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Metallic magnetic calorimeters have been used for several years for the determination of the shapes of beta spectra. Experimental spectra of the beta decays of $$^{63}$$ Ni and $$^{241}$$ Pu exhibit, at very low energy, strong deviations from standard theoretical calculations including corrections for screening, radiative, and nuclear size effects. These discrepancies can be attributed to the atomic exchange effect. In particular the spectrum of $$^{63}$$ Ni measured with an electroplated $$^{63}$$ Ni source is in excellent agreement with theory including the exchange effect. This underlines the quality of the experimental spectrum as well as the correctness of the calculation of the exchange effect. [ABSTRACT FROM AUTHOR]

Abstract: The low-lying spectroscopy of 6He was investigated via the 2-neutron transfer reaction with the 8He beam delivered by the SPIRAL facility at . The light charged particles produced by the direct reactions were measured using the MUST2 Si-strip telescope array. Above the known state, two new resonances were observed: at (width ) and at with . Through the analysis of the angular distributions, they correspond to a state and to an state, respectively. These new states, challenging the nuclear theories, could be used as benchmarks for checking the microscopic inputs of the newly improved structure models, and should trigger development of models including the treatments of both core excitation and continuum coupling effects. [Copyright &y& Elsevier]

The 8He(rf, p) reaction was studied in inverse kinematics at 15.4A MeV using the MUST2 Si-Csl array in order to shed light on the level structure of 9He. The well known l6O(d, p)17O reaction, performed here in reverse kinematics, was used as a test to validate the experimental methods. The 9He missing mass spectrum was deduced from the kinetic energies and emission angles of the recoiling protons. Several structures were observed above the neutron-emission threshold and the angular distributions were used to deduce the multipolarity of the transitions. This work confirms that the ground state of 9He is located very close to the neutron threshold of 8He and supports the occurrence of parity inversion in 9He. [ABSTRACT FROM AUTHOR]

Abstract: The LNE-LNHB is developing metallic magnetic calorimeters, a specific type of cryogenic detectors, for beta spectrometry. The aim is the determination of the shape factors of beta spectra. Our latest detector has been designed to measure the spectrum of 241Pu, a pure beta emitter with an endpoint energy of 20.8keV. In this paper, the detection principle of metallic magnetic calorimeters is explained and a detailed description is given of the realization of the detector enclosing a 241Pu source inside the detector absorber. A spectrum resulting from our first measurement is shown and compared with a theoretical spectrum. [Copyright &y& Elsevier]

Sterile neutrinos are natural extensions to the standard model of particle physics and provide a possible portal to the dark sector. We report a new search for the existence of sub-MeV sterile neutrinos using the decay-momentum reconstruction technique in the decay of 7Be. The experiment measures the total energy of the 7Li daughter atom from the electron capture decay of 7Be implanted into sensitive superconducting tunnel junction (STJ) quantum sensors. This first experiment presents data from a single STJ operated at a low count rate for a net total of 28 days, and provides exclusion limits on sterile neutrinos in the mass range from 100 to 850 keV that improve upon previous work by up to an order of magnitude. [ABSTRACT FROM AUTHOR]

We report a high-statistics measurement of the L / K orbital electron capture ratio in 7 Be embedded in cryogenic Ta. The thin Ta film formed part of a high-resolution superconducting tunnel junction radiation detector that was used to identify the signals from different decay channels. The measured L / K capture ratio of 0.070(7) is significantly larger than the only previous measurement of this quantity and the theoretical predictions that include in-medium effects. This value is a uniquely sensitive probe of the 1s and 2s orbital overlaps with the nucleus and is of relevance to nuclear and atomic physics, as well as Li production in novae and other astrophysical scenarios. This is the first experiment that uses superconducting tunnel junctions for nuclear-recoil detection, opening a new experimental avenue for low-energy precision measurements with rare isotopes. [ABSTRACT FROM AUTHOR]

Background: The understanding and description of forbidden decays provides interesting challenges for nuclear theory. These calculations could help to test underlying nuclear models and interpret experimental data. Purpose: Compare a direct measurement of the 138Laβ-decay Q value with the β-decay spectrum end-point energy measured by Quarati et al. using LaBr3 detectors [Appl. Radiat. Isot. 108, 30 (2016)]. Use new precise measurements of the 138Laβ-decay and electron capture (EC) Q values to improve theoretical calculations of the β-decay spectrum and EC probabilities. Method: High-precision Penning trap mass spectrometry was used to measure cyclotron frequency ratios of 138La, 138Ce, and 138Ba ions from which β-decay and EC Q values for 138La were obtained. Results: The 138Laβ-decay and EC Q values were measured to be Qβ=1052.42(41) keV and QEC=1748.41(34) keV, improving the precision compared to the values obtained in the most recent atomic mass evaluation [Wang et al., Chin. Phys. C 41, 030003 (2017)] by an order of magnitude. These results are used for improved calculations of the 138Laβ-decay shape factor and EC probabilities. New determinations for the 138Ce 2EC Q value and the atomic masses of 138La, 138Ce, and 138Ba are also reported. Conclusion: The 138Laβ-decay Q value measured by Quarati et al. is in excellent agreement with our new result, which is an order of magnitude more precise. Uncertainties in the shape factor calculations for 138Laβ decay using our new Q value are reduced by an order of magnitude. Uncertainties in the EC probability ratios are also reduced and show improved agreement with experimental data. [ABSTRACT FROM AUTHOR]

The theoretical modelling of the atomic exchange effect, until now only available for allowed beta decays, has been extended to the forbidden unique transitions. The required computing power for such calculations being important, an extensive tabulation of the correction factors has been conducted. These tables will be included in the future version of the BetaShape code, which atomic screening has also been revised to ensure the same level of accuracy as for exchange. Results for several radionuclides are discussed., Competing Interests: Declaration of competing interest The authors declare the following financial interests/personal relationships which may be considered as potential competing interests: X. Mougeot reports financial support was provided by European Commission., (Copyright © 2023 The Author. Published by Elsevier Ltd.. All rights reserved.)

We present a search for dark matter particles with sub-GeV/c^{2} masses whose interactions have final state electrons using the DarkSide-50 experiment's (12 306±184)  kg d low-radioactivity liquid argon exposure. By analyzing the ionization signals, we exclude new parameter space for the dark matter-electron cross section σ[over ¯]_{e}, the axioelectric coupling constant g_{Ae}, and the dark photon kinetic mixing parameter κ. We also set the first dark matter direct-detection constraints on the mixing angle |U_{e4}|^{2} for keV/c^{2} sterile neutrinos.

Dark matter elastic scattering off nuclei can result in the excitation and ionization of the recoiling atom through the so-called Migdal effect. The energy deposition from the ionization electron adds to the energy deposited by the recoiling nuclear system and allows for the detection of interactions of sub-GeV/c^{2} mass dark matter. We present new constraints for sub-GeV/c^{2} dark matter using the dual-phase liquid argon time projection chamber of the DarkSide-50 experiment with an exposure of (12 306±184)  kg d. The analysis is based on the ionization signal alone and significantly enhances the sensitivity of DarkSide-50, enabling sensitivity to dark matter with masses down to 40  MeV/c^{2}. Furthermore, it sets the most stringent upper limit on the spin independent dark matter nucleon cross section for masses below 3.6  GeV/c^{2}.

In this paper we describe experiments on two enriched 40 K solutions to accurately determine decay data. The first solution was measured in 2004/2005 by means of a gamma-ray spectrometer with low background and a liquid scintillation (LS) counter to apply the CIEMAT/NIST efficiency tracing method. A combination of results yields an emission probability of the 1461 keV gamma-rays of P γ  = 0.1030(11) which is lower than current results of data evaluations. The activity concentration of the second solution was also determined by means of LS counting, but here, the CIEMAT/NIST efficiency tracing method as well as the TDCR method were applied. Again, the result was combined with that of independent gamma-ray spectrometry and the gamma-ray emission probability was found to be P γ  = 0.1029(9) in good agreement with the result obtained from the first solution. A combination of both experiments yields P γ  = 0.1029(9). The spectra of a TriCarb LS counter were carefully analyzed and a beta minus emission probability [Formula: see text]  = 0.8954(14) was determined. The new results for P γ and [Formula: see text] indicate that the overall probability of the decay via EC in recent data evaluations is overestimated. The LS counting efficiencies were computed with a stochastic model and up-to-date calculations of the beta spectrum and fractional EC probabilities were used. The final activity result of the second solution is combined with the outcome of a comprehensive isotopic analysis to determine the half-life of 40 K which is found to be 1.2536(27) ·10 9 years. All above-stated uncertainties are standard uncertainties (k = 1)., (Copyright © 2022 Elsevier Ltd. All rights reserved.)

The beta decay of 151 Sm was measured by means of a metallic magnetic calorimeter. The measurement and subsequent analysis yielded a beta spectrum with an outstanding high-energy resolution of about 70 eV (FWHM) at 22 keV and a very low energy threshold well below 400 eV. The spectrum exhibited unexpectedly elevated beta emission probabilities at very low energy that we have not been able to reproduce in our theoretical study. The data analysis was thus scrutinized and an independent analysis of the same data set carried out. All new approaches have confirmed the previously found shape of the beta spectrum. The measured spectrum was compared to predictions from an advanced theoretical modeling that includes the atomic exchange effect, precise radiative corrections as well as the realistic nuclear structure that usually plays an important role in first forbidden non-unique transitions. The measured spectrum was then carefully analyzed to determine the maximum beta energy, which was found to be Q = 76.430(68) keV. The dominant beta decay of 151 Sm populates the ground state of 151 Eu, and a weak beta branch populates the first excited state of 151 Eu. From our measurements, the probabilities of these two branches were determined to be 99.31(11)% and 0.69(11)%, respectively., (Copyright © 2022 The Authors. Published by Elsevier Ltd.. All rights reserved.)

Radioactive strontium isotopes play an important role in environmental radioactivity. Reliable activity standards are required in order to validate radioanalytical techniques and related measurements. In this paper, improved methods for the primary activity standardization of 90 Sr/ 90 Y based on liquid scintillation counting are presented. To this end, two methods were used: the CIEMAT/NIST efficiency tracing technique with 3 H as a tracer and the triple-to-double coincidence ratio method. Non-negligible discrepancies between the two methods were found when applying existing analysis techniques. A detailed study was carried out to identify and eliminate the causes of these discrepancies. Eventually, excellent agreement between the two methods was obtained. This required advanced beta spectrum calculations which were carried out with a specific version of the BetaShape program taking the atomic exchange effect into account. In addition, it was found that the quench-indicating parameters determined in commercial liquid scintillation counters are biased, which can cause significant problems for the CIEMAT/NIST efficiency tracing method. The effect depends on the counting rate and can be explained by a superposition of the LS spectra generated by 90 Sr/ 90 Y and the external standard source., (Copyright © 2020 Elsevier Ltd. All rights reserved.)

Sterile neutrinos are natural extensions to the standard model of particle physics and provide a possible portal to the dark sector. We report a new search for the existence of sub-MeV sterile neutrinos using the decay-momentum reconstruction technique in the decay of ^{7}Be. The experiment measures the total energy of the ^{7}Li daughter atom from the electron capture decay of ^{7}Be implanted into sensitive superconducting tunnel junction (STJ) quantum sensors. This first experiment presents data from a single STJ operated at a low count rate for a net total of 28 days, and provides exclusion limits on sterile neutrinos in the mass range from 100 to 850 keV that improve upon previous work by up to an order of magnitude.

PENELOPE simulations of a Vinten ionization chamber (IC) were performed to investigate the influence of the thickness of glass-ampoules used in 222 Rn standardization. The simulation reveals a non-negligible variation of the energy deposited in the chamber gas region (which may induce a proportional variation of the measured current) when considering the β transition emissions of the daughters of 222 Rn. This reinforces the idea of using a specialist container (made of metal to preserve the integrity of the container) that would circulate between the metrology laboratories in the context of international comparison exercises using the BIPM international reference system (SIR)., (Copyright © 2019 Elsevier Ltd. All rights reserved.)

The activity concentration of a 60 Co solution was measured by means of two 4πβ-γ coincidence counting systems using a liquid scintillation counter and a proportional counter (PC) in the beta channel, respectively. Additional liquid scintillation measurements were carried out and CIEMAT/NIST efficiency tracing as well as the triple-to-double coincidence ratio (TDCR) methods were applied to analyse the data. The last two methods require computed beta spectra to determine the counting efficiencies. The results of both 4πβ-γ coincidence counting techniques are in very good agreement and yield a robust reference value. The initial activity concentration determined with liquid scintillation counting was found to be significantly lower than the results from 4πβ-γ coincidence counting. In addition, the results from TDCR and CIEMAT/NIST show some inconsistency. The discrepancies were resolved by applying new beta spectrum calculations for the dominant allowed beta transition of 60 Co. The use of calculations which take screening effects as well as the atomic exchange effect into account leads to good agreement between all four methods; the combination of these techniques delivers an important validation of beta spectra., (Copyright © 2017 The Authors. Published by Elsevier Ltd.. All rights reserved.)

The activity concentration of a (63)Ni solution was determined by means of two liquid scintillation counting techniques: the TDCR method and the CIEMAT/NIST efficiency tracing technique. The results of both methods are in excellent agreement, provided that the (63)Ni beta spectrum calculation accounts for the atomic exchange effect. Thus, new beta spectrum calculations resolve a discrepancy that has been found in previous analyses. The influence of the computed beta spectrum on the final uncertainty of the activity concentration is discussed., (Copyright © 2015 Elsevier Ltd. All rights reserved.)

An excited state in the proton-rich unbound nucleus 12O was identified at 1.8(4) MeV via missing-mass spectroscopy with the 14O(p,t) reaction at 51 AMeV. The spin-parity of the state was determined to be 0+ or 2+ by comparing the measured differential cross sections with distorted-wave calculations. The lowered location of the excited state in 12O indicates the breakdown of the major shell closure at Z=8 near the proton drip line. This demonstrates the persistence of mirror symmetry in the disappearance of the magic number 8 between 12O and its mirror partner 12Be.