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16 results on '"Arunoday Singh"'

1. Dual impression technique for fabrication of maxillary complete immediate denture

Author

Ashish Kumar Srivastava, Ujjal Chaterjee, Madhu Ranjan, and Arunoday Singh

Subjects
dual impression technique, esthetics, immediate denture, Dentistry, RK1-715
Abstract

Conventional complete denture apart from all its merits has the prominent disadvantage of leaving the patient for a brief period of edentulous state till definitive prosthesis can be fabricated. Therefore, the concept of immediate denture is to preserve the jaw relation, keep the patient habituated to the complete denture and in the process preserve the esthetic concern of the patient. In the process, the psychological well-being of the patient is preserved as the patient is not without teeth for any prolonged period. The challenge in this technique is to record the edentulous and dentulous portion of the arch in conjecture with each other so that the final impression is closest to the intraoral situation, enabling us to provide the best results in short-and long-term of complete denture fabrication.

Published
2016
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2. Fluorescent excimers and exciplexes of the purine base derivative 8-phenylethynyl-guanine in DNA hairpins

Author

Frederick D. Lewis, Arunoday Singh, Lin Ma, Yi Lin Wu, Ryan M. Young, Brian T. Phelan, Michael R. Wasielewski, Ashutosh Kumar Mishra, and Kristen E. Brown

Subjects
Nucleobase analog, Circular dichroism, Guanine, 010405 organic chemistry, DNA, 010402 general chemistry, Photochemistry, Excimer, 01 natural sciences, Fluorescence, 0104 chemical sciences, Nucleobase, Thymine, chemistry.chemical_compound, chemistry, Purines, Nucleic Acid Conformation, Physical and Theoretical Chemistry, Cytosine
Abstract

The ground- and excited-state electronic interactions between the nucleobase analog 8-(4′-phenylethynyl)deoxyguanosine, EG, with natural nucleobases and 7-deazaguanine, as well as between adjacent EG base analogs, have been characterized using a combination of steady-state spectroscopy and time-resolved fluorescence, absorption, and stimulated Raman spectroscopies. The properties of the nucleoside EG-H2 are only weakly perturbed upon incorporation into synthetic DNA hairpins in which thymine, cytosine or adenine are the bases flanking EG. Incorporation of the nucleoside to be adjacent to guanine or deazaguanine results in the formation of short-lived (40–80 ps) exciplexes, the charge transfer character of which increases as the oxidation potential of the donor decreases. Hairpins possessing two or three adjacent EG base analogs display exciton-coupled circular dichroism in the ground state and form long-lived fluorescent excited states upon electronic excitation. Incorporation of EG into the helical scaffold of the DNA hairpins places it adjacent to its neighboring nucleobases or a second EG, thus providing the close proximity required for the formation of exciplex or excimer intermediates upon geometric relaxation of the short-lived EG excited state. The three time-resolved spectroscopic methods employed permit both the characterization of the several intermediates and the kinetics of their formation and decay.

Published
2017

3. Tracking hole transport in DNA hairpins using a phenylethynylguanine nucleobase

Author

Jiawang Zhou, Ashutosh Kumar Mishra, Ryan M. Young, Kristen E. Brown, Arunoday Singh, Michael R. Wasielewski, Frederick D. Lewis, and Yi Lin Wu

Subjects
Electron donor, Electrons, 010402 general chemistry, Photochemistry, Spectrum Analysis, Raman, 01 natural sciences, Biochemistry, Catalysis, Nucleobase, Electron Transport, chemistry.chemical_compound, symbols.namesake, Colloid and Surface Chemistry, Stilbenes, chemistry.chemical_classification, 010405 organic chemistry, Chemistry, Deoxyguanosine, General Chemistry, DNA, Chromophore, Electron acceptor, Electron transport chain, Acceptor, 0104 chemical sciences, G-Quadruplexes, Radical ion, symbols, Nucleic Acid Conformation, Raman spectroscopy
Abstract

The hole transport dynamics of DNA hairpins possessing a stilbene electron acceptor and donor along with a modified guanine (G) nucleobase, specifically 8-(4′-phenylethynyl)deoxyguanosine, or EG, have been investigated. The nearly indistinguishable oxidation potentials of EG and G and unique spectroscopic characteristics of EG+• make it well-suited for directly observing transient hole occupation during charge transport between a stilbene electron donor and acceptor. In contrast to the cation radical G+•, EG+• possesses a strong absorption near 460 nm and has a distinct Raman-active ethynyl stretch. Both spectroscopic characteristics are easily distinguished from those of the stilbene donor/acceptor radical ion chromophores. Employing EG, we observe its role as a shallow hole trap, or as an intermediate hole transport site when a deeper trap state is present. Using a combination of ultrafast absorption and stimulated Raman spectroscopies, the hole-transport dynamics are observed to be similar in systems having EG vs G bases, with small perturbations to the charge transport rates and yields. These results show EG can be deployed at specified locations throughout the sequence to report on hole occupancy, thereby enabling detailed monitoring of the hole transport dynamics with base-site specificity

Published
2017

4. Structure and Electronic Spectra of Purine–Methyl Viologen Charge Transfer Complexes

Author

Frederick D. Lewis, George C. Schatz, Tomekia Simeon, Arunoday Singh, Almaz S. Jalilov, Sameer Patwardhan, and Amy A. Sarjeant

Subjects
Models, Molecular, Paraquat, Magnetic Resonance Spectroscopy, Molecular Structure, Absorption spectroscopy, Chemistry, Binding energy, Solvation, Nuclear magnetic resonance spectroscopy, Crystal structure, Crystallography, X-Ray, Electrostatics, Article, Surfaces, Coatings and Films, Purines, Materials Chemistry, Quantum Theory, Molecule, Physical chemistry, Spectrophotometry, Ultraviolet, Density functional theory, Protons, Physical and Theoretical Chemistry
Abstract

The structure and properties of the electron donor-acceptor complexes formed between methyl viologen (MV) and purine nucleosides and nucleotides in water and the solid state have been investigated using a combination of experimental and theoretical methods. Solution studies were performed using UV-vis and 1H NMR spectroscopy. Theoretical calculations were performed within the framework of density functional theory (DFT). Energy decomposition analysis indicates that dispersion and induction (charge-transfer) interactions dominate the total binding energy, whereas electrostatic interactions are largely repulsive. The appearance of charge transfer bands in the absorption spectra of the complexes are well described by time-dependent (TD) DFT and are further explained in terms of the redox properties of purine monomers and solvation effects. Crystal structures are reported for complexes of methyl viologen with the purines 2′-deoxyguanosine 3′-monophosphate GMP (DAD′DAD′ type) and 7-deazaguanosine zG (DAD′ADAD′ type). Comparison of the structures determined in the solid state and by theoretical methods in solution provides valuable insights into the nature of charge-transfer interactions involving purine bases as electron donors.

Published
2013
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5. Solution-Phase Synthesis of Branched DNA Hybrids Based on Dimer Phosphoramidites and Phenolic or Nucleosidic Cores

Author

Clemens Richert, Helmut Griesser, Arunoday Singh, Mariyan Tolev, Claudia Gerlach, and Thomas Sabirov

Subjects
Phosphoramidite, Oligonucleotide, Base pair, Dimer, Adamantane, Organic Chemistry, Oligonucleotides, Nucleosides, Trimer, DNA, Solutions, chemistry.chemical_compound, Organophosphorus Compounds, chemistry, Yield (chemistry), Solid-Phase Synthesis Techniques, Organic chemistry, Base Pairing
Abstract

Branched oligonucleotides with "CG zippers" as DNA arms assemble into materials from micromolar solutions. Their synthesis has been complicated by low yields in solid-phase syntheses. Here we present a solution-phase synthesis based on phosphoramidites of dimers and phenolic cores that produces six-arm or four-arm hybrids in up to 61% yield. On the level of hybrids, only the final product has to be purified by precipitation or chromatography. A total of five different hybrids were prepared via the solution-phase route, including new hybrid (TCG)(4)TTPA with a tetrakis(triazolylphenyl)adamantane core and trimer DNA arms. The new method is more readily scaled up than solid-phase syntheses, uses no more than 4 equiv of phosphoramidite per phenolic alcohol, and provides routine access to novel materials that assemble via predictable base-pairing interactions.

Published
2012
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6. Deep-hole transfer leads to ultrafast charge migration in DNA hairpins

Author

Michelle A. Harris, Frederick D. Lewis, Nicolas Renaud, Michael R. Wasielewski, Mark A. Ratner, Arunoday Singh, Ferdinand C. Grozema, and Yuri A. Berlin

Subjects
Models, Molecular, General Chemical Engineering, Nanotechnology, 02 engineering and technology, Deep hole, 010402 general chemistry, 01 natural sciences, Nucleobase, chemistry.chemical_compound, Electron transfer, Dna nanostructures, Atomic orbital, Stilbenes, Circular Dichroism, Charge (physics), General Chemistry, DNA, 021001 nanoscience & nanotechnology, 0104 chemical sciences, chemistry, Chemical physics, Nucleic Acid Conformation, Quantum Theory, Electronics, 0210 nano-technology, Ultrashort pulse
Abstract

Charge transport through the DNA double helix is of fundamental interest in chemistry and biochemistry, but also has potential technological applications such as for DNA-based nanoelectronics. For the latter, it is of considerable interest to explore ways to influence or enhance charge transfer. In this Article we demonstrate a new mechanism for DNA charge transport, namely 'deep-hole transfer', which involves long-range migration of a hole through low-lying electronic states of the nucleobases. Here, we demonstrate, in a combined experimental and theoretical study, that it is possible to achieve such transfer behaviour by changing the energetics of charge injection. This mechanism leads to an enhancement in transfer rates by up to two orders of magnitude and much weaker distance dependence. This transfer is faster than relaxation to the lowest-energy state, setting this mechanism apart from those previously described. This opens up a new direction to optimize charge transfer in DNA with unprecedented charge-transfer rates.

Published
2016
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7. Raising the barrier for photoinduced DNA charge injection with a cyclohexyl artificial base pair

Author

Ryan M. Young, Frederick D. Lewis, Michael R. Wasielewski, Arunoday Singh, Michelle A. Harris, and Stephen A. Miller

Subjects
Exergonic reaction, Base pair, Guanine, Photochemistry, Charge (physics), DNA, Imides, Acceptor, chemistry.chemical_compound, Photoinduced charge separation, chemistry, Cyclohexanes, Physical and Theoretical Chemistry, Base Pairing, Perylene, Recombination
Abstract

The effects of an artificial cyclohexyl base pair on the quantum yields of fluorescence and dynamics of charge separation and charge recombination have been investigated for several synthetic DNA hairpins. The hairpins possess stilbenedicarboxamide, perylenediimide, or naphthalenediimide linkers and base-paired stems. In the absence of the artificial base pair hole injection into both adenine and guanine purine bases is exergonic and irreversible, except in the case of stilbene with adenine for which it is slightly endergonic and reversible. Insertion of the artificial base pair renders hole injection endergonic or isoergonic except in the case of the powerful naphthalene acceptor for which it remains exergonic. Both hole injection and charge recombination are slower for the naphthalene acceptor in the presence of the artificial base pair than in its absence. The effect of an artificial base pair on charge separation and charge recombination in hairpins possessing stilbene and naphthalene acceptor linkers and a stilbenediether donor capping group has also been investigated. In the case of the stilbene acceptor–stilbene donor capped hairpins photoinduced charge separation across six base pairs is efficient in the absence of the artificial base pair but does not occur in its presence. In the case of the naphthalene acceptor–stilbene donor capped hairpins the artificial base pair slows but does not stop charge separation and charge recombination, leading to the formation of long-lived charge separated states.

Published
2015

8. Conformationally Gated Charge Transfer in DNA Three-Way Junctions

Author

Michael R. Wasielewski, Arun K. Thazhathveetil, Ryan M. Young, David N. Beratan, Frederick D. Lewis, Alexander A. Voityuk, Khatcharin Siriwong, Chaoren Liu, Nicolas Renaud, Yuqi Zhang, Arunoday Singh, Mark A. Ratner, Ferdinand C. Grozema, and Yuri A. Berlin

Subjects
Quantitative Biology::Biomolecules, Kinetics, Charge (physics), Gating, DNA, Nanosecond, Molecular Dynamics Simulation, chemistry.chemical_compound, Molecular dynamics, Crystallography, Electron transfer, chemistry, Chemical physics, General Materials Science, Physical and Theoretical Chemistry, Quantum
Abstract

Molecular structures that direct charge transport in two or three dimensions possess some of the essential functionality of electrical switches and gates. We use theory, modeling, and simulation to explore the conformational dynamics of DNA three-way junctions (TWJs) that may control the flow of charge through these structures. Molecular dynamics simulations and quantum calculations indicate that DNA TWJs undergo dynamic interconversion among "well stacked" conformations on the time scale of nanoseconds, a feature that makes the junctions very different from linear DNA duplexes. The studies further indicate that this conformational gating would control charge flow through these TWJs, distinguishing them from conventional (larger size scale) gated devices. Simulations also find that structures with polyethylene glycol linking groups ("extenders") lock conformations that favor CT for 25 ns or more. The simulations explain the kinetics observed experimentally in TWJs and rationalize their transport properties compared with double-stranded DNA.

Published
2015

9. Charge Transport across DNA-Based Three-Way Junctions

Author

George C. Schatz, Arun K. Thazhathveetil, Michael R. Wasielewski, Yuri A. Berlin, Nicolas Renaud, Ferdinand C. Grozema, Mark A. Ratner, Arunoday Singh, Yuqi Zhang, David N. Beratan, Frederick D. Lewis, Ryan M. Young, and Vincent Y. Cho

Subjects
Models, Molecular, Chemistry, Base pair, Spectrum Analysis, Molecular electronics, General Chemistry, DNA, Nanosecond, Molecular Dynamics Simulation, Biochemistry, Catalysis, Coupling (electronics), Electron Transport, Molecular dynamics, Kinetics, Colloid and Surface Chemistry, Chemical physics, Femtosecond, Ultrafast laser spectroscopy, A-DNA, Atomic physics, Base Pairing
Abstract

DNA-based molecular electronics will require charges to be transported from one site within a 2D or 3D architecture to another. While this has been shown previously in linear, π-stacked DNA sequences, the dynamics and efficiency of charge transport across DNA three-way junction (3WJ) have yet to be determined. Here, we present an investigation of hole transport and trapping across a DNA-based three-way junction systems by a combination of femtosecond transient absorption spectroscopy and molecular dynamics simulations. Hole transport across the junction is proposed to be gated by conformational fluctuations in the ground state which bring the transiently populated hole carrier nucleobases into better aligned geometries on the nanosecond time scale, thus modulating the π-π electronic coupling along the base pair sequence.

Published
2015

10. Measurement of jet fragmentation in PbPb andppcollisions atsNN=2.76TeV

Author

Richard Vidal, Alexandre Zabi, Vladimir Rekovic, Ian Shipsey, Matthias Kasemann, Stephen Sanders, Wesley H Smith, Vladimir Cherepanov, Hasan Ogul, R. K. Shivpuri, T. Dahms, Kenichi Hatakeyama, Anna Woodard, Petr Levchenko, Marco Costa, M. De Palma, Nikolai Golubev, D. R. Claes, Anders Ryd, Gavin Davies, J. Haley, T. Aliev, Alexander Lanev, Georgios Daskalakis, Alessandra Romero, Sergei Gninenko, Senka Duric, Guler Karapinar, S. Petrushanko, J. W. Gary, M. Rodenburg, John Paul Chou, Brian Paul Padley, J. Piedra Gomez, R. Wilken, Gregory Iles, S. Schael, R. Kroeger, K. Petridis, N. Ratnikova, V. Timciuc, Colin Bernet, Nadia Pastrone, Loic Quertenmont, Aram Apyan, Martti Raidal, Marcos Fernandez, John Perry Cumalat, Swagata Mukherjee, G. M. Chen, Burin Asavapibhop, A. Harel, Matthew Nguyen, W. Zou, Young-Il Choi, Florian Beaudette, X. Shi, Philip H Butler, M. Hansen, Inkyu Park, A. Mohapatra, Pedro G Mercadante, A. Bethani, C. Rogan, G. Zito, Cecilia Elena Gerber, Livia Soffi, Christopher Seez, Marcella Diemoz, P. Verdier, Marino Missiroli, Andrius Juodagalvis, Alexis Pompili, Stephen Wimpenny, Henning Flacher, K. Mishra, Nikolaos Manthos, Ada Solano, Artur Kalinowski, N. Dupont-Sagorin, Hans-Christian Kaestli, D. Meister, P. Goldenzweig, X. Aslanoglou, C. La Licata, N. Beaupere, B. Tali, D. Sunar Cerci, Oliver Gutsche, S. Dooling, Gaetano-Marco Dallavalle, Jose F Benitez, B. Hooberman, Martin Grunewald, A. Perieanu, O. Novgorodova, P. Juillot, P. Katsas, U. E. Surat, H. Gamsizkan, Wolfram Erdmann, Nicolo Cartiglia, J. Sekaric, V. Chetluru, Rajat Gupta, J. Puerta Pelayo, Indara Suarez, T. Seva, Yong Ban, L. Winstrom, Mara Senghi Soares, Serguei Ganjour, E. Torassa, E. Gurpinar, Silvia Taroni, Nikolai Shumeiko, Andreas Pfeiffer, R. Guida, Bora Akgun, Kreso Kadija, Jeffrey Richman, Gilvan Alves, Pierluigi Paolucci, Thomas Bergauer, Darien Wood, Jyothsna Rani Komaragiri, D. Klingebiel, F. Giordano, G. Wrochna, J. S. Werner, Frank Hartmann, Luciano Orsini, Luca Pacher, G. Merino, Vladimir Mossolov, Vardan Khachatryan, J. Anderson, G. Brona, Natascha Hörmann, Tejinder Virdee, Nicholas John Hadley, Jehad Mousa, P. E. Marage, T. Sinthuprasith, R. Stringer, D. Ryckbosch, D. Nash, M. Cardaci, A. Fahim, A. Gude, Hyunyong Kim, J. G. Shiu, M. Bontenackels, Luigi Guiducci, A. Mott, Nicolò Tosi, Karl Matthew Ecklund, B. Gobbo, Giuseppe Bagliesi, C. Beluffi, Gregory R Snow, J. H. Kim, Igor Volobouev, E. Takasugi, M. Jones, Seth Conrad Zenz, Georgia Karapostoli, Z. Meng, T. Weiler, A. Vorobyev, M. Vidal Marono, S. De Visscher, Julia Thom, Finn Rebassoo, Andreas Psallidas, Michael Kramer, C. Vander Velde, T. Christiansen, Claire Shepherd-Themistocleous, M. Naimuddin, Daniel Denegri, M. A. Mahmoud, Hartmut Stadie, C. Justus, Songkyo Lee, Markus Stoye, A. A. Ocampo Rios, N. Pietsch, M. Grothe, Alain Hervé, Ludivine Ceard, Xuejun Wang, V. Kozhuharov, A. Adiguzel, Ivan Vila, S. Carrillo Moreno, Elisabetta Gallo, A. Zuranski, Brian L Winer, Volker Blobel, Lucia Silvestris, Neeti Parashar, M. Zeinali, R. Wilkinson, M. Bergholz, Klaus Rabbertz, B. Betchart, Mehmet Özgür Sahin, Donato Creanza, Igor Lokhtin, Kadri Ozdemir, Heriberto Castilla-Valdez, Douglas Wright, Giacomo Fedi, M. Deniz, W. S. Hou, Vladimir Karjavin, Kerstin Borras, Andris Skuja, J. Wagner-Kuhr, Ivica Puljak, Hans Reithler, Ben Bylsma, C. Baus, W. Van Doninck, C. Lucas, Tomas Lindén, E. Tuovinen, Alice Florent, Christian Böser, Stephen Mrenna, K. Nawrocki, J. A. Gomez, Konstantin Androsov, G. Kukartsev, W. L. Aldá Júnior, Dietrich Liko, Mykhailo Dalchenko, D. Fehling, M. Sharma, A. Custódio, Riccardo Andrea Manzoni, D. Liang, Christian Veelken, Otilia Militaru, Sebastian Thüer, Carlo Civinini, J. Chen, S. Naumann-Emme, Christoph Schwick, Richard Lander, Yi Guo, Suyog Shrestha, Simone Gennai, G. Gomez Ceballos, P. Garcia-Abia, A. Kasmi, Nikos Varelas, Helen F Heath, S. Gowdy, A. A. Abdelalim, Tai Sakuma, K. Klapoetke, E. Dietz-Laursonn, J. Robles, Ferhat Ozok, L. Barone, Andreas Nürnberg, Roberto Tenchini, C. Dietz, J. Babb, W. De Boer, F. Nowak, Marc Weinberg, Marco Zanetti, Robert M Brown, Gabriella Pugliese, J. Heilman, S. A. Koay, Kevin Lannon, C. Martin, G. Della Ricca, H. Geenen, Giuseppe Iaselli, M. Chasco, Marc Dobson, M. Choi, N. Eggert, Jaehyeok Yoo, S. Kailas, Jacobo Konigsberg, N. Wickramage, Dong-Chul Son, Liliana Teodorescu, P. Paganini, Georgi Sultanov, Yu. Andreev, Markus Klute, C. Fabjan, Joel Goldstein, Luigi Calligaris, E. Luiggi Lopez, Yutaro Iiyama, E. Navarro De Martino, O. Charaf, Intae Yu, David Cutts, Kevin Stenson, K. Rose, Achim Stahl, T. Scarborough, M. R. Adams, D. Kcira, Tae Jeong Kim, Michael Murray, Jakob Salfeld-Nebgen, Kevin Pedro, Martin Görner, Lutz Feld, Tommaso Boccali, Adolf Bornheim, B. A. Barnett, Katerina Lipka, Martin Kirakosyan, S. C. Kao, L. Muniz, H. Van Haevermaet, J. Ott, Guenakh Mitselmakher, F. Margaroli, L. K. Gibbons, Anna Elliott-Peisert, Jordan Damgov, Alessandro Giassi, Giacomo Ortona, M. Grimes, Vuko Brigljevic, D. Burton, Julian Bunn, J. Ilic, H. Mermerkaya, J. D. Ruiz Alvarez, H. Schettler, M. Mohammadi Najafabadi, Panja-Riina Luukka, Giuseppe Codispoti, Roberto Salerno, Olga Kodolova, Bora Isildak, V. P. Andreev, Shahram Rahatlou, Daniele Bonacorsi, Silvano Tosi, G. Polese, I. Villella, Daniel Treille, W. J. Womersley, D. De Jesus Damiao, S. Ganguly, Aran Garcia-Bellido, L. M. Cremaldi, H. Snoek, Nazar Bartosik, David Stuart, Alice Mignerey, Marvin Johnson, G. Bianchi, C. A. Carrillo Montoya, G. H. Hammad, Franco Ligabue, J. Lingemann, Jose M Hernandez, S. Panwalkar, Y. J. Lu, Chayanit Asawatangtrakuldee, Yetkin Yilmaz, M. Marone, Vladimir Epshteyn, A. Ostapchuk, Claude Amsler, Laurent Favart, J. Ellison, Cristian Pena, Teng Ma, Thomas Reis, S. Maruyama, Viatcheslav Stolin, J. Marrouche, Maurizio Pierini, David Cussans, P. Siegrist, Andrea Carlo Marini, German Martinez, Cristina Botta, R. P. Kenny, E. Kwon, F. Vazquez Valencia, Po-Hsun Chen, Stefano Mersi, Alexander Tapper, H. A. Weber, Vyacheslav Krutelyov, L. Borrello, Frank Würthwein, Manas Maity, Alexi Mestvirishvili, Metin Yalvac, Daniel Noonan, Gobinda Majumder, Y. Assran, M. Z. Mehta, Dario Bisello, David Sperka, Gaelle Boudoul, Jiyeon Han, Alexis Kalogeropoulos, Alexander Nikitenko, Caterina Vernieri, A. Y. Rodríguez-Marrero, B. Michlin, U. Nauenberg, M. Chamizo Llatas, Jasvinder A. Singh, A. S. Yoon, Alessandro Gaz, Ulrich Goerlach, I Heredia-de La Cruz, Steve Nahn, Paolo Capiluppi, James Rohlf, Carlos Avila, S. K. Park, M. Chan, D. Puigh, David Stickland, Stefano Ragazzi, Jane Nachtman, Sergei Bitioukov, John L Wood, Jan Veverka, Ricardo Eusebi, Daniel Pitzl, S. Ozturk, Mithat Kaya, R. Gonzalez Suarez, Sergio F Novaes, M. Vutova, J. Bernardini, Teresa Rodrigo, A. Degano, G. Mesyats, A. Baden, Denis Favart, D. Silvers, Suyong Choi, Etiennette Auffray, Sridhara Dasu, Emilio Meschi, Sam Harper, R. Travaglini, R. Plestina, Shuichi Kunori, M. Quittnat, Maurizio Biasini, A. Heister, Marta Felcini, Josef Hrubec, T. Peiffer, M. Maes, J. Santaolalla, Evgueni Vlasov, Morgan Lethuillier, Yasar Onel, Dipanwita Dutta, I. Bucinskaite, S. Liang, Maksat Haytmyradov, S. Paktinat Mehdiabadi, Aruna Nayak, P. Jindal, Othmane Bouhali, Mani Tripathi, Pierre Piroué, Paolo Azzurri, M. Searle, Marco Peruzzi, Owen Rosser Long, Günther Dissertori, Yi Chen, Teresa Lenz, A. Gurtu, D. Hidas, Guido Tonelli, Zeljko Antunovic, T. Umer, Gervasio Gomez, A. Calamba, J. Zablocki, Claudia-Elisabeth Wulz, Christoph Paus, I. Topsis-Giotis, Enrico Robutti, S. D. Worm, Laurent Mirabito, C. Beirão Da Cruz E Silva, Steven Lowette, O. Oberst, Raman Khurana, D. Lazic, David Mason, Alexei Safonov, Y. H. Chang, P. Miné, Luigi Moroni, Luca Lista, Wolfgang Waltenberger, S. Flowers, Kurtis F Johnson, Greg P Heath, Elena Tikhonenko, Cesare Calabria, A. Delgado Peris, S. Wakefield, Archana Sharma, Nicola Amapane, Piergiulio Lenzi, Rylan Conway, Jordan Nash, J. F. de Trocóniz, Sung Keun Park, Matthias Ulrich Mozer, D. Barge, T. Y. Kim, S. S. Yu, Andreas Nowack, G. Breto, E. A. Albayrak, R. Carroll, A. Raval, Ignacio Redondo, Franco Gonella, Benjamin Stieger, A. Descroix, Bugra Bilin, Alexandros Attikis, Kati Lassila-Perini, R. Granier de Cassagnac, Maxime Gouzevitch, Saptaparna Bhattacharya, Paraskevas Sphicas, L. Sgandurra, Rachel Yohay, Salvatore My, James G Branson, S. A. Schmitz, A. Morelos Pineda, D. Knowlton, Daniele Pedrini, G. Broccolo, Victor Krychkine, J. G. Smith, L. Brigliadori, James Dolen, David Petyt, Yurii Maravin, Janos Erö, T. Mäenpää, Jesus Marco, Vladimir Gavrilov, Andrey Korytov, P. Chang, Eduardo De Moraes Gregores, David Krofcheck, Petra Merkel, A. Leonidov, Christoph Schäfer, Sergio P Ratti, A. Ershov, Freya Blekman, Ilse Krätschmer, Y. Pakhotin, Si Xie, J. Härkönen, Robert Stone, Ricardo Lopez-Fernandez, R. Walsh, M. Ivova Rikova, Bradley Cox, Y. M. Tzeng, Jonathan Hollar, Maria Agnese Ciocci, Sanjay Jain, Dave Pellett, Marko Kovac, L. Rebane, Vladimir Korenkov, S. Beranek, P. Fabbricatore, Maria Florencia Canelli, Julia Velkovska, P. Giubilato, F. Simonetto, J. P. Fernández Ramos, Willis Lin, Alexander Malakhov, Efe Yazgan, Aleko Khukhunaishvili, Y. Tu, C. Lin, Günter Flügge, Fabrizio Ferro, Thomas Ferbel, Dan Green, S. Boutle, Chiara Mariotti, David Michael Morse, G. Hamel de Monchenault, Mikko Voutilainen, G. P. Van Onsem, Robert Harr, Marta Ruspa, Kai-Feng Chen, D. Horton, Stepan Obraztsov, C. Barth, I. Katkov, J. Tucker, Sudha Ahuja, Hannes Sakulin, Yueh-Feng Liu, A. Singovsky, A. Sparrow, T. Caebergs, Tilman Rohe, Konrad Deiters, V. Pavlunin, Robert Clare, Ettore Focardi, Markus Merschmeyer, Arie Bodek, Frank Chlebana, M. Kenzie, W. Hopkins, John Rander, Yang Yang, M. Planer, Giovanni Organtini, Jing Wang, Halil Saka, Pietro Govoni, Lorenzo Foà, J. G. Bian, Mohsen Naseri, A. C. Le Bihan, Ozlem Kaya, G. De Lentdecker, Sevil Salur, Patrizia Azzi, John Michael Marraffino, R. Sacchi, Anna Cimmino, E. De La Cruz-Burelo, A. York, J. Caudron, H. Kalakhety, Alexei Raspereza, Jan Krolikowski, Luiz Mundim, Duccio Abbaneo, P. Lawson, Andrew Levin, J. S. Keller, Salvatore Nuzzo, Philippe Bloch, Cesar Augusto Bernardes, Aniello Spiezia, Hannes Jung, S. Di Guida, P. Symonds, Alexander Zhokin, Martijn Mulders, W. Clarida, Nancy Marinelli, K. H. Chen, A. Sakharov, M. Niegel, T. Schoerner-Sadenius, Plamen Iaydjiev, Gyorgy Bencze, Dimitri Bourilkov, Vassili Kachanov, Andrew Whitbeck, P. Jandir, Viktor Veszpremi, S. Song, B. Safarzadeh, I. Gonzalez Caballero, B. Gomez Moreno, Shabnam Jabeen, I. N. Naranjo, Thomas Hebbeker, Paul Lecoq, F. Duru, A. De Roeck, Ian Michael Nugent, Albert M. Sirunyan, D. Sabes, Y. Eshaq, P. 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Lo Vetere, V. Monaco, Markus Seidel, D. Mekterovic, Vineet Kumar, J. Martínez-Ortega, L. Forthomme, Vladimir Popov, Javier Duarte, Jacopo Pazzini, Subir Sarkar, J. Mccartin, Ying Lu, Raffaele Gerosa, Alexander Ledovskoy, Vincent J Smith, James Alexander, D. H. Kim, Lukasz Kreczko, E. Ron, Byung-Sik Hong, Michael Hildreth, T. Kypreos, Andrey Pozdnyakov, C. Riedl, M. Bansal, A. Quintario Olmeda, W. Dominik, Thomas Kress, Rosamaria Venditti, N. Pozzobon, M. Zielinski, A. T. Serban, A. Tropiano, Bożena Boimska, Kerem Cankocak, Harrison Prosper, D. Cline, Stephen Robert Wagner, F. Lacroix, H. Seo, S. Knutzen, Steve Reucroft, L. Tauscher, Umesh Joshi, M. Murumaa, Irina Vardanyan, Achim Geiser, C. Farrell, Javier Cuevas, S. Senkin, Marcello Abbrescia, Z. Tsamalaidze, Danila Tlisov, S. V. Rusakov, P. Van Hove, Francesco Pandolfi, T. Khurshid, A. David, M. Baber, A. C. Benvenuti, Andres Tiko, A. M. Rossi, Federica Fanzago, Viktor Konoplyanikov, Th. Müller, Paul Sheldon, Yuichi Kubota, R. Ciesielski, Colin Jessop, K. Sogut, and M. Calderon De La Barca Sanchez

Subjects
Quark, Physics, Nuclear and High Energy Physics, Particle physics, Large Hadron Collider, Astrophysics::High Energy Astrophysical Phenomena, Charged particle, Nuclear physics, Fragmentation (mass spectrometry), Transverse momentum, Fragmentation function, High Energy Physics::Experiment, Impact parameter, Nuclear Experiment
Abstract

The jet fragmentation function of inclusive jets with transverse momentum p_T above 100GeV/c in PbPb collisions has been measured using reconstructed charged particles with p_T above 1GeV/c in a cone of radius 0.3 around the jet axis. A data sample of PbPb collisions collected in 2011 at a nucleon-nucleon center-of-mass energy of √sNN = 2.76 TeV corresponding to an integrated luminosity of 150μb^(−1) is used. The results for PbPb collisions as a function of collision centrality and jet transverse momentum are compared to reference distributions based on pp data collected at the same center-of-mass energy in 2013, with an integrated luminosity of 5.3pb^(−1). A centrality-dependent modification of the fragmentation function is found. For the most central collisions, a significant enhancement is observed in the PbPb/pp fragmentation function ratio for charged particles with p_T less than 3GeV/c. This enhancement is observed for all jet p_T bins studied.

Published
2014
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11. Measurement of WZ and ZZ production in pp collisions at $$\sqrts = 8\,\text TeV $$ s = 8 TeV in final states with b-tagged jets

Author

R. Frazier, J. C. Yun, Robert M Harris, T. Yetkin, V. Khotilovich, K. Kovitanggoon, Dmitri Konstantinov, M. Hempel, H. Rohringer, Charles C. Richardson, Arun Kumar, Daniele Spiga, Tariq Aziz, Dave M Newbold, Colin Jessop, K. Sogut, M. Calderon De La Barca Sanchez, Nicholas Wardle, David Jonathan Hofman, Marko Dragicevic, Willard Johns, Richard Vidal, Matthias Kasemann, R. Kroeger, Paola Salvini, Giacomo Sguazzoni, Alan Campbell, Stephen Sanders, Wesley H Smith, Marco Meschini, J. Eugster, E. Ntomari, Francisco Yumiceva, Valentina Gori, Ritva Kinnunen, Petar Maksimovic, Patrick Janot, M. Pimiä, Jordan Nash, Sung Keun Park, S. Bilmis, W. Bertl, M. Feindt, Karl Gill, Vipin Bhatnagar, Raffaella Radogna, G. Christopher, D. Giordano, Andrea Castro, Y. Choi, E. M. Da Costa, E. Karavakis, K. Goebel, M. A. Shah, V. Timciuc, Colin Bernet, Nadia Pastrone, N. Van Remortel, Kamuran Dilsiz, D. Renker, Paolo Rumerio, Lorenzo Uplegger, William T. Ford, U. Grundler, Christian Autermann, Thorsten Chwalek, F. Drouhin, N. Zaganidis, E. Schlieckau, A. Descroix, Bugra Bilin, Kati Lassila-Perini, Petra Merkel, V. Maroussov, I. Ross, Jose Chinellato, Richard Cavanaugh, Stephanie Baffioni, Mauro Menichelli, Lesya Shchutska, Andrea Massironi, Andreas Hinzmann, B. Calpas, Matt J. Jarvis, Marcin Konecki, A. Sanchez-Hernandez, H. Mendez, Nathaniel Pastika, M. Pioppi, Ioannis Evangelou, S. Semenov, A. Chatterjee, L. Benucci, Paul Dauncey, M. Franco Sevilla, Damir Lelas, A. Léonard, Urs Langenegger, L. Lusito, Anil Kumar, Francesco Navarria, Marcos Fernandez, M. Cutajar, Young-Il Choi, Florian Beaudette, Marcella Diemoz, Marco Rovere, Valentin Knünz, S. Erhan, Alexey Vorobyev, V. E. Bazterra, Martti Raidal, J. E. Ramirez Vargas, Si Xie, J. Härkönen, Robert Stone, Jean-Baptiste Sauvan, Gigi Rolandi, Stefano Argiro, Lucia Masetti, D. Gyun, Kenneth Bloom, Thomas Perry, Hannsjoerg Artur Weber, Gordon H. Hanson, B. Marangelli, D. 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Newman-Holmes, Edward Laird, Aurore Savoy-Navarro, Luca Mastrolorenzo, Vieri Candelise, Ted Kolberg, Claude Charlot, Robert Clare, Patrizia Azzi, R. Sacchi, A. A. Ocampo Rios, N. Pietsch, M. Grothe, Alain Hervé, V. Kozhuharov, A. Adiguzel, Ivan Vila, S. Carrillo Moreno, W. Van Doninck, C. Lucas, I. N. Naranjo, Tomas Lindén, E. Tuovinen, Thomas Hebbeker, Alice Florent, Paul Lecoq, Carlo Civinini, J. Chen, F. Duru, S. Naumann-Emme, A. De Roeck, Andrea Triossi, Christoph Schwick, Richard Lander, Ian Michael Nugent, Yi Guo, Suyog Shrestha, Simone Gennai, G. Gomez Ceballos, P. Garcia-Abia, A. Kasmi, Nikos Varelas, Helen F Heath, S. Gowdy, R. K. Shivpuri, T. Dahms, Albert M. Sirunyan, D. Sabes, Kenichi Hatakeyama, Anna Woodard, Petr Levchenko, Marco Costa, M. De Palma, Nikolai Golubev, D. R. Claes, Anders Ryd, Gavin Davies, E. Di Marco, M. Rossini, J. Haley, T. Aliev, Alexander Lanev, Georgios Daskalakis, Alessandra Romero, Sergei Gninenko, Arunoday Singh, Nicolas Filipovic, Senka Duric, Guler Karapinar, S. Petrushanko, Frans Meijers, Shu Li, J. W. Gary, M. Rodenburg, John Paul Chou, S. Habib, Kristian Harder, Brian Paul Padley, Thomas N. Williams, R. Wilken, Gregory Iles, S. Schael, K. Petridis, N. Ratnikova, Simone Paoletti, Suchandra Dutta, A. Gozzelino, T. Pearson, Anne-Marie Magnan, Wagner Carvalho, Greg Landsberg, Cécile Caillol, Manjit Kaur, E. Daubie, J. Rodrigues Antunes, Francesco Fiori, Philippe Busson, P. Eller, M. F. Turner, Pedrame Bargassa, Francesca Cavallari, V. I. Martinez Outschoorn, Stefano Belforte, Massimo Casarsa, Andrés G Delannoy, Christopher Hill, Jongmin Lee, Stefano Colafranceschi, Paolo Gunnellini, D. Martschei, S. Lynch, T. Medvedeva, Juliet Ritchie Patterson, Joao Varela, Leander Litov, P. Van Mulders, Alexander Dermenev, Jean-Pierre Merlo, Joanne Cole, Nikolai Krasnikov, Eija Tuominen, Luigi Fiore, Sami Lehti, Adish Vartak, M. Vazquez Acosta, S. Schnetzer, Giovanna Selvaggi, B. Parida, Gagan Bihari Mohanty, Gabor Istvan Veres, Igor Golutvin, Mircho Rodozov, Sarah Catherine Eno, G. Bauer, S. Blyweert, H. Arfaei, D. Benedetti, Pieter Everaerts, Alexx Perloff, Roman Ryutin, Federica Primavera, Roberto Carlin, Pierre Depasse, Vyacheslav Klyukhin, F. Bachmair, S. Casasso, A. Olbrechts, A. Drozdetskiy, Jennifer Ngadiuba, Nicola Bacchetta, Attila Racz, Roberta Arcidiacono, Jonathan Fulcher, Anatoli Pashenkov, Avto Kharchilava, Mikhail Ignatenko, Tapio Lampén, F. Thyssen, Fabrizio Fabbri, Christoph Wissing, M. Zeise, Patrick Jarry, Y. J. Lei, Benjamin Charles Radburn-Smith, Valentina Dutta, and I. Marfin

Subjects
Quantum chromodynamics, Physics, Particle physics, Gauge boson, Large Hadron Collider, Physics and Astronomy (miscellaneous), Order (ring theory), Supersymmetry, 7. Clean energy, Luminosity, Nuclear physics, Production (computer science), High Energy Physics::Experiment, Nuclear Experiment, Engineering (miscellaneous)
Abstract

Measurements are reported of the WZ and ZZ production cross sections in proton-proton collisions at $\sqrt{s}$ = 8 TeV in final states where one Z boson decays to b-tagged jets. The other gauge boson, either W or Z, is detected through its leptonic decay (either $W \to e\nu, \mu\nu$ or $Z \to e^+ e^-, \mu^+ \mu^-$, or $\nu\bar{\nu})$. The results are based on data corresponding to an integrated luminosity of 18.9 inverse-femtobarns collected with the CMS detector at the Large Hadron Collider. The measured cross sections, $\sigma(pp \to WZ)$ = 30.7 $\pm$ 9.3 (stat.) $\pm$ 7.1 (syst.) $\pm$ 4.1 (th.) $\pm$ 1.0 (lum.) pb and $\sigma(pp \to ZZ)$ = 6.5 $\pm$ 1.7 (stat.) $\pm$ 1.0 (syst.) $\pm$ 0.9 (th.) $\pm$ 0.2 (lum.) pb, are consistent with next-to-leading order quantum chromodynamics calculations.

Published
2014

12. Solution-phase synthesis of branched DNA hybrids via H-phosphonate dimers

Author

Christine I. Schilling, Helmut Griesser, Clemens Richert, Stefan Bräse, Arunoday Singh, and Mariyan Tolev

Subjects
Aqueous solution, Magnetic Resonance Spectroscopy, Molecular Structure, Chemistry, Stereochemistry, Oligonucleotide, Dimer, Adamantane, Organic Chemistry, Oligonucleotides, Organophosphonates, DNA, Phosphonate, Solutions, chemistry.chemical_compound, Yield (chemistry), Molecule, Dinucleoside Phosphates
Abstract

A method for the solution-phase synthesis of branched oligonucleotides with tetrahedral or pseudo-octahedral geometry is described that involves the coupling of 3'-H-phosphonates of protected dinucleoside phosphates and organic core molecules. The dimer building blocks are produced by a synthesis that requires no chromatographic purification and that produces the dimer H-phosphonates in up to 44% yield in less than three days of laboratory work. A total of seven different branched hybrids were prepared, including a new hybrid of the sequence (CG)(4)TBA, where TBA stands for tetrakis(p-hydroxybiphenyl)adamantane that assembles into a material from micromolar aqueous solution upon addition of MgCl(2).

Published
2012

13. Branched DNA that forms a solid at 95 °C

Author

Stefan Bräse, Mariyan Tolev, Clemens Richert, Christine I. Schilling, Konstantin V. Klenin, Martin Nieger, Wolfgang Wenzel, Arunoday Singh, Thierry Muller, Martin Meng, and Oliver Plietzsch

Subjects
Models, Molecular, Hot Temperature, Molecular model, Molecular Structure, Oligonucleotide, 010405 organic chemistry, General Chemistry, General Medicine, DNA, 010402 general chemistry, 01 natural sciences, Catalysis, 0104 chemical sciences, chemistry.chemical_compound, Biochemistry, chemistry, Nucleic Acid Conformation
Published
2010

14. Two base pair duplexes suffice to build a novel material

Author

Wolfgang Wenzel, Matthias Bauer, Arunoday Singh, Oliver Plietzsch, Clemens Richert, Thierry Muller, Shahid A. Soomro, Martin Meng, Carolin Ahlborn, and Stefan Bräse

Subjects
Materials science, Base pair, Oligonucleotides, Nanotechnology, Biochemistry, law.invention, chemistry.chemical_compound, law, Benzyl Compounds, Transition Temperature, Crystallization, Molecular Biology, Base Pairing, Fluorescent Dyes, Oligonucleotide, Transition temperature, Organic Chemistry, DNA, Nanostructures, Crystallography, chemistry, Tetrahedron, Molecular Medicine, Spectrophotometry, Ultraviolet, Multivalent binding
Abstract

Tetrahedral DNA hybrids with tetrakis(p-hydroxyphenyl)methane cores hybridize in a sequence-specific fashion at much higher temperatures than isolated linear duplexes. Dinucleotide DNA arms suffice to induce the formation of a solid at room temperature; this demonstrates the strength of multivalent binding. The graphic shows a view of a modeled assembly.

Published
2009

15. Designed DNA Crystals: Triangles with Short Sticky Ends

Author

Martin Meng, Arunoday Singh, and Clemens Richert

Subjects
Materials science, Macromolecular Substances, Surface Properties, Oligonucleotide, Molecular Conformation, Adhesiveness, Nanotechnology, DNA, General Chemistry, Nanostructures, Biomaterials, chemistry.chemical_compound, chemistry, Sticky and blunt ends, Materials Testing, General Materials Science, Particle Size, Crystallization, Biotechnology
Published
2009
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