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Monolayer transition-metal dichalcogenides (TMDCs) show a wealth of exciton physics. Here, we report the existence of a new excitonic species, the high-lying exciton (HX), in single-layer WSe2 with an energy of ~3.4 eV, almost twice the band-edge A-exciton energy, with a linewidth as narrow as 5.8 meV. The HX is populated through momentum-selective optical excitation in the K-valleys and is identified in upconverted photoluminescence (UPL) in the UV spectral region. Strong electron-phonon coupling results in a cascaded phonon progression with equidistant peaks in the luminescence spectrum, resolvable to ninth order. Ab initio GW-BSE calculations with full electron-hole correlations explain HX formation and unmask the admixture of upper conduction-band states to this complex many-body excitation. These calculations suggest that the HX is comprised of electrons of negative mass. The coincidence of such high-lying excitonic species at around twice the energy of band-edge excitons rationalizes the excitonic quantum-interference phenomenon recently discovered in optical second-harmonic generation (SHG) and explains the efficient Auger-like annihilation of band-edge excitons.

Quantum control of solid-state spin qubits typically involves pulses in the microwave domain, drawing from the well-developed toolbox of magnetic resonance spectroscopy. Driving a solid-state spin by optical means offers a high-speed alternative, which in the presence of limited spin coherence makes it the preferred approach for high-fidelity quantum control. Bringing the full versatility of magnetic spin resonance to the optical domain requires full phase and amplitude control of the optical fields. Here, we imprint a programmable microwave sequence onto a laser field and perform electron spin resonance in a semiconductor quantum dot via a two-photon Raman process. We show that this approach yields full SU(2) spin control with over 98% pi-rotation fidelity. We then demonstrate its versatility by implementing a particular multi-axis control sequence, known as spin locking. Combined with electron-nuclear Hartmann-Hahn resonances which we also report in this work, this sequence will enable efficient coherent transfer of a quantum state from the electron spin to the mesoscopic nuclear ensemble., Comment: 11 pages, 10 figures

Optical fibre networks are advancing rapidly to meet growing traffic demands. Security issues, including attack management, have become increasingly important for optical communication networks because of the vulnerabilities associated with tapping light from optical fibre links. Physical layer security often requires restricting access to channels and periodic inspections of link performance. In this paper, we report how quantum communication techniques can be utilized to detect a physical layer attack. We present an efficient method for monitoring the physical layer security of a high-data-rate classical optical communication network using a modulated continuous-variable quantum signal. We describe the theoretical and experimental underpinnings of this monitoring system and the monitoring accuracy for different monitored parameters. We analyse its performance for both unamplified and amplified optical links. The technique represents a novel approach for applying quantum signal processing to practical optical communication networks and compares well with classical monitoring methods. We conclude by discussing the challenges facing its practical application, its differences with respect to existing quantum key distribution methods, and its usage in future secure optical transport network planning., Optical communication security: Sound the quantum alarm A quantum alarm system can detect eavesdropping on optical communication links faster than classical methods. The system was developed by Yupeng Gong and colleagues at the University of Cambridge, UK, and involves transmitting two modes that are indistinguishable to an eavesdropper over the same channel and at the same wavelength. One mode sends a classical data signal and the other sends the security-monitoring quantum modulated signal. The alarm system is low-cost and can easily be used with high data-rate communication links that are hundreds of kilometers long. It can also be used with other encryption methods. The quantum alarm overcomes issues in other attack detection techniques, including quantum key distribution, which is challenging to implement in high data-rate optical communication networks.

A practical way to link separate nodes in quantum networks is to send photons over the standard telecom fibre network. This requires sub-Poissonian photon sources in the telecom wavelength band around 1550 nm, where the photon coherence time has to be sufficient to enable the many interference-based technologies at the heart of quantum networks. Here, we show that droplet epitaxy InAs/InP quantum dots emitting in the telecom C-band can provide photons with coherence times exceeding 1 ns even under non-resonant excitation, more than a factor two longer than values reported for shorter wavelength quantum dots under similar conditions. We demonstrate that these coherence times enable near-optimal interference with a C-band laser qubit, with visibilities only limited by the quantum dot multiphoton emission. Using entangled photons, we further show teleportation of such qubits in six different bases with average fidelity reaching 88.3$\pm$4%. Beyond direct applications in long-distance quantum communication, the high degree of coherence in these quantum dots is promising for future spin based telecom quantum network applications., 8 pages, 3 figures