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A widespread unconformity between Ordovician metasedimentary rocks and nonmetamorphosed Mesozoic sedimentary rocks across the Eastern Cordillera of Bolivia provides evidence for significant pre-Late Cretaceous deformation and erosion. In this paper, we refine the middle to late Paleozoic tectonic history of the central Andean segment of Gondwana's western margin. We combine Raman spectroscopy of carbonaceous material (RSCM) thermometry with semi-quantitative deformation temperature estimates from quartz recrystallization microstructures and published illite crystallinity values from Cambrian-Devonian sedimentary rocks that span the Eastern Cordillera of southern Bolivia at ~21°S. Estimates of peak temperature and deformation temperature range primarily between ~220 and ~ 400 °C and show a general increase with depth that defines a metamorphic field gradient between ~37 and ~ 47 °C/km. Temperatures obtained from Ordovician rocks directly below the unconformity require erosion of a > ~5 km overburden prior to the Late Cretaceous, which was likely accomplished by a combination of distributed cleavage development and Paleozoic folding and thrust faulting revealed from cross-section reconstructions. The peak temperature data are incorporated into thermal models along with published illite K Ar, zircon (U Th)/He, and zircon fission-track cooling ages that refine the timing of Paleozoic orogenesis in the central Andes. We interpret shortening-related flexural subsidence driven by cratonward growth of a pre-Andean orogenic wedge along the western margin of Gondwana, with peak temperature conditions attained during eastward advance of a foreland basin between ~420 and ~ 318 Ma during the Devonian-Carboniferous Gondwanide Orogeny. Erosional exhumation between ~352 and ~ 294 Ma was the result of continued growth and eastward expansion of the associated Transpampean tectonic highland across the Eastern Cordillera. The growth of this pre-Andean contractional orogen coincided with global plate reorganization and the reestablishment of subduction and arc magmatism along the western margin of Gondwana, as indicated by a significant influx of Carboniferous arc-related detritus into the foreland basin system.

The Bolivian Andes are an archetypal convergent margin orogen with a paired fold-thrust belt and foreland basin. Existing chronostratigraphic constraints highlight a discrepancy between unroofing of the Eastern Cordillera and Interandean Zone fold-thrust systems since 40 Ma and the onset of rapid sediment accumulation in the Subandean Chaco foreland after 11 Ma, previously attributed to Miocene climate shifts. New results from magnetostratigraphic, backstripping, erosional volumetric calculations, and flexural modeling efforts are integrated with existing structural and thermochronologic datasets to investigate the linkages between shortening, exhumation, and subsidence. Magnetostratigraphic and backstripping results determine tectonic subsidence in the Chaco foreland basin, which informs flexural models that evaluate topographic load and lithospheric parameters. These models show that Chaco foreland subsidence is consistent with a range of loading scenarios. Eroded volumes from the fold-thrust belt were sufficient to fill the Chaco foreland basin, further supporting the linkage between sediment source and sink. Erosional beveling of the Eastern Cordillera, local intermontane sediment accumulation after 30–25 Ma, and regional development of the high-elevation San Juan del Oro geomorphic surface from 25 to 10 Ma suggest that the western Eastern Cordillera did not store the large sediment volume expected from erosion of the fold-thrust belt, which arrived in the Subandean Zone after 11 Ma. Eocene to middle Miocene foreland basin accumulation was likely focused between the Eastern Cordillera and Interandean Zone, and has been almost completely recycled into the modern Subandean foreland basin. The delay between initial fold-thrust belt exhumation (early Cenozoic) and rapid Subandean subsidence (late Cenozoic) highlights the interplay between protracted shortening, underthrusting, and foreland basin recycling. Only with sufficient crustal shortening, accommodated by eastward advance of the fold-thrust belt and attendant underthrusting of Brazilian Shield lithosphere beneath the Subandes, did the Subandean zone enter proximal foreland basin deposystems after ca. 11 Ma. Prior to the late Miocene, the precursor flexural basin was situated westward and not wide enough to incorporate the distal Subandean Zone. These results highlight the interplay between a range of crustal and surface processes linked to tectonics and Miocene climate shifts on the evolution of the southern Bolivian Andes.

Reliable crustal shortening estimates for the central Andes (South America) are a critical component in validating models of Cordilleran processes. In southern Bolivia, insight into crustal shortening and the kinematic development of the Andean thrust belt are limited by the lack of a unified structural evaluation across the entire width of the retroarc region. To address these shortcomings, we (1) estimate crustal shortening by integrating new geologic mapping with published geophysical data to construct a balanced cross section across the Subandean zone (SAZ), Interandean zone (IAZ), and Eastern Cordillera (EC) at 21°S; (2) develop a kinematic model for the retroarc thrust belt; and (3) estimate crustal budgets and average crustal thicknesses over the region. We estimate 337 ± 69 km (36% ± 7%) of total shortening (SAZ, 82 km; IAZ, 70 km; EC, 120 km; Altiplano, 65 km). The thrust belt developed from late Eocene time to the present by tectonic wedging and eastward emplacement of two ∼10–12-km-thick basement thrust sheets that distribute slip into overlying sedimentary rocks. Our range of crustal shortening values can account for 90%–118% of the current retroarc crustal area. Assuming an initial crustal thickness of 35 km, the EC and Altiplano did not achieve modern crustal thicknesses (∼65 km) until the present. However, assuming a 40-km-thick initial crust, the EC and Altiplano attained the critical thickness for either eclogitic phase changes or lower crustal flow (>45–50 km) by ca. 27–25 Ma, modern thicknesses by ca. 10 Ma, and currently exceed geophysically observed thicknesses by ∼2.5–14.5 km; this suggests crustal losses significant enough to have affected hinterland surface elevation.