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Free-electron lasers (FELs) are the world's most brilliant light sources with rapidly evolving technological capabilities in terms of ultrabright and ultrashort pulses over a large range of accessible photon energies. Their revolutionary and innovative developments have opened new fields of science regarding nonlinear light-matter interaction, the investigation of ultrafast processes from specific observer sites, and approaches to imaging matter with atomic resolution. A core aspect of FEL science is the study of isolated and prototypical systems in the gas phase with the possibility of addressing well-defined electronic transitions or particular atomic sites in molecules. Notably for polarization-controlled short-wavelength FELs, the gas phase offers new avenues for investigations of nonlinear and ultrafast phenomena in spin orientated systems, for decoding the function of the chiral building blocks of life as well as steering reactions and particle emission dynamics in otherwise inaccessible ways. This roadmap comprises descriptions of technological capabilities of facilities worldwide, innovative diagnostics and instrumentation, as well as recent scientific highlights, novel methodology and mathematical modeling. The experimental and theoretical landscape of using polarization controllable FELs for dichroic light-matter interaction in the gas phase will be discussed and comprehensively outlined to stimulate and strengthen global collaborative efforts of all disciplines.

The development of a new hard x-ray beamline I-TOMCAT equipped with a 1-meter-long short-period bulk high-temperature superconductor undulator (BHTSU) has been scheduled for the upgrade of the Swiss Light Source (SLS 2.0) at the Paul Scherrer Institute (PSI). The very hard x-ray source generated by the BHTSU will increase the brilliance at the beamline by over one order of magnitude in comparison to other state-of-the-art undulator technologies and allow experiments to be carried out with photon energies in excess of 60 keV. One of the key challenges for designing a 1-meter-long (100 periods) BHTSU is the large-scale simulation of the magnetization currents inside 200 staggered-array bulk superconductors. A feasible approach to simplify the electromagnetic model is to retain five periods from both ends of the 1-meter-long BHTSU, reducing the number of degrees of freedom (DOFs) to the scale of millions. In this paper, the theory of the recently-proposed 2D A-V formulation-based backward computation method is extended to calculate the critical state magnetization currents in the ten-period staggered-array BHTSU in 3D. The simulation results of the magnetization currents and the associated undulator field along the electron beam axis are compared with the well-known 3D H-formulation and the highly efficient 3D H-{\phi} formulation method, all methods showing excellent agreement with each other as well as with experimental results. The mixed H-{\phi} formulation avoids computing the eddy currents in the air subdomain and is significantly faster than the full H-formulation method, but is slower in comparison to the A-V formulation-based backward computation. Finally, the fastest and the most efficient A-V formulation in ANSYS 2020R1 Academic is adopted to optimize the integrals of the undulator field along the electron beam axis by optimizing the sizes of the end bulks., Comment: 19 pages, 12 figures

A backward computation method has been developed to accelerate modelling of the critical state magnetization current in a staggered-array bulk high-temperature superconducting (HTS) undulator. The key concept is as follows: i) a large magnetization current is first generated on the surface of the HTS bulks after rapid field-cooling (FC) magnetization; ii) the magnetization current then relaxes inwards step-by-step obeying the critical state model; iii) after tens of backward iterations the magnetization current reaches a steady state. The simulation results show excellent agreement with the H-formulation method for both the electromagnetic and electromagnetic-mechanical coupled analyses, but with significantly faster computation speed. Solving the FEA model with 1.8 million degrees of freedom (DOFs), the backward computation method takes less than 1.4 hours, an order of magnitude or higher faster than other state-of-the-art numerical methods. Finally, the models are used to investigate the influence of the mechanical stress on the distribution of the critical state magnetization current and the undulator field along the central axis., Comment: 12 pages, 7 figures

In this work we will introduce the A-V-A formulation based iterative algorithm method (IAM) for simulating the magnetization current of high temperature superconductors. This new method embedded in ANSYS can simulate the critical state model by forcing the trapped current density to the critical current density Jc for all meshed superconducting elements after each iterative load step, as well as simulate the flux creep model by updating the E-J power law based resistivity values. The simulation results of a disk-shaped ReBCO bulk during zero field cooling (ZFC) or field cooling (FC) magnetization agree well with the simulation results from using the H-formulation in COMSOL. The computation time is shortened by using the A-V formulation in superconductor areas and the A-formulation in non-superconductor areas. This iterative method is further proved friendly for adding ferromagnetic materials into the FEA model or taking into account the magnetic field-dependent or mechanical strain-related critical current density of the superconductors. The influence factors for the magnetization simulation, including the specified iterative load steps, the initial resistivity, the ramping time and the updating coefficient, are discussed in detail. The A-V-A formulation based IAM, implemented in ANSYS, shows its unique advantages in adjustable computation time, multi-frame restart analysis and easy-convergence.