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We present the Ultracool Dwarf Companion Catalogue of 278 multiple systems, 32 of which are newly discovered, each with at least one spectroscopically confirmed Ultracool Dwarf, within a 100 pc volume-limited sample. This catalogue is compiled using the Gaia Catalogue of Nearby Stars for stellar primaries and the Gaia Ultracool Dwarf Sample for low-mass companions and includes 241 doubles, 33 triples, and 4 higher-order systems established from positional, proper motion, and parallax constraints. The catalogue seeks to identify probable benchmark systems within 100 pc to obtain model-independent astrophysical parameters of Ultracool Dwarfs. Chance alignment probabilities are calculated to evaluate the physical nature of each system. Astrometric and photometric data from Gaia Data Release 3 and the Two Micron All Sky Survey are included for all objects. We identify potential unseen companions using a combination of the Renormalised Unit Weight Error, Image Parameter Determination statistics, Non-Single Star solutions, and photometric blending as provided by Gaia, identifying hierarchical Ultracool triple systems. Our catalogue includes 17 White Dwarf - Ultracool Dwarf systems, whose ages are determined using cooling models. We also use the Gaia FLAME results and the BANYAN $\Sigma$ procedures to age 40 and 34 systems respectively, and derive mass estimates from evolutionary models., Comment: 26 pages, 8 figures