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The possible existence of an exotic phase of matter rigid like a solid but able to sustain persistent and dissipation-less flow like a superfluid, a "supersolid", has been the subject of intense theoretical and experimental efforts since the discovery of superfluidity in Helium-4. Recently, it has been proposed that nonlinear periodic modulations known as cnoidal waves, that naturally emerge in Bose-Einstein condensates, provide a promising platform to find and study supersolidity in nonequilibrium phases of matter. Nevertheless, so far the analysis has been limited to a one-dimensional zero-temperature system. By combining the dissipative Gross-Pitaevskii equation with a finite temperature holographic model, we show that the proposed cnoidal wave supersolid phases of matter are always energetically and dynamically unstable at finite temperature. We ascribe this instability to the dynamics of the "elastic" Goldstone mode arising as a direct consequence of translational order. Finally, we study the dynamical instability of the supersolid state and connect it to the production of topological defects during the relaxation towards a final homogeneous equilibrium state with smaller superflow current, similar to the Landau instability dynamics in superfluids. Our results suggest that the supersolidity of cnoidal waves can emerge only as a transient phenomenon and not as a truly equilibrium and stable ground state., Comment: 12 pages, 10 figures

The notion of defects in crystalline phases of matter has been extremely powerful for understanding crystal growth, deformation and melting. These discontinuities in the periodic order of crystals are mathematically described by the Burgers vector, derived from the particle displacements, which encapsulates the direction and magnitude of slip relative to the undeformed state. Since the reference structure of the crystal is known a priori, the Burgers vector can be determined experimentally using both imaging and diffraction methods to measure the lattice distortion, and thus infer the particle displacements. Glasses have structures that lack the periodicity of crystals, and thus a well-defined reference state. Yet, measurable structural parameters can still be obtained from diffraction from a glass. Here we examine the usefulness of these parameters to probe deformation in glasses. We find that coordinated transformations in the centrosymmetry of local particle arrangements are a strong marker of plastic events. Moreover, we investigate two geometric indicators that can be derived from distortions in local diffraction patterns, namely the continuous Burgers vector and the quadrupolar strain. We find that the Burgers vector again emerges as a robust and sensitive metric for understanding local structural transformations due to mechanical deformation, even in structural glasses., Comment: 13 pages 5 figures

Mechanical THz vibrations in nanocrystals have recently been harnessed for quantum sensing and thermal management. The free boundaries of nanocrystals introduce new surface wave solutions, analogous to the seismic waves on Earth, yet the implications of these surface waves on nanocrystals have remained largely unexplored. Here, we use atomistic molecular dynamics simulations and experimental neutron spectroscopy to elucidate these THz-scale features in nanodiamond. Our key insight is that thermally induced Rayleigh surface phonons, which have a low group velocity and an amplitude that decays exponentially away from the surface, are responsible for the previously observed but unexplained linear scaling of the low-energy vibrational density of states in nanocrystals. Large thermal atomic displacements, relative to the nanoparticle radius, induce perpetual surface quakes, even at ambient conditions. Normalised to the radius, the surface displacement ratio in diamond nanocrystals exceeds that of the largest recorded earthquakes by a factor of $10^{5\pm1}$. We explicate how these dramatic Rayleigh waves coexist with other distinctive features including confined lattice phonons, soft surface modes, the acoustic gap, Love waves, and Lamb modes, thereby offering a complete framework for the vibrational dynamics of nanocrystals., Comment: 14 pages

Because of the inevitably disordered background, structural defects are not well-defined concepts in amorphous solids. In order to overcome this difficulty, it has been recently proposed that topological defects can be still identified in the pattern of vibrational modes, by looking at the corresponding eigenvector field at low frequency. Moreover, it has been verified that these defects strongly correlate with the location of soft spots in glasses, that are the regions more prone to plastic rearrangements. Here, we show that the topology of vibrational modes predicts the location of structural defects in crystals as well, including the cases of dislocations, disclinations and Eshelby inclusions. Our results suggest that in crystalline solids topological defects in the vibrational modes are directly connected to the well-established structural defects governing plastic deformations and present characteristics very similar to those observed in amorphous solids., Comment: v1: comments welcome

The vibrational density of states is key to understanding the mechanical, thermal, and transport properties of materials. In amorphous solids, this density shows an excess of vibrational modes compared to the Debye model, known as the boson peak, whose origin remains poorly understood. Previous studies have suggested a link between the boson peak and quasi-localized nonphononic vibrations, or "defects." However, it has been difficult to clearly identify these defects, possibly because they hybridize with extended phonons, casting doubt on their existence and connection to the boson peak. In this work, we introduce a simple and practical method for separating hybridized phonons from localized vibrations. We show that phonons at the boson peak frequency hybridize with localized defects. These defects are anisotropic, compact, and exhibit oscillatory pure shear deformations. Their density correlates with the excess of vibrational modes at the boson peak frequency across various two- and three-dimensional systems, confirming that they are the microscopic origin of the boson peak.

The absence of a well-defined equilibrium reference configuration and the inevitable frequent atomic rearrangements have long obstructed the achievement of a complete atomic-level understanding of liquid dynamics and properties, a challenge that continues to be unresolved. The instantaneous normal mode (INM) approach, based on the diagonalization of the potential energy Hessian matrix in instantaneous liquid configurations, has been shown to be a promising starting point to predict thermodynamic and dynamical properties of liquids but presents several conceptual difficulties that remain to be addressed. More in general, due to the inability of capturing anharmonic effects, what INMs can tell us about liquid dynamics remains an open question. In this work, we provide a general set of ``experimental facts'' by performing a comprehensive INM analysis of several simulated systems, including Ar, Xe, N$_2$, CS$_2$, Ga and Pb, in a large range of temperatures from the solid to the gas phase. We first study the INM density of states (DOS) and compare it to the density of state function obtained from the velocity auto-correlation function. Secondly, we analyze the temperature dependence of the fraction of unstable modes and of the low-frequency slope of the INM DOS, in search of possible universal behaviors. We then explore the connection between INMs and other properties of liquids including the liquid-like to gas-like dynamical crossover and the momentum gap of collective shear waves. Moreover, we investigate the INM spectrum at low temperature upon approaching the solid phase, revealing the existence of a large fraction of unstable modes also in crystalline solids. Finally, we verify the existence of a recently discussed cusp-like singularity in the INM eigenvalue spectrum and reveal its complex behavior upon dialing temperature that challenges the existing theoretical models., Comment: v1: comments welcome

Viscosity is the resistance of a liquid to flow, governed by atomic-scale friction between its constituent atoms. While viscosity can be directly computed using the Green-Kubo formalism, this method does not fully elucidate the physical mechanisms underlying such momentum transport coefficient. In fact, the microscopic origin of liquid viscosity remains poorly understood. In this work, we calculate the viscosity of a $\mathrm{Cu_{50}Zr_{50}}$ metallic liquid and a Kob-Andersen model in a large range of temperatures and compare the results with a theoretical formula based on nonaffine linear response and instantaneous normal mode theory. This analysis reveals that only unstable localized instantaneous normal modes (ULINMs) contribute to viscosity, providing a microscopic definition of viscosity as diffusive momentum transport facilitated by local structural excitations mediated by ULINMs as precursors. Leveraging on the concept of configurational entropy, a quantitative model to connect viscosity with ULINMs is also proposed and validated in both the Arrhenius and non-Arrhenius regimes. In summary, our work provides a microscopic definition of liquid viscosity and highlights the fundamental role of ULINMs as its building blocks, ultimately opening the path to an atomic-scale prediction of viscosity in liquids and glasses., Comment: v1: comments welcome!

The underlying structural disorder renders the concept of topological defects in amorphous solids difficult to apply and hinders a first-principle identification of the microscopic carriers of plasticity and of the regions more prone to structural rearrangements ("soft spots"). Recently, it has been proposed that well-defined topological defects can still be identified in glasses, and correlated to local and global plasticity, by looking at the eigenvector field or the particle displacement field. Nevertheless, all the existing proposals and analyses are only valid in two spatial dimensions. In this work, we propose the idea of using hedgehog topological defects to characterize the plasticity of 3D glasses and to geometrically predict the location of their soft spots. We corroborate our proposal by simulating a Kremer-Grest 3D polymer glass, and by using both the normal mode eigenvector field and the displacement field around large plastic events. Our results confirm that a topological characterization of plasticity in glasses is feasible, and provide a concrete realization of this program in 3D amorphous systems., Comment: v1: comments welcome

Krylov complexity has recently emerged as a new paradigm to characterize quantum chaos in many-body systems. However, which features of Krylov complexity are prerogative of quantum chaotic systems and how they relate to more standard probes, such as spectral statistics or out-of-time-order correlators (OTOCs), remain open questions. Recent insights have revealed that in quantum chaotic systems Krylov state complexity exhibits a distinct peak during time evolution before settling into a well-understood late-time plateau. In this work, we propose that this Krylov complexity peak (KCP) is a hallmark of quantum chaotic systems and suggest that its height could serve as an `order parameter' for quantum chaos. We demonstrate that the KCP effectively identifies chaotic-integrable transitions in the mass-deformed Sachdev-Ye-Kitaev model at both infinite and finite temperature, aligning with results from spectral statistics and OTOCs. Our findings offer a new diagnostic tool for quantum chaos that is operator-independent, potentially leading to more `universal' insights and a deeper understanding of general properties in quantum chaotic systems., Comment: v1: 6 pages, 3 figures, v2: references added, minor changes, supplemental material included

Without Lorentz symmetry, generic fixed points of the renormalization group (RG) are labelled by their dynamical (or `Lifshitz') exponent $z$. Hence, a rich variety of possible RG flows arises. The first example is already given by the standard non-relativistic limit, which can be viewed as the flow from a $z=1$ UV fixed point to a $z=2$ IR fixed point. In strongly coupled theories, there are good arguments suggesting that Lorentz invariance can emerge dynamically in the IR from a Lorentz violating UV. In this work, we perform a generic study of fixed points and the possible RG flows among them in a minimal bottom-up holographic model without Lorentz invariance, aiming to shed light on the possible options and the related phenomenology. We find: i) A minor generalization of previous models involving a massive vector field with allowed self-couplings leads to a much more efficient emergence of Lorentz invariance than in the previous attempts. Moreover, we find that generically the larger is the UV dynamical exponent $z_{UV}$ the faster is the recovery of Lorentz symmetry in the IR. ii) We construct explicitly a holographic model with a line of fixed points, realizing different Lifshitz scaling along the line. iii) We also confirm the monotonicity of a recently proposed a-function along all our Lorentz violating RG flows., Comment: v2: minor revisions, matching the published version that will appear in JHEP

Many physical systems, including classical fluids, present in their phase diagram the competition between two phases that are separated by a line of first-order phase transitions which terminates at a so-called critical point. Despite several proposals, in the supercritical region beyond the critical point, whether the two phases can still be distinguished and by which criterion remain open questions. In this work, we study the thermodynamics and linear dynamics of a holographic superfluid model with nonlinear potential terms in the supercritical region. We identify the presence of a dynamical crossover, akin to the liquid-like to gas-like Frenkel transition in supercritical fluids, and we define other separation lines of thermodynamic origin based on higher order derivatives of the free energy with respect to the charge density. Our results highlight the universal dynamical and thermodynamic features of supercritical systems from nuclear matter and classical fluids to superfluid systems., Comment: 17 pages, 9 figures

Symmetry breaking is an effective tool for tuning the transport and topological properties of 2D layered materials. Among these materials, twisted bilayer graphene (TBG) has emerged as a promising platform for new physics, characterized by a rich interplay between topological features and strongly correlated electronic behavior. In this study, we utilize time-reversal symmetry breaking (TRSB) to manipulate the topological properties of TBG. By varying the strength of TRSB, we discover a topological phase transition between a topological insulating phase, which exhibits a pair of flat bands with opposite Chern numbers, and a novel insulating state where the Chern number, but not the Berry curvature, of the flat bands vanishes. We demonstrate that this topological transition is mediated by a gap closing at the $\Gamma$ point, and we construct a three-dimensional phase diagram as a function of the twisting angle, the symmetry-breaking parameter, and the mismatch coupling between AA and AB stacking regions. Finally, we show that this novel electronic phase can be identified in the lab by measuring, as a function of the Fermi energy, its non-quantized anomalous Hall conductivity that is induced by the Berry dipole density of the lowest flat bands., Comment: v1: comments welcome!

Topological defects are singularities in the order parameter space that are mathematically described by topological invariants and cannot be removed by continuous transformations. These defects play a significant role in various fields, ranging from cosmology to solid-state physics and biological matter. The definition of these irregularities requires an ordered reference configuration, leading to decades of debate about the existence of topological defects in disordered systems, such as glasses. Recently, it has been proposed that well-defined topological defects might emerge in the dynamical properties of glasses under deformation, potentially relating to their plastic behavior. In this study, we investigate a two-dimensional colloidal glass system composed of particles interacting by an effective magnetic repulsion. We reveal the presence of topological defects in the eigenspace of the vibrational frequencies of this experimental 2D amorphous solid. The vibrational density of states of this 2D amorphous material exhibits distinct glassy properties such as the presence of a boson peak anomaly. Through extensive numerical and theoretical quantitative analysis, we establish a robust positive correlation between the vibrational characteristics and the total number of topological defects. We furthermore show that defects of opposite charge tend to pair together and prove their local statistical correlation with the "soft spots", the regions more prone to plastic flow. This work provides the experimental confirmation for the existence of topological defects in disordered systems revealing a complex interplay between topology, disorder, and vibrational behavior.

In recent years, active Brownian particles have emerged as a prominent model system for comprehending the behaviors of active matter, wherein particles demonstrate self-propelled motion by harnessing energy from the surrounding environment. A fundamental objective of studying active matter is to elucidate the physical mechanisms underlying its collective behaviors. Drawing inspiration from advancements in molecular glasses, our study unveils a low-energy ``flat mode" within the transverse spectrum of active Brownian vibrators -- a nearly two-dimensional, bi-disperse granular assembly. We demonstrate that this collective excitation induces an anomalous excess in the vibrational density of states (VDOS) beyond the phononic Debye contribution. We characterize the properties of this flat mode by exploring the parameter space of our experimental system and tuning the packing fraction, the vibrational frequency, the particle size ratio and the mixture ratio. Additionally, we establish through empirical evidence that string-like dynamical defects, discerned via the spatial distribution of each particle's contribution to the reduced transverse VDOS, serve as the microscopic origin of the flat mode and its associated anomalies., Comment: v2: revised version. additional experimental data and analysis added, expanded SI, added particle motion videos

The capability of hydrodynamics to accurately describe slow and long-wavelength fluctuations around non-equilibrium steady states (NESS), characterized by a stationary flow of energy or matter in the presence of a driving force, remains an open question. In this study, we explicitly construct a hydrodynamic description of electrically driven non-equilibrium charged steady states \new{in the limit in which the relaxation of the first non-hydrodynamic excitation is parametrically slow}. Our approach involves introducing gapped modes and extending the effective description into a relaxed hydrodynamic theory (RHT). Leveraging the gauge-gravity duality as a tool for controlled computations within non-equilibrium systems, we establish an ultraviolet complete model for these NESS that confirms the validity of our RHT. In summary, our findings provide a concrete realization of the validity of hydrodynamics beyond thermal equilibrium, offering valuable insights into the dynamics of non-equilibrium systems., Comment: v2: matching the published version in PRR

Solid materials that deviate from the harmonic crystal paradigm exhibit characteristic anomalies in the specific heat and vibrational density of states (VDOS) with respect to Debye's theory predictions. The boson peak (BP), a low-frequency excess in the VDOS over Debye law $g(\omega) \propto \omega^2$, is certainly the most famous among them; nevertheless, its origin is still subject of fierce debate. Recent simulation works provided strong evidence that localized one-dimensional string-like excitations (stringlets) might be the microscopic origin of the BP. In this work, we study the dynamics of acoustic phonons interacting with a bath of vibrating 1D stringlets with exponentially distributed size, as observed in simulations. We show that stringlets strongly renormalize the phonon propagator and naturally induce a BP anomaly in the vibrational density of states, corresponding to the emergence of a dispersionless BP flat mode. Additionally, phonon-stringlet interactions produce a strong enhancement of sound attenuation and a dip in the speed of sound near the BP frequency, consistent with experimental and simulation data. The qualitative trends of the BP frequency and intensity are predicted within the model and shown to be in good agreement with previous observations. In summary, our results substantiate with a simple theoretical model the recent simulation results by Hu and Tanaka claiming the origin of the BP from stringlet dynamics., Comment: v2: matching the published version in Journal of Physics: Condensed Matter

Unlike crystalline solids, liquids do not exhibit long-range order. Their atoms undergo frequent structural rearrangements, resulting in the long-wavelength dynamics of shear fluctuations in liquids being diffusive, rather than propagating waves, as observed in crystals. When considering shorter time and length scales, molecular dynamics simulations and theoretical propositions suggest that collective shear excitations in liquids display a gap in wave-vector space, referred to as the $k$-gap. Above this gap, solid-like transverse waves re-emerge. However, direct experimental verification of this phenomenon in classical liquids remains elusive, with the only documented evidence from studies in two-dimensional dusty plasmas. Active granular systems provide a novel platform for exploring the emergence of collective dynamics and showcasing a rich interplay of complex phases and phenomena. Our study focuses on bi-disperse active Brownian vibrators. Through measurements of the pair correlation functions, mean square displacements, velocity auto-correlation functions, vibrational density of states, and a detailed analysis of microscopic atomic motion, we demonstrate that this active system exhibits both gas-like and liquid-like phases, depending on the packing fraction, despite pure hard-disk-like repulsive interactions. Notably, within the granular liquid-like phase, we experimentally validate the existence of a $k$-gap in the dispersion of transverse excitations. This gap becomes more significant with a decrease in packing fraction and disappears into the gas phase, aligning with theoretical expectations. Our results offer a direct experimental confirmation of the $k$-gap phenomenon, extending its relevance beyond classical thermal liquids to active granular systems, and reveal the existence of intriguing similarities between the physics of active granular matter and supercritical fluids., Comment: v1: comments are welcome!

Quasicrystals have been observed in a variety of materials ranging from metal alloys to block copolymers and represent an "intermediate" form of matter between crystals and amorphous materials (glasses and liquids) in that their structural and dynamical properties can not readily described in terms of conventional solid-state models of liquids and solids. In the present work, we present a comprehensive analysis of basic thermodynamic and dynamic properties of quasicrystals to better understand the nature of the atomic motion underlying diffusion and structural relaxation in these materials. As our model system, we investigate a dodecagonal quasicrystal using molecular dynamics (MD) simulations in two dimensions (2D), subject to periodic boundary conditions. We observe a two-stage relaxation dynamics in the self-intermediate scattering function $F_s(k,t)$ of our quasicrystal material involving a fast $\beta$-relaxation on a ps timescale and $\alpha$ relaxation process having a highly temperature dependent relaxation time whose activation energy varies in concert with the extent of string-like collective motion. Multi-step relaxation of the intermediate scattering function and string-like collective atomic motion have similarly been observed ubiquitously in glass-forming liquids at low temperatures and in crystalline materials at elevated temperatures where structural relaxation and diffusion are both non-Arrhenius. After examining the dynamics of our quasi-crystalline material in great detail, we conclude that its dynamics more closely resemble observations on metallic glass-forming liquids, in qualitative accord with previous neutron scattering studies., Comment: v1: comments welcome

The deformation mechanism in amorphous solids subjected to external shear remains poorly understood because of the absence of well-defined topological defects mediating the plastic deformation. The notion of soft spots has emerged as a useful tool to characterize the onset of irreversible rearrangements and plastic flow, but these entities are not clearly defined in terms of geometry and topology. In this study, we unveil the phenomenology of recently discovered, precisely defined topological defects governing the microscopic mechanical and yielding behavior of a model 3D glass under shear deformation. We identify the existence of vortex-like and anti-vortex-like topological defects within the 3D non-affine displacement field. The number density of these defects exhibits a significant anti-correlation with the plastic events, with defect proliferation-annihilation cycles matching the alternation of elastic-like segments and catastrophic plastic drops, respectively. Furthermore, we observe collective annihilation of these point-like defects via plastic events, with large local topological charge fluctuations in the vicinity of regions that feature strong non-affine displacements. We reveal that plastic yielding is driven by several large sized clusters of net negative topological charge, the massive annihilation of which triggers the onset of plastic flow. These findings suggest a geometric and topological characterization of soft spots and pave the way for the mechanistic understanding of topological defects as mediators of plastic deformation in glassy materials., Comment: Accepted for publication in PNAS Nexus

Propagating chiral magnetic waves (CMW) are expected to exist in chiral plasmas due to the interplay between the chiral magnetic and chiral separation effects induced by the presence of a chiral anomaly. Unfortunately, it was pointed out that, because of the effects of electric conductivity and dissipation, CMW are overdamped and therefore their signatures are unlikely to be seen in heavy-ion collision experiments and in the quark gluon plasma. Nonetheless, the chiral anomaly plays a fundamental role in Weyl semimetals and their anomalous transport properties as well. Hence, CMW could be potentially observed in topological semimetals using table-top experiments. By using a holographic model for strongly coupled Weyl semimetals, we investigate in detail the nature of CMW in presence of Coulomb interactions and axial charge relaxation and estimate whether, and in which regimes, CMW could be observed as underdamped collective excitations in topological materials., Comment: 39 pages, 11 figures, published version

We study the linear stability of holographic homogeneous solids (HHS) at finite temperature and in presence of a background shear strain by means of a large scale quasi-normal mode analysis which extends beyond the hydrodynamic limit. We find that mechanical instability can arise either as a result of a complex speed of sound -- gradient instability -- or of a negative diffusion constant. Surprisingly, the simplest HHS models are linearly stable for arbitrarily large values of the background strain. For more complex HHS, the onset of the diffusive instability always precedes that of the gradient instability, which becomes the dominant destabilizing process only above a critical value of the background shear strain. Finally, we observe that the critical strains for the two instabilities approach each other at low temperatures. We conclude by presenting a phase diagram for HHS as a function of temperature and background shear strain which shows interesting similarities with the physics of superfluids in presence of background superfluid velocity., Comment: v2: manuscript revised and improved

We study the nonlinear dynamical evolution of spinodal decomposition in a first-order superfluid phase transition using a simple holographic model in the probe limit. We first confirm the linear stability analysis based on quasinormal modes and verify the existence of a critical length scale related to a gradient instability -- negative speed of sound squared -- of the superfluid sound mode, which is a consequence of a negative thermodynamic charge susceptibility. We present a comparison between our case and the standard Cahn-Hilliard equation for spinodal instability, in which a critical length scale can be also derived based on a diffusive instability. We then perform several numerical tests which include the nonlinear time evolution directly from an unstable state and fast quenches from a stable to an unstable state in the spinodal region. Our numerical results provide a real time description of spinodal decomposition and phase separation in one and two spatial dimensions. We reveal the existence of four different stages in the dynamical evolution, and characterize their main properties. Finally, we investigate the strength of dynamical heterogeneity using the spatial variance of the local chemical potential and we correlate the latter to other features of the dynamical evolution., Comment: 19 pages, 13 figures. A few typos have been corrected

The boson peak (BP), a low-energy excess in the vibrational density of states over the Debye contribution, is often identified as a characteristic of amorphous solid materials. Despite decades of efforts, its microscopic origin still remains a mystery. Recently, it has been proposed, and corroborated with simulations, that the BP might stem from intrinsic localized modes involving one-dimensional (1D) string-like excitations (``stringlets"). We build on a theory originally proposed by Lund that describes the localized modes as 1D vibrating strings, but we specify the stringlet size distribution to be exponential, as observed in simulations. We provide an analytical prediction for the BP frequency $\omega_{BP}$ in the temperature regime well below the observed glass transition temperature $T_g$. The prediction involves no free parameters and accords quantitatively with prior simulation observations in 2D and 3D model glasses based on inverse power law potentials. The comparison of the string model to observations is more uncertain when compared to simulations of an Al-Sm metallic glass material at temperatures well above $T_g$. Nonetheless, our stringlet model of the BP naturally reproduces the softening of the BP frequency upon heating and offers an analytical explanation for the experimentally observed scaling with the shear modulus in the glass state and changes in this scaling in simulations of glass-forming liquids. Finally, the theoretical analysis highlights the existence of a strong damping for the stringlet modes above $T_g$, which leads to a large low-frequency contribution to the 3D vibrational density of states, observed in both experiments and simulations., Comment: v3: matching the published version. arXiv admin note: substantial text overlap with arXiv:2307.12839

The boson peak (BP), a low-energy excess in the vibrational density of states over the phonon Debye contribution, is usually identified as one of the distinguishing features between ordered crystals and amorphous solid materials. Despite decades of efforts, its microscopic origin still remains a mystery and a consensus on its theoretical derivation has not yet been achieved. Recently, it has been proposed, and corroborated with simulations, that the BP might stem from intrinsic localized modes which involve string-like excitations ("stringlets") having a one-dimensional (1D) nature. In this work, we build on a theoretical framework originally proposed by Lund that describes the localized modes as 1D vibrating strings, but we specify the stringlet size distribution to be exponential, as observed in independent simulation studies. We show that a generalization of this framework provides an analytically prediction for the BP frequency $\omega_{BP}$ in the temperature regime well below the glass transition temperature in both 2D and 3D amorphous systems. The final result involves no free parameters and is in quantitative agreement with prior simulation observations. Additionally, this stringlet theory of the BP naturally reproduces the softening of the BP frequency upon heating and offers an analytical explanation for the experimentally observed scaling with the shear modulus in the glass state and changes in this scaling in cooled liquids. Finally, the theoretical analysis highlights the existence of a strong damping for the stringlet modes at finite temperature which leads to a large low-frequency contribution to the 3D vibrational density of states, as observed in both experiments and simulations., Comment: We withdraw the manuscript temporally to abide by the internal review requirements of one of the authors (Jack Douglas) at the National Institute of Standards and Technology. (NIST). The withdrawal has nothing to do with the content of the paper, and we plan to resubmit our paper to the arXiv once the paper has been approved for public release by the NIST internal review board

In the realm of nanoscience, the dynamic behaviors of liquids at scales beyond the conventional structural relaxation time, $\tau$, unfold a fascinating blend of solid-like characteristics, including the propagation of collective shear waves and the emergence of elasticity. However, in classical bulk liquids, where $\tau$ is typically of the order of 1 ps or less, this solid-like behavior remains elusive in the low-frequency region of the density of states (DOS). Here, we provide evidence for the emergent solid-like nature of liquids at short distances through inelastic neutron scattering measurements of the low-frequency DOS in liquid water and glycerol confined within graphene oxide membranes. In particular, upon increasing the strength of confinement, we observe a transition from a liquid-like DOS (linear in the frequency $\omega$) to a solid-like behavior (Debye law, $\sim\omega^2$) in the range of $1$-$4$ meV. Molecular dynamics simulations confirm these findings and reveal additional solid-like features, including propagating collective shear waves and a reduction in the self-diffusion constant. Finally, we show that the onset of solid-like dynamics is pushed towards low frequency along with the slowing-down of the relaxation processes upon confinement. This nanoconfinement-induced transition, aligning with k-gap theory, underscores the potential of leveraging liquid nanoconfinement in advancing nanoscale science and technology, building more connections between fluid dynamics and materials engineering., Comment: v3: matching the published version in ACS Nano

In the last decade, motivated by the concept of Planckian relaxation and the possible existence of a quantum critical point in cuprate materials, holographic techniques have been extensively used to tackle the problem of strange metals and high-$T_c$ superconductors. Among the various setups, the linear axion Gubser-Rocha model has often been considered as a promising holographic model for strange metals since endowed with the famous linear in $T$ resistivity property. As fiercely advocated by Phil Anderson, beyond $T$-linear resistivity, there are several additional anomalies unique to the strange metal phase, as for example a Fermi liquid like Hall angle -- the famous problem of the two relaxation scales. In this short note, we show that the linear axion holographic Gubser-Rocha model, which presents a single momentum relaxation time, fails in this respect and therefore is not able to capture the transport phenomenology of strange metals. We prove our statement by means of a direct numerical computation, a previously demonstrated scaling analysis and also a hydrodynamic argument. Finally, we conclude with an optimistic discussion on the possible improvements and generalizations which could lead to a holographic model for strange metals in all their glory., Comment: v2: minor revisions, matching the published version

We provide a mathematical description, based on d-wave Eliashberg theory, of the strong correlation between the experimentally observed softening of Raman modes associated with in-plane oxygen motions and the corresponding superconducting critical temperature $T_c$, as a function of oxygen doping $x$, in YBa$_2$Cu$_3$O$_x$. The theoretical model provides a direct link between physical trends of soft optical $A_g$ (in-plane) oxygen modes, the level of oxygen doping $x$, and the superconducting $T_c$. Different regimes observed in the trend of $T_c$ vs doping can be related to corresponding regimes of optical phonon softening in the Raman spectra. These results provide further evidence related to the physical origin of high-temperature superconductivity in rare-earth cuprate oxides and to the significant role of electron-phonon coupling therein., Comment: Accepted for publication in J. Phys. Materials

Twisted bilayer graphene (TBG) is a recently discovered two-dimensional superlattice structure which exhibits strongly-correlated quantum many-body physics, including strange metallic behavior and unconventional superconductivity. Most of TBG exotic properties are connected to the emergence of a pair of isolated and topological flat electronic bands at the so-called magic angle, $\theta \approx 1.05^{\circ}$, which are nevertheless very fragile. In this work, we show that, by employing chiral optical cavities, the topological flat bands can be stabilized away from the magic angle in an interval of approximately $0.8^{\circ}<\theta<1.3^{\circ}$. As highlighted by a simplified theoretical model, time reversal symmetry breaking (TRSB), induced by the chiral nature of the cavity, plays a fundamental role in flattening the isolated bands and gapping out the rest of the spectrum. Additionally, TRSB suppresses the Berry curvature and induces a topological phase transition, with a gap closing at the $\Gamma$ point, towards a band structure with two isolated flat bands with Chern number equal to $0$. The efficiency of the cavity is discussed as a function of the twisting angle, the light-matter coupling and the optical cavity characteristic frequency. Our results demonstrate the possibility of engineering flat bands in TBG using optical devices, extending the onset of strongly-correlated topological electronic phases in moir\'e superlattices to a wider range in the twisting angle., Comment: v2: matching published version in PRL

Mixing theoretical topological structures with cutting-edge simulation methods, a recent study in Nature Communications has finally confirmed the existence of topological defects in glasses and their crucial role for plasticity., Comment: News and Views commentary for the paper by Wu et Al. [Nat Commun 14, 2955 (2023)]

Phasons are collective low-energy modes that appear in disparate condensed matter systems such as quasicrystals, incommensurate structures, fluctuating charge density waves, and Moir\'e superlattices. They share several similarities with acoustic phonon modes, but they are not protected by any exact translational symmetry. As a consequence, they are subject to a wavevector independent damping, and they develop a finite pinning frequency, which destroy their acoustic linearly propagating dispersion. Under a few and simple well-motivated assumptions, we compute the phason density of states, and we derive the phason heat capacity as a function of the temperature. Finally, imagining a hypothetical s-wave pairing channel with electrons, we compute the critical temperature $T_c$ of the corresponding superconducting state as a function of phason damping using the Eliashberg formalism. We find that for large phason damping, the heat capacity is linear in temperature, showing a distinctive glass-like behavior. Additionally, we observe that the phason damping can strongly enhance the effective Eliashberg coupling, and we reveal a sharp non-monotonic dependence of the superconducting temperature $T_c$ on the phason damping, with a maximum located at the underdamped to overdamped crossover scale. Our simple computations confirm the potential role of overdamped modes in explaining the glassy properties of incommensurate structures, but also in possibly inducing strongly-coupled superconductivity therein, and enhancing the corresponding $T_c$., Comment: v2: appendices added, references added

Contrary to the case of solids and gases, where Debye theory and kinetic theory offer a good description for most of the physical properties, a complete theoretical understanding of the vibrational and thermodynamic properties of liquids is still missing. Liquids exhibit a vibrational density of states (VDOS) which does not obey Debye law, and a heat capacity which decreases monotonically with temperature, rather than growing as in solids. Despite many attempts, a simple, complete and widely accepted theoretical framework able to formally derive the aforementioned properties has not been found yet. Here, we revisit one of the theoretical proposals, and in particular we re-analyze the properties of liquids within the soft-potential model, originally formulated for glasses. We confirm that, at least at a qualitative level, many characteristic properties of liquids can be rationalized within this model. We discuss the validity of several phenomenological expressions proposed in the literature for the density of unstable modes, and in particular for its temperature and frequency dependence. We discuss the role of negative curvature regions and unstable modes as fundamental ingredients to have a linear in frequency VDOS. Finally, we compute the heat capacity within the soft potential model for liquids and we show that it decreases with temperature, in agreement with experimental and simulation data., Comment: revised manuscript matching the published version

We report neutron-scattering measurements of the density of states (DOS) of water and liquid Fomblin in a wide range of temperatures. In the liquid phase, we confirm the presence of a universal low-energy linear scaling of the experimental DOS as a function of the frequency, $g(\omega)= a(T) \omega$, which persists at all temperatures. The low-frequency scaling of the DOS exhibits a sharp jump at the melting point of water, below which the standard Debye's law, $g(\omega) \propto \omega^2$, is recovered. On the contrary, in Fomblin, we observe a continuous transition between the two exponents reflecting its glassy dynamics, which is confirmed by structure measurements. More importantly, in both systems, we find that the slope $a(T)$ grows with temperature following an exponential Arrhenius-like form, $a(T) \propto \exp(-\langle E \rangle /T)$. We confirm this experimental trend using molecular dynamics simulations and show that the prediction of instantaneous normal mode (INM) theory for $a(T)$ is in qualitative agreement with the experimental data., Comment: v3: revised manuscript

We study the quasi-hydrodynamics of a system with a softly broken $U(1)$ global symmetry using effective field theory (EFT) and holographic methods. In the gravity side, we consider a holographic Proca model in the limit of small bulk mass, which is responsible for a controllable explicit breaking of the $U(1)$ global symmetry in the boundary field theory. We perform a holographic Schwinger-Keldysh analysis, which allows us to derive the form of the boundary effective action in presence of dissipation. We compare our results with the previously proposed EFT and hydrodynamic theories, and we confirm their validity by computing the low-energy quasi-normal modes spectrum analytically and numerically. Additionally, we derive the broken holographic Ward identity for the $U(1)$ current, and discuss the recently proposed novel transport coefficients for systems with explicitly broken symmetries. The setup considered is expected to serve as a toy model for more realistic situations where quasi-hydrodynamics is at work, such as axial charge relaxation in QCD, spin relaxation in relativistic systems, electric field relaxation in magneto-hydrodynamics, or momentum relaxation in condensed matter systems., Comment: v3: matches published version, v2: new subsection, references added, minor edits; v1: 44 pages, 4 figures

Driving a system out of equilibrium enriches the paradigm of spontaneous symmetry breaking, which could then take place not only in space but also in time. The interplay between temporal and spatial symmetries, as well as symmetries from other internal degrees of freedom, can give rise to novel nonequilibrium phases of matter. In this study, we investigate a driven-dissipative superfluid model using holographic methods and reveal the existence of a space-time supersolid (STS) phase which concomitantly breaks the time translation, spatial translation, and the internal U(1) symmetry. The holographic methods naturally include finite temperature effects, which enables us to explore the complex phase diagram of this model and observe a cascade of out-of-equilibrium phase transitions from the STS phase to a synchronized superfluid phase, and finally to a normal fluid phase, by increasing the temperature., Comment: 9 pages, 7 figures

We revisit the computation of the shear viscosity to entropy ratio in a holographic p-wave superfluid model, focusing on the role of rotational symmetry breaking. We study the interplay between explicit and spontaneous symmetry breaking and derive a simple horizon formula for $\eta/s$, which is valid also in the presence of explicit breaking of rotations and is in perfect agreement with the numerical data. We observe that a source which explicitly breaks rotational invariance suppresses the value of $\eta/s$ in the broken phase, competing against the effects of spontaneous symmetry breaking. However, $\eta/s$ always reaches a constant value in the limit of zero temperature, which is never smaller than the Kovtun-Son-Starinets (KSS) bound, $1/4\pi$. This behavior appears to be in contrast with previous holographic anisotropic models which found a power-law vanishing of $\eta/s$ at small temperature. This difference is shown to arise from the properties of the near-horizon geometry in the extremal limit. Thus, our construction shows that the breaking of rotations itself does not necessarily imply a violation of the KSS bound., Comment: 20 pages, 7 figures

Equilibrium molecular dynamics simulations are performed to study two-dimensional (2D) dusty plasma liquids. Based on the stochastic thermal motion of simulated particles, the longitudinal and transverse phonon spectra are calculated, and used to determine the corresponding dispersion relations. From there, the longitudinal and transverse sound speeds of 2D dusty plasma liquids are obtained. It is discovered that, for wavenumbers beyond the hydrodynamic regime, the longitudinal sound speed of a 2D dusty plasma liquid exceeds its adiabatic value, i.e., the so-called fast sound. This phenomenon appears at roughly the same length scale of the cutoff wavenumber for transverse waves, confirming its relation to the emergent solidity of liquids in the non-hydrodynamic regime. Using the thermodynamic and transport coefficients extracted from the previous studies, and relying on the Frenkel theory, the ratio of the longitudinal to the adiabatic sound speeds is derived analytically, providing the optimal conditions for fast sound, which are in quantitative agreement with the current simulation results., Comment: v1: 7 pages, 6 figures

The role of anharmonicity on superconductivity has often been disregarded in the past. Recently, it has been recognized that anharmonic decoherence could play a fundamental role in determining the superconducting properties (electron-phonon coupling, critical temperature, etc) of a large class of materials, including systems close to structural soft-mode instabilities, amorphous solids and metals under extreme high-pressure conditions. Here, we review recent theoretical progress on the role of anharmonic effects, and in particular certain universal properties of anharmonic damping, on superconductivity. Our focus regards the combination of microscopic-agnostic effective theories for bosonic mediators with the well-established BCS theory and Migdal-Eliashberg theory for superconductivity. We discuss in detail the theoretical frameworks, their possible implementation within first-principles methods, and the experimental probes for anharmonic decoherence. Finally, we present several concrete applications to emerging quantum materials, including hydrides, ferroelectrics and systems with charge density wave instabilities., Comment: matching the published version

In the context of bottom-up holography, we demonstrate the power of mixed boundary conditions to promote the boundary gauge field to be dynamical. We provide two concrete applications of this idea. First, we consider a holographic dual for a strongly coupled plasma described by dissipative magnetohydrodynamics. Second, we reveal the expected features of the Higgs mechanism in a not counterfeit holographic superconductor., Comment: Proceedings for the 6$^{th}$ International Conference on Holography, String Theory and Spacetime, held in Da Nang (Vietnam), 20-24 of February 2023. Based on arXiv:2211.01760 and arXiv:2302.02364

Topological semimetals are a class of many-body systems exhibiting novel macroscopic quantum phenomena at the interplay between high energy and condensed matter physics. They display a topological quantum phase transition (TQPT) which evades the standard Landau paradigm. In the case of Weyl semimetals, the anomalous Hall effect is a good non-local order parameter for the TQPT, as it is proportional to the separation between the Weyl nodes in momentum space. On the contrary, for nodal line semimetals (NLSM), the quest for an order parameter is still open. By taking advantage of a recently proposed holographic model for strongly-coupled NLSM, we explicitly show that entanglement entropy (EE) provides an optimal probe for nodal topology. We propose a generalized $c$-function, constructed from the EE, as an order parameter for the TQPT. Moreover, we find that the derivative of the renormalized EE with respect to the external coupling driving the TQPT diverges at the critical point, signaling the rise of non-local quantum correlations. Finally, we show that these quantum information quantities might be able to characterize not only the critical point but the whole quantum critical region at finite temperature., Comment: 35 pages, 16 figures

The holographic superconductor is one of the most popular models in the context of applied holography. Despite what its name suggests, it does not describe a superconductor. On the contrary, the low temperature phase of its dual field theory is a superfluid with a spontaneously broken U(1) global symmetry. As already observed in the previous literature, a bona fide holographic superconductor can be constructed using mixed boundary conditions for the bulk gauge field. By exploiting this prescription, we study the near-equilibrium collective dynamics in the Higgs phase and reveal the characteristic features of the Anderson-Higgs mechanism. We show that second sound disappears from the spectrum and the gauge field acquires a finite energy gap of the order of the plasma frequency. We observe an overdamped to underdamped crossover for the Higgs mode which acquires a finite energy gap below $\approx T_c/2$, with $T_c$ the superconducting critical temperature. Interestingly, the energy gap of the Higgs mode at low temperature is significantly smaller than $2\Delta$, with $\Delta$ the superconducting energy gap. Finally, we interpret our results using Ginzburg-Landau theory and we confirm the validity of previously derived perturbative analytic expressions., Comment: v1: 43 pages, 18 figures; v2: minor revision (a reference added, a figure added, comments added); v3: minor revision, matching the published version

Dusty plasmas represent a powerful playground to study the collective dynamics of strongly coupled systems with important interdisciplinary connections to condensed matter physics. Due to the pure Yukawa repulsive interaction between dust particles, dusty plasmas do not display a traditional liquid-vapor phase transition, perfectly matching the definition of a supercritical fluid. Using molecular dynamics simulations, we verify the supercritical nature of dusty plasmas and reveal the existence of a dynamical liquid-like to gas-like crossover which perfectly matches the salient features of the Frenkel line in classical supercritical fluids. We present several diagnostics to locate this dynamical crossover spanning from local atomic connectivity, shear relaxation dynamics, velocity autocorrelation function, heat capacity, and various transport properties. All these different criteria well agree with each other and are able to successfully locate the Frenkel line in both 2D and 3D dusty plasmas. In addition, we propose the unity ratio of the instantaneous transverse sound speed $C_T$ to the average particle speed $\bar{v}_{p}$, i.e., $C_T / \bar{v}_{p} = 1$, as a new diagnostic to identify this dynamical crossover. Finally, we observe an emergent degree of universality in the collective dynamics and transport properties of dusty plasmas as a function of the screening parameter and dimensionality of the system. Intriguingly, the temperature of the dynamical transition is independent of the dimensionality, and it is found to be always $20$ times of the corresponding melting point. Our results open a new path for the study of single particle and collective dynamics in plasmas and their interrelation with supercritical fluids in general., Comment: v1: comments are welcome

Phonon softening is a ubiquitous phenomenon in condensed matter systems which is often associated with charge density wave (CDW) instabilities and anharmonicity. The interplay between phonon softening, CDW and superconductivity is a topic of intense debate. In this work, the effects of anomalous soft phonon instabilities on superconductivity are studied based on a recently developed theoretical framework that accounts for phonon damping and softening within the Migdal-Eliashberg theory. Model calculations show that the phonon softening in the form of a sharp dip in the phonon dispersion relation, either acoustic or optical (including the case of Kohn-type anomalies typically associated with CDW), can cause a manifold increase of the electron-phonon coupling constant $\lambda$. This, under certain conditions, which are consistent with the concept of optimal frequency introduced by Bergmann and Rainer, can produce a large increase of the superconducting transition temperature $T_c$. In summary, our results suggest the possibility of reaching high-temperature superconductivity by exploiting soft phonon anomalies restricted in momentum space., Comment: v3: matching the published version

Within the framework of holography, the Einstein-Maxwell action with Dirichlet boundary conditions corresponds to a dual conformal field theory in presence of an external gauge field. Nevertheless, in many real-world applications, e.g., magnetohydrodynamics, plasma physics, superconductors, etc. dynamical gauge fields and Coulomb interactions are fundamental. In this work, we consider bottom-up holographic models at finite magnetic field and (free) charge density in presence of dynamical boundary gauge fields which are introduced using mixed boundary conditions. We numerically study the spectrum of the lowest quasi-normal modes and successfully compare the obtained results to magnetohydrodynamics theory in $2+1$ dimensions. Surprisingly, as far as the electromagnetic coupling is small enough, we find perfect agreement even in the large magnetic field limit. Our results prove that a holographic description of magnetohydrodynamics does not necessarily need higher-form bulk fields but can be consistently derived using mixed boundary conditions for standard gauge fields., Comment: 54 pages, 22 figures

Pseudo-Goldstone modes appear in many physical systems and display robust universal features. First, their mass $m$ obeys the so-called Gell-Mann-Oakes-Renner (GMOR) relation $f^2\,m^2=H\,\bar{\sigma}$, with $f$ the Goldstone stiffness, $H$ the explicit breaking scale and $\bar{\sigma}$ the spontaneous condensate. More recently, it has been shown that their damping $\Omega$ is constrained to follow the relation $\Omega=m^2 D_\varphi$, where $D_\varphi$ is the Goldstone diffusivity in the purely spontaneous phase. Pions are the most paradigmatic example of pseudo-Goldstone modes and they are related to chiral symmetry breaking in QCD. In this work, we consider a bottom-up soft-wall AdS-QCD model with broken ${\rm{SU}}(2)_L \times {\rm{SU}}(2)_R$ symmetry and we study the nature of the associated pseudo-Goldstone modes -- the pions. In particular, we perform a detailed investigation of their dispersion relation in presence of dissipation, of the role of the explicit breaking induced by the quark masses and of the dynamics near the critical point. Taking advantage of the microscopic information provided by the holographic model, we give quantitative predictions for all the coefficients appearing in the effective description. In particular, we estimate the finite temperature behavior of the kinetic parameter $\mathfrak{r^2}$ defined as the ration between the Goldstone diffusivity $D_\varphi$ and the pion attenuation constant $D_A$. Interestingly, we observe important deviations from the value $\mathfrak{r^2}=3/4$ computed in chiral perturbation theory in the limit of zero temperature., Comment: 18 pages, 14 figures

Univalent functions are complex, analytic (holomorphic) and injective functions that have been widely discussed in complex analysis. It was recently proposed that the stringent constraints that univalence imposes on the growth of functions combined with sufficient analyticity conditions could be used to derive rigorous lower and upper bounds on hydrodynamic dispersion relation, i.e., on all terms appearing in their convergent series representations. The results are exact bounds on physical quantities such as the diffusivity and the speed of sound. The purpose of this paper is to further explore these ideas, investigate them in concrete holographic examples, and work towards a better intuitive understanding of the role of univalence in physics. More concretely, we study diffusive and sound modes in a family of holographic axion models and offer a set of observations, arguments and tests that support the applicability of univalence methods for bounding physical observables described in terms of effective field theories. Our work provides insight into expected `typical' regions of univalence, comparisons between the tightness of bounds and the corresponding exact values of certain quantities characterizing transport, tests of relations between diffusion and bounds that involve chaotic pole-skipping, as well as tests of a condition that implies the conformal bound on the speed of sound and a complementary condition that implies its violation., Comment: v2: minor revision, matching the published version

In this Colloquium, we review recent progress in the effective description of strongly-correlated phases of matter with spontaneously broken translations, such as charge density waves or Wigner crystals. In real materials, disorder is inevitable and pins the Goldstones of broken translations. We describe how pinning can be incorporated in the effective field theory at low energies, without making any assumption on the presence of boost symmetry. We review the essential role played by gauge-gravity duality models in establishing these effective field theories with only approximate symmetries. We close with a discussion on the relevance of these models for the phenomenology of dc and ac transport in strongly-correlated strange and bad metals, such as high temperature superconductors., Comment: final version accepted in Review of Modern Physics

A supersolid is a system that presents long-range order and shear rigidity as a solid but which also supports a non-dissipative superflow as a superfluid. From an effective perspective, supersolids are identified with phases of matter that break spontaneously translational invariance together with a global $U(1)$ symmetry. By using this symmetry prescription, we build a holographic bottom-up model for supersolids and we start the investigation of its thermodynamic and mechanical properties. More precisely, we analyze the behaviour of the critical temperature, the condensate, the shear modulus and the viscosity across all the phase diagram. Finally, we successfully compare our results with a simple Ginzburg-Landau model for supersolids deriving some universal physical correlations between the observables mentioned above., Comment: v2: Matches the version published in JHEP. Subsections 4.2.2 and 4.4.2, Appendix C added. 25(+8) pages, 10(+3) figures