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1. Roadmap on energy harvesting materials

Author

Pecunia, Vincenzo, Silva, S Ravi P, Phillips, Jamie D, Artegiani, Elisa, Romeo, Alessandro, Shim, Hongjae, Park, Jongsung, Kim, Jin Hyeok, Yun, Jae Sung, Welch, Gregory C, Larson, Bryon W, Creran, Myles, Laventure, Audrey, Sasitharan, Kezia, Flores-Diaz, Natalie, Freitag, Marina, Xu, Jie, Brown, Thomas M, Li, Benxuan, Wang, Yiwen, Li, Zhe, Hou, Bo, Hamadani, Behrang H, Defay, Emmanuel, Kovacova, Veronika, Glinsek, Sebastjan, Kar-Narayan, Sohini, Bai, Yang, Bin Kim, Da, Cho, Yong Soo, Žukauskaitė, Agnė, Barth, Stephan, Fan, Feng Ru, Wu, Wenzhuo, Costa, Pedro, del Campo, Javier, Lanceros-Mendez, Senentxu, Khanbareh, Hamideh, Wang, Zhong Lin, Pu, Xiong, Pan, Caofeng, Zhang, Renyun, Xu, Jing, Zhao, Xun, Zhou, Yihao, Chen, Guorui, Tat, Trinny, Ock, Il Woo, Chen, Jun, Graham, Sontyana Adonijah, Yu, Jae Su, Huang, Ling-Zhi, Li, Dan-Dan, Ma, Ming-Guo, Luo, Jikui, Jiang, Feng, Lee, Pooi See, Dudem, Bhaskar, Vivekananthan, Venkateswaran, Kanatzidis, Mercouri G, Xie, Hongyao, Shi, Xiao-Lei, Chen, Zhi-Gang, Riss, Alexander, Parzer, Michael, Garmroudi, Fabian, Bauer, Ernst, Zavanelli, Duncan, Brod, Madison K, Al Malki, Muath, Snyder, G Jeffrey, Kovnir, Kirill, Kauzlarich, Susan M, Uher, Ctirad, Lan, Jinle, Lin, Yuan-Hua, Fonseca, Luis, Morata, Alex, Martin-Gonzalez, Marisol, Pennelli, Giovanni, Berthebaud, David, Mori, Takao, Quinn, Robert J, Bos, Jan-Willem G, Candolfi, Christophe, Gougeon, Patrick, Gall, Philippe, Lenoir, Bertrand, Venkateshvaran, Deepak, Kaestner, Bernd, Zhao, Yunshan, Zhang, Gang, Nonoguchi, Yoshiyuki, Schroeder, Bob C, Bilotti, Emiliano, Menon, Akanksha K, Urban, Jeffrey J, Fenwick, Oliver, Asker, Ceyla, and Talin, A Alec

Subjects
Engineering, Materials Engineering, Affordable and Clean Energy, energy harvesting materials, photovoltaics, thermoelectric energy harvesting, piezoelectric energy harvesting, triboelectric energy harvesting, radiofrequency energy harvesting, sustainability, Macromolecular and materials chemistry, Physical chemistry, Materials engineering
Abstract

Ambient energy harvesting has great potential to contribute to sustainable development and address growing environmental challenges. Converting waste energy from energy-intensive processes and systems (e.g. combustion engines and furnaces) is crucial to reducing their environmental impact and achieving net-zero emissions. Compact energy harvesters will also be key to powering the exponentially growing smart devices ecosystem that is part of the Internet of Things, thus enabling futuristic applications that can improve our quality of life (e.g. smart homes, smart cities, smart manufacturing, and smart healthcare). To achieve these goals, innovative materials are needed to efficiently convert ambient energy into electricity through various physical mechanisms, such as the photovoltaic effect, thermoelectricity, piezoelectricity, triboelectricity, and radiofrequency wireless power transfer. By bringing together the perspectives of experts in various types of energy harvesting materials, this Roadmap provides extensive insights into recent advances and present challenges in the field. Additionally, the Roadmap analyses the key performance metrics of these technologies in relation to their ultimate energy conversion limits. Building on these insights, the Roadmap outlines promising directions for future research to fully harness the potential of energy harvesting materials for green energy anytime, anywhere.

Published
2023

2. Exceptional Performance of Room Temperature Sputtered Flexible Thermoelectric Thin Film Using High Target Utilisation Sputtering Technique.

Author

Tao, Xudong, Dutson, James, Zeng, Chongyang, Asker, Ceyla, Luong, Sally, Reza, Abdallah, Hao, Botao, Zhang, Zheng, Ellingford, Joshua, Bonilla, Ruy Sebastian, Fenwick, Oliver, Bilotti, Emiliano, Hofmann, Felix, Thwaites, Mike, and Assender, Hazel E.

Subjects
THIN films, THERMOELECTRIC materials, BISMUTH telluride, CARRIER density, THERMOELECTRIC apparatus & appliances, MANUFACTURING processes, MAGNETRON sputtering
Abstract

The High Target Utilisation Sputtering technique (HiTUS) is of interest for industrial processes, including in roll‐to‐roll manufacturing. This study marks the first application of HiTUS to thermoelectric materials, exemplified by bismuth telluride. The HiTUS technique separates the sputtering power into the plasma power and the target power, with additional kinetic energy in the sputtering particles from the applied electrical field, thus enabling a much wider sputter parameter space to modify the film performance. This study investigates how plasma power, target power, and substrate bias in HiTUS intricately influence crystal orientation/size, elemental composition, surface morphology, and other film properties. These factors subsequently affect carrier density/mobility, and consequently the thermoelectric performance of the bismuth telluride film. These deposited films reach a power factor of 6.5 × 10−4 W m−1 K−2 with a figure of merit ≈0.14 at room temperature, the highest value for room‐temperature sputtered un‐doped bismuth telluride. Subsequent post‐deposition annealing significantly enhances the crystallinity of the film (highly polycrystalline), further improving the power factor to 23.5 × 10−4 W m−1 K‐2, with a figure of merit ≈0.45 at room temperature. The excellent performance of the HiTUS fabricated thermoelectric film opens opportunities for the large‐area manufacture of thin‐film thermoelectric materials and devices. [ABSTRACT FROM AUTHOR]

Published
2024
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3. Roadmap on energy harvesting materials

Author

Fonds de Recherche du Québec, Canada Research Chairs, University of Calgary, Department of Energy (US), Pecunia, Vincenzo, Silva, S.Ravi P., Phillips, Jamie D., Artegiani, Elisa, Romeo, Alessandro, Shim, Hongjae, Park, Jongsung, Kim, Jin Hyeok, Yun, Jae Sung, Welch, Gregory C., Larson, Bryon W., Brod, Madison K., Al Malki, Muath, G Jeffrey Snyder, Kirill Kovnir, Kauzlarich, Susan M., Uher, Ctirad, Lan, Jinle, Lin, Yuan-Hua, Fonseca. Luis, Morata, Alex, Candolfi, Christophe, Martín-González, Marisol, Pennelli, Giovanni, Berthebaud, David, Mori, Takao, Quinn, Robert J., Bos, Jan-Willem G., Gougeon, Patrick, Gall, Philippe, Lenoir, Bertrand, Venkateshvaran, Deepak, Kaestner, Bernd, Zhao, Yunshan, Zhang, Gang, Nonoguchi, Yoshiyuki, Schroeder,Bob C., Anthopoulos, Thomas D., Bilotti, Emiliano, Menon, Akanksha K., Urban, Jeffrey J., Fenwick, Oliver, Asker, Ceyla, Talin, A. Alec, Losi, Tommaso, Viola, Fabrizio, Caironi, Mario., Georgiadou, Dimitra G., Ding, Li, Peng, Lian-Mao, Wang, Zhenxing, Wei,Muh-Dey, Negra, Renato, Creran, Myles, Lemme, Max C., Wagih, Mahmoud, Beeby, Steve, Ibn-Mohammed, Taofeeq, Mustapha, K. B., Joshi, A. P., Laventure, Audrey, Sasitharan, Kezia, Flores-Diaz, Natalie, Freitag, Marina, Xu, Jie, Brown, Thomas M., Li, Benxuan, Wang, Yiwen, Li, Zhe, Hou, Bo, Hamadani, Behrang H., Defay, Emmanuel, Kovacova, Veronika, Glinsek, Sebastjan, Kar-Narayan, Sohini, Bai, Yang, Kim, Da Bin, Cho, Yong Soo, Žukauskaitė, Agnė, Barth, Stephan, Fan, Feng Ru, Wu, Wenzhuo, Costa, Pedro, Campo, Javier del, Lanceros-Mendez, Senentxu, Khanbareh, Hamideh, Wang, Zhong Lin, Pu, Xiong, Pan, Caofeng, Zhang, Renyun, Xu, Jing, Zhao, Xun, Zhou, Yihao, Chen, Guorui, Tat, Trinny, Ock, Il Woo, Chen, Jun, Sontyana Adonijah Graham, Yu, Jae Su, Huang, Ling-Zhi, Li, Dan-Dan, Ma, Ming-Guo, Luo, Jikui, Jiang, Feng, Lee, Pooi See, Dudem, Bhaskar, Vivekananthan, Venkateswaran, Kanatzidis, Mercouri G., Xie, Hongyao, Shi, Xiao-Lei, Chen, Zhi-Gang, Riss, Alexander, Parzer, Michael, Garmroudi, Fabian, Bauer, Ernst, Zavanelli, Duncan, Fonds de Recherche du Québec, Canada Research Chairs, University of Calgary, Department of Energy (US), Pecunia, Vincenzo, Silva, S.Ravi P., Phillips, Jamie D., Artegiani, Elisa, Romeo, Alessandro, Shim, Hongjae, Park, Jongsung, Kim, Jin Hyeok, Yun, Jae Sung, Welch, Gregory C., Larson, Bryon W., Brod, Madison K., Al Malki, Muath, G Jeffrey Snyder, Kirill Kovnir, Kauzlarich, Susan M., Uher, Ctirad, Lan, Jinle, Lin, Yuan-Hua, Fonseca. Luis, Morata, Alex, Candolfi, Christophe, Martín-González, Marisol, Pennelli, Giovanni, Berthebaud, David, Mori, Takao, Quinn, Robert J., Bos, Jan-Willem G., Gougeon, Patrick, Gall, Philippe, Lenoir, Bertrand, Venkateshvaran, Deepak, Kaestner, Bernd, Zhao, Yunshan, Zhang, Gang, Nonoguchi, Yoshiyuki, Schroeder,Bob C., Anthopoulos, Thomas D., Bilotti, Emiliano, Menon, Akanksha K., Urban, Jeffrey J., Fenwick, Oliver, Asker, Ceyla, Talin, A. Alec, Losi, Tommaso, Viola, Fabrizio, Caironi, Mario., Georgiadou, Dimitra G., Ding, Li, Peng, Lian-Mao, Wang, Zhenxing, Wei,Muh-Dey, Negra, Renato, Creran, Myles, Lemme, Max C., Wagih, Mahmoud, Beeby, Steve, Ibn-Mohammed, Taofeeq, Mustapha, K. B., Joshi, A. P., Laventure, Audrey, Sasitharan, Kezia, Flores-Diaz, Natalie, Freitag, Marina, Xu, Jie, Brown, Thomas M., Li, Benxuan, Wang, Yiwen, Li, Zhe, Hou, Bo, Hamadani, Behrang H., Defay, Emmanuel, Kovacova, Veronika, Glinsek, Sebastjan, Kar-Narayan, Sohini, Bai, Yang, Kim, Da Bin, Cho, Yong Soo, Žukauskaitė, Agnė, Barth, Stephan, Fan, Feng Ru, Wu, Wenzhuo, Costa, Pedro, Campo, Javier del, Lanceros-Mendez, Senentxu, Khanbareh, Hamideh, Wang, Zhong Lin, Pu, Xiong, Pan, Caofeng, Zhang, Renyun, Xu, Jing, Zhao, Xun, Zhou, Yihao, Chen, Guorui, Tat, Trinny, Ock, Il Woo, Chen, Jun, Sontyana Adonijah Graham, Yu, Jae Su, Huang, Ling-Zhi, Li, Dan-Dan, Ma, Ming-Guo, Luo, Jikui, Jiang, Feng, Lee, Pooi See, Dudem, Bhaskar, Vivekananthan, Venkateswaran, Kanatzidis, Mercouri G., Xie, Hongyao, Shi, Xiao-Lei, Chen, Zhi-Gang, Riss, Alexander, Parzer, Michael, Garmroudi, Fabian, Bauer, Ernst, and Zavanelli, Duncan

Abstract

Ambient energy harvesting has great potential to contribute to sustainable development and address growing environmental challenges. Converting waste energy from energy-intensive processes and systems (e.g. combustion engines and furnaces) is crucial to reducing their environmental impact and achieving net-zero emissions. Compact energy harvesters will also be key to powering the exponentially growing smart devices ecosystem that is part of the Internet of Things, thus enabling futuristic applications that can improve our quality of life (e.g. smart homes, smart cities, smart manufacturing, and smart healthcare). To achieve these goals, innovative materials are needed to efficiently convert ambient energy into electricity through various physical mechanisms, such as the photovoltaic effect, thermoelectricity, piezoelectricity, triboelectricity, and radiofrequency wireless power transfer. By bringing together the perspectives of experts in various types of energy harvesting materials, this Roadmap provides extensive insights into recent advances and present challenges in the field. Additionally, the Roadmap analyses the key performance metrics of these technologies in relation to their ultimate energy conversion limits. Building on these insights, the Roadmap outlines promising directions for future research to fully harness the potential of energy harvesting materials for green energy anytime, anywhere.

Published
2023

6. Quasi-Zero Dimensional Halide Perovskite Derivates: Synthesis, Status, and Opportunity

Author

Trifiletti, V, Asker, C, Tseberlidis, G, Riva, S, Zhao, K, Tang, W, Binetti, S, Fenwick, O, Trifiletti, Vanira, Asker, Ceyla, Tseberlidis, Giorgio, Riva, Stefania, Zhao, Keran, Tang, Weidong, Binetti, Simona, Fenwick, Oliver, Trifiletti, V, Asker, C, Tseberlidis, G, Riva, S, Zhao, K, Tang, W, Binetti, S, Fenwick, O, Trifiletti, Vanira, Asker, Ceyla, Tseberlidis, Giorgio, Riva, Stefania, Zhao, Keran, Tang, Weidong, Binetti, Simona, and Fenwick, Oliver

Abstract

In recent decades, many technological advances have been enabled by nanoscale phenomena, giving rise to the field of nanotechnology. In particular, unique optical and electronic phenomena occur on length scales less than 10 nanometres, which enable novel applications. Halide perovskites have been the focus of intense research on their optoelectronic properties and have demonstrated impressive performance in photovoltaic devices and later in other optoelectronic technologies, such as lasers and light-emitting diodes. The most studied crystalline form is the three-dimensional one, but, recently, the exploration of the low-dimensional derivatives has enabled new sub-classes of halide perovskite materials to emerge with distinct properties. In these materials, low-dimensional metal halide structures responsible for the electronic properties are separated and partially insulated from one another by the (typically organic) cations. Confinement occurs on a crystal lattice level, enabling bulk or thin-film materials that retain a degree of low-dimensional character. In particular, quasi-zero dimensional perovskite derivatives are proving to have distinct electronic, absorption, and photoluminescence properties. They are being explored for various technologies beyond photovoltaics (e.g. thermoelectrics, lasing, photodetectors, memristors, capacitors, LEDs). This review brings together the recent literature on these zero-dimensional materials in an interdisciplinary way that can spur applications for these compounds. The synthesis methods, the electrical, optical, and chemical properties, the advances in applications, and the challenges that need to be overcome as candidates for future electronic devices have been covered.

Published
2021

7. (Invited) Atomic Layer Deposition of MOF from Dissolved Precursors ― ‘Solution ALD’ (sALD)

Author

Barr, Maissa K. S., primary, Nadiri, Soheila, additional, Chen, Dong-Hui, additional, Weidler, Peter G., additional, Baumgart, Helmut -, additional, Redel, Engelbert, additional, Asker, Ceyla, additional, Forberich, Karen, additional, Hoga, Felix, additional, Stubhan, Tobias, additional, Egelhaaf, Hans, additional, Brabec, Christoph, additional, and Bachmann, Julien, additional

Published
2020
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