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We present the results of a measurement of isotopic concentrations and atomic number ratio of a double-sided actinide target using α -spectroscopy and mass spectrometry. The double-sided actinide target, with predominantly 239Pu on one side and 235U on the other, was used in the fission Time Projection Chamber (fissionTPC) for a measurement of the neutron-induced fission cross-section ratio between the two isotopes. The measured atomic number ratio is needed to extract an absolute measurement fission cross-section ratio. The 239Pu/235U atom number ratio was measured with a combination of mass spectrometry and α -spectroscopy with a planar silicon detector achieving uncertainties of less than 1%. Different strategies for estimating isotopic concentration from the α -spectrum are presented to demonstrate the potential of these methods for non-destructive target assay. We found that a combination of fitting spectra with constraints from mass spectrometry, and summing counts in a region of the spectrum provided the most consistent results with the lowest uncertainty.

Properties of fission in $^{233}\mathrm{U}$ were measured at the Los Alamos Neutron Science Center at incident neutron energies from thermal to 40 MeV. Fragments were observed in coincidence by using a twin ionization chamber with Frisch grids. The average total kinetic energy released and fragment mass yields were determined by using the double energy analysis method based on conservation of mass and momentum. The experimental method was validated by using $^{232}\mathrm{Th}$ and absolute energy was calibrated by using thermal-neutron--induced fission of $^{235}\mathrm{U}$. This work incorporates novel applications of multi-chance fission channel cross sections and fission models to account for the complexities introduced by prompt neutron emission at high energy and extends results up to higher incident neutron energies than previously measured. Accurate experimental measurements of these parameters are necessary to better understand the fission process in isotopes central to the thorium fuel cycle.

The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) collaboration has performed measurements with a fission time projection chamber (fissionTPC) to study the fission process by reconstructing full three-dimensional tracks of fission fragments and other ionizing radiation. The amount of linear momentum imparted to the fissioning nucleus by the incident neutron can be inferred by measuring the opening angle between the fission fragments. Using this measured linear momentum, fission fragment angular distributions can be converted to the center-of-mass frame for anisotropy measurements. Angular anisotropy is an important experimental observable for understanding the quantum mechanical state of the fissioning nucleus and vital to determining detection efficiency for cross section measurements. Neutron linear momentum transfer to fissioning $^{235}$U, $^{238}$U, and $^{239}$Pu and fission fragment angular anisotropy of $^{235}$U and $^{238}$U as a function of neutron energies in the range 130 keV--250 MeV are presented.

Fission fragment angular distributions can provide an important constraint on fission theory, improving predictive fission codes, and are a prerequisite for a precise ratio cross section measurement. Available anisotropy data is sparse, especially at neutron energies above 5 MeV. For the first time, a three-dimensional tracking detector is employed to study fragment emission angles and provide a direct measurement of angular anisotropy. The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) collaboration has deployed the fission time projection chamber (fissionTPC) to measure nuclear data with unprecedented precision. The fission fragment anisotropy of $^{235}$U has been measured over a wide range of incident neutron energies from 180 keV to 200 MeV; a careful study of the systematic uncertainties complement the data.

Different aspects of the nuclear fission process have been studied at Los Alamos Neutron Science Center (LANSCE) using various instruments and experimental techniques. Properties of the fragments emitted in fission have been investigated using Frisch-grid ionization chambers, a Time Projection Chamber (TPC), and the SPIDER instrument which employs the 2v-2E method. These instruments and experimental techniques have been used to determine fission product mass yields, the energy dependent total kinetic energy (TKE) release, and anisotropy in neutron-induced fission of U-235, U-238 and Pu-239.

The MICROMEGAS (MICRO-MEsh GAseous Structure) charge amplification structure has found wide use in many detection applications, especially as a gain stage for the charge readout of Time Projection Chambers (TPCs). Here we report on the behavior of a MICROMEGAS TPC when operated in a high-energy (up to 800 MeV ) neutron beam. It is found that neutron-induced reactions can cause discharges in some drift gas mixtures that are stable in the absence of the neutron beam. The discharges result from recoil ions close to the MICROMEGAS that deposit high specific ionization density and have a limited diffusion time. For a binary drift gas, increasing the percentage of the molecular component (quench gas) relative to the noble component and operating at lower pressures generally improves stability.

The average Total Kinetic Energy (TKE ) release and fission-fragment yields in neutron-induced fission of 235 U and 238 U was measured using a Frisch-gridded ionization chamber. These observables are important nuclear data quantites that are relevant to applications and for informing the next generation of fission models. The measurements were performed a the Los Alamos Neutron Science Center and cover E n = 200 keV – 30 MeV. The double-energy (2E) method was used to determine the fission-fragment yields and two methods of correcting for prompt-neutron emission were explored. The results of this study are correlated mass and TKE data.

The average total kinetic energy $(\overline{TKE})$ in $^{239}\mathrm{Pu}(n,f)$ has been measured for incident neutron energies between 0.5 and 50 MeV. The experiment was performed at the Los Alamos Neutron Science Center (LANSCE) using the neutron time-of-flight technique, and the kinetic energy of fission fragments post-neutron emission was measured in a double Frisch-gridded ionization chamber. This represents the first experimental study of the energy dependence of $\overline{TKE}$ in $^{239}\mathrm{Pu}$ above neutron energies of 6 MeV.

2014 LANSCE run cycle data will provide a preliminary 239Pu(n,f) cross section and will quantify uncertainties: PID and Target/beam non-uniformities. Continued running during the 2015 LANSCE run cycle: Thin targets to see both fission fragments and 239Pu(n,f) cross section and fully quantified uncertainties

$\ensuremath{\gamma}$-ray transitions in ${}^{134}\text{Te}$, ${}^{135}\text{Te}$, and ${}^{136}\text{Te}$ were measured from ${}^{9}\text{Be}$-induced reactions with a radioactive ${}^{132}\text{Sn}$ beam at a sub-Coulomb barrier energy of 3 MeV per nucleon using particle-$\ensuremath{\gamma}$ coincidence spectroscopy. The transitions were selected by gating on alpha-like particles in a CsI detector following a combination of $({}^{9}\text{Be},\ensuremath{\alpha}1n)$, $({}^{9}\text{Be},\ensuremath{\alpha}2n)$, and $({}^{9}\text{Be},\ensuremath{\alpha}3n)$ incomplete fusion-evaporation reactions. Distorted-wave Born approximation calculations suggest little to no contribution from the $({}^{9}\text{Be},{}^{7}\text{He})$, $({}^{9}\text{Be},{}^{6}\text{He})$, and $({}^{9}\text{Be},{}^{5}\text{He})$ direct reactions.$\ensuremath{\gamma}$-ray transitions from previously known ${2}^{+}\ensuremath{\bigotimes}\ensuremath{\nu}\phantom{\rule{0.16em}{0ex}}2{f}_{7/2}$ and ${4}^{+}\ensuremath{\bigotimes}\ensuremath{\nu}\phantom{\rule{0.16em}{0ex}}2{f}_{7/2}$ multiplet members in ${}^{135}\text{Te}$ are observed. A new $\ensuremath{\gamma}$ ray is observed, assigned to the third-excited state in ${}^{135}\text{Te}$, and new ${2}^{+}\ensuremath{\bigotimes}\ensuremath{\nu}\phantom{\rule{0.16em}{0ex}}2{f}_{7/2}$ multiplet members are suggested. In addition, spin assignments are made by using recent one-neutron transfer data. The updated experimental data for ${}^{135}\text{Te}$ are compared to shell-model calculations for a relatively complete set of states up to the yrast ${15/2}^{\ensuremath{-}},{4}^{+}\ensuremath{\bigotimes}\ensuremath{\nu}\phantom{\rule{0.16em}{0ex}}2{f}_{7/2}$ multiplet member at 1505 keV.

Two generalized transfer reaction techniques have been used to exploit these beams in regions of the nuclear chart around N = 50 and N = 82. The first employs large silicon detector arrays to measure protons emitted from the (d,p) reaction in inverse kinematics [2 6]. The second uses HYBALL to detect the charged particles emitted from ( 9 Be, 8 Be), and ( 13 C, 12 C) reactions with gamma rays measured in coincidence in CLARION [6 7].

Nuclear data related to the fission process are needed for a wide variety of research areas, including fundamental science, nuclear energy and non-proliferation. While some of the relevant data have been measured to the required accuracies there are still many aspects of fission that need further investigation. One such aspect is how Total Kinetic Energy (TKE), fragment yields, angular distributions and other fission observables depend on excitation energy of the fissioning system. Another question is the correlation between mass, charge and energy of fission fragments. At the Los Alamos Neutron Science Center (LANSCE) we are studying neutron-induced fission at incident energies from thermal up to hundreds of MeV using the Lujan Center and Weapons Neutron Research (WNR) facilities. Advanced instruments such as SPIDER (time-of-flight and kinetic energy spectrometer), the NIFFTE Time Projection Chamber (TPC), and Frisch grid Ionization Chambers (FGIC) are used to investigate the properties of fission fragments, and some important results for the major actinides have been obtained.

The coincident detection of particles and gamma rays allows the study of the structure of exotic nuclei via inverse kinematics reactions using radioactive ion beams and thick targets. We report on the status of the project to couple the highresolution charged-particle detector ORRUBA to Gammasphere, a high-efficiency, high-resolution gamma ray detector.

The study of nuclei far from stability elucidates the evolution of nuclear shell structure, and also affects estimates of heavy element nucleosynthesis in supernova explosions. Measurement of transfer reactions in inverse kinematics with radioactive ion beams is a powerful technique for these types of studies. Rare isotope beams often have relatively low intensities, and this places difficult requirements on the detection systems for reaction products. The detectors must provide large solid angle coverage in the laboratory along with good position and energy resolution. The Super ORRUBA detector array has been developed for such measurements and is comprised of 18 double-sided, nonresistive silicon strip detectors. This configuration features low thresholds and improved resolution over detectors employing charge division. As a first implementation of this system, the 80Ge(d,p)81Ge neutron transfer reaction in inverse kinematics was measured at HRIBF at ORNL, to determine the properties of levels in 81Ge.

The (d, p) reaction was measured with the radioactive ion beams of 126Sn and 128Sn in inverse kinematics at the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory, utilizing the Super ORRUBA silicon detector array. Angular distributions of reaction protons were measured for several states in 127Sn and 129Sn to determine angular momentum transfers and deduce spectroscopic factors. Such information is critical for calculating direct (n,γ) cross sections for the r-process as well as for constraining shell model parameters in the A≈130 region. Combined with previous experiments on 130Sn and 132Sn, these results will provide a complete set of (d, p) reaction data on even tin isotopes between stable 124Sn and doubly-magic 132Sn.

The astrophysical rapid neutron-capture process (r-process) is believed to have produced approximately half of the nuclear species more massive than Fe. Unfortunately, almost nothing is known about the structure of the majority of the extremely neutron-rich nuclei involved in the reaction flow. At exotic beam facilities such as the Holifield Radioactive Ion Beam Facility (HRIBF), measurements with accelerated beams of fission fragments have provided some of the first spectroscopic information on many r-process nuclei. The new SuperORRUBA (Oak Ridge Rutgers University Barrel Array) detector has been constructed at the HRIBF to study such nuclei, and first results are presented.