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The tunneling of interacting charges in nanostructures is a random and noisy process, which gives rise to a variety of intriguing physical phenomena, including Coulomb blockade, the Kondo effect, and Fermi-edge singularities. Such correlation effects are visible in low-frequency measurements of the electric current or the shot noise, however, they are also expected to leave clear fingerprints in the tunneling times of individual charges. Here, we experimentally demonstrate the real-time detection and control of correlated charge tunneling in a dynamically driven quantum dot. To this end, we measure the joint distribution of waiting times between tunneling charges, and we show that subsequent waiting times are strongly correlated due to the Coulomb interactions between the tunneling charges and the external periodic drive. Our measurements are in excellent agreement with a theoretical model that allows us to develop a detailed understanding of the correlated tunneling events. We also demonstrate that the degree of correlations can be controlled by the external drive. Our experiment paves the way for systematic real-time investigations of correlated electron transport in low-dimensional nanostructures with potential applications in metrology and sensing., Comment: 7 pages, 5 figures

The Dicke model describes an ensemble of two-level atoms that are coupled to a confined light mode of an optical cavity. Above a critical coupling, the cavity becomes macroscopically occupied, and the system enters the superradiant phase. This phase transition can be observed by detecting the photons that are emitted from the cavity; however, it only becomes apparent in the limit of long observation times, while actual experiments are of a finite duration. To circumvent this problem, we here make use of recent advances in Lee-Yang theories of phase transitions to show that the superradiant phase transition can be inferred from the factorial cumulants of the photon emission statistics obtained during a finite measurement time. Specifically, from the factorial cumulants, we can determine the complex singularities of generating functions that describe the photon emission statistics, and by extrapolating their positions to the long-time limit, one can detect the superradiant phase transition. We also show that the convergence points determine the tails of the large-deviation statistics of the photon current. Our work demonstrates how phase transitions in the Dicke model and in other quantum many-body systems can be detected from measurements of a finite duration., Comment: 10 pages, 4 figures

Electron quantum optics aims to realize ideas from the quantum theory of light with the role of photons being played by charge pulses in electronic conductors. Experimentally, the charge pulses are excited by time-dependent voltages, however, one could also generate heat pulses by heating and cooling an electrode. Here, we explore this intriguing idea by formulating a Floquet scattering theory of heat pulses in mesoscopic conductors. The adiabatic emission of heat pulses leads to a heat current that in linear response is given by the thermal conductance quantum. However, we also find a high-frequency component, which ensures that the fluctuation-dissipation theorem for heat currents, whose validity has been debated, is fulfilled. The heat pulses are uncharged, and we probe their electron-hole content by evaluating the partition noise in the outputs of a quantum point contact. We also employ a Hong--Ou--Mandel setup to examine if the pulses bunch or antibunch. Finally, to generate an electric current, we use a Mach--Zehnder interferometer that breaks the electron-hole symmetry and thereby enables a thermoelectric effect. Our work paves the way for systematic investigations of heat pulses in mesoscopic conductors, and it may stimulate future experiments., Comment: 7+5 pages, 4 figures

Recent experiments have observed Cooper pair splitting in quantum dots coupled to superconductors, and efficient schemes for controlling and timing the splitting process are now called for. Here, we propose and analyze an adiabatic Cooper pair splitter that can produce a regular flow of spin-entangled electrons in response to a time-dependent and periodic gate voltage. The splitting process is controlled by moving adiabatically back and forth along an avoided crossing between the empty state and the singlet state of two quantum dots that are coupled to a superconductor, followed by the emission of the split Cooper pairs into two normal-state drains. The scheme does not rely on fine-tuned resonance conditions and is therefore robust against experimental imperfections in the driving signal. We identify a range of driving frequencies, where the output currents are quantized and proportional to the driving frequency combined with suppressed low-frequency noise. We also discuss the main sources of cycle-missing events and evaluate the statistics of electrons emitted within a period of the drive as well as the distribution of waiting times between them. Realistic parameter estimates indicate that the Cooper pair splitter can be operated in the gigahertz regime., Comment: 6+2 pages, 4 figures

Recent experimental advances have made it possible to detect individual quantum jumps in open quantum systems, such as the tunneling of single electrons in nanoscale conductors or the emission of photons from non-classical light sources. Here, we investigate theoretically the statistics of photons emitted from a microwave cavity that is driven resonantly by an external field. We focus on the differences between a parametric and a coherent drive, which either squeezes or displaces the cavity field. We employ a Lindblad master equation dressed with counting fields to obtain the generating function of the photon emission statistics using a theoretical framework based on Gaussian states. We then compare the distribution of photon waiting times for the two drives as well as the $g^{(2)}$-functions of the outgoing light, and we identify important differences between these observables. In the long-time limit, we analyze the factorial cumulants of the photon emission statistics and the large-deviation statistics of the emission currents, which are markedly different for the two drives. Our theoretical framework can readily be extended to more complicated systems, for instance, with several coupled microwave cavities, and our predictions may be tested in future experiments., Comment: 12 pages, 6 figures

Bose-Einstein condensation happens as a gas of bosons is cooled below its transition temperature, and the ground state becomes macroscopically occupied. The phase transition occurs in the thermodynamic limit of many particles. However, recent experimental progress has made it possible to assemble quantum many-body systems from the bottom up, for example, by adding single atoms to an optical lattice one at a time. Here, we show how one can predict the condensation temperature of a Bose gas from the energy fluctuations of a small number of bosons. To this end, we make use of recent advances in Lee-Yang theories of phase transitions, which allow us to determine the zeros and the poles of the partition function in the complex plane of the inverse temperature from the high cumulants of the energy fluctuations. By increasing the number of bosons in the trapping potential, we can predict the convergence point of the partition function zeros in the thermodynamic limit, where they reach the inverse critical temperature on the real axis. Using less than 100 bosons, we can estimate the condensation temperature for a Bose gas in a harmonic potential in two and three dimensions, and we also find that there is no phase transition in one dimension as one would expect., Comment: 11 pages, 6 figures

Controlling the temperature of nano-scale quantum systems is becoming increasingly important in the efforts to develop thermal devices such as quantum heat valves, heat engines, and refrigerators, and to explore fundamental concepts in quantum thermodynamics. In practice, however, it is challenging to generate arbitrary time-dependent temperatures, similarly to what has been achieved for electronic voltage pulses. To overcome this problem, we here propose a fully quantum mechanical scheme to control the time-dependent environment temperature of an open quantum system. To this end, we consider a collection of quantum harmonic oscillators that mediate the interactions between the quantum system and a thermal reservoir, and we show how an effective time-dependent temperature can be realized by modulating the oscillator frequencies in time. By doing so, we can apply effective temperature pulses to the quantum system, and it can be cooled below the temperature of the environment. Surprisingly, the scheme can be realized using only a few oscillators, and our proposal thereby paves the way for controlling the temperature of open quantum systems., Comment: 12 pages, 4 figures

Dynamical quantum phase transitions are at the forefront of current efforts to understand quantum matter out of equilibrium. Except for a few exactly solvable models, predictions of these critical phenomena typically rely on advanced numerical methods. However, those approaches are mostly restricted to one dimension, making investigations of two-dimensional systems highly challenging. Here, we present evidence of dynamical quantum phase transitions in strongly correlated spin lattices in two dimensions. To this end, we apply our recently developed cumulant method [Phys. Rev. X 11, 041018 (2021)] to determine the zeros of the Loschmidt amplitude in the complex plane of time and predict the crossing points of the thermodynamic lines of zeros with the real-time axis, where dynamical quantum phase transitions occur. We find the critical times of a two-dimensional quantum Ising lattice and the XYZ model with ferromagnetic or antiferromagnetic couplings. We also show how dynamical quantum phase transitions can be predicted by measuring the initial energy fluctuations, for example, in quantum simulators or other engineered quantum systems., Comment: 6 pages, 4 figures

Phase transitions occur in a wide range of physical systems and are characterized by the abrupt change of a physical observable in response to the variation of an external control parameter. Phase transitions are not restricted to equilibrium situations but can also be found in nonequilibrium settings, both for classical and quantum mechanical systems. Here, we investigate a nonequilibrium phase transition in a single-electron micromaser consisting of a microwave cavity that is driven by the electron transport in a double quantum dot. For weak electron-photon couplings, only a tiny fraction of the transferred electrons lead to the emission of photons into the cavity, which essentially remains empty. However, as the coupling is increased, many photons are suddenly emitted into the cavity. Employing ideas and concepts from full counting statistics and Lee-Yang theory, we analyze this nonequilibrium phase transition based on the dynamical zeros of the factorial moment generating function of the electronic charge transport, and we find that the phase transition can be predicted from short-time measurements of the higher-order factorial cumulants. These results pave the way for further investigations of critical behavior in open quantum systems., Comment: 13+ pages, 6 figures

The generation of spin-entangled electrons is an important prerequisite for future solid-state quantum technologies. Cooper pairs in a superconductor can be split into separate electrons in a spin-singlet state, however, detecting their entanglement remains an open experimental challenge. Proposals to detect the entanglement by violating a Bell inequality typically require a large number of current cross-correlation measurements, and not all entangled states can be detected in this way. Here, we instead formulate an entanglement witness that can detect the spin-entanglement using only three cross-correlation measurements of the currents in the outputs of a Cooper pair splitter. We identify the optimal measurement settings for witnessing the entanglement, and we illustrate the use of our entanglement witness with a realistic model of a Cooper pair splitter for which we evaluate the cross-correlations of the output currents. Specifically, we find that the entanglement of the spins can be detected even with a moderate level of decoherence. Our work thereby paves the way for an experimental detection of the entanglement produced by Cooper pair splitters., Comment: 11 pages, 4 figures

Cooper pair splitters are promising candidates for generating spin-entangled electrons. However, the splitting of Cooper pairs is a random and noisy process, which hinders further synchronized operations on the entangled electrons. To circumvent this problem, we here propose and analyze a dynamic Cooper pair splitter that produces a noiseless and regular flow of spin-entangled electrons. The Cooper pair splitter is based on a superconductor coupled to quantum dots, whose energy levels are tuned in and out of resonance to control the splitting process. We identify the optimal operating conditions for which exactly one Cooper pair is split per period of the external drive and the flow of entangled electrons becomes noiseless. To characterize the regularity of the Cooper pair splitter in the time domain, we analyze the $g^{(2)}$-function of the output currents and the distribution of waiting times between split Cooper pairs. Our proposal is feasible using current technology, and it paves the way for dynamic quantum information processing with spin-entangled electrons., Comment: 6 pages, 3 figures

Controlled generation and detection of quantum entanglement between spatially separated particles constitute an essential prerequisite both for testing the foundations of quantum mechanics and for realizing future quantum technologies. Splitting of Cooper pairs from a superconductor provides entangled electrons at separate locations. However, experimentally accessing the individual split Cooper pairs constitutes a major unresolved issue as they mix together with electrons from competing processes. Here, we overcome this challenge with the first real-time observation of the splitting of individual Cooper pairs, enabling direct access to the time-resolved statistics of Cooper pair splitting. We determine the correlation statistics arising from two-electron processes and find a pronounced peak that is two orders of magnitude larger than the background. Our experiment thereby allows to unambiguously pinpoint and select split Cooper pairs with 99 % fidelity. These results open up an avenue for performing experiments that tap into the spin-entanglement of split Cooper pairs.

Dynamical phase transitions extend the notion of criticality to non-stationary settings and are characterized by sudden changes in the macroscopic properties of time-evolving quantum systems. Investigations of dynamical phase transitions combine aspects of symmetry, topology, and non-equilibrium physics, however, progress has been hindered by the notorious difficulties of predicting the time evolution of large, interacting quantum systems. Here, we tackle this outstanding problem by determining the critical times of interacting many-body systems after a quench using Loschmidt cumulants. Specifically, we investigate dynamical topological phase transitions in the interacting Kitaev chain and in the spin-1 Heisenberg chain. To this end, we map out the thermodynamic lines of complex times, where the Loschmidt amplitude vanishes, and identify the intersections with the imaginary axis, which yield the real critical times after a quench. For the Kitaev chain, we can accurately predict how the critical behavior is affected by strong interactions, which gradually shift the time at which a dynamical phase transition occurs. We also discuss the experimental perspectives of predicting the first critical time of a quantum many-body system by measuring the energy fluctuations in the initial state, and we describe the prospects of implementing our method on a near-term quantum computer with a limited number of qubits. Our work demonstrates that Loschmidt cumulants are a powerful tool to unravel the far-from-equilibrium dynamics of strongly correlated many-body systems, and our approach can immediately be applied in higher dimensions., Comment: 9+5 pages, 4 figures

We investigate the Ising model in one, two, and three dimensions using a cumulant method that allows us to determine the Lee-Yang zeros from the magnetization fluctuations in small lattices. By doing so with increasing system size, we are able to determine the convergence point of the Lee-Yang zeros in the thermodynamic limit and thereby predict the occurrence of a phase transition. The cumulant method is attractive from an experimental point of view since it uses fluctuations of measurable quantities, such as the magnetization in a spin lattice, and it can be applied to a variety of equilibrium and non-equilibrium problems. We show that the Lee-Yang zeros encode important information about the rare fluctuations of the magnetization. Specifically, by using a simple ansatz for the free energy, we express the large-deviation function of the magnetization in terms of Lee-Yang zeros. This result may hold for many systems that exhibit a first-order phase transition., Comment: 13 pages, 8 figures, final version

Quantum technologies involving qubit measurements based on electronic interferometers rely critically on accurate single-particle emission. However, achieving precisely timed operations requires exquisite control of the single-particle sources in the time domain. Here, we demonstrate accurate control of the emission time statistics of a dynamic single-electron transistor by measuring the waiting times between emitted electrons. By ramping up the modulation frequency, we controllably drive the system through a crossover from adiabatic to nonadiabatic dynamics, which we visualize by measuring the temporal fluctuations at the single-electron level and explain using detailed theory. Our work paves the way for future technologies based on the ability to control, transmit, and detect single quanta of charge or heat in the form of electrons, photons, or phonons., Comment: 5+2 pages, 3 figures, published in Science Advances

We investigate theoretically the noise and the full counting statistics of electrons that are emitted from a superconductor into two spatially separated quantum dots by the splitting of Cooper pairs and further on collected in two normal-state electrodes. With negatively-biased drain electrodes and a large superconducting gap, the dynamics of the Cooper pair splitter can be described by a Markovian quantum master equation. Using techniques from full counting statistics, we evaluate the electrical currents, their noise power spectra, and the power-power correlations in the output leads. The current fluctuations can be attributed to the competition between Cooper pair splitting and elastic cotunneling between the quantum dots via the superconductor. In one regime, these processes can be clearly distinguished in the cross-correlation spectrum with peaks and dips appearing at characteristic frequencies associated with elastic cotunneling and Cooper pair splitting, respectively. We corroborate this interpretation by analyzing the charge transport fluctuations in the time domain, specifically by investigating the $g^{(2)}$-function of the output currents. Our work identifies several experimental signatures of the fundamental transport processes involved in Cooper pair splitting and provides specific means to quantify their relative strengths. As such, our results may help guide and interpret future experiments on current fluctuations in Cooper pair splitters., Comment: 15 pages, 6 figures

Almost a century ago, Johnson and Nyquist presented evidence of fluctuating electrical current and the governing fluctuation dissipation theorem (FDT). Whether, likewise, temperature T can fluctuate is a controversial topic and has led to scientific debates for several decades. To resolve this issue, there was an experiment initially in 1992 where the authors found good agreement between the FDT theory for heat and experiment on a macroscopic sample. A key question is what happens when we consider a nanoscale system with much fewer particles at 100 times lower temperatures. This challenge has not been addressed up to now, due to the demanding experimental requirement on fast and sensitive thermometry on a mesoscopic absorber. Here we observe equilibrium fluctuations of temperature in a canonical system of about 10^8 electrons exchanging energy with phonon bath at a fixed temperature. Moreover, temperature fluctuations under nonequilibrium conditions present a nontrivial dependence on the chemical potential bias of a hot electron source. These fundamental fluctuations of T set the ultimate lower bound of the energy resolution of a calorimeter.

The development of microwave photon detectors is paving the way for a wide range of quantum technologies and fundamental discoveries involving single photons. Here, we investigate the photon emission from a microwave cavity and find that distribution of photon waiting times contains information about few-photon processes, which cannot easily be extracted from standard correlation measurements. The factorial cumulants of the photon counting statistics are positive at all times, which may be intimately linked with the bosonic quantum nature of the photons. We obtain a simple expression for the rare fluctuations of the photon current, which is helpful in understanding earlier results on heat transport statistics and measurements of work distributions. Under non-equilibrium conditions, where a small temperature gradient drives a heat current through the cavity, we formulate a fluctuation-dissipation relation for the heat noise spectra. Our work suggests a number of experiments for the near future, and it offers theoretical questions for further investigation., Comment: 16 pages, 3 figures, final version as published in Phys. Rev. B

In mesoscopic and nanoscale systems at low temperatures, charge carriers are typically not in thermal equilibrium with the surrounding lattice. The resulting, non-equilibrium dynamics of electrons has only begun to be explored. Experimentally the time-dependence of the electron temperature (deviating from the lattice temperature) has been investigated in small metallic islands. Motivated by these experiments we investigate theoretically the electronic energy and temperature fluctuations in a metallic island in the Coulomb blockade regime, tunnel coupled to an electronic reservoir, i.e. a single electron box. We show that electronic quantum tunnelling between the island and the reservoir, in the absence of any net charge or energy transport, induces fluctuations of the island electron temperature. The full distribution of the energy transfer as well as the island temperature is derived within the framework of full counting statistics. In particular, the low-frequency temperature fluctuations are analysed, fully accounting for charging effects and non-zero reservoir temperature. The experimental requirements for measuring the predicted temperature fluctuations are discussed., Comment: 20 pages, 4 figures, submitted to NJP special issue on Quantum Thermodynamics