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The temperature and pressure dependence of the partial density of phonon states of iron atoms in superconducting Fe1.01Se was studied by 57Fe nuclear inelastic scattering (NIS). The high energy resolution allows for a detailed observation of spectral properties. A sharpening of the optical phonon modes and shift of all spectral features towards higher energies by ~4% with decreasing temperature from 296 K to 10 K was found. However, no detectable change at the tetragonal - orthorhombic phase transition around 100 K was observed. Application of a pressure of 6.7 GPa, connected with an increase of the superconducting temperature from 8 K to 34 K, results in an increase of the optical phonon mode energies at 296 K by ~12%, and an even more pronounced increase for the lowest-lying transversal acoustic mode. Despite these strong pressure-induced modifications of the phonon-DOS we conclude that the pronounced increase of Tc in Fe1.01Se with pressure cannot be described in the framework of classical electron-phonon coupling. This result suggests the importance of spin fluctuations to the observed superconductivity.

The paper contains a short description of the scientific papers of Professor Boris Ya. Sukharevsky on condensed matter physics. His basic scientific activity was related to following directions: structural vacancies concept; influence of point defects on statics and kinetics of phase transitions; DNA crystallization and low-dimensional systems properties; phase transitions in Jahn-Teller crystals; Thermophysics of superconductors e.a. The list of most essential papers of Prof. B.Ya. Sukharevsky is included., Comment: 16 pages, 53 references

SS433, located at the center of the supernova remnant W50, is a close proximity binary system consisting of a compact star and a normal star. Jets of material are directed outwards from the vicinity of the compact star symmetrically to the east and west. Non-thermal hard X-ray emission is detected from lobes lying on both sides. Shock accelerated electrons are expected to generate sub-TeV gamma rays through the inverse-Compton process in the lobes. Observations of the western X-ray lobe region of SS433/W50 system have been performed to detect sub-TeV gamma-rays using the 10m CANGAROO-II telescope in August and September, 2001, and July and September, 2002. The total observation times are 85.2 hours for ON source, and 80.8 hours for OFF source data. No significant excess of sub-TeV gamma rays has been found at 3 regions of the western X-ray lobe of SS433/W50 system. We have derived 99% confidence level upper limits to the fluxes of gamma rays and have set constraints on the strengths of the magnetic fields assuming the synchrotron/inverse-Compton model for the wide energy range of photon spectrum from radio to TeV. The derived lower limits are 4.3 microgauss for the center of the brightest X-ray emission region and 6.3 microgauss for the far end from SS433 in the western X-ray lobe. In addition, we suggest that the spot-like X-ray emission may provide a major contribution to the hardest X-ray spectrum in the lobe., Comment: 7 pages, 8 figures, to be published in Astroparticle Physics

The properties of the Galactic supernova remnant SN 1006 are theoretically reanalysed. Nonlinear kinetic theory is used to determine the acceleration efficiency of cosmic rays (CRs) in the supernova remnant SN 1006. The known range of astronomical parameters and the existing measurements of nonthermal emission are examined in order to define the values of the relevant physical parameters which determine the CR acceleration efficiency. It is shown that the parameter values -- proton injection rate, electron to proton ratio and downstream magnetic field strength -- are determined with the appropriate accuracy. In particular also the observed azimuthal variations in the gamma-ray morphology agree with the theoretical expectation. These parameter values, together with the reduction of the gamma-ray flux relative to a spherically symmetric acceleration geometry, allow a good fit to the existing data, including the recently detected TeV emission by H.E.S.S. SN 1006 represents the first example where a high efficiency of nuclear CR production, required for the Galactic CR sources, is consistently established., Comment: 10 pages, 6 figures, accepted for publication in A&A

Iron Selenide, Fe1.01Se, the layered parent compound of the recently discovered superconducting arsenide family, has previously been shown to be non magnetic and superconducting with a critical temperature of 8 K. Here we show that copper can be substituted at the iron site in Fe1.01Se up to a solubility limit of 20-30 %, after which a first order transition to the three-dimensional CuFeSe2 structure type is observed. As little as 1.5 % percent copper is sufficient to suppress the superconductivity, and 4 % drives the system through a metal-insulator transition. A local magnetic moment is introduced, which maximizes near 12% doping, where a spin-glass transition near 15 K is observed.

In this letter we show that superconducting Fe1.01Se undergoes a structural transition at 90 K from a tetragonal to an orthorhombic phase but that non-superconducting Fe1.03Se does not. Further, high resolution electron microscopy study at low temperatures reveals an unexpected additional modulation of the crystal structure of the superconducting phase involving displacements of the Fe atoms, and that the non-superconducting material shows a distinct, complex nanometer-scale structural modulation. Finally, we show that magnetism is not the driving force for the phase transition in the superconducting phase., Comment: 5 pages, 5 figures

In this letter, we report that the superconductivity transition temperature in beta-Fe1.01Se increases from 8.5 to 36.7 K under applied pressure of 8.9 GPa. It then decreases at higher pressure. A dramatic change in volume is observed at the same time Tc rises, due to a collapse of the separation between the Fe2Se2 layers. A clear transition to a linear resistivity normal state is seen on cooling at all pressures. No static magnetic ordering is observed for the whole p-T phase diagram. We also report that at higher pressure (starting around 7 GPa and completed at 38 GPa), Fe1.01Se transforms to a hexagonal NiAs-type structure and displays non-magnetic, insulating behavior. The inclusion of electron correlation in band structure caculations is necessary to describe this behavior, signifying that such correlations are important in this chemical system. Our results strongly support unconventional superconductivity in beta-Fe1.01Se., Comment: 17 pages, 4 figures

The recently discovered iron arsenide superconductors, which display superconducting transition temperatures as high as 55 K, appear to share a number of general features with high-Tc cuprates, including proximity to a magnetically ordered state and robustness of the superconductivity in the presence of disorder. Here we show that superconductivity in Fe1+dSe, the parent compound of the superconducting arsenide family, is destroyed by very small changes in stoichiometry. Further, we show that non-superconducting Fe1+dSe is not magnetically ordered down to low temperatures. These results suggest that robust superconductivity and immediate instability against an ordered magnetic state should not be considered as intrinsic characteristics of iron-based superconducting systems, and that Fe1+dSe may present a unique opportunity for determining which materials characteristics are critical to the existence of superconductivity in high Tc iron arsenide superconductors and which are not., Comment: Updated to reflect final version and include journal reference

We theoretically and phenomenologically investigate the question whether the gamma-ray emission from the remnants of the type Ia supernovae SN 1006, Tycho's SN and Kepler's SN can be the result of electron acceleration alone. The observed synchrotron spectra of the three remnants are used to determine the average momentum distribution of nonthermal electrons as a function of the assumed magnetic field strength. Then the inverse Compton emission spectrum in the Cosmic Microwave Background photon field is calculated and compared with the existing upper limits for the very high energy gamma-ray flux from these sources. It is shown that the expected interstellar magnetic fields substantially overpredict even these gamma-ray upper limits. Only rather strongly amplified magnetic fields could be compatible with such low gamma-ray fluxes. However this would require a strong component of accelerated nuclear particles whose energy density substantially exceeds that of the synchrotron electrons, compatible with existing theoretical acceleration models for nuclear particles and electrons. Even though the quantitative arguments are simplistic, they appear to eliminate simplistic phenomenological claims in favor of a inverse Compton gamma-ray scenario for these sources., Comment: 6 pages, 1 figure, accepted for publication in Astronomy and Astrophysics

The consequences of a newly suggested value for the SN explosion energy 1.2x10^{51} erg are explored for the case of Tycho's supernova remnant (SNR). A nonlinear kinetic theory of cosmic ray (CR) acceleration in SNRs is employed to investigate the properties of Tycho's SNR and their correspondence to the existing experimental data. It is demonstrated that the large mean ratio between the radii of the contact discontinuity and the forward shock is consistent with the very effective acceleration of nuclear energetic particles at the forward shock. It is also argued that consistency of the value E_{sn} = 1.2x10^{51} erg with the gas dynamics, acceleration theory, and the existing gamma-ray measurements requires the source distance to be greater than 3.3 kpc. The corresponding ambient gas number density is lower than 0.4 cm^{-3}. Since the expected gamma-ray flux strongly depends on the source distance, F_{\gamma}\propto d^{-7}, a future experimental determination of the actual gamma-ray flux from Tycho's SNR will make it possible to determine the values of the source distance and of the mean ambient gas density. A simple inverse Compton model without a dominant population of nuclear CRs is not compatible with the present upper limit for the gamma-ray emission for any reasonable ambient interstellar B-field. Given the consistency between acceleration theory and overall, as well as internal, gas dynamics, a future gamma-ray detection would make the case for nuclear particle acceleration in Tycho's SNR incontrovertible in our view., Comment: 8 pages, 4 figures, Accepted for publication in A&A

To explore its structural and magnetic properties, the Heusler compound Co2Cr0.6Fe0.4Al was investigated using Moessbauer spectroscopy. The results of both transmission and conversion electron Moessbauer spectroscopy (CEMS) are analyzed to obtain insight into both the disorder effects as well as the differences between bulk and surface properties. It was found that mechanical treatment of the surfaces of bulk samples causes disorder and phase segregation, effects that should be taken into consideration when performing studies using surface-informative techniques. Results from bulk sample CEMS measurements of Co2Cr0.6Fe0.4Al are used to interpret the thin film Moessbauer spectra of this compound.

Polycrystalline samples of the half-metallic ferromagnet Heusler compound Co$_2$TiSn have been prepared and studied using bulk techniques (X-ray diffraction and magnetization) as well as local probes ($^{119}$Sn M\"ossbauer spectroscopy and $^{59}$Co nuclear magnetic resonance spectroscopy) in order to determine how disorder affects half-metallic behavior and also, to establish the joint use of M\"ossbauer and NMR spectroscopies as a quantitative probe of local ion ordering in these compounds. Additionally, density functional electronic structure calculations on ordered and partially disordered Co$_2$TiSn compounds have been carried out at a number of different levels of theory in order to simultaneously understand how the particular choice of DFT scheme as well as disorder affect the computed magnetization. Our studies suggest that a sample which seems well-ordered by X-ray diffraction and magnetization measurements can possess up to 10% of antisite (Co/Ti) disordering. Computations similarly suggest that even 12.5% antisite Co/Ti disorder does not destroy the half-metallic character of this material. However, the use of an appropriate level of non-local DFT is crucial., Comment: 11 pages and 5 figures

A nonlinear kinetic theory of cosmic ray (CR) acceleration in supernova remnants is employed to investigate the properties of the remnant SN 1987A. It is shown that a large downstream magnetic field ~10 mG is required to fit the existing observational data. Such a strong field together with the strong shock modification due to CR backreaction provides the steep and concave radioemission spectrum and considerable synchrotron cooling of high energy electrons which diminish their X-ray synchrotron flux below the observed Chandra flux which has to be considered as an upper limit for nonthermal X-ray emission. The expected gamma-ray energy flux at TeV-energies at the current epoch is 2x10^{-13} erg/(cm^2 s)., Comment: 12 pages, 4 figures, accepted for publication in ApJ Letters

Nonlinear kinetic theory of cosmic ray (CR) acceleration in supernova remnants (SNRs) is used to investigate the properties of Kepler's SNR and, in particular, to predict the gamma-ray spectrum expected from this SNR. Observations of the nonthermal radio and X-ray emission spectra as well as theoretical constraints for the total supernova (SN) explosion energy E_sn are used to constrain the astronomical and particle acceleration parameters of the system. Under the assumption that Kepler's SN is a type Ia SN we determine for any given explosion energy E_sn and source distance d the mass density of the ambient interstellar medium (ISM) from a fit to the observed SNR size and expansion speed. This makes it possible to make predictions for the expected gamma-ray flux. Exploring the expected distance range we find that for a typical explosion energy E_sn=10^51 erg the expected energy flux of TeV gamma-rays varies from 2x10^{-11} to 10^{-13} erg/(cm^2 s) when the distance changes from d=3.4 kpc to 7 kpc. In all cases the gamma-ray emission is dominated by \pi^0-decay gamma-rays due to nuclear CRs. Therefore Kepler's SNR represents a very promising target for instruments like H.E.S.S., CANGAROO and GLAST. A non-detection of gamma-rays would mean that the actual source distance is larger than 7 kpc., Comment: 6 pages, 4 figures. Accepted for publication in Astronomy and Astrophysics, minor typos corrected

For the case of Tycho's supernova remnant (SNR) we present the relation between the blast wave and contact discontinuity radii calculated within the nonlinear kinetic theory of cosmic ray (CR) acceleration in SNRs. It is demonstrated that these radii are confirmed by recently published Chandra measurements which show that the observed contact discontinuity radius is so close to the shock radius that it can only be explained by efficient CR acceleration which in turn makes the medium more compressible. Together with the recently determined new value $E_{sn}=1.2\times 10^{51}$ erg of the SN explosion energy this also confirms our previous conclusion that a TeV gamma-ray flux of $(2-5)\times 10^{-13}$ erg/(cm$^2$s) is to be expected from Tycho's SNR. Chandra measurements and the HEGRA upper limit of the TeV gamma-ray flux together limit the source distance $d$ to $3.3\leq d\leq 4$ kpc., Comment: 5 pages, 4 figures. Accepted for publication in Astrophysics and Space Science, Proc. of "The Multi-Messenger Approach to High-Energy Gamma-ray Sources (Third Workshop on the Nature of Unidentified High-Energy Sources)", Barcelona, July 4-7, 2006

This work reports on structural and magnetic investigations of the Heusler compound Co$_2$FeSi. X-Ray diffraction and M\"o\ss bauer spectrometry indicate an ordered $L2_1$ structure. Magnetic measurements by means of X-ray magnetic circular dichroism and magnetometry revealed that this compound is, currently, the material with the highest magnetic moment ($6 \mu_B$) and Curie-temperature (1100K) in the classes of Heusler compounds as well as half-metallic ferromagnets.

Co$_2$FeSi crystallizes in the ordered L2$_1$ structure as proved by X-ray diffraction and M\"o\ss bauer spectroscopy. The magnetic moment of Co$_2$FeSi was measured to be about $6\mu_B$ at 5K. Magnetic circular dichroism spectra excited by soft X-rays (XMCD) were taken to determine the element specific magnetic moments of Co and Fe. The Curie temperature was measured with different methods to be ($1100\pm20$)K. Co$_2$FeSi was found to be the Heusler compound as well as the half-metallic ferromagnet with the highest magnetic moment and Curie temperature., Comment: conference contribution, MMM2005

We use nonlinear kinetic theory to study the remnant dynamics and the particle acceleration as well as the properties of the nonthermal emission from the supernova remnant SN 1006. The known range of astronomical parameters is examined to determine whether it encompasses the existing synchrotron emission data. Given the present-day spatial extent and expansion rate of the object, it is shown that the hadronic gamma-ray flux is very sensitive to the ambient gas density N_H and that the existing H.E.S.S. upper limit requires N_H < 0.1 cm^{-3}. The strength of the amplified magnetic field downstream of the shock is about 150 \mu G., Comment: 10 pages, 8 figures, to be published in Astronomy and Astrophysics

In this work a simple concept was used for a systematic search for new materials with high spin polarization. It is based on two semi-empirical models. Firstly, the Slater-Pauling rule was used for estimation of the magnetic moment. This model is well supported by electronic structure calculations. The second model was found particularly for Co$_2$ based Heusler compounds when comparing their magnetic properties. It turned out that these compounds exhibit seemingly a linear dependence of the Curie temperature as function of the magnetic moment. Stimulated by these models, Co$_2$FeSi was revisited. The compound was investigated in detail concerning its geometrical and magnetic structure by means of X-ray diffraction, X-ray absorption and M\"o\ss bauer spectroscopies as well as high and low temperature magnetometry. The measurements revealed that it is, currently, the material with the highest magnetic moment ($6\mu_B$) and Curie-temperature (1100K) in the classes of Heusler compounds as well as half-metallic ferromagnets. The experimental findings are supported by detailed electronic structure calculations.