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19 results on '"Chang, Feixiang"'

12. A One-Pot Hydrothermal Preparation of High Loading Ni/La 2 O 3 Catalyst for Efficient Hydrogenation of Cinnamaldehyde.

Author

Yan, Haoting, Ren, Yongwang, Zhang, Renkun, Chang, Feixiang, Wei, Qinhong, and Xu, Jing

Subjects
HYDROGENATION, CATALYSTS, CATALYSTS recycling, CATALYTIC hydrogenation, ADSORPTION capacity, CATALYST supports, NICKEL catalysts, TRANSITION metal oxides, STEAM reforming
Abstract

It is a challenging task for selective hydrogenation of cinnamaldehyde (CAL) to hydrocinnamaldehyde (HCAL) without additional by-product formation. In this work, a La2O3 supported high Ni content nanoparticle catalyst was prepared for CAL selective hydrogenation. Meanwhile, Co-La2O3 catalysts were used as a reference catalyst. XRD, TEM, STEM-HAADF, XPS, and H2-TPR measurements were used to investigate the physicochemical properties of Ni-La2O3 catalysts. The experimental results confirmed that the CAL conversion and HCAL selectivity were effectively promoted with the increase of Ni loading amounts. At a Ni/La molar ratio of four, a high HCAL selectivity of 87.4% was obtained at a CAL conversion of 88.1% under mild reaction conditions. The catalyst was recycled five times without activity loss. Combined with various characterizations, it could be inferred that the good hydrogen adsorption and dissociation capacity of Ni and the presence of a certain amount of oxygen vacancies on the La2O3 support have a positive effect on the improvement of HCAL selectivity. This work provided an effective path to design transition-metal-based supported oxide catalyst for the cinnamaldehyde hydrogenation to hydrocinnamaldehyde. [ABSTRACT FROM AUTHOR]

Published
2023
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19. Behaviors of Multi-Droplets Impacting on a Flat Wall

Author

Luo, Hongliang and Chang, Feixiang

Subjects
Science / Chemistry
Abstract

Microscopic characteristics of fuel spray are very important for atomization and mixture formation. The droplet size, number density, velocity distribution as well as minimum distance reveal the quality of spray and atomization, which affects the subsequent combustion and emissions for different engines such as vehicle, marine and aircraft. Moreover, in the internal combustion engine, the spray-wall impingement is difficult to avoid, which is the main source for soot emissions. Nowadays, regulations for emissions become straight by governments. Therefore, it is urgent for us to alleviate the energy and emissions crisis. In this study, the droplets behaviors will be characterized under the related engine working state. Firstly, the experimental setup and measurement were explained in detail. Then, images process method was induced to calculate the droplet size, velocity and distance among them. Finally, results of the impinging spray were presented. One thing should be noted, as the dense region is not available to detect the droplets by the observation. Therefore, a spray “slicer” was designed and applied to cut the spray slim. Finally, multi-droplets were generated, and the results can be concluded as well. All the results could provide insights into the impacting behaviors for better understanding the droplet dynamics.

Published
2022

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