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Undesired coupling to the surrounding environment destroys long-range correlations on quantum processors and hinders the coherent evolution in the nominally available computational space. This incoherent noise is an outstanding challenge to fully leverage the computation power of near-term quantum processors. It has been shown that benchmarking Random Circuit Sampling (RCS) with Cross-Entropy Benchmarking (XEB) can provide a reliable estimate of the effective size of the Hilbert space coherently available. The extent to which the presence of noise can trivialize the outputs of a given quantum algorithm, i.e. making it spoofable by a classical computation, is an unanswered question. Here, by implementing an RCS algorithm we demonstrate experimentally that there are two phase transitions observable with XEB, which we explain theoretically with a statistical model. The first is a dynamical transition as a function of the number of cycles and is the continuation of the anti-concentration point in the noiseless case. The second is a quantum phase transition controlled by the error per cycle; to identify it analytically and experimentally, we create a weak link model which allows varying the strength of noise versus coherent evolution. Furthermore, by presenting an RCS experiment with 67 qubits at 32 cycles, we demonstrate that the computational cost of our experiment is beyond the capabilities of existing classical supercomputers, even when accounting for the inevitable presence of noise. Our experimental and theoretical work establishes the existence of transitions to a stable computationally complex phase that is reachable with current quantum processors.

Surface acoustic waves are commonly used in classical electronics applications, and their use in quantum systems is beginning to be explored, as evidenced by recent experiments using acoustic Fabry-P\'erot resonators. Here we explore their use for quantum communication, where we demonstrate a single-phonon surface acoustic wave transmission line, which links two physically-separated qubit nodes. Each node comprises a microwave phonon transducer, an externally-controlled superconducting variable coupler, and a superconducting qubit. Using this system, precisely-shaped individual itinerant phonons are used to coherently transfer quantum information between the two physically-distinct quantum nodes, enabling the high-fidelity node-to-node transfer of quantum states as well as the generation of a two-node Bell state. We further explore the dispersive interactions between an itinerant phonon emitted from one node and interacting with the superconducting qubit in the remote node. The observed interactions between the phonon and the remote qubit promise future quantum optics-style experiments with itinerant phonons., Comment: 15 pages, 9 figures

Phonon modes at microwave frequencies can be cooled to their quantum ground state using conventional cryogenic refrigeration, providing a convenient way to study and manipulate quantum states at the single phonon level. Phonons are of particular interest because mechanical deformations can mediate interactions with a wide range of different quantum systems, including solid-state defects, superconducting qubits, as well as optical photons when using optomechanically-active constructs. Phonons thus hold promise for quantum-focused applications as diverse as sensing, information processing, and communication. Here, we describe a piezoelectric quantum bulk acoustic resonator (QBAR) with a 4.88 GHz resonant frequency that at cryogenic temperatures displays large electromechanical coupling strength combined with a high intrinsic mechanical quality factor $Q_i \approx 4.3 \times 10^4$. Using a recently-developed flip-chip technique, we couple this QBAR resonator to a superconducting qubit on a separate die and demonstrate quantum control of the mechanics in the coupled system. This approach promises a facile and flexible experimental approach to quantum acoustics and hybrid quantum systems.

Recent significant advances in coupling superconducting qubits to acoustic wave resonators has led to demonstrations of quantum control of surface and bulk acoustic resonant modes as well Wigner tomography of quantum states in these modes. These advances were achieved through the efficient coupling afforded by piezoelectric materials combined with GHz-frequency acoustic Fabry-Perot cavities. Quantum control of itinerant surface acoustic waves appears in reach, but is challenging due to the limitations of conventional transducers in the appropriate GHz-frequency band. In particular, GHz-frequency unidirectional transducers would provide an important addition to the desired quantum toolbox, promising unit efficiency with directional control over the surface acoustic wave emission pattern. Here we report the design, fabrication and experimental characterization of unidirectional distributed acoustic reflection transducers (DARTs) demonstrating a high transduction frequency of 4.8 GHz with a peak directivity larger than 25 dB and a directivity greater than 15 dB over a bandwidth of 17 MHz. A numerical model reproduces the main features of the transducer response quite well, with ten adjustable parameters (most of which are constrained by geometric and physical considerations). This represents a significant step towards quantum control of itinerant quantum acoustic waves., Comment: Main paper: 5 pages, 3 figures. Supplementary: 6 pages, 2 figures

Phonons, and in particular surface acoustic wave phonons, have been proposed as a means to coherently couple distant solid-state quantum systems. Recent experiments have shown that superconducting qubits can control and detect individual phonons in a resonant structure, enabling the coherent generation and measurement of complex stationary phonon states. Here, we report the deterministic emission and capture of itinerant surface acoustic wave phonons, enabling the quantum entanglement of two superconducting qubits. Using a 2 mm-long acoustic quantum communication channel, equivalent to a 500 ns delay line, we demonstrate the emission and re-capture of a phonon by one qubit; quantum state transfer between two qubits with a 67\% efficiency; and, by partial transfer of a phonon between two qubits, generation of an entangled Bell pair with a fidelity of $\mathcal{F}_B = 84 \pm 1$ %, Comment: 16 pages, 7 figures

Quantum communication relies on the efficient generation of entanglement between remote quantum nodes, due to entanglement's key role in achieving and verifying secure communications. Remote entanglement has been realized using a number of different probabilistic schemes, but deterministic remote entanglement has only recently been demonstrated, using a variety of superconducting circuit approaches. However, the deterministic violation of a Bell inequality, a strong measure of quantum correlation, has not to date been demonstrated in a superconducting quantum communication architecture, in part because achieving sufficiently strong correlation requires fast and accurate control of the emission and capture of the entangling photons. Here we present a simple and robust architecture for achieving this benchmark result in a superconducting system.

The superposition of quantum states is one of the hallmarks of quantum physics, and clear demonstrations of superposition have been achieved in a number of quantum systems. However, mechanical systems have remained a challenge, with only indirect demonstrations of mechanical state superpositions, in spite of the intellectual appeal and technical utility such a capability would bring. This is due in part to the highly linear response of most mechanical systems, making quantum operation difficult, as well as their characteristically low frequencies, making it difficult to reach the quantum ground state. In this work, we demonstrate full quantum control of the mechanical state of a macroscopic mechanical resonator. We strongly couple a surface acoustic wave resonator to a superconducting qubit, using the qubit to control and measure quantum states in the mechanical resonator. Most notably, we generate a quantum superposition of the zero and one phonon states and map this and other states using Wigner tomography. This precise, programmable quantum control is essential to a range of applications of surface acoustic waves in the quantum limit, including using surface acoustic waves to couple disparate quantum systems.

Point-defects in wide bandgap semiconductors are promising candidates for future applications that necessitate quantum light sources. Recently, defect-based single photon sources have been observed in ZnO that are very bright and remain photoactive from 4.5 K to room temperature. Despite several investigations, the structure and electronic states of these emitters remain unknown. In this work, we establish a procedure to distinguish a Z dipole from an XY dipole when studying quantum emitters that are randomly oriented. Our cryogenic and room temperature polarization measurements collectively establish that these unidentified ZnO quantum emitters have a Z dipole. We show that the associated absorption and emission dipoles are parallel within experimental uncertainty for all 32 individuals studied. Additionally, we apply group theory and find that assuming the defect symmetry belongs to a point-group relevant to the ZnO wurtzite lattice, the ground and excited states are orbital singlets. These results are a significant step in identifying the structure and electronic states of defect-based single photon sources in ZnO., Comment: 19 pages in manuscript format, 4 figures. Also a 9 page supplementary information

Investigations that probe defects one at a time offer a unique opportunity to observe properties and dynamics that are washed out of ensemble measurements. Here we present confocal fluorescence measurements of individual defects in Al-doped ZnO nanoparticles and undoped ZnO sputtered films that are excited with sub-bandgap energy light. Photon correlation measurements yield both antibunching and bunching, indicative of single-photon emission from isolated defects that possess a metastable shelving state. The single-photon emission is in the range 560 - 720 nm and typically exhibits two broad spectral peaks separated by approximately 150 meV. The excited state lifetimes range from 1 - 13 ns, consistent with the finite-size and surface effects of nanoparticles and small grains. We also observe discrete jumps in the fluorescence intensity between a bright state and a dark state. The dwell times in each state are exponentially distributed and the average dwell time in the bright (dark) state does (may) depend on the power of the exciting laser. Taken together, our measurements demonstrate the utility of a single-molecule approach to semiconductor defect studies and highlight ZnO as a potential host material for single-defect based applications., Comment: 33 pages, 7 figures