Search

The lifetimes of first excited 2$^+$, 4$^+$ and 6$^+$ states in $^{98}$Zr were measured with the Recoil-Distance Doppler Shift method in an experiment performed at GANIL. Excited states in $^{98}$Zr were populated using the fission reaction between a 6.2 MeV/u $^{238}$U beam and a $^{9}$Be target. The $\gamma$ rays were detected with the EXOGAM array in correlation with the fission fragments identified in mass and atomic number in the VAMOS++ spectrometer. Our result shows very small B(E2;2$_1^+$ $\rightarrow$ 0$_1^+$) value in $^{98}$Zr thereby confirming the very sudden onset of collectivity at $N=60$. The experimental results are compared to large-scale Monte Carlo Shell model and beyond mean field calculations. The present results indicate coexistence of two additional deformed shapes in this nucleus along with the spherical ground state.

High spin band structures of neutron-rich $^{152-158}$Pm isotopes have been obtained from the measurement of prompt $\gamma$-rays of isotopically identified fragments produced in fission of $^{238}$U+$^{9}$Be and detected using the VAMOS++ magnetic spectrometer and EXOGAM segmented Clover array at GANIL and also from the high statistics $\gamma$-$\gamma$-$\gamma$ and $\gamma$-$\gamma$-$\gamma$-$\gamma$ data from the spontaneous fission of $^{252}$Cf using Gammasphere. The excited states in $^{157}$Pm and those above the isomers in even-A Pm isotopes $^{152,154,156,158}$Pm have been identified for the first time. The spectroscopic information on the rotational band structures in odd-A Pm isotopes has been extended considerably to higher spins and the possibility of the presence of reflection asymmetric shapes is explored. The configuration assignments are based on the results of Cranked Relativistic Hartree-Bogoliubov calculations. From the systematics of bands in odd-A Pm isotopes and weak population of opposite parity bands, octupole deformed shapes in neutron rich Pm isotopes beyond $N=90$ seem unlikely to be present.

Excited states in the $T_z=-1$ nucleus $^{70}$Kr have been populated using inelastic scattering of a radioactive $^{70}$Kr beam as well as one- and two-neutron removal reactions from $^{71,72}$Kr at intermediate beam energies. The level scheme of $^{70}$Kr was constructed from the observed $\gamma$-ray transitions and coincidences. Tentative spin and parity assignments were made based on comparison with the mirror nucleus $^{70}$Se. A second $2^+$ state and a candidate for the corresponding $4^+_2$ state suggest shape coexistence in $^{70}$Kr., Comment: accepted Phys. Lett. B

The half-life of $^{19}$Ne has been measured using a real-time digital multiparametric acquisition system providing an accurate time-stamp and relevant information on the detectors signals for each decay event. An exhaustive offline analysis of the data gave unique access to experimental effects potentially biasing the measurement. After establishing the influence factors impacting the measurement such as after-pulses, pile-up, gain and base line fluctuations, their effects were accurately estimated and the event selection optimized. The resulting half-life, $17.2569\pm0.0019_{(stat)}\pm0.0009_{(syst)}$~s, is the most precise up to now for $^{19}$Ne. It is found in agreement with two recent precise measurements and not consistent with the most recent one [L.J. Broussard {\it et al.}, Phys. Rev. Lett. {\bf112}, 212301 (2014)] by 3.0 standard deviations. The full potential of the technique for nuclei with half-lives of a few seconds is discussed., Comment: 11 pages, 16 figures

The $\beta$ decay of the odd-odd nucleus $^{70}$Br has been investigated with the BigRIPS and EURICA setups at the Radioactive Ion Beam Factory (RIBF) of the RIKEN Nishina Center. The $T=0$ ($J^{\pi}=9^+$) and $T=1$ ($J^{\pi}=0^+$) isomers have both been produced in in-flight fragmentation of $^{78}$Kr with ratios of 41.6(8)\% and 58.4(8)\%, respectively. A half-life of $t_{1/2}=2157^{+53}_{-49}$ ms has been measured for the $J^{\pi}=9^+$ isomer from $\gamma$-ray time decay analysis. Based on this result, we provide a new value of the half-life for the $J^{\pi}=0^+$ ground state of $^{70}$Br, $t_{1/2}=78.42\pm0.51$ ms, which is slightly more precise, and in excellent agreement, with the best measurement reported hitherto in the literature. For this decay, we provide the first estimate of the total branching fraction decaying through the $2^+_1$ state in the daughter nucleus $^{70}$Se, $R(2^+_1)=1.3\pm1.1\%$. We also report four new low-intensity $\gamma$-ray transitions at 661, 1103, 1561, and 1749 keV following the $\beta$ decay of the $J^{\pi}=9^+$ isomer. Based on their coincidence relationships, we tentatively propose two new excited states at 3945 and 4752 keV in $^{70}$Se with most probable spins and parities of $J^{\pi}=(6^+)$ and $(8^+)$, respectively. The observed structure is interpreted with the help of shell-model calculations, which predict a complex interplay between oblate and prolate configurations at low excitation energies.

We report the first observation of the 2$^+$ isomer in $^{52}$Co, produced in the $\beta$ decay of the 0$^+$, $^{52}$Ni ground state. We have observed three $\gamma$-rays at 849, 1910, and 5185 keV characterizing the $\beta$ de-excitation of the isomer. We have measured a half-life of 102(6) ms for the isomeric state. The Fermi and Gamow-Teller transition strengths for the $\beta$ decay of $^{52m}$Co to $^{52}$Fe have been determined. We also add new information on the $\beta$ decay of the 6$^+$, $^{52}$Co ground state, for which we have measured a half-life of 112(3) ms., Comment: Accepted for publication in PRC. 8 pages, 7 figures

In an experiment with the BigRIPS separator at the RIKEN Nishina Center, the fragmentation of a $^{78}$Kr beam allowed the observation of new neutron-deficient isotopes at the proton drip-line. Clean identification spectra could be produced and $^{63}$Se, $^{67}$Kr, and $^{68}$Kr were identified for the first time. In addition, $^{59}$Ge was also observed. Three of these isotopes, $^{59}$Ge, $^{63}$Se, and $^{67}$Kr, are potential candidates for ground-state two-proton radioactivity. In addition, the isotopes $^{58}$Ge, $^{62}$Se, and $^{66}$Kr were also sought but without success. The present experiment also allowed the determination of production cross sections for some of the most exotic isotopes. These measurements confirm the trend already observed that the empirical parameterization of fragmentation cross sections, EPAX, significantly overestimates experimental cross sections in this mass region., Comment: accepted as Rapid Communication in PRC

The gamma-ray decay of excited states of the one-valence-proton nucleus 133Sb has been studied using cold-neutron induced fission of 235U and 241Pu targets, during the EXILL campaign at the ILL reactor in Grenoble. By using a highly efficient HPGe array, coincidences between gamma-rays prompt with the fission event and those delayed up to several tens of microseconds were investigated, allowing to observe, for the first time, high-spin excited states above the 16.6 micros isomer. Lifetimes analysis, performed by fast-timing techniques with LaBr3(Ce) scintillators, reveals a difference of almost two orders of magnitude in B(M1) strength for transitions between positive-parity medium-spin yrast states. The data are interpreted by a newly developed microscopic model which takes into account couplings between core excitations (both collective and non-collective) of the doubly magic nucleus 132Sn and the valence proton, using the Skyrme effective interaction in a consistent way. The results point to a fast change in the nature of particle-core excitations with increasing spin.

The previously reported levels assigned to 151,152,153Pr have recently been called into question regarding their mass assignment. The above questioned level assignments are clarified by measuring g-transitions tagged with A and Z in an in-beam experiment in addition to the measurements from 252Cf spontaneous fission (SF) and establish new spectroscopic information from $N=84$ to $N=94$ in the Pr isotopic chain. The isotopic chain 143-153Pr has been studied from the spontaneous fission of 252Cf by using Gammasphere and also from the measurement of the prompt g-rays in coincidence with isotopically-identified fission fragments using VAMOS++ and EXOGAM at GANIL. The latter were produced using 238U beams on a 9Be target at energies around the Coulomb barrier. The g-g-g-g data from 252Cf (SF) and those from the GANIL in-beam A- and Z-gated spectra were combined to unambiguously assign the various transitions and levels in 151,152,153Pr and other isotopes. New transitions and bands in 145,147,148,149,150Pr were identified by using g-g-g and g-g-g-g coincidences and A and Z gated g-g spectra. The transitions and levels previously assigned to 151,153Pr have been confirmed by the (A,Z) gated spectra. The transitions previously assigned to 152Pr are now assigned to 151Pr on the basis of the (A,Z) gated spectra. Two new bands with 20 new transitions in 152Pr and one new band with 7 new transitions in 153Pr are identified from the g-g-g-g coincidence spectra and the (A,Z) gated spectrum. In addition, new g-rays are also reported in 143-146Pr. New levels of 145,147-153Pr have been established, reliable mass assignments of the levels in 151,152,153Pr have been reported and new transitions have been identified in 143-146Pr showing the new avenues that are opened by combining the two experimental approaches., Comment: Accepted in Phys. Rev. C

Linear polarization measurements have been performed for $\gamma$-rays in $^{91}$Ru produced with the $^{58}$Ni($^{36}$Ar, $2p1n$$\gamma$)$^{91}$Ru reaction at a beam energy of 111 MeV. The EXOGAM Ge clover array has been used to measure the $\gamma$-$\gamma$ coincidences, $\gamma$-ray linear polarization and $\gamma$-ray angular distributions. The polarization sensitivity of the EXOGAM clover detectors acting as Compton polarimeters has been determined in the energy range 0.3$-$1.3 MeV. Several transitions have been observed for the first time. Measurements of linear polarization and angular distribution have led to the firm assignments of spin differences and parity of high-spin states in $^{91}$Ru. More specifically, calculations using a semi-empirical shell model were performed to understand the structures of the first and second (21/2$^{+}$) and (17/2$^{+}$) levels. The results are in good agreement with the experimental data, supporting the interpretation of the non yrast (21/2$^{+}$) and (17/2$^{+}$) states in terms of the $J_{\rm max}$ and $J_{\rm max}-2$ members of the seniority-three $\nu(g_{9/2})^{-3}$ multiplet., Comment: 19 pages, 8 figures, 2 tables

The decay of $^{19}$O($\beta^-$) and $^{19}$Ne($\beta^+$) implanted in niobium in its superconducting and metallic phase was measured using purified radioactive beams produced by the SPIRAL/GANIL facility. Half-lives and branching ratios measured in the two phases are consistent within one-sigma error bar. This measurement casts strong doubts on the predicted strong electron screening in superconductor, the so-called superscreening. The measured difference in screening potential energy is 110(90) eV for $^{19}$Ne and 400(320) eV for $^{19}$O. Precise determinations of the half-lives were obtained for $^{19}$O: 26.476(9) s and $^{19}$Ne: 17.254(5) s., Comment: 4 pages, 3 figures, accepted for publication in Physical Review Letters

We report on the observation of a new isomeric state in $^{68}$Ni. We suggest that the newly observed state at 168(1) keV above the first 2$^+$ state is a $\pi(2p-2h)$ 0$^{+}$ state across the major Z=28 shell gap. Comparison with theoretical calculations indicates a pure proton intruder configuration and the deduced low-lying structure of this key nucleus suggests a possible shape coexistence scenario involving a highly deformed state., Comment: 5 pages, 3 figures, accepted for publication in Physical Review C

The Advanced GAmma Tracking Array (AGATA) is a European project to develop and operate the next generation gamma-ray spectrometer. AGATA is based on the technique of gamma-ray energy tracking in electrically segmented high-purity germanium crystals. This technique requires the accurate determination of the energy, time and position of every interaction as a gamma ray deposits its energy within the detector volume. Reconstruction of the full interaction path results in a detector with very high efficiency and excellent spectral response. The realization of gamma-ray tracking and AGATA is a result of many technical advances. These include the development of encapsulated highly-segmented germanium detectors assembled in a triple cluster detector cryostat, an electronics system with fast digital sampling and a data acquisition system to process the data at a high rate. The full characterization of the crystals was measured and compared with detector-response simulations. This enabled pulse-shape analysis algorithms, to extract energy, time and position, to be employed. In addition, tracking algorithms for event reconstruction were developed. The first phase of AGATA is now complete and operational in its first physics campaign. In the future AGATA will be moved between laboratories in Europe and operated in a series of campaigns to take advantage of the different beams and facilities available to maximize its science output. The paper reviews all the achievements made in the AGATA project including all the necessary infrastructure to operate and support the spectrometer., Comment: This version contains a correction of a typing error in the caption of Fig. 2. The DOI to the article published in Nucl. Instr. Meth A was also added

Lifetimes of the $9/2^-_1$ and $3/2^-_1$ states in $^{63}$Co and the $9/2^-_1$ state in $^{65}$Co were measured using the recoil distance Doppler shift and the differential decay curve methods. The nuclei were populated by multi-nucleon transfer reactions in inverse kinematics. Gamma rays were measured with the EXOGAM Ge array and the recoiling fragments were fully identified using the large-acceptance VAMOS spectrometer. The E2 transition probabilities from the $3/2^-_1$ and $9/2^-_1$ states to the $7/2^-$ ground state could be extracted in $^{63}$Co as well as an upper limit for the $9/2^-_1\rightarrow7/2^-_1$ $B$(E2) value in $^{65}$Co. The experimental results were compared to large-scale shell-model calculations in the $pf$ and $pfg_{9/2}$ model spaces, allowing to draw conclusions on the single-particle or collective nature of the various states., Comment: 8 pages, 8 figures, 1 table, accepted for publication in Physical Review C

We report here the first direct lifetime measurement of the 2+1 state in 72,74Zn. The neutron-rich beam was produced by in-flight fragmentation of 76Ge at the Grand Acc\'el\'erateur National d'Ions Lourds and separated with the LISE spectrometer. The 2+1 state was excited by inelastic scattering and knock-out reaction on a CD2 target and its lifetime was measured by the recoil-distance Dopplershift method with the K\"oln plunger device combined with the EXOGAM detectors. The lifetimes of the 2+1 states in 72,74Zn were determined to be 17.9(18) and 27.0(24) ps, which correspond to reduced transition probabilities B(E2; 2+1 \rightarrow 0+) = 385(39) and 370(33) e2fm4, respectively. These values support the idea of a systematic maximum of collectivity at N = 42 for Zn, Ge and Se nuclei. In addition, the available systematics in the neighboring nuclei point towards a transition from a spherical oscillator at N = 40 to complete {\gamma}-softness at N = 42., Comment: 10 pages, 13 figures; accepted for publication in Phys. Rev. C

The general phenomenon of shell structure in atomic nuclei has been understood since the pioneering work of Goeppert-Mayer, Haxel, Jensen and Suess.They realized that the experimental evidence for nuclear magic numbers could be explained by introducing a strong spin-orbit interaction in the nuclear shell model potential. However, our detailed knowledge of nuclear forces and the mechanisms governing the structure of nuclei, in particular far from stability, is still incomplete. In nuclei with equal neutron and proton numbers ($N = Z$), the unique nature of the atomic nucleus as an object composed of two distinct types of fermions can be expressed as enhanced correlations arising between neutrons and protons occupying orbitals with the same quantum numbers. Such correlations have been predicted to favor a new type of nuclear superfluidity; isoscalar neutron-proton pairing, in addition to normal isovector pairing (see Fig. 1). Despite many experimental efforts these predictions have not been confirmed. Here, we report on the first observation of excited states in $N = Z = 46$ nucleus $^{92}$Pd. Gamma rays emitted following the $^{58}$Ni($^{36}$Ar,2$n$)$^{92}$Pd fusion-evaporation reaction were identified using a combination of state-of-the-art high-resolution {\gamma}-ray, charged-particle and neutron detector systems. Our results reveal evidence for a spin-aligned, isoscalar neutron-proton coupling scheme, different from the previous prediction. We suggest that this coupling scheme replaces normal superfluidity (characterized by seniority coupling) in the ground and low-lying excited states of the heaviest N = Z nuclei. The strong isoscalar neutron- proton correlations in these $N = Z$ nuclei are predicted to have a considerable impact on their level structures, and to influence the dynamics of the stellar rapid proton capture nucleosynthesis process., Comment: 13 pages, 3 figures

The spectroscopy of 21O has been investigated using a radioactive 20O beam and the (d,p) reaction in inverse kinematics. The ground and first excited states have been determined to be Jpi=5/2+ and Jpi=1/2+ respectively. Two neutron unbound states were observed at excitation energies of 4.76 +- 0.10 and 6.16 +- 0.11. The spectroscopic factor deduced for the lower of these interpreted as a 3/2+ level, reveals a rather pure 0d3/2 single-particle configuration. The large energy difference between the 3/2+ and 1/2+ states is indicative of the emergence of the N=16 magic number. For the higher lying resonance, which has a character consistent with a spin-parity assignment of 3/2+ or 7/2-, a 71% branching ratio to the first 2+ state in 20O has been observed. The results are compared with new shell model calculations., Comment: 5 pages, 2 figures

The transfer of neutrons onto 24Ne has been measured using a reaccelerated radioactive beam of 24Ne to study the (d,p) reaction in inverse kinematics. The unusual raising of the first 3/2+ level in 25Ne and its significance in terms of the migration of the neutron magic number from N=20 to N=16 is put on a firm footing by confirmation of this state's identity. The raised 3/2+ level is observed simultaneously with the intruder negative parity 7/2- and 3/2- levels, providing evidence for the reduction in the N=20 gap. The coincident gamma-ray decays allowed the assignment of spins as well as the transferred orbital angular momentum. The excitation energy of the 3/2+ state shows that the established USD shell model breaks down well within the sd model space and requires a revised treatment of the proton-neutron monopole interaction., Comment: Phys. Rev. Lett. in press (4 pages, 3 figures)

A compact, quasi-4pi position sensitive silicon array, TIARA, designed to study direct reactions induced by radioactive beams in inverse kinematics is described here. The Transfer and Inelastic All-angle Reaction Array (TIARA) consists of 8 resistive charge division detectors forming an octagonal barrel around the target and a set of double-sided silicon-strip annular detectors positioned at each end of the barrel. The detector was coupled to the -ray array EXOGAM and the spectrometer VAMOS at the GANIL Laboratory to demonstrate the potential of such an apparatus with radioactive beams. The 14N(d,p)15N reaction, well known in direct kinematics, has been carried out in inverse kinematics for that purpose. The observation of the 15N ground state and excited states at 7.16 and 7.86 MeV is presented here as well as the comparison of the measured proton angular distributions with DWBA calculations. Transferred l-values are in very good agreement with both theoretical calculations and previous experimental results obtained in direct kinematics., Comment: 12 figures, submitted to NIM A

Beta-decay branching ratios of 62Ga have been measured at the IGISOL facility of the Accelerator Laboratory of the University of Jyvaskyla. 62Ga is one of the heavier Tz = 0, 0+ -> 0+ beta-emitting nuclides used to determine the vector coupling constant of the weak interaction and the Vud quark-mixing matrix element. For part of the experimental studies presented here, the JYFLTRAP facility has been employed to prepare isotopically pure beams of 62Ga. The branching ratio obtained, BR= 99.893(24)%, for the super-allowed branch is in agreement with previous measurements and allows to determine the ft value and the universal Ft value for the super-allowed beta decay of 62Ga.

In an experiment at the SISSI/LISE3 facility of GANIL, the most proton-rich zinc isotopes 55,56Zn have been observed for the first time. The experiment was performed using a high-intensity 58Ni beam at 74.5 MeV/nucleon impinging on a nickel target. The identification of 55,56Zn opens the way to 54Zn, a good candidate for two-proton radioactivity according to theoretical predictions., Comment: 2 pages, 1 figure, accepted for publication in Eur. Phys. J. A

Decay studies of very neutron-deficient nuclei ranging from 39Ti to 49Ni have been performed during a projectile fragmentation experiment at the GANIL/LISE3 separator. For all nuclei studied in this work, 39,40Ti, 42,43Cr, 46Mn, 45,46,47Fe and 49Ni, half-lives and decay spectra have been measured. In a few cases, gamma coincidence measurements helped to successfully identify the initial and final states of transitions. In these cases, partial decay scheme are proposed. For the most exotic isotopes, 39Ti, 42Cr, 45Fe and 49Ni, which are candidates for two-proton radioactivity from the ground state, no clear evidence of this process is seen in our spectra and we conclude rather on a delayed particle decay., Comment: 12 pages, 15 figures, submitted for publication in Eur. Phys. J. A

The excitation of the giant dipole resonance by fusion is studied with N/Z asymmetry in the entrance channel. the TDHF solution exhibits a strong dipole vibration which can be associated with a giant vibration along the main axis of a fluctuating prolate shape. The consequences on the gamma-ray emission from hot compound nuclei are discussed., Comment: 4 pages, 4 figures, submitted to Physical Review Letter

The paper reports on the first observation of doubly-magic Nickel-48 in an experimental at the SISSI/LISE3 facility of GANIL. Four Nickel-48 isotopes were identified. In addition, roughly 100 Nickel-49, 50 Iron-45, and 290 Chromium-42 isotopes were observed. This opens the possibility to search for two-proton emission from these nuclei., Comment: 4 pages, 3 figures, accepted for publication in Phys. Rev. Lett