., Kashur L., Kazaryan N., Kearns E., Keener P., Kelly K.J., Kemp E., Ketchum W., Kettell S., Khabibullin M., Khotjantsev A., Khvedelidze A., Kim D., King B., Kirby B., Kirby M., Klein J., Koehler K., Koerner L.W., Kohn S., Koller P.P., Kordosky M., Kosc T., Kose U., Kostelecky V., Kothekar K., Krennrich F., Kreslo I., Kudenko Y., Kudryavtsev V., Kulagin S., Kumar J., Kumar R., Kuruppu C., Kus V., Kutter T., Lambert A., Lande K., Lane C.E., Lang K., Langford T., Lasorak P., Last D., Lastoria C., Laundrie A., Lawrence A., Lazanu I., Lazur R., Le T., Learned J., Lebrun P., Miotto G.L., Lehnert R., De Oliveira M.L., Leitner M., Leyton M., Li L., Li S., Li T., Li Y., Liao H., Lin C., Lin S., Lister A., Littlejohn B.R., Liu J., Lockwitz S., Loew T., Lokajicek M., Lomidze I., Long K., Loo K., Lorca D., Lord T., Losecco J., Louis W.C., Luk K., Luo X., Lurkin N., Lux T., Luzio V.P., MacFarland D., MacHado A., MacHado P., MacIas C., MacIer J., Maddalena A., Madigan P., Magill S., Mahn K., Maio A., Maloney J.A., Mandrioli G., Maneira J.C., 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Sacerdoti S., Safford T., Sahu N., Sala P., Samios N., Sanchez M., Sanders D.A., Sankey D., Santana S., Santos-Maldonado M., Saoulidou N., Sapienza P., Sarasty C., Sarcevic I., Savage G., Savinov V., Scaramelli A., Scarff A., Scarpelli A., Schaffer T., Schellman H., Schlabach P., Schmitz D., Scholberg K., Schukraft A., Segreto E., Sensenig J., Seong I., Sergi A., Sergiampietri F., Sgalaberna D., Shaevitz M., Shafaq S., Shamma M., Sharma H.R., Sharma R., Shaw T., Shepherd-Themistocleous C., Shin S., Shooltz D., Shrock R., Simard L., Simos N., Sinclair J., Sinev G., Singh J., Singh V., Sipos R., Sippach F., Sirri G., Sitraka A., Siyeon K., Smargianaki D., Smith A., Smith E., Smith P., Smolik J., Smy M., Snopok P., Nunes M.S., Sobel H., Soderberg M., Salinas C.J.S., Soldner-Rembold S., Solomey N., Solovov V., Sondheim W.E., Sorel M., Soto-Oton J., Sousa A., Soustruznik K., Spagliardi F., Spanu M., Spitz J., Spooner N.J., Spurgeon K., Staley R., Stancari M., Stanco L., Steiner H., Stewart J., Stillwell B., Stock J., Stocker F., Stokes T., Strait M., Strauss T., Striganov S., Stuart A., Summers D., Surdo A., Susic V., Suter L., Sutera C., Svoboda R., Szczerbinska B., Szelc A., Talaga R., Tanaka H., Oregui B.T., Tapper A., Tariq S., Tatar E., Tayloe R., Teklu A., Tenti M., Terao K., Ternes C.A., Terranova F., Testera G., Thea A., Thompson J.L., Thorn C., Timm S., Tonazzo A., Torti M., Tortola M., Tortorici F., Totani D., Toups M., Touramanis C., Trevor J., Trzaska W.H., Tsai Y.T., Tsamalaidze Z., Tsang K., Tsverava N., Tufanli S., Tull C., Tyley E., Tzanov M., Uchida M.A., Urheim J., Usher T., Vagins M., Vahle P., Valdiviesso G., Valencia E., Vallari Z., Valle J.W., Vallecorsa S., Berg R.V., De Water R.G.V., Forero D.V., Varanini F., Vargas D., Varner G., Vasel J., Vasseur G., Vaziri K., Ventura S., Verdugo A., Vergani S., Vermeulen M.A., Verzocchi M., De Souza H.V., Vignoli C., Vilela C., Viren B., Vrba T., Wachala T., Waldron A.V., Wallbank M., Wang H., Wang J., Wang Y., Warburton K., Warner D., Wascko M., Waters D., Watson A., Weatherly P., Weber A., Weber M., Wei H., Weinstein A., Wenman D., Wetstein M., While M.R., White A., Whitehead L.H., Whittington D., Wilking M.J., Wilkinson C., Williams Z., Wilson F., Wilson R.J., Wolcott J., Wongjirad T., Wood K., Wood L., Worcester E., Worcester M., Wret C., Wu W., Xiao Y., Yang G., Yang T., Yershov N., Yonehara K., Young T., Yu B., Yu J., Zalesak J., Zambelli L., Zamorano B., Zani A., Zazueta L., Zeller G., Zennamo J., Zeug K., Zhang C., Zhao M., Zhivun E., Zhu G., Zimmerman E.D., Zito M., Zucchelli S., Zuklin J., Zutshi V., and Zwaska R.
Subjects: Technology, 530 Physics, media_common.quotation_subject, Neutrino oscillations, liquid Argon TPC, DUNE technical design report, single phase LArTPC, Electrons, FREE-ELECTRONS, 01 natural sciences, 7. Clean energy, 09 Engineering, 030218 nuclear medicine & medical imaging, Standard Model, 03 medical and health sciences, neutrino, 0302 clinical medicine, LIQUID ARGON, 0103 physical sciences, Grand Unified Theory, High Energy Physics, Aerospace engineering, Instrumentation, Instruments & Instrumentation, Mathematical Physics, media_common, Physics, Science & Technology, 02 Physical Sciences, 010308 nuclear & particles physics, business.industry, Detector, Lıquıd Argonfree, Nuclear & Particles Physics, Symmetry (physics), Universe, Long baseline neutrino experiment, CP violation, Antimatter, Neutrino, business, Event (particle physics)
Abstract: This document was prepared by the DUNE collaboration using the resources of the Fermi National Accelerator Laboratory (Fermilab), a U.S. Department of Energy, Office of Science, HEP User Facility. Fermilab is managed by Fermi Research Alliance, LLC (FRA), acting under Contract No. DE-AC02-07CH11359. The DUNE collaboration also acknowledges the international, national, and regional funding agencies supporting the institutions who have contributed to completing this Technical Design Report., The preponderance of matter over antimatter in the early universe, the dynamics of the supernovae that produced the heavy elements necessary for life, and whether protons eventually decay—these mysteries at the forefront of particle physics and astrophysics are key to understanding the early evolution of our universe, its current state, and its eventual fate. DUNE is an international world-class experiment dedicated to addressing these questions as it searches for leptonic charge-parity symmetry violation, stands ready to capture supernova neutrino bursts, and seeks to observe nucleon decay as a signature of a grand unified theory underlying the standard model. Central to achieving DUNE's physics program is a far detector that combines the many tens-of-kiloton fiducial mass necessary for rare event searches with sub-centimeter spatial resolution in its ability to image those events, allowing identification of the physics signatures among the numerous backgrounds. In the single-phase liquid argon time-projection chamber (LArTPC) technology, ionization charges drift horizontally in the liquid argon under the influence of an electric field towards a vertical anode, where they are read out with fine granularity. A photon detection system supplements the TPC, directly enhancing physics capabilities for all three DUNE physics drivers and opening up prospects for further physics explorations. The DUNE far detector technical design report (TDR) describes the DUNE physics program and the technical designs of the single- and dual-phase DUNE liquid argon TPC far detector modules. Volume IV presents an overview of the basic operating principles of a single-phase LArTPC, followed by a description of the DUNE implementation. Each of the subsystems is described in detail, connecting the high-level design requirements and decisions to the overriding physics goals of DUNE., Fermi Research Alliance, LLC (FRA) DE-AC02-07CH11359
Published: 2020

31. Volume I. Introduction to DUNE

Author: E. Hazen, Armin Karcher, D. Smargianaki, Christopher L. Marshall, K. Spurgeon, M. Gold, C. Vignoli, C. J. Solano Salinas, M. J. Wilking, K. Kothekar, G. Sirri, Evgueni Goudzovski, H. Mendez, W. Flanagan, V. Papadimitriou, D. Redondo, S. R. Mishra, Y.-J. Jwa, G. Petrillo, M. Spanu, Xiaolu Ji, O. V. Mineev, M. Bishai, S. Menary, L. Molina Bueno, P. C. de Holanda, H. Berns, A. Gendotti, A. M. Szelc, R. Gandhi, A. Himmel, M. Rajaoalisoa, P. Bour, N. Kazaryan, L. Mualem, Gareth J. Barker, C. Cattadori, S. Ravat, W. Mu, D. Marfatia, T. Miedema, Kendall Mahn, Jorge Molina, Filippo Resnati, S. Magill, E. Niner, D. Autiero, Poonam Mehta, John Evans, J. S. Díaz, P. Novella, J. Fowler, G. Karagiorgi, S. J. M. Peeters, William J. Marciano, S. Bordoni, James Mueller, J. Martín-Albo, W. Fox, K. Grzelak, C. Hohl, R. Haenni, S. Alonso Monsalve, B. Howard, G. Ge, Alexander Tapper, Thomas Strauss, Silvia Pascoli, B. Stillwell, A. Lambert, A. Holin, K. V. Tsang, J. Maneira, R.A. Rameika, Juraj Bracinik, C. Wret, M. Tenti, Alberto Cervelli, Sukalyan Chattopadhyay, Laura Dominé, K. Herner, Hem Raj Sharma, S. Kasai, A. Higuera Pichardo, M. Betancourt, A. Scarff, R. Northrop, M. V. Diwan, D. J. Payne, C. Gotti, M. A. Vermeulen, R. M. Berner, J. J. De Vries, S. Shafaq, Yu. G. Kudenko, L. Pickering, B. Bhuyan, C. Kuruppu, Janet Conrad, D. Brailsford, R. Van Berg, J. Chaves, B. Paulos, R. Sipos, E. Pennacchio, F. W. Sippach, T. Li, S. Striganov, Laura Paulucci, S. Manly, P. Hamilton, R. G. Van de Water, R. Nandakumar, B. Szczerbinska, D. Cherdack, H. Carranza, Milos Lokajicek, K. Nishimura, E. Kearns, A. C. Ezeribe, J. Hoff, A. McNab, A. Stuart, G. Vasseur, C. Petta, M. Wetstein, M. M. Khabibullin, A. Bitadze, Yichen Li, G. Brunetti, L. Suter, L. Pasqualini, S. Martynenko, Ph. Lebrun, B. Morgan, L. Patrizii, A. Guglielmi, D. Wenman, S. C. Timm, R. Sharma, R. Saakyan, R. Gran, C. McGrew, C. Andreopoulos, A. Mann, F. Terranova, C. Cuesta, O. G. Miranda, C. Patrick, José W. F. Valle, A. Booth, G. Mandrioli, J. A. Nowak, S. Tufanli, R. Bajou, J. Urheim, J. Bian, Yasaman Farzan, M. Roda, J. G. Boissevain, J. Smolik, Thorsten Lux, L. Fields, D. Franco, S. P. Kasetti, M. Soares Nunes, A. Maddalena, M. Antonova, E. Kemp, N. Solomey, Laura Manenti, K. Francis, M. H. Shaevitz, N. Barros, C. Booth, I. Caro Terrazas, R. Itay, E. Ewart, R. J. Nichol, D. Totani, P. Snopok, M. Sorel, Kaushik De, M. Soderberg, A. C. Weber, Jonas Rademacker, E. Brianne, M. J. Rodriguez Alonso, T. Boschi, Sandhya Choubey, D. Montanari, Giorgio Riccobene, A. Mefodiev, M. A. Acero, A. Rappoldi, F. F. Wilson, Nektarios Benekos, Piera Sapienza, V. Savinov, P. Melas, Kenneth Long, Jianbei Liu, C. Mossey, Renato Potenza, M. Shamma, N. P. Samios, Y. Penichot, C. Bromberg, W. C. Louis, V. Paolone, V. Pec, J. Pillow, S. Vergani, S. Balasubramanian, B. Carlus, D. Boyden, Kam-Biu Luk, Simon Lin, Sofia Andringa, F. Jediny, K. Qi, K. Wood, M. Toups, Haleh Khani Hadavand, B. 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Subjects: detector: technology, deep underground detector [neutrino], 530 Physics, Physics::Instrumentation and Detectors, Data management, media_common.quotation_subject, far detector, Long baseline neutrino experiment CP violation, 01 natural sciences, 030218 nuclear medicine & medical imaging, Neutrino oscillations. Neutrino Detectors. CP violation. Matter stability, design [detector], 03 medical and health sciences, neutrino, neutrino: deep underground detector, 0302 clinical medicine, near detector, 0103 physical sciences, Deep Underground Neutrino Experiment, ddc:610, Neutrino oscillation, Instrumentation, detector: design, Mathematical Physics, activity report, media_common, 010308 nuclear & particles physics, business.industry, Detector, Volume (computing), Modular design, time projection chamber: liquid argon, Universe, technology [detector], liquid argon [time projection chamber], Systems engineering, High Energy Physics::Experiment, Neutrino oscillations, DUNE technical design report, executive summary, detector technologies, data management, Neutrino, business
Abstract: Journal of Instrumentation 15(08), T08008 (1-228) (2020). doi:10.1088/1748-0221/15/08/T08008, The preponderance of matter over antimatter in the early universe, the dynamics of the supernovae that produced the heavy elements necessary for life, and whether protons eventually decay—these mysteries at the forefront of particle physics and astrophysics are key to understanding the early evolution of our universe, its current state, and its eventual fate. The Deep Underground Neutrino Experiment (DUNE) is an international world-class experiment dedicated to addressing these questions as it searches for leptonic charge-parity symmetry violation, stands ready to capture supernova neutrino bursts, and seeks to observe nucleon decay as a signature of a grand unified theory underlying the standard model. The DUNE far detector technical design report (TDR) describes the DUNE physics program and the technical designs of the single- and dual-phase DUNE liquid argon TPC far detector modules. This TDR is intended to justify the technical choices for the far detector that flow down from the high-level physics goals through requirements at all levels of the Project. Volume I contains an executive summary that introduces the DUNE science program, the far detector and the strategy for its modular designs, and the organization and management of the Project. The remainder of Volume I provides more detail on the science program that drives the choice of detector technologies and on the technologies themselves. It also introduces the designs for the DUNE near detector and the DUNE computing model, for which DUNE is planning design reports. Volume II of this TDR describes DUNE's physics program in detail. Volume III describes the technical coordination required for the far detector design, construction, installation, and integration, and its organizational structure. Volume IV describes the single-phase far detector technology. A planned Volume V will describe the dual-phase technology., Published by Inst. of Physics, London
Published: 2020

32. Ultrafast Charge Transfer and Electron Delocalization in a Cyanide-Bridged Ru-Ru Dimer Investigated with Femtosecond Transient X-Ray and IR Spectroscopies

Author: Robert B. Weakly, Claudio Cirelli, Dimosthenis Sokaras, Niranjan Govind, Munira Khalil, Elisa Biasin, Robert W. Schoenlein, Benjamin I. Poulter, Christopher J. Milne, Phillip Johnson, Jason W. Sandwisch, Sven Augustin, Ivan Usov, Amy Cordones-Hahn, Chelsea Liekhus-Schmaltz, Marco Reinhard, Dmitry Ozerov, Christopher Arrell, Roberto Alonso Mori, and Gregor Knopp
Subjects: chemistry.chemical_compound, Electron density, Delocalized electron, Valence (chemistry), Materials science, chemistry, Dimer, Excited state, Femtosecond, Infrared spectroscopy, Electron, Photochemistry
Abstract: Transient IR and X-Ray spectroscopies were used to investigate excited state delocalization of a mixed valence Ru based donor-bridge-acceptor complex on a femtosecond timescale revealing the role of the electron density on the Ru-CN-Ru fragment.
Published: 2020

33. First results on ProtoDUNE-SP liquid argon time projection chamber performance from a beam test at the CERN Neutrino Platform

Author: Francesco Tortorici, Andrea Zani, J. Moon, P. E. L. Clarke, C. Palomares, M. B. Smy, M. Oberling, J. Migenda, F. Pietropaolo, T. Hasegawa, A. de Gouvea, N.V. Mokhov, S. Rescia, Andrés Castillo, F. Marinho, Mario Campanelli, Jürgen Pozimski, R. Raboanary, F. Sergiampietri, D. A. Sanders, John F. Beacom, Steven Gardiner, P. Madigan, R. Sulej, M. V. Diwan, D. J. Payne, L. Pickering, S. Manly, P. Hamilton, R. G. Van de Water, Chao Zhang, J. Wang, J. Hoff, Burak Bilki, Rex Tayloe, M. A. Uchida, A. Stuart, O. Dvornikov, P. De Lurgio, C. A. Ternes, J. A. Nowak, R. Bajou, P. Schlabach, E. Seltskaya, C. Lastoria, D. Naples, Kazuhiro Terao, A. Paudel, E. T. Worcester, C. Gotti, Michael Mulhearn, S. B. Boyd, T. Hill, D. Douglas, Daniel Gastler, G. A. Valdiviesso, S. Emery, M. C. Goodman, D. C. Christian, M. Newcomer, H. W. Sobel, N. Poonthottathil, Mingshui Chen, J. Urheim, B. Viren, D. Montanari, Giorgio Riccobene, I. Rakhno, M. A. Ramirez Delgado, J. Mousseau, Ara Ioannisian, H. T. Rakotondramanana, L. Molina Bueno, A. Rappoldi, Matthaeus Leitner, K. Fahey, S. J. Brice, M. E. Convery, Nicolas Lurkin, Bindu A. Bambah, S. Ravat, W. Mu, M. A. Arroyave, A. A. Machado, R. Petti, Rukmani Mohanta, Andrew Norman, V. N. Solovov, X. Pons, J. Marteau, Irakli Lomidze, Zviad Tsamalaidze, H. da Motta, M. Mellinato, M. Karolak, D. Autiero, Poonam Mehta, G. Karagiorgi, Sudarshan Paramesvaran, S. Davini, R. L. Talaga, V. Paolone, V. Pec, J. Pillow, S. Vergani, Simon Lin, K. Wood, Jaroslaw Pasternak, G. C. Blazey, Katsuya Yonehara, T. E. Coan, B. Radics, W. Gu, A. M. Teklu, E. Blucher, S. Childress, S. Matsuno, Christian Farnese, Akitaka Ariga, Marvin L Marshak, A. Chiriacescu, F. Terranova, E. Raguzin, L. C. J. Rice, L. Domine, M. Pozzato, T. Miao, L. Da Silva Peres, D. Mladenov, T. Durkin, H. Y. Wei, L. Escudero Sanchez, T. Usher, A. Rafique, A. Verdugo, B. Stillwell, A. Lambert, K. Negishi, A. Falcone, A. Holin, J. L. Bazo Alba, J. Rout, E. D. Zimmerman, M. A. Leigui de Oliveira, A. Olivier, J. Nesbit, Aldo Penzo, Kate Scholberg, Giovanni Bellettini, S. Kasai, O. Gogota, B. Ramson, P. de Jong, R. Zaki, A. Tonazzo, H. Schellman, E. Kemp, T. Rehak, I. De Bonis, Pedro A. N. Machado, B. T. Fleming, M. P. Andrews, M. Bishai, T. Alion, N. Martinez, L. Greenler, Deywis Moreno, T. Loew, H. Berns, P. Ding, M. J. Dolinski, R. J. Nichol, B. Guo, Frank Filthaut, Stefan Antusch, Nikolaos Charitonidis, Patrick Green, R. Howell, Z. Parsa, M. Sorel, J. C. Freeman, J. A. Musser, D. Gratieri, J. Reichenbacher, S. Ventura, Kaushik De, M. J. Rodriguez Alonso, Patrick Dunne, A. Scaramelli, M. Tenti, J. R. T. de Mello Neto, Raj Gandhi, Riccardo Papaleo, M. C. Sanchez, V. Zutshi, Sandeep Miryala, Enrique Calvo, N. Tsverava, V. Radeka, C. Touramanis, J. M. Paley, Antonio Ereditato, J. S. Díaz, Marco Pallavicini, D. MacFarland, G. Savage, J. Soto-Oton, P. Fernandez Menendez, J. Han, C. Y. Chi, M. Groh, N. Yershov, M. Chalifour, E. Hazen, M. A. Acero, C. Mossey, L. 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E., Lang, K., Langford, T., Lasorak, P., Last, D., Lastoria, C., Laundrie, A., Lawrence, A., Lazanu, I., Lazur, R., Le, T., Learned, J., Lebrun, P., Miotto, G. L., Lehnert, R., De Oliveira, M. A. L., Leitner, M., Leyton, M., Li, L., Li, S., Li, S. W., Li, T., Li, Y., Liao, H., Lin, C. S., Lin, S., Lister, A., Littlejohn, B. R., Liu, J., Liu, T., Lockwitz, S., Loew, T., Lokajicek, M., Lomidze, I., Long, K., Loo, K., Lorca, D., Lord, T., Losecco, J. M., Louis, W. C., Luk, K. B., Luo, X., Lurkin, N., Lux, T., Luzio, V. P., Macfarland, D., Machado, A. A., Machado, P., Macias, C. T., Macier, J. R., Maddalena, A., Madigan, P., Magill, S., Mahn, K., Maio, A., Maloney, J. A., Mandrioli, G., Maneira, J., Manenti, L., Manly, S., Mann, A., Manolopoulos, K., Plata, M. M., Marchionni, A., Marciano, W., Marfatia, D., Mariani, C., Maricic, J., Marinho, F., Marino, A. D., Marshak, M., Marshall, C., Marshall, J., Marteau, J., Martin-Albo, J., Martinez, N., Martinez Caicedo, D. A., Martynenko, S., Mason, K., Mastbaum, A., Masud, M., Matsuno, S., Matthews, J., Mauger, C., Mauri, N., Mavrokoridis, K., Mazza, R., Mazzacane, A., Mazzucato, E., Mccluskey, E., Mcconkey, N., Mcfarland, K. S., Mcgrew, C., Mcnab, A., Mefodiev, A., Mehta, P., Melas, P., Mellinato, M., Mena, O., Menary, S., Mendez, H., Menegolli, A., Meng, G., Messier, M. D., Metcalf, W., Mewes, M., Meyer, H., Miao, T., Michna, G., Miedema, T., Migenda, J., Milincic, R., Miller, W., Mills, J., Milne, C., Mineev, O., Miranda, O. G., Miryala, S., Mishra, C. S., Mishra, S. R., Mislivec, A., Mladenov, D., Mocioiu, I., Moffat, K., Moggi, N., Mohanta, R., Mohayai, T. A., Mokhov, N., Molina, J., Bueno, L. M., Montanari, A., Montanari, C., Montanari, D., Zetina, L. M. M., Moon, J., Mooney, M., Moor, A., Moreno, D., Morgan, B., Morris, C., Mossey, C., Motuk, E., Moura, C. A., Mousseau, J., Mu, W., Mualem, L., Mueller, J., Muether, M., Mufson, S., Muheim, F., Muir, A., Mulhearn, M., Muramatsu, H., Murphy, S., Musser, J., Nachtman, J., Nagu, S., Nalbandyan, M., Nandakumar, R., Naples, D., Narita, S., Navas-Nicolas, D., Nayak, N., Nebot-Guinot, M., Necib, L., Negishi, K., Nelson, J. K., Nesbit, J., Nessi, M., Newbold, D., Newcomer, M., Newhart, D., Nichol, R., Niner, E., Nishimura, K., Norman, A., Norrick, A., Northrop, R., Novella, P., Nowak, J. A., Oberling, M., Campo, A. O. D., Olivier, A., Onel, Y., Onishchuk, Y., Ott, J., Pagani, L., Pakvasa, S., Palamara, O., Palestini, S., Paley, J. M., Pallavicini, M., Palomares, C., Pantic, E., Paolone, V., Papadimitriou, V., Papaleo, R., Papanestis, A., Paramesvaran, S., Parke, S., Parsa, Z., Parvu, M., Pascoli, S., Pasqualini, L., Pasternak, J., Pater, J., Patrick, C., Patrizii, L., Patterson, R. B., Patton, S. J., Patzak, T., Paudel, A., Paulos, B., Paulucci, L., Pavlovic, Z., Pawloski, G., Payne, D., Pec, V., Peeters, S. J. M., Penichot, Y., Pennacchio, E., Penzo, A., Peres, O. L. G., Perry, J., Pershey, D., Pessina, G., Petrillo, G., Petta, C., Petti, R., Piastra, F., Pickering, L., Pietropaolo, F., Pillow, J., Pinzino, J., Plunkett, R., Poling, R., Pons, X., Poonthottathil, N., Pordes, S., Potekhin, M., Potenza, R., Potukuchi, B. V. K. S., Pozimski, J., Pozzato, M., Prakash, S., Prakash, T., Prince, S., Prior, G., Pugnere, D., Qi, K., Qian, X., Raaf, J. L., Raboanary, R., Radeka, V., Rademacker, J., Radics, B., Rafique, A., Raguzin, E., Rai, M., Rajaoalisoa, M., Rakhno, I., Rakotondramanana, H. T., Rakotondravohitra, L., Ramachers, Y. A., Rameika, R., Delgado, M. A. R., Ramson, B., Rappoldi, A., Raselli, G., Ratoff, P., Ravat, S., Razafinime, H., Real, J. S., Rebel, B., Redondo, D., Reggiani-Guzzo, M., Rehak, T., Reichenbacher, J., Reitzner, S. D., Renshaw, A., Rescia, S., Resnati, F., Reynolds, A., Riccobene, G., Rice, L. C. J., Rielage, K., Rigamonti, A., Rigaut, Y., Rivera, D., Rochester, L., Roda, M., Rodrigues, P., Alonso, M. J. R., Rondon, J. R., Roeth, A. J., Rogers, H., Rosauro-Alcaraz, S., Rosenthal, M., Rossella, M., Rout, J., Roy, S., Rubbia, A., Rubbia, C., Russell, B., Russell, J., Ruterbories, D., Saakyan, R., Sacerdoti, S., Safford, T., Sahu, N., Sala, P., Salukvadze, G., Samios, N., Sanchez, M. C., Sanders, D. A., Sankey, D., Santana, S., Santos-Maldonado, M., Saoulidou, N., Sapienza, P., Sarasty, C., Sarcevic, I., Savage, G., Savinov, V., Scaramelli, A., Scarff, A., Scarpelli, A., Schellman, H., Schlabach, P., Schmitz, D., Scholberg, K., Schukraft, A., Segreto, E., Seltskaya, E., Sensenig, J., Seong, I., Sergi, A., Sergiampietri, F., Sgalaberna, D., Shaevitz, M. H., Shafaq, S., Shamma, M., Sharma, H. 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A., Terranova, F., Testera, G., Thea, A., Thompson, J. L., Thorn, C., Timm, S. C., Tonazzo, A., Torti, M., Tortola, M., Tortorici, F., Totani, D., Toups, M., Touramanis, C., Trevor, J., Trzaska, W. H., Tsai, Y. T., Tsamalaidze, Z., Tsang, K. V., Tsverava, N., Tufanli, S., Tull, C., Tyley, E., Tzanov, M., Uchida, M. A., Urheim, J., Usher, T., Vagins, M. R., Vahle, P., Valdiviesso, G. A., Valencia, E., Vallari, Z., Valle, J. W. F., Vallecorsa, S., Berg, R. V., De Water, R. G. V., Forero, D. V., Varanini, F., Vargas, D., Varner, G., Vasel, J., Vasseur, G., Vaziri, K., Ventura, S., Verdugo, A., Vergani, S., Vermeulen, M. A., Verzocchi, M., De Souza, H. V., Vignoli, C., Vilela, C., Viren, B., Vrba, T., Wachala, T., Waldron, A. V., Wallbank, M., Wang, H., Wang, J., Wang, Y., Warburton, K., Warner, D., Wascko, M., Waters, D., Watson, A., Weatherly, P., Weber, A., Weber, M., Wei, H., Weinstein, A., Wenman, D., Wetstein, M., While, M. R., White, A., Whitehead, L. 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D., Zito, M., Zucchelli, S., Zuklin, J., Zutshi, V., Zwaska, R., Institut de Physique des 2 Infinis de Lyon (IP2I Lyon), Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Claude Bernard Lyon 1 (UCBL), Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS), AstroParticule et Cosmologie (APC (UMR_7164)), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Centre National de la Recherche Scientifique (CNRS)-Université de Paris (UP), Institut de Recherches sur les lois Fondamentales de l'Univers (IRFU), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay, Laboratoire de l'Accélérateur Linéaire (LAL), Centre National de la Recherche Scientifique (CNRS)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Sud - Paris 11 (UP11), Laboratoire d'Annecy de Physique des Particules (LAPP), Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS), Laboratoire de Physique Subatomique et de Cosmologie (LPSC), Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP ), Université Grenoble Alpes (UGA), DUNE, Abi, B, Abud, A, Acciarri, R, Acero, M, Adamov, G, Adamowski, M, Adams, D, Adrien, P, Adinolfi, M, Ahmad, Z, Ahmed, J, Alion, T, Monsalve, S, Alt, C, Anderson, J, Andreopoulos, C, Andrews, M, Andrianala, F, Andringa, S, Ankowski, A, Antonova, M, 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Almeida, R, Debbins, P, Bonis, I, Decowski, M, De Gouv a, A, Holanda, P, Astiz, I, Deisting, A, Jong, P, Delbart, A, Delepine, D, Delgado, M, Dell'Acqua, A, Lurgio, P, Neto, J, Demuth, D, Dennis, S, Densham, C, Deptuch, G, Roeck, A, Romeri, V, Vries, J, Dharmapalan, R, Dias, M, Diaz, F, Diaz, J, Domizio, S, Giulio, L, Ding, P, Noto, L, Distefano, C, Diurba, R, Diwan, M, Djurcic, Z, Dokania, N, Dolinski, M, Domine, L, Douglas, D, Drielsma, F, Duchesneau, D, Duffy, K, Dunne, P, Durkin, T, Duyang, H, Dvornikov, O, Dwyer, D, Dyshkant, A, Eads, M, Edmunds, D, Eisch, J, Emery, S, Ereditato, A, Escobar, C, Sanchez, L, Evans, J, Ewart, E, Ezeribe, A, Fabre, C, Fahey, K, Falcone, A, Farnese, C, Farzan, Y, Felix, J, Fernandez-Martinez, E, Menendez, P, Ferraro, F, Fields, L, Filkins, A, Filthaut, F, Fitzpatrick, R, Flanagan, W, Fleming, B, Flight, R, Fowler, J, Fox, W, Franc, J, Francis, K, Franco, D, Freeman, J, Freestone, J, Fried, J, Friedland, A, Fuess, S, Furic, I, Furmanski, A, Gago, A, Gallagher, H, Gallego-Ros, A, Gallice, N, Galymov, V, Gamberini, E, Gamble, T, Gandhi, R, Gandrajula, R, Gao, S, Garcia-Gamez, D, Garcia-Peris, M, Gardiner, S, Gastler, D, Ge, G, Gelli, B, Gendotti, A, Gent, S, Ghorbani-Moghaddam, Z, Gibin, D, Gil-Botella, I, Girerd, C, Giri, A, Gnani, D, Gogota, O, Gold, M, Gollapinni, S, Gollwitzer, K, Gomes, R, Bermeo, L, Fajardo, L, Gonnella, F, Gonzalez-Cuevas, J, Goodman, M, Goodwin, O, Goswami, S, Gotti, C, Goudzovski, E, Grace, C, Graham, M, Gramellini, E, Gran, R, Granados, E, Grant, A, Grant, C, Gratieri, D, Green, P, Green, S, Greenler, L, Greenwood, M, Greer, J, Griffith, W, Groh, M, Grudzinski, J, Grzelak, K, Gu, W, Guarino, V, Guenette, R, Guglielmi, A, Guo, B, Guthikonda, K, Gutierrez, R, Guzowski, P, Guzzo, M, Gwon, S, Haaf, K, Habig, A, Hackenburg, A, Hadavand, H, Haenni, R, Hahn, A, Haigh, J, Haiston, J, Hamernik, T, Hamilton, P, Han, J, Harder, K, Harris, D, Hartnell, J, Hasegawa, T, Hatcher, R, Hazen, E, Heavey, A, Heeger, K, Heise, J, Hennessy, K, Henry, S, Morquecho, M, Herner, K, Hertel, L, Hesam, A, Hewes, J, Higuera, A, Hill, T, Hillier, S, Himmel, A, Hoff, J, Hohl, C, Holin, A, Hoppe, E, Horton-Smith, G, Hostert, M, Hourlier, A, Howard, B, Howell, R, Hrivnak, J, Huang, J, Hugon, J, Iles, G, Ilic, N, Iliescu, A, Illingworth, R, Ioannisian, A, Itay, R, Izmaylov, A, James, E, Jargowsky, B, Jediny, F, Jes s-Valls, C, Ji, X, Jiang, L, Jimenez, S, Jipa, A, Joglekar, A, Johnson, C, Johnson, R, Jones, B, Jones, S, Jung, C, Junk, T, Jwa, Y, Kabirnezhad, M, Kaboth, A, Kadenko, I, Kamiya, F, Karagiorgi, G, Karcher, A, Karolak, M, Karyotakis, Y, Kasai, S, Kasetti, S, Kashur, L, Kazaryan, N, Kearns, E, Keener, P, Kelly, K, Kemp, E, Kendziora, C, Ketchum, W, Kettell, S, Khabibullin, M, Khotjantsev, A, Khvedelidze, A, Kim, D, King, B, Kirby, B, Kirby, M, Klein, J, Koehler, K, Koerner, L, Kohn, S, Koller, P, Kordosky, M, Kosc, T, Kose, U, Kostelecky, V, Kothekar, K, Krennrich, F, Kreslo, I, Kudenko, Y, Kudryavtsev, V, Kulagin, S, Kumar, J, Kumar, R, Kuruppu, C, Kus, V, Kutter, T, Lacarelle, B, Lambert, A, Lande, K, Lane, C, Lang, K, Langford, T, Lasorak, P, Last, D, Lastoria, C, Laundrie, A, Lawrence, A, Lazanu, I, Lazur, R, Le, T, Learned, J, Lebrun, P, Miotto, G, Lehnert, R, De Oliveira, M, Leitner, M, Leyton, M, Li, L, Li, S, Li, T, Li, Y, Liao, H, Lin, C, Lin, S, Lister, A, Littlejohn, B, Liu, J, Liu, T, Lockwitz, S, Loew, T, Lokajicek, M, Lomidze, I, Long, K, Loo, K, Lorca, D, Lord, T, Losecco, J, Louis, W, Luk, K, Luo, X, Lurkin, N, Lux, T, Luzio, V, Macfarland, D, Machado, A, Machado, P, Macias, C, Macier, J, Maddalena, A, Madigan, P, Magill, S, Mahn, K, Maio, A, Maloney, J, Mandrioli, G, Maneira, J, Manenti, L, Manly, S, Mann, A, Manolopoulos, K, Plata, M, Marchionni, A, Marciano, W, Marfatia, D, Mariani, C, Maricic, J, Marinho, F, Marino, A, Marshak, M, Marshall, C, Marshall, J, Marteau, J, Martin-Albo, J, Martinez, N, Martinez Caicedo, D, Martynenko, S, Mason, K, Mastbaum, A, Masud, M, Matsuno, S, Matthews, J, Mauger, C, Mauri, N, Mavrokoridis, K, Mazza, R, Mazzacane, A, Mazzucato, E, Mccluskey, E, Mcconkey, N, Mcfarland, K, Mcgrew, C, Mcnab, A, Mefodiev, A, Mehta, P, Melas, P, Mellinato, M, Mena, O, Menary, S, Mendez, H, Menegolli, A, Meng, G, Messier, M, Metcalf, W, Mewes, M, Meyer, H, Miao, T, Michna, G, Miedema, T, Migenda, J, Milincic, R, Miller, W, Mills, J, Milne, C, Mineev, O, Miranda, O, Miryala, S, Mishra, C, Mishra, S, Mislivec, A, Mladenov, D, Mocioiu, I, Moffat, K, Moggi, N, Mohanta, R, Mohayai, T, Mokhov, N, Molina, J, Bueno, L, Montanari, A, Montanari, C, Montanari, D, Zetina, L, Moon, J, Mooney, M, Moor, A, Moreno, D, Morgan, B, Morris, C, Mossey, C, Motuk, E, Moura, C, Mousseau, J, Mu, W, Mualem, L, Mueller, J, Muether, M, Mufson, S, Muheim, F, Muir, A, Mulhearn, M, Muramatsu, H, Murphy, S, Musser, J, Nachtman, J, Nagu, S, Nalbandyan, M, Nandakumar, R, Naples, D, Narita, S, Navas-Nicolas, D, Nayak, N, Nebot-Guinot, M, Necib, L, Negishi, K, Nelson, J, 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Qian, X, Raaf, J, Raboanary, R, Radeka, V, Rademacker, J, Radics, B, Rafique, A, Raguzin, E, Rai, M, Rajaoalisoa, M, Rakhno, I, Rakotondramanana, H, Rakotondravohitra, L, Ramachers, Y, Rameika, R, Ramson, B, Rappoldi, A, Raselli, G, Ratoff, P, Ravat, S, Razafinime, H, Real, J, Rebel, B, Redondo, D, Reggiani-Guzzo, M, Rehak, T, Reichenbacher, J, Reitzner, S, Renshaw, A, Rescia, S, Resnati, F, Reynolds, A, Riccobene, G, Rice, L, Rielage, K, Rigamonti, A, Rigaut, Y, Rivera, D, Rochester, L, Roda, M, Rodrigues, P, Alonso, M, Rondon, J, Roeth, A, Rogers, H, Rosauro-Alcaraz, S, Rosenthal, M, Rossella, M, Rout, J, Roy, S, Rubbia, A, Rubbia, C, Russell, B, Russell, J, Ruterbories, D, Saakyan, R, Sacerdoti, S, Safford, T, Sahu, N, Sala, P, Salukvadze, G, Samios, N, Sanchez, M, Sanders, D, Sankey, D, Santana, S, Santos-Maldonado, M, Saoulidou, N, Sapienza, P, Sarasty, C, Sarcevic, I, Savage, G, Savinov, V, Scaramelli, A, Scarff, A, Scarpelli, A, Schellman, H, Schlabach, P, Schmitz, D, Scholberg, 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Salinas C.J.S., Soldner-Rembold S., Solomey N., Solovov V., Sondheim W.E., Sorel M., Soto-Oton J., Sousa A., Soustruznik K., Spagliardi F., Spanu M., Spitz J., Spooner N.J.C., Spurgeon K., Staley R., Stancari M., Stanco L., Stefan D., Steiner H.M., Stewart J., Stillwell B., Stock J., Stocker F., Stokes T., Strait M., Strauss T., Striganov S., Stuart A., Sulej R., Summers D., Surdo A., Susic V., Suter L., Sutera C.M., Svoboda R., Szczerbinska B., Szelc A.M., Talaga R., Tanaka H.A., Oregui B.T., Tapper A., Tariq S., Tatar E., Tayloe R., Teklu A.M., Tenti M., Terao K., Ternes C.A., Terranova F., Testera G., Thea A., Thompson J.L., Thorn C., Timm S.C., Tonazzo A., Torti M., Tortola M., Tortorici F., Totani D., Toups M., Touramanis C., Trevor J., Trzaska W.H., Tsai Y.T., Tsamalaidze Z., Tsang K.V., Tsverava N., Tufanli S., Tull C., Tyley E., Tzanov M., Uchida M.A., Urheim J., Usher T., Vagins M.R., Vahle P., Valdiviesso G.A., Valencia E., Vallari Z., Valle J.W.F., Vallecorsa S., Berg R.V., De Water R.G.V., Forero D.V., Varanini F., Vargas D., Varner G., Vasel J., Vasseur G., Vaziri K., Ventura S., Verdugo A., Vergani S., Vermeulen M.A., Verzocchi M., De Souza H.V., Vignoli C., Vilela C., Viren B., Vrba T., Wachala T., Waldron A.V., Wallbank M., Wang H., Wang J., Wang Y., Warburton K., Warner D., Wascko M., Waters D., Watson A., Weatherly P., Weber A., Weber M., Wei H., Weinstein A., Wenman D., Wetstein M., While M.R., White A., Whitehead L.H., Whittington D., Wilking M.J., Wilkinson C., Williams Z., Wilson F., Wilson R.J., Wolcott J., Wongjirad T., Wood K., Wood L., Worcester E., Worcester M., Wret C., Wu W., Xiao Y., Yang G., Yang T., Yershov N., Yonehara K., Young T., Yu B., Yu H.W., Yu H.Z., Yu J., Yu Z.Y., Zaki R., Zalesak J., Zambelli L., Zamorano B., Zani A., Zazueta L., Zeller G.P., Zennamo J., Zeug K., Zhang C., Zhao M., Zhivun E., Zhu G., Zimmerman E.D., Zito M., Zucchelli S., Zuklin J., Zutshi V., Zwaska R., and Science and Technology Facilities Council (STFC)
Subjects: Technology, HIGH-ENERGY, Physics - Instrumentation and Detectors, Physics::Instrumentation and Detectors, far detector, beam transport, Noble liquid detectors (scintillation, ionization, double-phase), Cms Experıment, 01 natural sciences, 7. Clean energy, 09 Engineering, Particle identification, High Energy Physics - Experiment, 030218 nuclear medicine & medical imaging, High Energy Physics - Experiment (hep-ex), 0302 clinical medicine, Noble liquid detectors (scintillation, Detectors and Experimental Techniques, Instrumentation, Instruments & Instrumentation, physics.ins-det, time resolution, Mathematical Physics, Physics, 02 Physical Sciences, Time projection chamber, Large Hadron Collider, Detector, Instrumentation and Detectors (physics.ins-det), double-phase), Nuclear & Particles Physics, LIGHT, Neutrino, Particle Physics - Experiment, performance, Noble liquid detectors,(scintillation, ionization, double-phase), noise, CERN Lab, Large detector systems for particle and astroparticle physics, Noble liquid detectors (scintillation, ionization, double-phase), Time projection Chambers (TPC), 530 Physics, energy loss, Time projection chambers, FOS: Physical sciences, Particle detector, Nuclear physics, 03 medical and health sciences, neutrino: deep underground detector, 0103 physical sciences, ionization, Deep Underground Neutrino Experiment, High Energy Physics, [PHYS.PHYS.PHYS-INS-DET]Physics [physics]/Physics [physics]/Instrumentation and Detectors [physics.ins-det], signal processing, activity report, Science & Technology, 010308 nuclear & particles physics, hep-ex, Large detector systems for particle and astroparticle physics, Time projection Chambers (TPC), 530 Physik, sensitivity, calibration, time projection chamber: liquid argon, Experimental High Energy Physics, Large detector systems for particle and astroparticle physic, single-phase), High Energy Physics::Experiment, photon: detector, particle identification, charged particle: irradiation, Beam (structure)
Abstract: The ProtoDUNE-SP detector was constructed and operated on the CERN Neutrino Platform. We thank the CERN management for providing the infrastructure for this experiment and gratefully acknowledge the support of the CERN EP, BE, TE, EN, IT and IPT Departments for NP04/ProtoDUNE-SP. This documentwas prepared by theDUNEcollaboration using the resources of the Fermi National Accelerator Laboratory (Fermilab), a U.S. Department of Energy, Office of Science, HEP User Facility. Fermilab is managed by Fermi Research Alliance, LLC (FRA), acting under Contract No. DE-AC02-07CH11359. This work was supported by CNPq, FAPERJ, FAPEG and FAPESP, Brazil; CFI, IPP and NSERC, Canada; CERN; MSMT, Czech Republic; ERDF, H2020-EU and MSCA, European Union; CNRS/IN2P3 and CEA, France; INFN, Italy; FCT, Portugal; NRF, South Korea; CAM, Fundacion "La Caixa" and MICINN, Spain; SERI and SNSF, Switzerland; TUBITAK, Turkey; The Royal Society and UKRI/STFC, United Kingdom; DOE and NSF, United States of America. This research used resources of the National Energy Research Scientific Computing Center (NERSC), a U.S. Department of Energy Office of Science User Facility operated under Contract No. DE-AC02-05CH11231., The ProtoDUNE-SP detector is a single-phase liquid argon time projection chamber with an active volume of 7.2× 6.1× 7.0 m3. It is installed at the CERN Neutrino Platform in a specially-constructed beam that delivers charged pions, kaons, protons, muons and electrons with momenta in the range 0.3 GeV/c to 7 GeV/c. Beam line instrumentation provides accurate momentum measurements and particle identification. The ProtoDUNE-SP detector is a prototype for the first far detector module of the Deep Underground Neutrino Experiment, and it incorporates full-size components as designed for that module. This paper describes the beam line, the time projection chamber, the photon detectors, the cosmic-ray tagger, the signal processing and particle reconstruction. It presents the first results on ProtoDUNE-SP's performance, including noise and gain measurements, dE/dx calibration for muons, protons, pions and electrons, drift electron lifetime measurements, and photon detector noise, signal sensitivity and time resolution measurements. The measured values meet or exceed the specifications for the DUNE far detector, in several cases by large margins. ProtoDUNE-SP's successful operation starting in 2018 and its production of large samples of high-quality data demonstrate the effectiveness of the single-phase far detector design., National Council for Scientific and Technological Development (CNPq), Carlos Chagas Filho Foundation for Research Support of the State of Rio de Janeiro (FAPERJ), FAPEG, Brazil, Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP), Canada Foundation for Innovation, Natural Sciences and Engineering Research Council of Canada (NSERC), Ministry of Education, Youth & Sports - Czech Republic Czech Republic Government, European Union (EU), H2020-EU, French Atomic Energy Commission, Istituto Nazionale di Fisica Nucleare (INFN), NRF, South Korea, La Caixa Foundation, Spanish Government, Swiss National Science Foundation (SNSF), Turkiye Bilimsel ve Teknolojik Arastirma Kurumu (TUBITAK), Royal Society of London, United States Department of Energy (DOE), National Science Foundation (NSF) DE-AC02-05CH11231, IPP, Canada, CERN, MSCA, Centre National de la Recherche Scientifique (CNRS), Portuguese Foundation for Science and Technology, CAM, Spain, SERI, Switzerland, UKRI/STFC, United Kingdom, DE-AC02-07CH11359
Published: 2020

34. Heme Doming in Ferric Cytochrome c: Femtosecond X-ray Absorption and X-ray Emission Studies

Author: Camila Bacellar, Christopher Arrell, Katharina Kubicek, Oliviero Cannelli, Angel Rodriguez-Fernandez, Wojciech Gawelda, Philip J. M. Johnson, Georgios Pamfilidis, Giulia F. Mancini, Claudio Cirelli, Dmitry Khakhulin, Jakub Szlachetko, Gregor Knopp, Christopher J. Milne, Dominik Kinschel, Christian Bressler, Jérémy R. Rouxel, Majed Chergui, Frederico A. Lima, Mykola Biednov, Samuel Menzi, and Rebecca A. Ingle
Subjects: Quantitative Biology::Biomolecules, X-ray absorption spectroscopy, Materials science, Spin states, biology, Astrophysics::High Energy Astrophysical Phenomena, Cytochrome c, Photochemistry, Physics::Geophysics, Condensed Matter::Materials Science, chemistry.chemical_compound, chemistry, Condensed Matter::Superconductivity, Femtosecond, biology.protein, medicine, Ferric, Absorption (chemistry), Spectroscopy, Heme, medicine.drug
Abstract: The photoinduced dynamics of ferric Cytochrome c was investigated by ultrafast non-resonant X-ray emission (XES) and X-Ray Absorption (XAS) spectroscopies, and a cascade through high spin states accompanied by heme doming are observed for the first time.
Published: 2020

35. Taking a snapshot of the triplet excited state of an OLED organometallic luminophore using X-rays

Author: Matteo Levantino, Andrea Cannizzo, R. Bohinc, Michela Gazzetto, Daniel James, Jakub Szlachetko, Camila Bacellar, Alexander A. Guda, Sergey Yu. Ketkov, Kristoffer Haldrup, Martin Beck, Mathias Sander, Marian Olaru, Georgios Pamfilidis, Jens Beckmann, Claudio Cirelli, Victoria Kabanova, Elena Rychagova, Nicolo Azzaroli, Victor V. Shapovalov, Samuel Menzi, Joanna Czapla-Masztafiak, Andrei A. Tereshchenko, Giulia F. Mancini, Aldo Mozzanica, Christopher J. Milne, Wojciech M. Kwiatek, Grigory Smolentsev, Matthias Vogt, Gregor Knopp, and Dardan Gashi
Subjects: basis-sets, absorption spectroscopy, Materials science, electronic-structure, Photochemistry, 530 Physics, Science, activated delayed fluorescence, General Physics and Astronomy, 02 engineering and technology, 010402 general chemistry, 01 natural sciences, Article, General Biochemistry, Genetics and Molecular Biology, law.invention, chemistry.chemical_compound, law, 540 Chemistry, OLED, lcsh:Science, Structural rigidity, Multidisciplinary, Scattering, light-emitting-diodes, solvation dynamics, Excited states, transition, General Chemistry, 021001 nanoscience & nanotechnology, Laser, 620 Engineering, Fluorescence, emission spectroscopy, 0104 chemical sciences, chemistry, Chemical physics, Excited state, Luminophore, systems, lcsh:Q, 0210 nano-technology, Excitation, metal-complexes
Abstract: OLED technology beyond small or expensive devices requires light-emitters, luminophores, based on earth-abundant elements. Understanding and experimental verification of charge transfer in luminophores are needed for this development. An organometallic multicore Cu complex comprising Cu–C and Cu–P bonds represents an underexplored type of luminophore. To investigate the charge transfer and structural rearrangements in this material, we apply complementary pump-probe X-ray techniques: absorption, emission, and scattering including pump-probe measurements at the X-ray free-electron laser SwissFEL. We find that the excitation leads to charge movement from C- and P- coordinated Cu sites and from the phosphorus atoms to phenyl rings; the Cu core slightly rearranges with 0.05 Å increase of the shortest Cu–Cu distance. The use of a Cu cluster bonded to the ligands through C and P atoms is an efficient way to keep structural rigidity of luminophores. Obtained data can be used to verify computational methods for the development of luminophores., Nature Communications, 11 (1), ISSN:2041-1723
Published: 2020
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36. Long-baseline neutrino oscillation physics potential of the DUNE experiment: DUNE Collaboration

Author: M. Spanu, Xiaolu Ji, A. M. Szelc, Gareth J. Barker, C. Cattadori, J. Fried, J. Fowler, S. J. M. Peeters, S. Alonso Monsalve, G. Ge, Alexander Tapper, Thomas Strauss, B. Bhuyan, D. Vanegas Forero, A. L. Renshaw, A. P. Furmanski, P.T. Smith, D. Newhart, E. Raguzin, A. J. Roeth, R. Acciarri, Karol Lang, V. Savinov, P. Melas, A. Heavey, Grzegorz Deptuch, Kevin J. Kelly, D. Sgalaberna, R. LaZur, E. Pennacchio, F. W. Sippach, Kristian Harder, M. A. Uchida, J. Hewes, Sandro Palestini, K. Spurgeon, Sandip Pakvasa, F. Stocker, H. W. Sobel, A. Gallego-Ros, N. Buchanan, C. Grant, T. Li, T. Gamble, J. J. Grudzinski, N. Mauri, L. Molina Bueno, Jeremy Wolcott, Andrea Zani, M. J. Wilking, A. Olivares Del Campo, Joshua R. Klein, A. Hourlier, Jonas Rademacker, G. P. Zeller, A. Lawrence, D. Brailsford, M. Chalifour, I. Gil-Botella, R. Flight, H. Vieira de Souza, D. Redondo, S. R. Mishra, Paola Sala, Joshua Barrow, John Marshall, K. Francis, S. Ravat, W. Mu, D. Marfatia, Vasundhara Singh, Ranjan Dharmapalan, S. Striganov, Laura Paulucci, Mario Campanelli, D. Cherdack, M. A. Ramirez Delgado, S. J. Brice, Nicolas Lurkin, Wayne A. Barkhouse, A. Filkins, D. Autiero, Poonam Mehta, Dave Sankey, J. Asaadi, E. Valencia, E. James, N.V. Mokhov, A. Booth, E. Hazen, Armin Karcher, D. Smargianaki, S. Menary, P. C. de Holanda, J. Hugon, C. Brizzolari, M. Kirby, E. Kearns, A. C. Ezeribe, T. Lord, L. Zazueta, Daijin Kim, G.D. Barr, Junwei Huang, V. De Romeri, F. Piastra, C. Girerd, Christopher L. Marshall, A. Bitadze, Yichen Li, Alexander Deisting, H. Carranza, Milos Lokajicek, Roberto Gutiérrez, J. Pinzino, Janice L. Thompson, F. Kamiya, M. Wetstein, A. Cervera Villanueva, Robert Svoboda, L. C. J. Rice, L. Pasqualini, L. Di Giulio, J. Martin-Albo, H. Muramatsu, Z. Pavlovic, A. Falcone, R. Gran, A. A. Machado, R. Petti, M. Roda, Jianbei Liu, C. Vignoli, B. Rebel, Joleen Pater, David H. Adams, D. Caratelli, S. Martynenko, Ph. Lebrun, R. Staley, J. L. Bazo Alba, F. Marinho, L. Bellantoni, R. Cross, S. Jones, E. Bechetoille, Gustaaf Brooijmans, K. Moffat, Chao Zhang, M. Parvu, James A. Anderson, A. M. Gago, R. Diurba, G. Christodoulou, K. Nishimura, S. Calvez, Bo Yu, G. Karagiorgi, A. V. Waldron, Filippo Resnati, M. A. Hernandez Morquecho, A. Borkum, N. McConkey, J. Wang, Dario Gnani, F. F. Wilson, Nektarios Benekos, Renato Potenza, M. Toups, Haleh Khani Hadavand, Jaroslaw Pasternak, K. Kothekar, W. Flanagan, V. Papadimitriou, Y. Cui, P. A. Rodrigues, C. McGrew, M. P. Decowski, V. Galymov, E. Chardonnet, A. Hackenburg, D. Caiulo, T. Loew, P. Ding, B. V. K. S. Potukuchi, I. L. De Icaza Astiz, M. M. Khabibullin, D. Wenman, S. C. Timm, R. Sharma, Sergey A. Kulagin, A. Bashyal, A. Mislivec, B. Stillwell, A. Lambert, C. J. Solano Salinas, William J. Marciano, R. Saakyan, J. D. Eisch, D. Totani, Sandhya Choubey, J. Spitz, E. McCluskey, K. Zeug, Burak Bilki, L. Cremonesi, B. Tapia Oregui, N. Nayak, A. Holin, Olga Mena, C. Hohl, W. Gu, G. Zhu, Beatriz B. Siffert, J. Franc, B. R. Littlejohn, B. Morgan, T. Patzak, L. Patrizii, A. Weinstein, Katsuya Yonehara, R. Haenni, T. E. Coan, G. Mandrioli, M. T. Graham, A. Mefodiev, G.L. Raselli, A. de Gouvea, Alastair Grant, Giovanni Bellettini, A. Sitraka, L. Bagby, J. M. LoSecco, Stephen P. Gent, G. S. Davies, B. Radics, I. De Bonis, A. Marchionni, A. Mann, S. Balasubramanian, C. Andreopoulos, K. Mason, S. Kasai, O. V. Mineev, A. F. Moor, S. Centro, S. Henry, M. Bishai, H. Berns, A. Scarpelli, A. K. Giri, A. C. Kaboth, F. Terranova, J. Chaves, G. Sirri, T. Vrba, F. Bento Neves, M. Potekhin, D. Duchesneau, A. M. Teklu, L. Fields, E. Blucher, S. Childress, Andrew Smith, M. Manrique Plata, Andrew White, V. Susic, S. Berkman, L. Di Noto, T. Miao, Randall P. Johnson, N. Kazaryan, Kendall Mahn, Jorge Molina, C. Cuesta, Kenneth Long, S. D. Reitzner, E. Motuk, Evgueni Goudzovski, D. J. Summers, E. Gamberini, B. J. P. Jones, C. Vilela, J. S. Díaz, P. Novella, Andrew Brandt, D. M. DeMuth, B. Carlus, D. Boyden, G. Petrillo, André Rubbia, C. Barnes, A. S. Hesam, G. Yang, Patrick Dunne, W. Metcalf, I. Kreslo, Aldo Penzo, C. Castromonte, W. E. Sondheim, S. Rosauro-Alcaraz, Paolo Calafiura, Q. David, L. Da Silva Peres, H. Mendez, T. Wongjirad, F. Pietropaolo, Sofia Vallecorsa, K. E. Duffy, Nikolina Ilic, J. R. Macier, A. Chatterjee, S. Kohn, M. Torti, M. Tortola, O. G. Miranda, C. Patrick, José W. F. Valle, A. Delbart, N. J. C. Spooner, Paul Keener, C. E. Tull, Leigh H. Whitehead, T. Hasegawa, Ihn Sik Seong, K. Grzelak, A. Gendotti, S. H. Kettell, A. Himmel, M. Rajaoalisoa, P. Bour, A. Verdugo, H. S. Chen, C. M. Sutera, Y.-J. Jwa, Kam-Biu Luk, M. C. Sanchez, K. Qi, E. Segreto, Xin Qian, T. A. Mohayai, E. Pantic, O.V. Dvornikov, Z. Ahmad, F. Drielsma, B. Jargowsky, L. V. Gomez Bermeo, S. Tufanli, S. Rescia, L. Mualem, E. Smith, B. Szczerbinska, K. Mavrokoridis, J. Sinclair, James Stewart, Karol Hennessy, S. Söldner-Rembold, A. N. Khotjantsev, Andrés Castillo, C. Wret, F. Andrianala, F. Tortorici, V. A. Kudryavtsev, M. Bongrand, E. Niner, B. Zamorano, Warner A. Miller, J. I. Crespo-Anadón, N. Tsverava, F. Muheim, Ralf Lehnert, J. A. B. Coelho, L. W. Koerner, L. Montaño Zetina, W. Ketchum, D. A. Sanders, John F. Beacom, Robert Wilson, M. J. Dolinski, K. Soustruznik, A. Higuera, F. Ferraro, C. S. Lin, F. Sergiampietri, Wladyslaw Henryk Trzaska, Cari L. Johnson, Rex Tayloe, A. Lister, J. Freestone, D. Rivera, T. Wachala, Yu. Kudenko, A. Christensen, T. A. Bolton, D. Gratieri, P. Cotte, Diana Navas-Nicolas, G. C. Blazey, S. Bordoni, James Mueller, S. Jiménez, R. Zwaska, W. Fox, J. R. T. de Mello Neto, Barry King, Alexandru Jipa, Yi Chen, C. J. Densham, D. W. Schmitz, N. Moggi, B. Russell, M. Vagins, E. Zhivun, S. Li, Marco Verzocchi, Steven Gardiner, P. Madigan, J. Greer, Y. T. Tsai, L. Camilleri, J.V. Dawson, E. Kemp, Olga Beltramello, Silvia Pascoli, J. T. Haigh, S. P. Kasetti, S. Nagu, J. A. Maloney, F. Barao, S. Santana, R. Mazza, D. Douglas, Keith Rielage, Raj Gandhi, C. Mariani, R. J. Nichol, J. Zuklin, Marzio Nessi, Carlos Escobar, D. Lorca, Claire Shepherd-Themistocleous, Z. Vallari, J. Stock, T. Durkin, H. Y. Wei, Y. Penichot, K. Herner, J. Sensenig, L. Escudero Sanchez, M. Zito, J. Vasel, Daniel Gastler, J. Marteau, Irakli Lomidze, C. Wilkinson, M. Greenwood, Christopher J. Milne, N. Dokania, P. N. Ratoff, T. Kutter, M. Sorel, M. Masud, Giuseppe Benedetto Cerati, J. C. Freeman, Kaushik De, R. Guenette, J. A. Gonzalez-Cuevas, L. S. Gomez Fajardo, S. Pordes, P. Weatherly, T. Miedema, James John Brooke, M. Wallbank, S. J. Patton, B. Gelli, E. Church, A. Aranda-Fernandez, M. J. Rodriguez Alonso, M. A. Acero, Hem Raj Sharma, I. Rakhno, M. Rai, Juraj Bracinik, Zviad Tsamalaidze, H. da Motta, N. Bostan, David Delepine, M. Soderberg, Marco Pallavicini, S. Magill, Gregory J. Michna, Rukmani Mohanta, Konstantinos Manolopoulos, H. A. Tanaka, L. O. Arnold, G. S. Varner, A. C. Weber, E. Brianne, C. Mossey, H. Y. Liao, M. Betancourt, C. Montanari, E. Conley, R. K. Plunkett, B. Howard, S. Fuess, L. Corwin, E. Cristaldo, J. Rout, B. Viren, B. Kirby, A. Bross, J. Barranco Monarca, D. Warner, C. E. Thorn, Sukalyan Chattopadhyay, R. A. Gomes, E. Gramellini, Gabriella Carini, M. Dabrowski, Hui Wang, J. Mousseau, S. L. Mufson, P. Debbins, H. Razafinime, Alessandro Montanari, Dave M Newbold, C. K. Jung, Andrew Norman, F. Krennrich, C. Mauger, J. Yu, D. Gibin, John Evans, Laura Dominé, J. J. Russell, W. C. Louis, G. Savage, Carl Grace, M. Muether, P. de Jong, L. Wood, A. Joglekar, S. Roy, D. Shooltz, Francesco Gonnella, M. Stancari, F. Cavanna, Marc Weber, B. T. Fleming, A. Scarff, D. Mladenov, S. Di Domizio, G. Meng, Matthaeus Leitner, K. Fahey, V. Bellini, A. Rafique, C. Alt, B. Abi, W. C. Griffith, H. R. Gallagher, R. Northrop, A. Mastbaum, K. S. McFarland, C. T. Macias, Alessandro Thea, A. Muir, Jordan Ott, A. Surdo, Piera Sapienza, M. Shamma, V. N. Solovov, N. P. Samios, X. Pons, Niki Saoulidou, R. Poling, J. G. Learned, J. Urheim, K. Koehler, David Cussans, Bindu A. Bambah, Y. Bezawada, V. P. Luzio, N. Gallice, R. Van Berg, Wei Wu, B. Paulos, J. Soto-Oton, M. Oberling, Gregory Iles, Paolo Carniti, A. Friedland, A. Papanestis, A. Aurisano, A. Norrick, F. Bay, H.E. Rogers, Andrea Dell'Acqua, Yu. Onishchuk, T. Yang, K. M. Heeger, D. Montanari, Giorgio Riccobene, J. Hartnell, D. A. Harris, C. Distefano, Ornella Palamara, Sudarshan Paramesvaran, Ionel Lazanu, Pedro A. N. Machado, M. R. While, T. Alion, E. Mazzucato, V. Basque, A. Rappoldi, H. S. Budd, T. Hamernik, Srubabati Goswami, Z. Williams, H. Duyang, N. Simos, H. Meyer, Chia-Chan Chang, M. Nebot-Guinot, J. Bian, Yasaman Farzan, A. Schukraft, A. Sousa, Z. Ghorbani-Moghaddam, G. Pessina, J. Berger, Robert Shrock, J. G. Boissevain, J. Smolik, R. Illingworth, S. Davini, R. L. Talaga, S. Dennis, J. Zennamo, V. Paolone, V. Pec, E. Ewart, T. Kosc, Thorsten Lux, G. Testera, Alessandro Menegolli, A. De Roeck, M. Calin, J. Pillow, S. 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Vahle, G. A. Horton-Smith, Y. Rigaut, A. McNab, J. Ahmed, Narendra Sahu, A. G. Cocco, C. Morris, G. Vasseur, C. Petta, I. K. Furic, John Matthews, S. Murphy, M. D. Messier, A. Mazzacane, S. Gao, M. Bhattacharjee, D. Pugnere, F. Bonini, C. A. Moura, Amelia Maio, C. Backhouse, A. D. Marino, M. Worcester, S. Gwon, M. O. Wascko, C. Sarasty, Stephen J. Parke, J. Perry, Stephen Hillier, M. Biassoni, D. Pershey, P. De Lurgio, E. T. Worcester, O. Goodwin, Jitendra Kumar, Mingshui Chen, K. K. Guthikonda, J. L. Raaf, J. Singh, M. A. Arroyave, M. Karolak, Alan Watson, J. Mills, Irina Mocioiu, C. N. Booth, L. Zambelli, S. B. Boyd, A. M. Iliescu, Alex Reynolds, K. Biery, Yanchu Wang, Deywis Moreno, V. Aushev, J. Zalesak, L. Simard, Mafalda Dias, I. Kadenko, D. Waters, S. Prakash, D. Ruterbories, Antonino Sergi, L. Pagani, J. Rodriguez Rondon, R. Nandakumar, Alec Habig, A. Guglielmi, D. Franco, M. Eads, M. Soares Nunes, A. Maddalena, M. Antonova, S. Matsuno, T. Boschi, Y. Karyotakis, Artur M. Ankowski, R. Milincic, P. Bernardini, L. Kashur, D. Edmunds, T. Stokes, A. Scaramelli, C. Bromberg, T. Safford, E. Tatar, L. Li, Utku Kose, Z. Djurcic, M. Leyton, M. E. Convery, D. Vargas, S. Green, K. Lande, Matthew L Strait, G. Barenboim, P. Guzowski, George Adamov, Jane Nachtman, E. Granados, B. Behera, Y. A. Ramachers, D. A. Martinez Caicedo, R. M. de Almeida, Yasar Onel, P. Lasorak, A. Izmaylov, J. K. Nelson, M. H. Shaevitz, N. Barros, Marcelo M. Guzzo, I. Caro Terrazas, R. Itay, K. Vaziri, F. Azfar, T. R. Junk, N. Poonthottathil, Christian Farnese, M. V. Diwan, Akitaka Ariga, Marvin L Marshak, A. Chiriacescu, T. Rehak, N. Martinez, L. Greenler, B. Guo, Frank Filthaut, J. Reichenbacher, S. Ventura, Riccardo Papaleo, P. Fernandez Menendez, J. Han, C. Y. Chi, M. Groh, D. J. Payne, C. Gotti, S. Biagi, Marco Adinolfi, M. Kordosky, L. Stanco, C. Jesús-Valls, Andrew Blake, L. Jiang, V. J. Guarino, J. Bremer, V. A. Kostelecký, L. Pickering, S. Manly, P. Hamilton, R. G. Van de Water, J. 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Gold, Ministerio de Ciencia e Innovación (España), Abi, B, Acciarri, R, Acero, M, Adamov, G, Adams, D, Adinolfi, M, Ahmad, Z, Ahmed, J, Alion, T, Monsalve, S, Alt, C, Anderson, J, Andreopoulos, C, Andrews, M, Andrianala, F, Andringa, S, Ankowski, A, Antonova, M, Antusch, S, Aranda-Fernandez, A, Ariga, A, Arnold, L, Arroyave, M, Asaadi, J, Aurisano, A, Aushev, V, Autiero, D, Azfar, F, Back, H, Back, J, Backhouse, C, Baesso, P, Bagby, L, Bajou, R, Balasubramanian, S, Baldi, P, Bambah, B, Barao, F, Barenboim, G, Barker, G, Barkhouse, W, Barnes, C, Barr, G, Monarca, J, Barros, N, Barrow, J, Bashyal, A, Basque, V, Bay, F, Alba, J, Beacom, J, Bechetoille, E, Behera, B, Bellantoni, L, Bellettini, G, Bellini, V, Beltramello, O, Belver, D, Benekos, N, Neves, F, Berger, J, Berkman, S, Bernardini, P, Berner, R, Berns, H, Bertolucci, S, Betancourt, M, Bezawada, Y, Bhattacharjee, M, Bhuyan, B, Biagi, S, Bian, J, Biassoni, M, Biery, K, Bilki, B, Bishai, M, Bitadze, A, Blake, A, Siffert, B, 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Barnes C., Barr G., Monarca J.B., Barros N., Barrow J.L., Bashyal A., Basque V., Bay F., Alba J.L.B., Beacom J.F., Bechetoille E., Behera B., Bellantoni L., Bellettini G., Bellini V., Beltramello O., Belver D., Benekos N., Neves F.B., Berger J., Berkman S., Bernardini P., Berner R.M., Berns H., Bertolucci S., Betancourt M., Bezawada Y., Bhattacharjee M., Bhuyan B., Biagi S., Bian J., Biassoni M., Biery K., Bilki B., Bishai M., Bitadze A., Blake A., Siffert B.B., Blaszczyk F.D.M., Blazey G.C., Blucher E., Boissevain J., Bolognesi S., Bolton T., Bonesini M., Bongrand M., Bonini F., Booth A., Booth C., Bordoni S., Borkum A., Boschi T., Bostan N., Bour P., Boyd S.B., Boyden D., Bracinik J., Braga D., Brailsford D., Brandt A., Bremer J., Brew C., Brianne E., Brice S.J., Brizzolari C., Bromberg C., Brooijmans G., Brooke J., Bross A., Brunetti G., Buchanan N., Budd H., Caiulo D., Calafiura P., Calcutt J., Calin M., Calvez S., Calvo E., Camilleri L., Caminata A., Campanelli M., Caratelli D., Carini G., Carlus B., Carniti P., Terrazas I.C., Carranza H., Castillo A., Castromonte C., Cattadori C., Cavalier F., Cavanna F., Centro S., Cerati G., Cervelli A., Villanueva A.C., Chalifour M., Chang C., Chardonnet E., Chatterjee A., Chattopadhyay S., Chaves J., Chen H., Chen M., Chen Y., Cherdack D., Chi C., Childress S., Chiriacescu A., Cho K., Choubey S., Christensen A., Christian D., Christodoulou G., Church E., Clarke P., Coan T.E., Cocco A.G., Coelho J.A.B., Conley E., Conrad J.M., Convery M., Corwin L., Cotte P., Cremaldi L., Cremonesi L., Crespo-Anadon J.I., Cristaldo E., Cross R., Cuesta C., Cui Y., Cussans D., Dabrowski M., Motta H., Da Silva Peres L., David C., David Q., Davies G.S., Davini S., Dawson J., De K., De Almeida R.M., Debbins P., De Bonis I., Decowski M.P., de Gouvea A., De Holanda P.C., De Icaza Astiz I.L., Deisting A., De Jong P., Delbart A., Delepine D., Delgado M., Dell'Acqua A., De Lurgio P., de Mello Neto J.R.T., DeMuth D.M., Dennis S., Densham C., Deptuch 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Horton-Smith G.A., Hostert M., Hourlier A., Howard B., Howell R., Huang J., Hugon J., Iles G., Ilic N., Iliescu A.M., Illingworth R., Ioannisian A., Itay R., Izmaylov A., James E., Jargowsky B., Jediny F., Jesus-Valls C., Ji X., Jiang L., Jimenez S., Jipa A., Joglekar A., Johnson C., Johnson R., Jones B., Jones S., Jung C.K., Junk T., Jwa Y., Kabirnezhad M., Kaboth A., Kadenko I., Kamiya F., Karagiorgi G., Karcher A., Karolak M., Karyotakis Y., Kasai S., Kasetti S.P., Kashur L., Kazaryan N., Kearns E., Keener P., Kelly K.J., Kemp E., Ketchum W., Kettell S.H., Khabibullin M., Khotjantsev A., Khvedelidze A., Kim D., King B., Kirby B., Kirby M., Klein J., Koehler K., Koerner L.W., Kohn S., Koller P.P., Kordosky M., Kosc T., Kose U., Kostelecky V.A., Kothekar K., Krennrich F., Kreslo I., Kudenko Y., Kudryavtsev V.A., Kulagin S., Kumar J., Kumar R., Kuruppu C., Kus V., Kutter T., Lambert A., Lande K., Lane C.E., Lang K., Langford T., Lasorak P., Last D., Lastoria C., Laundrie A., Lawrence A., Lazanu I., LaZur R., Le T., Learned J., LeBrun P., Miotto G.L., Lehnert R., de Oliveira M.A.L., Leitner M., Leyton M., Li L., Li S., Li S.W., Li T., Li Y., Liao H., Lin C.S., Lin S., Lister A., Littlejohn B.R., Liu J., Lockwitz S., Loew T., Lokajicek M., Lomidze I., Long K., Loo K., Lorca D., Lord T., LoSecco J.M., Louis W.C., Luk K.B., Luo X., Lurkin N., Lux T., Luzio V.P., MacFarland D., Machado A.A., Machado P., Macias C.T., Macier J.R., Maddalena A., Madigan P., Magill S., Mahn K., Maio A., Maloney J.A., Mandrioli G., Maneira J., Manenti L., Manly S., Mann A., Manolopoulos K., Plata M.M., Marchionni A., Marciano W., Marfatia D., Mariani C., Maricic J., Marinho F., Marino A.D., Marshak M., Marshall C., Marshall J., Marteau J., Martin-Albo J., Martinez N., Caicedo D.A.M., Martynenko S., Mason K., Mastbaum A., Masud M., Matsuno S., Matthews J., Mauger C., Mauri N., Mavrokoridis K., Mazza R., Mazzacane A., Mazzucato E., McCluskey E., McConkey N., McFarland K.S., McGrew C., McNab A., Mefodiev A., Mehta P., Melas P., Mellinato M., Mena O., Menary S., Mendez H., Menegolli A., Meng G., Messier M.D., Metcalf W., Mewes M., Meyer H., Miao T., Michna G., Miedema T., Migenda J., Milincic R., Miller W., Mills J., Milne C., Mineev O., Miranda O.G., Miryala S., Mishra C.S., Mishra S.R., Mislivec A., Mladenov D., Mocioiu I., Moffat K., Moggi N., Mohanta R., Mohayai T.A., Mokhov N., Molina J., Bueno L.M., Montanari A., Montanari C., Montanari D., Zetina L.M.M., Moon J., Mooney M., Moor A., Moreno D., Morgan B., Morris C., Mossey C., Motuk E., Moura C.A., Mousseau J., Mu W., Mualem L., Mueller J., Muether M., Mufson S., Muheim F., Muir A., Mulhearn M., Muramatsu H., Murphy S., Musser J., Nachtman J., Nagu S., Nalbandyan M., Nandakumar R., Naples D., Narita S., Navas-Nicolas D., Nayak N., Nebot-Guinot M., Necib L., Negishi K., Nelson J.K., Nesbit J., Nessi M., Newbold D., Newcomer M., Newhart D., Nichol R., Niner E., Nishimura K., Norman A., Norrick A., Northrop R., Novella P., Nowak J.A., Oberling M., Campo A.O.D., Olivier A., Onel Y., Onishchuk Y., Ott J., Pagani L., Pakvasa S., Palamara O., Palestini S., Paley J.M., Pallavicini M., Palomares C., Pantic E., Paolone V., Papadimitriou V., Papaleo R., Papanestis A., Paramesvaran S., Parke S., Parsa Z., Parvu M., Pascoli S., Pasqualini L., Pasternak J., Pater J., Patrick C., Patrizii L., Patterson R.B., Patton S.J., Patzak T., Paudel A., Paulos B., Paulucci L., Pavlovic Z., Pawloski G., Payne D., Pec V., Peeters S.J.M., Penichot Y., Pennacchio E., Penzo A., Peres O.L.G., Perry J., Pershey D., Pessina G., Petrillo G., Petta C., Petti R., Piastra F., Pickering L., Pietropaolo F., Pillow J., Pinzino J., Plunkett R., Poling R., Pons X., Poonthottathil N., Pordes S., Potekhin M., Potenza R., Potukuchi B.V.K.S., Pozimski J., Pozzato M., Prakash S., Prakash T., Prince S., Prior G., Pugnere D., Qi K., Qian X., Raaf J.L., Raboanary R., Radeka V., Rademacker J., Radics B., Rafique A., Raguzin E., Rai M., Rajaoalisoa 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Shaevitz M.H., Shafaq S., Shamma M., Sharma H.R., Sharma R., Shaw T., Shepherd-Themistocleous C., Shin S., Shooltz D., Shrock R., Simard L., Simos N., Sinclair J., Sinev G., Singh J., Singh V., Sipos R., Sippach F.W., Sirri G., Sitraka A., Siyeon K., Smargianaki D., Smith A., Smith E., Smith P., Smolik J., Smy M., Snopok P., Nunes M.S., Sobel H., Soderberg M., Salinas C.J.S., Soldner-Rembold S., Solomey N., Solovov V., Sondheim W.E., Sorel M., Soto-Oton J., Sousa A., Soustruznik K., Spagliardi F., Spanu M., Spitz J., Spooner N.J.C., Spurgeon K., Staley R., Stancari M., Stanco L., Steiner H.M., Stewart J., Stillwell B., Stock J., Stocker F., Stokes T., Strait M., Strauss T., Striganov S., Stuart A., Summers D., Surdo A., Susic V., Suter L., Sutera C.M., Svoboda R., Szczerbinska B., Szelc A.M., Talaga R., Tanaka H.A., Oregui B.T., Tapper A., Tariq S., Tatar E., Tayloe R., Teklu A.M., Tenti M., Terao K., Ternes C.A., Terranova F., Testera G., Thea A., Thompson J.L., Thorn C., Timm S.C., Tonazzo A., Torti M., Tortola M., Tortorici F., Totani D., Toups M., Touramanis C., Trevor J., Trzaska W.H., Tsai Y.T., Tsamalaidze Z., Tsang K.V., Tsverava N., Tufanli S., Tull C., Tyley E., Tzanov M., Uchida M.A., Urheim J., Usher T., Vagins M.R., Vahle P., Valdiviesso G.A., Valencia E., Vallari Z., Valle J.W.F., Vallecorsa S., Van Berg R., Van de Water R.G., Forero D.V., Varanini F., Vargas D., Varner G., Vasel J., Vasseur G., Vaziri K., Ventura S., Verdugo A., Vergani S., Vermeulen M.A., Verzocchi M., de Souza H.V., Vignoli C., Vilela C., Viren B., Vrba T., Wachala T., Waldron A.V., Wallbank M., Wang H., Wang J., Wang Y., Warburton K., Warner D., Wascko M., Waters D., Watson A., Weatherly P., Weber A., Weber M., Wei H., Weinstein A., Wenman D., Wetstein M., While M.R., White A., Whitehead L.H., Whittington D., Wilking M.J., Wilkinson C., Williams Z., Wilson F., Wilson R.J., Wolcott J., Wongjirad T., Wood K., Wood L., Worcester E., Worcester M., Wret C., Wu W., Xiao Y., Yang G., Yang T., Yershov N., Yonehara K., Young T., Yu B., Yu J., Zaki R., Zalesak J., Zambelli L., Zamorano B., Zani A., Zazueta L., Zeller G.P., Zennamo J., Zeug K., Zhang C., Zhao M., Zhivun E., Zhu G., Zimmerman E.D., Zito M., Zucchelli S., Zuklin J., Zutshi V., Zwaska R., Abi, B., Acciarri, R., Acero, M. 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M., Berns, H., Bertolucci, S., Betancourt, M., Bezawada, Y., Bhattacharjee, M., Bhuyan, B., Biagi, S., Bian, J., Biassoni, M., Biery, K., Bilki, B., Bishai, M., Bitadze, A., Blake, A., Siffert, B. B., Blaszczyk, F. D. M., Blazey, G. C., Blucher, E., Boissevain, J., Bolognesi, S., Bolton, T., Bonesini, M., Bongrand, M., Bonini, F., Booth, A., Booth, C., Bordoni, S., Borkum, A., Boschi, T., Bostan, N., Bour, P., Boyd, S. B., Boyden, D., Bracinik, J., Braga, D., Brailsford, D., Brandt, A., Bremer, J., Brew, C., Brianne, E., Brice, S. J., Brizzolari, C., Bromberg, C., Brooijmans, G., Brooke, J., Bross, A., Brunetti, G., Buchanan, N., Budd, H., Caiulo, D., Calafiura, P., Calcutt, J., Calin, M., Calvez, S., Calvo, E., Camilleri, L., Caminata, A., Campanelli, M., Caratelli, D., Carini, G., Carlus, B., Carniti, P., Terrazas, I. C., Carranza, H., Castillo, A., Castromonte, C., Cattadori, C., Cavalier, F., Cavanna, F., Centro, S., Cerati, G., Cervelli, A., Villanueva, A. 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A., Gardiner, S., Gastler, D., Ge, G., Gelli, B., Gendotti, A., Gent, S., Ghorbani-Moghaddam, Z., Gibin, D., Gil-Botella, I., Girerd, C., Giri, A. K., Gnani, D., Gogota, O., Gold, M., Gollapinni, S., Gollwitzer, K., Gomes, R. A., Bermeo, L. V. G., Fajardo, L. S. G., Gonnella, F., Gonzalez-Cuevas, J. A., Goodman, M. C., Goodwin, O., Goswami, S., Gotti, C., Goudzovski, E., Grace, C., Graham, M., Gramellini, E., Gran, R., Granados, E., Grant, A., Grant, C., Gratieri, D., Green, P., Green, S., Greenler, L., Greenwood, M., Greer, J., Griffith, W. C., Groh, M., Grudzinski, J., Grzelak, K., Gu, W., Guarino, V., Guenette, R., Guglielmi, A., Guo, B., Guthikonda, K. K., Gutierrez, R., Guzowski, P., Guzzo, M. M., Gwon, S., Habig, A., Hackenburg, A., Hadavand, H., Haenni, R., Hahn, A., Haigh, J., Haiston, J., Hamernik, T., Hamilton, P., Han, J., Harder, K., Harris, D. A., Hartnell, J., Hasegawa, T., Hatcher, R., Hazen, E., Heavey, A., Heeger, K. M., Heise, J., Hennessy, K., Henry, S., Morquecho, M. A. H., Herner, K., Hertel, L., Hesam, A. S., Hewes, J., Higuera, A., Hill, T., Hillier, S. J., Himmel, A., Hoff, J., Hohl, C., Holin, A., Hoppe, E., Horton-Smith, G. A., Hostert, M., Hourlier, A., Howard, B., Howell, R., Huang, J., Hugon, J., Iles, G., Ilic, N., Iliescu, A. M., Illingworth, R., Ioannisian, A., Itay, R., Izmaylov, A., James, E., Jargowsky, B., Jediny, F., Jesus-Valls, C., Ji, X., Jiang, L., Jimenez, S., Jipa, A., Joglekar, A., Johnson, C., Johnson, R., Jones, B., Jones, S., Jung, C. K., Junk, T., Jwa, Y., Kabirnezhad, M., Kaboth, A., Kadenko, I., Kamiya, F., Karagiorgi, G., Karcher, A., Karolak, M., Karyotakis, Y., Kasai, S., Kasetti, S. P., Kashur, L., Kazaryan, N., Kearns, E., Keener, P., Kelly, K. J., Kemp, E., Ketchum, W., Kettell, S. H., Khabibullin, M., Khotjantsev, A., Khvedelidze, A., Kim, D., King, B., Kirby, B., Kirby, M., Klein, J., Koehler, K., Koerner, L. W., Kohn, S., Koller, P. P., Kordosky, M., Kosc, T., Kose, U., Kostelecky, V. A., Kothekar, K., Krennrich, F., Kreslo, I., Kudenko, Y., Kudryavtsev, V. A., Kulagin, S., Kumar, J., Kumar, R., Kuruppu, C., Kus, V., Kutter, T., Lambert, A., Lande, K., Lane, C. E., Lang, K., Langford, T., Lasorak, P., Last, D., Lastoria, C., Laundrie, A., Lawrence, A., Lazanu, I., Lazur, R., Le, T., Learned, J., Lebrun, P., Miotto, G. L., Lehnert, R., de Oliveira, M. A. L., Leitner, M., Leyton, M., Li, L., Li, S., Li, S. W., Li, T., Li, Y., Liao, H., Lin, C. S., Lin, S., Lister, A., Littlejohn, B. R., Liu, J., Lockwitz, S., Loew, T., Lokajicek, M., Lomidze, I., Long, K., Loo, K., Lorca, D., Lord, T., Losecco, J. M., Louis, W. C., Luk, K. B., Luo, X., Lurkin, N., Lux, T., Luzio, V. P., Macfarland, D., Machado, A. A., Machado, P., Macias, C. T., Macier, J. R., Maddalena, A., Madigan, P., Magill, S., Mahn, K., Maio, A., Maloney, J. A., Mandrioli, G., Maneira, J., Manenti, L., Manly, S., Mann, A., Manolopoulos, K., Plata, M. M., Marchionni, A., Marciano, W., Marfatia, D., Mariani, C., Maricic, J., Marinho, F., Marino, A. D., Marshak, M., Marshall, C., Marshall, J., Marteau, J., Martin-Albo, J., Martinez, N., Caicedo, D. A. M., Martynenko, S., Mason, K., Mastbaum, A., Masud, M., Matsuno, S., Matthews, J., Mauger, C., Mauri, N., Mavrokoridis, K., Mazza, R., Mazzacane, A., Mazzucato, E., Mccluskey, E., Mcconkey, N., Mcfarland, K. S., Mcgrew, C., Mcnab, A., Mefodiev, A., Mehta, P., Melas, P., Mellinato, M., Mena, O., Menary, S., Mendez, H., Menegolli, A., Meng, G., Messier, M. D., Metcalf, W., Mewes, M., Meyer, H., Miao, T., Michna, G., Miedema, T., Migenda, J., Milincic, R., Miller, W., Mills, J., Milne, C., Mineev, O., Miranda, O. G., Miryala, S., Mishra, C. S., Mishra, S. R., Mislivec, A., Mladenov, D., Mocioiu, I., Moffat, K., Moggi, N., Mohanta, R., Mohayai, T. A., Mokhov, N., Molina, J., Bueno, L. M., Montanari, A., Montanari, C., Montanari, D., Zetina, L. M. M., Moon, J., Mooney, M., Moor, A., Moreno, D., Morgan, B., Morris, C., Mossey, C., Motuk, E., Moura, C. A., Mousseau, J., Mu, W., Mualem, L., Mueller, J., Muether, M., Mufson, S., Muheim, F., Muir, A., Mulhearn, M., Muramatsu, H., Murphy, S., Musser, J., Nachtman, J., Nagu, S., Nalbandyan, M., Nandakumar, R., Naples, D., Narita, S., Navas-Nicolas, D., Nayak, N., Nebot-Guinot, M., Necib, L., Negishi, K., Nelson, J. K., Nesbit, J., Nessi, M., Newbold, D., Newcomer, M., Newhart, D., Nichol, R., Niner, E., Nishimura, K., Norman, A., Norrick, A., Northrop, R., Novella, P., Nowak, J. A., Oberling, M., Campo, A. O. D., Olivier, A., Onel, Y., Onishchuk, Y., Ott, J., Pagani, L., Pakvasa, S., Palamara, O., Palestini, S., Paley, J. M., Pallavicini, M., Palomares, C., Pantic, E., Paolone, V., Papadimitriou, V., Papaleo, R., Papanestis, A., Paramesvaran, S., Parke, S., Parsa, Z., Parvu, M., Pascoli, S., Pasqualini, L., Pasternak, J., Pater, J., Patrick, C., Patrizii, L., Patterson, R. B., Patton, S. J., Patzak, T., Paudel, A., Paulos, B., Paulucci, L., Pavlovic, Z., Pawloski, G., Payne, D., Pec, V., Peeters, S. J. M., Penichot, Y., Pennacchio, E., Penzo, A., Peres, O. L. G., Perry, J., Pershey, D., Pessina, G., Petrillo, G., Petta, C., Petti, R., Piastra, F., Pickering, L., Pietropaolo, F., Pillow, J., Pinzino, J., Plunkett, R., Poling, R., Pons, X., Poonthottathil, N., Pordes, S., Potekhin, M., Potenza, R., Potukuchi, B. V. K. S., Pozimski, J., Pozzato, M., Prakash, S., Prakash, T., Prince, S., Prior, G., Pugnere, D., Qi, K., Qian, X., Raaf, J. L., Raboanary, R., Radeka, V., Rademacker, J., Radics, B., Rafique, A., Raguzin, E., Rai, M., Rajaoalisoa, M., Rakhno, I., Rakotondramanana, H. T., Rakotondravohitra, L., Ramachers, Y. A., Rameika, R., Delgado, M. A. R., Ramson, B., Rappoldi, A., Raselli, G., Ratoff, P., Ravat, S., Razafinime, H., Real, J. S., Rebel, B., Redondo, D., Reggiani-Guzzo, M., Rehak, T., Reichenbacher, J., Reitzner, S. D., Renshaw, A., Rescia, S., Resnati, F., Reynolds, A., Riccobene, G., Rice, L. C. J., Rielage, K., Rigaut, Y., Rivera, D., Rochester, L., Roda, M., Rodrigues, P., Alonso, M. J. R., Rondon, J. R., Roeth, A. J., Rogers, H., Rosauro-Alcaraz, S., Rossella, M., Rout, J., Roy, S., Rubbia, A., Rubbia, C., Russell, B., Russell, J., Ruterbories, D., Saakyan, R., Sacerdoti, S., Safford, T., Sahu, N., Sala, P., Samios, N., Sanchez, M. C., Sanders, D. A., Sankey, D., Santana, S., Santos-Maldonado, M., Saoulidou, N., Sapienza, P., Sarasty, C., Sarcevic, I., Savage, G., Savinov, V., Scaramelli, A., Scarff, A., Scarpelli, A., Schaffer, T., Schellman, H., Schlabach, P., Schmitz, D., Scholberg, K., Schukraft, A., Segreto, E., Sensenig, J., Seong, I., Sergi, A., Sergiampietri, F., Sgalaberna, D., Shaevitz, M. H., Shafaq, S., Shamma, M., Sharma, H. R., Sharma, R., Shaw, T., Shepherd-Themistocleous, C., Shin, S., Shooltz, D., Shrock, R., Simard, L., Simos, N., Sinclair, J., Sinev, G., Singh, J., Singh, V., Sipos, R., Sippach, F. W., Sirri, G., Sitraka, A., Siyeon, K., Smargianaki, D., Smith, A., Smith, E., Smith, P., Smolik, J., Smy, M., Snopok, P., Nunes, M. S., Sobel, H., Soderberg, M., Salinas, C. J. S., Soldner-Rembold, S., Solomey, N., Solovov, V., Sondheim, W. E., Sorel, M., Soto-Oton, J., Sousa, A., Soustruznik, K., Spagliardi, F., Spanu, M., Spitz, J., Spooner, N. J. C., Spurgeon, K., Staley, R., Stancari, M., Stanco, L., Steiner, H. M., Stewart, J., Stillwell, B., Stock, J., Stocker, F., Stokes, T., Strait, M., Strauss, T., Striganov, S., Stuart, A., Summers, D., Surdo, A., Susic, V., Suter, L., Sutera, C. M., Svoboda, R., Szczerbinska, B., Szelc, A. M., Talaga, R., Tanaka, H. A., Oregui, B. T., Tapper, A., Tariq, S., Tatar, E., Tayloe, R., Teklu, A. M., Tenti, M., Terao, K., Ternes, C. A., Terranova, F., Testera, G., Thea, A., Thompson, J. L., Thorn, C., Timm, S. C., Tonazzo, A., Torti, M., Tortola, M., Tortorici, F., Totani, D., Toups, M., Touramanis, C., Trevor, J., Trzaska, W. H., Tsai, Y. T., Tsamalaidze, Z., Tsang, K. V., Tsverava, N., Tufanli, S., Tull, C., Tyley, E., Tzanov, M., Uchida, M. A., Urheim, J., Usher, T., Vagins, M. R., Vahle, P., Valdiviesso, G. A., Valencia, E., Vallari, Z., Valle, J. W. F., Vallecorsa, S., Van Berg, R., Van de Water, R. G., Forero, D. V., Varanini, F., Vargas, D., Varner, G., Vasel, J., Vasseur, G., Vaziri, K., Ventura, S., Verdugo, A., Vergani, S., Vermeulen, M. A., Verzocchi, M., de Souza, H. V., Vignoli, C., Vilela, C., Viren, B., Vrba, T., Wachala, T., Waldron, A. V., Wallbank, M., Wang, H., Wang, J., Wang, Y., Warburton, K., Warner, D., Wascko, M., Waters, D., Watson, A., Weatherly, P., Weber, A., Weber, M., Wei, H., Weinstein, A., Wenman, D., Wetstein, M., While, M. R., White, A., Whitehead, L. H., Whittington, D., Wilking, M. J., Wilkinson, C., Williams, Z., Wilson, F., Wilson, R. J., Wolcott, J., Wongjirad, T., Wood, K., Wood, L., Worcester, E., Worcester, M., Wret, C., Wu, W., Xiao, Y., Yang, G., Yang, T., Yershov, N., Yonehara, K., Young, T., Yu, B., Yu, J., Zaki, R., Zalesak, J., Zambelli, L., Zamorano, B., Zani, A., Zazueta, L., Zeller, G. P., Zennamo, J., Zeug, K., Zhang, C., Zhao, M., Zhivun, E., Zhu, G., Zimmerman, E. D., Zito, M., Zucchelli, S., Zuklin, J., Zutshi, V., and Zwaska, R.
Subjects: Physics and Astronomy (miscellaneous), Physics::Instrumentation and Detectors, 01 natural sciences, Particle detector, Physics, Particles & Fields, Nuclear physics, neutrino, 0103 physical sciences, Neutrino oscillations, neutrino physiscs, Deep Underground Neutrino Experiment, Deep Underground Neutrino Experiment, Neutrino oscillation experiment, DISTRIBUTIONS, Fermilab, High Energy Physics, LEPTON SCATTERING, 010306 general physics, Neutrino oscillation, Engineering (miscellaneous), Physics, Science & Technology, 010308 nuclear & particles physics, Detector, High Energy Physics::Phenomenology, Neutrino detector, Physical Sciences, High Energy Physics::Experiment, Neutrino, Lepton
Abstract: The sensitivity of the Deep Underground Neutrino Experiment (DUNE) to neutrino oscillation is determined, based on a full simulation, reconstruction, and event selection of the far detector and a full simulation and parameterized analysis of the near detector. Detailed uncertainties due to the flux prediction, neutrino interaction model, and detector effects are included. DUNE will resolve the neutrino mass ordering to a precision of 5$$\sigma $$ σ , for all $$\delta _{\mathrm{CP}}$$ δ CP values, after 2 years of running with the nominal detector design and beam configuration. It has the potential to observe charge-parity violation in the neutrino sector to a precision of 3$$\sigma $$ σ (5$$\sigma $$ σ ) after an exposure of 5 (10) years, for 50% of all $$\delta _{\mathrm{CP}}$$ δ CP values. It will also make precise measurements of other parameters governing long-baseline neutrino oscillation, and after an exposure of 15 years will achieve a similar sensitivity to $$\sin ^{2} 2\theta _{13}$$ sin 2 2 θ 13 to current reactor experiments.
Published: 2020

37. Resonant X-ray Emission Spectroscopy with a SASE Beam

Author: Christopher J. Milne, Yves Kayser, Jacinto Sá, Rafał Fanselow, Wojciech Błachucki, Anna Wach, and Jakub Szlachetko
Subjects: Technology, Materials science, QH301-705.5, Atom and Molecular Physics and Optics, QC1-999, Astrophysics::High Energy Astrophysical Phenomena, X-ray free-electron laser (XFEL), law.invention, Optics, law, Ionization, General Materials Science, Spontaneous emission, Emission spectrum, Irradiation, Biology (General), QD1-999, Instrumentation, Fluid Flow and Transfer Processes, Spectrometer, business.industry, Physics, X-ray free-electron laser (XFEL), resonant X-ray emission spectroscopy (RXES) with self-amplified spontaneous emission (SASE) XFEL beam, Process Chemistry and Technology, General Engineering, Reconstruction algorithm, resonant X-ray emission spectroscopy (RXES) with self-amplified spontaneous emission (SASE) XFEL beam, Engineering (General). Civil engineering (General), Laser, Computer Science Applications, Chemistry, Physics::Accelerator Physics, Atom- och molekylfysik och optik, TA1-2040, reconstruction of RXES planes, business, Beam (structure)
Abstract: Featured Application In the present work, RXES planes are reconstructed with high energy resolution from the experimental spectra of the X-ray radiation emitted from a sample and of incident X-ray pulses delivered by an XFEL operated in the raw SASE mode. The dependence of the reconstructed RXES planes' quality on the number of recorded XFEL shots is studied. Aqueous iron (III) oxide nanoparticles were irradiated with pure self-amplified spontaneous emission (SASE) X-ray free-electron laser (XFEL) pulses tuned to the energy around the Fe K-edge ionization threshold. For each XFEL shot, the incident X-ray pulse spectrum and Fe K beta emission spectrum were measured synchronously with dedicated spectrometers and processed through a reconstruction algorithm allowing for the determination of Fe K beta resonant X-ray emission spectroscopy (RXES) plane with high energy resolution. The influence of the number of X-ray shots employed in the experiment on the reconstructed data quality was evaluated, enabling the determination of thresholds for good data acquisition and experimental times essential for practical usage of scarce XFEL beam times.
Published: 2021

38. Erratum: 'Nonlinear XUV-optical transient grating spectroscopy at the Si L2,3-edge' [Appl. Phys. Lett. 114, 181101 (2019)]

Author: R. Cucini, Peter Radi, A. Simoncig, R. Bohinc, Andrea Cannizzo, Filippo Bencivenga, Nicola Mahne, Emanuele Pedersoli, Z. Ollmann, Gregor Knopp, Julien Réhault, Christopher J. Milne, Keith A. Nelson, Laura Foglia, A. A. Maznev, Flavio Capotondi, Jakub Szlachetko, Hans-Martin Frey, Thomas Feurer, Georgios Pamfilidis, Claudio Masciovecchio, and R. Mincigrucci
Subjects: Nonlinear system, Optics, Materials science, Physics and Astronomy (miscellaneous), business.industry, Extreme ultraviolet, Transient (oscillation), Edge (geometry), Grating, business, Spectroscopy
Published: 2021

39. Core-level nonlinear spectroscopy triggered by stochastic X-ray pulses

Author: Rafael Abela, Rolf Follath, Marcus Lundberg, Jens Rehanek, Christopher J. Milne, Wojciech Błachucki, Jakub Szlachetko, Krzysztof Tyrała, Joanna Czapla-Masztafiak, Yves Kayser, Mickaël G. Delcey, Roberto Alonso-Mori, Leonardo Sala, Jacinto Sá, Gregor Knopp, Pavle Juranić, Diling Zhu, and Matjaž Kavčič
Subjects: Science, Astrophysics::High Energy Astrophysical Phenomena, Ecology (disciplines), General Physics and Astronomy, Nonlinear spectroscopy, 02 engineering and technology, Physical Chemistry, 01 natural sciences, Article, General Biochemistry, Genetics and Molecular Biology, X-rays, 0103 physical sciences, Statistical physics, lcsh:Science, 010306 general physics, Fysikalisk kemi, Multidisciplinary, Stochastic process, Atomic and molecular interactions with photons, General Chemistry, 021001 nanoscience & nanotechnology, Fundamental physics, Core level, lcsh:Q, 0210 nano-technology
Abstract: Stochastic processes are highly relevant in research fields as different as neuroscience, economy, ecology, chemistry, and fundamental physics. However, due to their intrinsic unpredictability, stochastic mechanisms are very challenging for any kind of investigations and practical applications. Here we report the deliberate use of stochastic X-ray pulses in two-dimensional spectroscopy to the simultaneous mapping of unoccupied and occupied electronic states of atoms in a regime where the opacity and transparency properties of matter are subject to the incident intensity and photon energy. A readily transferable matrix formalism is presented to extract the electronic states from a dataset measured with the monitored input from a stochastic excitation source. The presented formalism enables investigations of the response of the electronic structure to irradiation with intense X-ray pulses while the time structure of the incident pulses is preserved., Free electron X-ray laser pulses, generated by self-amplified spontaneous emission, are stochastic in nature. Here the authors present a reconstruction method for 2D spectroscopy while preserving the intrinsic properties of the incident pulses and apply it to a study towards X-ray intensity induced effects.
Published: 2019

40. Towards X-ray transient grating spectroscopy

Author: Rolf Follath, Gerhard Ingold, Ulrich Wagner, C. Svetina, Claudio Cirelli, Benedikt Rösner, Maxime Lebugle, Henrik T. Lemke, Gediminas Seniutinas, Martin Beck, Paul Beaud, J. Krempasky, Gregor Knopp, Claude Pradervand, Serhane Zerdane, I Mochi, Adam Kubec, Frieder Koch, Vincent Esposito, Jérémy R. Rouxel, Uwe Flechsig, Giulia F. Mancini, Majed Chergui, Christopher J. Milne, Roman Mankowsky, Bill Pedrini, and Christian David
Subjects: Materials science, Physics::Optics, 02 engineering and technology, phase-contrast, Grating, 01 natural sciences, law.invention, 010309 optics, Optics, Interference (communication), law, 0103 physical sciences, Talbot effect, Spectroscopy, Diffraction grating, business.industry, 021001 nanoscience & nanotechnology, Laser, Atomic and Molecular Physics, and Optics, optics, radiation, Temporal resolution, Femtosecond, transport, 0210 nano-technology, business
Abstract: The extension of transient grating spectroscopy to the x-ray regime will create numerous opportunities, ranging from the study of thermal transport in the ballistic regime to charge, spin, and energy transfer processes with atomic spatial and femtosecond temporal resolution. Studies involving complicated split-and-delay lines have not yet been successful in achieving this goal. Here we propose a novel, simple method based on the Talbot effect for converging beams, which can easily be implemented at current x-ray free electron lasers. We validate our proposal by analyzing printed interference patterns on polymethyl methacrylate and gold samples using similar to 3 keV X-ray pulses. (C) 2019 Optical Society of America
Published: 2019

41. Femtosecond phase-transition in hard x-ray excited bismuth

Author: Celestino Padeste, Laura Vera, Sanghoon Song, Henrik Jonsson, Ana Diaz, Pavle Juranić, Istvan Mohacsi, Mikako Makita, Carl Caleman, Valerie Panneels, Nadia Opara, Ismo Vartiainen, Beata Ziaja-Motyka, Paul Beaud, Philip R. Willmott, Nikita Medvedev, Marcin Sikorski, Vikrant Saxena, Aldo Mozzanica, Christopher J. Milne, Alke Meents, and Christian David
Subjects: 0301 basic medicine, Phase transition, Materials science, Phonon, FOS: Physical sciences, lcsh:Medicine, Physics::Optics, chemistry.chemical_element, Crystal structure, Physical Chemistry, Article, law.invention, Bismuth, Condensed Matter::Materials Science, 03 medical and health sciences, 0302 clinical medicine, law, Condensed Matter::Superconductivity, lcsh:Science, Fysikalisk kemi, Condensed Matter - Materials Science, Multidisciplinary, lcsh:R, Materials Science (cond-mat.mtrl-sci), Condensed Matter Physics, Laser, 3. Good health, 030104 developmental biology, chemistry, Excited state, Femtosecond, lcsh:Q, Atomic physics, ddc:600, Den kondenserade materiens fysik, 030217 neurology & neurosurgery, Excitation
Abstract: The evolution of the bismuth crystal structure upon excitation of its A$_{1g}$ phonon has been intensely studied with short pulse optical lasers. Here we present the first-time observation of a hard x-ray induced ultrafast phase transition in a bismuth single crystal, at high intensities (~$10^{14}$ W/cm$^2$). The lattice evolution was followed using a recently demonstrated x-ray single-shot probing setup. The time evolution of the (111) Bragg peak intensity showed strong dependence on the excitation fluence. After exposure to a sufficiently intense x-ray pulse, the peak intensity dropped to zero within 300fs, i.e. faster than one oscillation period of the A1g mode at room temperature. Our analysis indicates a nonthermal origin of a lattice disordering process, and excludes interpretations based on electron-ion equilibration process, or on thermodynamic heating process leading to a plasma formation., Comment: Main text 10 pages, 3 figures. Appendix 3 pages, 2 figures
Published: 2019

42. Tracking multiple components of a nuclear wavepacket in photoexcited Cu(I)-phenanthroline complex using ultrafast X-ray spectroscopy

Author: Tokushi Sato, György Vankó, Christopher J. Milne, Tetsuo Katayama, Makina Yabashi, R. Bohinc, Dmitry Khakhulin, Shunsuke Nozawa, Jakub Szlachetko, Tadashi Togashi, Wojciech Gawelda, Christian Bressler, Shin-ichi Adachi, Thomas J. Penfold, Zoltán Németh, Frederico A. Lima, Thomas Northey, and Shigeki Owada
Subjects: 0301 basic medicine, Reaction kinetics and dynamics, Photochemistry, Wave packet, Science, Degrees of freedom (physics and chemistry), General Physics and Astronomy, 02 engineering and technology, Molecular physics, Article, General Biochemistry, Genetics and Molecular Biology, 03 medical and health sciences, Physics::Chemical Physics, lcsh:Science, Physics, Multidisciplinary, Relaxation (NMR), General Chemistry, 021001 nanoscience & nanotechnology, Potential energy, Bond length, 030104 developmental biology, Excited state, Molecular vibration, Femtosecond, lcsh:Q, ddc:500, 0210 nano-technology
Abstract: Nature Communications 10(1), 3606 (2019). doi:10.1038/s41467-019-11499-w, Disentangling the strong interplay between electronic and nuclear degrees of freedom is essential to achieve a full understanding of excited state processes during ultrafast nonadiabatic chemical reactions. However, the complexity of multi-dimensional potential energy surfaces means that this remains challenging. The energy flow during vibrational and electronic relaxation processes can be explored with structural sensitivity by probing a nuclear wavepacket using femtosecond time-resolved X-ray Absorption Near Edge Structure (TR-XANES). However, it remains unknown to what level of detail vibrational motions are observable in this X-ray technique. Herein we track the wavepacket dynamics of a prototypical [Cu(2,9-dimethyl-1,10-phenanthroline)2]+ complex using TR-XANES. We demonstrate that sensitivity to individual wavepacket components can be modulated by the probe energy and that the bond length change associated with molecular breathing mode can be tracked with a sub-Angstrom resolution beyond optical-domain observables. Importantly, our results reveal how state-of-the-art TR-XANES provides deeper insights of ultrafast nonadiabatic chemical reactions., Published by Nature Publishing Group UK, [London]
Published: 2019

43. Nonlinear XUV-optical transient grating spectroscopy at the Si L2,3-edge

Author: Gregor Knopp, Julien Réhault, R. Cucini, Nicola Mahne, Laura Foglia, Emanuele Pedersoli, Thomas Feurer, Flavio Capotondi, Jakub Szlachetko, Andrea Cannizzo, Hans-Martin Frey, Keith A. Nelson, A. A. Maznev, Filippo Bencivenga, A. Simoncig, Georgios Pamfilidis, Claudio Masciovecchio, Peter Radi, R. Mincigrucci, R. Bohinc, Z. Ollmann, and Christopher J. Milne
Subjects: 010302 applied physics, Photon, Materials science, Physics and Astronomy (miscellaneous), Auger effect, Physics::Optics, 02 engineering and technology, Photon energy, Grating, 021001 nanoscience & nanotechnology, Laser, 7. Clean energy, 01 natural sciences, law.invention, symbols.namesake, Absorption edge, law, Extreme ultraviolet, 0103 physical sciences, symbols, Atomic physics, 0210 nano-technology, Spectroscopy
Abstract: Time-resolved transient grating (TG) spectroscopy facilitates detailed studies of electron dynamics and transport phenomena by means of a periodic excitation of matter with coherent ultrashort light pulses. Several current and next generation free-electron laser (FEL) facilities provide fully coherent pulses with few femtosecond pulse durations and extreme ultraviolet (XUV) photon energies. Thus, they allow for transient grating experiments with periodicities as small as tens of nanometers and with element specific photon energies. Here, we demonstrate the element specificity of XUV TG (X-TG) experiments by tuning the photon energy across the Si L2,3-edge of Si3N4. We observe a shortening of the signal decay when increasing the XUV photon energy above the absorption edge. The analysis of the wavelength dependent signal shows that the faster decay is driven by the increase in the charge carrier density. From the decay constants the interband Auger coefficient at elevated temperatures and high electron densities has been determined.Time-resolved transient grating (TG) spectroscopy facilitates detailed studies of electron dynamics and transport phenomena by means of a periodic excitation of matter with coherent ultrashort light pulses. Several current and next generation free-electron laser (FEL) facilities provide fully coherent pulses with few femtosecond pulse durations and extreme ultraviolet (XUV) photon energies. Thus, they allow for transient grating experiments with periodicities as small as tens of nanometers and with element specific photon energies. Here, we demonstrate the element specificity of XUV TG (X-TG) experiments by tuning the photon energy across the Si L2,3-edge of Si3N4. We observe a shortening of the signal decay when increasing the XUV photon energy above the absorption edge. The analysis of the wavelength dependent signal shows that the faster decay is driven by the increase in the charge carrier density. From the decay constants the interband Auger coefficient at elevated temperatures and high electron dens...
Published: 2019

44. Inception of electronic damage of matter by photon-driven post-ionization mechanisms

Author: Wojciech Błachucki, Joanna Czapla-Masztafiak, Yves Kayser, Pavle Juranić, Meiyuan Guo, Jacinto Sá, Christopher J. Milne, Erik Källman, Matjaž Kavčič, Jens Rehanek, Jakub Szlachetko, Gregor Knopp, and Marcus Lundberg
Subjects: Fysikalisk kemi, Radiation, Materials science, Attosecond, Atom and Molecular Physics and Optics, Pulse duration, Electronic structure, Condensed Matter Physics, Laser, Solvated electron, Physical Chemistry, Spectral line, law.invention, ARTICLES, Liquids and Solutions, law, Ionization, Femtosecond, lcsh:QD901-999, Atom- och molekylfysik och optik, lcsh:Crystallography, Atomic physics, Instrumentation, Spectroscopy
Abstract: "Probe-before-destroy" methodology permitted diffraction and imaging measurements of intact specimens using ultrabright but highly destructive X-ray free-electron laser (XFEL) pulses. The methodology takes advantage of XFEL pulses ultrashort duration to outrun the destructive nature of the X-rays. Atomic movement, generally on the order of >50 fs, regulates the maximum pulse duration for intact specimen measurements. In this contribution, we report the electronic structure damage of a molecule with ultrashort X-ray pulses under preservation of the atoms' positions. A detailed investigation of the X-ray induced processes revealed that X-ray absorption events in the solvent produce a significant number of solvated electrons within attosecond and femtosecond timescales that are capable of coulombic interactions with the probed molecules. The presented findings show a strong influence on the experimental spectra coming from ionization of the probed atoms' surroundings leading to electronic structure modification much faster than direct absorption of photons. This work calls for consideration of this phenomenon in cases focused on samples embedded in, e.g., solutions or in matrices, which in fact concerns most of the experimental studies.
Published: 2019

45. Author Correction: Hard X-ray transient grating spectroscopy on bismuth germanate

Author: Eugenio Ferrari, Georgios Pamfilidis, Adam Kubec, Laura Foglia, Claudio Cirelli, Maria Grazia Izzo, Jérémy R. Rouxel, Paul Beaud, Danny Fainozzi, Edwin Divall, C. Svetina, Roman Mankowsky, Bill Pedrini, Andre Al Haddad, Frieder Koch, Renato Torre, Gediminas Seniutinas, Florian Döring, Riccardo Cucini, Christopher Arrell, Serhane Zerdane, Elia Razzoli, Urs Staub, Henrik T. Lemke, R. Mincigrucci, Sara Catalini, Filippo Bencivenga, Giulia F. Mancini, Yunpei Deng, Cettina Bottari, Aldo Mozzanica, Hiroki Ueda, Keith A. Nelson, Claudio Masciovecchio, Majed Chergui, Simon Gerber, Christopher J. Milne, Benedikt Rösner, Gregor Knopp, Alessandro Gessini, Philip J. M. Johnson, Dmitry Ozerov, Alexei Maznev, Max Burian, Mathias Sander, Luc Patthey, and Christian David
Subjects: chemistry.chemical_compound, Optics, Materials science, X-ray transient, chemistry, business.industry, Grating, business, Spectroscopy, Bismuth germanate, Atomic and Molecular Physics, and Optics, Electronic, Optical and Magnetic Materials
Published: 2021

46. Investigating DNA Radiation Damage Using X-Ray Absorption Spectroscopy

Author: Rafael Abela, Thomas Huthwelker, Jakub Szlachetko, Ewelina Lipiec, Camelia N. Borca, Thomas J. Penfold, Wojciech M. Kwiatek, Jacinto Sá, Christopher J. Milne, and Joanna Czapla-Masztafiak
Subjects: Genome instability, Absorption spectroscopy, DNA damage, Ultraviolet Rays, Biophysics, Radiation, 010402 general chemistry, 01 natural sciences, 03 medical and health sciences, chemistry.chemical_compound, 0302 clinical medicine, Radiation damage, Animals, Irradiation, X-ray absorption spectroscopy, Proteins, DNA, 0104 chemical sciences, X-Ray Absorption Spectroscopy, chemistry, Biochemistry, 030220 oncology & carcinogenesis, Cattle, Protons, DNA Damage
Abstract: The biological influence of radiation on living matter has been studied for years; however, several questions about the detailed mechanism of radiation damage formation remain largely unanswered. Among all biomolecules exposed to radiation, DNA plays an important role because any damage to its molecular structure can affect the whole cell and may lead to chromosomal rearrangements resulting in genomic instability or cell death. To identify and characterize damage induced in the DNA sugar-phosphate backbone, in this work we performed x-ray absorption spectroscopy at the P K-edge on DNA irradiated with either UVA light or protons. By combining the experimental results with theoretical calculations, we were able to establish the types and relative ratio of lesions produced by both UVA and protons around the phosphorus atoms in DNA.
Published: 2016
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47. Vibrational and condensed phase dynamics: general discussion

Author: R. J. Dwayne Miller, Junko Yano, Theo Keane, Lukas Miseikis, Hans Jakob Wörner, Peter M. Weber, Thomas J. Penfold, Oliver Schalk, Oleg Kornilov, Russell S. Minns, Oliver Gessner, Theis I. Sølling, Shaul Mukamel, Michael P. Minitti, Gareth Roberts, Kiyoshi Ueda, Wolfgang Domcke, Christopher J. Milne, Albert Stolow, Martin Centurion, Andrew J. Orr-Ewing, Vasilios G. Stavros, and Daniel M. Neumark
Subjects: Materials science, Phase dynamics, Chemical physics, Physical and Theoretical Chemistry
Published: 2016

48. Attosecond processes and X-ray spectroscopy: general discussion

Author: Daniel Rolles, Ágnes Vibók, Fernando Martín, Christopher J. Milne, Albert Stolow, Martin Centurion, Kiyoshi Ueda, Dave Townsend, Sebastian Mai, Adam Kirrander, Oliver Schalk, Shaul Mukamel, Morgane Vacher, Dane R. Austin, Misha Ivanov, Hans Jakob Wörner, Peter M. Weber, Jonathan P. Marangos, Victor Kimberg, Michael P. Minitti, Artem Rudenko, Jan Marcus Dahlström, R. J. Dwayne Miller, Zdenek Masin, Markus Kowalewski, Allan S. Johnson, Ruaridh Forbes, Alvaro Sanchez-Gonzalez, Nirit Dudovich, Danielle Dowek, Daniel M. Neumark, Filippo Bencivenga, Raluca Cireasa, Wolfgang Domcke, and Imperial College London
Subjects: X-ray spectroscopy, Materials science, Attosecond, [CHIM]Chemical Sciences, Physical and Theoretical Chemistry, Atomic physics, ComputingMilieux_MISCELLANEOUS
Abstract: International audience
Published: 2016

49. Optical second harmonic generation in LiB3O5 modulated by intense femtosecond X-ray pulses

Author: Gregor Knopp, Alex Oggenfuss, Philip J. M. Johnson, Claudio Cirelli, Christopher J. Milne, Xinhua Xie, C. Svetina, Serhane Zerdane, Roman Mankowsky, Yunpei Deng, Paul Beaud, Edwin Divall, Christopher Arrell, Steven L. Johnson, Henrik T. Lemke, and Christian Erny
Subjects: Materials science, business.industry, Physics::Optics, Second-harmonic generation, 02 engineering and technology, 021001 nanoscience & nanotechnology, Laser, 01 natural sciences, Atomic and Molecular Physics, and Optics, Pulse (physics), law.invention, 010309 optics, Wavelength, Optics, Modulation, law, 0103 physical sciences, Femtosecond, 0210 nano-technology, business, Ultrashort pulse, Jitter
Abstract: Many of the scientific applications for X-ray free-electron lasers seek to exploit the ultrashort pulse durations of intense X-rays to obtain femtosecond time resolution of various processes in a “pump-probe” scheme. One of the limiting factors for such experiments is the timing jitter between the X-rays and ultrashort pulses from more conventional lasers operating at near-optical wavelengths. In this work, we investigate the potential of using X-ray-induced changes in the optical second harmonic generation efficiency of a nonlinear crystal to retrieve single-shot arrival times of X-ray pulses with respect to optical laser pulses. Our experimental results and simulations show changes to the efficiency of the second harmonic generation of 12%, approximately three times larger than the measured changes in the transmission of the 800 nm center-wavelength fundamental pulse. Further experiments showing even larger changes in the transmission of 400 nm center-wavelength pulses show that the mechanism of the second harmonic generation efficiency modulation is mainly the result of X-ray-induced changes in the linear absorption coefficients near 400 nm. We demonstrate and characterize a cross-correlation tool based on this effect in reference to a previously demonstrated method of X-ray/optical cross-correlation.
Published: 2020

50. Temporal diagnostics from photons: the experience with the PALM

Author: Andreas Dax, Tsukasa Katayama, Pavle Juranić, Rasmus Ischebeck, Claude Pradervand, Luc Patthey, Christian Erny, Shigeki Owada, Henrik T. Lemke, Milan Radovic, I. Gorgisyan, Christopher J. Milne, Makina Yabashi, Christoph P. Hauri, and Tadashi Togashi
Subjects: Physics, SACLA, Photon, Optics, business.industry, Streak camera, Terahertz radiation, Instrumentation, Pulse duration, Laser pumping, Photonics, business
Abstract: The Photon Arrival and Length Monitor (PALM), a THz streak camera device developed by PSI for non-destructive hard x-ray measurements of photon pulse length and arrival time versus a pump laser[1], was brought to the SACLA XFEL[2] in Japan in a cross-calibration temporal diagnostics campaign after an initial experiment where only the PALM was being used[3]. The device was used with 9 keV pink beam and a 9.0 and 8.8 keV two-color mode, successfully measuring the temporal ifnromation of the pulses for several different FEL operating conditions. The most interesting achievement is the PALM’s ability to measure two arrival times of the two colorors as tey are shifted against each other by the FEL, opening up new possibilities in temporal accuracy for two-color experiments. SwissFEL will employ two such devices at the end stations for use by both operators and experimenters to improve the operation of the FEL and to better interpret experimental data. References [1]P. N. Juranic et. al, Journal of Instrumentation (2014) 9. [2]T. Ishikawa et. al., Nature Photonics (2012) 6(8). [3] P. N. Juranic et. al., Optics Express (2014) 22.
Published: 2018

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