1. Peeling graphite layer by layer reveals the charge exchange dynamics of ions inside a solid
- Author
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(0000-0002-5838-5789) Niggas, A., (0000-0002-4391-4270) Creutzburg, S., (0000-0002-7799-6606) Schwestka, J., Wöckinger, B., (0000-0002-9218-0605) Gupta, T., (0000-0003-0199-0520) Grande, P. L., (0000-0002-5395-564X) Eder, D., (0000-0002-3797-3880) Marques, J. P., (0000-0002-4829-3207) Bayer, B. C., (0000-0002-9788-0934) Aumayr, F., (0000-0001-6931-8840) Bennett, R., (0000-0001-9451-5440) Wilhelm, R. A., (0000-0002-5838-5789) Niggas, A., (0000-0002-4391-4270) Creutzburg, S., (0000-0002-7799-6606) Schwestka, J., Wöckinger, B., (0000-0002-9218-0605) Gupta, T., (0000-0003-0199-0520) Grande, P. L., (0000-0002-5395-564X) Eder, D., (0000-0002-3797-3880) Marques, J. P., (0000-0002-4829-3207) Bayer, B. C., (0000-0002-9788-0934) Aumayr, F., (0000-0001-6931-8840) Bennett, R., and (0000-0001-9451-5440) Wilhelm, R. A.
- Abstract
Over seventy years ago, Niels Bohr described how the charge state of an atomic ion moving through a solid changes dynamically as a result of electron capture and loss processes, eventually resulting in an equilibrium charge state. Although obvious, this process has so far eluded direct experimental observation. By peeling a solid, such as graphite, layer by layer, and studying the transmission of highly charged ions through single-, bi- and trilayer graphene, we can now observe dynamical changes in ion charge states with monolayer precision. In addition we present a new first-principles approach based on the virtual photon model for interparticle energy transfer to corroborate our findings. Our model that uses a Gaussian shaped dynamic polarisability rather than a spatial delta function is a major step in providing a self-consistent description for interparticle de-excitation processes at the limit of small separations.
- Published
- 2021