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Photonic quantum information processing in metropolitan quantum networks lays the foundation for cloud quantum computing [1, 2], secure communication [3, 4], and the realization of a global quantum internet [5, 6]. This paradigm shift requires on-demand and high-rate generation of flying qubits and their quantum state teleportation over long distances [7]. Despite the last decade has witnessed an impressive progress in the performances of deterministic photon sources [8-11], the exploitation of distinct quantum emitters to implement all-photonic quantum teleportation among distant parties has remained elusive. Here, we overcome this challenge by using dissimilar quantum dots whose electronic and optical properties are engineered by light-matter interaction [12], multi-axial strain [13] and magnetic fields [14] so as to make them suitable for the teleportation of polarization qubits. This is demonstrated in a hybrid quantum network harnessing both fiber connections and 270 m free-space optical link connecting two buildings of the University campus in the center of Rome. The protocol exploits GPS-assisted synchronization, ultra-fast single photon detectors as well as stabilization systems that compensate for atmospheric turbulence. The achieved teleportation state fidelity reaches up to 82+-1%, above the classical limit by more than 10 standard deviations. Our field demonstration of all-photonic quantum teleportation opens a new route to implement solid-state based quantum relays and builds the foundation for practical quantum networks.

Bosonic bunching is a term used to describe the well-known tendency of bosons to bunch together, and which differentiates their behaviour from that of fermions or classical particles. However, in some situations perfectly indistinguishable bosons may counter-intuitively bunch less than classical, distinguishable particles. Here we report two such counter-intuitive multiphoton bunching effects observed with three photons in a three-mode balanced photonic Fourier interferometer. In this setting, we show indistinguishable photons actually minimize the probability of bunching. We also show that any non-trivial value of the three-photon collective photonic phase leads to a decreased probability of all photons ending up in the same mode, even as we increase pairwise indistinguishability. Our experiments feature engineering of partial indistinguishability scenarios using both the time and the polarization photonic degrees of freedom, and a polarization-transparent 8-mode tunable interferometer with a quantum-dot source of single photons. Besides the foundational understanding, the observation of these counter-intuitive phenomena open news perspective in devising more efficient ways of routing photons for advantage in metrology and quantum computation., Comment: 10+8 pages, 5+1 figures

A Bernoulli factory is a randomness manipulation routine that takes as input a Bernoulli random variable, outputting another Bernoulli variable whose bias is a function of the input bias. Recently proposed quantum-to-quantum Bernoulli factory schemes encode both input and output variables in qubit amplitudes. This primitive could be used as a sub-routine for more complex quantum algorithms involving Bayesian inference and Monte Carlo methods. Here, we report an experimental implementation of a polarization-encoded photonic quantum-to-quantum Bernoulli factory. We present and test three interferometric set-ups implementing the basic operations of an algebraic field (inversion, multiplication, and addition) which, chained together, allow for the implementation of a generic quantum-to-quantum Bernoulli factory. These in-bulk schemes are validated using a quantum dot-based single-photon source featuring high brightness and indistinguishability, paired with a time-to-spatial demultiplexing setup to prepare input resources of up to three single-photon states.

In the current era of noisy intermediate-scale quantum computers, variational quantum algorithms represent one of the most viable approaches for their application to solve tasks of interest. These algorithms train a parameterized quantum circuit to execute a specific task encoded in a cost function that needs to be minimized using a classical optimizer. In this context, photonic platforms based on reconfigurable integrated optics appear as one of the prominent platforms for the implementation of variational algorithms. In the circuital model of quantum computation based on qubits, to train variational circuits, the parameter shift rule came into being, which allows for the exact calculation of the derivatives of many functions at the output of a quantum circuit, opening up the possibility of using classical optimisation algorithms based on gradient descent. In this paper, we derive a formulation of the parameter shift rule for reconfigurable optical linear circuits based on the Boson Sampling paradigm. This allows us to naturally embed the common types of experimental noise, such as partial distinguishability, and mixedness of the states, thus obtaining a resilient approach. We also present similar rules for the computations of integrals over the variational parameters. Finally, we employ the developed approach to experimentally test variational algorithms with single-photon states processed in a reconfigurable 6-mode universal integrated interferometer. Specifically, we apply the photonic parameter shift rules to the variational implementation, on a photonic platform, of both an eigensolver and a Universal-Not gate., Comment: 10 pages, 4 figures

Generation and manipulation of randomness is a relevant task for several applications of information technology. It has been shown that quantum mechanics offers some advantages for this type of task. A promising model for randomness manipulation is provided by the Bernoulli factories, protocols capable of changing the bias of Bernoulli random processes in a controlled way. At first, this framework was proposed and investigated in a fully classical regime. Recent extensions of this model to the quantum case showed the possibility of implementing a wider class of randomness manipulation functions. We propose a Bernoulli factory scheme with quantum states as input and output, using a photonic path-encoding approach. Our scheme is modular, universal, and its functioning is truly oblivious of the input bias, characteristics that were missing in earlier work. We report on experimental implementations using an integrated and fully programmable photonic platform, thus demonstrating the viability of our approach. These results open new paths for randomness manipulation with integrated quantum technologies.

The exploitation of certification tools by end users represents a fundamental aspect of the development of quantum technologies as the hardware scales up beyond the regime of classical simulatability. Certifying quantum networks becomes even more crucial when the privacy of their users is exposed to malicious quantum nodes or servers as in the case of multi-client distributed blind quantum computing, where several clients delegate a joint private computation to remote quantum servers, such as federated quantum machine learning. In such protocols, security must be provided not only by keeping data hidden but also by verifying that the server is correctly performing the requested computation while minimizing the hardware assumptions on the employed devices. Notably, standard verification techniques fail in scenarios where the clients receive quantum states from untrusted sources such as, for example, in a recently demonstrated linear quantum network performing multi-client blind quantum computation. However, recent theoretical results provide techniques to verify blind quantum computations even in the case of untrusted state preparation. Equipped with such theoretical tools, in this work, we provide the first experimental implementation of a two-client verifiable blind quantum computing protocol in a distributed architecture. The obtained results represent novel perspectives for the verification of multi-tenant distributed quantum computation in large-scale networks., Comment: Minor changes in the description of the experimental setup

A seminal task in quantum information theory is to realize a device able to produce copies of a generic input state with the highest possible output fidelity, thus realizing an \textit{optimal} quantum cloning machine. Recently, the concept of variational quantum cloning was introduced: a quantum machine learning algorithm through which, by exploiting a classical feedback loop informed by the output of a quantum processing unit, the system can self-learn the programming required for an optimal quantum cloning strategy. In this work, we experimentally implement a $1 \rightarrow 2$ variational cloning machine of dual-rail encoded photonic qubits, both for phase-covariant and state-dependent cloning. We exploit a fully programmable 6-mode universal integrated device and classical feedback to reach near-optimal cloning performances. Our results demonstrate the potential of programmable integrated photonic platforms for variational self-learning of quantum algorithms., Comment: 9 pages, 4 figures

Multiphoton indistinguishability is a central resource for quantum enhancement in sensing and computation. Developing and certifying large scale photonic devices requires reliable and accurate characterization of this resource, preferably using methods that are robust against experimental errors. Here, we propose a set of methods for the characterization of multiphoton indistinguishability, based on measurements of bunching and photon number variance. Our methods are robust in a semi-device independent way, in the sense of being effective even when the interferometers are incorrectly dialled. We demonstrate the effectiveness of this approach using an advanced photonic platform comprising a quantum-dot single-photon source and a universal fully-programmable integrated photonic processor. Our results show the practical usefulness of our methods, providing robust certification tools that can be scaled up to larger systems., Comment: 19 pages + 10 figures

Quantum Cellular Automaton (QCA) is a model for universal quantum computation and a natural candidate for digital quantum simulation of relativistic quantum fields. Here we introduce the first photonic platform for implementing QCA-simulation of a free relativistic Dirac quantum field in 1+1 dimension, through a Dirac Quantum Cellular Automaton (DQCA). Encoding the field position degree of freedom in the Orbital Angular Momentum (OAM) of single photons, our state-of-the-art setup experimentally realizes 8 steps of a DQCA, with the possibility of having complete control over the input OAM state preparation and the output measurement making use of two spatial light modulators. Therefore, studying the distribution in the OAM space at each step, we were able to reproduce the time evolution of the free Dirac field observing, the Zitterbewegung, an oscillatory movement extremely difficult to see in real case experimental scenario that is a signature of the interference of particle and antiparticle states. The accordance between the expected and measured Zitterbewegung oscillations certifies the simulator performances, paving the way towards the application of photonic platforms to the simulation of more complex relativistic effects.

Quantum superposition of high-dimensional states enables both computational speed-up and security in cryptographic protocols. However, the exponential complexity of tomographic processes makes certification of these properties a challenging task. In this work, we experimentally certify coherence witnesses tailored for quantum systems of increasing dimension, using pairwise overlap measurements enabled by a six-mode universal photonic processor fabricated with a femtosecond laser writing technology. In particular, we show the effectiveness of the proposed coherence and dimension witnesses for qudits of dimensions up to 5. We also demonstrate advantage in a quantum interrogation task, and show it is fueled by quantum contextuality. Our experimental results testify to the efficiency of this novel approach for the certification of quantum properties in programmable integrated photonic platforms, Comment: 9 pages, 5 figures + Supplementary Information

Quantum state teleportation represents a pillar of quantum information and a milestone on the roadmap towards quantum networks with a large number of nodes. Successful photonic demonstrations of this protocol have been carried out employing different qubit encodings. However, demonstrations in the Fock basis encoding are challenging, due to the impossibility of generating a coherent superposition of vacuum-one photon states on a single mode with linear optics. Indeed, previous realizations only allowed the teleportation of dual-rail entangled states, by exploiting ancillary electromagnetic modes. Here, instead, we enable the quantum teleportation of pure vacuum-one-photon qubits encoded in a single spatial mode, by exploiting coherent control of a resonantly excited semiconductor quantum dot in a micro-cavity. Within our setup, we can both teleport genuine single-rail vacuum-one-photon qubits and perform entanglement swapping. Our results may disclose new quantum information processing potentialities for this encoding, whose manipulation is achievable via quantum dot single-photon sources., Comment: 10 pages, 5 figures + Supplementary Information

Single-photon sources based on semiconductor quantum dots find several applications in quantum information processing due to their high single-photon indistinguishability, on-demand generation, and low multiphoton emission. In this context, the generation of entangled photons represents a challenging task with a possible solution relying on the interference in probabilistic gates of identical photons emitted at different pulses from the same source. In this work, we implement this approach via a simple and compact design that generates entangled photon pairs in the polarization degree of freedom. We operate the proposed platform with single photons produced through two different pumping schemes, the resonant excited one and the longitudinal-acoustic phonon-assisted configuration. We then characterize the produced entangled two-photon states by developing a complete model taking into account relevant experimental parameters, such as the second-order correlation function and the Hong-Ou-Mandel visibility. Our source shows long-term stability and high quality of the generated entangled states, thus constituting a reliable building block for optical quantum technologies.

Universal blind quantum computing allows users with minimal quantum resources to delegate a quantum computation to a remote quantum server, while keeping intrinsically hidden input, algorithm, and outcome. State-of-art experimental demonstrations of such a protocol have only involved one client. However, an increasing number of multi-party algorithms, e.g. federated machine learning, require the collaboration of multiple clients to carry out a given joint computation. In this work, we propose and experimentally demonstrate a lightweight multi-client blind quantum computation protocol based on a novel linear quantum network configuration (Qline). Our protocol originality resides in three main strengths: scalability, since we eliminate the need for each client to have its own trusted source or measurement device, low-loss, by optimizing the orchestration of classical communication between each client and server through fast classical electronic control, and compatibility with distributed architectures while remaining intact even against correlated attacks of server nodes and malicious clients.

Mutually entangled multi-photon states are at the heart of all-optical quantum technologies. While impressive progresses have been reported in the generation of such quantum light states using free space apparatus, high-fidelity high-rate on-chip entanglement generation is crucial for future scalability. In this work, we use a bright quantum-dot based single-photon source to demonstrate the high fidelity generation of 4-photon Greenberg-Horne-Zeilinger (GHZ) states with a low-loss reconfigurable glass photonic circuit. We reconstruct the density matrix of the generated states using full quantum-state tomography reaching an experimental fidelity to the target $|{\text{GHZ}_4}\rangle$ of $\mathcal{F}_{\text{GHZ}_4} (86.0\pm0.4)\,\%$, and a purity of $\mathcal{P}_{\text{GHZ}_4}=(76.3\pm0.6)\,\%$. The entanglement of the generated states is certified with a semi device-independent approach through the violation of a Bell-like inequality by more than 39 standard deviations. Finally, we carry out a four-partite quantum secret sharing protocol on-chip where a regulator shares with three interlocutors a sifted key with up to 1978 bits, achieving a qubit-error rate of $10.87\,\%$. These results establish that the quantum-dot technology combined with glass photonic circuitry for entanglement generation on chip offers a viable path for intermediate scale quantum computation and communication.

Engineering single-photon states endowed with Orbital Angular Momentum (OAM) is a powerful tool for quantum information photonic implementations. Indeed, thanks to its unbounded nature, OAM is suitable to encode qudits allowing a single carrier to transport a large amount of information. Nowadays, most of the experimental platforms use nonlinear crystals to generate single photons through Spontaneous Parametric Down Conversion processes, even if this kind of approach is intrinsically probabilistic leading to scalability issues for increasing number of qudits. Semiconductors Quantum Dots (QDs) have been used to get over these limitations being able to produce on demand pure and indistinguishable single-photon states, although only recently they were exploited to create OAM modes. Our work employs a bright QD single-photon source to generate a complete set of quantum states for information processing with OAM endowed photons. We first study the hybrid intra-particle entanglement between the OAM and the polarization degree of freedom of a single-photon. We certify the preparation of such a type of qudit states by means of the Hong-Ou-Mandel effect visibility which furnishes the pairwise overlap between consecutive OAM-encoded photons. Then, we investigate the hybrid inter-particle entanglement, by exploiting a probabilistic two qudit OAM-based entangling gate. The performances of our entanglement generation approach are assessed performing high dimensional quantum state tomography and violating Bell inequalities. Our results pave the way toward the use of deterministic sources (QDs) for the on demand generation of photonic quantum states in high dimensional Hilbert spaces.

In a Bell experiment, it is natural to seek a causal account of correlations wherein only a common cause acts on the outcomes. For this causal structure, Bell inequality violations can be explained only if causal dependencies are modelled as intrinsically quantum. There also exists a vast landscape of causal structures beyond Bell that can witness nonclassicality, in some cases without even requiring free external inputs. Here, we undertake a photonic experiment realizing one such example: the triangle causal network, consisting of three measurement stations pairwise connected by common causes and no external inputs. To demonstrate the nonclassicality of the data, we adapt and improve three known techniques: (i) a machine-learning-based heuristic test, (ii) a data-seeded inflation technique generating polynomial Bell-type inequalities and (iii) entropic inequalities. The demonstrated experimental and data analysis tools are broadly applicable paving the way for future networks of growing complexity., Comment: Version published in Nature Communications

Detecting gravity mediated entanglement can provide evidence that the gravitational field obeys quantum mechanics. We report the result of a simulation of the phenomenon using a photonic platform. The simulation tests the idea of probing the quantum nature of a variable by using it to mediate entanglement, and yields theoretical and experimental insights. We employed three methods to test the presence of entanglement: Bell test, entanglement witness and quantum state tomography. We also simulate the alternative scenario predicted by gravitational collapse models or due to imperfections in the experimental setup and use quantum state tomography to certify the absence of entanglement. Two main lessons arise from the simulation: 1) which--path information must be first encoded and subsequently coherently erased from the gravitational field, 2) performing a Bell test leads to stronger conclusions, certifying the existence of gravity mediated nonlocality.

Entanglement-based quantum key distribution can enable secure communication in trusted node-free networks and over long distances. Although implementations exist both in fiber and in free space, the latter approach is often considered challenging due to environmental factors. Here, we implement a quantum communication protocol during daytime for the first time using a quantum dot source. This technology presents advantages in terms of narrower spectral bandwidth -- beneficial for filtering out sunlight -- and negligible multiphoton emission at peak brightness. We demonstrate continuous operation over the course of three and a half days, across an urban 270-m-long free-space optical link, under different light and weather conditions., Comment: The first two authors contributed equally to this work. 10 pages, 3 figures

Quantum walks represent paradigmatic quantum evolutions, enabling powerful applications in the context of topological physics and quantum computation. They have been implemented in diverse photonic architectures, but the realization of a two-particle dynamics on a multi-dimensional lattice has hitherto been limited to continuous-time evolutions. To fully exploit the computational capabilities of quantum interference it is crucial to develop platforms handling multiple photons that propagate across multi-dimensional lattices. Here, we report a discrete-time quantum walk of two correlated photons in a two-dimensional lattice, synthetically engineered by manipulating a set of optical modes carrying quantized amounts of transverse momentum. Mode-couplings are introduced via the polarization-controlled diffractive action of thin geometric-phase optical elements. The entire platform is compact, efficient, scalable, and represents a versatile tool to simulate quantum evolutions on complex lattices. We expect that it will have a strong impact on diverse fields such as quantum state engineering, topological quantum photonics, and Boson Sampling., Comment: 18 pages, 11 figures

Quantum networks are the center of many of the recent advances in quantum science, not only leading to the discovery of new properties in the foundations of quantum theory but also allowing for novel communication and cryptography protocols. It is known that networks beyond that in the paradigmatic Bell's theorem imply new and sometimes stronger forms of nonclassicality. Due to a number of practical difficulties, however, the experimental implementation of such networks remains far less explored. Going beyond what has been previously tested, here we verify the nonlocality of an experimental triangle network, consisting of three independent sources of bipartite entangled photon states interconnecting three distant parties. By performing separable measurements only and evaluating parallel chained Bell inequalities, we show that such networks can lead to a genuine form of tripartite nonlocality, where classical models are unable to mimic the quantum predictions even if some of the parties are allowed to communicate.

Quantum networks play a crucial role for distributed quantum information processing, enabling the establishment of entanglement and quantum communication among distant nodes. Fundamentally, networks with independent sources allow for new forms of nonlocality, beyond the paradigmatic Bell's theorem. Here we implement the simplest of such networks -- the bilocality scenario -- in an urban network connecting different buildings with a fully scalable and hybrid approach. Two independent sources using different technologies, respectively a quantum dot and a nonlinear crystal, are used to share photonic entangled state among three nodes connected through a 270 m free-space channel and fiber links. By violating a suitable non-linear Bell inequality, we demonstrate the nonlocal behaviour of the correlations among the nodes of the network. Our results pave the way towards the realization of more complex networks and the implementation of quantum communication protocols in an urban environment, leveraging on the capabilities of hybrid photonic technologies.

Since Bell's theorem, it is known that the concept of local realism fails to explain quantum phenomena. Indeed, the violation of a Bell inequality has become a synonym of the incompatibility of quantum theory with our classical notion of cause and effect. As recently discovered, however, the instrumental scenario -- a tool of central importance in causal inference -- allows for signatures of nonclassicality that do not hinge on this paradigm. If, instead of relying on observational data only, we can also intervene in our experimental setup, quantum correlations can violate classical bounds on the causal influence even in scenarios where no violation of a Bell inequality is ever possible. That is, through interventions, we can witness the quantum behaviour of a system that would look classical otherwise. Using a photonic setup -- faithfully implementing the instrumental causal structure and allowing to switch between the observational and interventional modes in a run to run basis -- we experimentally observe this new witness of nonclassicality for the first time. In parallel, we also test quantum bounds for the causal influence, showing that they provide a reliable tool for quantum causal modelling., Comment: main: 10 pages, 5 figures -- supplementary: 4 pages

Boson Sampling is a computational paradigm representing one of the most viable and pursued approaches to demonstrate the regime of quantum advantage. Recent results have demonstrated significant technological leaps in single-photon generation and detection, leading to progressively larger experimental instances of Boson Sampling experiments in different photonic systems. However, a crucial requirement for a fully-fledged platform solving this problem is the capability of implementing large-scale interferometers, that must simultaneously exhibit low losses, high degree of reconfigurability and the realization of arbitrary transformations. In this work, we move a step forward in this direction by demonstrating the adoption of a compact and reconfigurable 3D-integrated platform for photonic Boson Sampling. We perform 3- and 4-photon experiments by using such platform, showing the possibility of programming the circuit to implement a large number of unitary transformations. These results show that such compact and highly-reconfigurable layout can be scaled up to experiments with larger number of photons and modes, and can provide a viable direction for hybrid computing with photonic processors., Comment: 17 pages, 15 figures

Bell's theorem is typically understood as the proof that quantum theory is incompatible with local-hidden-variable models. More generally, we can see the violation of a Bell inequality as witnessing the impossibility of explaining quantum correlations with classical causal models. The violation of a Bell inequality, however, does not exclude classical models where some level of measurement dependence is allowed, that is, the choice made by observers can be correlated with the source generating the systems to be measured. Here, we show that the level of measurement dependence can be quantitatively upper bounded if we arrange the Bell test within a network. Furthermore, we also prove that these results can be adapted in order to derive nonlinear Bell inequalities for a large class of causal networks and to identify quantumly realizable correlations that violate them., Comment: 18 pages, 10 figures. Updated to match published version

Quantum coherence marks a deviation from classical physics, and has been studied as a resource for metrology and quantum computation. Finding reliable and effective methods for assessing its presence is then highly desirable. Coherence witnesses rely on measuring observables whose outcomes can guarantee that a state is not diagonal in a known reference basis. Here we experimentally measure a novel type of coherence witness that uses pairwise state comparisons to identify superpositions in a basis-independent way. Our experiment uses a single interferometric set-up to simultaneously measure the three pairwise overlaps among three single-photon states via Hong-Ou-Mandel tests. Besides coherence witnesses, we show the measurements also serve as a Hilbert-space dimension witness. Our results attest to the effectiveness of pooling many two-state comparison tests to ascertain various relational properties of a set of quantum states., Comment: 10 pages, 7 figures

Self-testing is a method of quantum state and measurement estimation that does not rely on assumptions about the inner working of the used devices. Its experimental realization has been limited to sources producing single quantum states so far. In this work, we experimentally implement two significant building blocks of a quantum network involving two independent sources, i.e. a parallel configuration in which two parties share two copies of a state, and a tripartite configuration where a central node shares two independent states with peripheral nodes. Then, by extending previous self-testing techniques we provide device-independent lower bounds on the fidelity between the generated states and an ideal state made by the tensor product of two maximally entangled two-qubit states. Given its scalability and versatility, this technique can find application in the certification of larger networks of different topologies, for quantum communication and cryptography tasks and randomness generation protocols.

Quantum key distribution---exchanging a random secret key relying on a quantum mechanical resource---is the core feature of secure quantum networks. Entanglement-based protocols offer additional layers of security and scale favorably with quantum repeaters, but the stringent requirements set on the photon source have made their use situational so far. Semiconductor-based quantum emitters are a promising solution in this scenario, ensuring on-demand generation of near-unity-fidelity entangled photons with record-low multi-photon emission, the latter feature countering some of the best eavesdropping attacks. Here we first employ a quantum dot to experimentally demonstrate a modified Ekert quantum key distribution protocol with two quantum channel approaches: both a 250 meter long single mode fiber and in free-space, connecting two buildings within the campus of Sapienza University in Rome. Our field study highlights that quantum-dot entangled-photon sources are ready to go beyond laboratory experiments, thus opening the way to real-life quantum communication., Comment: The first two authors contributed equally to this work. 7 pages, 3 figures

Instrumental variables allow the estimation of cause and effect relations even in presence of unobserved latent factors, thus providing a powerful tool for any science wherein causal inference plays an important role. More recently, the instrumental scenario has also attracted increasing attention in quantum physics, since it is related to the seminal Bell's theorem and in fact allows the detection of even stronger quantum effects, thus enhancing our current capabilities to process information and becoming a valuable tool in quantum cryptography. In this work, we further explore this bridge between causality and quantum theory and apply a technique, originally developed in the field of quantum foundations, to express the constraints implied by causal relations in the language of graph theory. This new approach can be applied to any causal model containing a latent variable. Here, by focusing on the instrumental scenario, it allows us to easily reproduce known results as well as obtain new ones and gain new insights on the connections and differences between the instrumental and the Bell scenarios.

Photon indistinguishability plays a fundamental role in information processing, with applications such as linear-optical quantum computation and metrology. It is then necessary to develop appropriate tools to quantify the amount of this resource in a multiparticle scenario. Here we report a four-photon experiment in a linear-optical interferometer designed to simultaneously estimate the degree of indistinguishability between three pairs of photons. The interferometer design dispenses with the need of heralding for parametric down-conversion sources, resulting in an efficient and reliable optical scheme. We then use a recently proposed theoretical framework to quantify genuine four-photon indistinguishability, as well as to obtain bounds on three unmeasured two-photon overlaps. Our findings are in high agreement with the theory, and represent a new resource-effective technique for the characterization of multiphoton interference., Comment: 8+8 pages, 5+5 figures

The intrinsic random nature of quantum physics offers novel tools for the generation of random numbers, a central challenge for a plethora of fields. Bell non-local correlations obtained by measurements on entangled states allow for the generation of bit strings whose randomness is guaranteed in a device-independent manner, i.e. without assumptions on the measurement and state-generation devices. Here, we generate this strong form of certified randomness on a new platform: the so-called instrumental scenario, which is central to the field of causal inference. First, we theoretically show that certified random bits, private against general quantum adversaries, can be extracted exploiting device-independent quantum instrumental-inequality violations. To that end, we adapt techniques previously developed for the Bell scenario. Then, we experimentally implement the corresponding randomness-generation protocol using entangled photons and active feed-forward of information. Moreover, we show that, for low levels of noise, our protocol offers an advantage over the simplest Bell-nonlocality protocol based on the Clauser-Horn-Shimony-Holt inequality., Comment: Modified Supplementary Information: removed description of extractor algorithm introduced by arXiv:1212.0520. Implemented security of the protocol against general adversarial attacks

Entanglement distribution between distant parties is one of the most important and challenging tasks in quantum communication. Distribution of photonic entangled states using optical fiber links is a fundamental building block towards quantum networks. Among the different degrees of freedom, orbital angular momentum (OAM) is one of the most promising due to its natural capability to encode high dimensional quantum states. In this article, we experimentally demonstrate fiber distribution of hybrid polarization-vector vortex entangled photon pairs. To this end, we exploit a recently developed air-core fiber which supports OAM modes. High fidelity distribution of the entangled states is demonstrated by performing quantum state tomography in the polarization-OAM Hilbert space after fiber propagation, and by violations of Bell inequalities and multipartite entanglement tests. The present results open new scenarios for quantum applications where correlated complex states can be transmitted by exploiting the vectorial nature of light.

Inferring causal relations from experimental observations is of primal importance in science. Instrumental tests provide an essential tool for that aim, as they allow one to estimate causal dependencies even in the presence of unobserved common causes. In view of Bell's theorem, which implies that quantum mechanics is incompatible with our most basic notions of causality, it is of utmost importance to understand whether and how paradigmatic causal tools obtained in a classical setting can be carried over to the quantum realm. Here we show that quantum effects imply radically different predictions in the instrumental scenario. Among other results, we show that an instrumental test can be violated by entangled quantum states. Furthermore, we demonstrate such violation using a photonic set-up with active feed-forward of information, thus providing an experimental proof of this new form of non-classical behaviour. Our findings have fundamental implications in causal inference and may also lead to new applications of quantum technologies., Comment: Main manuscript (10 pages) + Supplementary Information (8 pages)

Quantum tomography is currently the mainly employed method to assess the information of a system and therefore plays a fundamental role when trying to characterize the action of a particular channel. Nonetheless, quantum tomography requires the trust that the devices used in the laboratory perform state generation and measurements correctly. This work is based on the theoretical framework for the device-independent inference of quantum channels that was recently developed and experimentally implemented with superconducting qubits in [Dall'Arno, Buscemi, Vedral, arXiv:1805.01159] and [Dall'Arno, Brandsen, Buscemi, PRSA 473, 20160721 (2017)]. Here, we present a complete experimental test on a photonic setup of two device-independent quantum channels falsification and characterization protocols to analyze, validate, and enhance the results obtained by conventional quantum process tomography. This framework has fundamental implications in quantum information processing and may also lead to the development of new methods removing the assumptions typically taken for granted in all the previous protocols.

Wave-particle duality has long been considered a fundamental signature of the non-classical behavior of quantum phenomena, specially in a delayed choice experiment (DCE), where the experimental setup revealing either the particle or wave nature of the system is decided after the system has entered the apparatus. However, as counter-intuitive as it might seem, usual DCEs do have a simple causal explanation. Here, we take a different route and under a natural assumption about the dimensionality of the system under test, we present an experimental proof of the non-classicality of a DCE based on the violation of a dimension witness inequality. Our conclusion is reached in a device-independent and loophole-free manner, that is, based solely on the observed data and without the need on any assumptions about the measurement apparatus.

Quantum teleportation establishes a correspondence between an entangled state shared by two separate par- ties that can communicate classically and the presence of a quantum channel connecting the two parties. The standard benchmark for quantum teleportation, based on the average fidelity between the input and output states, indicates that some entangled states do not lead to channels which can be certified to be quantum. It was re- cently shown that if one considers a finer-tuned witness, then all entangled states can be certified to produce a non-classical teleportation channel. Here we experimentally demonstrate a complete characterization of a new family of such witnesses, of the type proposed in Phys. Rev. Lett. 119, 110501 (2017) under different con- ditions of noise. Furthermore, we show non-classical teleportation using quantum states that can not achieve average teleportation fidelity above the classical limit. Our results have fundamental implications in quantum information protocols and may also lead to new applications and quality certification of quantum technologies., Comment: 5 pages + Supp. Materials

The number of parameters describing a quantum state is well known to grow exponentially with the number of particles. This scaling clearly limits our ability to do tomography to systems with no more than a few qubits and has been used to argue against the universal validity of quantum mechanics itself. However, from a computational learning theory perspective, it can be shown that, in a probabilistic setting, quantum states can be approximately learned using only a linear number of measurements. Here we experimentally demonstrate this linear scaling in optical systems with up to 6 qubits. Our results highlight the power of computational learning theory to investigate quantum information, provide the first experimental demonstration that quantum states can be "probably approximately learned" with access to a number of copies of the state that scales linearly with the number of qubits, and pave the way to probing quantum states at new, larger scales., Comment: 11 pages, 6 figures

Structured photons are nowadays an interesting resource in classical and quantum optics due to the richness of properties they show under propagation, focusing and in their interaction with matter. Vectorial modes of light in particular, a class of modes where the polarization varies across the beam profile, have already been used in several areas ranging from microscopy to quantum information. One of the key ingredients needed to exploit the full potential of complex light in quantum domain is the control of quantum interference, a crucial resource in fields like quantum communication, sensing and metrology. Here we report a tunable photon-photon interference between vectorial modes of light. We demonstrate how a properly designed spin-orbit device can be used to control quantum interference between vectorial modes of light by simply adjusting the device parameters and no need of interferometric setups. We believe our result can find applications in fundamental research and quantum technologies based on structured light by providing a new tool to control quantum interference in a compact, efficient and robust way.

In classical physics, properties of the objects exist independently on the context, i.e. whether and how measurements are performed. Quantum physics showed this assumption to be wrong and that Nature is indeed "contextual". Contextuality has been observed in the simplest physical systems such as single particles, and plays fundamental roles in quantum computation advantage. Here, we demonstrate for the first time quantum contextuality in an integrated photonic chip. The chip implements different combinations of measurements on a single photon delocalized on four distinct spatial modes. We show violations of a CHSH-like non-contextuality inequality by 14 standard deviations. This paves the way to compact and portable devices for contextuality-based quantum-powered protocols.

Non-classical correlations arising in complex quantum networks are attracting growing interest, both from a fundamental perspective and for potential applications in information processing. In particular, in an entanglement swapping scenario a new kind of correlations arise, the so-called nonbilocal correlations that are incompatible with local realism augmented with the assumption that the sources of states used in the experiment are independent. In practice, however, bilocality tests impose strict constraints on the experimental setup and in particular to presence of shared reference frames between the parties. Here, we experimentally address this point showing that false positive nonbilocal quantum correlations can be observed even though the sources of states are independent. To overcome this problem, we propose and demonstrate a new scheme for the violation of bilocality that does not require shared reference frames and thus constitute an important building block for future investigations of quantum correlations in complex networks., Comment: 10 pages

Bell's theorem was a cornerstone for our understanding of quantum theory, and the establishment of Bell non-locality played a crucial role in the development of quantum information. Recently, its extension to complex networks has been attracting a growing attention, but a deep characterization of quantum behaviour is still missing for this novel context. In this work we analyze quantum correlations arising in the bilocality scenario, that is a tripartite quantum network where the correlations between the parties are mediated by two independent sources of states. First, we prove that non-bilocal correlations witnessed through a Bell-state measurement in the central node of the network form a subset of those obtainable by means of a separable measurement. This leads us to derive the maximal violation of the bilocality inequality that can be achieved by arbitrary two-qubit quantum states and arbitrary projective separable measurements. We then analyze in details the relation between the violation of the bilocality inequality and the CHSH inequality. Finally, we show how our method can be extended to n-locality scenario consisting of n two-qubit quantum states distributed among n+1 nodes of a star-shaped network., Comment: 13 pages, 2 figures

Non-locality stands nowadays not only as one of the cornerstones of quantum theory, but also plays a crucial role in quantum information processing. Several experimental investigations of nonlocality have been carried out over the years. In spite of their fundamental relevance, however, all previous experiments do not consider a crucial ingredient that is ubiquitous in quantum networks: the fact that correlations between distant parties are mediated by several, typically independent, sources of quantum states. Here, using a photonic setup we investigate a quantum network consisting of three spatially separated nodes whose correlations are mediated by two independent sources. This scenario allows for the emergence of a new kind of non-local correlations that we experimentally witness by violating a novel Bell inequality. Our results provide the first experimental proof-of-principle of generalizations of Bell's theorem for networks, a topic that has attracted growing attention and promises a novel route for quantum communication protocols., Comment: 7 pages, 4 figures + 13 pages Supplementary Information

Greenberger-Horne-Zeilinger (GHZ) states and their mixtures exhibit fascinating properties. A complete basis of GHZ-states can be constructed by properly choosing local basis rotations. We demonstrate this experimentally for the Hilbert space C2x4 by entangling two photons in polarisation and orbital angular momentum. Mixing GHZ-states unmasks different entanglement features based on their particular local geometrical connectedness. In particular, a specific GHZ-state in a complete orthonormal basis has a twin GHZ-state for which equally mixing leads to full separability in opposition to any other basis-state. Exploiting these local geometrical relations provides a toolbox for generating specific types of multipartite entanglement, each providing different benefits in outperforming classical devices. Our experiment, based on hybrid entangled entanglement, investigates these GHZs properties showing a good stability and fidelity and allowing a scaling in degrees of freedom and advanced operational manipulations., Comment: 8 pages, 4 figures

Light beams having a vectorial field structure - or polarization - that varies over the transverse profile and a central optical singularity are called vector-vortex (VV) beams and may exhibit specific properties, such as focusing into "light needles" or rotation invariance, with applications ranging from microscopy and light trapping to communication and metrology. Individual photons in such beams exhibit a form of single-particle quantum entanglement between different degrees of freedom. On the other hand, the quantum states of two photons can be also entangled with each other. Here we combine these two concepts and demonstrate the generation of quantum entanglement between two photons that are both in VV states - a new form of quantum "entangled entanglement". This result may lead to quantum-enhanced applications of VV beams as well as to quantum-information protocols fully exploiting the vectorial features of light.

Device-independent (DI) quantum communication will require a loophole-free violation of Bell inequalities. In typical scenarios where line-of-sight between the communicating parties is not available, it is convenient to use energy-time entangled photons due to intrinsic robustness while propagating over optical fibers. Here we show an energy-time Clauser-Horne-Shimony-Holt Bell inequality violation with two parties separated by 3.7 km over the deployed optical fiber network belonging to the University of Concepci\'on in Chile. Remarkably, this is the first Bell violation with spatially separated parties that is free of the post-selection loophole, which affected all previous in-field long-distance energy-time experiments. Our work takes a further step towards a fiber-based loophole-free Bell test, which is highly desired for secure quantum communication due to the widespread existing telecommunication infrastructure., Comment: 5 pages, 3 figures. Matches published version