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Driven by applications in information technology, the search for new materials with stable, long-range magnetic ordering continues. Metalorganic magnets, involving the coordination of metal atoms with specific organic ligands, are a focus of intense research. These magnets offer customizable properties through synthetic adjustments to ligands or coordination chemistry. Here the synthesis, structural characterization, and magnetic properties of the 2D cyanocarbon magnet NiTCNE is reported. 2D-crystalline domains of this single-layered metalorganic network reach sizes exceeding 30 nanometers through co-deposition of the ligand TCNE (tetracyanoethylene) and Ni atoms on an Au(111) surface under ultrahigh vacuum conditions. Non-contact atomic force microscopy visualizes the structure with atomic resolution. X-ray magnetic circular dichroism establishes the 2D NiTCNE as a ferromagnet, with a very high magnetic remanence, a coercive field of around 1 tesla and a Curie temperature between 10 and 20 kelvin. As metalorganic chemistry opens a large variety of routes of synthesis, we anticipate that this materials research paves the way to new magnetic nanomaterials for spintronics applications.

Triboelectricity, when rubbing or contacting materials causes electric charge transfer, is ubiquitous across many fields, and has been studied in detail for centuries. Despite this, a complete description of triboelectricity remains elusive. Here, we analyze the contact between a metal asperity and a semiconductor, including contributions from the depletion zone of the semiconductor and from flexoelectric polarization that arises due to the strain gradients at asperity contacts. The free charges involved in charge transfer are then discussed and calculated. As a result, we develop a quantitative model for triboelectric charge transfer that details how charge transfer scales with contact parameters, the relative influence of depletion and flexoelectricity, and which agrees with various trends in multiple classes of triboelectric experiments.

We present a novel approach to the 3D sound source localization task for distributed ad-hoc microphone arrays by formulating it as a set-to-set regression problem. By training a multi-modal masked autoencoder model that operates on audio recordings and microphone coordinates, we show that such a formulation allows for accurate localization of the sound source, by reconstructing coordinates masked in the input. Our approach is flexible in the sense that a single model can be used with an arbitrary number of microphones, even when a subset of audio recordings and microphone coordinates are missing. We test our method on simulated and real-world recordings of music and speech in indoor environments, and demonstrate competitive performance compared to both classical and other learning based localization methods., Comment: IPIN 2024

We show that the Fr\'echet--Lie groups of the form $C^{\infty}(M)\rtimes \mathbb{R}$ resulting from smooth flows on compact manifolds $M$ fail to be locally exponential in several cases: when at least one non-periodic orbit is locally closed, or when the flow restricts to a linear one on an orbit closure diffeomorphic to a torus. As an application, we prove that the Bondi--Metzner--Sachs group of symmetries of an asymptotically flat space-time is not locally exponential., Comment: 26 pages, v2: Major revision, corrected a mistake in earlier version. Main results are still valid but were substantially expanded. New coauthor joined. v3: Corrected typos

Optically active solid-state spin systems play an important role in quantum technologies. We introduce a new readout scheme, termed Time to Space (T2S) encoding which decouples spin manipulation from optical readout both temporally and spatially. This is achieved by controlling the spin state within a region of interest, followed by rapid scanning of the optical readout position using an acousto-optic modulator. Time tracking allows the optical readout position to be encoded as a function of time. Using nitrogen-vacancy (NV) center ensembles in diamond, we first demonstrate that the T2S scheme enables correlated experiments for efficient common mode noise cancellation in various nano- and microscale sensing scenarios. In the second example, we show highly scalable multi-pixel imaging that does not require a camera and has the potential to accelerate data acquisition by several hundred times compared to conventional scanning methods. We anticipate widespread adoption of this technique, as it requires no additional components beyond those commonly used in optically addressable spin systems.

In this paper, we introduce a temporal logic-based safety filter for Autonomous Intersection Management (AIM), an emerging infrastructure technology for connected vehicles to coordinate traffic flow through intersections. Despite substantial work on AIM systems, the balance between intersection safety and efficiency persists as a significant challenge. Building on recent developments in formal methods that now have become computationally feasible for AIM applications, we introduce an approach that starts with a temporal logic specification for the intersection and then uses reachability analysis to compute safe time-state corridors for the connected vehicles that pass through the intersection. By analyzing these corridors, in contrast to single trajectories, we can make explicit design decisions regarding safety-efficiency trade-offs while taking each vehicle's decision uncertainty into account. Additionally, we compute safe driving limits to ensure that vehicles remain within their designated safe corridors. Combining these elements, we develop a service that provides safety filters for AIM coordination of connected vehicles. We evaluate the practical feasibility of our safety framework using a simulated 4-way intersection, showing that our approach performs in real-time for multiple scenarios., Comment: To be published in 27th IEEE International Conference on Intelligent Transportation Systems

The choice of lung protective ventilation settings for mechanical ventilation has a considerable impact on patient outcome, yet identifying optimal ventilatory settings for individual patients remains highly challenging due to the inherent inter- and intra-patient pathophysiological variability. In this validation study, we demonstrate that physics-based computational lung models tailored to individual patients can resolve this variability, allowing us to predict the otherwise unknown local state of the pathologically affected lung during mechanical ventilation. For seven ARDS patients undergoing invasive mechanical ventilation, physics-based, patient-specific lung models were created using chest CT scans and ventilatory data. By numerically resolving the interaction of the pathological lung with the airway pressure and flow imparted by the ventilator, we predict the time-dependent and heterogeneous local state of the lung for each patient and compare it against the regional ventilation obtained from bedside monitoring using Electrical Impedance Tomography. Excellent agreement between numerical simulations and experimental data was obtained, with the model-predicted anteroposterior ventilation profile achieving a Pearson correlation of 96% with the clinical reference data. Even when considering the regional ventilation within the entire transverse chest cross-section and across the entire dynamic ventilation range, an average correlation of more than 81% and an average root mean square error of less than 15% were achieved. The results of this first systematic validation study demonstrate the ability of computational models to provide clinically relevant information and thereby open the door for a truly patient-specific choice of ventilator settings on the basis of both individual anatomy and pathophysiology., Comment: 11 pages, 9 figures

One compelling use of citation networks is to characterize papers by their relationships to the surrounding literature. We propose a method to characterize papers by embedding them into two distinct "co-factor" spaces: one describing how papers send citations, and the other describing how papers receive citations. This approach presents several challenges. First, older documents cannot cite newer documents, and thus it is not clear that co-factors are even identifiable. We resolve this challenge by developing a co-factor model for asymmetric adjacency matrices with missing lower triangles and showing that identification is possible. We then frame estimation as a matrix completion problem and develop a specialized implementation of matrix completion because prior implementations are memory bound in our setting. Simulations show that our estimator has promising finite sample properties, and that naive approaches fail to recover latent co-factor structure. We leverage our estimator to investigate 237,794 papers published in statistics journals from 1898 to 2022, resulting in the most comprehensive topic model of the statistics literature to date. We find interpretable co-factors corresponding to many statistical subfields, including time series, variable selection, spatial methods, graphical models, GLM(M)s, causal inference, multiple testing, quantile regression, resampling, semi-parametrics, dimension reduction, and several more.

Multimodal foundation models (MFMs) such as OFASys show the potential to unlock analysis of complex data such as images, videos, and audio data via text prompts alone. However, their performance may suffer in the face of text input that differs even slightly from their training distribution, which is surprising considering the use of modality-specific data to "ground" the text input. This study demonstrates that prompt instability is a major concern for MFMs, leading to a consistent drop in performance across all modalities, but that instability can be mitigated with additional training with augmented data. We evaluate several methods for grounded prompt perturbation, where we generate perturbations and filter based on similarity to text and/or modality data. After re-training the models on the augmented data, we find improved accuracy and more stable performance on the perturbed test data regardless of perturbation condition, suggesting that the data augmentation strategy helps the models handle domain shifts more effectively. In error analysis, we find consistent patterns of performance improvement across domains, suggesting that retraining on prompt perturbations tends to help general reasoning capabilities in MFMs., Comment: in submission

Increasingly large imitation learning datasets are being collected with the goal of training foundation models for robotics. However, despite the fact that data selection has been of utmost importance in vision and natural language processing, little work in robotics has questioned what data such models should actually be trained on. In this work we investigate how to weigh different subsets or ``domains'' of robotics datasets for robot foundation model pre-training. Concrete, we use distributionally robust optimization (DRO) to maximize worst-case performance across all possible downstream domains. Our method, Re-Mix, addresses the wide range of challenges that arise when applying DRO to robotics datasets including variability in action spaces and dynamics across different datasets. Re-Mix employs early stopping, action normalization, and discretization to counteract these issues. Through extensive experimentation on the largest open-source robot manipulation dataset, the Open X-Embodiment dataset, we demonstrate that data curation can have an outsized impact on downstream performance. Specifically, domain weights learned by Re-Mix outperform uniform weights by 38\% on average and outperform human-selected weights by 32\% on datasets used to train existing generalist robot policies, specifically the RT-X models.

Quantum resonances in collisions and reactions are a sensitive probe of the intermolecular forces. They may dominate the final quantum state distribution, as recently observed for Feshbach resonances in a cold collision experiment (Science 380, 77 (2023)). This raises the question whether the sensitivity of such measurements is sufficient to assess the quality of theoretical models for the interaction. We here compare measured collision cross sections to those obtained with exact quantum coupled-channels scattering calculations for three different ab initio potential energy surfaces. We find that the ability to test the correct prediction of energy redistribution over molecular degrees of freedom is within reach, requiring only a modest improvement in energy resolution of current experiments. Such improvement will enable the separation of individual resonances and allow for an unambiguous experimental test of different theory approaches.

We investigate nonlinear model predictive control (MPC) with terminal conditions in the Koopman framework using extended dynamic mode decomposition (EDMD) to generate a data-based surrogate model for prediction and optimization. We rigorously show recursive feasibility and prove practical asymptotic stability w.r.t. the approximation accuracy. To this end, finite-data error bounds are employed. The construction of the terminal conditions is based on recently derived proportional error bounds to ensure the required Lyapunov decrease. Finally, we illustrate the effectiveness of the proposed data-driven predictive controller including the design procedure to construct the terminal region and controller., Comment: Accepted for presentation at the 63rd IEEE Conference on Decision and Control (CDC2024)

Extended Dynamic Mode Decomposition (EDMD) is a widely-used data-driven approach to learn an approximation of the Koopman operator. Consequently, it provides a powerful tool for data-driven analysis, prediction, and control of nonlinear dynamical (control) systems. In this work, we propose a novel modularized EDMD scheme tailored to interconnected systems. To this end, we utilize the structure of the Koopman generator that allows to learn the dynamics of subsystems individually and thus alleviates the curse of dimensionality by considering observable functions on smaller state spaces. Moreover, our approach canonically enables transfer learning if a system encompasses multiple copies of a model as well as efficient adaption to topology changes without retraining. We provide finite-data bounds on the estimation error using tools from graph theory. The efficacy of the method is illustrated by means of various numerical examples., Comment: 31 pages, 11 figures

Objectives: Evaluating the effects and artifacts introduced by medical foreign bodies in clinical dark-field chest radiographs and assessing their influence on the evaluation of pulmonary tissue, compared to conventional radiographs. Material & Methods: This retrospective study analyzed data from subjects enrolled in clinical trials conducted between 2018 and 2021, focusing on chronic obstructive pulmonary disease (COPD) and COVID-19 patients. All patients obtained a radiograph using an in-house developed clinical prototype for grating-based dark-field chest radiography. The prototype simultaneously delivers a conventional and dark-field radiograph. Two radiologists independently assessed the clinical studies to identify patients with foreign bodies. Subsequently, an analysis was conducted on the effects and artifacts attributed to distinct foreign bodies and their impact on the assessment of pulmonary tissue. Results: Overall, 30 subjects with foreign bodies were included in this study (mean age, 64 years +/- 11 [standard deviation]; 15 men). Foreign bodies composed of materials lacking microstructure exhibited a diminished dark-field signal or no discernible signal. Foreign bodies with a microstructure, in our investigations the cementation of the kyphoplasty, produce a positive dark-field signal. Since most foreign bodies lack microstructural features, dark-field imaging revealed fewer signals and artifacts by foreign bodies compared to conventional radiographs. Conclusion: Dark-field radiography enhances the assessment of pulmonary tissue with overlaying foreign bodies compared to conventional radiography. Reduced interfering signals result in fewer overlapping radiopaque artifacts within the investigated regions. This mitigates the impact on image quality and interpretability of the radiographs and the projection-related limitations of radiography compared to CT.

While recent zero-shot multispeaker text-to-speech (TTS) models achieve impressive results, they typically rely on extensive transcribed speech datasets from numerous speakers and intricate training pipelines. Meanwhile, self-supervised learning (SSL) speech features have emerged as effective intermediate representations for TTS. It was also observed that SSL features from different speakers that are linearly close share phonetic information while maintaining individual speaker identity, which enables straight-forward and robust voice cloning. In this study, we introduce SSL-TTS, a lightweight and efficient zero-shot TTS framework trained on transcribed speech from a single speaker. SSL-TTS leverages SSL features and retrieval methods for simple and robust zero-shot multi-speaker synthesis. Objective and subjective evaluations show that our approach achieves performance comparable to state-of-the-art models that require significantly larger training datasets. The low training data requirements mean that SSL-TTS is well suited for the development of multi-speaker TTS systems for low-resource domains and languages. We also introduce an interpolation parameter which enables fine control over the output speech by blending voices. Demo samples are available at https://idiap.github.io/ssl-tts

Over the past few years alone, the lensing community has discovered thousands of strong lens candidates, and spectroscopically confirmed hundreds of them. In this time of abundance, it becomes pragmatic to focus our time and resources on the few extraordinary systems, in order to most efficiently study the universe. In this paper, we present such a system: DESI-090.9854-35.9683, a cluster-scale lens at $z_{\rm l} = 0.49$, with seven observed lensed sources around the core, and additional lensed sources further out in the cluster. From the number and the textbook configuration of the lensed images, a tight constraint on the mass potential of the lens is possible. This would allow for detailed analysis on the dark and luminous matter content within galaxy clusters, as well as a probe into dark energy and high-redshift galaxies. We present our spatially resolved kinematic measurements of this system from the Very Large Telescope Multi Unit Spectroscopic Explorer, which confirm five of these source galaxies (in ascending order, at $z_{\rm s} = 0.962, 0.962, 1.166, 1.432,$ and $1.432$). With previous Hubble Space Telescope imaging in the F140W and F200LP bands, we also present a simple two power-law profile flux-based lens model that, for a cluster lens, well models the five lensed arc families with redshifts. We determine the mass to be $M(< \theta_{\rm E}) = 4.78\times10^{13} M_{\odot}$ for the primary mass potential. From the model, we extrapolate the redshift of one of the two source galaxies not yet spectroscopically confirmed to be at $z_{\rm s}=4.52^{+1.03}_{-0.71}$., Comment: 14 pages, 6 figures

While magnetic monopoles have extensive theoretical justification for their existence, but have proved elusive to observe, ball lightning is both relatively frequently observed and largely unexplained theoretically. It was first proposed in 1990 that ball lightning might result from the catalysis of nuclear fission by a magnetic monopole. The observed frequency of ball lightning does not conflict with current upper theoretical or observational bounds for magnetic monopole flux. Some possible mechanisms to account for the association of magnetic-monopole-caused ball lightning with thunderstorms are described, and proposals for further observational and theoretical research are made., Comment: 16 pages, 1 figure

Packing and shuffling tokens is a common practice in training auto-regressive language models (LMs) to prevent overfitting and improve efficiency. Typically documents are concatenated to chunks of maximum sequence length (MSL) and then shuffled. However setting the atom size, the length for each data chunk accompanied by random shuffling, to MSL may lead to contextual incoherence due to tokens from different documents being packed into the same chunk. An alternative approach is to utilize padding, another common data packing strategy, to avoid contextual incoherence by only including one document in each shuffled chunk. To optimize both packing strategies (concatenation vs padding), we investigated the optimal atom size for shuffling and compared their performance and efficiency. We found that matching atom size to MSL optimizes performance for both packing methods (concatenation and padding), and padding yields lower final perplexity (higher performance) than concatenation at the cost of more training steps and lower compute efficiency. This trade-off informs the choice of packing methods in training language models., Comment: 11 pages (include appendix), 26 figures, submitted to ACL ARR Aug 2024

The promise of quantum computing to circumvent the exponential scaling of quantum chemistry has sparked a race to develop chemistry algorithms for quantum architecture. However, most works neglect the quantum-inherent shot noise, let alone the effect of current noisy devices. Here, we present a comprehensive study of quantum linear response (qLR) theory obtaining spectroscopic properties on simulated fault-tolerant quantum computers and present-day near-term quantum hardware. This work introduces novel metrics to analyze and predict the origins of noise in the quantum algorithm, proposes an Ansatz-based error mitigation technique, and highlights the significant impact of Pauli saving in reducing measurement costs and noise. Our hardware results using up to cc-pVTZ basis set serve as proof-of-principle for obtaining absorption spectra on quantum hardware in a general approach with the accuracy of classical multi-configurational methods. Importantly, our results exemplify that substantial improvements in hardware error rates and measurement speed are necessary to lift quantum computational chemistry from proof-of-concept to an actual impact in the field.

Crop phenology determines crop growth stages and is valuable information for decision makers to plant and adapt agricultural management strategies to enhance food security. In the era of big Earth observation data ubiquity, attempts have been made to accurately predict crop phenology based on Remote Sensing (RS) data. However, most studies either focused on large scale interpretations of phenology or developed methods which are not adequate to help crop modeler communities on leveraging the value of RS data evaluated using more accurate and confident methods. Here, we estimate phenological developments for eight major crops and 13 phenological stages across Germany at 30m scale using a novel framework which fuses Landsat and Sentinel 2 (Harmonized Landsat and Sentinel data base; HLS) and radar of Sentinel 1 with a Machine Learning (ML) model. We proposed a thorough feature fusion analysis to find the best combinations of RS data on detecting phenological developments based on the national phenology network of Germany (German Meteorological Service; DWD) between 2017 and 2021. The nation-wide predicted crop phenology at 30 m resolution showed a very high precision of R2 > 0.9 and a very low Mean Absolute Error (MAE) < 2 (days). These results indicate that our fusing strategy of optical and radar datasets is highly performant with an accuracy highly relevant for practical applications, too. The subsequent uncertainty analysis indicated that fusing optical and radar data increases the reliability of the RS predicted crop growth stages. These improvements are expected to be useful for crop model calibrations and evaluations, facilitate informed agricultural decisions, and contribute to sustainable food production to address the increasing global food demand.

Obtaining exact solutions to combinatorial optimization problems using classical computing is computationally expensive. The current tenet in the field is that quantum computers can address these problems more efficiently. While promising algorithms require fault-tolerant quantum hardware, variational algorithms have emerged as viable candidates for near-term devices. The success of these algorithms hinges on multiple factors, with the design of the ansatz having the utmost importance. It is known that popular approaches such as quantum approximate optimization algorithm (QAOA) and quantum annealing suffer from adiabatic bottlenecks, that lead to either larger circuit depth or evolution time. On the other hand, the evolution time of imaginary time evolution is bounded by the inverse energy gap of the Hamiltonian, which is constant for most non-critical physical systems. In this work, we propose imaginary Hamiltonian variational ansatz ($i$HVA) inspired by quantum imaginary time evolution to solve the MaxCut problem. We introduce a tree arrangement of the parametrized quantum gates, enabling the exact solution of arbitrary tree graphs using the one-round $i$HVA. For randomly generated $D$-regular graphs, we numerically demonstrate that the $i$HVA solves the MaxCut problem with a small constant number of rounds and sublinear depth, outperforming QAOA, which requires rounds increasing with the graph size. Furthermore, our ansatz solves MaxCut exactly for graphs with up to 24 nodes and $D \leq 5$, whereas only approximate solutions can be derived by the classical near-optimal Goemans-Williamson algorithm. We validate our simulated results with hardware experiments on a graph with 63 nodes., Comment: 23 pages, 15 figures

Recently, interest in quantum computing has significantly increased, driven by its potential advantages over classical techniques. Quantum machine learning (QML) exemplifies one of the important quantum computing applications that are expected to surpass classical machine learning in a wide range of instances. This paper addresses the performance of QML in the context of high-energy physics (HEP). As an example, we focus on the top-quark tagging, for which classical convolutional neural networks (CNNs) have been effective but fall short in accuracy when dealing with highly energetic jet images. In this paper, we use a quantum convolutional neural network (QCNN) for this task and compare its performance with CNN using a classical noiseless simulator. We compare various setups for the QCNN, varying the convolutional circuit, type of encoding, loss function, and batch sizes. For every quantum setup, we design a similar setup to the corresponding classical model for a fair comparison. Our results indicate that QCNN with proper setups tend to perform better than their CNN counterparts, particularly when the convolution block has a lower number of parameters. This suggests that quantum models, especially with appropriate encodings, can hold potential promise for enhancing performance in HEP tasks such as top quark jet tagging.

Decentralized optimization has become a standard paradigm for solving large-scale decision-making problems and training large machine learning models without centralizing data. However, this paradigm introduces new privacy and security risks, with malicious agents potentially able to infer private data or impair the model accuracy. Over the past decade, significant advancements have been made in developing secure decentralized optimization and learning frameworks and algorithms. This survey provides a comprehensive tutorial on these advancements. We begin with the fundamentals of decentralized optimization and learning, highlighting centralized aggregation and distributed consensus as key modules exposed to security risks in federated and distributed optimization, respectively. Next, we focus on privacy-preserving algorithms, detailing three cryptographic tools and their integration into decentralized optimization and learning systems. Additionally, we examine resilient algorithms, exploring the design and analysis of resilient aggregation and consensus protocols that support these systems. We conclude the survey by discussing current trends and potential future directions., Comment: 38 pages

Integral field spectroscopy (IFS) is a powerful tool for understanding the formation of galaxies across cosmic history. We present the observing strategy and first results of MSA-3D, a novel JWST program using multi-object spectroscopy in a slit-stepping strategy to produce IFS data cubes. The program observed 43 normal star-forming galaxies at redshifts $0.5 \lesssim z \lesssim 1.5$, corresponding to the epoch when spiral thin-disk galaxies of the modern Hubble sequence are thought to emerge, obtaining kpc-scale maps of rest-frame optical nebular emission lines with spectral resolution $R\simeq2700$. Here we describe the multiplexed slit-stepping method which is $>15$ times more efficient than the NIRSpec IFS mode for our program. As an example of the data quality, we present a case study of an individual galaxy at $z=1.104$ (stellar mass $M_{*} = 10^{10.3}~M_{\odot}$, star formation rate~$=3~M_{\odot}$ yr$^{-1}$) with prominent face-on spiral structure. We show that the galaxy exhibits a rotationally supported disk with moderate velocity dispersion ($\sigma = 36^{+5}_{-4}$~\kms), a negative radial metallicity gradient ($-0.020\pm0.002$~dex\,kpc$^{-1}$), a dust attenuation gradient, and an exponential star formation rate density profile which closely matches the stellar continuum. These properties are characteristic of local spirals, indicating that mature galaxies are in place at $z\sim1$. We also describe the customized data reduction and original cube-building software pipelines which we have developed to exploit the powerful slit-stepping technique. Our results demonstrate the ability of JWST slit-stepping to study galaxy populations at intermediate to high redshifts, with data quality similar to current surveys of the $z\sim0.1$ universe., Comment: 24 pages, 12 figures, 1 table; submitted to ApJ, comments welcome. Our custom designed data reduction pipeline (MSA3D) and example processed data-cube will be publicly released before the JWST Cycle 4 deadline. MSA3D package on GitHub: https://github.com/barisiciv/msa3d.git

Intensity interferometry is a reemerging astronomical technique for performing high angular resolution studies at visible wavelengths, benefiting immensely from the recent improvements in (single) photon detection instrumentation. Contrary to direct imaging or amplitude interferometry, intensity interferometry correlates light intensities rather than light amplitudes, circumventing atmospheric seeing limitations at the cost of reduced sensitivity. In this paper we present measurements with the 1.04 m Omicron telescope of C2PU (Centre P\'edagogique Plan\`ete Univers) at the Calern Observatory in the south of France featuring hybrid single photon counting detectors (HPDs). We successfully measured photon bunching from temporal correlations of three different A-type stars - Vega, Altair and Deneb - in the blue at 405 nm. In all cases the observed coherence time fits well to both the pre-calculated expectations as well as the values measured in preceding laboratory tests. The best signal to noise ratio (SNR), with a value of 12, is obtained for Vega for an observation time of 12.1 h. The combination of HPDs and time to digital converter (TDC) results in a timing jitter of the detection system < 50 ps. Our setup demonstrates stable and efficient detection of the starlight owed to the large active area of the HPDs. Utilizing a new class of large area single photon detectors based on multichannel plate amplification, high resolution spatial intensity interferometry experiments are within reach at 1 m diameter class telescopes within one night of observation time for bright stars.

This study investigates thermal transport across nanocrystalline diamond/AlGaN interfaces, crucial for enhancing thermal management in AlGaN/AlGaN-based devices. Chemical vapor deposition growth of diamond directly on AlGaN resulted in a disordered interface with a high thermal boundary resistance (TBR) of 20.6 m^2-K/GW. We employed sputtered carbide interlayers (e.g., $B_4C$, $SiC$, $B_4C/SiC$) to reduce thermal boundary resistance in diamond/AlGaN interfaces. The carbide interlayers resulted in record-low thermal boundary resistance values of 3.4 and 3.7 m^2-K/GW for Al$_{0.65}$Ga$_{0.35}$N samples with $B_4C$ and $SiC$ interlayers, respectively. STEM imaging of the interface reveals interlayer thicknesses between 1.7-2.5 nm, with an amorphous structure. Additionally, Fast-Fourier Transform (FFT) characterization of sections of the STEM images displayed sharp crystalline fringes in the AlGaN layer, confirming it was properly protected from damage from hydrogen plasma during the diamond growth. In order to accurately measure the thermal boundary resistance we develop a hybrid technique, combining time-domain thermoreflectance and steady-state thermoreflectance fitting, offering superior sensitivity to buried thermal resistances. Our findings underscore the efficacy of interlayer engineering in enhancing thermal transport and demonstrate the importance of innovative measurement techniques in accurately characterizing complex thermal interfaces. This study provides a foundation for future research in improving thermal properties of semiconductor devices through interface engineering and advanced measurement methodologies.

We present new JWST observations of the nearby, prototypical edge-on, spiral galaxy NGC 891. The northern half of the disk was observed with NIRCam in its F150W and F277W filters. Absorption is clearly visible in the mid-plane of the F150W image, along with vertical dusty plumes that closely resemble the ones seen in the optical. A $\sim 10 \times 3~{\rm kpc}^2$ area of the lower circumgalactic medium (CGM) was mapped with MIRI F770W at 12 pc scales. Thanks to the sensitivity and resolution of JWST, we detect dust emission out to $\sim 4$ kpc from the disk, in the form of filaments, arcs, and super-bubbles. Some of these filaments can be traced back to regions with recent star formation activity, suggesting that feedback-driven galactic winds play an important role in regulating baryonic cycling. The presence of dust at these altitudes raises questions about the transport mechanisms at play and suggests that small dust grains are able to survive for several tens of million years after having been ejected by galactic winds in the disk-halo interface. We lay out several scenarios that could explain this emission: dust grains may be shielded in the outer layers of cool dense clouds expelled from the galaxy disk, and/or the emission comes from the mixing layers around these cool clumps where material from the hot gas is able to cool down and mix with these cool cloudlets. This first set of data and upcoming spectroscopy will be very helpful to understand the survival of dust grains in energetic environments, and their contribution to recycling baryonic material in the mid-plane of galaxies., Comment: Accepted for publication in Astronomy & Astrophysics; 16 pages, 8 figures

While quiescent galaxies have comparable amounts of cool gas in their outer circumgalactic medium (CGM) compared to star-forming galaxies, they have significantly less interstellar gas. However, open questions remain on the processes causing galaxies to stop forming stars and stay quiescent . Theories suggest dynamical interactions with the hot corona prevent cool gas from reaching the galaxy, therefore predicting the inner regions of quiescent galaxy CGMs are devoid of cool gas. However, there is a lack of understanding of the inner regions of CGMs due to the lack of spatial information in quasar-sightline methods. We present integral-field spectroscopy probing 10--20~kpc (2.4--4.8 R\textsubscript{e}) around a massive quiescent galaxy using a gravitationally lensed star-forming galaxy. We detect absorption from Magnesium (MgII) implying large amounts of cool atomic gas (10\textsuperscript{8.4} -- 10\textsuperscript{9.3} M\textsubscript{$\odot$} with T$\sim$10\textsuperscript{4} Kelvin), in comparable amounts to star-forming galaxies. Lens modeling of Hubble imaging also reveals a diffuse asymmetric component of significant mass consistent with the spatial extent of the MgII absorption, and offset from the galaxy light profile. This study demonstrates the power of galaxy-scale gravitational lenses to not only probe the gas around galaxies, but to also independently probe the mass of the CGM due to it's gravitational effect., Comment: accepted nature communications physics

New particles beyond the Standard Model of particle physics, such as axions, can be effectively searched through their interactions with electrons. We use the large liquid xenon detector PandaX-4T to search for novel electronic recoil signals induced by solar axions, neutrinos with anomalous magnetic moment, axion-like particles, dark photons, and light fermionic dark matter. A detailed background model is established with the latest datasets with 1.54 $\rm tonne \cdot year$ exposure. No significant excess above the background has been observed, and we have obtained competitive constraints for axion couplings, neutrino magnetic moment, and fermionic dark matter interactions.

In previous publications, we have presented an alternative approach to determine essential detector properties like the Modulation Transfer Function (MTF), the Noise Power Spectrum (NPS) and the Detective Quantum Efficiency (DQE) based on a Monte Carlo model of the detection process. If a Monte Carlo model for the detector response to photons impinging at various locations of a pixel is available, the full statistics of the detector can be derived in a straightforward manner. The purpose of this paper is to describe the method in detail and to apply it to four types of realistic detectors: direct converting detectors using CdTe and silicon, a CdTe photon counter with additional coincidence counters and an optical counting system using LaBr3 as scintillator., Comment: 13 pages

The European Central Bank is preparing for the potential issuance of a central bank digital currency (CBDC), called the digital euro. A recent regulatory proposal by the European Commission defines several requirements for the digital euro, such as support for both online and offline payments. Offline payments are expected to enable cash-like privacy, local payment settlement, and the enforcement of holding limits. While other central banks have expressed similar desired functionality, achieving such offline payments poses a novel technical challenge. We observe that none of the existing research solutions, including offline E-cash schemes, are fully compliant. Proposed solutions based on secure elements offer no guarantees in case of compromise and can therefore lead to significant payment fraud. The main contribution of this paper is PayOff, a novel CBDC design motivated by the digital euro regulation, which focuses on offline payments. We analyze the security implications of local payment settlement and identify new security objectives. PayOff protects user privacy, supports complex regulations such as holding limits, and implements safeguards to increase robustness against secure element failure. Our analysis shows that PayOff provides strong privacy and identifies residual leakages that may arise in real-world deployments. Our evaluation shows that offline payments can be fast and that the central bank can handle high payment loads with moderate computing resources. However, the main limitation of PayOff is that offline payment messages and storage requirements grow in the number of payments that the sender makes or receives without going online in between.

We study the quasinormal modes of a holographic model of a Weyl semimetal. The model features quantum phase transition between a topological phase and a trivial phase. We put particular emphasis on the hydrodynamic modes and show that a hydrodynamic mode is present only in the topological Weyl semimetal phase., Comment: 20 Pages, 12 Figures

In this work, we present a transformer-based framework for predicting future pedestrian states based on clustered historical trajectory data. In previous studies, researchers propose enhancing pedestrian trajectory predictions by using manually crafted labels to categorize pedestrian behaviors and intentions. However, these approaches often only capture a limited range of pedestrian behaviors and introduce human bias into the predictions. To alleviate the dependency on manually crafted labels, we utilize a transformer encoder coupled with hierarchical density-based clustering to automatically identify diverse behavior patterns, and use these clusters in data-driven reachability analysis. By using a transformer-based approach, we seek to enhance the representation of pedestrian trajectories and uncover characteristics or features that are subsequently used to group trajectories into different "behavior" clusters. We show that these behavior clusters can be used with data-driven reachability analysis, yielding an end-to-end data-driven approach to predicting the future motion of pedestrians. We train and evaluate our approach on a real pedestrian dataset, showcasing its effectiveness in forecasting pedestrian movements.

We use JWST/NIRSpec observations from the Assembly of Ultradeep Rest-optical Observations Revealing Astrophysics (AURORA) survey to constrain the shape of the nebular attenuation curve of a star-forming galaxy at z=4.41, GOODSN-17940. We utilize 11 unblended HI recombination lines to derive the attenuation curve spanning optical to near-infrared wavelengths (3751-9550 \r{A}). We then leverage a high-S/N spectroscopic detection of the rest-frame ultraviolet continuum in combination with rest-UV photometric measurements to constrain the shape of the curve at ultraviolet wavelengths. While this UV constraint is predominantly based on stellar emission, the large measured equivalent widths of H$\alpha$ and H$\beta$ indicate that GOODSN-17940 is dominated by an extremely young stellar population <10 Myr in age such that the UV stellar continuum experiences the same attenuation as the nebular emission. The resulting combined nebular attenuation curve spans 1400-9550 \r{A} and has a shape that deviates significantly from commonly assumed dust curves in high-redshift studies. Relative to the Milky Way, SMC, and Calzetti curves, the new curve has a steeper slope at long wavelengths ($\lambda>5000$ \r{A}) while displaying a similar slope across blue-optical wavelengths ($\lambda=3750-5000$ \r{A}). In the ultraviolet, the new curve is shallower than the SMC and Calzetti curves and displays no significant 2175 \r{A} bump. This work demonstrates that the most commonly assumed dust curves are not appropriate for all high-redshift galaxies. These results highlight the ability to derive nebular attenuation curves for individual high-redshift sources with deep JWST/NIRSpec spectroscopy, thereby improving the accuracy of physical properties inferred from nebular emission lines., Comment: 21 pages, 6 figures, 1 table, submitted to ApJ

The projected sensitivity of the effective electron neutrino-mass measurement with the KATRIN experiment is below 0.3 eV (90 % CL) after five years of data acquisition. The sensitivity is affected by the increased rate of the background electrons from KATRIN's main spectrometer. A special shifted-analysing-plane (SAP) configuration was developed to reduce this background by a factor of two. The complex layout of electromagnetic fields in the SAP configuration requires a robust method of estimating these fields. We present in this paper a dedicated calibration measurement of the fields using conversion electrons of gaseous $^\mathrm{83m}$Kr, which enables the neutrino-mass measurements in the SAP configuration., Comment: 19 pages, 11 figures

This paper investigates the use of the cubic-regularized Newton method within a federated learning framework while addressing two major concerns that commonly arise in federated learning: privacy leakage and communication bottleneck. We introduce a federated learning algorithm called Differentially Private Federated Cubic Regularized Newton (DP-FCRN). By leveraging second-order techniques, our algorithm achieves lower iteration complexity compared to first-order methods. We also incorporate noise perturbation during local computations to ensure privacy. Furthermore, we employ sparsification in uplink transmission, which not only reduces the communication costs but also amplifies the privacy guarantee. Specifically, this approach reduces the necessary noise intensity without compromising privacy protection. We analyze the convergence properties of our algorithm and establish the privacy guarantee. Finally, we validate the effectiveness of the proposed algorithm through experiments on a benchmark dataset.

AI assistants are being increasingly used by students enrolled in higher education institutions. While these tools provide opportunities for improved teaching and education, they also pose significant challenges for assessment and learning outcomes. We conceptualize these challenges through the lens of vulnerability, the potential for university assessments and learning outcomes to be impacted by student use of generative AI. We investigate the potential scale of this vulnerability by measuring the degree to which AI assistants can complete assessment questions in standard university-level STEM courses. Specifically, we compile a novel dataset of textual assessment questions from 50 courses at EPFL and evaluate whether two AI assistants, GPT-3.5 and GPT-4 can adequately answer these questions. We use eight prompting strategies to produce responses and find that GPT-4 answers an average of 65.8% of questions correctly, and can even produce the correct answer across at least one prompting strategy for 85.1% of questions. When grouping courses in our dataset by degree program, these systems already pass non-project assessments of large numbers of core courses in various degree programs, posing risks to higher education accreditation that will be amplified as these models improve. Our results call for revising program-level assessment design in higher education in light of advances in generative AI., Comment: 20 pages, 8 figures

We present the design and observations of low resolution JWST/NIRSpec PRISM spectroscopy from the Ultradeep NIRSpec and NIRCam ObserVations before the Epoch of Reionization (UNCOVER) Cycle 1 JWST Treasury program. Targets are selected using JWST/NIRCam photometry from UNCOVER and other programs, and cover a wide range of categories and redshifts to ensure the legacy value of the survey. These categories include the first galaxies at $z\gtrsim10$, faint galaxies during the Epoch of Reionization ($z\sim6-8$), high redshift AGN ($z\gtrsim6$), Population III star candidates, distant quiescent and dusty galaxies ($1\lesssim z \lesssim 6$), and filler galaxies sampling redshift--color--magnitude space from $z\sim 0.1-13$. Seven NIRSpec MSA masks across the extended Abell 2744 cluster were observed, along with NIRCam parallel imaging in 8 filters (F090W, F115W, F150W, F200W, F277W, F356W, F410M, F444W, F480M) over a total area of ~26 arcmin$^2$, overlapping existing HST coverage from programs including the Hubble Frontier Fields and BUFFALO. We successfully observed 553 objects down to $m_{\mathrm{F444W}}\sim30\mathrm{AB}$, and by leveraging mask overlaps, we reach total on-target exposure times ranging from 2.4-16.7h. We demonstrate the success rate and distribution of confirmed redshifts, and also highlight the rich information revealed by these ultradeep spectra for a subset of our targets. An updated lens model of Abell 2744 is also presented, including 14 additional spectroscopic redshifts and finding a total cluster mass of $M_{\mathrm{SL}}=(2.1\pm0.3)\times10^{15}\,\mathrm{M}_{\odot}$. We publicly release reduced 1D and 2D spectra for all objects observed in Summer 2023 along with a spectroscopic redshift catalog and the updated lens model of the cluster (https://jwst-uncover.github.io/DR4.html)., Comment: 19 pages, 9 figures, 4 tables, submitted to ApJ, comments welcome! Data available at: https://jwst-uncover.github.io/DR4.html (v2: figure format correction)

Axions are a well-motivated dark matter candidate particle. Haloscopes aim to detect axions in the galactic halo by measuring the photon signal resulting from axions interacting with a strong magnetic field. Existing haloscopes are primarily targeting axion masses which produce microwave-range photons and rely on microwave resonators to enhance the signal power. Only a limited subset of resonator modes are useful for this process, and current cylindrical-style cavities suffer from mode mixing and crowding from other fundamental modes. The majority of these modes can be eliminated by using photonic band gap (PBG) resonators. The band gap behavior of these structures allows for a resonator with mode selectivity based on frequency. We present results from the first tunable PBG resonator, a proof-of-concept design with a footprint compatible with axion haloscopes. We have thoroughly characterized the tuning range of two versions of the structure and report the successful confinement of the operating TM$_{010}$ mode and the elimination of all TE modes within the tuning range., Comment: 7 pages, 8 figures

This paper presents a unified algorithm for motion and force control for a six degree-of-freedom spatial manipulator. The motion-force controller performs trajectory tracking, maneuvering the manipulator's end-effector through desired position, orientations and rates. When contacting an obstacle or target object, the force module of the controller restricts the manipulator movements with a novel force exertion method, which prevents damage to the manipulator, the end-effector, and the objects during the contact or collision. The core strategy presented in this paper is to design the linear acceleration for the end-effector which ensures both trajectory tracking and restriction of any contact force at the end-effector. The design of the controller is validated through numerical simulations and digital twin validation.

Recent Atacama Large Millimeter/submillimeter Array (ALMA) observations of protoplanetary disks in the millimeter continuum have shown a variety of radial gaps, cavities, and spiral features. These substructures may be signposts for ongoing planet formation, and therefore these systems are promising targets for direct imaging planet searches in the near-infrared. To this end, we present results from a deep imaging survey in the $L'$-band (3.8 $\mu$m) with the Keck/NIRC2 vortex coronagraph to search for young planets in 43 disks with resolved features in the millimeter continuum or evidence for gaps/central cavities from their spectral energy distributions. Although we do not detect any new point sources, using the vortex coronagraph allows for high sensitivity to faint sources at small angular separations (down to ${\sim}$0$^{\prime\prime}$.1), allowing us to place strong upper limits on the masses of potential gas giant planets. We compare our mass sensitivities to the masses of planets derived using ALMA observations, and while we are sensitive to $\sim$1 M$_{Jup}$ planets in the gaps in some of our systems, we are generally not sensitive to planets of the masses expected from the ALMA observations. In addition to placing upper limits on the masses of gas giant planets that could be interacting with the dust in the disks to form the observed millimeter substructures, we are also able to map the micron-sized dust as seen in scattered light for 8 of these systems. Our large sample of systems also allows us to investigate limits on planetary accretion rates and disk viscosities., Comment: 23 pages, 14 figures, 3 tables, accepted for publication in AJ

Crush curves are of fundamental importance to numerical modeling of small and porous astrophysical bodies. The empirical literature often measures them for silica grains, and different studies have used various methods, sizes, textures, and pressure conditions. Here we review past studies and supplement further experiments in order to develop a full and overarching understanding of the silica crush curve behavior. We suggest a new power-law function that can be used in impact simulations of analog materials similar to micro-granular silica. We perform a benchmarking study to compare this new crush curve to the parametric quadratic crush curve often used in other studies, based on the study case of the DART impact onto the asteroid Dimorphos. We find that the typical quadratic crush curve parameters do not closely follow the silica crushing experiments, and as a consequence they under (over) estimate compression close (far) from the impact site. The new crush curve presented here, applicable to pressures between a few hundred Pa and up to 1.1 GPa, might therefore be more precise. Additionally, it is not calibrated by case-specific parameters, and can be used universally for comet- or asteroid-like bodies, given an assumed composition similar to micro-granular silica., Comment: Accepted to ApJ

Variational quantum algorithms and, in particular, variants of the varational quantum eigensolver have been proposed to address combinatorial optimization (CO) problems. Using only shallow ansatz circuits, these approaches are deemed suitable for current noisy intermediate-scale quantum hardware. However, the resources required for training shallow variational quantum circuits often scale superpolynomially in problem size. In this study we numerically investigate what this scaling result means in practice for solving CO problems using Max-Cut as a benchmark. For fixed resources, we compare the average performance of training a shallow variational quantum circuit, sampling with replacement, and a greedy algorithm starting from the same initial point as the quantum algorithm. We identify a minimum problem size for which the quantum algorithm can consistently outperform sampling and, for each problem size, characterize the separation between the quantum algorithm and the greedy algorithm. Furthermore, we extend the average case analysis by investigating the correlation between the performance of the algorithms by instance. Our results provide a step towards meaningful benchmarks of variational quantum algorithms for CO problems for a realistic set of resources.

The gas-phase velocity dispersions in disk galaxies, which trace turbulence in the interstellar medium, are observed to increase with lookback time. However, the mechanisms that set this rise in turbulence are observationally poorly constrained. To address this, we combine kiloparsec-scale ALMA observations of CO(3-2) and CO(4-3) with HST observations of H$\alpha$ to characterize the molecular gas and star formation properties of seven local analogues of main sequence galaxies at $z \sim 1-2$, drawn from the DYNAMO sample. Investigating the ''molecular gas main sequence'' on kpc-scales, we find that galaxies in our sample are more gas-rich than local star-forming galaxies at all disk positions. We measure beam smearing corrected molecular gas velocity dispersions and relate them to the molecular gas and star formation rate surface densities. Despite being relatively nearby ($z \sim 0.1$), DYNAMO galaxies exhibit high velocity dispersions and gas and star formation rate surface densities throughout their disks, when compared to local star forming samples. Comparing these measurements to predictions from star formation theory, we find very good agreements with the latest feedback-regulated star formation models. However, we find that theories which combine gravitational energy dissipation from radial gas transport with feedback over-estimate the observed molecular gas velocity dispersions., Comment: 24 pages, 12 figures, 2 tables, accepted for publication in The Astrophysical Journal

The unsupervised and principled diagnosis of multi-scale data is a fundamental obstacle in modern scientific problems from, for instance, weather and climate prediction, neurology, epidemiology, and turbulence. Multi-scale data is characterized by a combination of processes acting along multiple dimensions simultaneously, spatiotemporal scales across orders of magnitude, non-stationarity, and/or invariances such as translation and rotation. Existing methods are not well-suited to multi-scale data, usually requiring supervised strategies such as human intervention, extensive tuning, or selection of ideal time periods. We present the multi-resolution Coherent Spatio-Temporal Scale Separation (mrCOSTS), a hierarchical and automated algorithm for the diagnosis of coherent patterns or modes in multi-scale data. mrCOSTS is a variant of Dynamic Mode Decomposition which decomposes data into bands of spatial patterns with shared time dynamics, thereby providing a robust method for analyzing multi-scale data. It requires no training but instead takes advantage of the hierarchical nature of multi-scale systems. We demonstrate mrCOSTS using complex multi-scale data sets that are canonically difficult to analyze: 1) climate patterns of sea surface temperature, 2) electrophysiological observations of neural signals of the motor cortex, and 3) horizontal wind in the mountain boundary layer. With mrCOSTS, we trivially retrieve complex dynamics that were previously difficult to resolve while additionally extracting hitherto unknown patterns of activity embedded in the dynamics, allowing for advancing the understanding of these fields of study. This method is an important advancement for addressing the multi-scale data which characterize many of the grand challenges in science and engineering., Comment: SI Movies and Figures are available as Ancillary Files

We introduce a real-time identification method for discrete-time state-dependent switching systems in both the input--output and state-space domains. In particular, we design a system of adaptive algorithms running in two timescales; a stochastic approximation algorithm implements an online deterministic annealing scheme at a slow timescale and estimates the mode-switching signal, and an recursive identification algorithm runs at a faster timescale and updates the parameters of the local models based on the estimate of the switching signal. We first focus on piece-wise affine systems and discuss identifiability conditions and convergence properties based on the theory of two-timescale stochastic approximation. In contrast to standard identification algorithms for switched systems, the proposed approach gradually estimates the number of modes and is appropriate for real-time system identification using sequential data acquisition. The progressive nature of the algorithm improves computational efficiency and provides real-time control over the performance-complexity trade-off. Finally, we address specific challenges that arise in the application of the proposed methodology in identification of more general switching systems. Simulation results validate the efficacy of the proposed methodology.

In this letter, we report the dark matter search results from the commissioning run and the first science run of the PandaX-4T experiment. A blind analysis is carried out on the entire data set. The data processing is improved compared to previous work, unifying the low-level signal reconstruction in a wide energy range up to 120 keV. With a total exposure of 1.54 tonne$\cdot$year, no significant excess of nuclear recoil events is found. The lowest 90% confidence level exclusion on the spin-independent cross section is $1.6 \times 10^{-47} \mathrm{cm}^2$ at a dark matter mass of 40 GeV$/c^2$. Our results represent the most stringent constraint for a dark matter mass above 100 GeV$/c^2$.

This paper introduces a novel nonlinear stochastic model predictive control path integral (MPPI) method, which considers chance constraints on system states. The proposed belief-space stochastic MPPI (BSS-MPPI) applies Monte-Carlo sampling to evaluate state distributions resulting from underlying systematic disturbances, and utilizes a Control Barrier Function (CBF) inspired heuristic in belief space to fulfill the specified chance constraints. Compared to several previous stochastic predictive control methods, our approach applies to general nonlinear dynamics without requiring the computationally expensive system linearization step. Moreover, the BSS-MPPI controller can solve optimization problems without limiting the form of the objective function and chance constraints. By multi-threading the sampling process using a GPU, we can achieve fast real-time planning for time- and safety-critical tasks such as autonomous racing. Our results on a realistic race-car simulation study show significant reductions in constraint violation compared to some of the prior MPPI approaches, while being comparable in computation times.

The question of which triangular numbers have a decimal representation containing a single repeated digit seamed to be settled since at least the 1970s: Ballew and Weger provided a complete list and a proof that these are the only numbers of this kind. This assertion is referenced by other authors in the field. However, their proof is flawed. We present a new and elementary proof of the statement, which corrects the error.

We develop a novel perspective on reflection positivity (RP) on the strip by systematically developing the analogies with the unit disc and the upper half plane in the complex plane. These domains correspond to the three conjugacy classes of one-parameter groups in the M\"obius group (elliptic for the disc, parabolic for the upper half plane and hyperbolic for the strip). In all cases, reflection positive functions correspond to positive functionals on $H^\infty$ for a suitable involution. For the strip, reflection positivity naturally connects with Kubo--Martin--Schwinger (KMS) conditions on the real line and further to standard pairs, as they appear in Algebraic Quantum Field Theory. We also exhibit a curious connection between Hilbert spaces on the strip and the upper half plane, based on a periodization process.