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Non-yrast, excited states in neutron-rich $^{186}$W were populated via inelastic-scattering reactions using beams of $^{136}$Xe nuclei accelerated to 725 and 800 MeV. Levels populated in the reactions were investigated via particle-$ \gamma $ coincidence techniques using the Gammasphere array of High-Purity Germanium detectors and the compact heavy-ion counter, CHICO2. The $ K^{\pi} = 2 ^{+} $ ($\gamma$), $ K^{\pi} = 0^{+}$ and $ K^{\pi} = 2^{-} $ (octupole) rotational side bands were extended to spins $ 14\hbar $, $ 12\hbar $, and $ 13\hbar $, respectively. A staggering pattern observed in the energies of levels in the $ K^{\pi} = 2^{+} $ band was found to be consistent with a potential that gets softer to vibration in the $ \gamma $ degree of freedom with increasing spin. The odd-even staggering of states in the $ K^{\pi} = 2^{-}$ band was found to exhibit a phase opposite to that seen in the $ \gamma $ band; an effect most probably associated with Coriolis coupling to other, unobserved octupole vibrational bands in $^{186}$W., Comment: 14 pages, 16 figures

Employing the Argonne Fragment Mass Analyzer and the implantation-decay-decay correlation technique, a weak 0.50(21)% proton decay branch was identified in 108I for the first time. The 108I proton-decay width is consistent with a hindered l = 2 emission, suggesting a d 5 2 origin. Using the extracted 108I proton-decay Q value of 597(13) keV, and the Q α values of the 108I and 107Te isotopes, a proton-decay Q value of 510(20) keV for 104Sb was deduced. Similarly to the 112,113Cs proton-emitter pair, the Q p ( I 108 ) value is lower than that for the less-exotic neighbor 109I, possibly due to enhanced proton-neutron interactions in N ≈ Z nuclei. In contrast, the present Q p ( Sb 104 ) is higher than that of 105Sb, suggesting a weaker interaction energy. For the present Q p ( Sb 104 ) value, network calculations with the one-zone X-ray burst model Mazzocchi et al. (2007) [18] predict no significant branching into the Sn-Sb-Te cycle at 103Sn.

The astrophysical $^{25}\mathrm{Al}(p,\ensuremath{\gamma})\phantom{\rule{0.16em}{0ex}}^{26}\mathrm{Si}$ reaction represents one of the key remaining uncertainties in accurately modeling the abundance of radiogenic $^{26}\mathrm{Al}$ ejected from classical novae. Specifically, the strengths of key proton-unbound resonances in $^{26}\mathrm{Si}$, that govern the rate of the $^{25}\mathrm{Al}(p,\ensuremath{\gamma})$ reaction under explosive astrophysical conditions, remain unsettled. Here, we present a detailed spectroscopy study of the $^{26}\mathrm{Si}$ mirror nucleus $^{26}\mathrm{Mg}$. We have measured the lifetime of the ${3}^{+}$, 6.125-MeV state in $^{26}\mathrm{Mg}$ to be $19(3)\phantom{\rule{0.28em}{0ex}}\mathrm{fs}$ and provide compelling evidence for the existence of a ${1}^{\ensuremath{-}}$ state in the $T=1,\phantom{\rule{0.28em}{0ex}}A=26$ system, indicating a previously unaccounted for $\ensuremath{\ell}=1$ resonance in the $^{25}\mathrm{Al}(p,\ensuremath{\gamma})$ reaction. Using the presently measured lifetime, together with the assumption that the likely ${1}^{\ensuremath{-}}$ state corresponds to a resonance in the $^{25}\mathrm{Al}+p$ system at 435.7(53) keV, we find considerable differences in the $^{25}\mathrm{Al}(p,\ensuremath{\gamma})$ reaction rate compared to previous works. Based on current nova models, we estimate that classical novae may be responsible for up to $\ensuremath{\approx}15%$ of the observed galactic abundance of $^{26}\mathrm{Al}$.

A novel approach for isomer depletion in ion-atom collisions is proposed and considered theoretically. Analyses are performed for the depletion of the ^{93m}Mo isomer for which an unexpectedly large probability was measured in the beam-based experiment of Chiara et al. [Nature (London) 554, 216 (2018)NATUAS0028-083610.1038/nature25483]. The subsequent attempt at a theoretical description based on state-of-the-art atomic theory did not reproduce the experimental result [Wu et al., Phys. Rev. Lett. 122, 212501 (2019)PRLTAO0031-900710.1103/PhysRevLett.122.212501] and showed a dramatic disagreement with the experiment (by many orders of magnitude). This conflict calls for further research on the nature of isomer depletion mechanisms occurring in atomic processes. Here, we propose to consider the ^{93m}Mo isomer depletion as the nuclear excitation by electron capture in resonant transfer process taking into account the momentum distribution of the target electrons. Although our results only slightly shift the upper theoretical limit for the total ^{93m}Mo isomer depletion probability toward the experimental value, they show the importance of considering the Compton profile in the theoretical description, in particular for the L shell, for which the depletion probability increases by many orders of magnitude.

The 92-keV resonance in the 25Mg ( p , γ ) 26 Al reaction plays a key role in the production of 26Al at astrophysical burning temperatures of ≈100 MK in the Mg-Al cycle. However, the state can decay to feed either the ground, 26 g Al, or isomeric state, 26 m Al. It is the ground state that is critical as the source of cosmic γ rays. It is therefore important to precisely determine the ground-state branching fraction f 0 of this resonance. Here we report on the identification of four γ-ray transitions from the 92-keV resonance, and determine the spin of the state and its ground-state branching fraction f 0 = 0.52 ( 2 ) s t a t ( 6 ) s y s t . The f 0 value is the most precise reported to date, and at the lower end of the range of previously adopted values, implying a lower production rate of 26 g Al and its cosmic 1809-keV γ rays.

A novel approach for isomer depletion in ion-atom collisions is proposed and considered theoretically. Analyses are performed for the depletion of the ^{93m}Mo isomer for which an unexpectedly large probability was measured in the beam-based experiment of Chiara et al. [Nature (London) 554, 216 (2018)NATUAS0028-083610.1038/nature25483]. The subsequent attempt at a theoretical description based on state-of-the-art atomic theory did not reproduce the experimental result [Wu et al., Phys. Rev. Lett. 122, 212501 (2019)PRLTAO0031-900710.1103/PhysRevLett.122.212501] and showed a dramatic disagreement with the experiment (by many orders of magnitude). This conflict calls for further research on the nature of isomer depletion mechanisms occurring in atomic processes. Here, we propose to consider the ^{93m}Mo isomer depletion as the nuclear excitation by electron capture in resonant transfer process taking into account the momentum distribution of the target electrons. Although our results only slightly shift the upper theoretical limit for the total ^{93m}Mo isomer depletion probability toward the experimental value, they show the importance of considering the Compton profile in the theoretical description, in particular for the L shell, for which the depletion probability increases by many orders of magnitude.

The beta-decay of Zn-81 to the neutron magic N = 50 nucleus Ga-81, with only three valence protons with respect to Ni-78, was investigated. The study was performed at the ISOLDE facility at CERN by means of gamma spectroscopy. The 81Zn half-life was determined to be T-1/2 = 290(4) ms while the beta-delayed neutron emission probability was measured as P-n = 23(4)%. The analysis of the beta-gated gamma-ray singles and gamma-gamma coincidences from the decay of Zn-81 provides 47 new levels and 70 new transitions in Ga-81. The beta(-)n decay of Zn-81 was observed and a new decay scheme into the odd-odd Ga-80 nucleus was established. The half-lives of the first and second excited states of Ga-81 were measured via the fast-timing method using LaBr3(Ce) detectors. The level scheme and transition rates are compared to large-scale shell-model calculations. The low-lying structure of (81)Gais interpreted in terms of the coupling of the three valence protons outside the doubly magic Ni-78 core.

Rotational structures have been measured using the Jurogam II and GAMMASPHERE arrays at low spin following the Gd155(α,2n)Dy157 and Nd148(C12,5n)Dy155 reactions at 25 and 65 MeV, respectively. We report high-K bands, which are conjectured to be the first candidates of a Kπ=2+γ vibrational band, built on the [505]11/2− neutron orbital, in both odd-ADy155,157 isotopes. The coupling of the first excited K=0+ states or the so-called β vibrational bands at 661 and 676 keV in Dy154 and Dy156 to the [505]11/2− orbital, to produce a Kπ=11/2− band, was not observed in both Dy155 and Dy157, respectively. The implication of these findings on the interpretation of the first excited 0+ states in the core nuclei Dy154 and Dy156 are also discussed.

Beta-delayed neutron emission is being studied by detecting the β particles and recoiling ions emerging from the Beta-decay Paul Trap. For β decays to the ground state or γ -emitting states of the daughter nucleus, the fraction of recoiling ions which reach the ion detector in coincidence with a β particle has been determined for 134, 135Sb, 137, 138, 140I, and 144, 145Cs. This value is needed for the determination of the β -delayed neutron emission branching ratio solely from the recoil-ion time-of-flight (TOF) spectrum. The β -particle energy and recoil-ion TOF spectra were used to constrain a simple decay model, which can be used to determine the detection efficiency. The method is compared to simulations to estimate the uncertainty introduced by incomplete knowledge of the decay pattern. By fitting the simulation results to several β -ion coincidence properties measured during the experiment, the fraction of ions which reach the microchannel plate detector can be determined to within ± 4 % . This result opens the possibility of using the recoil-ion TOF spectra for high precision β -delayed neutron branching-ratio measurements.

The structure of 71Zn was investigated by one-neutron transfer and heavy-ion induced complex (deep-inelastic) reactions using the GRETINA-CHICO2 and the Gammasphere setups, respectively. The observed inversion between the 9/2+ and 1/2− states is explained in terms of the role of neutron pairing correlations. Non-collective sequences of levels were delineated above the 9/2+ isomeric state. These are interpreted as being associated with a modest oblate deformation in the framework of Monte-Carlo shell-model calculations carried out with the A3DA-m Hamiltonian in the p f g 9 / 2 d 5 / 2 valence space. Similarities with the structure of Ni 40 28 68 were observed and the shape-coexistence mechanism in the N = 40 region of neutron-rich nuclei is discussed in terms of the so-called Type-II shell evolution, with an emphasis on proton–neutron correlations between valence nucleons, especially those involving the shape-driving g 9 / 2 neutron orbital.

A detailed study of the $\ensuremath{\beta}$-delayed neutron emission properties of $^{137,138}\mathrm{I}$ and $^{144,145}\mathrm{Cs}$ has been performed by confining ions in the Beta-decay Paul Trap. The daughter ions following $\ensuremath{\beta}$ decay emerge from the trapped-ion cloud with negligible scattering allowing reconstruction of the recoil-ion energy from the time of flight. From this information, the neutron-emission branching ratios and neutron-energy spectra were deduced. The results for the $^{137}\mathrm{I}$ and $^{144,145}\mathrm{Cs}$ decays are in agreement with previous results performed using direct neutron-detection techniques. In the case of $^{138}\mathrm{I}$, a branching ratio of 6.18(50)% is obtained, yielding a value consistent with the more recent results, which are a factor of two larger than measurements made prior to 1978.

Beta-delayed-neutron ($\ensuremath{\beta}n$) spectroscopy was performed using the Beta-decay Paul Trap and an array of radiation detectors. The $\ensuremath{\beta}n$ branching ratios and energy spectra for $^{135,136}\mathrm{Sb}$ and $^{140}\mathrm{I}$ were obtained by measuring the time of flight of recoil ions emerging from the trapped ion cloud. These nuclei are located at the edge of an isotopic region identified as having $\ensuremath{\beta}n$ branching ratios that impact the $r$-process abundance pattern around the $A\ensuremath{\approx}130$ peak. For $^{135,136}\mathrm{Sb}$ and $^{140}\mathrm{I}, \ensuremath{\beta}n$ branching ratios of $14.6(13)%, 17.6(29)%$, and $7.6(28)%$ were determined, respectively. The $\ensuremath{\beta}n$ energy spectra obtained for $^{135}\mathrm{Sb}$ and $^{140}\mathrm{I}$ are compared with results from direct neutron measurements, and the $\ensuremath{\beta}n$ energy spectrum for $^{136}\mathrm{Sb}$ has been measured for the first time.

Garrett et al. systematically investigated band-crossing frequencies resulting from the rotational alignment of the first pair of i13/2 neutrons (AB) in rare-earth nuclei. In that study, evidence was found for an odd-even neutron number dependence attributed to changes in the strength of neutron pairing correlations. The present paper carries out a similar investigation at higher rotational frequencies for the second pair of aligning i13/2 neutrons (BC). Again, a systematic difference in band-crossing frequencies is observed between odd-N and even-N Er, Yb, Hf, and W nuclei, but in the BC case, it is opposite to the AB neutron-number dependence. These results are discussed in terms of a reduction of neutron pairing correlations at high rotational frequencies and of the effects of Pauli blocking on the pairing field by higher-seniority configurations. Also playing a significant role are the changes in deformation with proton and neutron numbers, the changes in location of single-particle orbitals as a function of quadrupole deformation, and the position of the Fermi surface with regard to the various ω components of the neutron i13/2 shell.

The 22Ne($ \alpha$, n) reaction is expected to provide the dominant neutron source for the weak s process in massive stars and intermediate-mass (IM) Asymptotic Giant Branch (AGB) stars. However, the production of neutrons in such environments is hindered by the competing 22Ne($\alpha$,$\gamma$)26Mg reaction. Here, the 11B(16O,p) fusion-evaporation reaction was used to identify $\gamma$-decay transitions from 22Ne + $\alpha$ resonant states in 26Mg. Spin-parity restrictions have been placed on a number of $ \alpha$-unbound excited states in 26 Mg and their role in the 22Ne($\alpha$,$\gamma$)26Mg reaction has been investigated. In particular, a suspected natural-parity resonance at Ec.m. = 557(3) keV, that lies above the neutron threshold in 26Mg, and is known to exhibit a strong $ \alpha$-cluster character, was observed to $ \gamma$ decay. Furthermore, a known resonance at $ E_{c.m.} = 466(4)$ keV has been definitively assigned 2+ spin and parity. Consequently, uncertainties in the 22Ne($ \alpha$,$ \gamma$) stellar reaction rate have been reduced by a factor of ∼ 20 for temperatures ∼ 0.2 GK.

Following the first experimental observation of $^{93m}\mathrm{Mo}$ isomer depletion via nuclear excitation by electron capture (NEEC), we consider another experimental scenario related to the $^{242m}\mathrm{Am}$ isomer for which the probability of the NEEC process is expected to be even higher than for the $^{93m}\mathrm{Mo}$ isomer. The optimum experimental conditions for the production and depletion of the $^{242m}\mathrm{Am}$ isomer in a beam-based scenario are discussed. The relevant beam-target reaction cross sections have been calculated striving to ensure effective production of the $^{242m}\mathrm{Am}$ isomer. Kinetic energies required for the NEEC process to occur have been predicted for the $n=5$, 6, and 7 subshells of $^{242m}\mathrm{Am}$ ions and combined with available ion charge states at subsequent stages of the ion stopping process. The NEEC resonance strengths have been estimated for the partial contributions of individual subshells to the whole NEEC process.

The atomic nucleus and its electrons are often thought of as independent systems that are held together in the atom by their mutual attraction. Their interaction, however, leads to other important effects, such as providing an additional decay mode for excited nuclear states, whereby the nucleus releases energy by ejecting an atomic electron instead of by emitting a γ-ray. This 'internal conversion' has been known for about a hundred years and can be used to study nuclei and their interaction with their electrons. In the inverse process-nuclear excitation by electron capture (NEEC)-a free electron is captured into an atomic vacancy and can excite the nucleus to a higher-energy state, provided that the kinetic energy of the free electron plus the magnitude of its binding energy once captured matches the nuclear energy difference between the two states. NEEC was predicted in 1976 and has not hitherto been observed. Here we report evidence of NEEC in molybdenum-93 and determine the probability and cross-section for the process in a beam-based experimental scenario. Our results provide a standard for the assessment of theoretical models relevant to NEEC, which predict cross-sections that span many orders of magnitude. The greatest practical effect of the NEEC process may be on the survival of nuclei in stellar environments, in which it could excite isomers (that is, long-lived nuclear states) to shorter-lived states. Such excitations may reduce the abundance of the isotope after its production. This is an example of 'isomer depletion', which has been investigated previously through other reactions, but is used here to obtain evidence for NEEC.

We report the first observation of the ^{108}Xe→^{104}Te→^{100}Sn α-decay chain. The α emitters, ^{108}Xe [E_{α}=4.4(2) MeV, T_{1/2}=58_{-23}^{+106} μs] and ^{104}Te [E_{α}=4.9(2) MeV, T_{1/2}

Yrast and near-yrast levels up to an I=17ℏ spin value and a 6-MeV excitation energy have been delineated in the “two-neutron” 210Pb nucleus following deep-inelastic reactions involving 208Pb targets and a number of heavy-ion beams at energies ∼25% above the Coulomb barrier. The level scheme was established on the basis of multifold prompt and delayed coincidence relationships measured with the Gammasphere array. In addition to the previously known states, many new levels were identified. For most of the strongly populated states, spin-parity assignments are proposed on the basis of angular distributions. The reinvestigation of the ν(g9/2)2, 8+ isomeric decay results in the firm identification of the low-energy E2 transitions involved in the 8+→6+→4+ cascade, and in a revised 6+ level half-life of 92(10) ns, nearly a factor of 2 longer than previously measured. Among the newly identified states figure spin I=4–10ℏ levels associated with the νg9/2i11/2 multiplet, as well as yrast states involving νg9/2j15/2, νi11/2j15/2, and ν(j15/2)2 neutron couplings. The highest-spin excitations are understood as 1p−1h core excitations and the yrast population is found to be fragmented to the extent that levels of spin higher than I=17ℏ could not be reached. Four E3 transitions are present in the 210Pb yrast decay; three of these involve the g9/2→j15/2 octupole component, as reflected in the 21(2) and >10 Weisskopf unit enhancements of the B(E3) rates of the first two. The fourth, 16+→13−E3 transition corresponds to the 3− core octupole excitation built on the νi11/2j15/2 state, in analogy to a similar E3 coupling to the νj15/2 level in 209Pb. Shell-model calculations performed for two-neutron states and 1p−1h 208Pb core excitations are in good agreement with the data. Evidence was found for the existence of a hitherto unknown high-spin β-decaying isomer in 210Tl. Shell-model calculations of the 210Tl levels suggest the possibility of a 11+ long-lived, β-decaying state, and the delayed yields observed in various reactions fit rather well with a 210Tl assignment.

A sequence of low-energy levels in _{32}^{78}Ge_{46} has been identified with spins and parity of 2^{+}, 3^{+}, 4^{+}, 5^{+}, and 6^{+}. Decays within this band proceed strictly through ΔJ=1 transitions, unlike similar sequences in neighboring Ge and Se nuclei. Above the 2^{+} level, members of this sequence do not decay into the ground-state band. Moreover, the energy staggering of this sequence has the phase that would be expected for a γ-rigid structure. The energies and branching ratios of many of the levels are described well by shell-model calculations. However, the calculated reduced transition probabilities for the ΔJ=2 in-band transitions imply that they should have been observed, in contradiction with the experiment. Within the calculations of Davydov, Filippov, and Rostovsky for rigid-triaxial rotors with γ=30°, there are sequences of higher-spin levels connected by strong ΔJ=1 transitions which decay in the same manner as those observed experimentally, yet are calculated at too high an excitation energy.

Author(s): Lubna, RS; Tripathi, V; Tabor, SL; Tai, PL; Kravvaris, K; Bender, PC; Volya, A; Bouhelal, M; Chiara, CJ; Carpenter, MP; Janssens, RVF; Lauritsen, T; McCutchan, EA; Zhu, S; Clark, RM; Fallon, P; MacChiavelli, AO; Paschalis, S; Petri, M; Reviol, W; Sarantites, DG | Abstract: Excited states in the neutron-rich isotopes P33 and P34 were populated by the O18+O18 fusion-evaporation reaction at Elab=24 MeV. The Gammasphere array was used along with the Microball particle detector array to detect γ transitions in coincidence with the charged particles emitted from the compound nucleus S36. The use of Microball enabled the selection of the proton emission channel. It also helped in determining the exact position and energy of the emitted proton; this was later employed in kinematic Doppler corrections. 16 new transitions and 13 new states were observed in P33 and 21 γ rays and 20 energy levels were observed in P34 for the first time. The nearly 4π geometry of Gammasphere allowed the measurement of γ-ray angular distributions leading to spin assignments for many states. The experimental observations for both isotopes were interpreted with the help of shell-model calculations using the (0+1)ω PSDPF interaction. The calculations accounted for both the 0p-0h and 1p-1h states reasonably well and indicated that 2p-2h excitations might dominate the higher-spin configurations in both P33 and P34.

A sequence of low-energy levels in _{32}^{78}Ge_{46} has been identified with spins and parity of 2^{+}, 3^{+}, 4^{+}, 5^{+}, and 6^{+}. Decays within this band proceed strictly through ΔJ=1 transitions, unlike similar sequences in neighboring Ge and Se nuclei. Above the 2^{+} level, members of this sequence do not decay into the ground-state band. Moreover, the energy staggering of this sequence has the phase that would be expected for a γ-rigid structure. The energies and branching ratios of many of the levels are described well by shell-model calculations. However, the calculated reduced transition probabilities for the ΔJ=2 in-band transitions imply that they should have been observed, in contradiction with the experiment. Within the calculations of Davydov, Filippov, and Rostovsky for rigid-triaxial rotors with γ=30°, there are sequences of higher-spin levels connected by strong ΔJ=1 transitions which decay in the same manner as those observed experimentally, yet are calculated at too high an excitation energy.

The low-energy recoiling ions from the $\ensuremath{\beta}$ decay of $^{134}\mathrm{Sb}$ were studied by using the Beta-decay Paul Trap. Using this apparatus, singly charged ions were suspended in vacuum at the center of a detector array used to detect emitted $\ensuremath{\beta}$ particles, $\ensuremath{\gamma}$ rays, and recoil ions in coincidence. The recoil ions emerge from the trap with negligible scattering, allowing $\ensuremath{\beta}$-decay properties and the charge-state distribution of the daughter ions to be determined from the $\ensuremath{\beta}$-ion coincidences. First-forbidden $\ensuremath{\beta}$-decay theory predicts a $\ensuremath{\beta}\text{\ensuremath{-}}\ensuremath{\nu}$ correlation coefficient of nearly unity for the ${0}^{\ensuremath{-}}$ to ${0}^{+}$ transition from the ground state of $^{134}\mathrm{Sb}$ to the ground state of $^{134}\mathrm{Te}$. Although this transition was expected to have a nearly 100% branching ratio, an additional 17.2(52)% of the $\ensuremath{\beta}$-decay strength must populate high-lying excited states to obtain an angular correlation consistent with unity. The extracted charge-state distribution of the recoiling ions was compared with existing $\ensuremath{\beta}$-decay results and the average charge state was found to be consistent with the results from lighter nuclei.

We report the first observation of the 108Xe→104Te→100Sn α-decay chain. The α emitters, 108Xe [Eα=4.4(2) MeV, T1/2=58+106−23 μs] and 104Te [Eα=4.9(2) MeV, T1/2100Sn were produced using a fusion-evaporation reaction 54Fe(58Ni,4n)108Xe, and identified with a recoil mass separator and an implantation-decay correlation technique. This is the first time α radioactivity has been observed to a heavy self-conjugate nucleus. A previous benchmark for study of this fundamental decay mode has been the decay of 212Po into doubly magic 208Pb. Enhanced proton-neutron interactions in the N=Z parent nuclei may result in superallowed α decays with reduced α-decay widths significantly greater than that for 212Po. From the decay chain, we deduce that the α-reduced width for 108Xe or 104Te is more than a factor of 5 larger than that for 212Po.© 2018 American Physical Society

The existence of two close-lying nuclear states in ⁷³Ga has recently been experimentally determined: a 1/2⁻ spin-parity for the ground state was measured in a laser spectroscopy experiment, while a J_π = 3/2⁻ level was observed in transfer reactions. This scenario is supported by Coulomb excitation studies, which set a limit for the energy splitting of 0.8 keV. In this work, we report on the study of the excited structure of ⁷³Ga populated in the β decay of ⁷³Zn produced at ISOLDE, CERN. Using β-gated, γ-ray singles, and γ –γ coincidences, we have searched for energy differences to try to delimit the ground-state energy splitting, providing a more stringent energy difference limit. Three new half-lives of excited states in ⁷³Ga have been measured using the fast-timing ;method with LaBr₃(Ce) detectors. From our study, we help clarify the excited structure of ⁷³G and we extend the existing ⁷³Zn decay to ⁷³Ga with 8 new energy levels and 35 γ transitions. We observe a 195-keV transition consistent with a γ ray de-exciting a short-lived state in the β-decay parent ⁷³Zn.

Excited states in Re186 with spins up to J=12 were investigated in two separate experiments using W186(d,2n) reactions at beam energies of 12.5 and 14.5 MeV. Two- and threefold γ-ray coincidence data were collected using the CAESAR and CAGRA spectrometers, respectively, each composed of Compton-suppressed high-purity germanium detectors. Analysis of the data revealed rotational bands built on several two-quasiparticle intrinsic states, including a long-lived Kπ=(8+) isomer. Configuration assignments were supported by an analysis of in-band properties, such as gK-gR values. The excitation energies of the observed intrinsic states were compared with results from multi-quasiparticle blocking calculations, based on the Lipkin-Nogami pairing approach, that included contributions from the residual proton-neutron interactions.

The nucleus ${}^{208}$Pb provides an iconic test of the nuclear shell model because its 82 protons and 126 neutrons are both magic numbers. When excited levels are discovered and characterized, this nucleus provides a means to investigate the mechanisms responsible for the generation of angular momentum and, ultimately, for the development of collectivity. This experiment is a tour de force that reveals extensive new information on ${}^{208}$Pb about high-angular-momentum states, isomeric states, and collective states of octupole nature; thus it serves as a showcase for shell-model descriptions. Many of the states explored show good overall agreement with theory, but others at the highest energies reveal discrepancies, pointing to the need for improved calculations. Above the highest-lying ${28}^{-}$ isomer $\ensuremath{\gamma}$ transitions arising from yet higher spin levels could be identified in two separate experiments as displayed in the figure.

International audience; Neutron-rich isotopes are an important source of new information on nuclear physics. Specifically, the spin-isospin components in the nucleon-nucleon (NN) interaction, e.g., the proton-neutron tensor force, are expected to modify shell structure in exotic nuclei. These potential changes in the intrinsic shell structure are of fundamental interest. The study of the excitation energy of states corresponding to specific configurations in even-even isotopes, together with the single-particle character of the first excited states of odd-A, neutron-rich Ni isotopes, probes the evolution of the neutron orbitals around the Fermi surface as a function of the neutron number a step forward in the understanding of the region and the nature of the NN interaction at large N/Z ratios. In an experiment carried out at the National Superconducting Cyclotron Laboratory [1], new spectroscopic information was obtained for 68Ni and the distribution of single-particle strengths in 67,69Ni was characterized by means of single-neutron knockout from 68,70Ni secondary beams. The spectroscopic strengths, deduced from the measured partial cross sections to the individual states tagged by their de-exciting gamma rays, is used to identify and quantify configurations that involve neutron excitations across the N = 40 harmonic oscillator shell closure. The de-excitation γ rays were measured with the GRETINA tracking array [2]. The results challenge the validity of the most current shell-model Hamiltonians and effective interactions, highlighting shortcomings that cannot yet be explained. These results suggest that our understanding of the low-energy states in such nuclei is not complete and requires further investigation.

We present here a comprehensive analysis to understand the optimal atomic conditions for the first experimental observation of nuclear excitation by electron capture (NEEC) for the 6.85 h $^{93m}\mathrm{Mo}$ isomer with spin parity $21/{2}^{+}$. The NEEC process would provide an excitation from the long-lived isomer to a depletion level with spin parity $17/{2}^{+}$, which lies only 4.85 keV higher in energy, and is itself a shorter-lived isomer that subsequently decays, releasing a substantial amount of stored energy (2429.8 keV). The depletion level decays to a $13/{2}^{+}$ state through a 267.9-keV transition that offers the opportunity for identification of NEEC because it does not occur in the natural decay of the long-lived isomer. It has been shown that, for the proposed approach, high-precision atomic predictions are essential to understanding the proper physical conditions under which the experimental observation of the NEEC process will be possible using a beam-based scenario.

Fast-rotating N = 151 isotones 245 Pu, 247 Cm and 249 Cf have been studied through inelastic excitation and transfer reactions with radioactive targets. While all have a ground-state band built on a ν j 15 / 2 [ 734 ] 9 / 2 − Nilsson configuration, new excited bands have also been observed in each isotone. These odd- N excited bands allow a comparison of the alignment behavior for two different configurations, where the ν j 15 / 2 alignment is either blocked or allowed. The effect of higher order deformations is explored through cranking calculations, which help clarify the elusive nature of ν j 15 / 2 alignments.

New, low-lying levels in the odd-odd, N=Z nucleus 62Ga have been identified using a sensitive technique, where in-beam γ rays from short-lived nuclei are tagged with β decays following recoil mass identification. A comparison of the results with shell-model and IBM-4 calculations demonstrates good agreement between theory and experiment, with the majority of predicted low-lying, low-spin T=0 states now identified. There is a dramatic change in the level density at low excitation energies for the N=Z nucleus 62Ga when compared with neighbouring odd-odd Ga isotopes where, in contrast, the low-lying level structure is dominated by configurations with T=1 pairing interactions between excess neutrons. This illustrates the distinctively different aspects of nuclear structure exhibited by nuclei with N=Z. © 2013 Elsevier B.V.

States in $^{209}\mathrm{Tl}$ were populated using a multinucleon transfer reaction with a $^{136}\mathrm{Xe}$ beam impinging on a thick $^{208}\mathrm{Pb}$ target at $E=785$ MeV. The beam was pulsed at 825-ns intervals in order to perform isomer decay spectroscopy. The known ${J}^{\ensuremath{\pi}}=17/{2}^{+}$ isomer in $^{209}\mathrm{Tl}$ was located at 1228(4) keV and measured to have a half-life of ${T}_{1/2}=146(10)$ ns. A second isomer with ${J}^{\ensuremath{\pi}}=13/{2}^{+}$ was found to have ${T}_{1/2}=14(5)$ ns. The previously suggested low-energy X and Y transitions were found to have energies 57(2) and 47(2) keV respectively, while the measurement of conversion coefficients and a new decay path make the spin assignments below the isomers experimentally firm. Correlating the delayed $\ensuremath{\gamma}$ transitions with the prompt beam flash allowed the decay of states above the isomer to be found. The longer-lived isomer represents full alignment of the simplest two-particle, one-hole configuration and illuminates the remarkably weak coupling of the proton hole to the $^{210}\mathrm{Pb}$ core.

The first rotational sequences have been assigned to the odd-odd nucleus $^{168}\mathrm{Re}$. Coincidence relationships of these structures with rhenium x rays confirm the isotopic assignment, while arguments based on the $\ensuremath{\gamma}$-ray multiplicity ($K$-fold) distributions observed with the new bands lead to the mass assignment. Configurations for the two bands were determined through analysis of the rotational alignments of the structures and a comparison of the experimental $B(M1)/B(E2)$ ratios with theory. Tentative spin assignments are proposed for the $\ensuremath{\pi}{h}_{11/2}\ensuremath{\nu}{i}_{13/2}$ band, based on energy level systematics for other known sequences in neighboring odd-odd rhenium nuclei, as well as on systematics seen for the signature inversion feature that is well known in this region. The spin assignment for the $\ensuremath{\pi}{h}_{11/2}\ensuremath{\nu}({h}_{9/2}/{f}_{7/2})$ structure provides additional validation of the proposed spins and configurations for isomers in the $^{176}\mathrm{Au} \ensuremath{\rightarrow} ^{172}\mathrm{Ir}\ensuremath{\rightarrow}^{168}\mathrm{Re} \ensuremath{\alpha}$-decay chain.

The distribution of single-particle strength in 67,69Ni was characterized with one-neutron knockout reactions from intermediate-energy 68,70Ni secondary beams, selectively populating neutron-hole configurations at N = 39 and 41, respectively. The spectroscopic strengths deduced from the measured partial cross sections to the individual final states, as tagged by their γ-ray decays, are used to identify and quantify neutron configurations in the wave functions. While 69Ni compares well to shell-model predictions, the results for 67Ni challenge the validity of current effective shell-model Hamiltonians by revealing discrepancies that cannot be explained so far. These results suggest that our understanding of the low-lying states in the neutron-rich, semi-magic Ni isotopes may be incomplete and requires further investigation on both the experimental and theoretical sides.

{\bf Background:} Level sequences of rotational character have been observed in several nuclei in the $A=60$ mass region. The importance of the deformation-driving $\pi f_{7/2}$ and $\nu g_{9/2}$ orbitals on the onset of nuclear deformation is stressed.\\ {\bf Purpose:} A measurement was performed in order to identify collective rotational structures in the relatively neutron-rich $^{62}$Ni isotope. \\ {\bf Method:} The $^{26}$Mg($^{48}$Ca,2$\alpha$4$n\gamma$)$^{62}$Ni complex reaction at beam energies between 275 and 320~MeV was utilized. Reaction products were identified in mass ($A$) and charge ($Z$) with the Fragment Mass Analyzer (FMA) and $\gamma$ rays were detected with the Gammasphere array. \\ {\bf Results:} Two collective bands, built upon states of single-particle character, were identified and sizable deformation was assigned to both sequences based on the measured transitional quadrupole moments, herewith quantifying the deformation at high spin. \\ {\bf Conclusions:} Based on Cranked Nilsson-Strutinsky calculations and comparisons with deformed bands in the $A=60$ mass region, the two rotational bands are understood as being associated with configurations involving multiple $f_{7/2}$ protons and $g_{9/2}$ neutrons, driving the nucleus to sizable prolate deformation.

Here, the decay of a Kπ = 8– isomer in 244Pu and the collective band structures populating the isomer were studied using deep inelastic excitations with 47Ti and 208Pb beams, respectively. Precise measurements of M1/E2 branching ratios in the band confirm a 9/2–[734]νⓍ7/2+[624]ν configuration assignment for the isomer, validating the systematics of Kπ = 8–, two-quasineutron isomers observed in even-Z, N = 150 isotones. These isomers around the deformed shell gap at N = 152 provide critical benchmarks for theoretical predictions of single-particle energies in this gateway region to superheavy nuclei.

International audience; Superheavy nuclei exist solely due to quantum shell effects,which create a pocket in the potential-energy surface of the nucleus, thusproviding a barrier against spontaneous fission. Determining the height ofthe fission barrier and its angular-momentum dependence is important toquantify the role that microscopic shell corrections play in enhancing andextending the limits of nuclear stability. In this talk, the first measurement ofa fission barrier in the very heavy nucleus 254No will be presented.

An array of nine 811 cm3 LaBr3:Ce crystals coupled to photomultiplier tubes is used to detect γ rays induced from materials by neutrons emitted from a Deuterium-Tritium neutron generator. The accompanying digital data acquisition system has been developed to understand operational limits for remote detection of explosive contraband and analysis of material composition. Results are presented demonstrating current system performance, with the eventual goal of detecting a small (less than 5%) change in the composition of a material. Improvement expected over existing analog data collection systems are described along with discussion of the enhancements.

The neutron-rich nucleus $^{144}$Ba ($t_{1/2}$=11.5 s) is expected to exhibit some of the strongest octupole correlations among nuclei with mass numbers $A$ less than 200. Until now, indirect evidence for such strong correlations has been inferred from observations such as enhanced $E1$ transitions and interleaving positive- and negative-parity levels in the ground-state band. In this experiment, the octupole strength was measured directly by sub-barrier, multi-step Coulomb excitation of a post-accelerated 650-MeV $^{144}$Ba beam on a 1.0-mg/cm$^2$ $^{208}$Pb target. The measured value of the matrix element, $\langle 3_1^- \| \mathcal{M}(E3) \| 0_1^+ \rangle=0.65(^{+17}_{-23})$ $e$b$^{3/2}$, corresponds to a reduced $B(E3)$ transition probability of 48($^{+25}_{-34}$) W.u. This result represents an unambiguous determination of the octupole collectivity, is larger than any available theoretical prediction, and is consistent with octupole deformation., Comment: 5 pages, 2 figures, 1 table, Physical Review Letters 2016

The transition quadrupole moments. Q(t), of four weakly populated collective bands up to spin similar to 65h in Er-157,Er-158 have been measured to be similar to II eb demonstrating that these sequences are associated with large deformations. However, the data are inconsistent with calculated values from cranked Nilsson-Strutinsky calculations that predict the lowest energy triaxial shape to be associated with rotation about the short principal axis. The data appear to favor either a stable triaxial shape rotating about the intermediate axis or, alternatively, a triaxial shape with larger deformation rotating about the short axis. These new results challenge the present understanding of triaxiality in nuclei. (C) 2011 Elsevier B.V. All rights reserved. (Less)