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It is shown that whenever the edges of a connected simple graph on n vertices are colored with $$n-1$$ colors appearing so that no cycle in G is rainbow, there must be a monochromatic edge cut in G. From this it follows that such colorings of G can be represented, or ‘encoded,’ by full binary trees with n leaves, with vertices labeled by subsets of V(G), such that the leaf labels are singletons, the label of each non-leaf is the union of the labels of its children, and each label set induces a connected subgraph of G. It is also shown that $$n-1$$ is the largest integer for which the main theorem holds, for each n, although for some graphs a certain strengthening of the hypothesis makes the theorem conclusion true with $$n-1$$ replaced by $$n-2$$.

The number of measurements demanded by hybrid quantum-classical algorithms such as the variational quantum eigensolver (VQE) is prohibitively high for many problems of practical value. For such problems, realizing quantum advantage will require methods which dramatically reduce this cost. Previous quantum algorithms that reduce the measurement cost (e.g. quantum amplitude and phase estimation) require error rates that are too low for near-term implementation. Here we propose methods that take advantage of the available quantum coherence to maximally enhance the power of sampling on noisy quantum devices, reducing measurement number and runtime compared to the standard sampling method of the variational quantum eigensolver (VQE). Our scheme derives inspiration from quantum metrology, phase estimation, and the more recent "alpha-VQE" proposal, arriving at a general formulation that is robust to error and does not require ancilla qubits. The central object of this method is what we call the "engineered likelihood function" (ELF), used for carrying out Bayesian inference. We show how the ELF formalism enhances the rate of information gain in sampling as the physical hardware transitions from the regime of noisy intermediate-scale quantum computers into that of quantum error corrected ones. This technique speeds up a central component of many quantum algorithms, with applications including chemistry, materials, finance, and beyond. Similar to VQE, we expect small-scale implementations to be realizable on today's quantum devices., 49 pages, 32 figures

The unconventional normal-state properties of the cuprates are often discussed in terms of emergent electronic order that onsets below a putative critical doping of xc = 0.19. Charge-density wave (CDW) correlations represent one such order; however, experimental evidence for such order generally spans a limited range of doping that falls short of the critical value xc, leading to questions regarding its essential relevance. Here, we use x-ray diffraction to demonstrate that CDW correlations in La2-xSrxCuO4 persist up to a doping of at least x = 0.21. The correlations show strong changes through the superconducting transition, but no obvious discontinuity through xc = 0.19, despite changes in Fermi surface topology and electronic transport at this doping. These results demonstrate the interaction between CDWs and superconductivity even in overdoped cuprates and prompt a reconsideration of the role of CDW correlations in the high-temperature cuprate phase diagram., Comment: 8 pages + 5 pages of supplemental material; accepted in npj Quantum Materials

We formalize the problem of dissipative quantum encoding, and explore the advantages of using Markovian evolution to prepare a quantum code in the desired logical space, with emphasis on discrete-time dynamics and the possibility of exact finite-time convergence. In particular, we investigate robustness of the encoding dynamics and their ability to tolerate initialization errors, thanks to the existence of non-trivial basins of attraction. As a key application, we show that for stabilizer quantum codes on qubits, a finite-time dissipative encoder may always be constructed, by using at most a number of quantum maps determined by the number of stabilizer generators. We find that even in situations where the target code lacks gauge degrees of freedom in its subsystem form, dissipative encoders afford nontrivial robustness against initialization errors, thus overcoming a limitation of purely unitary encoding procedures. Our general results are illustrated in a number of relevant examples, including Kitaev's toric code., 29 pages, 4 figures

Spectroscopic Imaging Scanning Tunneling Microscopy (SI-STM) measurements have previously been applied to the study of the heavy-fermion system CeCoIn5 to examine the superconducting gap structure and band dispersions via quasiparticle intereference. Here we directly measure the dispersing electron bands with angle-resolved photoelectron spectroscopy (ARPES) and compare with first-principles electronic structure calculations. By autocorrelating the ARPES-resolved bands with themselves we can measure the potential q vectors and discern exactly which bands the STM is measuring. We find that the STM results are dominated by scattering associated with a cloverleaf shaped band centered at the zone corners. This same band is also a viable candidate to host the superconducting gap. The electronic structure calculations indicate that this region of the Fermi surface involves significant contributions from the Co d electrons, an indication that the superconductivity in these materials is more three dimensional than that found in the related unconventional superconductors, the cuprates and the pnictides. publishedVersion

Surface magnetism and its correlation with the electronic structure are critical to understanding the topological surface state in the intrinsic magnetic topological insulator MnBi_{2}Te_{4}. Here, using static and time resolved angle-resolved photoemission spectroscopy (ARPES), we find a significant ARPES intensity change together with a gap opening on a Rashba-like conduction band. Comparison with a model simulation strongly indicates that the surface magnetism on cleaved MnBi_{2}Te_{4} is the same as its bulk state. The inability of surface ferromagnetism to open a gap in the topological surface state uncovers the novel complexity of MnBi_{2}Te_{4} that may be responsible for the low quantum anomalous Hall temperature of exfoliated MnBi_{2}Te_{4}.

The idea of employing non-Abelian statistics for error-free quantum computing ignited interest in reports of topological surface superconductivity and Majorana zero modes (MZMs) in FeTe

We present mathematical and conceptual foundations for the task of robust amplitude estimation using engineered likelihood functions (ELFs), a framework introduced in Wang et al. [PRX Quantum 2, 010346 (2021)] that uses Bayesian inference to enhance the rate of information gain in quantum sampling. These ELFs, which are obtained by choosing tunable parameters in a parametrized quantum circuit to minimize the expected posterior variance of an estimated parameter, play an important role in estimating the expectation values of quantum observables. We give a thorough characterization and analysis of likelihood functions arising from certain classes of quantum circuits and combine this with the tools of Bayesian inference to give a procedure for picking optimal ELF tunable parameters. Finally, we present numerical results to demonstrate the performance of ELFs., 56 pages, 5 figures

The symmetries of superconducting gap functions remain an important question of iron-based superconductivity. Motivated by the recent angle-resolved photoemission spectroscopic measurements on iron-chalcogenide superconductors, we investigate the influence of pairing symmetries on the topological surface state. If the surface Dirac cone becomes gapped in the superconducting phase, it implies magnetization induced from time-reversal symmetry breaking pairing via spin-orbit coupling. Based on the crystalline symmetry constraints on the Ginzburg-Landau free energy, the gap function symmetries are among the possibilities of $A_{1g(u)}\pm iA_{2g(u)}$, $B_{1g(u)}\pm iB_{2g(u)}$, or, $E_{g(u)}\pm i E_{g(u)}$. This time-reversal symmetry breaking effect can exist in the normal state very close to $T_c$ with the relative phase between two gap functions locked at $\pm \frac{\pi}{2}$. The coupling between magnetization and superconducting gap functions is calculated based on a three-orbital model for the band structure of iron-chalcogenides. This study provides the connection between the gap function symmetries and topological properties of the surface state., Comment: 11 pages, 8 figures. Comments are welcome!

A comparative study of the gaps measured in two techniques, angle-resolved photoelectron spectroscopy and spectroscopic imaging scanning tunneling microscopy, is presented. In particular the study focuses on the more overdoped region of the cuprate phase diagram in the superconducting state. While the total densities of states measured in the two techniques agree very well, it is shown that the peak in the density of states, ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{DOS}}$, is consistently displaced to higher energies relative to the maximal superconducting gap, ${\mathrm{\ensuremath{\Delta}}}_{0}$, determined in photoemission. The difference between the two gaps is more evident for the less doped samples reflecting increased normalization of bands. This observation will clearly influence the boundaries in the phase diagrams of the cuprates defined by these two techniques.

In cuprate superconductors, the doping of carriers into the parent Mott insulator induces superconductivity and various other phases whose characteristic temperatures are typically plotted versus the doping level $p$. In most materials, $p$ cannot be determined from the chemical composition, but it is derived from the superconducting transition temperature, $T_\mathrm{c}$, using the assumption that $T_\mathrm{c}$ dependence on doping is universal. Here, we present angle-resolved photoemission studies of Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$, cleaved and annealed in vacuum or in ozone to reduce or increase the doping from the initial value corresponding to $T_\mathrm{c}=91$ K. We show that $p$ can be determined from the underlying Fermi surfaces and that $in-situ$ annealing allows mapping of a wide doping regime, covering the superconducting dome and the non-superconducting phase on the overdoped side. Our results show a surprisingly smooth dependence of the inferred Fermi surface with doping. In the highly overdoped regime, the superconducting gap approaches the value of $2\Delta_0=(4\pm1)k_\mathrm{B}T_\mathrm{c}$, Comment: 8 pages, 4 figures

An edge-regular graph is a regular graph in which, for some $\lambda$, any two adjacent vertices have exactly $\lambda$ common neighbors. This paper is about the existence and structure of edge-regular graphs with $\lambda =1$ and about edge-regular graphs with $\lambda >1$ which have local neighborhood structure analogous to that of the edge-regular graphs with $\lambda =1$.

For any (finite simple) graph G the secure domination number of G satisfies γ s ( G ) ≥ | V ( G ) | 2 . Here we find a secure-dominating set S in G such that | S | = ⌈ | V ( G ) | 2 ⌉ in all cases when G is a grid, and in the majority of cases when G is a cylindrical or toroidal grid. In all such cases, S satisfies the additional requirement that G [ S ] is connected. We make note that the concept of secure-dominating sets considered in this paper is quite different from the other secure domination currently of interest. 1

We report the temperature-dependent optical conductivity and ARPES studies of the iron-based superconductor (SC) Sr$_{0.67}$Na$_{0.33}$Fe$_2$As$_2$ in the high-temperature tetragonal paramagnetic phase; below the structural and magnetic transitions at $T_{\rm N}\simeq$125 K in the orthorhombic spin-density-wave (SDW)-like phase, and $T_r\simeq$42 K in the reentrant tetragonal double-Q magnetic phase where both charge and SDW order exist; and below the SC transition at $T_c\simeq$10 K. The free-carrier component in the optical conductivity is described by two Drude contributions; one strong and broad, the other weak and narrow. The broad Drude component decreases dramatically below $T_{\rm N}$ and $T_r$, with much of its strength being transferred to a bound excitation in the mid-infrared, while the narrow Drude component shows no anomalies at either of the transitions, actually increasing in strength at low temperature while narrowing dramatically. The behavior of an infrared-active mode suggests zone-folding below $T_r$. Below $T_c$ the dramatic decrease in the low-frequency optical conductivity signals the formation of a SC energy gap. ARPES reveals hole-like bands at the center of the Brillouin zone (BZ), with both electron- and hole-like bands at the corners. Below $T_{\rm N}$, the hole pockets at the center of the BZ decrease in size, consistent with the behavior of the broad Drude component; while below $T_r$ the electron-like bands shift and split, giving rise to a low-energy excitation in the optical conductivity at ~20 meV. The magnetic states, with resulting SDW and charge-SDW order, respectively, lead to a significant reconstruction of the Fermi surface that has profound implications for the transport originating from the electron and hole pockets, but appears to have relatively little impact on the SC in this material.

Over the past two decades, advances in computational algorithms have revealed a curious property of the two-dimensional Hubbard model (and related theories) with hole doping: the presence of close-in-energy competing ground states that display very different physical properties. On the one hand, there is a complicated state exhibiting intertwined spin, charge, and pair density wave orders. We call this `type A'. On the other hand, there is a uniform d-wave superconducting state that we denote as `type B'. We advocate, with the support of both microscopic theoretical calculations and experimental data, dividing the high-temperature cuprate superconductors into two corresponding families, whose properties reflect either the type A or type B ground states at low temperatures. We review the anomalous properties of the pseudogap phase that led us to this picture, and present a modern perspective on the role that umklapp scattering plays in these phenomena in the type B materials. This reflects a consistent framework that has emerged over the last decade, in which Mott correlations at weak coupling drive the formation of the pseudogap. We discuss this development, recent theory and experiments, and open issues., 95 pages, 33 figures

Practical challenges in simulating quantum systems on classical computers have been widely recognized in the quantum physics and quantum chemistry communities over the past century. Although many approximation methods have been introduced, the complexity of quantum mechanics remains hard to appease. The advent of quantum computation brings new pathways to navigate this challenging complexity landscape. By manipulating quantum states of matter and taking advantage of their unique features such as superposition and entanglement, quantum computers promise to efficiently deliver accurate results for many important problems in quantum chemistry such as the electronic structure of molecules. In the past two decades significant advances have been made in developing algorithms and physical hardware for quantum computing, heralding a revolution in simulation of quantum systems. This article is an overview of the algorithms and results that are relevant for quantum chemistry. The intended audience is both quantum chemists who seek to learn more about quantum computing, and quantum computing researchers who would like to explore applications in quantum chemistry., 194 pages, 13 figures, 5 tables and 404 references. Fixed formatting issues from the previous version. Comments welcome

When Cooper pairs are formed with finite center-of-mass momentum, the defining characteristic is a spatially modulating superconducting energy gap $\Delta(r)$. Recently, this concept has been generalized to the pair density wave (PDW) state predicted to exist in a variety of strongly correlated electronic materials such as the cuprates. Although the signature of a cuprate PDW has been detected in Cooper-pair tunnelling, the distinctive signature in single-electron tunneling of a periodic $\Delta(r)$ modulation has never been observed. Here, using a new approach, we discover strong $\Delta(r)$ modulations in Bi$_2$Sr$_2$CaCu$_2$O$_8$+$\delta$ that have eight-unit-cell periodicity or wavevectors $Q=2{\pi}/a_0(1/8,0)$; $2{\pi}/a_0(0,1/8)$. This constitutes the first energy-resolved spectroscopic evidence for the cuprate PDW state. An analysis of spatial arrangements of $\Delta(r)$ modulations then reveals that this PDW is predominantly unidirectional, but with an arrangement of nanoscale domains indicative of a vestigial PDW. Simultaneous imaging of the local-density-of-states $N(r,E)$ reveals electronic modulations with wavevectors $Q$ and $2Q$, as anticipated when the PDW coexists with superconductivity. Finally, by visualizing the topological defects in these $N(r,E)$ density waves at $2Q$, we discover them to be concentrated in areas where the PDW spatial phase changes by $\pi$, as predicted by the theory of half-vortices in a PDW state. Overall, this is a compelling demonstration, from multiple single-electron signatures, of a PDW state coexisting with superconductivity at zero magnetic field, in the canonical cuprate Bi$_2$Sr$_2$CaCu$_2$O$_8$+$\delta$., Comment: Final submitted version. arXiv admin note: text overlap with arXiv:2109.14031

We consider the problem of characterizing states of a multipartite quantum system from restricted, quasi-local information, with emphasis on uniquely determined pure states. By leveraging tools from dissipative quantum control theory, we show how the search for states consistent with an assigned list of reduced density matrices may be restricted to a proper subspace, which is determined solely by their supports. The existence of a quasi-local observable which attains its unique minimum over such a subspace further provides a sufficient criterion for a pure state to be uniquely determined by its reduced states. While the condition that a pure state is uniquely determined is necessary for it to arise as a non-degenerate ground state of a quasi-local Hamiltonian, we prove the opposite implication to be false in general, by exhibiting an explicit analytic counterexample. We show how the problem of determining whether a quasi-local parent Hamiltonian admitting a given pure state as its unique ground state is dual, in the sense of semidefinite programming, to the one of determining whether such a state is uniquely determined by the quasi-local information. Failure of this dual program to attain its optimal value is what prevents these two classes of states to coincide., 17 pages, 1 figure

The high-${T}_{c}$ superconductor, $\mathrm{FeT}{\mathrm{e}}_{0.55}\mathrm{S}{\mathrm{e}}_{0.45}$, has recently been shown to support a surface state with topological character. Here we use low-energy laser-based angle-resolved photoemission spectroscopy with variable light polarization, including both linear and circular polarizations, to reexamine the same material and the related $\mathrm{FeT}{\mathrm{e}}_{0.7}\mathrm{S}{\mathrm{e}}_{0.3}$, with a larger Te concentration. In both cases, we observe the presence of a surface state displaying linear dispersion in a cone-like configuration. The use of circular polarization confirms the presence of a helical spin structure. These experimental studies are compared with theoretical studies that account for the local magnetic effects related to the paramagnetism observed in this system in the normal state. In contrast to previous studies, we find that including the magnetic contributions is necessary to bring the chemical potential of the calculated electronic band structure naturally into alignment with the experimental observations.

Topological superconductivity has been sought for in a variety of heterostructure systems, the interest being that a material displaying such a phenomenon could prove to be the ideal platform to support Majorana fermions, which in turn could be the basis for advanced qubit technologies. Recently the high Tc family of superconductors, $FeSe_{x}Te_{1-x}$, have been shown to exhibit the property of topological superconductivity and further, evidence has been found for the presence of Majorana fermions. We have studied the interplay of topology, magnetism and superconductivity in the $FeSe_{x}Te_{1-x}$ family using high-resolution laser-based photoemission. At the bulk superconducting transition, a gap opens at the chemical potential as expected. However, a second gap is observed to open at the Dirac point in the topological surface state. The associated mass acquisition in the topological state points to time-reversal symmetry breaking, probably associated with the formation of ferromagnetism in the surface layer. The presence of intrinsic ferromagnetism combined with strong spin-orbit coupling provides an ideal platform for a range of exotic topological phenomena.

The high-${T}_{c}$ superconducting cuprates are recognized as doped Mott insulators. Several studies indicate that as a function of doping and temperature, there is a crossover from this regime into a phase characterized as a marginal Fermi liquid. Several calculations of the doped Mott insulating phase indicate that the Fermi surface defines small pockets which at the higher doping levels switch to a full closed Fermi surface, characteristic of a more metallic system. Here we use femtosecond laser-based pump-probe techniques to investigate the structure of the Fermi surface in the underdoped region of $\mathrm{B}{\mathrm{i}}_{2}\mathrm{S}{\mathrm{r}}_{2}\mathrm{CaC}{\mathrm{u}}_{2}{\mathrm{O}}_{8+\ensuremath{\delta}}$ and compare it with that associated with the optimally doped material. We confirm the concept of a small pocket in the underdoped system consistent with theoretical predictions in this strongly correlated state.

Parameterized quantum circuits play an essential role in the performance of many variational hybrid quantum-classical (HQC) algorithms. One challenge in implementing such algorithms is to choose an effective circuit that well represents the solution space while maintaining a low circuit depth and number of parameters. To characterize and identify expressible, yet compact, parameterized circuits, we propose several descriptors, including measures of expressibility and entangling capability, that can be statistically estimated from classical simulations of parameterized quantum circuits. We compute these descriptors for different circuit structures, varying the qubit connectivity and selection of gates. From our simulations, we identify circuit fragments that perform well with respect to the descriptors. In particular, we quantify the substantial improvement in performance of two-qubit gates in a ring or all-to-all connected arrangement compared to that of those on a line. Furthermore, we quantify the improvement in expressibility and entangling capability achieved by sequences of controlled X-rotation gates compared to sequences of controlled Z-rotation gates. In addition, we investigate how expressibility "saturates" with increased circuit depth, finding that the rate and saturated-value appear to be distinguishing features of a parameterized quantum circuit template. While the correlation between each descriptor and performance of an algorithm remains to be investigated, methods and results from this study can be useful for both algorithm development and design of experiments for general variational HQC algorithms.

Here, we use angle-resolved photoemission spectroscopy to study superconductivity that emerges in two extreme cases, from a Fermi-liquid phase (LiFeAs) and an incoherent bad-metal phase (${\mathrm{FeTe}}_{0.55}{\mathrm{Se}}_{0.45}$). We find that although the electronic coherence can strongly reshape the single-particle spectral function in the superconducting state, it is decoupled from the maximum-superconducting-gap and ${T}_{c}$ ratio $2{\mathrm{\ensuremath{\Delta}}}_{max}/{k}_{B}{T}_{c}$, which shows a universal scaling that is valid for all iron-based superconductors (FeSCs). Our observation excludes pairing scenarios in the BCS and the BEC limit for FeSCs and calls for a universal strong-coupling pairing mechanism for the FeSCs.

The interplay between the electronic and lattice degrees of freedom in nonequilibrium states of strongly correlated systems has been debated for decades. Although progress has been made in establishing a hierarchy of electronic interactions with the use of time-resolved techniques, the role of the phonons often remains in dispute, a situation highlighting the need for tools that directly probe the lattice. We present the first combined megaelectron volt ultrafast electron diffraction and time- and angle-resolved photoemission spectroscopy study of optimally doped Bi2Sr2CaCu2O8+δ. Quantitative analysis of the lattice and electron subsystems’ dynamics provides a unified picture of nonequilibrium electron-phonon interactions in the cuprates beyond the N-temperature model. The work provides new insights on the specific phonon branches involved in the nonequilibrium heat dissipation from the high-energy Cu–O bond stretching “hot” phonons to the lowest-energy acoustic phonons with correlated atomic motion along the crystal directions and their characteristic time scales. It reveals a highly nonthermal phonon population during the first several picoseconds after the photoexcitation. The approach, taking advantage of the distinct nature of electrons and photons as probes, is applicable for studying energy relaxation in other strongly correlated electron systems. OA gold - CA extern

Preparation of pure states on networks of quantum systems by controlled dissipative dynamics offers important advantages with respect to circuit-based schemes. Unlike in continuous-time scenarios, when discrete-time dynamics are considered, dead-beat stabilization becomes possible in principle. Here, we focus on pure states that can be stabilized by distributed, unsupervised dynamics in finite time on a network of quantum systems subject to realistic quasi-locality constraints. In particular, we define a class of quasi-locality notions, that we name "tree-like hypergraphs," and show that the states that are robustly stabilizable in finite time are then unique ground states of a frustration-free, commuting quasi-local Hamiltonian. A structural characterization of such states is also provided, building on a simple yet relevant example., 6 pages, 3 figures

We investigate whether a generic multipartite pure state can be the unique asymptotic steady state of locality-constrained purely dissipative Markovian dynamics. In the simplest tripartite setting, we show that the problem is equivalent to characterizing the solution space of a set of linear equations and establish that the set of pure states obeying the above property has either measure zero or measure one, solely depending on the subsystems' dimension. A complete analytical characterization is given when the central subsystem is a qubit. In the N-partite case, we provide conditions on the subsystems' size and the nature of the locality constraint, under which random pure states cannot be quasi-locally stabilized generically. Beside allowing for the possibility to approximately stabilize entangled pure states that cannot be exact steady states in settings where stabilizability is generic, our results offer insights into the extent to which random pure states may arise as unique ground states of frustration free parent Hamiltonians. We further argue that, to high probability, pure quantum states sampled from a t-design enjoy the same stabilizability properties of Haar-random ones as long as suitable dimension constraints are obeyed and t is sufficiently large. Lastly, we demonstrate a connection between the tasks of quasi-local state stabilization and unique state reconstruction from local tomographic information, and provide a constructive procedure for determining a generic N-partite pure state based only on knowledge of the support of any two of the reduced density matrices of about half the parties, improving over existing results., 36 pages (including appendix), 2 figures

It is well known that if the edges of a finite simple connected graph on n vertices are colored so that no cycle is rainbow, then no more than n-1 colors can appear on the edges. In previous work it has been shown that the essentially different rainbow-cycle-forbidding edge colorings of Kn with n-1 colors appearing are in 1-1 correspondence with (can be encoded by) the (isomorphism classes of) full binary trees with n leafs. In the encoding, the natural Huffman labeling of each tree arising from the assignment of 1 to each leaf plays a role. Very recently it has been shown that a similar encoding holds for rainbow-cycle-forbidding edge colorings of Ka,b with a+b-1 colors appearing. In this case the binary trees are given Huffman labelings arising from certain assignments of (0,1) or (1,0) to the leafs. (Sibling leafs are not allowed to be assigned the same label.) In this paper we prove the analogous result for complete r-partite graphs, for r > 2.

One of the most fundamental properties of an interacting electron system is its frequency- and wave-vector-dependent density response function, $\chi({\bf q},\omega)$. The imaginary part, $\chi''({\bf q},\omega)$, defines the fundamental bosonic charge excitations of the system, exhibiting peaks wherever collective modes are present. $\chi$ quantifies the electronic compressibility of a material, its response to external fields, its ability to screen charge, and its tendency to form charge density waves. Unfortunately, there has never been a fully momentum-resolved means to measure $\chi({\bf q},\omega)$ at the meV energy scale relevant to modern elecronic materials. Here, we demonstrate a way to measure $\chi$ with quantitative momentum resolution by applying alignment techniques from x-ray and neutron scattering to surface high-resolution electron energy-loss spectroscopy (HR-EELS). This approach, which we refer to here as "M-EELS," allows direct measurement of $\chi''({\bf q},\omega)$ with meV resolution while controlling the momentum with an accuracy better than a percent of a typical Brillouin zone. We apply this technique to finite-q excitations in the optimally-doped high temperature superconductor, Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$ (Bi2212), which exhibits several phonons potentially relevant to dispersion anomalies observed in ARPES and STM experiments. Our study defines a path to studying the long-sought collective charge modes in quantum materials at the meV scale and with full momentum control., Comment: 26 pages, 10 sections, 7 figures, and an appendix

Both electron and lattice dynamics are directly observed in the nonequilibrium state of strongly correlated Bi-2212., The interplay between the electronic and lattice degrees of freedom in nonequilibrium states of strongly correlated systems has been debated for decades. Although progress has been made in establishing a hierarchy of electronic interactions with the use of time-resolved techniques, the role of the phonons often remains in dispute, a situation highlighting the need for tools that directly probe the lattice. We present the first combined megaelectron volt ultrafast electron diffraction and time- and angle-resolved photoemission spectroscopy study of optimally doped Bi2Sr2CaCu2O8+δ. Quantitative analysis of the lattice and electron subsystems’ dynamics provides a unified picture of nonequilibrium electron-phonon interactions in the cuprates beyond the N-temperature model. The work provides new insights on the specific phonon branches involved in the nonequilibrium heat dissipation from the high-energy Cu–O bond stretching “hot” phonons to the lowest-energy acoustic phonons with correlated atomic motion along the crystal directions and their characteristic time scales. It reveals a highly nonthermal phonon population during the first several picoseconds after the photoexcitation. The approach, taking advantage of the distinct nature of electrons and photons as probes, is applicable for studying energy relaxation in other strongly correlated electron systems.

Open quantum systems evolving according to discrete-time dynamics are capable, unlike continuous-time counterparts, to converge to a stable equilibrium in finite time with zero error. We consider dissipative quantum circuits consisting of sequences of quantum channels subject to specified quasi-locality constraints, and determine conditions under which stabilization of a pure multipartite entangled state of interest may be exactly achieved in finite time. Special emphasis is devoted to characterizing scenarios where finite-time stabilization may be achieved robustly with respect to the order of the applied quantum maps, as suitable for unsupervised control architectures. We show that if a decomposition of the physical Hilbert space into virtual subsystems is found, which is compatible with the locality constraint and relative to which the target state factorizes, then robust stabilization may be achieved by independently cooling each component. We further show that if the same condition holds for a scalable class of pure states, a continuous-time quasi-local Markov semigroup ensuring rapid mixing can be obtained. Somewhat surprisingly, we find that the commutativity of the canonical parent Hamiltonian one may associate to the target state does not directly relate to its finite-time stabilizability properties, although in all cases where we can guarantee robust stabilization, a (possibly non-canonical) commuting parent Hamiltonian may be found. Beside graph states, quantum states amenable to finite-time robust stabilization include a class of universal resource states displaying two-dimensional symmetry-protected topological order, along with tensor network states obtained by generalizing a construction due to Bravyi and Vyalyi. Extensions to representative classes of mixed graph-product and thermal states are also discussed., 20 + 9 pages, 9 figures

An extremal result about vertex covers, attributed by Hajnal to Erdős and Gallai, is applied to prove the following: If n, k, and t are integers satisfying n ≥ k ≥ t ≥ 3 and k ≤ 2t - 2, and G is a graph with the minimum number of edges among graphs on n vertices with the property that every induced subgraph on k vertices contains a complete subgraph on t vertices, then every component of G is complete.

The phase diagram associated with the high Tc superconductors is complicated by an array of different ground states. The parent material represents an antiferromagnetic insulator but with doping superconductivity becomes possible with transition temperatures previously thought unattainable. The underdoped region of the phase diagram is dominated by the so-called pseudogap phenomena whereby in the normal state the system mimics superconductivity in its spectra response but does not show the complete loss of resistivity associated with the superconducting state. An understanding of this regime presents one of the great challenges for the field. In the present study we revisit the structure of the phase diagram as determined in photoemission studies. By careful analysis of the role of nanoscale inhomogeneities in the overdoped region we are able to more carefully separate out the gaps due to the pseudogap phenomena from the gaps due to the superconducting transition. Within a mean field description we are thus able to link the magnitude of the gap directly to the Heisenberg exchange interaction term, $J\sum{s_i \cdot s_j}$, contained in the $t-J$ model. This approach provides a clear indication that the pseudogap is that associated with spin singlet formation., Comment: revised to include supplementary section and correct references in Fig. 5

In complex materials various interactions have important roles in determining electronic properties. Angle-resolved photoelectron spectroscopy (ARPES) is used to study these processes by resolving the complex single-particle self-energy and quantifying how quantum interactions modify bare electronic states. However, ambiguities in the measurement of the real part of the self-energy and an intrinsic inability to disentangle various contributions to the imaginary part of the self-energy can leave the implications of such measurements open to debate. Here we employ a combined theoretical and experimental treatment of femtosecond time-resolved ARPES (tr-ARPES) show how population dynamics measured using tr-ARPES can be used to separate electron–boson interactions from electron–electron interactions. We demonstrate a quantitative analysis of a well-defined electron–boson interaction in the unoccupied spectrum of the cuprate Bi2Sr2CaCu2O8+x characterized by an excited population decay time that maps directly to a discrete component of the equilibrium self-energy not readily isolated by static ARPES experiments., Differentiation of quantum interactions in correlated materials is ambiguous in measurements of the single particle self-energy. Here, Rameau et al. employ a combined theoretical and experimental time domain treatment to separate electron-boson interactions from electron-electron interactions in Bi2Sr2CaCu2O8+x .