Search

A sequence of excited states has been established for the first time in the proton-rich nucleus 48Fe (Z=26, N=22). The technique of mirrored (i.e. analogue) one-nucleon knockout reactions was applied, in which the T z = ±2 mirror pair, 48Fe/48Ti were populated via one-neutron/one-proton knockout from the secondary beams 49Fe/49V, respectively. The analogue properties of the reactions were used to help establish the new level scheme of 48Fe. The inclusive and exclusive cross sections were determined for the populated states. Large differences between the cross sections for the two mirrored reactions were observed and have been interpreted in terms of different degrees of binding of the mirror nuclei and in the context of the recent observations of suppression of spectroscopic strength as a function of nuclear binding, for knockout reactions on light solid targets. Mirror energy differences (MED) have been determined between the analogue T = 2 states and compared with the shell model predictions. MED for this mirror pair, due to their location in the shell, are especially sensitive to excitations out of the f 7 / 2 shell, and present a stringent test of the shell-model prescription.

The signatures of inversion between normal and intruder configurations of particle-hole excitations across the $N=20$ shell gap in the neutron-rich isotope $^{32}\mathrm{Mg}$ have long been of keen interest. Electromagnetic transition rates in the ground-state band are key quantities that provide insights into collective properties associated with the contributions of the 2p2h and 4p4h intruder configurations. The combination of TRIPLEX, GRETINA, and the S800 spectrograph enables model-independent lifetime measurements to determine electromagnetic transition rates in rare isotopes. The reduced $E2$ transition rates in $^{32}\mathrm{Mg}$ between the ${2}_{1}^{+}$ and ${0}_{1}^{+}$ states and between the ${4}_{1}^{+}$ and ${2}_{1}^{+}$ states have been measured, the latter representing the first experimental $B(E2)$ value for this transition. The $B(E2)$ strengths indicate large collectivity and strong contributions from the 2p2h and 4p4h intruder configurations that may change with spin in the ground-state band of $^{32}\mathrm{Mg}$.

The level schemes of the neutron-rich $^{37--42}\mathrm{P}$ isotopes are investigated via in-beam $\ensuremath{\gamma}$-ray spectroscopy following the fragmentation of a $^{45}\mathrm{Cl}$ projectile beam at intermediate beam energies. Information on $\ensuremath{\gamma}\ensuremath{\gamma}$ coincidence relationships complemented by comparisons to shell-model calculations in the $sd\text{\ensuremath{-}}pf$ model space were used to construct excitation level schemes for these neutron-rich nuclei. For the odd-mass $^{37,39}\mathrm{P}$ isotopes, a level scheme is presented that appears essentially complete at low energies and exhausts the states predicted by the SDPF-MU shell-model Hamiltonian. Simple Nilsson configurations are proposed for the low-lying excited states of $^{38,39,40,41}\mathrm{P}$ from an analysis of the $E2$ transition matrix elements and moments calculated within the shell model.

Electromagnetic transition strengths in the even-even neutron-rich sulfur isotopes $^{38,40,42,44}\mathrm{S}$ were measured using intermediate-energy Coulomb excitation at the National Superconducting Cyclotron Laboratory. By utilizing the sensitivity of the experimental technique to $E2$ excitations from the ground state, the evolution of the pattern of $B(E2)$ strengths to several low-lying ${2}^{+}$ states was investigated at $Z=16$ from near stability to the $N=28$ island of inversion. The experimental results allowed a detailed comparison with predictions from shell-model calculations using the SDPF-MU Hamiltonian, which was designed to describe collectivity in this region of the nuclear chart. While the shell-model calculations succeeded in modeling transition strengths at $N=22,24,26$, the experimental $B(E2;{0}_{1}^{+}\ensuremath{\rightarrow}{2}_{1}^{+})$ at $N=28$ was smaller than the predicted value by about a factor of 2, similar to previous observations for chlorine and argon isotopes around $N=28$. The dependence of this overprediction by theory on the choice of effective charges was explored.

Discovering unexplored high-spin states in neutron-rich nuclei can open up a new direction to study band structure and the associated shell structure in isospin-asymmetric many-body systems. However, experimental reach has so far been limited to neutron-deficient or stable nuclei which are preferentially produced in fusion reactions used in such studies. Here, we report the first $\ensuremath{\gamma}$-ray spectroscopy with fusion reactions using a reaccelerated rare-isotope beam of $^{45}\mathrm{K}$ performed at the ReA3 facility of the National Superconducting Cyclotron Laboratory. Using particle and $\ensuremath{\gamma}$-ray coincidence techniques, three new higher-lying states around 6 MeV and five new $\ensuremath{\gamma}$-ray transitions were identified for $^{46}\mathrm{Ca}$, suggesting three independent band structures formed from different particle-hole configurations. The rotational-like band built on the ${0}_{2}^{+}$ state is established up to the tentatively assigned ${6}_{2}^{+}$ state. New results are compared to large-scale shell model calculations, confirming the validity of the effective interaction describing particle-hole excitations across the $Z=20$ and $N=28$ shell gaps in the vicinity of doubly magic $^{48}\mathrm{Ca}$.

The shape and collectivity of $^{106}\mathrm{Cd}$ was investigated via a sub-barrier-energy Coulomb excitation experiment performed at the National Superconducting Cyclotron Laboratory Re-accelerator facility using the JANUS setup. Transition matrix elements between low-lying states were found to agree with adopted values, and information on the shape and collectivity of higher-lying states was extracted for the first time. Locally optimized large-scale shell-model calculations were found to describe well the $B(E2)$ transition strengths but failed to reproduce the spectroscopic quadrupole moments ${Q}_{s}$. An analysis of the $E2$ rotational invariants and the normalized quadrupole moment ${q}_{s}$ indicates that this may be due to a significant degree of triaxiality in $^{106}\mathrm{Cd}$ which is not captured by the present shell-model calculations. Analogous calculations for the Fe isotopes (two protons below the $Z=28$ magic number) reveal the critical role of high-$j$ neutron configurations for the description of quadrupole moments in the heavy Fe and Cd isotopes (two protons below magic $Z=50$), but this effect is insufficient to explain the shape of $^{106}\mathrm{Cd}$, posing a puzzle for the understanding of nuclear structure towards $N=50$.

The neutron-rich nuclei in the $N=28$ island of inversion have attracted considerable experimental and theoretical attention, providing great insight into the evolution of shell structure and nuclear shape in exotic nuclei. In this work, for the first time, quadrupole collectivity is assessed simultaneously on top of the $3/{2}^{\ensuremath{-}}$ ground state and the $7/{2}^{\ensuremath{-}}$ shape-coexisting isomer of $^{43}\mathrm{S}$, putting the unique interpretation of shape and configuration coexistence at $N=27$ and 28 in the sulfur isotopic chain to the test. From an analysis of the electromagnetic transition strengths and quadrupole moments predicted within the shell model, it is shown that the onset of shape coexistence and the emergence of a simple collective structure appear suddenly in $^{43}\mathrm{S}$ with no indication of such patterns in the $N=27$ isotone $^{45}\mathrm{Ar}$.

Proton capture on the excited isomeric state of ^{26}Al strongly influences the abundance of ^{26}Mg ejected in explosive astronomical events and, as such, plays a critical role in determining the initial content of radiogenic ^{26}Al in presolar grains. This reaction also affects the temperature range for thermal equilibrium between the ground and isomeric levels. We present a novel technique, which exploits the isospin symmetry of the nuclear force, to address the long-standing challenge of determining proton-capture rates on excited nuclear levels. Such a technique has in-built tests that strongly support its veracity and, for the first time, we have experimentally constrained the strengths of resonances that dominate the astrophysical ^{26m}Al(p,γ)^{27}Si reaction. These constraints demonstrate that the rate is at least a factor ∼8 lower than previously expected, indicating an increase in the stellar production of ^{26}Mg and a possible need to reinvestigate sensitivity studies involving the thermal equilibration of ^{26}Al.

The structure of exotic nuclei provides valuable tests for state-of-the-art nuclear theory. In particular electromagnetic transition rates are more sensitive to aspects of nuclear forces and many-body physics than excitation energies alone. We report the first lifetime measurement of excited states in $^{21}$O, finding $\tau_{1/2^+}=420^{+35}_{-32}\text{(stat)}^{+34}_{-12}\text{(sys)}$\,ps. This result together with the deduced level scheme and branching ratio of several $\gamma$-ray decays are compared to both phenomenological shell-model and ab initio calculations based on two- and three-nucleon forces derived from chiral effective field theory. We find that the electric quadrupole reduced transition probability of $\rm B(E2;1/2^+ \rightarrow 5/2^+_{g.s.}) = 0.71^{+0.07\ +0.02}_{-0.06\ -0.06}$~e$^2$fm$^4$, derived from the lifetime of the $1/2^+$ state, is smaller than the phenomenological result where standard effective charges are employed, suggesting the need for modifications of the latter in neutron-rich oxygen isotopes. We compare this result to both large-space and valence-space ab initio calculations, and by using multiple input interactions we explore the sensitivity of this observable to underlying details of nuclear forces., Comment: 23 pages, 3 figures

The single-particle structure of the N = 27 isotones provides insights into the shell evolution of neutron-rich nuclei from the doubly-magic 48Ca toward the drip line. 43S was studied employing the one-neutron knockout reaction from a radioactive 44S beam. Using a combination of prompt and delayed γ-ray spectroscopy the level structure of 43S was clarified. Momentum distributions were analyzed and allowed for spin and parity assignments. The deduced spectroscopic factors show that the 44S ground-state configuration has a strong intruder component. The results were confronted with shell model calculations using two effective interactions. General agreement was found between the calculations, but strong population of states originating from the removal of neutrons from the 2p3/2 orbital in the experiment indicates that the breakdown of the N = 28 magic number is more rapid than the theoretical calculations suggest.

The lifetimes of the first excited 2^{+} states in the N=Z nuclei ^{80}Zr, ^{78}Y, and ^{76}Sr have been measured using the γ-ray line shape method following population via nucleon-knockout reactions from intermediate-energy rare-isotope beams. The extracted reduced electromagnetic transition strengths yield new information on where the collectivity is maximized and provide evidence for a significant, and as yet unexplained, odd-odd vs even-even staggering in the observed values. The experimental results are analyzed in the context of state-of-the-art nuclear density-functional model calculations.

Simpson and Tostevin proposed that the width and shape of exclusive parallel momentum distributions of the A

New experimental data obtained from γ-ray tagged one-neutron and one-proton knockout from 55Co is presented. A candidate for the sought-after T = 1, T z = 0, Jπ = 6+ state in 54Co is proposed based on a comparison to the new data on 54Fe, the corresponding observables predicted by large-scale-shell-model (LSSM) calculations in the full fp-model space employing charge-dependent contributions, and isospin-symmetry arguments. Furthermore, possible isospin-symmetry breaking in the A = 54, T = 1 triplet is studied by calculating the experimental c coefficients of the isobaric mass multiplet equation (IMME) up to the maximum possible spin J = 6 expected for the (1f7/2)-2 two-hole configuration relative to the doubly-magic nucleus 56Ni. The experimental quantities are compared to the theoretically predicted c coefficients from LSSM calculations using two-body matrix elements obtained from a realistic chiral effective field theory potential at next-to-next-to-next-to leading order (N3LO).

A new experimental setup for low-energy Coulomb excitation experiments was constructed in a collaboration between the National Superconducting Cyclotron Laboratory (NSCL), Lawrence Livermore National Laboratory (LLNL), and the University of Rochester and was commissioned at the general purpose beam line of NSCL’s ReA3 reaccelerator facility. The so-called JANUS setup combines γ -ray detection with the Se gmented G e A rray (SeGA) and scattered particle detection using a pair of segmented double-sided Si detectors (Bambino 2). The low-energy Coulomb excitation program that JANUS enables will complement intermediate-energy Coulomb excitation studies that have long been performed at NSCL by providing access to observables that quantify collectivity beyond the first excited state, including the sign and magnitude of excited-state quadrupole moments. In this work, the setup and its performance will be described based on the commissioning run that used stable 78Kr impinging onto a 1.09 mg/cm 2 208Pb target at a beam energy of 3.9 MeV/u.

Author(s): Titus, R; Ney, EM; Zegers, RGT; Bazin, D; Belarge, J; Bender, PC; Brown, BA; Campbell, CM; Elman, B; Engel, J; Gade, A; Gao, B; Kwan, E; Lipschutz, S; Longfellow, B; Lunderberg, E; Mijatovic, T; Noji, S; Pereira, J; Schmitt, J; Sullivan, C; Weisshaar, D; Zamora, JC | Abstract: Background: In the late stages of stellar core collapse just prior to core bounce, electron captures on medium-heavy nuclei drive deleptonization. Therefore, simulations require the use of accurate reaction rates. Nuclei with neutron number near N=50 above atomic number Z=28 play an important role. Rates presently used in astrophysical simulations rely primarily on a relatively simple single-state approximation. In order to improve the accuracy of the astrophysical simulations, experimental data are needed to test the electron-capture rates and to guide the development of better theoretical models and astrophysical simulations. Purpose: The purpose of the present work was to measure the Gamow-Teller transition strength from Kr86 to Br86, to derive the stellar electron-capture rates based on the extracted strengths, and to compare the derived rates with rates based on shell-model and quasiparticle random-phase approximation (QRPA) Gamow-Teller strengths calculations, as well as the single-state approximation. An additional purpose was to test the impact of using improved electron-capture rates on the late evolution of core-collapse supernovae. Method: The Gamow-Teller strengths from Kr86 were extracted from the Kr86(t,He3+γ) charge-exchange reaction at 115MeV/u. The electron-capture rates were calculated as a function of stellar density and temperature. Besides the case of Kr86, the electron-capture rates based on the QRPA calculations were calculated for 78 additional isotopes near N=50 above Z=28. The impact of using these rates instead of those based on the single-state approximation is studied in a spherically symmetrical simulation of core collapse just prior to bounce. Results: The derived electron-capture rates on Kr86 from the experimental Gamow-Teller strength distribution are much smaller than the rates estimated based on the single-state approximation. Rates based on Gamow-Teller strengths estimated in shell-model and QRPA calculations are more accurate. The core-collapse supernova simulation with electron-capture rates based on the QRPA calculations indicate a significant reduction in the deleptonization during the collapse phase. Conclusions: It is important to utilize microscopic theoretical models that are tested by experimental data to constrain and estimate Gamow-Teller strengths and derived electron-capture rates for nuclei near N=50 that are inputs for astrophysical simulations of core-collapse supernovae and their multimessenger signals, such as the emission of neutrinos and gravitational waves.

Excited states of the neutron-rich isotopes $^{42,44}\mathrm{S}$ and $^{41,43}\mathrm{P}$ have been studied via inverse-kinematics proton scattering from a liquid hydrogen target, using the GRETINA $\ensuremath{\gamma}$-ray tracking array to extract inelastic-scattering cross sections. Deformation lengths of the ${2}_{1}^{+}$ excitations in $^{42,44}\mathrm{S}$ have been determined and, when combined with deformation lengths determined with electromagnetic probes, yield the ratio of neutron-to-proton matrix elements ${M}_{n}/{M}_{p}$ for the ${2}_{1}^{+}$ excitations in these nuclei. The present results for $^{41,43}\mathrm{P}(p,{p}^{\ensuremath{'}})$ are used to compare two shell-model interactions, SDPF-U and SDPF-MU. As in a recent study of $^{42}\mathrm{Si}$, the present results on $^{41,43}\mathrm{P}$ favor the SDPF-MU interaction.

The development of advanced γ-ray tracking arrays allows for a sensitive new technique to investigate elusive states of exotic nuclei with fast rare-isotope beams. By taking advantage of the excellent energy and position resolution of the Gamma-Ray Energy Tracking In-beam Nuclear Array, we developed a novel technique to identify in-flight isomeric decays of the 0⁺₂ state in 32Mg populated in a two-proton removal reaction. We confirm the 0⁺₂→2+1γ-ray transition of ³²Mg and constrain the 0⁺₂ decay lifetime, suggesting a large collectivity. The small partial cross section populating the 0⁺₂ state in this reaction provides experimental evidence for the reduced occupancy of the normal configuration of the 0⁺₂ state, indicating the intruder dominance of this state.

Angle-integrated cross-section measurements of the $^{56}$Ni(d,n) and (d,p) stripping reactions have been performed to determine the single-particle strengths of low-lying excited states in the mirror nuclei pair $^{57}$Cu-$^{57}$Ni situated adjacent to the doubly magic nucleus $^{56}$Ni. The reactions were studied in inverse kinematics utilizing a beam of radioactive $^{56}$Ni ions in conjunction with the GRETINA $\gamma$-array. Spectroscopic factors are compared with new shell-model calculations using a full $pf$ model space with the GPFX1A Hamiltonian for the isospin-conserving strong interaction plus Coulomb and charge-dependent Hamiltonians. These results were used to set new constraints on the $^{56}$Ni(p,$\gamma$)$^{57}$Cu reaction rate for explosive burning conditions in x-ray bursts, where $^{56}$Ni represents a key waiting point in the astrophysical rp-process., Comment: Final version accepted and published. 5 pages, 2 figures

Author(s): Elman, B; Gade, A; Janssens, RVF; Ayangeakaa, AD; Bazin, D; Belarge, J; Bender, PC; Brown, BA; Campbell, CM; Carpenter, MP; Crawford, HL; Crider, BP; Fallon, P; Forney, AM; Harker, J; Liddick, SN; Longfellow, B; Lunderberg, E; Prokop, CJ; Sethi, J; Taniuchi, R; Walters, WB; Weisshaar, D; Zhu, S | Abstract: The neutron-rich Ni isotopes have attracted attention in recent years because of the occurrence of shape or configuration coexistence. We report on the difference in population of excited final states in Ni70 following γ-ray tagged one-proton, one-neutron, and two-proton knockout from Cu71, Ni71, and Zn72 rare-isotope beams, respectively. Using variations observed in the relative transition intensities, signaling the changed population of specific final states in the different reactions, the role of neutron and proton configurations in excited states of Ni70 is probed schematically, with the goal of identifying those that carry, as leading configuration, proton excitations across the Z=28 shell closure. Such states are suggested in the literature to form a collective structure associated with prolate deformation. Adding to the body of knowledge for Ni70, 29 new transitions are reported, of which 15 are placed in its level scheme.

We report on the observation of excited states in the neutron-deficient phosphorus isotopes $^{26,27,28}\mathrm{P}$ via in-beam $\ensuremath{\gamma}$-ray spectroscopy with both high-efficiency and high-resolution detector arrays. In $^{26}\mathrm{P}$, a previously unobserved level has been identified at 244(3) keV, two new measurements of the astrophysically important $3/{2}^{+}$ resonance in $^{27}\mathrm{P}$ have been performed, $\ensuremath{\gamma}$ decays have been assigned to the proton-unbound levels at 2216 and 2483 keV in $^{28}\mathrm{P}$, and the $\ensuremath{\gamma}$-ray line-shape method has been used to make the first determination of the lifetimes of the two lowest-lying excited states in $^{28}\mathrm{P}$. The expected Thomas-Ehrman shifts were calculated and applied to levels in the mirror nuclei. The resulting level energies from this procedure were then compared with the energies of known states in $^{26,27,28}\mathrm{P}$.

The ^{23}Al(p,γ)^{24}Si reaction is among the most important reactions driving the energy generation in type-I x-ray bursts. However, the present reaction-rate uncertainty limits constraints on neutron star properties that can be achieved with burst model-observation comparisons. Here, we present a novel technique for constraining this important reaction by combining the GRETINA array with the neutron detector LENDA coupled to the S800 spectrograph at the National Superconducting Cyclotron Laboratory. The ^{23}Al(d,n) reaction was used to populate the astrophysically important states in ^{24}Si. This enables a measurement in complete kinematics for extracting all relevant inputs necessary to calculate the reaction rate. For the first time, a predicted close-lying doublet of a 2_{2}^{+} and (4_{1}^{+},0_{2}^{+}) state in ^{24}Si was disentangled, finally resolving conflicting results from two previous measurements. Moreover, it was possible to extract spectroscopic factors using GRETINA and LENDA simultaneously. This new technique may be used to constrain other important reaction rates for various astrophysical scenarios.

A more detailed test of the implementation of nuclear forces that drive shell evolution in the pivotal nucleus ^{42}Si-going beyond earlier comparisons of excited-state energies-is important. The two leading shell-model effective interactions, SDPF-MU and SDPF-U-Si, both of which reproduce the low-lying ^{42}Si(2_{1}^{+}) energy, but whose predictions for other observables differ significantly, are interrogated by the population of states in neutron-rich ^{42}Si with a one-proton removal reaction from ^{43}P projectiles at 81 MeV/nucleon. The measured cross sections to the individual ^{42}Si final states are compared to calculations that combine eikonal reaction dynamics with these shell-model nuclear structure overlaps. The differences in the two shell-model descriptions are examined and linked to predicted low-lying excited 0^{+} states and shape coexistence. Based on the present data, which are in better agreement with the SDPF-MU calculations, the state observed at 2150(13) keV in ^{42}Si is proposed to be the (0_{2}^{+}) level.

We present a high-resolution in-beam γ-ray spectroscopy study of excited states in the mirror nuclei 55Co and 56Ni following one-nucleon knockout from a projectile beam of 56Ni. The newly determined partial cross sections and the γ-decay properties of excited states provide a test of state-of-the-art nuclear structure models and probe mirror symmetry in unique ways. The new experimental data are compared to large-scale shell-model calculations in the full pf space and including charge-dependent contributions. A mirror asymmetry for the partial cross sections leading to the two lowest 3/2− states in the A = 55 mirror pair was identified as well as a significant difference in the E1 decays from the 1/21+ state to the same two 3/2− states. The mirror asymmetry in the partial cross sections cannot be reconciled with the present shell-model picture or small mixing introduced in a two-state model. The observed mirror asymmetry in the E decay pattern, however, points at stronger mixing between the two lowest 3/2− states in 55Co than in its mirror 55Ni.

Excited states in the neutron-rich 70 Fe nucleus were populated in a one-proton removal reaction from 71 Co projectiles at 87 MeV/nucleon. A new transition was observed with the γ -ray tracking array GRETINA and shown to feed the previously assigned 4+ 1 state. In comparison to reaction theory calculations with shell-model spectroscopic factors, it is argued that the new γ ray possibly originates from the 6+ 1 state. It is further shown that the Doppler-reconstructed γ -ray spectra are sensitive to the very different lifetimes of the 2+ and 4+ states, enabling their approximate measurement. The emerging structure of 70 Fe is discussed in comparison to LNPS-new large-scale shell-model calculations.

Background: Selenium and germanium nuclei are associated with both triaxiality and shape coexistence. The relative influence of these deformation effects on the low-lying nuclear structure remains the subject of much discussion with additional attention drawn to $^{76}\mathrm{Se}$ and $^{76}\mathrm{Ge}$ due to the potential for the observation of neutrinoless double-$\ensuremath{\beta}$ decay.Purpose: Experimental observables related to the deformation of $^{76}\mathrm{Se}$ are lacking in precision. The purpose of the present paper is to provide electric quadrupole matrix elements with improved precision in order to determine the deformation of low-lying states in a model-independent manner.Methods: Sub-barrier Coulomb excitation was employed at the reaccelerated beam facility of the National Superconducting Cyclotron Laboratory using the JANUS setup. Using this method nineteen $E2$ matrix elements were extracted.Results: Extracted matrix elements agree within uncertainties with those in the literature but with improved precision. Through both a comparison with geometric models and a model-independent evaluation of $E2$ matrix elements using rotational invariants, the ground state of $^{76}\mathrm{Se}$ is best described as having a significant triaxial component, but is not maximally triaxially deformed.Conclusions: Selenium-76 exhibits a significant degree of triaxiality in its ground state. A detailed comparison with configuration-interaction calculations indicates that this can be well reproduced theoretically.

An enhanced low-energy electric dipole ($E1$) strength is identified for the weakly bound excited states of the neutron-rich isotope $^{27}\mathrm{Ne}$. The Doppler-shift lifetime measurements employing a combination of the $\ensuremath{\gamma}$-ray tracking array GRETINA, the plunger device, and the S800 spectrograph determine the lower limit of $0.030\text{ }\text{ }{e}^{2}\text{ }{\mathrm{fm}}^{2}$ or 0.052 W.u. for the $1/{2}^{+}\ensuremath{\rightarrow}3/{2}^{\ensuremath{-}}\text{ }\text{ }E1$ transition in $^{27}\mathrm{Ne}$, representing one of the strongest $E1$ strengths observed among the bound discrete states in this mass region. This value is at least 30 times larger than that measured for the $3/{2}^{\ensuremath{-}}$ decay to the $3/{2}_{gs}^{+}$ ground state. A comparison of the present results to large-scale shell-model calculations points to an important role of core excitations and deformation in the observed $E1$ enhancement, suggesting a novel example of the electric dipole modes manifested in weakly bound deformed systems.

Energy differences between isobaric analogue states have been extracted for the A = 79 , 79Zr/79Y mirror pair following their population via nucleon-knockout reactions from intermediate-energy rare-isotope beams. These are the heaviest nuclei where such measurements have been made to date. The deduced mirror energy differences (MED) are compared with predictions from a new density-functional based approach, incorporating isospin-breaking effects of both Coulomb and nuclear charge-symmetry breaking and configuration mixing.

Neutron-deficient selenium isotopes are thought to undergo a rapid shape change from a prolate deformation near the line of beta stability towards oblate deformation around the line of N=Z. The point at which this shape change occurs is unknown, with inconsistent predictions from available theoretical models. A common feature in the models is the delicate nature of the point of transition, with the introduction of even a modest spin to the system sufficient to change the ordering of the prolate and oblate configurations. We present a measurement of the quadrupole moment of the first-excited state in radioactive ^{72}Se-a potential point of transition-by safe Coulomb excitation. This is the first low-energy Coulomb excitation to be performed with a rare-isotope beam at the reaccelerated beam facility at the National Superconducting Cyclotron Laboratory. By demonstrating a negative spectroscopic quadrupole moment for the first-excited 2^{+} state, it is found that any low-spin shape change in neutron-deficient selenium does not occur until ^{70}Se.

Lifetime measurements of excited states in the neutron-rich nucleus $^{43}\mathrm{S}$ were performed by applying the recoil-distance method on fast rare-isotope beams in conjunction with the Gamma-Ray Energy Tracking In-beam Nuclear Array. The new data based on $\ensuremath{\gamma}\ensuremath{\gamma}$ coincidences and lifetime measurements resolve a doublet of $(3/{2}^{\ensuremath{-}})$ and $(5/{2}^{\ensuremath{-}})$ states at low excitation energies. Results were compared to the $\ensuremath{\pi}(sd)\ensuremath{-}\ensuremath{\nu}(pf)$ shell model and antisymmetrized molecular dynamics calculations. The consistency with the theoretical calculations identifies a possible appearance of three coexisting bands near the ground state of $^{43}\mathrm{S}$: the ${K}^{\ensuremath{\pi}}=1/{2}^{\ensuremath{-}}$ band built on a prolate-deformed ground state, a band built on an isomer with a $1{f}_{7/2}^{\ensuremath{-}1}$ character, and a suggested excited band built on a newly discovered doublet state. The latter further confirms the collapse of the $N=28$ shell closure in the neutron-rich region.

CITATION: Longfellow, B., et al. 2018. Measurement of key resonances for the 24Al( p,γ )25Si reaction rate using in-beam γ -ray spectroscopy. Physical Review C, 97(5):054307, doi:10.1103/PhysRevC.97.054307.

We report $B(E2;{0}_{1}^{+}\ensuremath{\rightarrow}{2}_{n}^{+})$ strengths for the neutron-rich $^{88,90}\mathrm{Kr}$ and $^{86}\mathrm{Se}$ isotopes from intermediate-energy Coulomb excitation. The electric quadrupole transition strengths to the first ${2}^{+}$ states complete, with considerably improved uncertainties, the evolution of quadrupole collectivity in the Kr and Se isotopes approaching $N=60$, for which $^{90}\mathrm{Kr}$ and $^{86}\mathrm{Se}$ had previously been the most uncertain. We also report significant excitation strength to several higher-lying ${2}^{+}$ states in the krypton isotopes. This fragmentation of $B(E2)$ strength in $^{88,90}\mathrm{Kr}$ confirms shell-model calculations in the $\ensuremath{\pi}(fpg)\text{\ensuremath{-}}\ensuremath{\nu}(sdgh)$ shell with an only minimally tuned shell-model setup that is based on a nucleon-nucleon interaction derived from effective field theory and effective charges adjusted to $^{86}\mathrm{Kr}$.

The 23 Al(p, γ)24 Si stellar reaction rate has a significant impact on the light-curve emitted in X-ray bursts. Theoretical calculations show that the reaction rate is mainly determined by the properties of direct capture as well as low-lying 2+ states and a possible 4+ state in 24 Si. Currently, there is little experimental information on the properties of these states.In this proceeding we will present a new experimental study to investigate this reaction, using the surrogate reaction 23 Al(d,n) at 47 AMeV at the National Superconducting Cyclotron Laboratory (NSCL). We will discuss our new experimental setup which allows us to use full kinematics employing the Gamma-Ray Energy Tracking In-beam Nuclear Array (GRETINA) to detect the γ-rays following the de-excitation of excited states of the reaction products and the Low Energy Neutron Detector Array (LENDA) to detect the recoiling neutrons. The S800 was used for identification of the 24 Si recoils. As a proof of principle to show the feasibility of this concept the Q-value spectrum of 22 Mg(d,n)23 Al is reconstructed.

© 2016 Elsevier B.V. The γ-ray tracking array GRETINA was coupled to the S800 magnetic spectrometer for spectroscopy with fast beams of rare isotopes at the National Superconducting Cyclotron Laboratory on the campus of Michigan State University. We describe the technical details of this powerful setup and report on GRETINA's performance achieved with source and in-beam measurements. The γ-ray multiplicity encountered in experiments with fast beams is usually low, allowing for a simplified and efficient treatment of the data in the γ-ray analysis in terms of Doppler reconstruction and spectral quality. The results reported in this work were obtained from GRETINA consisting of 8 detector modules hosting four high-purity germanium crystals each. Currently, GRETINA consists of 10 detector modules.

Markov state models (MSMs), which model conformational dynamics as a network of transitions between metastable states, have been increasingly used to model the thermodynamics and kinetics of biomolecules. In considering perturbations to molecular dynamics induced by sequence mutations, chemical modifications, or changes in external conditions, it is important to assess how transition rates change, independent of changes in metastable state definitions. Here, we present a surprisal metric to quantify the difference in metastable state transitions for two closely related MSMs, taking into account the statistical uncertainty in observed transition counts. We show that the surprisal is a relative entropy metric closely related to the Jensen-Shannon divergence between two MSMs, which can be used to identify conformational states most affected by perturbations. As examples, we apply the surprisal metric to a two-dimensional lattice model of a protein hairpin with mutations to hydrophobic residues, all-atom simulations of the Fs peptide α-helix with a salt-bridge mutation, and a comparison of protein G β-hairpin with its trpzip4 variant. Moreover, we show that surprisal-based adaptive sampling is an efficient strategy to reduce the statistical uncertainty in the Jensen-Shannon divergence, which could be a useful strategy for molecular simulation-based ab initio design.

Markov State Model (MSM) approaches model the conformational dynamics of proteins as a kinetic network of metastable states. This allows one to obtain long-timescale and equilibrium information from ensembles of much shorter non-equilibrium trajectories sampling local transition rates between states. To explore the possibility of using MSMs to efficiently characterize the effects of sequence perturbations, we construct “wildtype” and “mutant” MSMs built from molecular dynamics simulations of Fs peptide, the GB1 hairpin, and WW domain. We show that metastable states are generally robust to perturbation, although unfolded states may suffer from finite sampling. To assess the statistical significance of changes in observed transition counts that occur upon mutation, we develop a log-likelihood surprisal metric. We validate the metric in simple lattice models, and apply it to study sequence-dependent folding mechanisms and our ability to efficiently sample them.