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We report on the initial analysis of Herschel/HIFI carbon monoxide (CO) observations of the Martian atmosphere performed between 11 and 16 April 2010. We selected the (7-6) rotational transitions of the isotopes ^{13}CO at 771 GHz and C^{18}O at 768 GHz in order to retrieve the mean vertical profile of temperature and the mean volume mixing ratio of carbon monoxide. The derived temperature profile agrees within less than 5 K with general circulation model (GCM) predictions up to an altitude of 45 km, however, show about 12-15 K lower values at 60 km. The CO mixing ratio was determined as 980 \pm 150 ppm, in agreement with the 900 ppm derived from Herschel/SPIRE observations in November 2009., Comment: Accepted for publication in Astronomy and Astrophysics (special issue on HIFI first results); minor changes to match published version

The high spectral resolution and sensitivity of Herschel/HIFI allows for the detection of multiple rotational water lines and accurate determinations of water production rates in comets. In this letter we present HIFI observations of the fundamental 110-101 (557 GHz) ortho and 111-000 (1113 GHz) para rotational transitions of water in comet 81P/Wild 2 acquired in February 2010. We mapped the extent of the water line emission with five point scans. Line profiles are computed using excitation models which include excitation by collisions with electrons and neutrals and solar infrared radiation. We derive a mean water production rate of $1.0 \times 10^{28}$ molecules s$^{-1}$ at a heliocentric distance of 1.61 AU about 20 days before perihelion, in agreement with production rates measured from the ground using observations of the 18-cm OH lines. Furthermore, we constrain the electron density profile and gas kinetic temperature, and estimate the coma expansion velocity by fitting the water line shapes., Comment: Accepted for publication in A&A (special issue on HIFI first results)

We report on the initial analysis of a Herschel/PACS full range spectrum of Neptune, covering the 51-220 micrometer range with a mean resolving power of ~ 3000, and complemented by a dedicated observation of CH4 at 120 micrometers. Numerous spectral features due to HD (R(0) and R(1)), H2O, CH4, and CO are present, but so far no new species have been found. Our results indicate that (i) Neptune's mean thermal profile is warmer by ~ 3 K than inferred from the Voyager radio-occultation; (ii) the D/H mixing ratio is (4.5+/-1) X 10**-5, confirming the enrichment of Neptune in deuterium over the protosolar value (~ 2.1 X 10**-5); (iii) the CH4 mixing ratio in the mid stratosphere is (1.5+/-0.2) X 10**-3, and CH4 appears to decrease in the lower stratosphere at a rate consistent with local saturation, in agreement with the scenario of CH4 stratospheric injection from Neptune's warm south polar region; (iv) the H2O stratospheric column is (2.1+/-0.5) X 10**14 cm-2 but its vertical distribution is still to be determined, so the H2O external flux remains uncertain by over an order of magnitude; and (v) the CO stratospheric abundance is about twice the tropospheric value, confirming the dual origin of CO suspected from ground-based millimeter/submillimeter observations., Comment: Accepted for publication in Astronomy & Astrophysics (special issue on Herschel first results)

We report on an initial analysis of Herschel/HIFI observations of hydrogen chloride (HCl), hydrogen peroxide (H_2O_2), and molecular oxygen (O_2) in the Martian atmosphere performed on 13 and 16 April 2010 (L_s ~ 77{\deg}). We derived a constant volume mixing ratio of 1400 +/- 120 ppm for O_2 and determined upper limits of 200 ppt for HCl and 2 ppb for H_2O_2. Radiative transfer model calculations indicate that the vertical profile of O_2 may not be constant. Photochemical models determine the lowest values of H_2O_2 to be around L_s ~ 75{\deg} but overestimate the volume mixing ratio compared to our measurements., Comment: Accepted for publication in Astronomy and Astrophysics (special issue on HIFI first results); minor changes to match published version

High-resolution far-infrared and sub-millimetre spectroscopy of water lines is an important tool to understand the physical and chemical properties of cometary atmospheres. We present observations of several rotational ortho- and para-water transitions in comet C/2008 Q3 (Garradd) performed with HIFI on Herschel. These observations have provided the first detection of the 2_{12}-1_{01} (1669 GHz) ortho and 1_{11}-0_{00} (1113 GHz) para transitions of water in a cometary spectrum. In addition, the ground-state transition 1_{10}-1_{01} at 557 GHz is detected and mapped. By detecting several water lines quasi-simultaneously and mapping their emission we can constrain the excitation parameters in the coma. Synthetic line profiles are computed using excitation models which include excitation by collisions, solar infrared radiation, and radiation trapping. We obtain the gas kinetic temperature, constrain the electron density profile, and estimate the coma expansion velocity by analyzing the map and line shapes. We derive water production rates of 1.7-2.8 x 10^{28} s^{-1} over the range r_h = 1.83-1.85 AU., Comment: 7 figures, v2: minor changes, updated version of arXiv:1005.2969v1. Accepted for publication in Astronomy and Astrophysics, Herschel special issue on Herschel First Science Results

Comet C/2006 W3 (Christensen) was observed in November 2009 at 3.3 AU from the Sun with Herschel. The PACS instrument acquired images of the dust coma in 70- and 160-micrometers filters, and spectra covering several H2O rotational lines. Spectra in the range 450-1550 GHz were acquired with SPIRE. The comet emission continuum from 70 to 672 micrometers was measured, but no lines were detected. The spectral energy distribution indicates thermal emission from large particles and provides a measure of the size distribution index and dust production rate. The upper limit to the water production rate is compared to the production rates of other species (CO, CH3OH, HCN, H2S, OH) measured with the IRAM 30-m and Nancay telescopes. The coma is found to be strongly enriched in species more volatile than water, in comparison to comets observed closer to the Sun. The CO to H2O production rate ratio exceeds 220%. The dust to gas production rate ratio is on the order of 1., Comment: Accepted for publication in Astronomy & Astrophysics (special issue on Herschel first results)

Based on long-slit infrared spectroscopic observations, it has been suggested that half of the carbon monoxide present in the atmosphere of comet C/1995 O1 (Hale-Bopp) close to perihelion was released by a distributed source in the coma, whose nature (dust or gas) remains unidentified. We re-assess the origin of CO in Hale-Bopp's coma from millimeter interferometric data and a re-analysis of the IR lines. Simultaneous observations of the CO J(1-0) (115 GHz) and J(2-1) (230 GHz) lines were undertaken with the IRAM interferometer in single-dish and interferometric modes. The diversity of angular resolutions (from 1700 to 42000 km diameter at the comet) is suitable to study the radial distribution of CO and detect the extended source observed in the infrared. We used excitation and radiative transfer models to simulate the observations. Various CO density distributions were considered, including 3D time-dependent hydrodynamical simulations which reproduce a CO rotating jet. The CO J(1-0) and J(2-1) observations can be consistently explained by a nuclear production of CO. Composite 50:50 nuclear/extended productions with characteristic scale lengths of CO parent L_p > 1500 km are rejected. Based on similar radiation transfer calculations, we show that the CO v = 1-0 ro-vibrational lines observed in comet Hale-Bopp at heliocentric distances less than 1.5 AU are severely optically thick. The broad extent of the CO brightness distribution in the infrared is mainly due to optical depth effects. Additional factors can be found in the complex structure of the CO coma, and non-ideal slit positioning caused by the anisotropy of dust IR emission. We conclude that both CO millimeter and infrared lines do not provide compelling evidence for a distributed source of CO in Hale-Bopp's atmosphere., Comment: Accepted for publication in Icarus (55 pages, 13 figures)

Observations of the CO J(1-0) 115 GHz and J(2-1) 230 GHz lines in comet C/1995 O1 (Hale-Bopp) were performed with the IRAM Plateau de Bure interferometer on 11 March, 1997. The observations were conducted in both single-dish (ON-OFF) and interferometric modes with 0.13 km s-1 spectral resolution. Images of CO emission with 1.7 to 3" angular resolution were obtained. The ON-OFF and interferometric spectra show a velocity shift with sinusoidal time variations related to the Hale-Bopp nucleus rotation of 11.35 h. The peak position of the CO images moves perpendicularly to the spin axis direction in the plane of the sky. This suggests the presence of a CO jet, which is active night and day at about the same extent, and is spiralling with nucleus rotation. The high quality of the data allows us to constrain the characteristics of this CO jet. We have developed a 3-D model to interpret the temporal evolution of CO spectra and maps. The CO coma is represented as the combination of an isotropic distribution and a spiralling gas jet, both of nucleus origin. Spectra and visibilities (the direct output of interferometric data) analysis shows that the CO jet comprises ~40% the total CO production and is located at a latitude ~20 degrees North on the nucleus surface. Our inability to reproduce all observational characteristics shows that the real structure of the CO coma is more complex than assumed, especially in the first thousand kilometres from the nucleus. The presence of another moving CO structure, faint but compact and possibly created by an outburst, is identified., Comment: 20 pages, 26 figures. Accepted for publication in Astronomy & Astrophysics

A fundamental question in cometary science is whether the different dynamical classes of comets have different chemical compositions, which would reflect different initial conditions. From the ground or Earth orbit, radio and infrared spectroscopic observations of a now significant sample of comets indeed reveal deep differences in the relative abundances of cometary ices. However, no obvious correlation with dynamical classes is found. Further results come, or are expected, from space exploration. Such investigations, by nature limited to a small number of objects, are unfortunately focussed on short-period comets (mainly Jupiter-family). But these in situ studies provide "ground truth" for remote sensing. We discuss the chemical differences in comets from our database of spectroscopic radio observations, which has been recently enriched by several Jupiter-family and Halley-type comets., Comment: In press in Earth, Moon and Planets (proceedings of the workshop "Future Ground-based Solar System Research: Synergies with Space Probes and Space Telescopes", Portoferraio, Isola d'Elba, Livorno (Italy), 8-12 September 2008). 6 pages with 2 figures

In 2005, as part of a world-wide multi-wavelength investigation of comet 9P/Tempel 1 in support to the Deep Impact mission, we conducted radio spectroscopic observations with the Nançay radio telescope, the Odin satellite, the CSO 10-m and the IRAM 30-m telescopes. We report here our results concerning the chemical composition of the comet. The relative abundances of the detected species (H₂O, CH₃OH, H₂S, HCN) or their upper limits (CO, H₂CO, CS) are comparable to the mean values observed in other comets. No significant changes of the outgassing rates (except possibly for CH₃OH) or of the molecular abundances were observed following the impact.

Radio observations from decimetric to submillimetric wavelengths are now a basic tool for the investigation of comets. Spectroscopic observations allow us i) to monitor the gas production rate of the comets, by directly observing the water molecule, or by observing secondary products (e.g., the OH radical) or minor species (e.g., HCN); ii) to investigate the chemical composition of comets; iii) to probe the physical conditions of cometary atmospheres: kinetic temperature and expansion velocity. Continuum observations probe large-size dust particles and (for the largest objects) cometary nuclei. Comets are classified from their orbital characteristics into two separate classes: i) nearly-isotropic, mainly long-period comets and ii) ecliptic, short-period comets, the so-called Jupiter-family comets. These two classes apparently come from two different reservoirs, respectively the Oort cloud and the trans-Neptunian scattered disc. Due to their different history and - possibly - their different origin, they may have different chemical and physical properties that are worth being investigated. The present article reviews the contribution of radio observations to our knowledge of the Jupiter-family comets (JFCs). The difficulty of such a study is the commonly low gas and dust productions of these comets. Long-period, nearly-isotropic comets from the Oort cloud are better known from Earth-based observations. On the other hand, Jupiter-family comets are more easily accessed by space missions. However, unique opportunities to observe Jupiter-family comets are offered when these objects come by chance close to the Earth. About a dozen JFCs were successfully observed by radio techniques up to now. No obvious evidence for different properties between JFCs and other families of comets is found., Comment: Accepted for publication in Planetary and Space Science (special issue on Jupiter-family comets). 18 pages including 12 figures and 7 tables

From millimeter and optical observations of the Jupiter-family comet 17P/Holmes performed soon after its huge outburst of October 24, 2007, we derive 14 N/15N = 139 +/- 26 in HCN, and 14N/15N = 165 +/- 40 in CN, establishing that HCN has the same non-terrestrial isotopic composition as CN. The same conclusion is obtained for the long-period comet C/1995 O1 (Hale-Bopp) after a reanalysis of previously published measurements. These results are compatible with HCN being the prime parent of CN in cometary atmospheres. The 15N excess relative to the Earth atmospheric value indicates that N-bearing volatiles in the solar nebula underwent important N isotopic fractionation at some stage of Solar System formation. HCN molecules never isotopically equilibrated with the main nitrogen reservoir in the solar nebula before being incorporated in Oort-cloud and Kuiper-belt comets. The 12C/13C ratios in HCN and CN are measured to be consistent with the terrestrial value., Comment: Accepted for publication in the Astrophysical Journal (Letters) 4 pages

We present a sensitive 3 sigma upper limit of 1.1% for the HNC/HCN abundance ratio in comet 73P/SchwassmannWachmann (fragment B), obtained on 2006 May 10-11, using Caltech Submillimeter Observatory (CSO). This limit is a factor of ~7 lower than the values measured previously in moderately active comets at 1 AU from the Sun. Comet 73P/Schwassmann-Wachmann was depleted in most volatile species, except of HCN. The low HNC/HCN ratio thus argues against HNC production from polymers produced from HCN. However, thermal degradation of macromolecules, or polymers, produced from ammonia and carbon compounds, such as acetylene, methane, or ethane appears a plausible explanation for the observed variations of the HNC/HCN ratio in moderately active comets, including the very low ratio in comet 73P/Schwassmann-Wachmann reported here. Similar polymers have been invoked previously to explain anomalous N-14/N-15 ratios measured in cometary CN.

We retrieve the H_2O expansion velocity in a number of comets, using the 18-cm line shapes of the OH radical observed with the Nan\c{c}ay radio telescope. The H_2O velocity is derived from the large base of a trapezium fitted to the observed spectra. This method, which was previously applied to 9 comets, is now extended to 30 further comets. This allows us to study the evolution of their water molecule outflow velocity over a large range of heliocentric distances and gas production rates. Our analysis confirms and extends previous analyses. The retrieved expansion velocities increases with increasing gas production rates and decreasing heliocentric distances. Heuristic laws are proposed, which could be used for the interpretation of observations of cometary molecules and as a touchstone for hydrodynamical models. The expansion velocities retrieved from 18 cm line shapes are larger than those obtained from millimetric observations of parent molecules with smaller fields of view, which demonstrates the acceleration of the gas with cometocentric distance. Our results are in reasonable quantitative agreement with current hydrodynamical models of cometary atmospheres., Comment: Accepted for publication in Astronomy & Astrophysics

We present observations of rotational lines of H2S, SO and CS performed in comet C/1995 O1 (Hale-Bopp) in March 1997 with the Plateau de Bure interferometer (IRAM). The observations provide informations on the spatial and velocity distributions of these molecules. They can be used to constrain their photodissociation rate and their origin. We use a radiative transfer code which allows us to compute synthetic line profiles and interferometric maps, to be compared to the observations. Both single-dish spectra and interferometric spectral maps show a day/night asymmetry in the outgassing. From the analysis of the spectral maps, including the astrometry, we show that SO and CS present in addition a jet-like structure that may be the gaseous counterpart of the dust high-latitude jet observed in optical images. A CS rotating jet is also observed. Using the astrometry provided by continuum radio maps obtained in parallel, we conclude that there is no need to invoke of nongravitational forces acting on this comet, and provide an updated orbit. The radial extension of H2S is found to be consistent with direct release from the nucleus. SO displays an extended radial distribution. Assuming that SO2 is the parent of SO, the photodissociation rate of SO is measured to be 1.5 E-4 s-1 at 1 AU from the Sun. This is lower than most laboratory-based estimates and may suggest that SO is not solely produced by SO2 photolysis. From the observations of J(2-1) and J(5-4) CS lines, we deduce a CS photodissociation rate of 1 to 5 E-5 s-1. The photodissociation rate of CS2, the likely parent of CS, cannot be constrained due to insufficient resolution, but our data are consistent with published values. These observations illustrate the cometary science that will be performed with the future ALMA interferometer., Comment: Accepted for publication in Astronomy & Astrophysics

Comet 9P/Tempel 1 was the target of a multi-wavelength worldwide investigation in 2005. The NASA Deep Impact mission reached the comet on 4.24 July 2005, delivering a 370 kg impactor which hit the comet at 10.3 km/s. Following this impact, a cloud of gas and dust was excavated from the comet nucleus. The comet was observed in 2005 prior to and after the impact, at 18-cm wavelength with the Nan\c{c}ay radio telescope, in the millimetre range with the IRAM and CSO radio telescopes, and at 557 GHz with the Odin satellite. Post-impact observations at IRAM and CSO did not reveal a significant change of the outgassing rates and relative abundances, with the exception of CH_3OH which may have been more abundant by up to one order of magnitude in the ejecta. Most other variations are linked to the intrinsic variability of the comet. The Odin satellite monitored nearly continuously the H_2O line at 557 GHz during the 38 hours following the impact on the 4th of July, in addition to weekly monitoring. Once the periodic variations related to the nucleus rotation are removed, a small increase of outgassing related to the impact is present, which corresponds to the release of \approx 5000+/-2000 tons of water. Two other bursts of activity, also observed at other wavelengths, were seen on 23 June and 7 July; they correspond to even larger releases of gas., Comment: accepted for publication in Icarus

The Odin satellite, launched in Feb. 2001, is equipped with a 1.1-m submillimetre telescope. Odin was used to observe the 557 GHz line of water with high spectral resolution in 12 comets between 2001 and 2005. Line shapes and spatial mapping provide information on the anisotropy of the outgassing and constraints on water excitation, enabling accurate measurements of the water production rate. Five comets were regularly observed over periods of more than one month to monitor the variation of their water outgassing rate with heliocentric distance. Observing campaigns have been generally coordinated with ground-based observations of molecular lines at Nan\c{c}ay, CSO or IRAM 30-m telescopes to obtain molecular abundances relative to water. Thanks to Odin's frequency coverage, it was also possible to detect the H_2^18O 548GHz line, first in comet 153P/Ikeya-Zhang in April 2002 (Lecacheux et al., 2003) and then in comets C/2002 T7 (LINEAR), C/2001 Q4 (NEAT) and C/2004 Q2 (Machholz). The ^16O/^18O isotopic ratio (\approx450) is consistent with the terrestrial value. Ammonia has been searched for in three comets through its J_K = 1_0-0_0 line at 572 GHz and was tentatively detected in C/2001 Q4 and C/2002 T7. The derived abundances of NH_3 relative to water are 0.5 % and 0.3 %, respectively, similar to values obtained in other comets with different techniques., Comment: accepted for publication in Planetary and Space Science