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We present an experimental realization of a compact and reliable way to build a nondegenerate polarization-entangled photon-pair source based on a dual-periodically-poled $ {\rm Ti}:{{\rm LiNbO}_3} $Ti:LiNbO

Optical microcavities have been widely used in nonlinear optics, quantum optics, and laser technologies. Here we demonstrate the self-injection locking of a distributed feedback diode laser using home-made high-finesse Fabry-Perot microcavity. The Fabry-Perot microcavity is fabricated from an x-cut lithium niobate crystal with highly reflective coatings. Frequency pulling effect can be observed for a successful locking, and results in a single-longitudinal mode lasing with narrow linewidth. The lasing wavelength and output power are found robust to the laser-diode current and temperature variations, in comparison to the free-running case. We further characterize the laser linewidth with beat note measurement with a high-performance external cavity diode laser, with beat-note linewidth of 601.85 kHz. This results shows a new method for laser frequency stabilization in a simple setup, and may find applications in telecommunication and spectroscopy.

We study the effect of waveguide thickness variations on the frequency spectrum of spontaneous parametric down-conversion in the periodically-poled lithium niobate on insulator (LNOI) waveguide. We analyze several variation models and our simulation results show that thickness variations in several nanometers can induce distinct effects on the central peak of the spectrum, such as narrowing, broadening, and splitting. We also prove that the effects of positive and negative variations can be canceled and thus lead to a variation-robust feature and an ultra-broad bandwidth. Our study may promote the development of on-chip photon sources in the LNOI platform, as well as opensup a way to engineer photon frequency state.

Metal–semiconductor junctions are at the heart of modern electronics. Various two-dimensional materials (2D) based electronic devices have been reported. However, Ohmic contacts between evaporated metal contacts and semiconducting 2D materials are still hard to achieve. Thus, design and fabrication of Schottky diodes based on layered WSe2 remain challenging. Here, we report a doping-free strategy to achieve Ohmic contacts in WSe2 diodes via van der Waals (vdW) contacts. We designed and fabricated vertical WSe2/Pd Schottky diodes, in which Ohmic and Schottky junctions can be realized simultaneously via vdW contacts and evaporated contacts, respectively. The specific contact resistance of the vdW contact is about 74.5 kΩ·μm2. The Schottky diodes exhibit strong rectification behavior with rectification ratio up to 105.

Narrowband photonic entanglement is a crucial resource for long-distance quantum communication and quantum information processing, including quantum memories. We demonstrate the first polarization entanglement with 7.1 GHz inherent bandwidth by counterpropagating domain engineering, which is also confirmed by Hong–Ou–Mandel interference with 155-ps base-to-base dip width and ( 97.1 ± 0.59 ) % high visibility. The entanglement is harnessed with 18.5-standard-deviations Bell inequality violation, and further characterized with state tomography of ( 95.71 ± 0.61 ) % fidelity. Such narrowband entanglement sets a cornerstone for practical quantum information applications.

We demonstrate a broadband optical parametric oscillation, using a sheet cavity, via cavity phase-matching. A 21.2 THz broad comb-like spectrum is achieved, with a uniform line spacing of 133.0 GHz, despite a relatively large dispersion of 275.4 fs2/mm around 1064 nm. With 22.6% high slope efficiency, and 14.9 kW peak power handling, this sheet optical parametric oscillator can be further developed for χ (2) comb.

Mid-infrared (MIR) radiation is essential for remote gas sensing, ranging, and lidar applications, where high pulse energy and narrow linewidth are the keys to the high sensitivity over long distance. However, complex optical and electronic locking schemes are normally required to achieve both features at the same time. Here, we demonstrate pulse-pumped single-longitudinal-mode (SLM) MIR generation using a microresonator seed in the form of a sheet optical parametric oscillator (SOPO). The SOPO features a sub-coherence-length thickness of 400 µm, which enables SLM and high-energy oscillation using cavity phase matching. Its output around 1.55 µm is seeded into an optical parametric amplifier and locks the MIR output in SLM at 3.38 µm. In a simple and compact setup, up to 21% conversion efficiency and 22% slope efficiency are measured with a MIR output energy of 54 µJ. This SLM MIR source with the SOPO seed greatly reduces the system size and is compatible for further integration for field-deployable devices and thus has broad applications in the field of remote gas sensing.

We report a novel turn-on two-photon fluorescent probe (TPNF) for detecting formaldehyde based on aza-Cope rearrangement and intramolecular charge transfer (ICT). The probe, containing a 1,8-naphthalimide dye with a homoallylamino group, has was shown with high selectivity, sensitivity and low cytotoxicity and it was capable of detecting formaldehyde in live cells. Moreover, a time-dependent density functional theory (TD-DFT) calculation was performed to demonstrate the turn on mechanism of the probe via ICT effect. Finally, a zebrafish larvae imaging experiment reveals that TPNF displayed a significant signal change when treated with FA in vivo. These results indicated that TPNF is a promising tool in more biomedical researches.

Frequency upconversion for single photons at telecom wavelengths is important to simultaneously meet the different wavelength requirements for long-distance communications and quantum memories in a quantum nodal network. It also enables the detection for the telecom "flying qubit" photons with silicon-based efficient single-photon detectors with low dark count (DC) rates. Here, we demonstrate the frequency upconversion of attenuated single photons, using a low-loss titanium-indiffused periodically poled lithium niobate waveguide, pumped with a readily available erbium-doped fiber amplifier in the L-band. Internal and conversion efficiencies up to 84.4% and 49.9% have been achieved, respectively. The DC rates are suppressed down to 44 kHz at 13.9% end-to-end quantum efficiency (including full conversion and detection), enabled by our long-wavelength pump configuration and narrow 3.5-GHz bandpass filtering.

Partially-reduced graphene oxide (prGO) inner-coated and fiber-calibrated Fabry-Perot dye resonator for biochemical detection enables the functionalized FRET-gain-assistance and intermode heterodyne interference, we achieve individual molecule sensitivity for dopamine, nicotine and ssDNA.

High-dimensional quantum entangled states are a highly desired resource for their extended possibilities in quantum information processing. In this paper, we introduce on-chip engineering of a variety of path-entangled states based on the simultaneous enabling of spontaneous parametric down-conversion and efficient coupling between waveguides in a quadratic coupled-waveguide system. By varying the properties of pump beams, the phase-matching conditions, and the coupling coefficients in a three-coupled-waveguide system, it is possible to generate the deterministic and robust three-path biphoton entangled states without any postprocessing, as well as to transform the output photons among different types of path entanglement. This integrated implementation of the entanglement source will become an important building block for practical applications of on-chip quantum technologies.

Photonic entanglement is central resource to quantum information sciences, such as quantum communication and quantum computation. The entangled photons generated in conventional spontaneous parametric down-conversion usually yield THz bandwidth which becomes very dim in many applications call for narrow-band entanglement sources. Here we demonstrate the polarization-entanglement photon source with counterpropagating phase matching, which results in an inherent bandwidth of 7.1 GHz at telecom wavelength. The entanglement is measured to violate the Bell inequality by up to 18.5 standard deviations, with Clauser–Horne–Shimony–Holt S-parameter of 2.720±0.039. The quantum state tomography further characterizes the entanglement, with fidelity F=(95.71±0.61)%.

The convolution layer has been the dominant feature extractor in computer vision for years. However, the spatial aggregation in convolution is basically a pattern matching process that applies fixed filters which are inefficient at modeling visual elements with varying spatial distributions. This paper presents a new image feature extractor, called the local relation layer, that adaptively determines aggregation weights based on the compositional relationship of local pixel pairs. With this relational approach, it can composite visual elements into higher-level entities in a more efficient manner that benefits semantic inference. A network built with local relation layers, called the Local Relation Network (LR-Net), is found to provide greater modeling capacity than its counterpart built with regular convolution on large-scale recognition tasks such as ImageNet classification.

We report χ(2) and χ(3) frequency up-conversion in silicon nitride microcavities. Pumped by C-/L- band, a broadband frequency conversion from 437 nm to 816 nm is obtained based on regenerative satellite comb structures, with χ(2) process supported by nitride-oxide surface symmetry breaking.

We demonstrate the first mid-infrared frequency comb generation via optical parametric down conversion from a high-Q χ(2) optical superlattice box resonator. Low noise comb is achieved with high output power.

Narrow-linewidth lasers are essential for various applications, but are limited by their size, weight, power, and cost requirements. Here we demonstrate a self-injection locked diode laser fabricated with a high quality factor fiber Fabry–Perot resonator, with a 145 Hz free-running linewidth. The locking scheme is all-fiber for plug-and-play operation. White frequency noise of 50 H z 2 / H z is measured with over 42 dB reduction from the low-cost TO-can distributed feedback laser diode, and shows its wide applications in a compact and cost-effective way.

We study the effect of dimension variation for second-harmonic generation (SHG) in lithium niobate on insulator (LNOI) waveguides. Non-trivial SHG profiles in both type-0 and type-I quasi-phase matching are observed during the wavelength tuning of the fundamental light. Theoretical modeling shows that the SHG profile and efficiency can be greatly affected by the waveguide cross-section dimension variations, especially the thickness variations. In particular, our analysis shows that a thickness variation of tens of nanometers is in good agreement with the experimental results. Such investigations could be used to evaluate fabrication performance of LNOI-based nonlinear optical devices.

We demonstrate a tunable optical parametric oscillator in a periodically poled congruently grown lithium tantalite whispering gallery mode resonator. The resonator is mechanically polished to millimeter size, and the quality factor is approximately 107 at 1064 nm. Our experiments show that this kind of resonator is capable of reaching a very low threshold and having a wide tuning range. Combined with its narrow resonant linewidth, it is potentially used as a compact, widely tunable, and narrow-linewidth infrared to mid-infrared laser source.

Multiphoton absorption (MPA) has been utilized for important technological applications. High-order multiphoton harvesting (e.g., five-photon absorption, 5PA) exhibits unique properties that could benefit biophotonics. Within this field, perovskite oxide ferroelectrics (e.g., BaTiO3 ) enable low-order optical nonlinearities of 2PA/3PA processes. However, it is challenging to obtain efficient, high-order 5PA effects. Herein, for the first time, giant and broadband MPA properties are presented in the 2D hybrid perovskite ferroelectric (IA)2 (MA)2 Pb3 Br10 (1; IA = isoamylammonium and MA = methylammonium), where multiphoton-excited optical nonlinearities related to different MPA mechanisms over a broadband range of 550-2400 nm are observed. Strikingly, its 5PA absorption cross-section (σ5 ) reaches up to 1.2 × 10-132 cm10 s4 photon-4 (at 2400 nm), almost 10 orders larger than some state-of-the-art organic molecules and a record-high value among all known ferroelectrics. This unprecedented 5PA effect results from the quantum-confined motif of inorganic trilayer sheets (wells) and organic cations (barriers) in 1. Moreover, its large ferroelectric polarization of 5 µC cm-2 could promote modulation of MPA effects under external electric fields. As far as it is known, this is the first report on giant, broadband high-order MPA properties in ferroelectrics, which provides potential, novel electric-ordered materials for next-generation biophotonic applications.

We propose a scheme for the generation of counterpropagating polarization-entangled photon pairs from a periodically poled lithium niobate on insulator waveguide. The waveguide is designed to enable a special dispersion relationship between the T M 00 and T E 00 modes that allows two concurrent counterpropagating quasi-phase-matching type-II spontaneous parametric downconversion processes with a single reciprocal wave vector. Due to the counterpropagating phase-matching geometry, the source has a narrow bandwidth in the order of several gigahertz. The compact source opens up a new method for integrated photonic technologies.

Lithium niobate on insulator (LNOI) is a unique platform for integrated photonic applications and especially for high-efficiency nonlinear frequency converters because of the strong optical field confinement. In this work, we fabricated a 6-mm-long periodically poled LNOI ridge waveguide with an optimized duty cycle (50:50) using an active domain structure monitoring method. The performance of the single-pass second-harmonic generation and difference-frequency generation in the nanophotonic waveguide was characterized, and the normalized conversion efficiencies were ∼80% of the theoretical values. These high-quality frequency conversion devices can pave the way for the application of LNOI in nonlinear integrated photonics.

Alloying in two-dimension has been a hot spot in the development of new, versatile systems of optics and electronics. Alloys have been demonstrated to be a fascinating strategy to modulate the chemical and electronic properties of two-dimensional nanosheets. We firstly reported ultra-broadband enhanced nonlinear saturable absorption of Mo0.53W0.47Te2 alloy at 0.6, 1.0, and 2.0 μm. The nonlinear saturable absorption of Mo0.53W0.47Te2 saturable absorber (SA) was measured by the open aperture Z-scan technique. Compared to MoTe2 and WTe2 SAs, the Mo0.53W0.47Te2 SA showed five times deeper modulation depth, 8.6% lower saturable intensity, and one order larger figure of merit. Thus, our research provides a method of alloys to find novel materials with more outstanding properties for optics and optoelectronic applications.

We report an observation of the second-order correlation between twin beams generated by amplified spontaneous parametric down-conversion operating above threshold with kilowatt-level peak power, from a periodically poled LiTaO3 crystal via a single-pass scheme. Photocurrent correlation was measured because of the bright photon streams, with raw visibility of 37.9% or 97.3% after electronic filtering. As expected in our theory, this correlation is robust and insensitive to parametric gain and detection loss, enabling important applications in optical communications, precision measurement, and nonlocal imaging.

We demonstrated the efficient plasmon-induced nonlinear absorption of liquid metal GaInSn nanospheres prepared by a facile liquid-phase method. With GaInSn as saturable absorbers, a passively Q-switching operation was obtained at both 1.3 and 2 μm. The pulse width of 32 ns was achieved at 1.3 μm with repetition rate of 44 kHz, single pulse energy of 51.9 μJ, and output power of 425 mW. Meanwhile, 510 ns and 92 kHz pulses with energy of 36.1 μJ and output power of 2.48 W were obtained at 2 μm. This work provides the potential of liquid metal for improving metal functions and flexible optical devices.

In this study, a single fluorescent probe (DPFP) containing a 1,8-naphthalimide dye and a homoallylamino group for imaging pH and formaldehyde (FA) has been developed that exhibits significant blue fluorescence (λem at 455 nm) under acidic pH conditions (pH < 7.0) and green fluorescence (λem at 555 nm) in the presence of FA, respectively. Furthermore, probe DPFP was successfully applied to image acidic lysosomes and exogenous or endogenous FA in living HeLa cells.

Quantum entanglement is a fundamental resource for secure information processing and communications. The canonical optical quantum information processing encodes a single qubit per photon, with remarkable demonstrations of secure quantum communications, linear optical quantum computing amongst others. Often the polarization qubit, a discrete variable with entangled Bell states, is used. Continuous variables such as energy-time modes and spatial modes, however, present a dramatically larger Hilbert space for quantum information processing. The high-dimensional entanglement capture more qubits per photon, enabling dramatically higher secure key rates over longer distances and with better error resilience. Here I will describe our results on high-dimensional entanglement in quantum frequency combs for dense quantum communications. We first demonstrate revival of the Hong-Ou-Mandel interferences, long postulated by theorists more than a decade ago, up to 19-dimensions and with visibilities up to 96.5%. The mode-locked two-photon state in high-dimensions is further witnessed through a stabilized Franson interferometer, as a generalized Bell’s inequality test and hyperentangled through multiple degrees-of-freedom. Entanglement revivals of the non-local interference at discrete time-bins are uncovered, up to 97.8% visibility, as a fundamental resource for dense secure information processing.

We report Kerr frequency combs with two types of satellites, enabled by multiple phase matching in microcavities. Satellite comb clusters at ≈ 1.3 μm and 2.0 μm regimes are simultaneously generated with the central comb, with a demonstrated high external conversion efficiency reaching up to -30dB.

We demonstrate here a compact optical parametric oscillator module for mid-infrared generation via nonlinear frequency conversion. This module weighs only 2.5 kg and fits within a small volume of 220 × 60 × 55 mm3. The module can be easily aligned to various pump laser sources, and here we use a 50 W ytterbium (Yb)-doped fiber laser as an example. With a two-channel MgO-doped periodically poled lithium niobate crystal (MgO:PPLN), our module covers a tuning range of 2416.17–2932.25 nm and 3142.18–3452.15 nm. The highest output power exceeds 10.4 W at 2.7 μm, corresponding to a conversion efficiency of 24%. The measured power stability is 2.13% Root Meat Square (RMS) for a 10 h duration under outdoor conditions.

Graphene, a unique two-dimensional material comprising carbon in a honeycomb lattice 1 , has brought breakthroughs across electronics, mechanics and thermal transport, driven by the quasiparticle Dirac fermions obeying a linear dispersion 2,3 . Here, we demonstrate a counter-pumped all-optical difference frequency process to coherently generate and control terahertz plasmons in atomic-layer graphene with octave-level tunability and high efficiency. We leverage the inherent surface asymmetry of graphene for strong second-order nonlinear polarizability 4,5 , which, together with tight plasmon field confinement, enables a robust difference frequency signal at terahertz frequencies. The counter-pumped resonant process on graphene uniquely achieves both energy and momentum conservation. Consequently, we demonstrate a dual-layer graphene heterostructure with terahertz charge- and gate-tunability over an octave, from 4.7 THz to 9.4 THz, bounded only by the pump amplifier optical bandwidth. Theoretical modelling supports our single-volt-level gate tuning and optical-bandwidth-bounded 4.7 THz phase-matching measurements through the random phase approximation, with phonon coupling, saturable absorption and below the Landau damping, to predict and understand graphene plasmon physics. An all-optical difference frequency process is exploited to generate terahertz graphene plasmons that are tunable over an octave.

Quantum entanglement is a fundamental resource for secure information processing and communications, and hyperentanglement or high-dimensional entanglement has been separately proposed for its high data capacity and error resilience. The continuous-variable nature of the energy–time entanglement makes it an ideal candidate for efficient high-dimensional coding with minimal limitations. Here, we demonstrate the first simultaneous high-dimensional hyperentanglement using a biphoton frequency comb to harness the full potential in both the energy and time domain. Long-postulated Hong–Ou–Mandel quantum revival is exhibited, with up to 19 time-bins and 96.5% visibilities. We further witness the high-dimensional energy–time entanglement through Franson revivals, observed periodically at integer time-bins, with 97.8% visibility. This qudit state is observed to simultaneously violate the generalized Bell inequality by up to 10.95 standard deviations while observing recurrent Clauser–Horne–Shimony–Holt S-parameters up to 2.76. Our biphoton frequency comb provides a platform for photon-efficient quantum communications towards the ultimate channel capacity through energy–time–polarization high-dimensional encoding., United States. Defense Advanced Research Projects Agency. Information in a Photon (InPho) Program (Contract W911NF-10-1-0416)

The MoS 2 /Graphene heterojunction prepared through a facile hydrothermal method is used as an optical modulator to realize 2.8 μm passively Q-switched solid state pulse laser for the first time as far as we know. This work certifies that the two-dimensional material heterojunction is a kind of outstanding mid-infrared modulators.

We demonstrate a widely-tunable mid-infrared optical parametric oscillator in a monolithic periodically poled lithium Tantalate whispering-gallery-mode resonator. Low-threshold oscillation is achieved with 57.6% slope efficiency, covering the spectral range from 1.7 to 2.85μm.

We demonstrate a single-photon SWAP gate between polarization and spatial momentum on a SOI chip. 19.8% error ratio is obtained, and phase coherence of the SWAP operation is measured via single photon interference with up to 58.7% visibility.

Multipartite quantum entanglement is a powerful resource for enriching the functionality of quantum computation and quantum communication. In this Letter, we propose a new method to generate a two-photon multipath Dicke state with concurrent spontaneous parametric downconversion processes from a single periodically poled nonlinear photonic crystal. We design the poling structure to produce a three-path Dicke state where three quasi-phase-matching conditions are fulfilled simultaneously by a hybrid one- and two-dimensionally poled nonlinear photonic crystal. We use genuine multipartite entanglement concurrence to quantify the entanglement of the Dicke state. Using a more complicated poling configuration like multiple-periodically poled two-dimensional nonlinear photonic crystal, we can also produce four-path, five-path, or multipath Dicke states by a single crystal. The multiple-periodically poled two-dimensional nonlinear photonic crystal provides a new method, to the best of our knowledge, for the integrated generation of multipartite quantum light sources.

Due to the composition-dependent properties of two-dimensional (2D) transition metal dichalcogenides (TMDs), alloying of existing dissimilar TMDs architecture is a novel and controllable route to tailor crystal structures with superior optical and optoelectronic properties. Here, we reported the hexagonal-phase WSe1.4Te0.6 alloy can enable great promise for enhanced saturable absorption response exceeding the parent component WSe2 and WTe2, with larger modulation depth and lower saturable intensity. These advantages allowed the 1064 nm passively Q-switched lasers based on WSe1.4Te0.6 to be more efficient, with pulse duration narrowed to 45%, and slope efficiency increased by 232%. Our findings highlighted the appropriate alloying of TMDs as an effective strategy for development of saturable absorbers.

We theoretically study the propagation dynamics of input light in one-dimensional mixed linear-nonlinear photonic lattices with a complex parity-time symmetric potential. Numerical computation shows simultaneous localization and steering of the optical beam due to the asymmetric scatter and interplay between Kerr-type nonlinearity and PT symmetry. This may provide a feasible measure for manipulation light in optical communications, integrated optics and so on.

We demonstrate a method to substantially increase the observation duty ratio in temporal-magnification system without sacrificing the temporal resolution. 30% or even 100% observation duty ratio can be achieved on a 10-ns or longer waveform.

We demonstrate a graphene-alumina-graphene heterostructured semiconductor chip, on which THz plasmons are generated via backward phase-matched 2nd nonlinearity all-optically. The on-chip plasmons are effectively gate tunable, with photon-efficiency ∼10−4, and Q factor > 60.

We report the first correlation measurement between the twin beams generated by optical parametric process above threshold. This high-visibility correlation can be observed at significant power levels with up to a conversion efficiency of 19.7%.

We demonstrate a high efficiency mid-infrared laser source based on optical parametric oscillator (OPO) assisted by an intracavity optical parametric amplification (OPA). The OPA-assisted-OPO scheme was realized in one piece of commensurable dual-periodic superlattice in which the signal light generated from the OPO process serves as the pump light for the OPA process. A maximum output power of 508 mW at 3.92 μm was achieved under a pump power of 2.85 W at 1.064 μm. The pump-to-idler conversion efficiency is 17.8% and the slope efficiency is 23.8%, and the enhancements of them are 58.9% and 67.6%, respectively, comparing with the standard OPO scheme.

WTe2 is a unique material in the family of transition metal dichalcogenides and it has been proposed as a candidate for type-II Weyl semimetals. However, thus far, studies on the optical properties of this emerging material have been significantly hindered by the lack of large-area, high-quality WTe2 materials. Here, we grow a centimeter-scale, highly crystalline WTe2 ultrathin film (∼35 nm) by a pulsed laser deposition technique. Broadband pump-probe spectroscopy (1.2–2.5 μm) reveals a peculiar ultrafast optical response where an initial photo-bleaching signal (lasting ∼3 ps) is followed by a long-lived photoinduced absorption signature. Nonlinear absorption characterization using femtosecond pulses confirms the saturable absorption response of the WTe2 ultrathin films, and we further demonstrated a mode-locked Thulium fiber laser using a WTe2 absorber. Our work provides important insights into linear and nonlinear optical responses of WTe2 thin films.

We report the fabrication of an MoS2 black phosphorus (BP) composite saturable absorber by liquid phase exfoliation and the spin-coating method and further exploitation to build a 2 μm passively Q-switched Tm:YAP laser. Such a composite based Q-switched laser with a duration of 488 ns and corresponding peak power of 85.9 W is obtained, which shows an improved saturable absorption effect than that of single MoS2 (616 ns, 68.7 W) and BP (932 ns, 22.4 W). The results indicate that simple and reasonable fabrication of the vertical composite from two-dimensional atomic layer materials opens up the possibility to create an unprecedented saturable absorber with exciting properties.