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Efficient synthesis recipes are needed both to streamline the manufacturing of complex materials and to accelerate the realization of theoretically predicted materials. Oftentimes the solid-state synthesis of multicomponent oxides is impeded by undesired byproduct phases, which can kinetically trap reactions in an incomplete non-equilibrium state. We present a thermodynamic strategy to navigate high-dimensional phase diagrams in search of precursors that circumvent low-energy competing byproducts, while maximizing the reaction energy to drive fast phase transformation kinetics. Using a robotic inorganic materials synthesis laboratory, we perform a large-scale experimental validation of our precursor selection principles. For a set of 35 target quaternary oxides with chemistries representative of intercalation battery cathodes and solid-state electrolytes, we perform 224 reactions spanning 27 elements with 28 unique precursors. Our predicted precursors frequently yield target materials with higher phase purity than when starting from traditional precursors. Robotic laboratories offer an exciting new platform for data-driven experimental science, from which we can develop new insights into materials synthesis for both robot and human chemists.

A brain-computer interface (BCI) based on electroencephalography (EEG) can be useful for rehabilitation and the control of external devices. Five grasping tasks were decoded for motor execution (ME) and motor imagery (MI). During this experiment, eight healthy subjects were asked to imagine and grasp five objects. Analysis of EEG signals was performed after detecting muscle signals on electromyograms (EMG) with a time interval selection technique on data taken from these ME and MI experiments. By refining only data corresponding to the exact time when the users performed the motor intention, the proposed method can train the decoding model using only the EEG data generated by various motor intentions with strong correlation with a specific class. There was an accuracy of 70.73% for ME and 47.95% for MI for the five offline tasks. This method may be applied to future applications, such as controlling robot hands with BCIs., Comment: Submitted to 2023 11th IEEE International Winter Conference on Brain-Computer Interface

Brain-computer interface (BCI) uses brain signals to communicate with external devices without actual control. Particularly, BCI is one of the interfaces for controlling the robotic arm. In this study, we propose a knowledge distillation-based framework to manipulate robotic arm through hybrid paradigm induced EEG signals for practical use. The teacher model is designed to decode input data hierarchically and transfer knowledge to student model. To this end, soft labels and distillation loss functions are applied to the student model training. According to experimental results, student model achieved the best performance among the singular architecture-based methods. It is confirmed that using hierarchical models and knowledge distillation, the performance of a simple architecture can be improved. Since it is uncertain what knowledge is transferred, it is important to clarify this part in future studies.

Data augmentation approaches are widely explored for the enhancement of decoding electroencephalogram signals. In subject-independent brain-computer interface system, domain adaption and generalization are utilized to shift source subjects' data distribution to match the target subject as an augmentation. However, previous works either introduce noises (e.g., by noise addition or generation with random noises) or modify target data, thus, cannot well depict the target data distribution and hinder further analysis. In this paper, we propose a target-centered subject transfer framework as a data augmentation approach. A subset of source data is first constructed to maximize the source-target relevance. Then, the generative model is applied to transfer the data to target domain. The proposed framework enriches the explainability of target domain by adding extra real data, instead of noises. It shows superior performance compared with other data augmentation methods. Extensive experiments are conducted to verify the effectiveness and robustness of our approach as a prosperous tool for further research.

An electroencephalogram is an effective approach that provides a bidirectional pathway between the user and computer in a non-invasive way. In this study, we adopted the visual imagery data for controlling the BCI-based robotic arm. Visual imagery increases the power of the alpha frequency range of the visual cortex over time as the user performs the task. We proposed a deep learning architecture to decode the visual imagery data using only two channels and also we investigated the combination of two EEG channels that has significant classification performance. When using the proposed method, the highest classification performance using two channels in the offline experiment was 0.661. Also, the highest success rate in the online experiment using two channels (AF3-Oz) was 0.78. Our results provide the possibility of controlling the BCI-based robotic arm using visual imagery data., Comment: 4 pages, 2 figures, 3 tables

Recently, advanced technologies have unlimited potential in solving various problems with a large amount of data. However, these technologies have yet to show competitive performance in brain-computer interfaces (BCIs) which deal with brain signals. Basically, brain signals are difficult to collect in large quantities, in particular, the amount of information would be sparse in spontaneous BCIs. In addition, we conjecture that high spatial and temporal similarities between tasks increase the prediction difficulty. We define this problem as sparse condition. To solve this, a factorization approach is introduced to allow the model to obtain distinct representations from latent space. To this end, we propose two feature extractors: A class-common module is trained through adversarial learning acting as a generator; Class-specific module utilizes loss function generated from classification so that features are extracted with traditional methods. To minimize the latent space shared by the class-common and class-specific features, the model is trained under orthogonal constraint. As a result, EEG signals are factorized into two separate latent spaces. Evaluations were conducted on a single-arm motor imagery dataset. From the results, we demonstrated that factorizing the EEG signal allows the model to extract rich and decisive features under sparse condition., Comment: 8 pages

Brain-computer interface (BCI) is a practical pathway to interpret users' intentions by decoding motor execution (ME) or motor imagery (MI) from electroencephalogram (EEG) signals. However, developing a BCI system driven by ME or MI is challenging, particularly in the case of containing continual and compound muscles movements. This study analyzes three grasping actions from EEG under both ME and MI paradigms. We also investigate the classification performance in offline and pseudo-online experiments. We propose a novel approach that uses muscle activity pattern (MAP) images for the convolutional neural network (CNN) to improve classification accuracy. We record the EEG and electromyogram (EMG) signals simultaneously and create the MAP images by decoding both signals to estimate specific hand grasping. As a result, we obtained an average classification accuracy of 63.6($\pm$6.7)% in ME and 45.8($\pm$4.4)% in MI across all fifteen subjects for four classes. Also, we performed pseudo-online experiments and obtained classification accuracies of 60.5($\pm$8.4)% in ME and 42.7($\pm$6.8)% in MI. The proposed method MAP-CNN, shows stable classification performance, even in the pseudo-online experiment. We expect that MAP-CNN could be used in various BCI applications in the future., Comment: Submitted to 2022 10th IEEE International Winter Conference on Brain-Computer Interface

Touch is the first sense among human senses. Not only that, but it is also one of the most important senses that are indispensable. However, compared to sight and hearing, it is often neglected. In particular, since humans use the tactile sense of the skin to recognize and manipulate objects, without tactile sensation, it is very difficult to recognize or skillfully manipulate objects. In addition, the importance and interest of haptic technology related to touch are increasing with the development of technologies such as VR and AR in recent years. So far, the focus is only on haptic technology based on mechanical devices. Especially, there are not many studies on tactile sensation in the field of brain-computer interface based on EEG. There have been some studies that measured the surface roughness of artificial structures in relation to EEG-based tactile sensation. However, most studies have used passive contact methods in which the object moves, while the human subject remains still. Additionally, there have been no EEG-based tactile studies of active skin touch. In reality, we directly move our hands to feel the sense of touch. Therefore, as a preliminary study for our future research, we collected EEG signals for tactile sensation upon skin touch based on active touch and compared and analyzed differences in brain changes during touch and movement tasks. Through time-frequency analysis and statistical analysis, significant differences in power changes in alpha, beta, gamma, and high-gamma regions were observed. In addition, major spatial differences were observed in the sensory-motor region of the brain., Comment: Submitted to 2022 10th IEEE International Winter Conference on Brain-Computer Interface

Brain-computer interface uses brain signals to communicate with external devices without actual control. Many studies have been conducted to classify motor imagery based on machine learning. However, classifying imagery data with sparse spatial characteristics, such as single-arm motor imagery, remains a challenge. In this paper, we proposed a method to factorize EEG signals into two groups to classify motor imagery even if spatial features are sparse. Based on adversarial learning, we focused on extracting common features of EEG signals which are robust to noise and extracting only signal features. In addition, class-specific features were extracted which are specialized for class classification. Finally, the proposed method classifies the classes by representing the features of the two groups as one embedding space. Through experiments, we confirmed the feasibility that extracting features into two groups is advantageous for datasets that contain sparse spatial features., Comment: 4 pages

An electroencephalogram is an effective approach that provides a bidirectional pathway between user and computer in a non-invasive way. In this study, we adopted the visual perception data for training the visual imagery decoding network. We proposed a visual perception-guided network training approach for decoding visual imagery. Visual perception decreases the power of the alpha frequency range of the visual cortex over time when the user performed the task, and visual imagery increases the power of the alpha frequency range of the visual cortex over time as the user performed with the task. Generated brain signals when the user performing visual imagery and visual perception have opposite brain activity tendencies, and we used these characteristics to design the proposed network. When using the proposed method, the average classification performance of visual imagery with the visual perception data was 0.7008. Our results provide the possibility of using the visual perception data as a guide of the visual imagery classification network training., Comment: 4 pages, 2 figures, 3 tables