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The past two decades witnessed important developments in the field of non-equilibrium statistical mechanics. Among these developments, the Jarzynski equality, being a milestone following the landmark work of Clausius and Kelvin, stands out. The Jarzynski equality relates the free energy difference between two equilibrium states and the work done on the system through far from equilibrium processes. While experimental tests of the equality have been performed in classical regime, the verification of the quantum Jarzynski equality has not yet been fully demonstrated due to experimental challenges. Here, we report an experimental test of the quantum Jarzynski equality with a single \Yb ion trapped in a harmonic potential. We perform projective measurements to obtain phonon distributions of the initial thermal state. Following that we apply the laser induced force on the projected energy eigenstate, and find transition probabilities to final energy eigenstates after the work is done. By varying the speed of applying the force from equilibrium to far-from equilibrium regime, we verified the quantum Jarzynski equality in an isolated system., Comment: 18 pages, 4 figures, 1 table

Quantum mechanical particles in a confining potential interfere with each other while undergoing thermodynamic processes far from thermal equilibrium. By evaluating the corresponding transition probabilities between many-particle eigenstates we obtain the quantum work distribution function, for identical Bosons and Fermions, which we compare with the case of distinguishable particles. We find that the quantum work distributions for Bosons and Fermions significantly differ at low temperatures, while, as expected, at high temperatures the work distributions converge to the classical expression. These findings are illustrated with two analytically solvable examples, namely the time-dependent infinite square well and the parametric harmonic oscillator., Comment: 17 pages, 9 figures; published version

We study the maximum efficiency of a Carnot cycle heat engine based on a small system. It is revealed that due to the finiteness of the system, irreversibility may arise when the working substance contacts with a heat bath. As a result, there is a working-substance-dependent correction to the usual Carnot efficiency, which is valid only when the working substance is in the thermodynamic limit. We derives a general and simple expression for the maximum efficiency of a Carnot cycle heat engine in terms of the relative entropy. This maximum efficiency approaches the usual Carnot efficiency asymptotically when the size of the working substance increases to the thermodynamic limit. Our study extends the Carnot's result to cases with arbitrary size working substance and demonstrates the subtlety of thermodynamics in small systems., Comment: 5 pages, 3 figures. References and supplemental material added. Parts of the manuscript rewritten

We describe a simple and solvable model of a device that -- like the "neat-fingered being" in Maxwell's famous thought experiment -- transfers energy from a cold system to a hot system by rectifying thermal fluctuations. In order to accomplish this task, our device requires a memory register to which it can write information: the increase in the Shannon entropy of the memory compensates the decrease in the thermodynamic entropy arising from the flow of heat against a thermal gradient. We construct the nonequilibrium phase diagram for this device, and find that it can alternatively act as an eraser of information. We discuss our model in the context of the second law of thermodynamics., Comment: 9 pages (Main Text + Supplemental Material), 3 figures, to appear in Physical Review Letters

This is a reply to the comment from Patrick Bruno (arXiv:1211.4792) on our paper (Phys. Rev. Lett. 109, 163001 (2012)).

Spontaneous symmetry breaking can lead to the formation of time crystals, as well as spatial crystals. Here we propose a space-time crystal of trapped ions and a method to realize it experimentally by confining ions in a ring-shaped trapping potential with a static magnetic field. The ions spontaneously form a spatial ring crystal due to Coulomb repulsion. This ion crystal can rotate persistently at the lowest quantum energy state in magnetic fields with fractional fluxes. The persistent rotation of trapped ions produces the temporal order, leading to the formation of a space-time crystal. We show that these space-time crystals are robust for direct experimental observation. We also study the effects of finite temperatures on the persistent rotation. The proposed space-time crystals of trapped ions provide a new dimension for exploring many-body physics and emerging properties of matter., Comment: updated to the version published in PRL

Recent work by Teifel and Mahler [Eur. Phys. J. B 75, 275 (2010)] raises legitimate concerns regarding the validity of quantum nonequilibrium work relations in processes involving moving hard walls. We study this issue in the context of the rapidly expanding one-dimensional quantum piston. Utilizing exact solutions of the time-dependent Schrodinger equation, we find that the evolution of the wave function can be decomposed into static and dynamic components, which have simple semiclassical interpretations in terms of particle-piston collisions. We show that nonequilibrium work relations remains valid at any finite piston speed, provided both components are included, and we study explicitly the work distribution for this model system., Comment: 16 pages, 4 figures

The radical-pair-based chemical reaction could be used by birds for the navigation via the geomagnetic direction. An inherent physical mechanism is that the quantum coherent transition from a singlet state to triplet states of the radical pair could response to the weak magnetic field and be sensitive to the direction of such a field and then results in different photopigments in the avian eyes to be sensed. Here, we propose a quantum bionic setup for the ultra-sensitive probe of a weak magnetic field based on the quantum phase transition of the environments of the two electrons in the radical pair. We prove that the yield of the chemical products via the recombination from the singlet state is determined by the Loschmidt echo of the environments with interacting nuclear spins. Thus quantum criticality of environments could enhance the sensitivity of the detection of the weak magnetic field., Comment: 4 pages, 3 figures

Based on a microscopic model, we study the interplay between superconductivity and antiferromagnetism in a multi-layered system, where two superconductors are separated by an antiferromagnetic region. Within a self-consistent mean-field theory, this system is solved numerically. We find that the antiferromagnetism in the middle layers profoundly affects the supercurrent flowing across the junction, while the phase difference across the junction influences the development of antiferromagnetism in the middle layers. This study may not only shed new light on the mechanism for high-$T_{c}$ superconductors, but also bring important insights to building Josephson-junction-based quantum devices, such as SQUID and superconducting qubit., Comment: 4+ pages, 5 figures, Accepted for publication in Phys. Rev. B

Adiabaticity of quantum evolution is important in many settings. One example is the adiabatic quantum computation. Nevertheless, up to now, there is no effective method to test the adiabaticity of the evolution when the eigenenergies of the driven Hamiltonian are not known. We propose a simple method to check adiabaticity of a quantum process for an arbitrary quantum system. We further propose a operational method for finding a uniformly adiabatic quench scheme based on Kibble-Zurek mechanism for the case when the initial and the final Hamiltonians are given. This method should help in implementing adiabatic quantum computation., Comment: This is a new version. Some typos in the New Journal of Physics version have been corrected

We study decoherence induced by a dynamic environment undergoing a quantum phase transition. Environment's susceptibility to perturbations - and, consequently, efficiency of decoherence - is amplified near a critical point. Over and above this near-critical susceptibility increase, we show that decoherence is dramatically enhanced by non-equilibrium critical dynamics of the environment. We derive a simple expression relating decoherence to the universal critical exponents exhibiting deep connections with the theory of topological defect creation in non-equilibrium phase transitions., Comment: 8 pages; version accepted in PRA

Quantum Darwinism provides an information-theoretic framework for the emergence of the objective, classical world from the quantum substrate. The key to this emergence is the proliferation of redundant information throughout the environment where observers can then intercept it. We study this process for a purely decohering interaction when the environment, E, is in a non-ideal (e.g., mixed) initial state. In the case of good decoherence, that is, after the pointer states have been unambiguously selected, the mutual information between the system, S, and an environment fragment, F, is given solely by F's entropy increase. This demonstrates that the environment's capacity for recording the state of S is directly related to its ability to increase its entropy. Environments that remain nearly invariant under the interaction with S, either because they have a large initial entropy or a misaligned initial state, therefore have a diminished ability to acquire information. To elucidate the concept of good decoherence, we show that - when decoherence is not complete - the deviation of the mutual information from F's entropy change is quantified by the quantum discord, i.e., the excess mutual information between S and F is information regarding the initial coherence between pointer states of S. In addition to illustrating these results with a single qubit system interacting with a multi-qubit environment, we find scaling relations for the redundancy of information acquired by the environment that display a universal behavior independent of the initial state of S. Our results demonstrate that Quantum Darwinism is robust with respect to non-ideal initial states of the environment: the environment almost always acquires redundant information about the system but its rate of acquisition can be reduced., Comment: 16 pages, 9 figures

We study the phase diagram of a superconducting ring threaded by an Aharonov-Bohm flux and an in-plane magnetic Zeeman field. The simultaneous presence of both the external flux and the in-plane magnetic field leads to the competition between the Fulde-Ferrell (FF) phase and the Larkin-Ovchinnikov (LO) phase. Using the Bogoliubov-de Gennes equation, we investigate the spacial profile of the order parameter. Both the FF phase and the LO phase are found to exist stably in this system. The phase boundary is determined by comparing the free energy. The distortion of the phase diagrams due to the mesoscopic effect is also studied., Comment: 6 pages, 4 figures

Quantum Darwinism recognizes that we - the observers - acquire our information about the "systems of interest" indirectly from their imprints on the environment. Here, we show that information about a system can be acquired from a mixed-state, or hazy, environment, but the storage capacity of an environment fragment is suppressed by its initial entropy. In the case of good decoherence, the mutual information between the system and the fragment is given solely by the fragment's entropy increase. For fairly mixed environments, this means a reduction by a factor 1-h, where h is the haziness of the environment, i.e., the initial entropy of an environment qubit. Thus, even such hazy environments eventually reveal the state of the system, although now the intercepted environment fragment must be larger by ~1/(1-h) to gain the same information about the system., Comment: 4 pages, 3 figures

We consider the quantum mechanical generalization of Crooks Fluctuation Theorem and Jarzynski Equality for an open quantum system. The explicit expression for microscopic work for an arbitrary prescribed protocol is obtained, and the relation between quantum Crooks Fluctuation Theorem, quantum Jarzynski Equality and their classical counterparts are clarified. Numerical simulations based on a two-level toy model are used to demonstrate the validity of the quantum version of the two theorems beyond linear response theory regime., Comment: 6 pages, 3 figures, any comments are welcome

We study the quantum mechanical generalization of force or pressure, and then we extend the classical thermodynamic isobaric process to quantum mechanical systems. Based on these efforts, we are able to study the quantum version of thermodynamic cycles that consist of quantum isobaric process, such as quantum Brayton cycle and quantum Diesel cycle. We also consider the implementation of quantum Brayton cycle and quantum Diesel cycle with some model systems, such as single particle in 1D box and single-mode radiation field in a cavity. These studies lay the microscopic (quantum mechanical) foundation for Szilard-Zurek single molecule engine., Comment: 9 pages, 5 figures

We study the quantum fidelity approach to characterize thermal phase transitions. Specifically, we focus on the mixed-state fidelity induced by a perturbation in temperature. We consider the behavior of fidelity in two types of second-order thermal phase transitions (based on the type of non-analiticity of free energy), and we find that usual fidelity criteria for identifying critical points is more applicable to the case of $\lambda$ transitions (divergent second derivatives of free energy). Our study also reveals limitations of the fidelity approach: sensitivity to high temperature thermal fluctuations that wash out information about the transition, and inability of fidelity to distinguish between crossovers and proper phase transitions. In spite of these limitations, however, we find that fidelity remains a good pre-criterion for testing thermal phase transitions, which we use to analyze the non-zero temperature phase diagram of the Lipkin-Meshkov-Glick model.

We study the magnetic susceptibility of 1D quantum XY model, and show that when the temperature approaches zero, the magnetic susceptibility exhibits the finite-temperature scaling behavior. This scaling behavior of the magnetic susceptibility in 1D quantum XY model, due to the quantum-classical mapping, can be easily experimentally tested. Furthermore, the universality in the critical properties of the magnetic susceptibility in quantum XY model is verified. Our study also reveals the close relation between the magnetic susceptibility and the geometric phase in some spin systems, where the quantum phase transitions are driven by an external magnetic field., Comment: 6 pages, 4 figures, get accepted for publication by J. Phys. A: Math. Theor

For a two-level quantum mechanical system, we derive microscopically the exact expression for the fluctuation of microscopic work in a multi-step non-equilibrium process, and we rigorously prove that in an isothermal process, the fluctuation is vanishingly small, and the most probabilistic work just equals to the difference of the free energy. Our study demonstrates that the convergence of the microscopic work in the isothermal process is due to the nature of isothermal process rather than usual thermodynamic limit condition. Our investigation justifies the validity of "minimum work principle" formulation of the second law even for a small system far from thermodynamic limit., Comment: LAUR 08-2152, 5 pages, 2 figures

We explore a dynamic signature of quantum phase transition (QPT) in an isotropic Lipkin-Meshkov-Glick (LMG) model by studying the time evolution of a central qubit coupled to it. We evaluate exactly the time-dependent purity, which can be used to measure quantum coherence, of the central qubit. It is found that distinctly different behaviors of the purity as a function of the parameter reveal clearly the QPT point in the system. It is also clarified that the present model is equivalent to an anti Jaynes-Cummings model under certain conditions., Comment: 8 pages, 4 figures

We extend to finite temperature the fidelity approach to quantum phase transitions (QPTs). This is done by resorting to the notion of mixed-state fidelity that allows one to compare two density matrices corresponding to two different thermal states. By exploiting the same concept we also propose a finite-temperature generalization of the Loschmidt echo. Explicit analytical expressions of these quantities are given for a class of quasi-free fermionic Hamiltonians. A numerical analysis is performed as well showing that the associated QPTs show their signatures in a finite range of temperatures., Comment: 7 pages, 4 figures

In order to describe quantum heat engines, here we systematically study isothermal and isochoric processes for quantum thermodynamic cycles. Based on these results the quantum versions of both the Carnot heat engine and the Otto heat engine are defined without ambiguities. We also study the properties of quantum Carnot and Otto heat engines in comparison with their classical counterparts. Relations and mappings between these two quantum heat engines are also investigated by considering their respective quantum thermodynamic processes. In addition, we discuss the role of Maxwell's demon in quantum thermodynamic cycles. We find that there is no violation of the second law, even in the existence of such a demon, when the demon is included correctly as part of the working substance of the heat engine., Comment: 17 pages, 9 figures, 4 tables

Cavity quantum electrodynamic (QED) is studied for two strongly-coupled charge qubits interacting with a single-mode quantized field, which is provided by a on-chip transmission line resonator. We analyze the dressed state structure of this superconducting circuit QED system and the selection rules of electromagnetic-induced transitions between any two of these dressed states. Its macroscopic quantum criticality, in the form of ground state level crossing, is also analyzed, resulting from competition between the Ising-type inter-qubit coupling and the controllable on-site potentials., Comment: 4 pages, 3 figures

We propose a quantum analog of the internal combustion engine used in most cars. Specifically, we study how to implement the Otto-type quantum heat engine (QHE) with the assistance of a Maxwell's demon. Three steps are required: thermalization, quantum measurement, and quantum feedback controlled by the Maxwell demon. We derive the positive-work condition of this composite QHE. Our QHE can be constructed using superconducting quantum circuits. We explicitly demonstrate the essential role of the demon in this macroscopic QHE., Comment: 4 pages, 2 figures

We study the transition of a quantum system $S $ from a pure state to a mixed one, which is induced by the quantum criticality of the surrounding system $E$ coupled to it. To characterize this transition quantitatively, we carefully examine the behavior of the Loschmidt echo (LE) of $E$ modelled as an Ising model in a transverse field, which behaves as a measuring apparatus in quantum measurement. It is found that the quantum critical behavior of $E$ strongly affects its capability of enhancing the decay of LE: near the critical value of the transverse field entailing the happening of quantum phase transition, the off-diagonal elements of the reduced density matrix describing $S$ vanish sharply., Comment: 4 pages, 3 figures

We study the physical implementation of the Photon Carnot engine (PCE) based on the cavity QED system [M. Scully et al, Science, \textbf{299}, 862 (2003)]. Here, we analyze two decoherence mechanisms for the more practical systems of PCE, the dissipation of photon field and the pure dephasing of the input atoms. As a result we find that (I) the PCE can work well to some extent even in the existence of the cavity loss (photon dissipation); and (II) the short-time atomic dephasing, which can destroy the PCE, is a fatal problem to be overcome., Comment: 6 pages, 3 figures

By reformulating the first law of thermodynamics in the fashion of quantum-mechanical operators on the parameter manifold, we propose a universal class of quantum heat engines (QHE) using the multi-level quantum system as the working substance. We obtain a general expression of work for the thermodynamic cycle with two thermodynamic adiabatic processes, which are microscopically quantum adiabatic processes. We also classify the conditions for a 3-level QHE to extract positive work from a heat bath. Our result is counter-intuitively different from that of a 2-level system. As a more realistic illustration, a 3-level atom system with dark state configuration manipulated by classical light is used to demonstrate our central idea., Comment: 10 pages, 11 figures

We, based on the photoassociation of fermion atoms into bosonic molecules, propose a scheme to create the steady entanglement between the atom state and the molecule state inside an optical lattice. The stability of entanglement state is guaranteed by sweeping the frequency of Ramman laser beam through resonance according to the second Demkov-Kunike (DK2) nonadiabatic transition model\cite{DK,models}. The probability amplitude of each components can be precisely controlled by adjusting the sweeping parameter., Comment: 5 pages, 4 figures