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This work proposes a new route to overcome the limits of the thermal poling technique for the creation of second order nonlinearity in conventional silica optical fibers. We prove that it is possible to enhance the nonlinear behavior of periodically poled fibers merging the effects of poling with the nonlinear intrinsic properties of some materials, such as MoS2, which are deposited inside the cladding holes of a twin-hole silica fiber. The optical waves involved in a second harmonic generation process partially overlap inside the thin film of the nonlinear material and exploit its higher third order susceptibility to produce an enhanced SHG., SCOPUS: ar.j, info:eu-repo/semantics/published

Thermal poling, a technique to create permanently effective second-order susceptibility in silica optical fibers, has recently been improved by the discovery of an "induction poling" technique1 and the adoption of liquid electrodes2, allowing for poling fibers of any length and geometry. Nevertheless, the nonlinearity created via thermal poling is always limited by the ooelig;'(3)of the optical fiber material and by the maximum electric field that can be frozen inside the glass. For these reasons research is ongoing to determine routes for further improving the nonlinear effects due to the thermal poling process. In this work, we propose to enhance the effects of the thermal poling by exploiting the intrinsic nonlinear properties of some 2D materials3, which are deposited inside the cladding holes of a twin-hole silica fiber. The materials we focused on are 2D Transition Metal Chalcogenide (2D TMDC) MoS2 and WS2 and the technique adopted to realize the deposition inside the cladding channels of a twin-hole step index silica fiber consists of a thermal decomposition process4 of the precursor ammonium tetrathiomolybdate (NH4)2MoS4 in 6% H2/Ar flow. The technique has allowed us to uniformly coat the two cladding channels for a length of 25 cm with a film nominally consisting in a bi-layer of the 2D materials. A Raman based analysis has been used to test the morphology of the coating. The fiber deposited with 2D materials was later thermally poled and periodically erased via exposure to UV light to reach the QPM condition at a wavelength of 1550 nm. The effective oœ'(2) of the fiber was measured via SHG for both the deposited and the pristine fiber, showing an enhancement of the nonlinearity in favor of the deposited one. The phenomenon can be explained by the exploitation of a higher oœ'(3) seen by the pump wave due to the presence of the 2D layer deposited inside the cladding holes and opens the possibility of exploiting the higher intrinsic material oœ'(2), in case o, SCOPUS: cp.p, info:eu-repo/semantics/published

Thulium-doped fiber lasers (TDFLs) offer a broad 3 F 4 → 3 H emission band ~1600-2200 nm. Thanks to "two-for-one" cross-relaxation process in TDFLs [1], that enables to achieve output power > 1 kW at ~2045 nm with 0.79-μm cladding-pumping. Efficient cross-relaxation requires high Tm-concentration (> 3wt%) [1, 2, references therein]. This results in a high core refractive index (thus higher V-number) that degrades the beam quality. It also increases the thermal load per unit length, although this can be reduced by a large cladding-to-core area ratio that increases the absorption length of the fiber. A long fiber also shifts the emission to long wavelengths with more signal re-absorption. For short-wavelength emission the re-absorption must be reduced in some other way, which also ensures adequate total pump absorption. Simplest technique is to reduce the area ratio, but then excessive thermal load or inefficient cross-relaxation (if the Tm-concentration is low to reduce the thermal load per unit length) hampers power-scaling.

info:eu-repo/semantics/published

info:eu-repo/semantics/published