51. Transition-metal adatoms on 2D-GaAs: a route to chiral magnetic 2D materials by design
- Author
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Alvaro González-García, Milorad V. Milošević, Cihan Bacaksiz, Rafael González-Hernández, François M. Peeters, Denis Sabani, and William López-Pérez
- Subjects
Materials science ,Physics ,02 engineering and technology ,021001 nanoscience & nanotechnology ,Condensed Matter Physics ,01 natural sciences ,Molecular physics ,Close range ,Condensed Matter::Materials Science ,Magnetic anisotropy ,Magnetization ,Adsorption ,Transition metal ,0103 physical sciences ,Atom ,General Materials Science ,010306 general physics ,0210 nano-technology ,Anisotropy - Abstract
Using relativistic density-functional calculations, we examine the magneto-crystalline anisotropy and exchange properties of transition-metal atoms adsorbed on 2D-GaAs. We show that single Mn and Mo atom (Co and Os) strongly bind on 2D-GaAs, and induce local out-of-plane (in-plane) magnetic anisotropy. When a pair of TM atoms is adsorbed on 2D-GaAs in a close range from each other, magnetisation properties change (become tunable) with respect to concentrations and ordering of the adatoms. In all cases, we reveal presence of strong Dzyaloshinskii–Moriya interaction. These results indicate novel pathways towards two-dimensional chiral magnetic materials by design, tailored for desired applications in magneto-electronics.
- Published
- 2021
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