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Background: There have been measurements on roughly 230 nuclei that are β-delayed neutron emitters. They range from 8 He up to 150La. Apart from 210Tl, with a branching ratio of only 0.007%, no other neutron emitter has been measured beyond A = 150. Therefore, new data are needed, particularly in the region of heavy nuclei around N = 126, in order to guide theoretical models and help understand the formation of the third r-process peak at A ∼ 195. Purpose: To measure both β-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb, and Bi isotopes beyond N = 126. Method: Ions of interest were produced by fragmentation of a 238U beam, selected and identified via the GSI-FRS fragment separator. A stack of segmented silicon detectors (SIMBA) was used to measure ion implants and β decays. An array of 30 3 He tubes embedded in a polyethylene matrix (BELEN) was used to detect neutrons with high efficiency and selectivity. A self-triggered digital system is employed to acquire data and to enable time correlations. The latter were analyzed with an analytical model and results for the half-lives and neutron-branching ratios were derived by using the binned maximum-likelihood method. Results: Twenty new β-decay half-lives are reported for 204−206Au, 208–211Hg, 211–216Tl, 215–218Pb, and 218–220Bi, nine of them for the first time. Neutron emission probabilities are reported for 210,211Hg and 211–216Tl. Conclusions: The new β-decay half-lives are in good agreement with previous measurements on nuclei in this region. The measured neutron emission probabilities are comparable to or smaller than values predicted by global models such as relativistic Hartree Bogoliubov plus the relativistic quasi-particle random phase approximation (RHB + RQRPA). Spanish Ministerio de Economía y Competitividad-FPA2011- 28770-C03-03, FPA2008-04972-C03-3, AIC-D2011-0705, FPA2011-24553, FPA2008-6419, FPA2010-17142, FPA2014-52823-C2-1-P, FPA2014- 52823-C2-2-P, and CPAN CSD-2007-00042 (Ingenio2010) Program Severo Ochoa-SEV-2014-0398 German Helmholtz Association (Young Investigators)-VH-NG 627 (LISA-Lifetime Spectroscopy for Astrophysics) Nuclear Astrophysics Virtual Institute-VH-VI-417 German Bundesministerium für Bildung und Forschung-06MT7178 / 05P12WOFNF Spanish Nuclear Security Council (CSN)-Catedra Argos UK Science & Technology Facilities Council (STFC)-ST/F012012/1

The β-delayed neutron emission probabilities of neutron rich Hg and Tl nuclei have been measured together with β-decay half-lives for 20 isotopes of Au, Hg, Tl, Pb, and Bi in the mass region N≳126. These are the heaviest species where neutron emission has been observed so far. These measurements provide key information to evaluate the performance of nuclear microscopic and phenomenological models in reproducing the high-energy part of the β-decay strength distribution. This provides important constraints on global theoretical models currently used in r-process nucleosynthesis. Ministerio de Economia y Competitividad SEV-2014-0398 FPA2011-24553 FPA2011-28770-C03-03 FPA2014-52823-C2-1-P AIC-D-2011-0705 Catedra Argos VH-NG 627 German Bundesministerium für Bildung und Forschung 06MT7178 / 05P12WOFNF. UK

In this work we explore for the first time the applicability of using $\gamma$-ray imaging in neutron capture measurements to identify and suppress spatially localized background. For this aim, a pinhole gamma camera is assembled, tested and characterized in terms of energy and spatial performance. It consists of a monolithic CeBr$_3$ scintillating crystal coupled to a position-sensitive photomultiplier and readout through an integrated circuit AMIC2GR. The pinhole collimator is a massive carven block of lead. A series of dedicated measurements with calibrated sources and with a neutron beam incident on a $^{197}$Au sample have been carried out at n_TOF, achieving an enhancement of a factor of two in the signal-to-background ratio when selecting only those events coming from the direction of the sample., Comment: Preprint submitted to Nucl. Instr. and Meth. A