Search

The double-electron capture and the electron capture with positron emission in $^{168}$Yb have been investigated for the first time at the STELLA facility of the Gran Sasso underground laboratory (Italy) measuring 371 g of highly purified ytterbium oxide placed on the end-cap of a 465 cm$^3$ ultra-low-background high purity Germanium detector (HPGe). No gamma associated to double beta processes in $^{168}$Yb have been observed after 2074 h of data taking. This has allowed setting the half-life limits on the level of $\lim T_{1/2}\sim$ $10^{14}-10^{18}$ yr at 90\% C.L. Particularly, a lower half-life limit on a possible resonant neutrinoless double-electron capture in $^{168}$Yb to the $(2)^-$ 1403.7 keV excited state of $^{168}$Er is set as $T_{1/2}\geq1.9\times 10^{18}$ yr at 90\% C.L. Half-life limits $T_{1/2}^{2\nu(0\nu)}\geq 4.5(4.3)\times10^{16}$ yr were set on the $2\nu(0\nu)2\beta^-$ decay of $^{176}$Yb to the $2^+$ 84.3 keV first excited level of $^{176}$Hf., Comment: 23 pages, 6 figures, 4 tables

The first search for double electron capture ($2\varepsilon$) and electron capture with positron emission ($\varepsilon\beta^+$) of $^{162}$Er to the ground state and to several excited levels of $^{162}$Dy was realized with 326 g of highly purified erbium oxide. The sample was measured over 1934 h by the ultra-low background HP Ge $\gamma$ spectrometer GeCris (465 cm$^3$) at the Gran Sasso underground laboratory. No effect was observed, the half-life limits were estimated at the level of $\lim T_{1/2}\sim 10^{15}-10^{18}$ yr. A possible resonant $0\nu KL_1$ capture in $^{162}$Er to the $2^+$ 1782.7 keV excited state of $^{162}$Dy is restricted as $T_{1/2}\geq5.0\times 10^{17}$ yr at 90% C.L. A new improved half-life limit $T_{1/2}\geq4.1\times 10^{17}$ yr was set on the $2\beta^-$ decay of $^{170}$Er to the $2^+$ 84.3 keV first excited state of $^{170}$Yb., Comment: 23 pages, 6 figures and 4 tables

We report recent achievements in the development of scintillating bolometers to search for neutrinoless double-beta decay of $^{100}$Mo. The presented results have been obtained in the framework of the LUMINEU, LUCIFER and EDELWEISS collaborations, and are now part of the R\&D activities towards CUPID (CUORE Update with Particle IDentification), a proposed next-generation double-beta decay experiment based on the CUORE experience. We have developed a technology for the production of large mass ($\sim$1 kg), high optical quality, radiopure zinc and lithium molybdate crystal scintillators (ZnMoO$_4$ and Li$_2$MoO$_4$, respectively) from deeply purified natural and $^{100}$Mo-enriched molybdenum. The procedure is applied for a routine production of enriched crystals. Furthermore, the technology of a single detector module consisting of a large-volume ($\sim 100$~cm$^3$) Zn$^{100}$MoO$_4$ and Li$_2$$^{100}$MoO$_4$ scintillating bolometer has been established, demonstrating performance and radiopurity that are close to satisfy the demands of CUPID. In particular, the FWHM energy resolution of the detectors at 2615 keV --- near the $Q$-value of the double-beta transition of $^{100}$Mo (3034~keV) --- is $\approx$ 4--10~keV. The achieved rejection of $\alpha$-induced dominant background above 2.6~MeV is at the level of more than 99.9\%. The bulk activity of $^{232}$Th ($^{228}$Th) and $^{226}$Ra in the crystals is below 10 $\mu$Bq/kg. Both crystallization and detector technologies favor Li$_2$MoO$_4$, which was selected as a main element for the realization of a CUPID demonstrator (CUPID-0/Mo) with $\sim$7 kg of $^{100}$Mo.

The technology of scintillating bolometers based on zinc molybdate (ZnMoO4) crystals is under development within the LUMINEU project to search for decay of 100Mo with the goal to set the basis for large scale experiments capable to explore the inverted hierarchy region of the neutrino mass pattern. Advanced ZnMoO4 crystal scintillators with mass of ∼0.3 kg were developed and Zn100MoO4 crystal from enriched 100Mo was produced for the first time by using the low-thermal-gradient Czochralski technique. One ZnMoO4 scintillator and two samples (59 g and 63 g) cut from the enriched boule were tested aboveground at milli-Kelvin temperature as scintillating bolometers showing a high detection performance. The first results of the low background measurements with three ZnMoO4 and two enriched detectors installed in the EDELWEISS set-up at the Modane Underground Laboratory (France) are presented.

A search for double β processes in 106Cd was carried out at the Gran Sasso National Laboratories of the INFN (Italy) with the help of a 106CdWO4 crystal scintillator (215 g) enriched in 106Cd up to 66%. After 6590 h of data taking, new improved half-life limits on the double β decay processes in 106Cd were established at the level of 1019–1021 yr; in particular, T 2νεβ+ 1/2 2.1 × 1020 yr, T 2ν2β+ 1/2 4.3 × 1020 yr, and T 0ν2ε 1/2 1.0 × 1021 yr. The resonant neutrinoless double-electron captures to the 2718-, 2741-, and 2748-keV excited states of 106Pd are restricted to T 0ν2K 1/2 4.3 × 1020 yr, T 0νKL1 1/2 9.5 × 1020 yr, and T 0νKL3 1/2 4.3 × 1020 yr, respectively (all limits at 90% confidence level). A possible resonant enhancement of the 0ν2ε processes is estimated in the framework of the quasiparticle random phase approximation (QRPA) approach. Radioactive contamination of the 106CdWO4 crystal scintillator is reported. peerReviewed