Search

From August 13 to September 25, the Southern African Regional Science Initiative's (SAFARI 2000) dry-season airborne campaign studied the complex interactions between the region's ecosystems, air pollution, atmospheric circulation, land-atmosphere interactions, and land use change. The field campaign was timed to coincide with the annual winter fire season in Southern Africa. This challenging campaign. which coordinated ground-based measurement teams, multiple research aircraft, and satellite overpasses across nine African nations, was head quartered at the Petersburg International Airport in South Africa's Northern Province. Among many others, unique coordinated observations were made of the evolution of massive, thick haze layers produced by industrial emissions, biomass burning, marine and biogenic sources. The NASA Ames Airborne Tracking 14-channel Sunphotometer (AATS-14) was operated successfully aboard the University of Washington CV-580 during 24 data flights. The AATS-14 instrument measures the transmission of the direct solar beam at 14 discrete wavelengths (3501558 nm) from which we derive spectral aerosol optical depths (AOD), columnar water vapor (CWV) and columnar ozone. Flying at different altitudes over a fixed location allows derivation of layer AOD and CWV. Data taken during feasible vertical profiles allows derivation of aerosol extinction and water vapor density. In the talk, we show comparisons with ground-based AERONET sun/sky photometer results, with ground based MPL-Net lidar data, and with measurements from a lidar aboard the high flying ER-2 aircraft. We will use measurements from the Ames Solar Spectral Flux Radiometer to derive estimates of solar spectral forcing as a function of aerosol thickness. Validations of TOMS and Terra satellite aerosol and water-vapor retrievals will also be discussed.

In the Spring 2001 phase of the Asian Pacific Regional Aerosol Characterization Experiment (ACE-Asia), the 6-channel NASA Ames Airborne Tracking Sunphotometer (AATS-6) operated on 15 of the 19 research flights of the NCAR C-130, while its 14-channel counterpart (AATS- 14) flew successfully on all 18 research flights of the CIRPAS Twin Otter. ACE-Asia studied aerosol outflow from the Asian continent to the Pacific basin. It was designed to integrate suborbital and satellite measurements and models so as to reduce the uncertainty in calculations of the climate forcing due to aerosols. AATS-6 and AATS-14 measured solar beam transmission at 6 and 14 wavelengths (380-1021 and 354-1558 nm, respectively), yielding aerosol optical depth (AOD) spectra and column water vapor (CWV). Vertical differentiation in profiles yielded aerosol extinction spectra and water vapor concentration. The wavelength dependence of these AOD and extinction spectra indicates that supermicron dust was often a major component of the ACE-Asia aerosol. Frequently this dust-containing aerosol extended to high altitudes. For example, in AATS- 14 profiles analyzed to date, 36% of full-column AOD at 525 nm was above 3 km. In contrast, only 10% of CWV was above 3 km. Analyses and applications of AATS-6 and AATS-14 data to date include comparisons to (i) extinction products derived using in situ measurements, (ii) extinction profiles derived from lidar measurements, and (iii) AOD retrievals from the Multi-angle Imaging Spectro-Radiometer (MISR) aboard the TERRA satellite. Other planned collaborative studies include comparisons to results from size spectrometers, chemical measurements, other satellite sensors, flux radiometers, and chemical transport models. Early results of these studies will be presented.

Belmiloud, et al have recently suggested that the HITRAN line intensities in the 1130 nm water vapor band are much too weak. Giver, et at corrected unit conversion errors to make the HITRAN intensities compatible with the original measurements of Mandin, et al, but Belmiloud, et al believe that many of those line intensity measurements were too weak, and they propose the total intensity of the 1130 nm water vapor band is 38% stronger than the sum of the HITRAN line intensities in this region. We have made independent assessments of this proposal using 2 spectra obtained with the Ames 25 meter base path White cell. The first was made using the moderate resolution (8 nm) solar spectral flux radiometer (SSFR) flight instrument with a White cell absorbing path of 506 meters and 10 torr water vapor pressure. Modeling this spectrum using the HITRAN linelist gives a reasonable match, and the model is not compatible when the HITRAN line intensities are increased by 38%. The second spectrum was obtained with a White cell path of 1106 meters and 12 torr water vapor pressure, using a Bomem FTIR with near Doppler width resolution. This spectrum is useful for measuring intensities of isolated weak lines to compare with the measurements of Mandin, et al. Unfortunately, as Belmiloud et al point out, at these conditions the strong lines are much too saturated for good intensity measurements. Our measurements of the weak lines are in reasonable agreement with those of Mandin, et al. Neither of our spectra supports the proposal of Belmiloud et al for a general 38% increase of the absorption intensity in the 1130 nm water vapor band.

During the Puerto Rico Dust Experiment (PRIDE) upwelling and downwelling solar spectral irradiance was measured on board the SPAWAR Navajo and downwelling solar spectral flux was measured at a surface site using the NASA Ames Solar Spectral Flux Radiometer. These data will be used to determine the net solar radiative forcing of dust aerosol and to quantify the solar spectral radiative energy budget in the presence of elevated aerosol loading. We will assess the variability in spectral irradiance using formal principal component analysis procedures and relate the radiative variability to aerosol microphysical properties. Finally, we will characterize the sea surface reflectance to improve aerosol optical depth retrievals from the AVHRR satellite and to validate SeaWiFS ocean color products.

Moderate resolution spectra of the downwelling solar irradiance at the ground in north central Oklahoma were measured during the Department of Energy Atmospheric Radiation Measurement Program Intensive Observation Period in the fall of 1997. Spectra obtained under cloud-free conditions were compared with calculations using a coarse resolution radiative transfer model to examine the dependency of model-measurement bias on water vapor. It was found that the bias was highly correlated with water vapor and increased at a rate of 9 Wm(exp -2) per cm of water. The source of the discrepancy remains undetermined because of the complex dependencies of other variables, most notably aerosol optical depth, on water vapor.

We deployed a suite of ground-based remote sensing instruments - SMART (Surface Measurements for Atmospheric Radiative Transfer), at the Roosevelt Road Naval Station in Puerto Rico during the Puerto Rico Dust Experiment (PRIDE). The instruments include several solar and infrared broadband radiometers, a sunphotometer, a shadow-band radiometer, a micro-pulse lidar, a total-sky imager, a microwave radiometer, and two solar spectrometers. These radiometers were set up on a mobile platform and a solar tracker. During 27 June - 23 July, about 25 days of data were acquired under partially cloudy sky conditions. The diurnal air temperature was fluctuating around 28.6 C to within a few degrees. Daytime average of solar irradiance reaching at the surface was ranged from about 400 W/sq m on a rainy day to about 640 W/sq m on a cloud-free day. The infrared irradiance at the surface during the measurement period was averaged about 408 W/sq m. The heights of boundary layer, dusts and clouds were captured by lidar images. Based on sunphotometer and shadow-band radiometer retrievals, the aerosol optical thickness varied from below 0.1 to over 0.6. Combining with radiative transfer modeling and other in-situ and remote sensing measurements, our ground-based measurements provide vital information on understanding the long-range transport of African dust into the Caribbean.

A new technique to retrieve cloud optical depth for broken clouds above green vegetation using ground-based zenith radiance measurements is developed. By analogy with the Normalized Difference Vegetation Index NDVI), the Normalized Difference Cloud Index (NDCI) is defined as a ratio between the difference and the sum of two zenith radiances measured for two narrow spectral bands in the visible and near-IR regions. The very different spectral behavior of cloud liquid water drops and green vegetation is the key physics behind the NDCI. It provides extra tools to remove the radiative effects of the 3D cloud structure. Numerical calculations based on fractal clouds and real measurements of NDCI and cloud liquid water path confirm the improvements.

During the Subsonic Contrail and Cloud Effect Special Study (SUCCESS) a Solar Spectral Flux Radiometer was deployed at the surface in a zenith observing position. The instrument measured the solar spectral downwelling irradiance between 350 and 2500 nm with 10 nm resolution. From April 12 through April 29 approximately 18000 spectra were acquired, under a variety of meteorological conditions including cloud free, cirrus, Stearns, and cumulonimbus clouds. This study focuses on the effect of cirrus and cirrus contrails on the spectral distribution of solar irradiance at the surface and on inferring cirrus properties from their spectral transmittance. The observations have also proven to be useful for comparing the solar spectral irradiance measurements with model predictions, and in particular, for inferring the amount of solar radiation absorbed in the clear and cloudy atmosphere.

The impact of cirrus clouds on climate is an issue of research interest currently. Whether cirrus clouds heat or cool the Earth-atmosphere system depends on the cloud shortwave albedo and infrared reflectance and absorptance. These in turn are determined by the size distribution, phase, and composition of particles in the clouds. The TOGA-COARE campaign presented an excellent opportunity to study cirrus clouds and their influence on climate. In this campaign, a microphysics instrument package was flown aboard the DC-8 aircraft at medium altitudes in cirrus clouds. This package included a 2D Greyscale Cloud Particle Probe, a Forward Scattering Spectrometer Aerosol Probe, and an ice crystal replicator. At the same time the ER-2 equipped with a radiation measurement system flew coordinated flight tracks above the DC-8 at very high altitude. The radiation measurement made were short and long wave fluxes, as well as narrowband fluxes, both upwelling and downwelling. In addition LIDAR data is available. The existence of these data sets allows for a the comparison of radiation measurement with microphysical measurements. For example, the optical depth and effective radius retrieved from the ER-2 radiation measurements can be compared to the microphysical data. Conversely, the optical properties and fluxes produced by the clouds can be calculated from the microphysical measurements and compared to those measured aboard the ER-2. The assumptions required to make these comparisons are discussed. Typical microphysical results show a prevalence of micron-sized particles, in addition to the cloud particles that exceed 100 mm. The large number of small particles or "haze" cause the effective cloud radii to shift to smaller sizes, leading to changes in optical parameters.

The Ames airborne tracking sunphotometer was operated at the National Oceanic and Atmospheric Administration (NOAA) Mauna Loa Observatory (MLO) in 1991 and 1992 along with the NOAA Climate Monitoring and Diagnostics Laboratory (CMDL) automated tracking sunphotometer and lidar. June 1991 measurements provided calibrations, optical-depth spectra, and intercomparisons under relatively clean conditions; later measurements provided spectra and comparisons for the Pinatubo cloud plus calibration checks. June 1991 results are similar to previous MLO springtime measurements, with midvisible particle optical depth tau(sub p)(lambda = 0.526 microns) at the near-background level of 0.012 +/- 0.006 and no significant wavelength dependence in the measured range (lambda = 0.38 to 1.06 microns). The arrival of the Pinatubo cloud in July 1991 increased midvisible particle optical depth by more than an order of magnitude and changed the spectral shape of tau(sub p)(lambda) to an approximate power law with an exponent of about -1.4. By early September 1991, the spectrum was broadly peaked near 0.5 microns, and by July 1992, it was peaked near 0.8 microns. Our optical-depth spectra include corrections for diffuse light which increase postvolcanic midvisible tau(sub p) values by 1 to 3% (i.e., 0.0015 to 0.0023). NOAA- and Ames Research Center (ARC)-measured spectra are in good agreement. Columnar size distributions inverted from the spectra show that the initial (July 1991) post-Pinatubo cloud was relatively rich in small particles (r less than 0.25 microns), which were progressively depleted in the August-September 1991 and July 1992 periods. Conversely, both of the later periods had more of the optically efficient medium-sized particles (0.25 less than r less than 1 micron) than did the fresh July 1991 cloud. These changes are consistent with particle growth by condensation and coagulation. The effective, or area-weighted, radius increased from 0.22 +/- 0.06 micron in July 1991 to 0.56 +/- 0.12 micron in August-September 1991 and to 0.86 +/- 0.29 micron in July 1992. Corresponding column mass values were 4.8 +/- 0.7, 9.1 +/- 2.7, and 5.5 +/- 2 micro g/sq cm, and corresponding column surface areas were 4.4 +/- 0.5, 2.9 +/- 0.2, and 1.1 +/- 0.1 sq micron/sq cm,. Photometer-inferred column backscatter values agree with those measured by the CMDL lidar on nearby nights. Combining lidar-measured backscatter profiles with photometer-derived backscatter-to-area ratios gives peak particle areas that could cause rapid heterogeneous loss of ozone, given sufficiently low particle acidity and suitable solar zenith angles (achieved at mid- to high latitudes). Top-of-troposphere radiative forcings for the September 1991 and July 1992 optical depths and size distributions over MLO are about -5 and -3 W 1/sq m, respectively (hence comparable in magnitude but opposite in sign to the radiative forcing caused by the increase in manmade greenhouse gases since the industrial revolution). Heating rates in Pinatubo layer over MLO are 0.55 +/- 0.13 and 0.41 +/- 0.14 K/d for September 1991 and July 1992, respectively.