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We show that a temporal soliton can induce resonant radiation by three-wave mixing nonlinearities. This constitutes a new class of resonant radiation whose spectral positions are parametrically tunable. The experimental verification is done in a periodically poled lithium niobate crystal, where a femtosecond near-IR soliton is excited and resonant radiation waves are observed exactly at the calculated soliton phase-matching wavelengths via the sum- and difference-frequency generation nonlinearities. This extends the supercontinuum bandwidth well into the mid-IR to span 550-5000 nm and the mid-IR edge is parametrically tunable over 1000 nm by changing the three-wave mixing phase-matching condition. The results are important for bright and broadband supercontinuum generation and for frequency comb generation in quadratic nonlinear microresonators., Comment: in press, Physical Review Letters

Generating energetic femtosecond mid-IR pulses is crucial for ultrafast spectroscopy, and currently relies on parametric processes that, while efficient, are also complex. Here we experimentally show a simple alternative that uses a single pump wavelength without any pump synchronization and without critical phase-matching requirements. Pumping a bulk quadratic nonlinear crystal (unpoled LiNbO$_3$ cut for noncritical phase-mismatched interaction) with sub-mJ near-IR 50-fs pulses, tunable and broadband ($\sim 1,000$ cm$^{-1}$) mid-IR pulses around $3.0~\mu\rm m$ are generated with excellent spatio-temporal pulse quality, having up to 10.5 $\mu$J energy (6.3% conversion). The mid-IR pulses are dispersive waves phase-matched to near-IR self-defocusing solitons created by the induced self-defocusing cascaded nonlinearity. This process is filament-free and the input pulse energy can therefore be scaled arbitrarily by using large-aperture crystals. The technique can readily be implemented with other crystals and laser wavelengths, and can therefore potentially replace current ultrafast frequency-conversion processes to the mid-IR., Comment: submitted

We discuss a novel method for generating octave-spanning supercontinua and few-cycle pulses in the important mid-IR wavelength range. The technique relies on strongly phase-mismatched cascaded second-harmonic generation (SHG) in mid-IR nonlinear frequency conversion crystals. Importantly we here investigate the so-called noncritical SHG case, where no phase matching can be achieved but as a compensation the largest quadratic nonlinearities are exploited. A self-defocusing temporal soliton can be excited if the cascading nonlinearity is larger than the competing material self-focusing nonlinearity, and we define a suitable figure of merit to screen a wide range of mid-IR dielectric and semiconductor materials with large effective second-order nonlinearities $d_{\rm eff}$. The best candidates have simultaneously a large bandgap and a large $d_{\rm eff}$. We show selected realistic numerical examples using one of the promising crystals: in one case soliton pulse compression from 50 fs to 15 fs (1.5 cycles) at $3.0\mic$ is achieved, and at the same time a 3-cycle dispersive wave at $5.0\mic$ is formed that can be isolated using a long-pass filter. In another example we show that extremely broadband supercontinua can form spanning the near-IR to the end of the mid-IR (nearly 4 octaves)., Comment: submitted to Optics Materials Express special issue on mid-IR photonics

Cascaded nonlinearities have attracted much interest, but ultrafast applications have been seriously hampered by the simultaneous requirements of being near phase-matching and having ultrafast femtosecond response times. Here we show that in strongly phase-mismatched nonlinear frequency conversion crystals the pump pulse can experience a large and extremely broadband self-defocusing cascaded Kerr-like nonlinearity. The large cascaded nonlinearity is ensured through interaction with the largest quadratic tensor element in the crystal, and the strong phase-mismatch ensures an ultrafast nonlinear response with an octave-spanning bandwidth. We verify this experimentally by showing few-cycle soliton compression with noncritical cascaded second-harmonic generation: Energetic 47 fs infrared pulses are compressed in a just 1-mm long bulk lithium niobate crystal to 17 fs (under 4 optical cycles) with 80% efficiency, and upon further propagation an octave-spanning supercontinuum is observed. Such ultrafast cascading is expected to occur for a broad range of pump wavelengths spanning the near- and mid-IR using standard nonlinear crystals., Comment: resubmitted, revised version, accepted for Phys. Rev. Lett

When ultrafast noncritical cascaded second-harmonic generation of energetic femtosecond pulses occur in a bulk lithium niobate crystal optical Cherenkov waves are formed in the near- to mid-IR. Numerical simulations show that the few-cycle solitons radiate Cherenkov (dispersive) waves in the $\lambda=2.2-4.5\mic$ range when pumping at $\lambda_1=1.2-1.8\mic$. The exact phase-matching point depends on the soliton wavelength, and we show that a simple longpass filter can separate the Cherenkov waves from the solitons. The Cherenkov waves are born few-cycle with an excellent Gaussian pulse shape, and the conversion efficiency is up to 25%. Thus, optical Cherenkov waves formed with cascaded nonlinearities could become an efficient source of energetic near- to mid-IR few-cycle pulses., Comment: Extended version of Nonlinear Optics 2011 contribution http://www.opticsinfobase.org/abstract.cfm?URI=NLO-2011-NTuA7. Submitted for Optics Express special issue for NLO conference

The dispersion of index-guiding microstructured polymer optical fibers is calculated for second-harmonic generation. The quadratic nonlinearity is assumed to come from poling of the polymer, which in this study is chosen to be the cyclic olefin copolymer Topas. We found a very large phase mismatch between the pump and the second-harmonic waves. Therefore the potential for cascaded quadratic second-harmonic generation is investigated in particular for soliton compression of fs pulses. We found that excitation of temporal solitons from cascaded quadratic nonlinearities requires an effective quadratic nonlinearity of 5 pm/V or more. This might be reduced if a polymer with a low Kerr nonlinear refractive index is used. We also found that the group-velocity mismatch could be minimized if the design parameters of the microstructured fiber are chosen so the relative hole size is large and the hole pitch is on the order of the pump wavelength. Almost all design-parameter combinations resulted in cascaded effects in the stationary regime, where efficient and clean soliton compression can be found. We therefore did not see any benefit from choosing a fiber design where the group-velocity mismatch was minimized. Instead numerical simulations showed excellent compression of $\lambda=800$ nm 120 fs pulses with nJ pulse energy to few-cycle duration using a standard endlessly single-mode design with a relative hole size of 0.4., Comment: 11 pages, 8 figures, submitted to JOSAB

We study cascaded quadratic soliton compressors and address the physical mechanisms that limit the compression. A nonlocal model is derived, and the nonlocal response is shown to have an additional oscillatory component in the nonstationary regime when the group-velocity mismatch (GVM) is strong. This inhibits efficient compression. Raman-like perturbations from the cascaded nonlinearity, competing cubic nonlinearities, higher-order dispersion, and soliton energy may also limit compression, and through realistic numerical simulations we point out when each factor becomes important. We find that it is theoretically possible to reach the single-cycle regime by compressing high-energy fs pulses for wavelengths $\lambda=1.0-1.3 \mu{\rm m}$ in a $\beta$-barium-borate crystal, and it requires that the system is in the stationary regime, where the phase mismatch is large enough to overcome the detrimental GVM effects. However, the simulations show that reaching single-cycle duration is ultimately inhibited by competing cubic nonlinearities as well as dispersive waves, that only show up when taking higher-order dispersion into account., Comment: 16 pages, 5 figures, submitted to Optics Express

We study soliton pulse compression in materials with cascaded quadratic nonlinearities, and show that the group-velocity mismatch creates two different temporally nonlocal regimes. They correspond to what is known as the stationary and nonstationary regimes. The theory accurately predicts the transition to the stationary regime, where highly efficient pulse compression is possible., Comment: 3 pages, 2 figures, published verison in Optics Letters. Contains revised equations, including an updated model

We present a detailed study of soliton compression of ultra-short pulses based on phase-mismatched second-harmonic generation (\textit{i.e.}, the cascaded quadratic nonlinearity) in bulk quadratic nonlinear media. The single-cycle propagation equations in the temporal domain including higher-order nonlinear terms are presented. The balance between the quadratic (SHG) and the cubic (Kerr) nonlinearity plays a crucial role: we define an effective soliton number -- related to the difference between the SHG and the Kerr soliton numbers -- and show that it has to be larger than unity for successful pulse compression to take place. This requires that the phase mismatch be below a critical level, which is high in a material where the quadratic nonlinearity dominates over the cubic Kerr nonlinearity. Through extensive numerical simulations we find dimensionless scaling laws, expressed through the effective soliton number, which control the behaviour of the compressed pulses. These laws hold in the stationary regime, in which group-velocity mismatch effects are small, and they are similar to the ones observed for fiber soliton compressors. The numerical simulations indicate that clean compressed pulses below two optical cycles can be achieved in a $\beta$-barium borate crystal at appropriate wavelengths, even for picosecond input pulses., Comment: 11 pages, 8 figures, resubmitted version, to appear in October issue of J. Opt. Soc. Am. B. Substantially revised, updated model

By using the ghost imaging technique, we experimentally demonstrate the reconstruction of the diffraction pattern of a {\em pure phase} object by using the classical correlation of incoherent thermal light split on a beam splitter. The results once again underline that entanglement is not a necessary feature of ghost imaging. The light we use is spatially highly incoherent with respect to the object ($\approx 2 \mu$m speckle size) and is produced by a pseudo-thermal source relying on the principle of near-field scattering. We show that in these conditions no information on the phase object can be retrieved by only measuring the light that passed through it, neither in a direct measurement nor in a Hanbury Brown-Twiss (HBT) scheme. In general, we show a remarkable complementarity between ghost imaging and the HBT scheme when dealing with a phase object., Comment: 13 pages, 11 figures. Published in Physical Review A. Replaced version fixes some problems with Figs. 1, 4 and 10

Comment on A.F. Abouraddy, P.R. Stone, A.V. Sergienko, B.E.A. Saleh, and M.C. Teich, ``Entangled-Photon Imaging of a Pure Phase Object,'' Phys. Rev. Lett. 93, 213903 (2004). Unpublished (rejected by Physical Review Letters), but for a publication holding main points see A. Gatti, M. Bache, D. Magatti, E. Brambilla, F. Ferri, and L.A. Lugiato "Coherent imaging with pseudo-thermal incoherent light", Journal of Modern Optics 53, 739-760 (2006), quant-ph/0504082., Comment: Comment on A.F. Abouraddy, P.R. Stone, A.V. Sergienko, B.E.A. Saleh, and M.C. Teich, ``Entangled-Photon Imaging of a Pure Phase Object,'' Phys. Rev. Lett. 93, 213903 (2004). Unpublished (rejected by Physical Review Letters), but for a publication holding main points see A. Gatti, M. Bache, D. Magatti, E. Brambilla, F. Ferri, and L.A. Lugiato "Coherent imaging with pseudo-thermal incoherent light", Journal of Modern Optics 53, 739-760 (2006), quant-ph/0504082. 1 page, 1 figure

We investigate experimentally fundamental properties of coherent ghost imaging using spatially incoherent beams generated from a pseudo-thermal source. A complementarity between the coherence of the beams and the correlation between them is demonstrated by showing a complementarity between ghost diffraction and ordinary diffraction patterns. In order for the ghost imaging scheme to work it is therefore crucial to have incoherent beams. The visibility of the information is shown for the ghost image to become better as the object size relative to the speckle size is decreased, and therefore a remarkable tradeoff between resolution and visibility exists. The experimental conclusions are backed up by both theory and numerical simulations., Comment: 11 pages, 12 figures, to appear in J. Mod. Opt

We consider travelling-wave parametric down-conversion in the high-gain regime and present the experimental demonstration of the quantum character of the spatial fluctuations in the system. In addition to showing the presence of sub-shot noise fluctuations in the intensity difference, we demonstrate that the peak value of the normalized spatial correlations between signal and idler lies well above the line marking the boundary between the classical and the quantum domain. This effect is equivalent to the apparent violation of the Cauchy-Schwartz inequality, predicted by some of us years ago, which represents a spatial analogue of photon antibunching in time. Finally, we analyse numerically the transition from the quantum to the classical regime when the gain is increased and we emphasize the role of the inaccuracy in the determination of the symmetry center of the signal/idler pattern in the far-field plane., Comment: 21 pages, 11 figures, submitted to J. Mod. Opt. special issue on Quantum Imaging

In ghost imaging schemes information about an object is extracted by measuring the correlation between a beam that passed the object and a reference beam. We present a spatial averaging technique that substantially improves the imaging bandwidth of such schemes, which implies that information about high-frequency Fourier components can be observed in the reconstructed diffraction pattern. In the many-photon regime the averaging can be done in parallel and we show that this leads to a much faster convergence of the correlations. We also consider the reconstruction of the object image, and discuss the differences between a pixel-like detector and a bucket detector in the object arm. Finally, it is shown how to non-locally make spatial filtering of a reconstructed image. The results are presented using entangled beams created by parametric down-conversion, but they are general and can be extended also to the important case of using classically correlated thermal-like beams., Comment: 15 pages, published in Optics Express. Figures in online version miss some information in axes labels, therefore we have updated the arXiv version to the published version and with the correct axes labels. The movies are available at the Optics Express home page

Using a 1GW-1ps pump laser pulse in high gain parametric down-conversion allows us to detect sub-shot-noise spatial quantum correlation with up to one hundred photoelectrons per mode, by means of a high efficiency CCD. The statistics is performed in single-shot over independent spatial replica of the system. The paper highlights the evidence of quantum correlation between symmetrical signal and idler spatial areas in the far field, in the high gain regime. In accordance with the predictions of numerical calculations the observed transition from the quantum to the classical regime is interpreted as a consequence of the narrowing of the down-converted beams in the very high gain regime., Comment: 4,2 pages, 4 figures

We analytically show that it is possible to perform coherent imaging by using the classical correlation of two beams obtained by splitting incoherent thermal radiation. A formal analogy is demonstrated between two such classically correlated beams and two entangled beams produced by parametric down-conversion. Because of this analogy, the classical beams can mimic qualitatively all the imaging properties of the entangled beams, even in ways which up to now were not believed possible. A key feature is that these classical beams are spatially correlated both in the near-field and in the far-field. Using realistic numerical simulations the performances of a quasi-thermal and a parametric down-conversion source are shown to be closely similar, both for what concerns the resolution and statistical properties. The results of this paper provide a new scenario for the discussion of what role the entanglement plays in correlated imaging., Comment: 9 pages, 6 figures, in press in Phys. Rev. A (May 2004)

We present a theoretical study of ghost imaging based on correlated beams arising from parametric down-conversion, and which uses balanced homodyne detection to measure both the signal and idler fields. We analytically show that the signal-idler correlations contain the full amplitude and phase information about an object located in the signal path, both in the near-field and the far-field case. To this end we discuss how to optimize the optical setups in the two imaging paths, including the crucial point regarding how to engineer the phase of the idler local oscillator as to observe the desired orthogonal quadrature components of the image. We point out an inherent link between the far-field bandwidth and the near-field resolution of the reproduced image, determined by the bandwidth of the source of the correlated beams. However, we show how to circumvent this limitation by using a spatial averaging technique which dramatically improves the imaging bandwidth of the far-field correlations as well as speeds up the convergence rate. The results are backed up by numerical simulations taking into account the finite size and duration of the pump pulse., Comment: 17 pages, 10 figures, submitted to Phys. Rev. A

We study the spatial correlations of quantum fluctuations that can be observed in multi-mode spontaneous parametric down-conversion in the regime of high gain. A stochastic model has been solved numerically to obtain quantitative results beyond the stationary plane-wave pump approximation. The pulsed shape of the pump beam and other features of the system, such as spatial walk-off and diffraction are taken into account. Their effect on the spatial quantum correlations predicted by the plane-wave pump theory is investigated, both for near field and far field measurements, in a type I and in a type II phase-matching configuration., Comment: 18 pages, 10 figures

A model is proposed where two $\chi^{(2)}$ nonlinear waveguides are contained in a cavity suited for second-harmonic generation. The evanescent wave coupling between the waveguides is considered as weak, and the interplay between this coupling and the nonlinear interaction within the waveguides gives rise to quantum violations of the classical limit. These violations are particularly strong when two instabilities are competing, where twin-beam behavior is found as almost complete noise suppression in the difference of the fundamental intensities. Moreover, close to bistable transitions perfect twin-beam correlations are seen in the sum of the fundamental intensities, and also the self-pulsing instability as well as the transition from symmetric to asymmetric states display nonclassical twin-beam correlations of both fundamental and second-harmonic intensities. The results are based on the full quantum Langevin equations derived from the Hamiltonian and including cavity damping effects. The intensity correlations of the output fields are calculated semi-analytically using a linearized version of the Langevin equations derived through the positive-P representation. Confirmation of the analytical results are obtained by numerical simulations of the nonlinear Langevin equations derived using the truncated Wigner representation., Comment: 15 pages, 8 figures, submitted to Phys. Rev. A

We investigate the spatial quantum noise properties of the one dimensional transverse pattern formation instability in intra-cavity second-harmonic generation. The Q representation of a quasi-probability distribution is implemented in terms of nonlinear stochastic Langevin equations. We study these equations through extensive numerical simulations and analytically in the linearized limit. Our study, made below and above the threshold of pattern formation, is guided by a microscopic scheme of photon interaction underlying pattern formation in second-harmonic generation. Close to the threshold for pattern formation, beams with opposite direction of the off-axis critical wave numbers are shown to be highly correlated. This is observed for the fundamental field, for the second harmonic field and also for the cross-correlation between the two fields. Nonlinear correlations involving the homogeneous transverse wave number, which are not identified in a linearized analysis, are also described. The intensity differences between opposite points of the far fields are shown to exhibit sub-Poissonian statistics, revealing the quantum nature of the correlations. We observe twin beam correlations in both the fundamental and second-harmonic fields, and also nonclassical correlations between them., Comment: 18 pages, 17 figures, submitted to Phys. Rev. A