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13 results on '"Bellosta von Colbe, J. M."'

1. Magnesium based materials for hydrogen based energy storage: Past, present and future

Author

Yartys, V. A., Lototskyy, M. V., Akiba, E., Albert, R., Antonov, V. E., Ares, J. R., Baricco, M., Bourgeois, N., Buckley, C. E., Bellosta von Colbe, J. M., Crivello, J. C., Cuevas, F., Denys, R. V., Dornheim, M., Felderhoff, M., Grant, D. M., Hauback, B. C., Humphries, T. D., Jacob, I., Jensen, T. R., de Jongh, P. E., Joubert, J. M., Kuzovnikov, M. A., Latroche, M., Paskevicius, M., Pasquini, L., Popilevsky, L., Skripnyuk, V. M., Rabkin, E., Sofianos, M. V., Stuart, A., Walker, G., Wang, Hui, Webb, C. J., Zhu, Min, Yartys, V. A., Lototskyy, M. V., Akiba, E., Albert, R., Antonov, V. E., Ares, J. R., Baricco, M., Bourgeois, N., Buckley, C. E., Bellosta von Colbe, J. M., Crivello, J. C., Cuevas, F., Denys, R. V., Dornheim, M., Felderhoff, M., Grant, D. M., Hauback, B. C., Humphries, T. D., Jacob, I., Jensen, T. R., de Jongh, P. E., Joubert, J. M., Kuzovnikov, M. A., Latroche, M., Paskevicius, M., Pasquini, L., Popilevsky, L., Skripnyuk, V. M., Rabkin, E., Sofianos, M. V., Stuart, A., Walker, G., Wang, Hui, Webb, C. J., and Zhu, Min

Abstract

Magnesium hydride owns the largest share of publications on solid materials for hydrogen storage. The “Magnesium group” of international experts contributing to IEA Task 32 “Hydrogen Based Energy Storage” recently published two review papers presenting the activities of the group focused on magnesium hydride based materials and on Mg based compounds for hydrogen and energy storage. This review article not only overviews the latest activities on both fundamental aspects of Mg-based hydrides and their applications, but also presents a historic overview on the topic and outlines projected future developments. Particular attention is paid to the theoretical and experimental studies of Mg-H system at extreme pressures, kinetics and thermodynamics of the systems based on MgH 2 , nanostructuring, new Mg-based compounds and novel composites, and catalysis in the Mg based H storage systems. Finally, thermal energy storage and upscaled H storage systems accommodating MgH 2 are presented.

Published
2019

2. Magnesium based materials for hydrogen based energy storage: Past, present and future

Author

Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Yartys, V. A., Lototskyy, M. V., Akiba, E., Albert, R., Antonov, V. E., Ares, J. R., Baricco, M., Bourgeois, N., Buckley, C. E., Bellosta von Colbe, J. M., Crivello, J. C., Cuevas, F., Denys, R. V., Dornheim, M., Felderhoff, M., Grant, D. M., Hauback, B. C., Humphries, T. D., Jacob, I., Jensen, T. R., de Jongh, P. E., Joubert, J. M., Kuzovnikov, M. A., Latroche, M., Paskevicius, M., Pasquini, L., Popilevsky, L., Skripnyuk, V. M., Rabkin, E., Sofianos, M. V., Stuart, A., Walker, G., Wang, Hui, Webb, C. J., Zhu, Min, Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Yartys, V. A., Lototskyy, M. V., Akiba, E., Albert, R., Antonov, V. E., Ares, J. R., Baricco, M., Bourgeois, N., Buckley, C. E., Bellosta von Colbe, J. M., Crivello, J. C., Cuevas, F., Denys, R. V., Dornheim, M., Felderhoff, M., Grant, D. M., Hauback, B. C., Humphries, T. D., Jacob, I., Jensen, T. R., de Jongh, P. E., Joubert, J. M., Kuzovnikov, M. A., Latroche, M., Paskevicius, M., Pasquini, L., Popilevsky, L., Skripnyuk, V. M., Rabkin, E., Sofianos, M. V., Stuart, A., Walker, G., Wang, Hui, Webb, C. J., and Zhu, Min

Published
2019

4. A novel catalytic route for hydrogenation–dehydrogenation of 2LiH + MgB2via in situ formed core–shell LixTiO2 nanoparticles

Author

Puszkiel, J. A., primary, Castro Riglos, M. V., additional, Ramallo-López, J. M., additional, Mizrahi, M., additional, Karimi, F., additional, Santoru, A., additional, Hoell, A., additional, Gennari, F. C., additional, Larochette, P. Arneodo, additional, Pistidda, C., additional, Klassen, T., additional, Bellosta von Colbe, J. M., additional, and Dornheim, M., additional

Published
2017
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6. A novel catalytic route for hydrogenation–dehydrogenation of 2LiH + MgB2via in situ formed core–shell LixTiO2 nanoparticles.

Author

Puszkiel, J. A., Castro Riglos, M. V., Ramallo-López, J. M., Mizrahi, M., Karimi, F., Santoru, A., Hoell, A., Gennari, F. C., Larochette, P. Arneodo, Pistidda, C., Klassen, T., Bellosta von Colbe, J. M., and Dornheim, M.

Abstract

Aiming to improve the hydrogen storage properties of 2LiH + MgB2 (Li-RHC), the effect of TiO2 addition to Li-RHC is investigated. The presence of TiO2 leads to the in situ formation of core–shell LixTiO2 nanoparticles during milling and upon heating. These nanoparticles markedly enhance the hydrogen storage properties of Li-RHC. Throughout hydrogenation–dehydrogenation cycling at 400 °C a 1 mol% TiO2 doped Li-RHC material shows sustainable hydrogen capacity of ∼10 wt% and short hydrogenation and dehydrogenation times of just 25 and 50 minutes, respectively. The in situ formed core–shell LixTiO2 nanoparticles confer proper microstructural refinement to the Li-RHC, thus preventing the material's agglomeration upon cycling. An analysis of the kinetic mechanisms shows that the presence of the core–shell LixTiO2 nanoparticles accelerates the one-dimensional interface-controlled mechanism during hydrogenation owing to the high Li+ mobility through the LixTiO2 lattice. Upon dehydrogenation, the in situ formed core–shell LixTiO2 nanoparticles do not modify the dehydrogenation thermodynamic properties of the Li-RHC itself. A new approach by the combination of two kinetic models evidences that the activation energy of both MgH2 decomposition and MgB2 formation is reduced. These improvements are due to a novel catalytic mechanism via Li+ source/sink reversible reactions. [ABSTRACT FROM AUTHOR]

Published
2017
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7. Changing the dehydrogenation pathway of LiBH4–MgH2via nanosized lithiated TiO2.

Author

Puszkiel, J. A., Castro Riglos, M. V., Karimi, F., Santoru, A., Pistidda, C., Klassen, T., Bellosta von Colbe, J. M., and Dornheim, M.

Abstract

Nanosized lithiated titanium oxide (LixTiO2) noticeably improves the kinetic behaviour of 2LiBH4 + MgH2. The presence of LixTiO2 reduces the time required for the first dehydrogenation by suppressing the intermediate reaction to Li2B12H12, leading to direct MgB2 formation. [ABSTRACT FROM AUTHOR]

Published
2017
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8. LiF−MgB2 System for Reversible Hydrogen Storage

Author

Gosalawit-Utke, R., primary, Bellosta von Colbe, J. M., additional, Dornheim, M., additional, Jensen, T. R., additional, Cerenius, Y., additional, Bonatto Minella, Christian, additional, Peschke, Maik, additional, and Bormann, R., additional

Published
2010
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11. LiF−MgB2System for Reversible Hydrogen Storage

Author

Gosalawit-Utke, R., Bellosta von Colbe, J. M., Dornheim, M., Jensen, T. R., Cerenius, Y., Bonatto Minella, Christian, Peschke, Maik, and Bormann, R.

Abstract

LiF−MgB2composites are proposed for reversible hydrogen storage. With respect to pure LiBH4, a significantly kinetic destabilization regarding hydrogenation and dehydrogenation is accomplished. The reversible hydrogen storage capacity is up to 6.4 wt %. The kinetic properties are improved significantly during cycling. The formations of the hydridofluoride phases (LiBH4−yFyand LiH1−xFx) are observed by in situ synchrotron X-ray diffraction (XRD) and attenuated total reflection Fourier transform infrared spectroscopy (ATR-FTIR). Hydrogenation and dehydrogenation mechanisms are described on the basis of the formation and decomposition of the hydridofluoride phases, respectively.

Published
2010
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12. Magnesium based materials for hydrogen based energy storage: Past, present and future

Author

Yartys, V. A., Lototskyy, M. V., Akiba, E., Albert, R., Antonov, V. E., Ares, J. R., Baricco, M., Bourgeois, N., Buckley, C. E., Bellosta von Colbe, J. M., Crivello, J. C., Cuevas, F., Denys, R. V., Dornheim, M., Felderhoff, M., Grant, D. M., Hauback, B. C., Humphries, T. D., Jacob, I., Jensen, T. R., de Jongh, P. E., Joubert, J. M., Kuzovnikov, M. A., Latroche, M., Paskevicius, M., Pasquini, L., Popilevsky, L., Skripnyuk, V. M., Rabkin, E., Sofianos, M. V., Stuart, A., Walker, G., Wang, Hui, Webb, C. J., Zhu, Min, Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Institute for Energy Technology, PO Box 40, 2007, Kjeller, Norway (INSTITUTE FOR ENERGY TECHNOLOGY, PO BOX 40, 2007, KJELLER, NORWAY), Institute for Energy Technology, PO Box 40, 2007, Kjeller, Norway, University of the Western Cape, Kyushu University [Fukuoka], Max-Planck-Institut für Kohlenforschung (Coal Research), Max-Planck-Gesellschaft, Institute of Solid State Physics (ISSP, RAS), Russian Academy of Sciences [Moscow] (RAS), Universidad Autonoma de Madrid (UAM), Dipartimento di Chimica IFM, Università degli studi di Torino (UNITO), Institut de Chimie et des Matériaux Paris-Est (ICMPE), Institut de Chimie du CNRS (INC)-Université Paris-Est Créteil Val-de-Marne - Paris 12 (UPEC UP12)-Centre National de la Recherche Scientifique (CNRS), Curtin University [Perth], Planning and Transport Research Centre (PATREC), Helmholtz-Zentrum Geesthacht (GKSS), University of Nottingham, UK (UON), Ben-Gurion University of the Negev (BGU), Interdisciplinary Nanoscience Center (iNANO), Aarhus University [Aarhus], Utrecht University [Utrecht], Max Planck Institute for Chemistry (MPIC), University of Bologna [Italy], Technion - Israel Institute of Technology [Haifa], South China University of Technology [Guangzhou] (SCUT), Griffith University [Brisbane], Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Osipyan Institute of Solid State Physics (ISSP), Universidad Autónoma de Madrid (UAM), Università degli studi di Torino = University of Turin (UNITO), Université Paris-Est Créteil Val-de-Marne - Paris 12 (UPEC UP12)-Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie du CNRS (INC), Yartys, V.A., Lototskyy, M.V., Akiba, E., Albert, R., Antonov, V.E., Ares, J.R., Baricco, M., Bourgeois, N., Buckley, C.E., Bellosta von Colbe, J.M., Crivello, J.-C., Cuevas, F., Denys, R.V., Dornheim, M., Felderhoff, M., Grant, D.M., Hauback, B.C., Humphries, T.D., Jacob, I., Jensen, T.R., de Jongh, P.E., Joubert, J.-M., Kuzovnikov, M.A., Latroche, M., Paskevicius, M., Pasquini, L., Popilevsky, L., Skripnyuk, V.M., Rabkin, E., Sofianos, M.V., Stuart, A., Walker, G., Wang, Hui, Webb, C.J., and Zhu, Min

Subjects
Magnesium-based hydrides, Materials science, Hydrogen, chemistry.chemical_element, Energy Engineering and Power Technology, 02 engineering and technology, Solid material, Applications, Catalysis, High pressures, Kinetics, Nanostructuring, Renewable Energy, Sustainability and the Environment, Fuel Technology, Condensed Matter Physics, 010402 general chemistry, Thermal energy storage, 01 natural sciences, 7. Clean energy, Energy storage, Catalysi, Hydrogen storage, chemistry.chemical_compound, Renewable Energy, Process engineering, Kinetic, Sustainability and the Environment, Magnesium, business.industry, Magnesium hydride, [CHIM.MATE]Chemical Sciences/Material chemistry, 021001 nanoscience & nanotechnology, 0104 chemical sciences, High pressure, chemistry, 13. Climate action, Magnesium-based hydride, 0210 nano-technology, business
Abstract

Magnesium hydride owns the largest share of publications on solid materials for hydrogen storage. The “Magnesium group” of international experts contributing to IEA Task 32 “Hydrogen Based Energy Storage” recently published two review papers presenting the activities of the group focused on magnesium hydride based materials and on Mg based compounds for hydrogen and energy storage. This review article not only overviews the latest activities on both fundamental aspects of Mg-based hydrides and their applications, but also presents a historic overview on the topic and outlines projected future developments. Particular attention is paid to the theoretical and experimental studies of Mg-H system at extreme pressures, kinetics and thermodynamics of the systems based on MgH 2 , nanostructuring, new Mg-based compounds and novel composites, and catalysis in the Mg based H storage systems. Finally, thermal energy storage and upscaled H storage systems accommodating MgH 2 are presented.

Full Text
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13. Changing the dehydrogenation pathway of LiBH 4 -MgH 2 via nanosized lithiated TiO 2 .

Author

Puszkiel JA, Castro Riglos MV, Karimi F, Santoru A, Pistidda C, Klassen T, Bellosta von Colbe JM, and Dornheim M

Abstract

Nanosized lithiated titanium oxide (Li x TiO 2 ) noticeably improves the kinetic behaviour of 2LiBH 4 + MgH 2 . The presence of Li x TiO 2 reduces the time required for the first dehydrogenation by suppressing the intermediate reaction to Li 2 B 12 H 12 , leading to direct MgB 2 formation.

Published
2017
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