151. Radiative neutron capture on $^{242}\mathrm{Pu}$ in the resonance region at the CERN n_TOF-EAR1 facility
- Author
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Lerendegui-Marco, J., Guerrero, C., Mendoza, E., Quesada, J.M., Eberhardt, K., Junghans, A.R., Krtička, M., Aberle, O., Andrzejewski, J., Audouin, L., Bécares, V., Bacak, M., Balibrea, J., Barbagallo, M., Barros, S., Bečvář, F., Beinrucker, C., Berthoumieux, E., Billowes, J., Bosnar, D., Brugger, M., Caamaño, M., Calviño, F., Calviani, M., Cano-Ott, D., Cardella, R., Casanovas, A., Castelluccio, D.M., Cerutti, F., Chen, Y.H., Chiaveri, E., Colonna, N., Cortés, G., Cortés-Giraldo, M.A., Cosentino, L., Damone, L.A., Diakaki, M., Dietz, M., Domingo-Pardo, C., Dressler, R., Dupont, E., Durán, I., Fernández-Domínguez, B., Ferrari, A., Ferreira, P., Finocchiaro, P., Furman, V., Göbel, K., García, A.R., Gawlik, A., Glodariu, T., Gonçalves, I.F., González-Romero, E., Goverdovski, A., Griesmayer, E., Gunsing, F., Harada, H., Heftrich, T., Heinitz, S., Heyse, J., Jenkins, D.G., Jericha, E., Käppeler, F., Kadi, Y., Katabuchi, T., Kavrigin, P., Ketlerov, V., Khryachkov, V., Kimura, A., Kivel, N., Kokkoris, M., Leal-Cidoncha, E., Lederer, C., Leeb, H., Lo Meo, S., Lonsdale, S.J., Losito, R., Macina, D., Marganiec, J., Martínez, T., Massimi, C., Mastinu, P., Mastromarco, M., Matteucci, F., Maugeri, E.a., Mengoni, A., Milazzo, P.M., Mingrone, F., Mirea, M., Montesano, S., Musumarra, A., Nolte, R., Oprea, A., Patronis, N., Pavlik, A., Perkowski, J., Porras, J.I., Praena, J., Rajeev, K., Rauscher, T., Reifarth, R., Riego-Perez, A., Rout, P.C., Rubbia, C., Ryan, J.A., Sabaté-Gilarte, M., Saxena, A., Schillebeeckx, P., Schmidt, S., Schumann, D., Sedyshev, P., Smith, A.G., Stamatopoulos, A., Tagliente, G., Tain, J.L., Tarifeño-Saldivia, A., Tassan-Got, L., Tsinganis, A., Valenta, S., Vannini, G., Variale, V., Vaz, P., Ventura, A., Vlachoudis, V., Vlastou, R., Wallner, A., Warren, S., Weigand, M., Weiss, C., Wolf, C., Woods, P.J., Wright, T., Žugec, P., Institut de Physique Nucléaire d'Orsay (IPNO), Centre National de la Recherche Scientifique (CNRS)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Sud - Paris 11 (UP11), Institut de Recherches sur les lois Fondamentales de l'Univers (IRFU), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay, n_TOF, and Université Paris-Sud - Paris 11 (UP11)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS)
- Subjects
Nuclear Physics - Experiment ,[PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex] - Abstract
International audience; The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of $^{242}$Pu there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on $^{242}$Pu carried out at n_TOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The $^{242}$Pu(n,$\gamma$) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C$_6$D$_6$ detectors and applying the total energy detection technique. The high neutron energy resolution of n_TOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA.
- Published
- 2018