Search

We report a compact source of high power, tunable, ultrafast yellow radiation using fourth-harmonic generation of a mid-IR laser in two-stage frequency-doubling processes. Using C r 2+ : Z n S laser at 2360 nm frequency-doubled in a multi-grating MgO:PPLN crystal, we have generated near-IR radiation tunable across 1137-1200 nm with average output power as high as 2.4 W and pulse width of ∼60 f s . Subsequently, the near-IR radiation is frequency-doubled using a bismuth triborate (BIBO) crystal to produce coherent yellow radiation tunable across 570-596 nm with a maximum average power of ∼1 W . The source has a maximum mid-IR to yellow (near-IR to yellow) single-pass conversion efficiency as high as ∼29.4 % (∼47 % ). Without any pulse compression, the yellow source has output pulses at a repetition rate of 80 MHz with a pulse width of ∼130 f s in Gaussian-shaped and a spectral width of ∼4 n m corresponding to a time-bandwidth product of 0.45. The generated output beam has a Gaussian transverse beam profile with measured M 2 values of M x 2∼1.07 and M y 2∼1.01.

We report on a compact and simple ultrafast source producing tunable radiation in the near-IR wavelength range. Based on single-pass frequency doubling of an ultrafast Cr 2+ :ZnS laser at 2360 nm with pulse width of 43 fs at a repetition rate of 80 MHz in MgO:PPLN crystal, the source produces maximum average output power of ∼2.43  W tunable across 1137-1200 nm with a maximum single-pass conversion efficiency as high as 65%. Without use of any pulse compression technique, the source produces output pulses in Gaussian shape with measured pulse width of ∼60  fs and spectral width of 39 nm centered at 1180 nm corresponding to a time-bandwidth product of 0.5. The output beam has a Gaussian spatial profile with measured M 2 <1.32 and a peak-to-peak power fluctuation of 3% over 2 h. Using MgO:PPLN crystal of two different lengths, 1 mm and 2 mm, we have observed that the optimum second-harmonic generation efficiency of an ultrafast pulse laser, even in the presence of temporal walk-off, appears in the low pump focusing condition.

We report on frequency-doubling characteristics of high-power, ultrafast optical vortex beams in a nonlinear medium. Based on single-pass second-harmonic generation (SHG) of optical vortices in 1.2 mm long bismuth triborate (BIBO) crystal, we studied the effect of different parameters influencing the SHG process in generating high-power and higher-order vortices. We observed a decrease in SHG efficiency with the order, which can be attributed to the increase of the vortex beam area with order. Like a Gaussian beam, optical vortices show focusing-dependent conversion efficiency. However, under similar experimental conditions, the optimum focusing condition for optical vortices is reached at tighter focusing with orders. We observed higher angular acceptance bandwidth in the case of optical vortices than that of a Gaussian beam; however, there is no substantial change in angular acceptance bandwidth with vortex order. We also observed that in the frequency-doubling process, the topological charge has negligible or no effect in temporal and spectral properties of the beams. We have generated ultrafast vortices at 532 nm with power as much as 900 mW and order as high as 12. In addition, we have devised a novel scheme based on linear optical elements to double the order of any optical vortex at the same wavelength.

We report on experimental realization of optimum focusing condition for type-I second-harmonic generation (SHG) of high-power, ultrafast laser in "thick" nonlinear crystal. Using single-pass, frequency doubling of a 5 W Yb-fiber laser of pulse width ~260 fs at repetition rate of 78 MHz in a 5-mm-long bismuth triborate (BIBO) crystal we observed that the optimum focusing condition is more dependent on the birefringence of the crystal than its group-velocity mismatch (GVM). A theoretical fit to our experimental results reveals that even in the presence of GVM, the optimum focusing condition matches the theoretical model of Boyd and Kleinman, predicted for continuous-wave and long-pulse SHG. Using a focusing factor of ξ=1.16 close to the estimated optimum value of ξ=1.72 for our experimental conditions, we generated 2.25 W of green radiation of pulse width 176 fs with single-pass conversion efficiency as high as 46.5%. Our study also verifies the effect of pulse narrowing and broadening of angular phase-matching bandwidth of SHG at tighter focusing. This study signifies the advantage of SHG in "thick" crystal in controlling SH-pulse width by changing the focusing lens while accessing high conversion efficiency and broad angular phase-matching bandwidth.