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The decay properties of {sup 290}116 and {sup 291}116, and the dependence of their production cross sections on the excitation energies of the compound nucleus, {sup 293}116, have been measured in the {sup 245}Cm({sup 48}Ca,xn){sup 293-x}116 reaction. These isotopes of element 116 are the decay daughters of element 118 isotopes, which are produced via the {sup 249}Cf+{sup 48}Ca reaction. They performed the element 118 experiment at two projectile energies, corresponding to {sup 297}118 compound nucleus excitation energies of E* = 29.2 {+-} 2.5 and 34.4 {+-} 2.3 MeV. During an irradiation with a total beam dose of 4.1 x 10{sup 19} {sup 48}Ca projectiles, three similar decay chains consisting of two or three consecutive {alpha} decays and terminated by a spontaneous fission (SF) with high total kinetic energy of about 230 MeV were observed. The three decay chains originated from the even-even isotope {sup 294}118 (E{sub {alpha}} = 11.65 {+-} 0.06 MeV, T{sub {alpha}} = 0.89{sub -0.31}{sup +1.07} ms) produced in the 3n-evaporation channel of the {sup 249}Cf+{sup 48}Ca reaction with a maximum cross section of 0.5{sub -0.3}{sup +1.6} pb.

The results of two experiments designed to synthesize element 115 isotopes in the {sup 243}Am+{sup 48}Ca reaction are presented. Two new elements with atomic numbers 113 and 115 were observed for the first time. With 248-MeV {sup 48}Ca projectiles, we observed three similar decay chains consisting of five consecutive {alpha} decays, all detected in a total time interval of 30 s. Each chain was terminated by a spontaneous fission (SF) with a high-energy release and a lifetime of about a day. With 253-MeV {sup 48}Ca projectiles, we registered a different decay chain of consecutive {alpha} decays detected in a time interval of 0.5 s, also terminated by spontaneous fission, but after 1.8 h. The decay properties of the eleven new {alpha}- and SF-decaying nuclei are consistent with expectations for consecutive {alpha} decays originating from the parent isotopes {sup 288}115 and {sup 287}115, produced in the 3n- and 4n-evaporation channels, respectively. Support for the assignment of the atomic numbers of all of the nuclei in the {sup 288}115 decay chain was obtained in an independent experiment in which a long-lived spontaneous fission activity, {sup 268}Db (15 events), was found to be chemically consistent with the fifth group of the periodic table.more » The odd-odd isotope {sup 288}115 was observed with largest cross section of about 4 pb. In the SF decay of {sup 268}Db, a total kinetic energy of 230 MeV and a neutron multiplicity per fission of 4.2 were measured. The decay properties of the 11 new isotopes with Z=105-115 and the production cross sections are in agreement with modern concepts of the role of nuclear shells in the stability of superheavy nuclei. The experiments were carried out at the Flerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research.« less

We have studied the dependence of the production cross sections of the isotopes {sup 282,283}112 and {sup 286,287}114 on the excitation energy of the compound nuclei {sup 286}112 and {sup 290}114. The maximum cross section values of the xn-evaporation channels for the reaction {sup 238}U({sup 48}Ca,xn){sup 286-x}112 were measured to be {sigma}{sub 3n}=2.5{sub -1.1}{sup +1.8} pb and {sigma}{sub 4n}=0.6{sub -0.5}{sup +1.6} pb; for the reaction {sup 242}Pu({sup 48}Ca,xn){sup 290-x}114: {sigma}{sub 2n}{approx}0.5 pb, {sigma}{sub 3n}=3.6{sub -1.7}{sup +3.4} pb, and {sigma}{sub 4n}=4.5{sub -1.9}{sup +3.6} pb. In the reaction {sup 233}U({sup 48}Ca,2-4n){sup 277-279}112 at E*=34.9=2.2 MeV we measured an upper cross section limit of {sigma}{sub xn}{

We have studied the excitation functions of the reactions $^{244}\mathrm{Pu}$($^{48}\mathrm{Ca}$,$xn$). Maximum cross sections for the evaporation of 3--5 neutrons in the complete-fusion reaction $^{244}\mathrm{Pu+}^{48}\mathrm{Ca}$ were measured to be ${\ensuremath{\sigma}}_{3n}=2\phantom{\rule{0.3em}{0ex}}\text{pb}$, ${\ensuremath{\sigma}}_{4n}=5\phantom{\rule{0.3em}{0ex}}\text{pb}$, and ${\ensuremath{\sigma}}_{5n}=1\phantom{\rule{0.3em}{0ex}}\text{pb}$. The decay properties of $3n$-evaporation product $^{289}114$, in the decay chains observed at low $^{48}\mathrm{Ca}$ energy coincide well with those previously observed in the $^{244}\mathrm{Pu+}^{48}\mathrm{Ca}$ and $^{248}\mathrm{Cm+}^{48}\mathrm{Ca}$ reactions and assigned to $^{288}114$. Two isotopes of element 114 and their descendant nuclei were identified for the first time at higher bombarding energies: $^{288}114$ (${E}_{\ensuremath{\alpha}}=9.95\phantom{\rule{0.3em}{0ex}}\text{MeV}$, ${T}_{1∕2}=0.6\phantom{\rule{0.3em}{0ex}}\mathrm{s}$) and $^{287}114$ (${E}_{\ensuremath{\alpha}}=10.04\phantom{\rule{0.3em}{0ex}}\text{MeV}$, ${T}_{1∕2}=1\phantom{\rule{0.3em}{0ex}}\mathrm{s}$). We also report on the observation of new isotopes of element 116, $^{290,291}116$, produced in the $^{245}\mathrm{Cm}+^{48}\mathrm{Ca}$ reaction with cross sections of about $1\phantom{\rule{0.3em}{0ex}}\text{pb}$. A discussion of self-consistent interpretations of all observed decay chains originating at $Z=118$, 116, and 114 is presented.

This paper presents results of experiments aimed at producing long-lived superheavy elements located near the spherical shell closures with Z ≥114 and N ≥172 in the reactions of neutron-rich isotopes 244Pu, 245,248Cm and 249Cf with 48Ca projectiles. The decay properties of the synthesized nuclei are consistent with the consecutive α-decays originating in the decays of parent nuclides 289114, 290,291,293116 and 294118 produced in the 2n and 3n-evaporation channels. The present observations can be considered to be experimental evidence of the existence of the “island of stability” of superheavy elements.

The present paper reports the results of an attempt aimed at the synthesis of element 118 in the reaction {sup 249}Cf({sup 48}Ca,3n){sup 294}118. The experiment was performed employing the Dubna Gas-filled Recoil Separator and the U400 heavy-ion cyclotron at FLNR, JINR, Dubna. In the course of a 2300-hour irradiation of an enriched {sup 249}Cf target (0.23 mg/cm{sup 2}) with a beam of 245-MeV {sup 48}Ca ions, we accumulated a total beam dose of 2.5 x 10{sup 19} ions. We detected two events that may be attributed to the formation and decay of nuclei with Z=118. For one event, we observed a decay chain of two correlated {alpha}-decays with corresponding energies and correlation times of E{sub {alpha}1} = 11.65 {+-} 0.06 MeV, t{sub {alpha}1} = 2.55 ms and E{sub {alpha}2} = 10.71 {+-} 0.17 MeV, t{sub {alpha}2} = 42.1 ms and, finally, a spontaneous fission with the sum of the kinetic energies of the fission fragments E{sub tot} = 207 MeV (TKE {approx} 230 MeV) and t{sub SF} = 0.52 s. In the second event chain, the recoil nucleus decayed into two fission fragments with E{sub tot} = 223 MeV (TKE {approx} 245 MeV) 3.16 ms later, without intervening {alpha} decays.more » The probabilities that these events were caused by the chance correlations of unrelated signals are negligible. Both events were observed at an excitation energy of the compound nucleus {sup 297}118 of E* = 30.0 {+-} 2.4 MeV, close to the expected maximum of the 3n-evaporation channel. The relationship between the decay energy Q{sub {alpha}} and decay period T{sub {alpha}} shows that sequential {alpha}-transitions in the first event correspond to the decay chain with Z = 118{_}116{_}114. Decay characteristics of the newly observed nuclides are compared with radioactive decay properties of the even-even isotopes with Z = 116, 114 and 112 previously produced in the reactions {sup 244}Pu, {sup 248}Cm + {sup 48}Ca and calculations made in various nuclear models.« less

A PC-based data acquisition system for heavy element research is described. Some special electronic modules were designed for the mentioned system. The system was tested for heavy-ion reactions at the main FLNR cyclotron U400. The detection module design is also described. This system was successfully applied in experiments to discover the shell closure at N=162 and Z=108 as well as for the discovery of new elements (two isotopes). A specific point of real-time detection of short recoil-alpha energy-time-position correlations is also presented.

We measured the average electronic charge $〈q〉$ of heavy ions with atomic numbers $Z=89$ through 116 traversing dilute hydrogen gas with velocities ranging from 1 to 2.6 times the Bohr velocity. We observe a strong linear dependence of the average charge on the velocity of the ions, and only a weak dependence on their atomic number Z. A more detailed examination of the experimental results shows that the $〈q〉$ values reflect the influence of the $5f$ electron shell on the properties of these elements.

This paper presents results of the experiments aimed at producing long-lived superheavy elements located near the spherical-shell closures with Z ⩾ 114 and N ⩾ 172 in the 244Pu + 48Ca and 248Cm + 48Ca reactions. The large measured α-particle energies of the newly observed nuclei, together with the long decay times and spontaneous fission terminating the chains, offer evidence of the decay of nuclei with high atomic numbers. The decay properties of the synthesized nuclei are consistent with the consecutive α-decays originating from the parent nuclides 288, 289114 and 292116, produced in the 3n and 4n evaporation channels with cross-sections of about a picobarn. The present observations can be considered as experimental evidence of the existence of the “island of stability” of superheavy elements.

In preparation for recent experiments on the synthesis of superheavy nuclei with $Z=114$ in the reaction ${}^{244}\mathrm{Pu}{+}^{48}\mathrm{Ca},$ we modified the Dubna gas-filled recoil separator and its detection system and carried out bombardments of lead targets with ${}^{48}\mathrm{Ca}$ projectiles. We studied excitation functions of the reactions ${}^{206}\mathrm{Pb}{(}^{48}\mathrm{Ca},1\ensuremath{-}4n)$ and ${}^{204,207,208}\mathrm{Pb}{(}^{48}\mathrm{Ca},2n).$ Maximum cross sections for the evaporation of 1--4 neutrons in the complete fusion reaction ${}^{206}\mathrm{Pb}{+}^{48}\mathrm{Ca}$ were measured to be ${\ensuremath{\sigma}}_{1n}=60 \mathrm{nb},$ ${\ensuremath{\sigma}}_{2n}=500 \mathrm{nb},$ ${\ensuremath{\sigma}}_{3n}=30 \mathrm{nb},$ and ${\ensuremath{\sigma}}_{4n}=0.3 \mathrm{nb}.$ In the bombardment of an enriched ${}^{204}\mathrm{Pb}$ target, we simultaneously obtained excitation functions of the ${}^{204,206,207,208}\mathrm{Pb}{(}^{48}\mathrm{Ca},2n)$ reactions induced on the isotopic admixtures present in the target material. The maximum cross sections for the evaporation of two neutrons from the compound nuclei ${}^{256}\mathrm{No},$ ${}^{255}\mathrm{No},$ and ${}^{252}\mathrm{No}$ were measured to be 2.1 $\ensuremath{\mu}\mathrm{b},$ 1.3 $\ensuremath{\mu}\mathrm{b},$ and 10 nb, respectively. The spontaneously fissioning even-even isotope ${}^{250}\mathrm{No},$ with a half-life ${T}_{1/2}=36 \ensuremath{\mu}\mathrm{s},$ was identified for the first time in this experiment. In the reaction ${}^{207}\mathrm{Pb}{+}^{34}\mathrm{S},$ we measured the excitation function for the production of the 21-ms spontaneously fissioning isotope ${}^{238}\mathrm{Cf},$ confirming our preliminary identification of this nuclide based on the results of cross bombardments.

We present the observation of the first decay event of the new nuclide {sup 292}116 in the running experiment on the synthesis of Z=116 nuclei in the reaction {sup 248}Cm+{sup 48}Ca. The experiment is in progress at FLNR, JINR, Dubna.

In bombardments of ${}^{244}\mathrm{Pu}$ targets with 114- and 120-MeV ${}^{22}\mathrm{Ne}$ projectiles we detected 69 $\ensuremath{\alpha}\ensuremath{-}\ensuremath{\alpha}$ correlations linking $\ensuremath{\alpha}$ decays of ${}^{261}\mathrm{Rf}$ and ${}^{257}\mathrm{No}.$ We observed one $\ensuremath{\alpha}$ peak with ${E}_{\ensuremath{\alpha}}=8.30\ifmmode\pm\else\textpm\fi{}0.06$ MeV for ${}^{261}\mathrm{Rf}$ and peaks with \ensuremath{\alpha}-particle energies 8.07\char21{}8.40 MeV for ${}^{257}\mathrm{No}.$ The half-life of ${}^{257}\mathrm{No}$ was measured to be $25\ifmmode\pm\else\textpm\fi{}3$ s. No correlations were found between $\ensuremath{\alpha}$ decays and subsequent spontaneous fission events, from which we calculated an upper limit of 1.5% for the fission branch of ${}^{257}\mathrm{No}$ and estimated an upper limit of 3% for the \ensuremath{\alpha}-decay branch of ${}^{262}\mathrm{Rf}.$ The cross section of the ${}^{244}\mathrm{Pu}{(}^{22}\mathrm{Ne}{,5n)}^{261}\mathrm{Rf}$ reaction was measured to be about 4 nb at both ${}^{22}\mathrm{Ne}$ energies used. We also report on some results from ${}^{242}\mathrm{Pu}{+}^{22}\mathrm{Ne}$ and ${}^{238}\mathrm{U}{+}^{26}\mathrm{Mg}$ bombardments.

118 s); for the spontaneous fission (T1/257.522.9 114 s), the total energies deposited in the detector array were 213 62 and 221 62 MeV. The decay properties of the synthesized nuclei are consistent with the consecutive a decays originating from the parent even-even nucleus 288 114, produced in the 4n-evaporation channel with a cross section of about 1 pb. 288 114 and 284 112 are the heaviest known a-decaying even-even nuclides, following the production of 260 Sg and 266 Sg (Z5106) and the observation of a decay of 264 Hs (Z5108). The observed radioactive properties of 288 114 and the daughter nuclides match the decay scenario predicted by the macroscopic-microscopic theory.

The reaction 243Am + 48Ca has been reinvestigated to provide new evidence for the discovery of elements 113, 115. Twenty eight new 288115 decay chains were detected in this reaction to increase from three to 31 the number of 288115 atoms observed. In addition, four new decay chains were observed for the first time and assigned to the decay of 289115. These new 289115 events have the same properties for their decay chains as those observed for 289115 populated in the alpha decay of 293117 produced in the 249Bk + 48Ca reaction to provide cross-bombardment evidence. These new high statistics data sets and the cross-bombardment agreement provide definitive evidence for the discoveries of the new elements with Z = 113, 115, 117.

The synthesis of the new chemical element with atomic number Z=117 is presented. The isotopes 293117 and 294117were produced in fusion reactions between 48Ca and 249Bk. The 249Bk was produced in the High Flux Isotope Reactor and chemically separated at Oak Ridge. Decay chains involving eleven new nuclei were identified by means of the Dubna Gas Filled Recoil Separator. The measured decay properties show a strong rise of stability for super-heavy nuclei toward N=184.

Formulation and solution of the problem of the U‐400 cyclotron arc ion source mode control optimization are considered. The optimization criterion is formulated as follows: to get the preset or maximum beam current in a limited range of the discharge and sputtering parameters. The ion source mode control is fulfilled by six input parameters variation. The algorithms of control are realized on the basis of CAMAC crate microprocessor controller and microcomputer compatible with IBM PC/XT/AT.

An automatic control system is described for the multiply charged ion source of the U‐400 cyclotron based on CAMAC apparatus and microprocessor controllers. The system allows the automatic tuning of the ion source to the necessary regime, including the automatic start‐up of discharge, determination of the necessary parameters of sputtering, and the automatic search for a maximum beam current for given discharge parameters. The system performs the tuning of the ion source to the quasioptimal regime in 10–15 min with up to 5% deviation from the preset parameters. It is possible to stabilize the beam current within 3% using the automatic correction of the discharge regime.