Search

Direct optical detection and imaging of single nanoparticles on substrate in wide field underpin vast applications across different research fields. However, the speckles originating from the unavoidable random surface undulations of the substrate ultimately limit the size of the decipherable nanoparticles by the current optical techniques, including the ultrasensitive interferometric scattering microscopy (iSCAT). Here we report a defocus-integration iSCAT to suppress the speckle noise and to enhance the detection and imaging of single nanoparticles on ultra-flat glass substrate and silicon wafer. In particular, we discover distinct symmetry properties of the scattering phase between the nanoparticle and the surface undulations that cause the speckles. Consequently, we develop the defocus-integration technique to suppress the speckles.We experimentally achieve an enhancement of the signal to noise ratio by 6.9 dB for the nanoparticle detection. We demonstrate that the technique is generally applicable for nanoparticles of various materials and for both low and high refractive-index substrates., Comment: 5 pages, 4 figures

In this study, we conducted a detailed analysis of the core parameter of Warm Higgs Inflation (WHI) $-$ the dissipation coefficient ($Q$). As a crucial parameter in the warm inflation process, $Q$ exerts profound influences on the entire evolutionary process. By meticulously deriving the relationships between various quantities and $Q$, we successfully circumvented the common preconceptions regarding strong and weak dissipation, laying the foundation for a more accurate exploration of their interconnections. Taking into account the constraints imposed by Cosmic Microwave Background, we observed that the dissipation coefficient $Q$ remains at extremely low levels throughout the entire warm inflation process, i.e., $Q \ll 1$. This observation indicates that WHI falls under the category of weakly dissipative warm inflation. Despite being weakly dissipative, $Q$ still plays a crucial role in the evolution of temperature, energy, and other quantities, highlighting its significance and non-negligibility. We delved deeper into the impact of the primordial power spectrum on the dissipation coefficient $Q$ during the warm inflation process, discovering that the dependency is not significant. Consequently, this naturally leads to the unobtrusive dependence of the gravitational wave power spectrum on $Q$. Finally, we found that gravitational waves generated by WHI hold the potential for verification in future observational experiments, especially through the SKA100 experiment. These findings provide a theoretical support for a more profound understanding of the early evolution of the universe., Comment: 16 pages, 5 figures

We report the construction of a passive, deterministic and near-unity-fidelity controlled-$\pi$-phase gate for single-photon wavepackets with a node comprising a two-level emitter and a small number of cavities. The proposed gate is rooted in the concept of time-reversal symmetric photon transport, which makes the entire photon transport process into a perfect absorption and re-emission process. Consequently, it can circumvent the longstanding issue of wavepacket distortion inherent in photonic phase gates employing nonlinear media. Moreover, such time-reversal symmetric transport ensures the nonlinear $\pi$ phase shift by a single two-level emitter for the two-photon case. We develop analytical solutions to reveal the temporal dynamics of the nonlinear photon transport and to optimize the gate structure. Notably, the gate fidelity can exceed 99\% for a node with only four cavities for both single-photon and two-photon operations. Moreover, the proposed gate architecture is compatible with the platforms of integrated photonics., Comment: 6 pages, 2 figures

Colloidal semiconductor quantum dots (QDs) are excellent luminescent nanomaterials for a broad range of optoelectronic applications. Their photoluminescence blinking, however, hinders their practical use in many aspects. It has been shown that coupling QDs to plasmonic nanostructures may provide a viable way to suppress blinking. Nevertheless, the underlying mechanism of blinking suppression remains unclear and debated. Here, by deterministically coupling a single QD to a plasmonic nanocavity, we clarify the mechanism of blinking suppression, and demonstrate unprecedentedly bright emission from a single colloidal QD. In particular, we report for the first time that the coupled system exhibits nonblinking photoluminescence with blinking lifetime, which shows that the elimination of photoluminescence blinking originates from enhanced quantum yield of the charged states. We identify that the radiative decay rate is boosted from (48 ns)-1 to (0.7 ns)-1, which outcompetes Auger processes and enables similar quantum yields for charged and neutral excitons. Moreover, we demonstrate ultrabright photoluminescence of up to 17 million detected photons per second from a single QD. This work sheds new light on the goal of achieving ultrabright nonblinking QDs and may benefit a variety of QD-based applications., Comment: 17 pages; 3 figures

We report that flat substrates such as glass coverslips with surface roughness well below 0.5 nm feature notable speckle patterns when observed with high-sensitivity interference microscopy. We uncover that these speckle patterns unambiguously originate from the subnanometer surface undulations, and develop an intuitive model to illustrate how subnanometer non-resonant dielectric features could generate pronounced interference contrast in the far field. We introduce the concept of optical fingerprint for the deterministic speckle pattern associated with a particular substrate surface area and intentionally enhance the speckle amplitudes for potential applications. We demonstrate such optical fingerprints can be leveraged for reproducible position identification and marker-free lateral displacement detection with an experimental precision of 0.22 nm. The reproducible position identification allows us to detect new nanoscopic features developed during laborious processes performed outside of the microscope. The demonstrated capability for ultrasensitive displacement detection may find applications in the semiconductor industry and super-resolution optical microscopy., Comment: 6 pages, 4 figures

Quantum hydrodynamic model (QHDM) has become a versatile and efficient tool for studying plasmonics at the nanoscopic length scale. Yet its application to noble metals has not been sufficiently justified, in particular for situations where the metallic structures interface with dielectric material and electrons spill over the interfaces. In a recent work, we developed a refined QHDM, where the near-field effects and static polarization of metal ion lattice, and the electron affinity and static permittivity of the dielectric are incorporated. Here we perform a careful calibration of the model parameters for the refined QHDM. The model parameters are determined by benchmarking with (time-dependent) density functional theory calculations for special cases of simple metal. The predictive power of the refined QHDM with calibrated model parameters is faithfully demonstrated by the calculations of the optical responses from gold nanomatryoshkas of different sizes. The refined QHDM approach allows the quasinormal mode analysis for revealing the intrinsic optical properties of the nanoscopic metallic structures. We expect the well-calibrated refined QHDM would provide the nanoplasmonics community with a useful tool., Comment: 9 pages, 6 figures

We report a self-consistent quasinormal mode theory for nanometer scale electromagnetism where the possible nonlocal and quantum effects are treated through quantum surface responses. With Feibelman's frequency-dependent \textit{d} parameters to describe the quantum surface responses, we formulate the source-free Maxwell's equations into a generalized linear eigenvalue problem to define the quasinormal modes. We then construct an orthonormal relation for the modes and consequently unlock the powerful toolbox of modal analysis. The orthonormal relation is validated by the reconstruction of the full numerical results through modal contributions. Significant changes in the landscape of the modes are observed due to the incorporation of the quantum surface responses for a number of nanostructures. Our semi-analytical modal analysis enables transparent physical interpretation of the spontaneous emission enhancement of a dipolar emitter as well as the near-field and far-field responses of planewave excitations in the nanostructures., Comment: 8 pages, 4 figures

Optical phenomena associated with extremely localized field should be understood with considerations of nonlocal and quantum effects, which pose a hurdle to conceptualize the physics with a picture of eigenmodes. Here we first propose a generalized Lorentz model to describe general nonlocal media under linear mean-field approximation and formulate source-free Maxwell's equations as a linear eigenvalue problem to define the quasinormal modes. Then we introduce an orthonormalization scheme for the modes and establish a canonical quasinormal mode framework for general nonlocal media. Explicit formalisms for metals described by quantum hydrodynamic model and polar dielectrics with nonlocal response are exemplified. The framework enables for the first time direct modal analysis of mode transition in the quantum tunneling regime and provides physical insights beyond usual far-field spectroscopic analysis. Applied to nonlocal polar dielectrics, the framework also unveils the important roles of longitudinal phonon polaritons in optical response., Comment: 6 pages, 2 figures

Concentrating optical field in an eigenmode with a tiny volume is vitally important for light-matter interactions at the fundamental level and underpins new technologies. In the past decades, researchers have investigated various approaches to shrink light and so far managed to reduce the volume of optical eigenmodes, under the quantum-optical definition, down to several ten nm3. Here we report on the discovery, characterization and engineering of a class of extremely localized eigenmodes that are resonances of atomistic protrusions on a metallic host nanoparticle and feature quantum-optical mode volumes of below 1 nm3. We theoretically demonstrate that these extremely localized modes can be made bright with radiation efficiencies reaching 30% and provide up to 4x10^7 times intensity enhancement. The existence of bright eigenmodes with the volume comparable to a photon emitter foresees exciting new optical physics, such as ultrastrong coupling with single optical emitters, angstrom-resolution optical imaging, and atomic-scale single-molecule photochemistry.

We propose a novel antenna structure which funnels single photons from a single emitter with unprecedented efficiency into a low-divergence fundamental Gaussian mode. Our device relies on the concept of creating an omnidirectional photonic bandgap to inhibit unwanted large-angle emission and to enhance small-angle defect-guided-mode emission. The new photon collection strategy is intuitively illustrated, rigorously verified and optimized by implementing an efficient body-of-revolution finite-difference time-domain method for in-plane dipole emitters. We investigate a few antenna designs to cover various boundary conditions posed by fabrication processes or material restrictions and theoretically demonstrate that collection efficiencies into the fundamental Gaussian mode exceeding 95% are achievable. Our antennas are broadband, insensitive to fabrication imperfections and compatible with a variety of solid-state emitters such as organic molecules, quantum dots and defect centers in diamond. Unidirectional and low-divergence Gaussian-mode emission from a single emitter may enable the realization of a variety of photonic quantum computer architectures as well as highly efficient light-matter interfaces., Comment: 9 pages, 4 figures

Interferometric scattering microscopy (iSCAT), as an ultrasensitive fluorescence-free imaging modality, has recently gain enormous attention and been rapidly developing from demonstration of principle to quantitative sensing. Here we report on a theoretical and experimental study for iSCAT with samples having structural dimensions that differ by 4-5 orders of magnitude. In particular, we demonstrate and intuitively explain the profound effects of sub-nanometer surface roughness of a glass coverslip and of a mica surface on the absolute signal and the shape of the point spread function of a gold nanoparticle. These quantities significantly affect the accuracies for determining the target size and position in all three dimensions. Moreover, we investigate a sample system mimicking a gold nanoparticle in a simplified cell environment and show position-dependent and even asymmetric point spread function of the nanoparticle. The multiscale study will facilitate the development of high fidelity iSCAT in real applications., Comment: Expanded the discussion on the effect of surface roughness

Single molecules in solids have been considered as an attractive class of solid-state single quantum systems because they can be chemically synthesized at low cost to have stable narrow transitions at desired wavelengths. Here we report and demonstrate single dibenzoterrylene molecules in crystalline anthracene nanosheets as a robust and versatile solid-state platform for delicate photophysics studies and building blocks of single-photon devices. The high-quality nanosheet sample enables robust studies of delicate single-molecule photophysics at room temperature, including the first real-time observation of single molecule insertion site jump, quantitative measurements of the associated changes of dipole moment orientation and magnitude, unambiguous determination of excitation-power dependent intersystem crossing rate and triplet lifetime. Moreover, we demonstrate the flexible assembly of the nanosheets into a planar antenna device to achieve bright single-molecule emission with a Gaussian emission pattern. The thin thickness, good photostability and mechanical stability make the dibenzoterrylene-in-anthracene nanosheet system an excellent candidate of static quantum nodes in integrated photonic circuit.

Classical wisdom of wave-particle duality says that it is impossible to observe simultaneously the wave and particle nature of microscopic object. Mathematically the principle requests that the interference visibility V and which-path distinguishability D satisfy an orthodox limit of square(V)+square(D)<=1. This work presents a new wave-particle duality test experiment with single photon in a modified Mach-Zehnder interferometer and convincingly show the possibility of breaking the limit. The key element of the interferometer is a weakly-scattering total-internal reflection prism surface, which exhibits pronounced single-photon interference with a visibility up to 0.97 and simultaneously provides path distinguishability of 0.83. Apparently square(V)+square(D)=1.63 far exceeds the orthodox limit set by the principle of wave-particle duality for single photon. It is expected that more delicate experiments in future should be able to demonstrate the ultimate regime of square(V)+square(D) approaching 2 and shed new light on the foundations of contemporary quantum mechanics., Comment: 14 pages, 4 figures

Integrated quantum photonics hold the promise to scale up the system size and form an on-chip quantum network with distributed information processing and simulation units. An outstanding need of such quantum network is to have high fidelity and efficiency on-chip state transfer between distant nodes. Although the nodes are naturally connected via waveguides, it is challenging to fulfill this need because stringent conditions such as spatial mode-matching configuration and time-reversal symmetry have to be satisfied. Here we report a type of quantum photonic nodes consisting of single quantum emitters and cascaded microring resonators for on-chip state transfer. By interfacing the node with a waveguide, we show that all the emission from the node can be funneled into the waveguide and its temporal profile can be synthesized to be time-reversal symmetric. We demonstrate theoretically on-chip quantum state transfer between two distant nodes with near-unity overall success rate can be achieved without any dynamic control. Moreover, we discuss the experimental implementation of our scheme with CMOS compatible integrated photonic platforms and solid-state quantum optics techniques., Comment: 6 pages,4 figures

Single nanoscopic emitters embedded in crystalline matrix have become a valuable resource for emerging nanophotonic and quantum technologies. The generally anisotropic nature of the matrix strongly affects the emission properties of the quantum emitters, in particular, when the matrix is assembled in nanophotonic structures. We report on rigorous analysis and engineering of spontaneous emission from single emitters coupled to nanoantenna and planar anisotropic antenna structures. By developing a convenient theoretical method with efficient numerical implementation, we show that accurate modeling of the anisotropy is essential in predicting the emission pattern for many important systems, such as single molecules in solid-state matrix, isolated defects in 2D materials and so on. In particular, we illustrate the amplified effects of material anisotropy and geometrical anisotropy for emitters coupled to planar antenna and nanoantenna structures. We show that with proper design of the anisotropies strong enhancement of the emission rate and nearly collimated beam from single emitters can be simultaneously achieved.

This paper investigates long-term face tracking of a specific person given his/her face image in a single frame as a query in a video stream. Through taking advantage of pre-trained deep learning models on big data, a novel system is developed for accurate video face tracking in the unconstrained environments depicting various people and objects moving in and out of the frame. In the proposed system, we present a detection-verification-tracking method (dubbed as 'DVT') which accomplishes the long-term face tracking task through the collaboration of face detection, face verification, and (short-term) face tracking. An offline trained detector based on cascaded convolutional neural networks localizes all faces appeared in the frames, and an offline trained face verifier based on deep convolutional neural networks and similarity metric learning decides if any face or which face corresponds to the queried person. An online trained tracker follows the face from frame to frame. When validated on a sitcom episode and a TV show, the DVT method outperforms tracking-learning-detection (TLD) and face-TLD in terms of recall and precision. The proposed system is also tested on many other types of videos and shows very promising results., Comment: KDD Workshop on Large-scale Deep Learning for Data Mining, August 2016, San Fransisco, CA, USA

Upon photo- or electrical-excitation, colloidal quantum dots (QDs) are often found in multi-carrier states due to multi-photon absorption and photo-charging of the QDs. While many of these multi-carrier states are observed in single-dot spectroscopy, their properties are not well studied due to random charging/discharging, emission intensity intermittency, and uncontrolled surface defects of single QD. Here we report in-situ deciphering the charging status, and precisely assessing the absorption cross section, and determining the absolute emission quantum yield of mono-exciton and biexciton states for neutral, positively-charged, and negatively-charged single core/shell CdSe/CdS QD. We uncover very different photon statistics of the three charge states in single QD and unambiguously identify their charge sign together with the information of their photoluminescence decay dynamics. We then show their distinct photoluminescence saturation behaviors and evaluated the absolute values of absorption cross sections and quantum efficiencies of monoexcitons and biexcitons. We demonstrate that addition of an extra hole or electron in a QD changes not only its emission properties but also varies its absorption cross section.

Optical coherence tomography (OCT) is a prevalent, interferometric, high-resolution imaging method with broad biomedical applications. Nonetheless, OCT images suffer from an artifact, called speckle which degrades the image quality. Digital filters offer an opportunity for image improvement in clinical OCT devices where hardware modification to enhance images is expensive. To reduce speckle, a wide variety of digital filters have been proposed, selecting the most appropriate filter for each OCT image/image set is a challenging decision. To tackle this challenge, we propose an expandable learnable despeckling framework, we called LDF. LDF decides which speckle reduction algorithm is most effective on a given image by learning a figure of merit (FOM) as a single quantitative image assessment measure. The architecture of LDF includes two main parts: (i) an autoencoder neural network, (ii) filter classifier. The autoencoder learns the figure of merit based on the quality assessment measures obtained from the OCT image including.Subsequently, the filter classifier identifies the most efficient filter from the following categories: (a) sliding window filters including median, mean, and symmetric nearest neighborhood, (b) adaptive statistical based filters including Wiener, homomorphic Lee, and Kuwahara, and, (c) edge preserved patch or pixel correlation based filters including non-local mean, total variation, and block matching 3D filtering., Comment: under review

Optical coherence tomography (OCT) has become a favorable device in the Dermatology discipline due to its moderate resolution and penetration depth. OCT images however contain a grainy pattern, called speckle, due to the use of a broadband source in the configuration of OCT. So far, a variety of filtering (de-speckling) techniques is introduced to reduce speckle in OCT images. Most of these methods are generic and can be applied to OCT images of different tissues. The ambition of this work is to provide a de-speckling framework specialized for filtering skin tissues for the community to utilize, adapt or build upon. In this paper, we present an adaptive cluster-based filtering framework, optimized for speckle reduction of OCT skin images. In this framework, by considering the layered structure of skin, first the OCT skin images are segmented into differentiable layers utilizing clustering algorithms, and then each cluster is de-speckled individually using adaptive filtering techniques. In this study, hierarchical clustering algorithm and adaptive Wiener filtering technique are utilized to develop the framework. The proposed method is tested on optical solid phantoms with predetermined optical properties. The method is also tested on healthy human skin images. The results show that the proposed cluster-based filtering method can effectively reduce the speckle and increase the signal-to-noise ratio and contrast while preserving the edges in the image. The proposed cluster-based filtering framework enables researchers to develop unsupervised learning solutions for de-speckling OCT skin images using adaptive filtering methods, or extend the framework to new applications., Comment: 17 pages, 6 figures, 2 tables

We theoretically demonstrate the generation and radiation of coherent nanoplasmons powered by a single three-level quantum emitter on a plasmonic nanoresonator. By pumping the three-level emitter in a Raman configuration, we show a pathway to achieve macroscopic accumulation of nanoplasmons due to stimulated emission in the nanoresonator despite their fast relaxation. Thanks to the antenna effect of the nanoresonator, the system acts as an efficient and bright nanoscopic coherent light source with a photon emission rate of hundreds of Terahertz and could be realized with solid-state emitters at room temperatures in pulse mode. We provide physical interpretations of the results and discuss their realization and implications for ultra-compact integration of optoelectronics., Comment: 15 pages, 7 figures

In this work, we study a basic and practically important strategy to help prevent and/or delay an outbreak in the context of network: limiting the contact between individuals. In this paper, we introduce the average neighborhood size as a new measure for the degree of being small-world and utilize it to formally define the desmall- world network problem. We also prove the NP-hardness of the general reachable pair cut problem and propose a greedy edge betweenness based approach as the benchmark in selecting the candidate edges for solving our problem. Furthermore, we transform the de-small-world network problem as an OR-AND Boolean function maximization problem, which is also an NP-hardness problem. In addition, we develop a numerical relaxation approach to solve the Boolean function maximization and the de-small-world problem. Also, we introduce the short-betweenness, which measures the edge importance in terms of all short paths with distance no greater than a certain threshold, and utilize it to speed up our numerical relaxation approach. The experimental evaluation demonstrates the effectiveness and efficiency of our approaches., Comment: 9 pages

We provide a general theoretical platform based on quantized radiation in absorptive and inhomogeneous media for investigating the coherent interaction of light with metallic structures in the immediate vicinity of quantum emitters. In the case of a very small metallic cluster, we demonstrate extreme regimes where a single emitter can either counteract or enhance particle absorption by three orders of magnitude. For larger structures, we show that an emitter can eliminate both scattering and absorption and cloak a plasmonic antenna. We provide physical interpretations of our results and discuss their applications in active metamaterials and quantum plasmonics.

We devise new optical antennas that reduce the excited-state radiative lifetimes of emitters to the order of 100 femtoseconds while maintaining quantum efficiencies of about 80% at a broadband operation. Here, we combine metallic nanoparticles with planar dielectric structures and exploit design strategies from plasmonic nanoantennas and concepts from Cavity Quantum Electrodynamics to maximize the local density of states and minimize the nonradiative losses incurred by the metallic constituents. The proposed metallo-dielectric hybrid antennas promise important impact on various fundamental and applied research fields, including photophysics, ultrafast plasmonics, bright single photon sources and Raman spectroscopy.

In Nature Photonics 5, 166 (2011), we reported on a planar dielectric antenna that achieved 96% efficiency in collecting the photons emitted by a single molecule. In that work the transition dipole moment of the molecule was set perpendicular to the antenna plane. Here, we present an extension of that scheme that reaches collection efficiencies beyond 99% for emitters with arbitrarily oriented dipole moments. Our work opens important doors in a wide range of contexts including quantum optics, quantum metrology, nano-analytics, and biophysics. In particular, we provide antenna parameters to realize ultrabright single-photon sources in high-index materials such as semiconductor quantum dots and color centers in diamond, as well as sensitive detection of single molecules in nanofluidic devices.

The production of heavy-flavored hadron at the hadronic colliders provides a challenging opportunity to test the validity of pQCD predictions. There are two mechanisms for the $B^{(*)}_s$ hadroproduction, i.e. the gluon-gluon fusion mechanism via the subprocess $g+g\rightarrow B^{(*)}_s+b+\bar{s}$ and the extrinsic heavy quark mechanism via the subprocesses $g+\bar{b}\to B^{(*)}_s +\bar{s}$ and $g+s\to B^{(*)}_s +b$, both of which shall have sizable contributions in proper kinematic region. Different from the fixed-flavor-number scheme (FFNS) previously adopted in the literature, we study the $B^{(*)}_s$ hadroproduction under the general-mass variable-flavor-number scheme (GM-VFNS), in which we can consistently deal with the double counting problem from the above two mechanisms. Properties for the $B^{(*)}_s$ hadroproduction are discussed. To be useful reference, a comparative study of FFNS and GM-VFNS is presented. Both of which can provide reasonable estimations for the $B^{(*)}_s$ hadroproduction. At the Tevatron, the difference between these two schemes is small, however such difference is obvious at the LHC. The forthcoming more precise data on LHC shall provide a good chance to check which scheme is more appropriate to deal with the $B^{(*)}_s$-meson production and to further study the heavy quark components in hadrons., Comment: 18 pages, 8 figures, 4 tables. To match the published version. To be published in Eur.Phys.J.C

Single gold nanoparticles can act as nanoantennas for enhancing the fluorescence of emitters in their near-fields. Here we present experimental and theoretical studies of scanning antenna-based fluorescence microscopy as a function of the diameter of the gold nanoparticle. We examine the interplay between fluorescence enhancement and spatial resolution and discuss the requirements for deciphering single molecules in a dense sample. Resolutions better than 20 nm and fluorescence enhancement up to 30 times are demonstrated experimentally. By accounting for the tip shaft and the sample interface in finite-difference time-domain calculations, we explain why the measured fluorescence enhancements are higher in the presence of an interface than the values predicted for a homogeneous environment., Comment: 10 pages, 3 figures. accepted for publication in Nano Letters

Successful exploitations of strongly confined surface plasmon-polaritons critically rely on their efficient and rapid conversion to lossless channels. We demonstrate a simple, robust, and broad-band butt-coupling technique for connecting a metallic nanowire and a dielectric nanofiber. Conversion efficiencies above 95% in the visible and close to 100% in the near infrared can be achieved with realistic parameters. Moreover, by combining butt-coupling with nanofocusing, we propose a broad-band high-throughput near-field optical microscope., Comment: 5 figures