Search

COSINE-100 is a direct dark matter search experiment, with the primary goal of testing the annual modulation signal observed by DAMA/LIBRA, using the same target material, NaI(Tl). In previous analyses, we achieved the same 1 keV energy threshold used in the DAMA/LIBRA's analysis that reported an annual modulation signal with 11.6$\sigma$ significance. In this article, we report an improved analysis that lowered the threshold to 0.7 keV, thanks to the application of Multi-Layer Perception network and a new likelihood parameter with waveforms in the frequency domain. The lower threshold would enable a better comparison of COSINE-100 with new DAMA results with a 0.75 keV threshold and account for differences in quenching factors. Furthermore the lower threshold can enhance COSINE-100's sensitivity to sub-GeV dark matter searches.

COSINE-100 aims to conclusively test the claimed dark matter annual modulation signal detected by DAMA/LIBRA collaboration. DAMA/LIBRA has released updated analysis results by lowering the energy threshold to 0.75 keV through various upgrades. They have consistently claimed to have observed the annual modulation. In COSINE-100, it is crucial to lower the energy threshold for a direct comparison with DAMA/LIBRA, which also enhances the sensitivity of the search for low-mass dark matter, enabling COSINE-100 to explore this area. Therefore, it is essential to have a precise and quantitative understanding of the background spectrum across all energy ranges. This study expands the background modeling from 0.7 to 4000 keV using 2.82 years of COSINE-100 data. The modeling has been improved to describe the background spectrum across all energy ranges accurately. Assessments of the background spectrum are presented, considering the nonproportionality of NaI(Tl) crystals at both low and high energies and the characteristic X-rays produced by the interaction of external backgrounds with materials such as copper. Additionally, constraints on the fit parameters obtained from the alpha spectrum modeling fit are integrated into this model. These improvements are detailed in the paper.

We report new results from the Neutrino Elastic Scattering Observation with NaI (NEON) experiment in the search for light dark matter (LDM) using 2,636 kg$\cdot$days of NaI(Tl) exposure. The experiment employs an array of NaI(Tl) crystals with a total mass of 16.7 kg, located 23.7 meters away from a 2.8 GW thermal power nuclear reactor. We investigated LDM produced by the $\textit{invisible decay}$ of dark photons generated by high-flux photons during reactor operation. The energy spectra collected during reactor-on and reactor-off periods were compared within the LDM signal region of $1-10$ keV. No signal consistent with LDM interaction with electrons was observed, allowing us to set 90% confidence level exclusion limits for the dark matter-electron scattering cross-section ($\sigma_e$) across dark matter masses ranging from 1 keV/c$^2$ to 1 MeV/c$^2$. Our results set a 90% confidence level upper limit of $\sigma_e = 3.17\times10^{-35}~\mathrm{cm^2}$ for a dark matter mass of 100 keV/c$^2$, marking the best laboratory result in this mass range. Additionally, our search extends the coverage of LDM below 100 keV/c$^2$ first time.

The Neutrino Elastic-scattering Observation with NaI(Tl) experiment (NEON) aims to detect coherent elastic neutrino-nucleus scattering~(\cenns) in a NaI(Tl) crystal using reactor anti-electron neutrinos at the Hanbit nuclear power plant complex. A total of 13.3 kg of NaI(Tl) crystals were initially installed in December 2020 at the tendon gallery, 23.7$\pm$0.3\,m away from the reactor core, which operates at a thermal power of 2.8\,GW. Initial engineering operation was performed from May 2021 to March 2022 and observed unexpected photomultiplier-induced noise and a decreased light yield that were caused by leakage of liquid scintillator into the detector due to weakness of detector encapsulation. We upgraded the detector encapsulation design to prevent the leakage of the liquid scintillator. Meanwhile two small-sized detectors were replaced with larger ones resulting in a total mass of 16.7\,kg. With this new design implementation, the detector system has been operating stably since April 2022 for over a year without detector gain drop. In this paper, we present an improved crystal encapsulation design and stability of the NEON experiment.

The lowering of the energy threshold in the NaI detector is crucial not only for comprehensive validation of DAMA/LIBRA but also for exploring new possibilities in the search for low-mass dark matter and observing coherent elastic scattering between neutrino and nucleus. Alongside hardware enhancements, extensive efforts have focused on refining event selection to discern noise, achieved through parameter development and the application of machine learning. Acquiring pure, unbiased datasets is crucial in this endeavor, for which a waveform simulation was developed. The simulation data were compared with the experimental data using several pulse shape discrimination parameters to test its performance in describing the experimental data. Additionally, we present the outcomes of multi-variable machine learning trained with simulation data as a scintillation signal sample. The distributions of outcomes for experimental and simulation data show a good agreement. As an application of the waveform simulation, we validate the trigger efficiency alongside estimations derived from the minimally biased measurement data.

We present a comprehensive study of the nonproportionality of NaI(Tl) scintillation detectors within the context of dark matter search experiments. Our investigation, which integrates COSINE-100 data with supplementary $\gamma$ spectroscopy, measures light yields across diverse energy levels from full-energy $\gamma$ peaks produced by the decays of various isotopes. These $\gamma$ peaks of interest were produced by decays supported by both long and short-lived isotopes. Analyzing peaks from decays supported only by short-lived isotopes presented a unique challenge due to their limited statistics and overlapping energies, which was overcome by long-term data collection and a time-dependent analysis. A key achievement is the direct measurement of the 0.87 keV light yield, resulting from the cascade following electron capture decay of $^{22}$Na from internal contamination. This measurement, previously accessible only indirectly, deepens our understanding of NaI(Tl) scintillator behavior in the region of interest for dark matter searches. This study holds substantial implications for background modeling and the interpretation of dark matter signals in NaI(Tl) experiments., Comment: 12 pages, 7 figures

COSINE-100 is a dark matter direct detection experiment with 106 kg NaI(Tl) as the target material. 210Pb and daughter isotopes are a dominant background in the WIMP region of interest and are detected via beta decay and alpha decay. Analysis of the alpha channel complements the background model as observed in the beta/gamma channel. We present the measurement of the quenching factors and Monte Carlo simulation results and activity quantification of the alpha decay components of the COSINE-100 NaI(Tl) crystals. The data strongly indicate that the alpha decays probabilistically undergo two possible quenching factors but require further investigation. The fitted results are consistent with independent measurements and improve the overall understanding of the COSINE-100 backgrounds. Furthermore, the half-life of 216Po has been measured to be 143.4 +/- 1.2 ms, which is consistent with and more precise than recent measurements.

We report the results of a search for inelastic scattering of weakly interacting massive particles (WIMPs) off $^{127}$I nuclei using NaI(Tl) crystals with a data exposure of 97.7 kg$\cdot$years from the COSINE-100 experiment. The signature of inelastic WIMP-$^{127}$I scattering is a nuclear recoil accompanied by a 57.6 keV $\gamma$-ray from the prompt deexcitation, producing a more energetic signal compared to the typical WIMP nuclear recoil signal. We found no evidence for this inelastic scattering signature and set a 90 $\%$ confidence level upper limit on the WIMP-proton spin-dependent, inelastic scattering cross section of $1.2 \times 10^{-37} {\rm cm^{2}}$ at the WIMP mass 500 ${\rm GeV/c^{2}}$., Comment: 8 pages, 5 figures. arXiv admin note: text overlap with arXiv:2104.03537

Using muon spin relaxation ($\mu$SR) measurements on formamidinium lead iodide [FAPbI$_3$, where FA denotes HC(NH$_2)_2$] we show that, among the five structurally distinct phases of FAPbI$_3$ exhibited through two different temperature hysteresis, the reorientation motion of FA molecules is quasi-static below $\approx50$ K over the time scale of 10$^{-6}$ s in the low-temperature (LT) hexagonal (Hex-LT, $<160$ K) phase which has relatively longer photo-excited charge carrier lifetime ($\tau_{\rm c}\sim$10$^{-6}$ s). In contrast, a sharp increase in the FA molecular motion was found above $\approx50$ K in the Hex-LT phase, LT-tetragonal phase (Tet-LT, $<140$ K), the high-temperature (HT) hexagonal phase (Hex-HT, 160-380 K), and the HT-tetragonal phase (Tet-HT, 140-280 K) where $\tau_{\rm c}$ decreases with increasing temperature. More interestingly, the reorientation motion is further promoted in the cubic phase at higher temperatures ($>380/280$ K), while $\tau_{\rm c}$ is recovered to comparable or larger than that of the LT phases. These results indicate that there are two factors that determine $\tau_{\rm c}$, one related to the local reorientation of cationic molecules that is not unencumbered by phonons, and the other to the high symmetry of the bulk crystal structure., Comment: 7 pages, 4 figures

We search for energetic electron recoil signals induced by boosted dark matter (BDM) from the galactic center using the COSINE-100 array of NaI(Tl) crystal detectors at the Yangyang Underground Laboratory. The signal would be an excess of events with energies above 4 MeV over the well-understood background. Because no excess of events are observed in a 97.7 kg$\cdot$years exposure, we set limits on BDM interactions under a variety of hypotheses. Notably, we explored the dark photon parameter space, leading to competitive limits compared to direct dark photon search experiments, particularly for dark photon masses below 4\,MeV and considering the invisible decay mode. Furthermore, by comparing our results with a previous BDM search conducted by the Super-Kamionkande experiment, we found that the COSINE-100 detector has advantages in searching for low-mass dark matter. This analysis demonstrates the potential of the COSINE-100 detector to search for MeV electron recoil signals produced by the dark sector particle interactions., Comment: 7 pages, 4 figures

We present results of a search for bosonic super-weakly interacting massive particles (BSW) as keV scale dark matter candidates that is based on an exposure of 97.7 kg$\cdot$year from the COSINE experiment. In this search, we employ, for the first time, Compton-like as well as absorption processes for pseudoscalar and vector BSWs. No evidence for BSWs is found in the mass range from 10 $\mathrm{keV/c}^2$ to 1 $\mathrm{MeV/c}^2$, and we present the exclusion limits on the dimensionless coupling constants to electrons $g_{ae}$ for pseudoscalar and $\kappa$ for vector BSWs at 90% confidence level. Our results show that these limits are improved by including the Compton-like process in masses of BSW, above $\mathcal{O}(100\,\mathrm{keV/c}^2)$.

We present results from a search for solar bosonic dark matter using the annual modulation method with the COSINE-100 experiment. The results were interpreted considering three dark sector bosons models: solar dark photon; DFSZ and KSVZ solar axion; and Kaluza-Klein solar axion. No modulation signal that is compatible with the expected from the models was found from a data-set of 2.82 yr, using 61.3 kg of NaI(Tl) crystals. Therefore, we set a 90$\%$ confidence level upper limits for each of the three models studied. For the solar dark photon model, the most stringent mixing parameter upper limit is $1.61 \times 10^{-14}$ for dark photons with a mass of 215 eV. For the DFSZ and KSVZ solar axion, and the Kaluza-Klein axion models, the upper limits exclude axion-electron couplings, $g_{ae}$, above $1.61 \times 10^{-11}$ for axion mass below 0.2 keV; and axion-photon couplings, $g_{a\gamma\gamma}$, above $1.83 \times 10^{-11}$ GeV$^{-1}$ for an axion number density of $4.07 \times 10^{13}$ cm$^{-3}$. This is the first experimental search for solar dark photons and DFSZ and KSVZ solar axions using the annual modulation method. The lower background, higher light yield and reduced threshold of NaI(Tl) crystals of the future COSINE-200 experiment are expected to enhance the sensitivity of the analysis shown in this paper. We show the sensitivities for the three models studied, considering the same search method with COSINE-200., Comment: 13 pages, 16 figures

The DAMA/LIBRA collaboration has reported the observation of an annual modulation in the event rate that has been attributed to dark matter interactions over the last two decades. However, even though tremendous efforts to detect similar dark matter interactions were pursued, no definitive evidence has been observed to corroborate the DAMA/LIBRA signal. Many studies assuming various dark matter models have attempted to reconcile DAMA/LIBRA's modulation signals and null results from other experiments, however no clear conclusion can be drawn. Apart from the dark matter hypothesis, several studies have examined the possibility that the modulation is induced by variations in their detector's environment or their specific analysis methods. In particular, a recent study presents a possible cause of the annual modulation from an analysis method adopted by the DAMA/LIBRA experiment in which the observed annual modulation could be reproduced by a slowly varying time-dependent background. Here, we study the COSINE-100 data using an analysis method similar to the one adopted by the DAMA/LIBRA experiment and observe a significant annual modulation, although the modulation phase is almost opposite to that of the DAMA/LIBRA data. Assuming the same background composition for COSINE-100 and DAMA/LIBRA, simulated experiments for the DAMA/LIBRA without dark matter signals also provide significant annual modulation with an amplitude similar to DAMA/LIBRA with opposite phase. Even though this observation does not explain the DAMA/LIBRA's results directly, this interesting phenomenon motivates deeper studies of the time-dependent DAMA/LIBRA background data.

Neutrino elastic scattering observation with NaI (NEON) is an experiment designed to detect neutrino-nucleus coherent scattering using reactor electron antineutrinos. NEON is based on an array of six NaI(Tl) crystals with a total mass of 13.3 kg, located at the tendon gallery that is 23.7 m away from a reactor core with a thermal power of 2.8 GW in the Hanbit nuclear power complex. The installation of the NEON detector was completed in December 2020, and since May 2021, the detector has acquired data at full reactor power. Based on the observed light yields of the NaI crystals of approximately 22, number of photoelectrons per unit keV electron-equivalent energy (keVee), and 6 counts/kg/keV/day background level at 2-6 keVee energy, coherent elastic neutrino-nucleus scattering observation sensitivity is evaluated as more than 3$\sigma$ assuming one-year reactor-on and 100 days reactor-off data, 0.2 keVee energy threshold, and 7 counts/keV/kg/day background in the signal region of 0.2-0.5 keVee. This paper describes the design of the NEON detector, including the shielding arrangement, configuration of NaI(Tl) crystals, and associated operating systems. The initial performance and associated sensitivity of the experiment are also presented., Comment: 21 pages 27 figures

The long charge carrier lifetime of the hybrid organic-inorganic perovskites (HOIPs) is the key for their remarkable performance as a solar cell material. The microscopic mechanism for the long lifetime is still in debate. Here, by using muon spin relaxation technique that probes the fluctuation of local magnetic fields, we show that the muon depolarization rate ($\Delta$) of a prototype HOIP methylammonium lead iodide (MAPbI$_3$) shows a sharp decrease with increasing temperature in two steps above 120 K and 190 K across the structural transition from orthorhombic to tetragonal structure at 162 K. Our analysis shows that the reduction of $\Delta$ is quantitatively in agreement with the expected behavior due to the rapid development of MA jumping rotation around the $C_3$ and $C_4$ symmetry axes. Our results provide direct evidence for the intimate relation between the rotation of the electric dipoles of MA molecules and the charge carrier lifetime in HOIPs., Comment: 7 pages, 4 figures

COSINE-100 is a direct detection dark matter experiment that aims to test DAMA/LIBRA's claim of dark matter discovery by searching for a dark matter-induced annual modulation signal with NaI(Tl) detectors. We present new constraints on the annual modulation signal from a dataset with a 2.82 yr livetime utilizing an active mass of 61.3 kg, for a total exposure of 173 kg$\cdot$yr. This new result features an improved event selection that allows for both lowering the energy threshold to 1 keV and a more precise time-dependent background model. In the 1-6 keV and 2-6 keV energy intervals, we observe best-fit values for the modulation amplitude of 0.0067$\pm$0.0042 and 0.0051$\pm$0.0047 counts/(day$\cdot$kg$\cdot$keV), respectively, with a phase fixed at 152.5 days., Comment: 11 pages, 8 figures

We report on the search for weakly interacting massive particle (WIMP) dark matter candidates in the galactic halo that interact with sodium and iodine nuclei in the COSINE-100 experiment and produce energetic electrons that accompany recoil nuclei via the the Migdal effect. The WIMP mass sensitivity of previous COSINE-100 searches that relied on the detection of ionization signals produced by target nuclei recoiling from elastic WIMP-nucleus scattering was restricted to WIMP masses above $\sim$5 GeV/$c^2$ by the detectors' 1 keVee energy-electron-equivalent threshold. The search reported here looks for recoil signals enhanced by the Migdal electrons that are ejected during the scattering process. This is particularly effective for the detection of low-mass WIMP scattering from the crystals' sodium nuclei in which a relatively larger fraction of the WIMP's energy is transferred to the nucleus recoil energy and the excitation of its orbital electrons. In this analysis, the low-mass WIMP search window of the COSINE-100 experiment is extended to WIMP mass down to 200 MeV/$c^2$. The low-mass WIMP sensitivity will be further improved by lowering the analysis threshold based on a multivariable analysis technique. We consider the influence of these improvements and recent developments in detector performance to re-evaluate sensitivities for the future COSINE-200 experiment. With a 0.2 keVee analysis threshold and high light-yield NaI(Tl) detectors (22 photoelectrons/keVee), the COSINE-200 experiment can explore low-mass WIMPs down to 20 MeV/$c^2$ and probe previously unexplored regions of parameter space., Comment: 10 pages, 8 figures

The COSINE-100 experiment is designed to test the DAMA experiment which claimed an observation of a dark matter signal from an annual modulation in their residual event rate. To measure the 1 %-level signal amplitude, it is crucial to control and monitor nearly all environmental quantities that might systematically mimic the signal. The environmental monitoring also helps ensure a stable operation of the experiment. Here, we describe the design and performance of the centralized environmental monitoring system for the COSINE-100 experiment., Comment: 13 pages, 11 figures

We present new constraints on dark matter interactions using 1.7 years of COSINE-100 data. The COSINE-100 experiment, consisting of 106 kg of tallium-doped sodium iodide (NaI(Tl)) target material, is aimed at testing DAMA's claim of dark matter observation using the same NaI(Tl) detectors. Improved event selection requirements, a more precise understanding of the detector background and the use of a larger data set considerably enhances the COSINE-100 sensitivity for dark matter detection. No signal consistent with the dark matter interaction is identified, and rules out model-dependent dark matter interpretations of the DAMA signals in the specific context of standard halo model with the same NaI(Tl) target for various interaction hypotheses.

We report the identification of metastable isomeric states of $^{228}$Ac at 6.28 keV, 6.67 keV and 20.19 keV, with lifetimes of an order of 100 ns. These states are produced by the $\beta$-decay of $^{228}$Ra, a component of the $^{232}$Th decay chain, with $\beta$ Q-values of 39.52 keV, 39.13 keV and 25.61 keV, respectively. Due to its low Q-value as well as the relative abundance of $^{232}$Th and their progeny in low background experiments, these observations potentially impact the low-energy background modeling of dark matter search experiments., Comment: 9 pages, 9 figures

We present a background model for dark matter searches using an array of NaI(Tl) crystals in the COSINE-100 experiment that is located in the Yangyang underground laboratory. The model includes background contributions from both internal and external sources, including cosmogenic radionuclides and surface $^{210}$Pb contamination. To build the model in the low energy region, with a threshold of 1 keV, we used a depth profile of $^{210}$Pb contamination in the surface of the NaI(Tl) crystals determined in a comparison between measured and simulated spectra. We also considered the effect of the energy scale errors propagated from the statistical uncertainties and the nonlinear detector response at low energies. The 1.7 years COSINE-100 data taken between October 21, 2016 and July 18, 2018 were used for this analysis. Our Monte Carlo simulation provides a non-Gaussian peak around 50 keV originating from beta decays of bulk $^{210}$Pb in a good agreement with the measured background. This model estimates that the activities of bulk $^{210}$Pb and $^{3}$H are dominating the background rate that amounts to an average level of 2.85$\pm$0.15 counts/day/keV/kg in the energy region of (1-6) keV, using COSINE-100 data with a total exposure of 97.7 kg$\cdot$years.

For the GBAR (Gravitational Behaviour of Antihydrogen at Rest) experiment at CERN's Antiproton Decelerator (AD) facility we have constructed a source of slow positrons, which uses a low-energy electron linear accelerator (linac). The driver linac produces electrons of 9 MeV kinetic energy that create positrons from bremsstrahlung-induced pair production. Staying below 10 MeV ensures no persistent radioactive activation in the target zone and that the radiation level outside the biological shield is safe for public access. An annealed tungsten-mesh assembly placed directly behind the target acts as a positron moderator. The system produces $5\times10^7$ slow positrons per second, a performance demonstrating that a low-energy electron linac is a superior choice over positron-emitting radioactive sources for high positron flux., Comment: published in NIM A. 33 pages 9 figures

NaI(Tl) crystals are used as particle detectors in a variety of rare-event search experiments because of their superb light-emission quality. The crystal light yield is generally high, above 10 photoelectrons per keV, and its emission spectrum is peaked around 400 nm, which matches well to the sensitive region of bialkali photocathode photomultiplier tubes. However, since NaI(Tl) crystals are hygroscopic, a sophisticated method of encapsulation has to be applied that prevents moisture from chemically attacking the crystal and thereby degrading the emission. In addition, operation with low energy thresholds, which is essential for a number of new phenomenon searches, is usually limited by the crystal light yield; in these cases higher light yields can translate into lower thresholds that improve the experimental sensitivity. Here we describe the development of an encapsulation technique that simplifies the overall design by attaching the photo sensors directly to the crystal so that light losses are minimized. The light yield of a NaI(Tl) crystal encapsulated with this technique was improved by more than 30%, and as many as 22 photoelectrons per keV have been measured. Consequently, the energy threshold can be lowered and the energy resolution improved. Detectors with this higher light yield are sensitive to events with sub-keV energies and well suited for low-mass dark matter particle searches and measurements of neutrino-nucleus coherent scattering., Comment: 15 pages, 7 figures (minor edits)

COSINE-100 is a dark matter detection experiment that uses NaI(Tl) crystal detectors operating at the Yangyang underground laboratory in Korea since September 2016. Its main goal is to test the annual modulation observed by the DAMA/LIBRA experiment with the same target medium. Recently DAMA/LIBRA has released data with an energy threshold lowered to 1 keV, and the persistent annual modulation behavior is still observed at 9.5$\sigma$. By lowering the energy threshold for electron recoils to 1 keV, COSINE-100 annual modulation results can be compared to those of DAMA/LIBRA in a model-independent way. Additionally, the event selection methods provide an access to a few to sub-GeV dark matter particles using constant rate studies. In this article, we discuss the COSINE-100 event selection algorithm, its validation, and efficiencies near the threshold.

We report measurements of annual and diurnal modulations of the cosmic-ray muon rate in the Yangyang underground laboratory (Y2L) using 952 days of COSINE-100 data acquired between September 2016 and July 2019. A correlation of the muon rate with the atmospheric temperature is observed and its amplitude on the muon rate is determined. The effective atmospheric temperature and muon rate variations are positively correlated with a measured effective temperature coefficient of $\alpha_{T}$ = 0.80 $\pm$ 0.11. This result is consistent with a model of meson production in the atmosphere. We also searched for a diurnal modulation in the underground muon rate by comparing one-hour intervals. No significant diurnal modulation of the muon rate was observed., Comment: 12 pages, 9 figures

This paper describes the liquid scintillator veto system for the COSINE-100 dark matter experiment and its performance. The COSINE-100 detector consists of eight NaI(Tl) crystals immersed in 2200~L of linear alkylbenzene-based liquid scintillator. The liquid scintillator tags between 65 and 75\% of the internal $^{40}$K background in the 2--6 keV energy region. We also describe the background model for the liquid scintillator, which is primarily used to assess its energy calibration and threshold.

There is a long standing debate about whether or not the annual modulation signal reported by the DAMA/LIBRA collaboration is induced by Weakly Interacting Massive Particles~(WIMP) in the galaxy's dark matter halo scattering from nuclides in their NaI(Tl) crystal target/detector. This is because regions of WIMP-mass vs. WIMP-nucleon cross-section parameter space that can accommodate the DAMA/LIBRA-phase1 modulation signal in the context of the standard WIMP dark matter galactic halo and isospin-conserving~(canonical), spin-independent~(SI) WIMP-nucleon interactions have been excluded by many of other dark matter search experiments including COSINE-100, which uses the same NaI(Tl) target/detector material. Moreover, the recently released DAMA/LIBRA-phase2 results are inconsistent with an interpretation as WIMP-nuclide scattering via the canonical SI interaction and prefer, instead, isospin-violating or spin-dependent interactions. Dark matter interpretations of the DAMA/LIBRA signal are sensitive to the NaI(Tl) scintillation efficiency for nuclear recoils, which is characterized by so-called quenching factors~(QF), and the QF values used in previous studies differ significantly from recently reported measurements, which may have led to incorrect interpretations of the DAMA/LIBRA signal. In this article, the compatibility of the DAMA/LIBRA and COSINE-100 results, in light of the new QF measurements is examined for different possible types of WIMP-nucleon interactions. The resulting allowed parameter space regions associated with the DAMA/LIBRA signal are explicitly compared with 90\% confidence level upper limits from the initial 59.5~day COSINE-100 exposure. With the newly measured QF values, the allowed 3$\sigma$ regions from the DAMA/LIBRA data are still generally excluded by the COSINE-100 data., Comment: Accepted in JCAP

COSINE-100 is a direct detection dark matter search experiment that uses a 106 kg array of eight NaI(Tl) crystals that are kept underground at the Yangyang Underground Laboratory to avoid cosmogenic activation of radioisotopes by cosmic rays. Even though the cosmogenic activity is declining with time, there are still significant background rates from the remnant nuclides. In this paper, we report measurements of cosmogenic isotope contaminations with less than one year half-lives that are based on extrapolations of the time dependent activities of their characteristic energy peaks to activity rates at the time the crystals were deployed underground. For longer-lived $^{109}$Cd ($T_{1/2}=1.6$ y) and $^{22}$Na ($T_{1/2}=2.6$ y), we investigate time correlations of characteristic $\gamma$/X-ray peaks. The inferred sea-level production rates are compared with caluclations based on the ACTIVIA and MENDL-2 model calculations and experimental data. For $^{3}$H, which has a long, 12.3 year half-life, we evaluated the activity levels from the exposure times and determined a cosmogenic activation rate that is consistent with other measurements.

Methylammonium lead iodide (CH3NH3PbI3) based solar cells have shown impressive power conversion efficiencies of above 20%. However, the microscopic mechanism of the high photovoltaic performance is yet to be fully understood. Particularly, the dynamics of CH3NH3+ cations and their impact on relevant processes such as charge recombination and exciton dissociation are still poorly understood. Here, using elastic and quasi-elastic neutron scattering techniques and group theoretical analysis, we studied rotational modes of the CH3NH3+ cation in CH3NH3PbI3. Our results show that, in the cubic (T > 327K) and tetragonal (165K < T < 327K) phases, the CH3NH3+ ions exhibit four-fold rotational symmetry of the C-N axis (C4) along with three-fold rotation around the C-N axis (C3), while in orthorhombic phase (T < 165K) only C3 rotation is present. Around room temperature, the characteristic relaxation times for the C4 rotation is found to be ps while for the C3 rotation ps. The -dependent rotational relaxation times were fitted with Arrhenius equations to obtain activation energies. Our data show a close correlation between the C4 rotational mode and the temperature dependent dielectric permittivity. Our findings on the rotational dynamics of CH3NH3+ and the associated dipole have important implications on understanding the low exciton binding energy and slow charge recombination rate in CH3NH3PbI3 which are directly relevant for the high solar cell performance.