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Quantum simulators are controllable quantum systems that can reproduce the dynamics of the system of interest, which are unfeasible for classical computers. Recent developments in quantum technology enable the precise control of individual quantum particles as required for studying complex quantum systems. Particularly, quantum simulators capable of simulating frustrated Heisenberg spin systems provide platforms for understanding exotic matter such as high-temperature superconductors. Here we report the analog quantum simulation of the ground-state wavefunction to probe arbitrary Heisenberg-type interactions among four spin-1/2 particles . Depending on the interaction strength, frustration within the system emerges such that the ground state evolves from a localized to a resonating valence-bond state. This spin-1/2 tetramer is created using the polarization states of four photons. The single-particle addressability and tunable measurement-induced interactions provide us insights into entanglement dynamics among individual particles. We directly extract ground-state energies and pair-wise quantum correlations to observe the monogamy of entanglement.

Entangled photons are a crucial resource for quantum communication and linear optical quantum computation. Unfortunately, the applicability of many photon-based schemes is limited due to the stochastic character of the photon sources. Therefore, a worldwide effort has focused in overcoming the limitation of probabilistic emission by generating two-photon entangled states conditioned on the detection of auxiliary photons. Here we present the first heralded generation of photon states that are maximally entangled in polarization with linear optics and standard photon detection from spontaneous parametric down-conversion. We utilize the down-conversion state corresponding to the generation of three photon pairs, where the coincident detection of four auxiliary photons unambiguously heralds the successful preparation of the entangled state. This controlled generation of entangled photon states is a significant step towards the applicability of a linear optics quantum network, in particular for entanglement swapping, quantum teleportation, quantum cryptography and scalable approaches towards photonics-based quantum computing.

We report the first experimental generation and characterization of a six-photon Dicke state. The produced state shows a fidelity of F=0.56+/-0.02 with respect to an ideal Dicke state and violates a witness detecting genuine six-qubit entanglement by four standard deviations. We confirm characteristic Dicke properties of our resource and demonstrate its versatility by projecting out four- and five-photon Dicke states, as well as four-photon GHZ and W states. We also show that Dicke states have interesting applications in multiparty quantum networking protocols such as open-destination teleportation, telecloning and quantum secret sharing., Comment: 4 pages, 4 figures, RevTeX4

We present a scheme, based only on linear optics and standard photon detection, that allows to generate heralded multiphoton entangled states of arbitrary photon number from spontaneous parametric downconversion (PDC) in the weak interaction regime. The scheme also works in the strong interaction regime, i.e., for the production of large photon numbers, when photon-number resolving detectors with nearly perfect quantum efficiency are used. In addition, the same setup can be used for quantum metrology as multiphoton interferometer with sensitivity at the Heisenberg limit., Comment: 5 pages, 2 figures

Pair creation by spontaneous parametric down-conversion (SPDC) has become a reliable source for single-photon states, used in many kinds of quantum information experiments and applications. In order to be spectrally pure, the two photons within a generated pair should be as frequency-uncorrelated as possible. For this purpose most experiments use narrow bandpass filters, having to put up with a drastic decrease in count rates. This article elaborates (theoretically and by numerical evaluation) the alternative method to engineer a setup such that the SPDC-generated quantum states are intrinsically pure. Using pulsed pump lasers and periodically poled crystals this approach makes bandpass filtering obsolete and allows for significantly higher output intensities and therefore count rates in the detectors. After numerically scanning all common wavelength regimes, polarisation configurations and three different non-linear crystals, we present a broad variety of setups which allow for an implementation of this method.

In the emerging field of quantum information technology the two basic subfields are quantum communication and quantum computation. Photonic qubits are considered as most promising information carriers for this new technology due to the immense advantage of suffering negligible decoherence. Additionally, the very small photon-photon interactions can be replaced by inducing effective nonlinearities via measurements which allow for the implementation of crucial two-qubit gate operations. Although the spontaneous parametric down-conversion gives access to the generation of highly entangled few-photon states, such as four-qubit cluster states which allow to demonstrate the new concept of the one-way quantum computer, its applicability is highly limited due to the poor scaling of the simultaneous emission of more than one-entangled photon pair. Therefore of particular interest is the reversible mapping of qubits from photon states to atomic states. This might allow the implementation of photonic quantum repeaters for long-distance quantum communication or the generation of arbitrary multi-photon states as required for linear-optics quantum computing. Thus for the realization of such a quantum network several approaches for achieving the required quantum control between matter and photons have been studied during the past few years. Recent experiments demonstrating the generation of narrow-bandwidth single photons using a room-temperature ensemble of 87 Rb atoms and electromagnetically induced transparency should emphasize the progress towards such a quantum network.

All previous tests of local realism have studied correlations between single-particle measurements. In the present experiment, we have performed a Bell experiment on three particles in which one of the measurements corresponds to a projection onto a maximally-entangled state. We show theoretically and experimentally, that correlations between these entangled measurements and single-particle measurements are too strong for any local-realistic theory and are experimentally exploited to violate a CHSH-Bell inequality by more than 5 standard deviations. We refer to this possibility as "entangled entanglement"., Comment: 4 figures, published version

Efficient teleportation is a crucial step for quantum computation and quantum networking. In the case of qubits, four different entangled Bell states have to be distinguished. We have realized a probabilistic, but in principle deterministic, Bell-state analyzer for two photonic quantum bits by the use of a nondestructive controlled-NOT gate based on entirely linear optical elements. This gate was capable of distinguishing between all of the Bell states with higher than 75% fidelity without any noise substraction due to utilizing quantum interference effects., Comment: 4 pages, 4 figures

We have performed the first experimental tomographic reconstruction of a three-photon polarization state. Quantum state tomography is a powerful tool for fully describing the density matrix of a quantum system. We measured 64 three-photon polarization correlations and used a ``maximum-likelihood'' reconstruction method to reconstruct the Greenberger-Horne-Zeilinger state. The entanglement class has been characterized using an entanglement witness operator and the maximum predicted values for the Mermin inequality were extracted.

Entangled photons are distributed directly through the atmosphere to a receiver station 7.8 km away at night over the city center of Vienna, Austria. Without a time-stable connection, the two stations found coincidence counts in the detection events through the cross-correlation of locally-recorded time stamps shared over a public Internet channel. As such, the sending and receiver stations were completely independent. The polarization correlations contained in the measured time tags are sufficient to convincingly violate a CHSH-Bell inequality and demonstrate entanglement between the two city buildings.

Cluster states are a new type of multiqubit entangled states with entanglement properties exceptionally well suited for quantum computation. In the present work, we experimentally demonstrate that correlations in a four-qubit linear cluster state cannot be described by local realism. This exploration is based on a recently derived Bell-type inequality [V. Scarani et al., Phys. Rev A 71, 042325 (2005)] which is tailored, by using a combination of three- and four-particle correlations, to be maximally violated by cluster states but not violated at all by GHZ states. We observe a cluster state Bell parameter of $2.59\pm 0.08$, which is more than 7 standard deviations larger than the threshold of 2 imposed by local realism., Comment: 4 pages, 2 figures

Quantum metrology utilizes nonclassical states (of light) to outperform the accuracy limits of its classical counterpart. We demonstrate the relevance of photon number Fock states and polarization entanglement for the experimental realization of interferometric quantum metrology applications.

Standard quantum computation is based on sequences of unitary quantum logic gates which process qubits. The one-way quantum computer proposed by Raussendorf and Briegel is entirely different. It has changed our understanding of the requirements for quantum computation and more generally how we think about quantum physics. This new model requires qubits to be initialized in a highly-entangled cluster state. From this point, the quantum computation proceeds by a sequence of single-qubit measurements with classical feedforward of their outcomes. Because of the essential role of measurement a one-way quantum computer is irreversible. In the one-way quantum computer the order and choices of measurements determine the algorithm computed. We have experimentally realized four-qubit cluster states encoded into the polarization state of four photons. We fully characterize the quantum state by implementing the first experimental four-qubit quantum state tomography. Using this cluster state we demonstrate the feasibility of one-way quantum computing through a universal set of one- and two-qubit operations. Finally, our implementation of Grover's search algorithm demonstrates that one-way quantum computation is ideally suited for such tasks., Comment: 36 pages, 6 figures, 2 tables

We have applied an entanglement purification protocol to produce a single entangled pair of photons capable of violating a CHSH Bell inequality from two pairs that individually could not. The initial poorly-entangled photons were created by a controllable decoherence that introduced complex errors. All of the states were reconstructed using quantum state tomography which allowed for a quantitative description of the improvement of the state after purification., Comment: 4 pages, 4 figures

Efficient long-distance quantum teleportation is crucial for quantum communication and quantum networking schemes. Here we describe the high-fidelity teleportation of photons over a distance of 600 metres across the River Danube in Vienna, with the optimal efficiency that can be achieved using linear optics. Our result is a step towards the implementation of a quantum repeater, which will enable pure entanglement to be shared between distant parties in a public environment and eventually on a worldwide scale.

We report the first experimental demonstration of a quantum controlled-NOT gate for different photons, which is classically feed forwardable. In the experiment, we achieved this goal with only the use of linear optics, an entangled ancillary pair of photons, and postselection. The techniques developed in our experiment are of significant importance for quantum information processing with linear optics.

Superposition is one of the most distinctive features of quantum theory and has been demonstrated in numerous single-particle interference experiments. Quantum entanglement, the coherent superposition of states in multi-particle systems, yields more complex phenomena. One important type of multi-particle experiment uses path-entangled number states, which exhibit pure higher-order interference and the potential for applications in metrology and imaging; these include quantum interferometry and spectroscopy with phase sensitivity at the Heisenberg limit, or quantum lithography beyond the classical diffraction limit. It has been generally understood that in optical implementations of such schemes, lower-order interference effects always decrease the overall performance at higher particle numbers. Such experiments have therefore been limited to two photons. Here we overcome this limitation, demonstrating a four-photon interferometer based on linear optics. We observe interference fringes with a periodicity of one-quarter of the single-photon wavelength, confirming the presence of a four-particle mode-entangled state. We anticipate that this scheme should be extendable to arbitrary photon numbers, holding promise for realizable applications with entanglement-enhanced performance.

We demonstrate the distribution of quantum entanglement via optical free-space links to independent receivers separated by 600 m, with no line of sight between each other. A Bell inequality between those receivers is violated by more than four standard deviations, confirming the quality of the entanglement. This outdoor experiment represents a step toward satellite-based distributed quantum entanglement.

The use of a new measure of what it means for a system to be quantum has profound technological and philosophical ramifications for the field of quantum information processing.

By utilizing the spatial quantum correlations of light, Italian researchers have now performed imaging at significantly higher signal-to-noise ratios than those possible through classical techniques.

Quantum teleportation in itself is intriguing. But now the combined states of two photons have been teleported — while preserving their entanglement — and this could bring large-scale quantum communication and computation a step closer.

The dynamics of carboxylate ligands on the surface of zirconium oxo clusters was investigated in two case studies. Zr4O2(methacrylate)12 was investigated by one- and two dimensional NMR spectra both in the solid state and in solution. In solution, the cluster is C2h symmetric; stepwise intramolecular exchange of the four non-equivalent ligands was observed when the temperature was raised from -80 degrees C to -50 degrees C. The individual exchange processes were assigned to different ligand positions. Ab initio molecular dynamics simulations were performed for Zr6(OH)4O4(formate)12 to study the trajectory for the rearrangement of three chelating ligands into bridging positions, i.e. the conversion of the C3-symmetric into an Oh-symmetric cluster. The observation of a dip in the energy barrier along the reaction coordinate was related to the intermediate formation of hydrogen bonds between the moving oxygen atom of the rearranging ligand and a micro3-OH group of the cluster. Thus, the motion of the ligand requires a concerted motion in three dimensions.

We report the first demonstration of a quantum game on an all-optical one-way quantum computer. Following a recent theoretical proposal we implement a quantum version of Prisoner's Dilemma, where the quantum circuit is realized by a 4-qubit box-cluster configuration and the player's local strategies by measurements performed on the physical qubits of the cluster. This demonstration underlines the strength and versatility of the one-way model and we expect that this will trigger further interest in designing quantum protocols and algorithms to be tested in state-of-the-art cluster resources., 13 pages, 4 figures

We have distributed entangled photons directly through the atmosphere to a receiver station 7.8 km away over the city of Vienna, Austria at night. Detection of one photon from our entangled pairs constitutes a triggered single photon source from the sender. With no direct time-stable connection, the two stations found coincidence counts in the detection events by calculating the cross-correlation of locally-recorded time stamps shared over a public internet channel. For this experiment, our quantum channel was maintained for a total of 40 minutes during which time a coincidence lock found approximately 60000 coincident detection events. The polarization correlations in those events yielded a Bell parameter, S=2.27/pm0.019, which violates the CHSH-Bell inequality by 14 standard deviations. This result is promising for entanglement-based free-space quantum communication in high-density urban areas. It is also encouraging for optical quantum communication between ground stations and satellites since the length of our free-space link exceeds the atmospheric equivalent., 8 pages including 1 figure and 2 tables. The first two authors contributed equally to this work

A real-world experiment marks a step towards worldwide quantum communication. Efficient long-distance quantum teleportation1 is crucial for quantum communication and quantum networking schemes2. Here we describe the high-fidelity teleportation of photons over a distance of 600 metres across the River Danube in Vienna, with the optimal efficiency that can be achieved using linear optics. Our result is a step towards the implementation of a quantum repeater3, which will enable pure entanglement to be shared between distant parties in a public environment and eventually on a worldwide scale.

A new entanglement-verification method is introduced and experimentally verified with a six-photon cluster state. We demonstrate that it is possible to efficiently detect multipartite entanglement with only a few copies of the state.

It has been proven theoretically and confirmed experimentally that quantum mechanics exhibits only second-order interference. However, this makes several implicit assumptions. Here we highlight these assumptions experimentally, showing that optical nonlinearities can induce higher-order interference.

We experimentally demonstrate that quantum superposition permits two-way communication between two distant parties that can exchange only one photon and show that the transmitted bits and the direction of communication remain private.

Quantum computers promise to be more efficient and powerful than their classical counterparts. In the one-way quantum computer model [1], a sequence of measurements processes qubits, which are initially prepared in a highly entangled cluster state. We present here an optical implementation of a 4-qubit cluster state and we show how different algorithms can be experimentally realized by performing the corresponding sequence of measurements. The key advantage of this scheme over the standard network approach of quantum computing is that inherent, randomly induced measurement errors can classically be fed-forward and corrected by adapting the basis of subsequent measurement.

We investigate high-harmonic generation in graphene heterostructures consisting of metallic nanoribbons separated from a graphene sheet by either a few-nanometer layer of aluminum oxide or an atomic monolayer of hexagonal boron nitride. The nanoribbons amplify the near-field at the graphene layer relative to the externally applied pumping, thus allowing us to observe third- and fifth-harmonic generation in the carbon monolayer at modest pump powers in the mid-infrared. We study the dependence of the nonlinear signals on the ribbon width and spacer thickness, as well as pump power and polarization, and demonstrate enhancement factors relative to bare graphene reaching 1600 and 4100 for third- and fifth-harmonic generation, respectively. Our work supports the use of graphene heterostructures to selectively enhance specific nonlinear processes of interest, an essential capability for the design of nanoscale nonlinear devices.